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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 973 records · Page 54
All sourcesNASA NTRSDOE OSTI
DOE OSTI2013

Magnetic reconnection process in transient coaxial helicity injection

The physics of magnetic reconnection and fast flux closure in transient coaxial helicity injection experiments in NSTX is examined using resistive MHD simulations. These simulations have been performed using the NIMROD code with fixed boundary flux (including NSTX poloidal coil currents) in the NSTX experimental geometry. Simulations show that an X point is formed in the injector region, followed by formation of closed flux surfaces within 0.5 ms after the driven injector voltage and injector current begin to rapidly decrease. As the injector voltage is turned off, the field lines tend to untwist in the toroidal direction and magnetic field compression exerts a radial J × B force and generates a bi-directional radial E{sub toroidal}×B{sub poloidal} pinch flow to bring oppositely directed field lines closer together to reconnect. At sufficiently low magnetic diffusivity (high Lundquist number), and with a sufficiently narrow injector flux footprint width, the oppositely directed field lines have sufficient time to reconnect (before dissipating), leading to the formation of closed flux surfaces. The reconnection process is shown to have transient Sweet-Parker characteristics.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2013

Transient Rayleigh scattering from single semiconductor nanowires

Transient Rayleigh scattering spectroscopy is a new pump-probe technique to study the dynamics and cooling of photo-excited carriers in single semiconductor nanowires. By studying the evolution of the transient Rayleigh spectrum in time after excitation, one can measure the time evolution of the density and temperature of photo-excited electron-hole plasma (EHP) as they equilibrate with lattice. This provides detailed information of dynamics and cooling of carriers including linear and bimolecular recombination properties, carrier transport characteristics, and the energy-loss rate of hot electron-hole plasma through the emission of LO and acoustic phonons.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2014

Transient and persistent current induced conductivity changes in GaAs/AlGaAs high-electron-mobility transistors

We report the observation of a current induced change of the low temperature conductivity of two-dimensional electron gases in GaAs/AlGaAs-high-electron-mobility transistors. By applying voltage pulses on the ohmic contacts of a Hall bar-mesa-structure, both sheet-carrier-density n{sub 2D} and electron mobility μ are decreased. At temperatures below 50 K, a persistent change combined with a partial transient recovery of n{sub 2D} has been observed. The transient behaviour and the lateral spreading of the effect are studied. Moreover, a temperature dependent investigation has been done in order to get insight into the addressed defect energy levels. A model based on the phenomenology of the effect is proposed. The observed effect is not a permanent degradation as the original carrier concentration can be restored by warming up the sample to room temperature and recooling it.

36 MATERIALS SCIENCE↗
DOE OSTI2014

Simultaneous investigation of ultrafast structural dynamics and transient electric field by sub-picosecond electron pulses

The ultrafast structure dynamics and surface transient electric field, which are concurrently induced by laser excited electrons of an aluminum nanofilm, have been investigated simultaneously by the same transmission electron diffraction patterns. These two processes are found to be significantly different and distinguishable by tracing the time dependent changes of electron diffraction and deflection angles, respectively. This study also provides a practical means to evaluate simultaneously the effect of transient electric field during the study of structural dynamics under low pump fluence by transmission ultrafast electron diffraction.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2014

Dynamics of the time-resolved stimulated Raman scattering spectrum in presence of transient vibronic inversion of population on the example of optically excited trans-β-apo-8{sup ′}-carotenal

We have studied the effect of transient vibrational inversion of population in trans-β-apo-8{sup ′}-carotenal on the time-resolved femtosecond stimulated Raman scattering (TR-FSRS) signal. The experimental data are interpreted by applying a quantum mechanical approach, using the formalism of projection operators for constructing the theoretical model of TR-FSRS. Within this theoretical frame we explain the presence of transient Raman losses on the Stokes side of the TR-FSRS spectrum as the effect of vibrational inversion of population. In view of the obtained experimental and theoretical results, we conclude that the excited S{sub 2} electronic level of trans-β-apo-8{sup ′}-carotenal relaxes towards the S{sub 0} ground state through a set of four vibrational sublevels of S{sub 1} state.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2014

Radiation effects on bifurcation and dual solutions in transient natural convection in a horizontal annulus

Transitions and bifurcations of transient natural convection in a horizontal annulus with radiatively participating medium are numerically investigated using the coupled lattice Boltzmann and direct collocation meshless (LB-DCM) method. As a hybrid approach based on a common multi-scale Boltzmann-type model, the LB-DCM scheme is easy to implement and has an excellent flexibility in dealing with the irregular geometries. Separate particle distribution functions in the LBM are used to calculate the density field, the velocity field and the thermal field. In the radiatively participating medium, the contribution of thermal radiation to natural convection must be taken into account, and it is considered as a radiative term in the energy equation that is solved by the meshless method with moving least-squares (MLS) approximation. The occurrence of various instabilities and bifurcative phenomena is analyzed for different Rayleigh number Ra and Prandtl number Pr with and without radiation. Then, bifurcation diagrams and dual solutions are presented for relevant radiative parameters, such as convection-radiation parameter Rc and optical thickness τ. Numerical results show that the presence of volumetric radiation changes the static temperature gradient of the fluid, and generally results in an increase in the flow critical value. Besides, the existence and development of dual solutions of transient convection in the presence of radiation are greatly affected by radiative parameters. Finally, the advantage of LB-DCM combination is discussed, and the potential benefits of applying the LB-DCM method to multi-field coupling problems are demonstrated.

42 ENGINEERING↗
DOE OSTI2021

Mapping wave packet bifurcation at a conical intersection in CH 3 I by attosecond XUV transient absorption spectroscopy

Extreme ultraviolet (XUV) transient absorption spectroscopy has emerged as a sensitive tool for mapping the real-time structural and electronic evolution of molecules. Here, attosecond XUV transient absorption is used to track dynamics in the A-band of methyl iodide (CH 3 I). Gaseous CH 3 I molecules are excited to the A-band by a UV pump (277 nm, ~20 fs) and probed by attosecond XUV pulses targeting iodine I(4d) core-to-valence transitions. Owing to the excellent temporal resolution of the technique, passage through a conical intersection is mapped through spectral signatures of nonadiabatic wave packet bifurcation observed to occur at 15 ± 4 fs following UV photoexcitation. The observed XUV signatures and time dynamics are in agreement with previous simulations [H. Wang, M. Odelius, and D. Prendergast, J. Chem. Phys. 151, 124106 (2019)]. Furthermore, due to the short duration of the UV pump pulse, coherent vibrational motion in the CH 3 I ground state along the C-I stretch mode (538 ± 7 cm -1 ) launched by resonant impulsive stimulated Raman scattering and dynamics in multiphoton excited states of CH 3 I are also detected.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Perturbative theoretical model of electronic transient circular dichroism spectroscopy of molecular aggregates

A chiral analog of transient absorption spectroscopy, transient circular dichroism (TCD) spectroscopy is an emerging time-resolved method. Both spectroscopic methods can probe the electronic transitions of a sample, and TCD is additionally sensitive to the dynamic aspects of chirality, such as those induced by molecular excitons. Here, we develop a theoretical description of TCD for electronic multi-level models in which the pump pulse is linearly polarized and probe pulse is alternately left- and right-circularly polarized. We derive effective response functions analogous to those often used to describe other four-wave mixing methods and then simulate and analyze TCD spectra for three representative multi-level electronic model systems. We elaborate on the presence and detection of the spectral signatures of electronic coherences.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2023

Efficiency of charge transfer in changing the dissociation dynamics of OD + transients formed after the photo-fragmentation of D 2 O

Here, we present an investigation of the relaxation dynamics of deuterated water molecules after direct photo-double ionization at 61 eV. We focus on the very rare D + + O + + D reaction channel in which the sequential fragmentation mechanisms were found to dominate the dynamics. Aided by theory, the state-selective formation and breakup of the transient OD + (a 1 Δ, b 1 Σ + ) is traced, and the most likely dissociation path—OD + : a 1 Δ or b 1 Σ + → A 3 Π → X 3 Σ – → B 3 Σ – —involving a combination of spin–orbit and non-adiabatic charge transfer transitions is determined. The multi-step transition probability of this complex transition sequence in the intermediate fragment ion is directly evaluated as a function of the energy of the transient OD + above its lowest dissociation limit from the measured ratio of the D + + O + + D and competing D + + D + + O sequential fragmentation channels, which are measured simultaneously. Our coupled-channel time-dependent dynamics calculations reproduce the general trends of these multi-state relative transition rates toward the three-body fragmentation channels.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2014

Theoretical study of collinear optical frequency comb generation under multi-wave, transient stimulated Raman scattering in crystals

Using mathematical modelling we have studied the conditions of low-threshold collinear optical frequency comb generation under transient (picosecond) stimulated Raman scattering (SRS) and parametric four-wave coupling of SRS components in crystals. It is shown that Raman-parametric generation of an octave-spanning optical frequency comb occurs most effectively under intermediate, transient SRS at a pump pulse duration exceeding the dephasing time by five-to-twenty times. We have found the optimal values of not only the laser pump pulse duration, but also of the Raman crystal lengths corresponding to highly efficient generation of an optical frequency comb from the second anti-Stokes to the fourth Stokes Raman components. For the KGd(WO{sub 4}){sub 2} (high dispersion) and Ba(NO{sub 3}){sub 2} (low dispersion) crystals pumped at a wavelength of 1.064 μm and a pulse duration five or more times greater than the dephasing time, the optimum length of the crystal was 0.3 and 0.6 cm, respectively, which is consistent with the condition of the most effective Stokes – anti-Stokes coupling ΔkL ≈ 15, where Δk is the wave detuning from phase matching of Stokes – anti-Stokes coupling, determined by the refractive index dispersion of the SRS medium. (nonlinear optical phenomena)

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Restart of the Transient Reactor Test (TREAT) Facility Neutron Radiography Program

The TREAT radiography system is used to perform neutron radiography of fuels, experiments, and other specimens before and after irradiation within the TREAT reactor. The TREAT neutron radiography facility performed approximately 5,000 radiographs by the spring of 1977. Originally built in 1958, the TREAT Facility was in operation until it was placed in a shutdown status in 1994. Following the Fukishima disaster and seeing a need for enhanced accident tolerant fuels, the United Stated Department of Energy decided to restart the TREAT facility and resume transient operations. In November 2017, the TREAT reactor was successfully restarted and is currently performing operational testing in preparation for initial experiment irradiations and transient testing. This paper discusses efforts to reactivate the TREAT neutron radiography facility. To characterize the neutron beam, gold foil activation measurements were made to determine an average neutron flux and flux profile. An open beam image provides the information about variations in the beam profile. In conclusion, a series of system qualification radiographs have been acquired to determine the effective image acquisition parameters, resulting image quality, and the relationships between the two.

36 MATERIALS SCIENCE↗
DOE OSTI2013

A SEARCH FOR RAPIDLY SPINNING PULSARS AND FAST TRANSIENTS IN UNIDENTIFIED RADIO SOURCES WITH THE NRAO 43 METER TELESCOPE

We have searched 75 unidentified radio sources selected from the NRAO VLA Sky Survey catalog for the presence of rapidly spinning pulsars and short, dispersed radio bursts. The sources are radio bright, have no identifications or optical source coincidences, are more than 5% linearly polarized, and are spatially unresolved in the catalog. If these sources are fast-spinning pulsars (e.g., sub-millisecond pulsars), previous large-scale pulsar surveys may have missed detection due to instrumental and computational limitations, eclipsing effects, or diffractive scintillation. The discovery of a sub-millisecond pulsar would significantly constrain the neutron star equation of state and would have implications for models predicting a rapid slowdown of highly recycled X-ray pulsars to millisecond periods from, e.g., accretion disk decoupling. These same sources were previously searched unsuccessfully for pulsations at 610 MHz with the Lovell Telescope at Jodrell Bank. This new search was conducted at a different epoch with a new 800 MHz backend on the NRAO 43 m Telescope at a center frequency of 1200 MHz. Our search was sensitive to sub-millisecond pulsars in highly accelerated binary systems and to short transient pulses. No periodic or transient signals were detected from any of the target sources. We conclude that diffractive scintillation, dispersive smearing, and binary acceleration are unlikely to have prevented detection of the large majority of the sources if they are pulsars, though we cannot rule out eclipsing, nulling or intermittent emission, or radio interference as possible factors for some non-detections. Other (speculative) possibilities for what these sources might include radio-emitting magnetic cataclysmic variables or older pulsars with aligned magnetic and spin axes.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2013

ASTROPULSE: A SEARCH FOR MICROSECOND TRANSIENT RADIO SIGNALS USING DISTRIBUTED COMPUTING. I. METHODOLOGY

We are performing a transient, microsecond timescale radio sky survey, called 'Astropulse', using the Arecibo telescope. Astropulse searches for brief (0.4 {mu}s to 204.8 {mu}s ), wideband (relative to its 2.5 MHz bandwidth) radio pulses centered at 1420 MHz. Astropulse is a commensal (piggyback) survey, and scans the sky between declinations of -1. Degree-Sign 33 and 38. Degree-Sign 03. We obtained 1540 hr of data in each of seven beams of the ALFA receiver, with two polarizations per beam. The data are one-bit complex sampled at the Nyquist limit of 0.4 {mu}s per sample. Examination of timescales on the order of microseconds is possible because we used coherent dedispersion, a technique that has frequently been used for targeted observations, but has never been associated with a radio sky survey. The more usual technique, incoherent dedispersion, cannot resolve signals below a minimum timescale which depends on the signal's dispersion measure (DM) and frequency. However, coherent dedispersion requires more intensive computation than incoherent dedispersion. The required processing power was provided by BOINC, the Berkeley Open Infrastructure for Network Computing. BOINC is a distributed computing system, allowing us to utilize hundreds of thousands of volunteers' computers to perform the necessary calculations for coherent dedispersion. Astrophysical events that might produce brief radio pulses include giant pulses from pulsars, rotating radio transients, exploding primordial black holes, or new sources yet to be imagined. Radio frequency interference and noise contaminate the data; these are mitigated by a number of techniques including multi-polarization correlation, DM repetition detection, and frequency profiling.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2013

MULTIWAVELENGTH OBSERVATIONS OF THE BLACK HOLE TRANSIENT XTE J1752-223 DURING ITS 2010 OUTBURST DECAY

Galactic black hole transients show many interesting phenomena during outburst decays. We present simultaneous X-ray (RXTE, Swift, and INTEGRAL), and optical/near-infrared (O/NIR) observations (SMARTS) of the X-ray transient XTE J1752-223 during its outburst decay in 2010. The multiwavelength observations over 150 days in 2010 cover the transition from soft to hard spectral state. We discuss the evolution of radio emission with respect to the O/NIR light curve which shows several flares. One of those flares is bright and long, starting about 60 days after the transition in X-ray timing properties. During this flare, the radio spectral index becomes harder. Other smaller flares occur along with the X-ray timing transition, and also right after the detection of the radio core. We discuss the significances of these flares. Furthermore, using the simultaneous broadband X-ray spectra including INTEGRAL, we find that a high energy cut-off with a folding energy near 250 keV is necessary around the time that the compact jet is forming. The broadband spectrum can be fitted equally well with a Comptonization model. In addition, using photoelectric absorption edges in the XMM-Newton Reflection Grating Spectrometer X-ray spectra and the extinction of red clump giants in the direction of the source, we find a lower limit on the distance of >5 kpc.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2013

THE SECOND ULTRALUMINOUS X-RAY SOURCE TRANSIENT IN M31: CHANDRA, HUBBLE SPACE TELESCOPE, AND XMM OBSERVATIONS, AND EVIDENCE FOR AN EXTENDED CORONA

XMMU J004243.6+412519 is a transient X-ray source in M31, first discovered 2012 January 15. Different approaches to fitting the brightest follow-up observation gave luminosities 1.3-2.5 Multiplication-Sign 10{sup 39} erg s{sup -1}, making it the second ultraluminous X-ray source (ULX) in M31, with a probable black hole accretor. These different models represent different scenarios for the corona: optically thick and compact, or optically thin and extended. We obtained Chandra ACIS and Hubble Space Telescope Advanced Camera for Surveys observations of this object as part of our transient monitoring program, and also observed it serendipitously in a 120 ks XMM-Newton observation. We identify an optical counterpart at J2000 position 00:42:43.70 +41:25:18.54; its F435W ({approx}B band) magnitude was 25.97 {+-} 0.03 in the 2012 March 7 observation, and >28.4 at the 4{sigma} level during the 2012 September 7 observation, indicating a low-mass donor. We created two alternative light curves, using the different corona scenarios, finding linear decay for the compact corona and exponential decay for the extended corona; linear decay implies a disk that is >5 mag brighter than we observed. We therefore favor the extended corona scenario, but caution that there is no statistical preference for this model in the X-ray spectra alone. Using two empirical relations between the X-ray to optical ratio and the orbital period, we estimate a period of {approx}9-30 hr; this period is consistent with that of the first ULX in M31 (18{sup +5}{sub -6} hr)

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2013

Case study of a magnetic transient in NOAA 11429 observed by SDO/HMI during the M7.9 flare on 2012 march 13

NOAA 11429 was the source of an M7.9 X-ray flare at the western solar limb (N18° W63°) on 2012 March 13 at 17:12 UT. Observations of the line-of-sight magnetic flux and the Stokes I and V profiles from which it is derived were carried out by the Solar Dynamics Observatory Helioseismic and Magnetic Imager (SDO/HMI) with a 45 s cadence over the full disk, at a spatial sampling of 0.''5. During flare onset, a transient patch of negative flux can be observed in SDO/HMI magnetograms to rapidly appear within the positive polarity penumbra of NOAA 11429. We present here a detailed study of this magnetic transient and offer interpretations as to whether this highly debated phenomenon represents a 'real' change in the structure of the magnetic field at the site of the flare, or is instead a product of instrumental/algorithmic artifacts related to particular SDO/HMI data reduction techniques.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2013

Discovery of a new kind of explosive X-ray transient near M86

We present the discovery of a new type of explosive X-ray flash in Chandra images of the old elliptical galaxy M86. This unique event is characterized by the peak luminosity of 6 × 10{sup 42} erg s{sup –1} for the distance of M86, the presence of precursor events, the timescale between the precursors and the main event (∼4000 s), the absence of detectable hard X-ray and γ-ray emission, the total duration of the event, and the detection of a faint associated optical signal. The transient is located close to M86 in the Virgo cluster at the location where gas and stars are seen protruding from the galaxy probably due to an ongoing wet minor merger. We discuss the possible mechanisms for the transient and conclude that the X-ray flash could have been caused by the disruption of a compact white dwarf star by a ∼10{sup 4} M {sub ☉} black hole. Alternative scenarios such that of a foreground neutron star accreting an asteroid or the detection of an off-axis (short) γ-ray burst cannot be excluded at present.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

The ultraviolet-bright, slowly declining transient PS1-11af as a partial tidal disruption event

We present the Pan-STARRS1 discovery of the long-lived and blue transient PS1-11af, which was also detected by Galaxy Evolution Explorer with coordinated observations in the near-ultraviolet (NUV) band. PS1-11af is associated with the nucleus of an early type galaxy at redshift z = 0.4046 that exhibits no evidence for star formation or active galactic nucleus activity. Four epochs of spectroscopy reveal a pair of transient broad absorption features in the UV on otherwise featureless spectra. Despite the superficial similarity of these features to P-Cygni absorptions of supernovae (SNe), we conclude that PS1-11af is not consistent with the properties of known types of SNe. Blackbody fits to the spectral energy distribution are inconsistent with the cooling, expanding ejecta of a SN, and the velocities of the absorption features are too high to represent material in homologous expansion near a SN photosphere. However, the constant blue colors and slow evolution of the luminosity are similar to previous optically selected tidal disruption events (TDEs). The shape of the optical light curve is consistent with models for TDEs, but the minimum accreted mass necessary to power the observed luminosity is only ∼0.002 M {sub ☉}, which points to a partial disruption model. A full disruption model predicts higher bolometric luminosities, which would require most of the radiation to be emitted in a separate component at high energies where we lack observations. In addition, the observed temperature is lower than that predicted by pure accretion disk models for TDEs and requires reprocessing to a constant, lower temperature. Three deep non-detections in the radio with the Very Large Array over the first two years after the event set strict limits on the production of any relativistic outflow comparable to Swift J1644+57, even if off-axis.

79 ASTRONOMY AND ASTROPHYSICS↗