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At least 937 records · Page 52

Radiative Flux and Forcing Parameterization Error in Aerosol-Free Clear Skies

This article reports on the accuracy in aerosol- and cloud-free conditions of the radiation parameterizations used in climate models. Accuracy is assessed relative to observationally validated reference models for fluxes under present-day conditions and forcing (flux changes) from quadrupled concentrations of carbon dioxide. Agreement among reference models is typically within 1 W/m2, while parameterized calculations are roughly half as accurate in the longwave and even less accurate, and more variable, in the shortwave. Absorption of shortwave radiation is underestimated by most parameterizations in the present day and has relatively large errors in forcing. Error in present-day conditions is essentially unrelated to error in forcing calculations. Recent revisions to parameterizations have reduced error in most cases. A dependence on atmospheric conditions, including integrated water vapor, means that global estimates of parameterization error relevant for the radiative forcing of climate change will require much more ambitious calculations.

Climate↗

An A-Train Climatology of Extratropical Cyclone Clouds

Extratropical cyclones (ETCs) are the main purveyors of precipitation in the mid-latitudes, especially in winter, and have a significant radiative impact through the clouds they generate. However, general circulation models (GCMs) have trouble representing precipitation and clouds in ETCs, and this might partly explain why current GCMs disagree on to the evolution of these systems in a warming climate. Collectively, the A-train observations of MODIS, CloudSat, CALIPSO, AIRS and AMSR-E have given us a unique perspective on ETCs: over the past 10 years these observations have allowed us to construct a climatology of clouds and precipitation associated with these storms. This has proved very useful for model evaluation as well in studies aimed at improving understanding of moist processes in these dynamically active conditions. Using the A-train observational suite and an objective cyclone and front identification algorithm we have constructed cyclone centric datasets that consist of an observation-based characterization of clouds and precipitation in ETCs and their sensitivity to large scale environments. In this presentation, we will summarize the advances in our knowledge of the climatological properties of cloud and precipitation in ETCs acquired with this unique dataset. In particular, we will present what we have learned about southern ocean ETCs, for which the A-train observations have filled a gap in this data sparse region. In addition, CloudSat and CALIPSO have for the first time provided information on the vertical distribution of clouds in ETCs and across warm and cold fronts. We will also discuss how these observations have helped identify key areas for improvement in moist processes in recent GCMs. Recently, we have begun to explore the interaction between aerosol and cloud cover in ETCs using MODIS, CloudSat and CALIPSO. We will show how aerosols are climatologically distributed within northern hemisphere ETCs, and how this relates to cloud cover.

clouds↗

TPSAS-NF1676L-10888-DND

Hyperspectrally-resolved surface emissivities are derived with an algorithm utilizes a combined fast radiative transfer model (RTM) with a molecular RTM and a cloud RTM accounting for both atmospheric absorption and cloud absorption/scattering. Clouds are automatically detected and cloud microphysical parameters are retrieved; and emissivity is retrieved under clear and optically thin cloud conditions. The retrieval technique separates surface emissivity from skin temperature by representing the emissivity spectrum with eigenvectors derived from a laboratory measured emissivity database. Global land emissivities retrieved under the optically thin clouds are investigated by means of their accuracy in comparison with that under cloud-free conditions. Here we present the emissivity derived under optically thin clouds, their accuracy, and the inter-comparison with that under clear conditions.

Daniel K Zhou↗

Uncertainty in Aerosol–Cloud Radiative Forcing Is Driven By Clean Conditions

Atmospheric aerosols and their impact on cloud properties remain the largest uncertainty in the human forcing of the climate system. By increasing the concentration of cloud droplets (Nd), aerosols reduce droplet size and increase the reflectivity of clouds (a negative radiative forcing). Central to this climate impact is the susceptibility of cloud droplet number to aerosol (β), the diversity of which explains much of the variation in the radiative forcing from aerosol–cloud interactions (RFaci) in global climate models. This has made measuring β a key target for developing observational constraints of the aerosol forcing.

Edward Gryspeerdt↗

Evaluating Subgrid-Scale Properties of Low Clouds over the Beaufort Sea in Arctic System Reanalysis using ARISE Airborne In Situ Observations

Arctic low clouds influence the evolution of the Arctic system through their effects on radiative fluxes, boundary layer mixing, stability, turbulence, humidity, and precipitation. Unfortunately, atmospheric models and retrospective analysis (reanalysis) products struggle to accurately simulate the occurrence and properties of low clouds in the Arctic. To better understand the magnitude and possible causes of this problem, we analyze the disagreements between the Arctic System Reanalysis version 2 (ASR) and data taken during the September 2014 Arctic Radiation-IceBridge Sea and Ice Experiment (ARISE) airborne campaign conducted over the Beaufort Sea. Previous analysis of grid scale-averaged meteorological variables revealed a lack of cloud water produced in ASR, related to warm/dry biases, a failure to produce sufficient cloud water in conditions that are observed to be favorable for large cloud water values, and sampling issues with the ARISE flight paths. However, ARISE collected meteorological observations at one second intervals, offering spatial data resolution comparable to the subgrid scale of ASR. Subgrid scale properties and processes must be parameterized in conventional atmospheric models and reanalyses such as ASR, and often rely on assumed distributions of meteorological variables about the grid box mean state. To enable an examination of the realism of ASR’s subgrid scale properties, we use high resolution data from ARISE determine the “subgrid scale” distributions of cloud water and thermodynamic variables in the real atmosphere. Preliminary results show that the subgrid scale distribution of thermodynamic variables about the grid scale mean resembles the triangular distribution assumed in many bulk microphysical parameterization schemes, but also with tails resembling Gaussian distributions. The main goal is to understand the partitioning of the total available atmospheric water into water vapor and cloud water. Models typically covert some percentage of total water in a grid box to cloud water based on the estimated amount of supersaturation from the assumed vapor distribution. The ARISE measurements can reveal the relationship between subgrid scale supersaturation and the partition between cloud water and water vapor.

Jason Brant Dodson↗

Subseasonal Tropical Convection Characteristics in the Energy Exascale Earth System Model Version 2

Accurate simulation of subseasonal tropical moist convection remains a key challenge for Earth system models. The difficulties stem from the reliance of cumulus cloud processes on model parameterizations and the need to represent the multiscale nature of interactions among clouds, radiation, moisture, circulation, and surface energy fluxes. Equatorial convection drives circulation anomalies that can affect weather patterns and extremes globally, motivating efforts to better understand and simulate these tropical disturbances. Here, a detailed review of subseasonal tropical convective behavior as simulated in the Energy Exascale Earth System Model version 2 (E3SMv2) is presented, with comparison to its predecessor version 1 (E3SMv1) and reference data sets. Model structural changes to the deep convective trigger function and surface fluxes, along with parametric tuning of the cloud and microphysics schemes, together result in an improved depiction of organized tropical convection across scales. In particular, E3SMv2 exhibits a more realistic Madden‐Julian oscillation (MJO) and low‐frequency Kelvin waves—owing to a sharper time mean equatorial meridional moisture gradient and improved convection‐circulation coupling —as well as a better depiction of MJO Northern Hemisphere teleconnections. Despite these improvements, subseasonal precipitation variance continues to be strongly underestimated in E3SMv2. Use of a cloud plume model also reveals that the coupling between daily averaged tropical precipitation and lower tropospheric instability in E3SM is inconsistent with observations, a bias that could potentially impact the simulation of intraseasonal disturbances.

54 ENVIRONMENTAL SCIENCES↗

Incorporating an Interactive Fire Plume-Rise Model in the DOE's Energy Exascale Earth System Model Version 1 (E3SMv1) and Examining Aerosol Radiative Effect

The vertical distribution of biomass burning aerosol (BBA) is important in regulating their impacts on weather and climate. The plume-rise process affects the injection height of BBA and interacts with the air parcel lifting and cloud processes. However, these processes are not represented in most global climate models. In this study, we replaced the fixed vertical profiles of monthly BBA emissions in the Department of Energy's Energy Exascale Earth System Model version 1 (E3SMv1) with an interactive fire plume-rise model. The vertical distribution of BBA emissions was calculated as a function of ambient thermodynamic conditions from the host E3SMv1, with distributions of fire sizes and sensible heat fluxes derived from the observations. The maximum fire radiative power (FRP) technique was used to determine the fire size. Scaling-FRP technique is used to calculate the wildfire heat release. Daily BBA emission, superimposed with a fire diurnal cycle retrieved from the satellite observation, was included in model simulations. The model shows improved agreement with satellite retrievals and in situ measurement during the National Oceanic and Atmospheric Administration Wildfire Experiment for Cloud chemistry, Aerosol absorption, and Nitrogen campaign. The model-observation comparison demonstrates the importance of the plume-rise model and fire diurnal cycle assumption in determining the BBA fields. We also find that E3SMv1 with new features produces a larger carbonaceous aerosol burden, leading to 0.13 W m –2 warming at the top of atmosphere compared to the default E3SMv1. This highlights the importance of accurately representing the BBA injection height and indicates a no-linear nature in the BBA-induced radiative effect.

54 ENVIRONMENTAL SCIENCES↗

Influences of cloud vertical overlapping on the calculated cloud albedo and their validation with satellite observations

Cloud albedo is expected to influence cloud radiative forcing in addition to cloud fraction, and inadequate description of the cloud overlapping effects on the cloud fraction may influence the simulated cloud fraction, and thus the relative cloud radiative forcing (RCRF) and cloud albedo. In this study, we first present a new formula by extending that presented previously in Liu et al. (2011) to consider multilayer clouds directly in the relationship between cloud albedo, cloud fraction and RCRF, and then quantitatively evaluate the effects of different cloud vertical overlapping structures, represented by the decorrelation length scales (L cf ), on the simulated cloud albedos. We use the BCC_AGCM2.0_CUACE/Aero model with simultaneous validation by observations from the Clouds and the Earth's Radiation Energy System (CERES) satellite. When L cf < 4 km (i.e., the cloud overlap is closer to the random overlap), the simulated cloud albedos are generally in good agreement with the satellite-based albedos for December– February and June–August; when L cf ≥ 4 km (i.e., the cloud vertical overlap is closer to the maximum overlap), the difference between simulated and observed cloud albedos became larger, due mainly to significant differences in cloud fractions and RCRF. Further quantitative analysis shows that the relative Euclidean distance, which represents the degree of overall model–observation disagreement, increases with the L cf for all three variables (cloud albedo, cloud fraction and RCRF), indicating the importance of cloud vertical overlapping in determining the accuracy of the calculated cloud albedo for multilayer clouds.

54 ENVIRONMENTAL SCIENCES↗

3D Radiative Transfer in Cloudy Atmospheres

3D cloud radiative community has matured enough to prepare a volume on 3D radiative transfer in cloudy atmosphere that will be published by Springer-Verlag this year. Many leading 3D radiative transfer scientists are amongst the co-authors of the book. The book starts with the basic 3D radiative transfer problem, describes its solutions and models, discusses the effects of cloud inhomogeneity for remote sensing, addresses climate problems in realistic atmosphere and studies cloud-vegetation interactions.

Marshak, Alexander↗

Cloudiness and the radiation budget

The problem of obtaining data for quantification of the effects of clouds on radiation budget measurements is discussed. Areas considered include the relationship between observed cloud characteristics and model predicted characteristics and selection of an angular distribution function for conversion of scanning radiometer radiance to irradiance. Storage of meteorological satellite data related to cloud-radiation interactions is discussed.

Source record↗

The Discrepancy Between Measured and Modeled Downwelling Solar Irradiance at the Ground: Dependence on Water Vapor

Moderate resolution spectra of the downwelling solar irradiance at the around in north central Oklahoma were measured during the Department of Energy Atmospheric Radiation Measurement Program Intensive Observation Period in the fall of 1997. Spectra obtained under cloud-free conditions were compared with calculations using a coarse resolution radiative transfer model to examine the dependency of model-measurement bias on water vapor. It was found that the bias was highly correlated with water vapor and increased at a rate of 9 W/sq m per cm of water. The source of the discrepancy remains undetermined because of the complex dependencies of other variables, most notably aerosol optical depth, on water vapor.

Pilewskie, P.↗

The Discrepancy Between Measured and Modeled Downwelling Solar Irradiance at the Ground: Dependence on Water Vapor

Moderate resolution spectra of the downwelling solar irradiance at the ground in north central Oklahoma were measured during the Department of Energy Atmospheric Radiation Measurement Program Intensive Observation Period in the fall of 1997. Spectra obtained under-cloud-free conditions were compared with calculations using a coarse resolution radiative transfer model to examine the dependency of model-measurement bias on water vapor. It was found that the bias was highly correlated with water vapor and increased at a rate of 9 Wm per cm of water. The source of the discrepancy remains undetermined because of the complex dependencies of other variables, most notably aerosol optical depth, on water vapor.

Pilewski, P.↗

The Discrepancy Between Measured and Modeled Downwelling Solar Irradiance at the Ground: Dependence on Water Vapor

Moderate resolution spectra of the downwelling solar irradiance at the ground in north central Oklahoma were measured during the Department of Energy Atmospheric Radiation Measurement Program Intensive Observation Period in the fall of 1997. Spectra obtained under cloud-free conditions were compared with calculations using a coarse resolution radiative transfer model to examine the dependency of model-measurement bias on water vapor. It was found that the bias was highly correlated with water vapor and increased at a rate of 9 Wm(exp -2) per cm of water. The source of the discrepancy remains undetermined because of the complex dependencies of other variables, most notably aerosol optical depth, on water vapor.

Pilewskie, P.↗

A three-dimensional sectional representation of aerosol mixing state for simulating optical properties and cloud condensation nuclei

Light absorption by black carbon (BC) particles emitted from fossil fuel combustion depends on the how thickly they are coated with non-refractory species such as ammonium, sulfate, nitrate, organics, and water. The cloud condensation nuclei (CCN) activation property of a particle depends on its dry size and the hygroscopicities of all the individual species mixed together. It is therefore necessary to represent both size and mixing state of aerosols to reliably predict their climate-relevant properties in atmospheric models. Here we describe and evaluate a novel sectional framework in the Model for Simulating Aerosol Interactions and Chemistry, referred to as MOSAIC-mix, that represents the mixing state by resolving aerosol dry size (D dry ), BC dry mass fraction (w BC ), and hygroscopicity (κ). Using ten idealized urban plume scenarios in which different types of aerosols evolve over 24 hours under a range of atmospherically relevant environmental conditions, we examine errors in CCN concentrations and optical properties with respect to a more explicit aerosol mixing state representation. We find that only a small number of w BC and κ bins are needed to achieve significant reductions in the errors, and propose a configuration consisting of 24 D dry bins, 2 w BC bins, and 2 κ bins that gives 24-hour average errors of about 5% or less in CCN concentrations and optical properties, 3-4 times lower than those from size-only-resolved simulations. Here, these results show that MOSAIC-mix is suitable for use in regional and global models to examine the effects of evolving aerosol mixing states on aerosol-radiation-cloud feedbacks.

54 ENVIRONMENTAL SCIENCES↗

Ice and Supercooled Liquid Water Distributions over the Southern Ocean based on In Situ Observations and Climate Model Simulations

Three climate models are evaluated using in situ airborne observations from the Southern Ocean Clouds, Radiation, Aerosol Transport Experimental Study (SOCRATES) campaign. The evaluation targets cloud phases, microphysical properties, thermodynamic conditions, and aerosol indirect effects from –40°C to 0°C. Compared with 580-s averaged observations (i.e., 100 km horizontal scale), the Community Atmosphere Model version 6 (CAM6) shows the most similar result for cloud phase frequency distribution and allows more liquid-containing clouds below –10°C compared with its predecessor—CAM5. The Energy Exascale Earth System Model (E3SM) underestimates (overestimates) ice phase frequencies below (above) –20°C. CAM6 and E3SM show liquid and ice water contents (i.e., LWC and IWC) similar to observations from –25°C to 0°C, but higher LWC and lower IWC than observations at lower temperatures. Simulated in-cloud RH shows higher minimum values than observations, possibly restricting ice growth during sedimentation. As number concentrations of aerosols larger than 500 nm (Na 500 ) increase, observations show increases of LWC, IWC, liquid, and ice number concentrations (N liq , N ice ). Number concentrations of aerosols larger than 100 nm (Na 100 ) only show positive correlations with LWC and N liq . From –20°C to 0°C, higher aerosol number concentrations are correlated with lower glaciation ratio and higher cloud fraction. From –40°C to –20°C, large aerosols show positive correlations with glaciation ratio. CAM6 shows small increases of LWC and N liq with Na 500 and Na 100 . E3SM shows small increases of N ice with Na 500 . Altogether, CAM6 and E3SM underestimate aerosol indirect effects on ice crystals and supercooled liquid droplets over the Southern Ocean.

54 ENVIRONMENTAL SCIENCES↗

The Influence of Sea Ice on Arctic Low Cloud Properties and Radiative Effects

The Arctic is one of the most climatically sensitive regions of the Earth. Climate models robustly project the Arctic to warm 2-3 times faster than the global mean surface temperature, termed polar warming amplification (PWA), but also display the widest range of surface temperature projections in this region. The response of the Arctic to increased CO2 modulates the response in tropical and extra-tropical regions through teleconnections in the atmospheric circulation. An increased frequency of extreme precipitation events in the northern mid-latitudes, for example, has been linked to the change in the background equator-to-pole temperature gradient implied by PWA. Understanding the Arctic climate system is therefore important for predicting global climate change. The ice albedo feedback is the primary mechanism driving PWA, however cloud and dynamical feedbacks significantly contribute. These feedback mechanisms, however, do not operate independently. How do clouds respond to variations in sea ice? This critical question is addressed by combining sea ice, cloud, and radiation observations from satellites, including CERES, CloudSAT, CALIPSO, MODIS, and microwave radiometers, to investigate sea ice-cloud interactions at the interannual timescale in the Arctic. Cloud characteristics are strongly tied to the atmospheric dynamic and thermodynamic state. Therefore, the sensitivity of Arctic cloud characteristics, vertical distribution and optical properties, to sea ice anomalies is computed within atmospheric dynamic and thermodynamic regimes. Results indicate that the cloud response to changes in sea ice concentration differs significantly between atmospheric state regimes. This suggests that (1) the atmospheric dynamic and thermodynamic characteristics and (2) the characteristics of the marginal ice zone are important for determining the seasonal forcing by cloud on sea ice variability.

Taylor, Patrick C.↗

Dust energetics in the gas phases of the interstellar medium - The origin of the Galactic large-scale far-infrared emission observed by IRAS

The large-scale Galactic properties within the most massive gas phases of the ISM are derived along with the distribution of total Galactic FIR luminosity among the three phases. Most of the Galaxy's total FIR luminosity is found to be emitted by cold dust associated with diffuse H I clouds and molecular gas. The total FIR luminosity of dust associated with extended low-density H II regions accounts for less than 10 percent of the Galaxy's total FIR output. The absence of a significant variation with longitude in the observed temperature of the dust associated with H I gas suggests that diffuse neutral clouds contain very small dust grains that are stochastically heated by the interstellar radiation field. The results are consistent with a model in which most of the FIR luminosity of molecular clouds arises from dust that is associated with giant molecular clouds and heated by embedded and nearby OB stars. H II regions in the inner Galaxy have a mean IR excess ratio of about 2.5, suggesting that the dust in these regions is heated primarily by directly absorbed stellar photons.

Sodroski, T. J.↗

Cloud-radiation Interactions and Cloud-climate Feedbacks from an Active-sensor Satellite Perspective

Clouds are ubiquitous in the troposphere. Their interactions with radiation may result in either a warming or a cooling of the Earth system and generate diverse climate feedbacks. The vertical structure of the radiative effects of clouds as well as the response of clouds to global warming (i.e., the cloud feedbacks) are inadequately constrained within the diversity of current climate models, which limits our ability to project the magnitude of future warming. In this chapter we show how relatively recent active-sensor spaceborne observations have narrowed constraints on cloud feedbacks. The value added beyond what can be retrieved from passive sensors is only just beginning to be exploited.

Cloud radiation↗