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At least 955 records · Page 53

Dust energetics in the gas phases of the interstellar medium - The origin of the Galactic large-scale far-infrared emission observed by IRAS

The large-scale Galactic properties within the most massive gas phases of the ISM are derived along with the distribution of total Galactic FIR luminosity among the three phases. Most of the Galaxy's total FIR luminosity is found to be emitted by cold dust associated with diffuse H I clouds and molecular gas. The total FIR luminosity of dust associated with extended low-density H II regions accounts for less than 10 percent of the Galaxy's total FIR output. The absence of a significant variation with longitude in the observed temperature of the dust associated with H I gas suggests that diffuse neutral clouds contain very small dust grains that are stochastically heated by the interstellar radiation field. The results are consistent with a model in which most of the FIR luminosity of molecular clouds arises from dust that is associated with giant molecular clouds and heated by embedded and nearby OB stars. H II regions in the inner Galaxy have a mean IR excess ratio of about 2.5, suggesting that the dust in these regions is heated primarily by directly absorbed stellar photons.

Sodroski, T. J.↗

Cloud-radiation Interactions and Cloud-climate Feedbacks from an Active-sensor Satellite Perspective

Clouds are ubiquitous in the troposphere. Their interactions with radiation may result in either a warming or a cooling of the Earth system and generate diverse climate feedbacks. The vertical structure of the radiative effects of clouds as well as the response of clouds to global warming (i.e., the cloud feedbacks) are inadequately constrained within the diversity of current climate models, which limits our ability to project the magnitude of future warming. In this chapter we show how relatively recent active-sensor spaceborne observations have narrowed constraints on cloud feedbacks. The value added beyond what can be retrieved from passive sensors is only just beginning to be exploited.

Cloud radiation↗

Understanding Uncertainty of Snow Radiative Transfer Modeling Within a Mixed Deciduous and Evergreen Forest

Satellite-based passive microwave observations provide the best available continuous observational estimates of global snow water storage due to their broad geographic footprint and low sensitivity to clouds and precipitation. However, these observations are subject to substantial uncertainty due to the complex radiative properties of snow and from interference in forested areas. Physical radiative transfer models can be leveraged to improve the fidelity of these observations and as a data-assimilation tool. In this article, the Dense Media Radiative Transfer model with Multiple Layers (DMRT-ML) is used to simulate snow brightness temperatures from data collected from snow pits excavated during a two-day-long field study performed a temperate forest in the Northeast United States. The simulations are evaluated against surface-based radiometer observations collected at the snow pits. The DMRT-ML is configured with varying complexity to determine the snowpack characteristics most essential toward simulating brightness temperature within a temperate forest with complicated snow stratigraphy. In general, the single-layer configurations were not sufficiently complex to accurately simulate snow brightness temperature without significant tuning. The most accurate simulation was a two-layer configuration with a prescribed ice layer separating the snow layers. This simulation had a root-mean-square error <;15 K for the 37-GHz frequency. More complicated snowpack stratigraphy configurations did not substantively improve the results over the two-layer model configuration. The DMRT-ML was also used to examine differences between redundant datasets of density and grain size. It was determined that similar snow data collection and radiative transfer model configuration techniques are critical to ensure cross-study comparability.

Theodore Letcher↗

Enhancing Convection Parameterization for Next Generation E3SM (Final Technical Report)

This technical report summarizes the achievements during the project period. The general goal of the project is to enhance the representation of atmospheric deep convection in the DOE global climate model E3SM. By implementing a stochastic convection scheme into E3SM, we improved the simulation of precipitation intensity and frequency. As a result, it has a profound impact on the simulation of other fields in the model, including aerosol scavenging by precipitation and aerosol radiative effects. We also implemented a convective cloud microphysics scheme into E3SMv2 to represent more accurately the interaction between convection and grid-scale clouds. An extensive analysis of model simulations as part of the Next Generation Development (NGD) convection scheme assessment project found that including the convective microphysics scheme improved the simulation of Madden-Julian oscillations (MJO) in the model. To make convective parameterization schemes more scale-aware as the GCM resolution increases, we analyzed the output from cloud-resolving model (CRM) simulations of both organized and unorganized convection by coarse-graining the CRM data to different GCM resolutions. Using a novel approach to modify the convective closure, we demonstrated that the convection scheme used in E3SM (ZM scheme) can be made scale-aware.

54 ENVIRONMENTAL SCIENCES↗

Cloud shadow effects on remote sensing

On relatively clear days, the shadow cast by an isolated, optically dense cloud produces an effect which is similar in extent and magnitude to the adjacency effects associated with high-contrast ground albedo boundaries. A Monte Carlo radiative transfer model has been used to examine the intensity and its components, comparing the cloud shadow case with that for a Lambertian albedo boundary. Although the behavior of the total intensity is nearly the same for both cases, the behaviors of the intensity components differ significantly.

Pearce, W. A.↗

Comparison of 30 day integrations with and without interactive clouds

A cloud radiation interaction parameterization package has recently been incorporated into a global spectral General Circulation Model (GCM) used for extended range prediction studies at GFDL. The elements of this package are summarized. Analysis of the time mean radiative and dynamical responses suggests that cloud radiation interaction has a favorable impact, overall, on systematic errors. The possible relevance of this sensitivity study to FIRE is mentioned.

Gordon, C. T.↗

Hyperspectral Remote Sensing of Atmosphere and Surface Properties

Atmospheric Infrared Sounder (AIRS), Infrared Atmospheric Sounding Interferometer (IASI), and Cross-track Infrared Sounder (CrIS) are all hyper-spectral satellite sensors with thousands of spectral channels. Top of atmospheric radiance spectra measured by these sensors contain high information content on atmospheric, cloud, and surface properties. Exploring high information content contained in these high spectral resolution spectra is a challenging task due to computation e ort involved in modeling thousands of spectral channels. Usually, only very small fractions (4{10 percent) of the available channels are included in physical retrieval systems or numerical weather forecast (NWP) satellite data assimilations. We will describe a method of simultaneously retrieving atmospheric temperature, moisture, cloud, and surface properties using all available spectral channels without sacrificing computational speed. The essence of the method is to convert channel radiance spectra into super-channels by an Empirical Orthogonal Function (EOF) transformation. Because the EOFs are orthogonal to each other, about 100 super-channels are adequate to capture the information content of the radiance spectra. A Principal Component-based Radiative Transfer Model (PCRTM) developed at NASA Langley Research Center is used to calculate both the super-channel magnitudes and derivatives with respect to atmospheric profiles and other properties. There is no need to perform EOF transformations to convert super channels back to spectral space at each iteration step for a one-dimensional variational retrieval or a NWP data assimilation system. The PCRTM forward model is also capable of calculating radiative contributions due to multiple-layer clouds. The multiple scattering effects of the clouds are efficiently parameterized. A physical retrieval algorithm then performs an inversion of atmospheric, cloud, and surface properties in super channel domain directly therefore both reducing the computational need and preserving the information content of the IASI measurements. The inversion algorithm is based on a non-linear Levenberg-Marquardt method with climatology covariance matrices and a priori information as constraints. One advantage of this approach is that it uses all information content from the hyper-spectral data so that the retrieval is less sensitive to instrument noise and eliminates the need for selecting a sub-set of the channels.

Liu, Xu↗

Far-ultraviolet emission from the Taurus molecular cloud

Far-ultraviolet spectra of diffuse emission from a region in the Taurus molecular cloud are presented. These data were obtained with the Berkeley spectrometer on NASA's Ultraviolet Experiment (UVX) payload. The intensity of the continuum emission drops as the optical depth increases toward the denser part of the cloud, an effect which is the opposite of that observed for the diffuse flux at high galactic latitudes. At the center of the aperture, the optical depth is very large, and the continuum emission must be produced by backscattering. At the edges of the cloud, the continuum intensity rises by a factor of 2. The data are interpreted with a new radiative transfer model, which is significantly more sophisticated than its predecessors. If the grain scattering properties are constant across the cloud, a unique best-fit combination can be determined from the data. The best-fit albedo is 0.6 +/- 0.1 at 1600 A. The best-fit value for the phase factor g is 0.5 +/- 0.15. The intensity of the flourescence of H2, combined with an upper limit to the column density of atomic hydrogen associated with the cloud, sets a lower limit of about 130/cm to the density in the flourescence region. Our estimate of the flux incident on the cloud at 1000 A is a factor of 2 to 3 lower than the value required to produce the measured flourescence intensity. Most mechanisms which might reconcile the discrepancy reduce the derived albedo and phase factor.

Hurwitz, M.↗

Use of MERRA-2 in the National Solar Radiation Database and Beyond

The National Solar Radiation Database (NSRDB) is a flagship product of NREL that provides solar radiation and ancillary meteorological information through a GIS based portal. This data is provided at a 4kmx4km spatial and 30 minute temporal resolution covering the period between 1998-2015. The gridded data that is distributed by the NSRDB is derived from satellite measurements using the Physical Solar Model (PSM) that contains a 2-stage approach. This 2-stage approach consists of first retrieving cloud properties using measurement from the GOES series of satellites and using that information in a radiative transfer model to estimate solar radiation at the surface. In addition to the satellite data the model requires ancillary meteorological information that is provided mainly by NASA's Modern Era Retrospecitve Analysis for Research and Applications (MERRA-2) 2 model output. This presentation provides an insight into how the NSRDB is developed using the PSM and how the various sources of data including the MERRA-2 data is used during the process.

14 SOLAR ENERGY↗

Advancing Understanding of Deep Convective Anvil Clouds

In this project we use ground-based DOE ARM observations, satellite observations, and Weather Research and Forecasting (WRF) model simulations to arrive at a more complete understanding (or, new theory) of how atmospheric heating profiles in thunderstorm cores drives how quickly air rises in the storms. The rate at which air motion increases or decreases with altitude directly relates to how much cloud mass is ejected laterally into the adjacent atmosphere, which then influences the development and maintenance of “stratiform raining cloud anvils”. Our work has led to new equations connecting the heating in these thunderstorms to these stratiform clouds, with the connection modulated by the stability structure of the atmosphere (i.e., if more stable, then a more rapid change in thunderstorm heating with altitude results in more stratiform cloud, independent of whether over land or ocean, or how organized the thunderstorms are). Improving knowledge of stratiform clouds is important, since they contribute to substantial accumulated rainfall (important to agriculture and local hydrology) as well as radiation, given their large areal extents and lifetime. The radiation impacts likely impact simulated cloud feedback in all Earth System models (ESMs).

54 ENVIRONMENTAL SCIENCES↗

The effects of atmospheric cloud radiative forcing on climate

In order to isolate the effects of atmospheric cloud radiative forcing (ACRF) on climate, the general circulation of an ocean-covered earth called 'Seaworld' was simulated using the Colorado State University GCM. Most current climate models, however, do not include an interactive ocean. The key simplifications in 'Seaworld' are the fixed boundary temperature with no land points, the lack of mountains and the zonal uniformity of the boundary conditions. Two 90-day 'perpetual July' simulations were performed and analyzed the last sixty days of each. The first run included all the model's physical parameterizations, while the second omitted the effects of clouds in both the solar and terrestrial radiation parameterizations. Fixed and identical boundary temperatures were set for the two runs, and resulted in differences revealing the direct and indirect effects of the ACRF on the large-scale circulation and the parameterized hydrologic processes.

Randall, David A.↗

Radiative effects of polar stratospheric clouds during the Airborne Antarctic Ozone Experiment and the Airborne Arctic Stratospheric Expedition

Results are presented of a study of the radiative effects of polar stratospheric clouds during the Airborne Antarctic Ozone Experiment (AAOE) and the Airborne Arctic Stratospheric Expedition (AASE) in which daily 3D Type I nitric acid trihydrate (NAT) and Type II water ice polar stratospheric clouds (PSCs) were generated in the polar regions during AAOE and the AASE aircraft missions. Mission data on particular composition and size, together with NMC-analyzed temperatures, are used. For AAOE, both Type I and Type II clouds were formed for the time period August 23 to September 17, after which only Type I clouds formed. During AASE, while Type I clouds were formed for each day between January 3 and February 10, Type II clouds formed on only two days, January 24 and 31. Mie theory and a radiative transfer model are used to compute the radiative heating rates during the mission periods, for clear and cloudy lower sky cases. Only the Type II water ice clouds have a significant radiative effect, with the Type I NATO PSCs generating a net heating or cooling of 0.1 K/d or less.

Rosenfield, Joan E.↗

Improving GCM Predictability of Mixed-Phase Clouds and Aerosol Interactions at High Latitudes with ARM Observations

The overachieving goal of this project is to improve the predictability of mixed-phase clouds and aerosol interactions in the Community Atmosphere Model version 6 (CAM6) through comparison with the ARM observations. There are three main objectives of the proposed study: (1) Improve the representation of ice microphysical processes in mixed-phase clouds; (2) Test the performance of ice microphysics in CESM-CAM6 with the ARM observations in northern and southern high latitudes; and (3) Examine mixed-phase cloud microphysics-aerosol-turbulence-radiation interactions in CESM-CAM6. In this project, we have (1) Improved the representation of ice microphysical processes in mixed-phase clouds in CESM-CAM6 by implementing the marine organic aerosol (MOA) and treating the ice nucleating particles (INPs) from MOA and its impacts on mixed-phase clouds. We improved the treatment of ice depositional growth through the Wegener–Bergeron–Findeisen (WBF) process by considering the subgrid heterogeneous distributions between liquid droplets and ice crystals in mixed-phase clouds; (2) Tested the performance of ice microphysics in CESM-CAM6 with the ARM observations at high latitudes. We compared the simulated INP concentrations with the ARM observations, e.g., from M-PACE, ISDAC, INPOP, and other data (Mace Head, Zeppelin, CAPRICORN). We examined the impact of improved WBF treatment on model simulated Arctic mixed-phase clouds observed in the M-PACE field campaign. Seasonal variations of modeled mixed-phase cloud properties (LWO, IWP) are compared with the ground-based remote sensing retrievals at the ARM’s NSA $Utqia\dot{g}vik$ site; and (3) Examined mixed-phase cloud microphysics-aerosol-dynamics-radiation interactions in CESM-CAM6 that include the impacts of MOA INPs, and impacts of different model parameterizations (CLUBB versus UW turbulence & shallow convection schemes, MG2 versus MG1) on high-latitude mixed-phase cloud properties. Aerosol indirect effects of MOA through the liquid phase (droplet activation) and ice phase processes (e.g., the glaciation indirect effect) were investigated.

54 ENVIRONMENTAL SCIENCES↗

Radiative effects of interannually varying vs. interannually invariant aerosol emissions from fires

Abstract. Open-burning fires play an important role in the earth's climate system. In addition to contributing a substantial fraction of global emissions of carbon dioxide, they are a major source of atmospheric aerosols containing organic carbon, black carbon, and sulfate. These “fire aerosols” can influence the climate via direct and indirect radiative effects. In this study, we investigate these radiative effects and the hydrological fast response using the Community Atmosphere Model version 5 (CAM5). Emissions of fire aerosols exert a global mean net radiative effect of −1.0 W m−2, dominated by the cloud shortwave response to organic carbon aerosol. The net radiative effect is particularly strong over boreal regions. Conventionally, many climate modelling studies have used an interannually invariant monthly climatology of emissions of fire aerosols. However, by comparing simulations using interannually varying emissions vs. interannually invariant emissions, we find that ignoring the interannual variability of the emissions can lead to systematic overestimation of the strength of the net radiative effect of the fire aerosols. Globally, the overestimation is +23 % (−0.2 W m−2). Regionally, the overestimation can be substantially larger. For example, over Australia and New Zealand the overestimation is +58 % (−1.2 W m−2), while over Boreal Asia the overestimation is +43 % (−1.9 W m−2). The systematic overestimation of the net radiative effect of the fire aerosols is likely due to the non-linear influence of aerosols on clouds. However, ignoring interannual variability in the emissions does not appear to significantly impact the hydrological fast response. In order to improve understanding of the climate system, we need to take into account the interannual variability of aerosol emissions.

54 ENVIRONMENTAL SCIENCES↗

The Emissions Model Intercomparison Project (Emissions-MIP): quantifying model sensitivity to emission characteristics

Abstract. Anthropogenic emissions of aerosols and precursor compounds are known to significantly affect the energy balance of the Earth–atmosphere system, alter the formation of clouds and precipitation, and have a substantial impact on human health and the environment. Global models are an essential tool for examining the impacts of these emissions. In this study, we examine the sensitivity of model results to the assumed height of SO2 injection, seasonality of SO2 and black carbon (BC) particulate emissions, and the assumed fraction of SO2 emissions that is injected into the atmosphere as particulate phase sulfate (SO4) in 11 climate and chemistry models, including both chemical transport models and the atmospheric component of Earth system models. We find large variation in atmospheric lifetime across models for SO2, SO4, and BC, with a particularly large relative variation for SO2, which indicates that fundamental aspects of atmospheric sulfur chemistry remain uncertain. Of the perturbations examined in this study, the assumed height of SO2 injection had the largest overall impacts, particularly on global mean net radiative flux (maximum difference of −0.35 W m−2), SO2 lifetime over Northern Hemisphere land (maximum difference of 0.8 d), surface SO2 concentration (up to 59 % decrease), and surface sulfate concentration (up to 23 % increase). Emitting SO2 at height consistently increased SO2 and SO4 column burdens and shortwave cooling, with varying magnitudes, but had inconsistent effects across models on the sign of the change in implied cloud forcing. The assumed SO4 emission fraction also had a significant impact on net radiative flux and surface sulfate concentration. Because these properties are not standardized across models this is a source of inter-model diversity typically neglected in model intercomparisons. These results imply a need to ensure that anthropogenic emission injection height and SO4 emission fraction are accurately and consistently represented in global models.

54 ENVIRONMENTAL SCIENCES↗

Science support for the Earth radiation budget experiment

The work undertaken as part of the Earth Radiation Budget Experiment (ERBE) included the following major components: The development and application of a new cloud retrieval scheme to assess errors in the radiative fluxes arising from errors in the ERBE identification of cloud conditions. The comparison of the anisotropy of reflected sunlight and emitted thermal radiation with the anisotropy predicted by the Angular Dependence Models (ADM's) used to obtain the radiative fluxes. Additional studies included the comparison of calculated longwave cloud-free radiances with those observed by the ERBE scanner and the use of ERBE scanner data to track the calibration of the shortwave channels of the Advanced Very High Resolution Radiometer (AVHRR). Major findings included: the misidentification of cloud conditions by the ERBE scene identification algorithm could cause 15 percent errors in the shortwave flux reflected by certain scene types. For regions containing mixtures of scene types, the errors were typically less than 5 percent, and the anisotropies of the shortwave and longwave radiances exhibited a spatial scale dependence which, because of the growth of the scanner field of view from nadir to limb, gave rise to a view zenith angle dependent bias in the radiative fluxes.

Coakley, James A., Jr.↗

Raman Lidar Measurements of Water Vapor and Cirrus Clouds During the Passage of Hurricane Bonnie

The NASA/GSFC Scanning Raman Lidar (SRL) was stationed on Andros Island in the Bahamas during August - September, 1998 as a part of the third Convection and Moisture Experiment (CAMEX-3) which focussed on hurricane development and tracking. During the period August 21 - 24, hurricane Bonnie passed near Andros Island and influenced the water vapor and cirrus cloud measurements acquired by the SRL. Two drying signatures related to the hurricane were recorded by the SRL (Scanning Raman Lidar) and other sensors. Cirrus cloud optical depths (at 351 nm) were also measured during this period. Optical depth values ranged from approximately 0.01 to 1.4. The influence of multiple scattering on these optical depth measurements was studied with the conclusion that the measured values of optical depth are less than the actual value by up to 20% . The UV/IR cirrus cloud optical depth ratio was estimated based on a comparison of lidar and GOES measurements. Simple radiative transfer model calculations compared with GOES satellite brightness temperatures indicate that satellite radiances are significantly affected by the presence of cirrus clouds if IR optical depths are approximately 0.02 or greater. This has implications for satellite cirrus detection requirements.

Whiteman, D. N.↗

Raman Lidar Measurements of Water Vapor and Cirrus Clouds During the Passage of Hurricane Bonnie

The NASA/GSFC Scanning Raman Lidar (SRL) was stationed on Andros Island in the Bahamas during August - September, 1998 as a part of the third Convection and Moisture Experiment (CAMEX-3) which focussed on hurricane development and tracking. During the period August 21 - 24, hurricane Bonnie passed near Andros Island and influenced the water vapor and cirrus cloud measurements acquired by the SRL. Two drying signatures related to the hurricane were recorded by the SRL and other sensors. Cirrus cloud optical depths (at 351 nm) were also measured during this period. Optical depth values ranged from approximately 0.01 to 1.4. The influence of multiple scattering on these optical depth measurements was studied with the conclusion that the measured values of optical depth are less than the actual value by up to 20%. The UV/lR cirrus cloud optical depth ratio was estimated based on a comparison of lidar and GOES measurements. Simple radiative transfer model calculations compared with GOES satellite brightness temperatures indicate that satellite radiances are significantly affected by the presence of cirrus clouds if IR optical depths are approximately 0.02 or greater. This has implications for satellite cirrus detection requirements.

Whiteman, D. N.↗