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All sourcesNASA NTRSDOE OSTI
DOE OSTI2015

Effect of gamma irradiation on DC electrical conductivity of ZnO nanoparticles

The temperature dependent dc electrical conductivity of gamma irradiated Zinc oxide (ZnO) nanoparticles is presented in this paper. The X-ray diffraction (XRD) pattern shows hexagonal wurtzite structure of ZnO. Fourier Transform Infrared Spectroscopy (FTIR) confirms Zn-O stretching vibrations. UV-Visible spectroscopy studies show that the energy band gap (E{sub g}) of the prepared ZnO nanoparticles increases with respect to gamma irradiation dose, which can be related to room temperature dc electrical conductivity. The result shows significant variation in the high temperature dc electrical conductivity of ZnO nanoparticles due to gamma irradiation.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

Detecting new γ-ray sources based on multi-frequency data the case of 1WHSPJ031423.9+061956

We use the Fermi Science Tools in an attempt to unveil faint γ-ray blazars that may be above the threshold for detectability with Fermi-LAT and are not identified by automated methods. Our search for new sources in the 100MeV-300GeV band is mainly driven by the 1/2WHSP catalogs, which list high synchrotron peaked blazars expected to be emitters of VHE photons. Here we present the γ-ray detection of 1WHSP J031423.9+061956, modelling its high energy spectrum as a power law. We describe an example where multi-frequency selection, performed at much lower energies (from radio to X-ray), helps to pin-point a high energy source. The 1/2WHSP catalogs are built with the aim of providing a list of TeV targets for the VHE arrays of Cherenkov telescopes. Moreover, these catalogs provide useful seeds for identifying new high energy sources within the raw-data from Fermi. With the aid of multi-frequency data, we can explore the very high energy domain in greater details, improving the description of the γ-ray sky.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2016

The gamma irradiation effects on structural and optical properties of silk fibroin/HPMC blend films

In this paper the structural, chemical and optical properties of gamma irradiated silk fibroin/Hydroxypropyl methyl cellulose (SF-HPMC) blend films were studied using X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FTIR) and UV-visible spectroscopy. The results indicate that the gamma radiation did not affect significantly the primary structure of polypeptide arrangement in the blend films. But the optical properties of the blends changed with gamma irradiation dosage.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2013

THE AFTERGLOW AND ULIRG HOST GALAXY OF THE DARK SHORT GRB 120804A

We present the optical discovery and subarcsecond optical and X-ray localization of the afterglow of the short GRB 120804A, as well as optical, near-IR, and radio detections of its host galaxy. X-ray observations with Swift/XRT, Chandra, and XMM-Newton extending to {delta}t Almost-Equal-To 19 days reveal a single power-law decline. The optical afterglow is faint, and comparison to the X-ray flux indicates that GRB 120804A is ''dark'', with a rest-frame extinction of A {sup host}{sub V} Almost-Equal-To 2.5 mag (at z = 1.3). The intrinsic neutral hydrogen column density inferred from the X-ray spectrum, N{sub H,{sub int}}(z = 1.3) Almost-Equal-To 2 Multiplication-Sign 10{sup 22} cm{sup -2}, is commensurate with the large extinction. The host galaxy exhibits red optical/near-IR colors. Equally important, JVLA observations at Almost-Equal-To 0.9-11 days reveal a constant flux density of F{sub {nu}}(5.8 GHz) = 35 {+-} 4 {mu}Jy and an optically thin spectrum, unprecedented for GRB afterglows, but suggestive instead of emission from the host galaxy. The optical/near-IR and radio fluxes are well fit with the scaled spectral energy distribution of the local ultraluminous infrared galaxy (ULIRG) Arp 220 at z Almost-Equal-To 1.3, with a resulting star formation rate of x Almost-Equal-To 300 M{sub Sun} yr{sup -1}. The inferred extinction and small projected offset (2.2 {+-} 1.2 kpc) are also consistent with the ULIRG scenario, as is the presence of a companion galaxy at the same redshift and with a separation of about 11 kpc. The limits on radio afterglow emission, in conjunction with the observed X-ray and optical emission, require a circumburst density of n {approx} 10{sup -3} cm{sup -3}, an isotropic-equivalent energy scale of E{sub {gamma},{sub iso}} Almost-Equal-To E{sub K,{sub iso}} Almost-Equal-To 7 Multiplication-Sign 10{sup 51} erg, and a jet opening angle of {theta}{sub j} {approx}> 11 Degree-Sign . The expected fraction of luminous infrared galaxies in the short GRB host sample is {approx}0.01 and {approx}0.25 (for pure stellar mass and star formation weighting, respectively). Thus, the observed fraction of two events in about 25 hosts (GRBs 120804A and 100206A) appears to support our previous conclusion that short GRBs track both stellar mass and star formation activity.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2013

SUZAKU/WAM AND RHESSI OBSERVATIONS OF NON-THERMAL ELECTRONS IN SOLAR MICROFLARES

We report on hard X-ray spectroscopy of solar microflares observed by the Wide-band All-sky Monitor (WAM), on board the Suzaku satellite, and by RHESSI. WAM transient data provide wide energy band (50 keV-5 MeV) spectra over a large field of view ({approx}2{pi} sr) with a time resolution of 1 s. WAM is attractive as a hard X-ray solar flare monitor due to its large effective area ({approx}800 cm{sup 2} at 100 keV, {approx}13 times larger than that of RHESSI). In particular, this makes it possible to search for high energy emission in microflares that is well below the RHESSI background. The WAM solar flare list contains six GOES B-class microflares that were simultaneously observed by RHESSI between the launch of Suzaku in 2005 July and 2010 March. At 100 keV, the detected WAM fluxes are more than {approx}20 times below the typical RHESSI instrumental background count rates. The RHESSI and WAM non-thermal spectra are in good agreement with a single power law with photon spectral indices between 3.3 and 4.5. In a second step, we also searched the RHESSI microflare list for events that should be detectable by WAM, assuming that the non-thermal power-law emission seen by RHESSI extends to >50 keV. From the 12 detectable events between 2005 July and 2007 February, 11 were indeed seen by WAM. This shows that microflares, similar to regular flares, can accelerate electrons to energies up to at least 100 keV.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Particle densities within the acceleration region of a solar flare

The limb flare SOL2012-07-19T05:58 (M7.7) provides the best example of a non-thermal above-the-loop-top hard X-ray source with simultaneous observations by the Reuven Ramaty High Energy Solar Spectroscopic Imager (RHESSI) and the Atmospheric Imaging Assembly on board the Solar Dynamic Observatory. By combining the two sets of observations, we present the first direct measurement of the thermal proton density and non-thermal electron density within the above-the-loop-top source where particle acceleration occurs. We find that both densities are of the same order of magnitude of a few times 10{sup 9} cm{sup –3}, about 30 times lower than the density in the underlying thermal flare loops. The equal densities indicate that the entire electron population within the above-the-loop-top source is energized. While the derived densities depend on the unknown source depth and filling factor, the ratio of these two densities does not. Within the uncertainties, the ratio is one for a low energy cutoff of the non-thermal electron spectrum between 10 and 15 keV. RHESSI observations only constrain the cutoff energy to below ∼15 keV, leaving the spectral shape of the electrons within the above-the-loop-top source at lower energies unknown. Nevertheless, these robust results strongly corroborate earlier findings that the above-the-loop-top source is the acceleration region where a bulk energization process acts on all electrons.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Spectral lag features of GRB 060814 from swift bat and Suzaku observations

This work reports a study on the spectral lag of the prompt emission spectrum of a multi-pulse gamma-ray burst (GRB) GRB 060814 (z = 0.84) using the observations of the Swift Burst Alert Telescope and the Suzaku Wide Area Monitor. We found that the spectral lag for GRB 060814 is positive for the first two and the fourth pulses, while the third pulse exhibits negative lag. However, the time variation of the E {sub peak} of all the stated pulses shows a similar trend. The leading models for spectral lags in GRBs are thus found inadequate to explain the observed spectral lag features of GRB 060814. Probable causes of the spectral lag characteristics of GRB 060814 are discussed.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

The study of TeV variability and the duty cycle of Mrk 421 from 3 Yr of observations with the milagro observatory

TeV-flaring activity with timescales as short as tens of minutes and an orphan TeV flare have been observed from the blazar Markarian 421 (Mrk 421). The TeV emission from Mrk 421 is believed to be produced by leptonic synchrotron self-Compton (SSC) emission. In this scenario, correlations between the X-ray and the TeV fluxes are expected, TeV orphan flares are hardly explained, and the activity (measured as duty cycle) of the source at TeV energies is expected to be equal to or less than that observed in X-rays if only SSC is considered. To estimate the TeV duty cycle of Mrk 421 and to establish limits on its variability at different timescales, we continuously observed Mrk 421 with the Milagro observatory. Mrk 421 was detected by Milagro with a statistical significance of 7.1 standard deviations between 2005 September 21 and 2008 March 15. The observed spectrum is consistent with previous observations by VERITAS. We estimate the duty cycle of Mrk 421 for energies above 1 TeV for different hypotheses of the baseline flux and for different flare selections and we compared our results with the X-ray duty cycle estimated by Resconi et al. The robustness of the results is discussed.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Is the ultra-high energy cosmic-ray excess observed by the telescope array correlated with IceCube neutrinos?

The Telescope Array (TA) has observed a statistically significant excess in cosmic rays with energies above 57 EeV in a region of approximately 1150 deg{sup 2} centered on coordinates R.A. = 146.7, decl. = 43.2. We note that the location of this excess correlates with 2 of the 28 extraterrestrial neutrinos recently observed by IceCube. The overlap between the two IceCube neutrinos and the TA excess is statistically significant at the 2σ level. Furthermore, the spectrum and intensity of the IceCube neutrinos is consistent with a single source which would also produce the TA excess. Finally, we discuss possible source classes with the correct characteristics to explain the cosmic-ray and neutrino fluxes with a single source.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Observation of small-scale anisotropy in the arrival direction distribution of TeV cosmic rays with HAWC

The High-Altitude Water Cherenkov (HAWC) Observatory is sensitive to gamma rays and charged cosmic rays at TeV energies. The detector is still under construction, but data acquisition with the partially deployed detector started in 2013. An analysis of the cosmic-ray arrival direction distribution based on 4.9 × 10{sup 10} events recorded between 2013 June and 2014 February shows anisotropy at the 10{sup –4} level on angular scales of about 10°. The HAWC cosmic-ray sky map exhibits three regions of significantly enhanced cosmic-ray flux; two of these regions were first reported by the Milagro experiment. A third region coincides with an excess recently reported by the ARGO-YBJ experiment. An angular power spectrum analysis of the sky shows that all terms up to ℓ = 15 contribute significantly to the excesses.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

ALMA observations of the host galaxy of GRB 090423 at z = 8.23: deep limits on obscured star formation 630 million years after the big bang

We present rest-frame far-infrared (FIR) and optical observations of the host galaxy of GRB 090423 at z = 8.23 from the Atacama Large Millimeter Array (ALMA) and the Spitzer Space Telescope, respectively. The host remains undetected to 3σ limits of F {sub ν}(222 GHz) ≲ 33 μJy and F {sub ν}(3.6 μm) ≲ 81 nJy. The FIR limit is about 20 times fainter than the luminosity of the local ULIRG Arp 220 and comparable to the local starburst M 82. Comparing this with model spectral energy distributions, we place a limit on the infrared (IR) luminosity of L {sub IR}(8-1000 μm) ≲ 3 × 10{sup 10} L {sub ☉}, corresponding to a limit on the obscured star formation rate of SFR{sub IR}≲5 M {sub ☉} yr{sup –1}. For comparison, the limit on the unobscured star formation rate from Hubble Space Telescope rest-frame ultraviolet (UV) observations is SFR{sub UV} ≲ 1 M {sub ☉} yr{sup –1}. We also place a limit on the host galaxy stellar mass of M {sub *} ≲ 5 × 10{sup 7} M {sub ☉} (for a stellar population age of 100 Myr and constant star formation rate). Finally, we compare our millimeter observations to those of field galaxies at z ≳ 4 (Lyman break galaxies, Lyα emitters, and submillimeter galaxies) and find that our limit on the FIR luminosity is the most constraining to date, although the field galaxies have much larger rest-frame UV/optical luminosities than the host of GRB 090423 by virtue of their selection techniques. We conclude that GRB host galaxies at z ≳ 4, especially those with measured interstellar medium metallicities from afterglow spectroscopy, are an attractive sample for future ALMA studies of high redshift obscured star formation.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

COLLISIONAL RELAXATION OF ELECTRONS IN A WARM PLASMA AND ACCELERATED NONTHERMAL ELECTRON SPECTRA IN SOLAR FLARES

Extending previous studies of nonthermal electron transport in solar flares, which include the effects of collisional energy diffusion and thermalization of fast electrons, we present an analytic method to infer more accurate estimates of the accelerated electron spectrum in solar flares from observations of the hard X-ray spectrum. Unlike for the standard cold-target model, the spatial characteristics of the flaring region, especially the necessity to consider a finite volume of hot plasma in the source, need to be taken into account in order to correctly obtain the injected electron spectrum from the source-integrated electron flux spectrum (a quantity straightforwardly obtained from hard X-ray observations). We show that the effect of electron thermalization can be significant enough to nullify the need to introduce an ad hoc low-energy cutoff to the injected electron spectrum in order to keep the injected power in non-thermal electrons at a reasonable value. Rather, the suppression of the inferred low-energy end of the injected spectrum compared to that deduced from a cold-target analysis allows the inference from hard X-ray observations of a more realistic energy in injected non-thermal electrons in solar flares.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

Modeling the multi-band afterglow of GRB 091127: Evidence of a hard electron energy spectrum with an injection break

The afterglows of gamma-ray bursts (GRBs) are believed to originate from the synchrotron emission of shock-accelerated electrons produced by the interaction between the outflow and the external medium. The accelerated electrons are usually assumed to follow a power-law energy distribution with an index of p. Observationally, although most GRB afterglows have a p larger than 2, there are still a few GRBs suggestive of a hard (p<2) electron spectrum. The well-sampled broad-band afterglow data for GRB 091127 show evidence of a hard electron spectrum and strong spectral evolution, with a spectral break moving from high to lower energies. The spectral break evolves very fast and cannot be explained by the cooling break in the standard afterglow model, unless evolving microphysical parameters are assumed. In addition, the multi-band afterglow light curves show an achromatic break at around 33 ks. Based on the model of a hard electron spectrum with an injection break, we interpret the observed spectral break as the synchrotron frequency corresponding to the injection break, and the achromatic break as a jet break caused by the jet-edge effect. It is shown that the spectral evolution and the multi-band afterglow light curves of GRB 091127 can be well reproduced by this model.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

THE UNUSUAL RADIO AFTERGLOW OF THE ULTRA-LONG GAMMA-RAY BURST GRB 130925A

GRB 130925A is one of the recent additions to the growing family of ultra-long gamma-ray bursts (GRBs; T90 ≳1000 s). While the X-ray emission of ultra-long GRBs have been studied extensively in the past, no comprehensive radio data set has been obtained so far. We report here the early discovery of an unusual radio afterglow associated with the ultra-long GRB 130925A. The radio emission peaks at low-frequencies (∼7 GHz) at early times, only 2.2 days after the burst occurred. More notably, the radio spectrum at frequencies above 10 GHz exhibits a rather steep cut-off, compared to other long GRB radio afterglows. This cut-off can be explained if the emitting electrons are either mono-energetic or originate from a rather steep, dN/dE ∝ E{sup −4}, power-law energy distribution. An alternative electron acceleration mechanism may be required to produce such an electron energy distribution. Furthermore, the radio spectrum exhibits a secondary underlying and slowly varying component. This may hint that the radio emission we observed is comprised of emission from both a reverse and a forward shock. We discuss our results in comparison with previous works that studied the unusual X-ray spectrum of this event and discuss the implications of our findings on progenitor scenarios.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

THE WISE BLAZAR-LIKE RADIO-LOUD SOURCES: AN ALL-SKY CATALOG OF CANDIDATE γ-RAY BLAZARS

We present a catalog of radio-loud candidate γ-ray emitting blazars with WISE mid-infrared colors similar to the colors of confirmed γ-ray blazars. The catalog is assembled from WISE sources detected in all four WISE filters, with colors compatible with the three-dimensional locus of the WISE γ-ray emitting blazars, and which can be spatially cross-matched with radio sources from one of the three radio surveys: NVSS, FIRST, and/or SUMSS. Our initial WISE selection uses a slightly modified version of previously successful algorithms. We then select only the radio-loud sources using a measure of the radio-to-IR flux, the q {sub 22} parameter, which is analogous to the q {sub 24} parameter known in the literature but which instead uses the WISE band-four flux at 22 μm. Our final catalog contains 7855 sources classified as BL Lacs, FSRQs, or mixed candidate blazars; 1295 of these sources can be spatially re-associated as confirmed blazars. We describe the properties of the final catalog of WISE blazar-like radio-loud sources and consider possible contaminants. Finally, we discuss why this large catalog of candidate γ-ray emitting blazars represents a new and useful resource to address the problem of finding low-energy counterparts to currently unidentified high-energy sources.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2013

RADIATION MECHANISM AND JET COMPOSITION OF GAMMA-RAY BURSTS AND GeV-TeV-SELECTED RADIO-LOUD ACTIVE GALACTIC NUCLEI

Gamma-ray bursts (GRBs) and GeV-TeV-selected radio-loud active galactic nuclei (AGNs) are compared based on our systematic modeling of the observed spectral energy distributions of a sample of AGNs with a single-zone leptonic model. We show that the correlation between the jet power (P{sub jet}) and the prompt gamma-ray luminosity (L{sub jet}) of GRBs is consistent, within the uncertainties, with the correlation between jet power and the synchrotron peak luminosity (L{sub s,jet}) of flat spectrum radio quasars (FSRQs). Their radiation efficiencies ({epsilon}) are also comparable (>10% for most sources), which increase with the bolometric jet luminosity (L{sub bol,jet}) for FSRQs and with the L{sub jet} for GRBs with similar power-law indices. BL Lac objects (BL Lacs) do not follow the P{sub jet}-L{sub s,jet} relation of FSRQs. They have lower {epsilon} and L{sub bol,jet} values than FSRQs, and a tentative L{sub bol,jet}-{epsilon} relation is also found, with a power-law index different from that of the FSRQs. The magnetization parameters ({sigma}) of FSRQs are on average larger than that of BL Lacs. They are anti-correlated with {epsilon} for the FSRQs, but positively correlated with {epsilon} for the BL Lacs. GeV narrow-line Seyfert 1 galaxies potentially share similar properties with FSRQs. Based on the analogy between GRBs and FSRQs, we suggest that the prompt gamma-ray emission of GRBs is likely produced by the synchrotron process in a magnetized jet with high radiation efficiency, similar to FSRQs. The jets of BL Lacs, on the other hand, are less efficient and are likely more matter-dominated.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

Neutron activation of natural materials in a PWR spectrum: feedback on {sup 116m}In relative γ emission intensities and half-life

During the MAESTRO program, carried out between 2011 and 2014 in MINERVE zero power reactor, common Gen-II and Gen-III light water reactor materials were irradiated. For some of these materials, the decay of their activation products was also measured by γ spectrometry. Initially devoted to the measurement of the integral capture cross section by activation and reactivity-oscillation method, these results can also provide useful information on decay data of various radionuclides. This approach of this experiment led to a common roadmap shared by the Experimental Physics Section and the Henri Becquerel National Laboratory to improve decay data in nuclear data libraries. Results discussed in this paper concern the relative emission intensities of the main γ rays of {sup 116m}In. Six irradiations of samples with various physical forms of {sup nat}In were carried out. Measurements were analyzed using decay data from several evaluations and it is shown that γ ray activities are not consistent. Analyses were carried out to provide new relative γ emission intensities from these measurements. The {sup 116m}In half-life has also been measured and shows a good agreement with existing values. Finally, an overview of the foreseen results on additional decay data from the MAESTRO program is given. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2017

Methods of chemical and phase composition analysis of gallstones

This review presents the instrumental methods used for chemical and phase composition investigation of gallstones. A great body of data has been collected in the literature on the presence of elements and their concentrations, obtained by fluorescence microscopy, X-ray fluorescence spectroscopy, neutron activation analysis, proton (particle) induced X-ray emission, atomic absorption spectroscopy, high-resolution gamma-ray spectrometry, electron paramagnetic resonance. Structural methods—powder X-ray diffraction, infrared spectroscopy, Raman spectroscopy—provide information about organic and inorganic phases in gallstones. Stone morphology was studied at the macrolevel with optical microscopy. Results obtained by analytical scanning and transmission electron microscopy with X-ray energy dispersive spectrometry are discussed. The chemical composition and structure of gallstones determine the strategy of removing stone from the body and treatment of patients: surgery or dissolution in the body. Therefore one chapter of the review describes the potential of dissolution methods. Early diagnosis and appropriate treatment of the disease depend on the development of clinical methods for in vivo investigation, which gave grounds to present the main characteristics and potential of ultrasonography (ultrasound scanning), magnetic resonance imaging, and X-ray computed tomography.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗