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NASA NTRS1999

Radiative Importance of Aerosol-Cloud Interaction

Aerosol particles are input into the troposphere by biomass burning, among other sources. These aerosol palls cover large expanses of the earth's surface. Aerosols may directly scatter solar radiation back to space, thus increasing the earth's albedo and act to cool the earth's surface and atmosphere. Aerosols also contribute to the earth's energy balance indirectly. Hygroscopic aerosol act as cloud condensation nuclei (CCN) and thus affects cloud properties. In 1977, Twomey theorized that additional available CCN would create smaller but more numerous cloud droplets in a cloud with a given amount of liquid water. This in turn would increase the cloud albedo which would scatter additional radiation back to space and create a similar cooling pattern as the direct aerosol effect. Estimates of the magnitude of the aerosol indirect effect on a global scale range from 0.0 to -4.8 W/sq m. Thus the indirect effect can be of comparable magnitude and opposite in sign to the estimates of global greenhouse gas forcing Aerosol-cloud interaction is not a one-way process. Just as aerosols have an influence on clouds through the cloud microphysics, clouds have an influence on aerosols. Cloud droplets are solutions of liquid water and CCN, now dissolved. When the cloud droplet evaporates it leaves behind an aerosol particle. This new particle does not have to have the same properties as the original CCN. In fact, studies show that aerosol particles that result from cloud processing are larger in size than the original CCN. Optical properties of aerosol particles are dependent on the size of the particles. Larger particles have a smaller backscattering fraction, and thus less incoming solar radiation will be backscattered to space if the aerosol particles are larger. Therefore, we see that aerosols and clouds modify each other to influence the radiative balance of the earth. Understanding and quantifying the spatial and seasonal patterns of the aerosol indirect forcing may have even greater consequences. Presently we know that through the use of fossil fuel and land-use changes we have increased the concentration of greenhouse gases in the atmosphere. In parallel, we have seen a modest increase of global temperature in the last century. These two observations have been linked as cause and effect by climate models, but this connection is still experimentally not verified. The spatial and seasonal distribution of aerosol forcing is different from that of greenhouse gases, thus generating a different spatial fingerprint of climate change. This fingerprint was suggested as a method to identify the response of the climate system to anthropogenic forcing of greenhouse gases and aerosol. The aerosol fingerprint may be the only way to firmly establish the presence (or absence) of human impact on climate. Aerosol-cloud interaction through the indirect effect will be an important component of establishing this fingerprint.

Tsay, Si-Chee↗

DOE OSTI2026

The remarkable inefficiency of stratocumulus

Marine stratocumulus clouds play a central role in Earth's climate system by reflecting incoming solar radiation and exerting a strong cooling effect. Their organization into open and closed mesoscale cellular morphologies can be thought of as an example of bistable dynamics driven by aerosol–cloud interactions and mesoscale processes. From the perspective of non-equilibrium thermodynamics, these structures are an example of a far-from-equilibrium open system that continuously produces and exports entropy. While entropy production has been studied in idealized deep convective systems, it has not yet been quantified for shallow clouds. Here, we compute and decompose the internal entropy production of open- and closed-cell stratocumulus using an ensemble of large-eddy simulations. We show that the overall entropy production of stratocumulus is low, reflecting the limited vertical extent and corresponding reduced ability to utilize the energy fluxes at the system's boundaries. Moist processes dominate the overall irreversibility, which, combined with their low entropy production, leads to a mechanical efficiency about an order of magnitude smaller than in deep convective systems. Although the dominant irreversible processes differ between open- and closed-cell regimes, the distributions of total entropy production largely overlap across the ensemble, limiting the ability to distinguish the dynamics of individual cases based solely on total entropy production.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2016

Aerosol effects on the anvil characteristics of mesoscale convective systems

Abstract Simulations of two mesoscale convective systems (MCSs) that occurred during the Midlatitude Continental Convective Clouds Experiment were performed to examine the impact of aerosol number concentration on the vertical distributions of liquid and ice condensate and the macrophysical, microphysical, and radiative properties of the cirrus‐anvil cloud shield. Analyses indicate that for an increase in aerosol concentration from a clean continental to a highly polluted state, there was an increase in the rime collection rate of cloud water, which led to less lofted cloud water. Aerosol‐induced trends in the cloud mixing ratio profiles were, however, nonmonotonic in the mixed phase region, such that a moderate increase in aerosol concentration produced the greatest reduction in cloud water. Generally, less lofted cloud water led to less anvil ice mixing ratio but more numerous, small ice crystals within the anvil. In spite of reduced anvil ice mixing ratio, the anvil clouds exhibited greater areal coverage, increased albedo, reduced cloud top cooling, and reduced net radiative flux, which led to an aerosol‐induced warming (reduced cooling) effect in these squall lines.

Saleeby, S. M.↗

DOE OSTI2022

Charge carrier motion and effect of fixed oxide charge in a microstructured silicon radiation detector

Signal formation in a microstructured semiconductor neutron detector is more complex than in planar diode geometry. Three-dimensional microstructures are laterally smaller than the ionization cloud length, and the electric fields may be weak enough to exhibit plasma time effects. This work is the first detailed treatment of charge carrier motion in these complex semiconductor devices to replicate the time profile and signal magnitude. Simulations were performed using COMSOL Multiphysics to investigate various parameters that affect the propagation of the charge cloud. It was observed that the size of the simulated three-dimensional structure had an impact on the induced current pulse, indicating the importance of simulation geometry optimization to accurately simulate charge cloud expansion. COMSOL Multiphysics was used to replicate accurate charge creation profiles using energy deposition information imported from radiation transport codes. A detailed simulation methodology is presented to benchmark preamplifier event pulses along with complexities in modeling the charge carrier motion along the etched microstructured trenches with Si–SiO 2 boundary conditions, including fixed oxide charge and interface trapping.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2013

Effects of external radiation fields on line emission—application to star-forming regions

A variety of astronomical environments contain clouds irradiated by a combination of isotropic and beamed radiation fields. For example, molecular clouds may be irradiated by the isotropic cosmic microwave background, as well as by a nearby active galactic nucleus. These radiation fields excite atoms and molecules and produce emission in different ways. We revisit the escape probability theorem and derive a novel expression that accounts for the presence of external radiation fields. We show that when the field is isotropic the escape probability is reduced relative to that in the absence of external radiation. This is in agreement with previous results obtained under ad hoc assumptions or with the two-level system, but can be applied to complex many-level models of atoms or molecules. This treatment is in the development version of the spectral synthesis code CLOUDY. We examine the spectrum of a Spitzer cloud embedded in the local interstellar radiation field and show that about 60% of its emission lines are sensitive to background subtraction. We argue that this geometric approach could provide an additional tool toward understanding the complex radiation fields of starburst galaxies.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2024

Aerosol-induced closure of marine cloud cells: enhanced effects in the presence of precipitation

Abstract. The Weather Research Forecasting (WRF) version 4.3 model is configured within a Lagrangian framework to quantify the impact of aerosols on evolving cloud fields. Kilometer-scale simulations utilizing meteorological boundary conditions are based on 10 case study days offering diverse meteorology during the Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA). Measurements from aircraft, the ground-based Atmosphere Radiation Measurement (ARM) site at Graciosa Island in the Azores, and A-Train and geostationary satellites are utilized for validation, demonstrating good agreement with the WRF-simulated cloud and aerosol properties. Higher aerosol concentration leads to suppressed drizzle and increased cloud water content in all case study days. These changes lead to larger radiative cooling rates at cloud top, enhanced vertical velocity variance, and increased vertical and horizontal wind speed near the base of the lower-tropospheric inversion. As a result, marine cloud cell area expands, narrowing the gap between shallow clouds and increasing cloud optical thickness, liquid water content, and the top-of-atmosphere outgoing shortwave flux. While similar aerosol effects are observed in lightly to non-raining clouds, they tend to be smaller by comparison. These simulations show a relationship between cloud cell area expansion and the radiative adjustments caused by liquid water path and cloud fraction changes. The adjustments are positive and scale as 74 % and 51 %, respectively, relative to the Twomey effect. While higher-resolution large-eddy simulations may provide improved representation of cloud-top mixing processes, these results emphasize the importance of addressing mesoscale cloud-state transitions in the quantification of aerosol radiative forcing that cannot be attained from traditional climate models.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2005

Spatial and Temporal Distribution of Tropospheric Clouds Observed by MODIS Onboard the Terra and Aqua Satellites

The Moderate Resolution Imaging Spectroradiometer (MODIS) was developed by NASA and launched onboard the Terra spacecraft on December 18,1999 and Aqua spacecraft on May 4, 2002. It achieved its final orbit and began Earth observations on February 24, 2000 for Terra and June 24, 2002 for Aqua. A comprehensive set of remote sensing algorithms for cloud masking and the retrieval of cloud physical and optical properties has been developed by members of the MODIS atmosphere science team. The archived products from these algorithms have applications in climate change studies, climate modeling, numerical weather prediction, as well as fundamental atmospheric research. In addition to an extensive cloud mask, products include cloud-top properties (temperature, pressure, effective emissivity), cloud thermodynamic phase, cloud optical and microphysical parameters (optical thickness, effective particle radius, water path), as well as derived statistics. We will describe the various cloud properties being analyzed on a global basis from both Terra and Aqua. These include the latitudinal distribution of cloud optical and radiative properties of both liquid water and ice clouds, as well as joint histograms of cloud optical thickness and effective radius for selected geographical locations around the world.

King, Michael D.↗

NASA NTRS2005

Spatial and Temporal Distribution of Tropospheric Clouds Observed by MODIS Onboard the Terra and Aqua Satellites

The Moderate Resolution Imaging Spectroradiometer (MODIS) was developed by NASA and launched onboard the Terra spacecraft on December 18, 1999 and Aqua spacecraft on May 4, 2002. It achieved its final orbit and began Earth observations on February 24, 2000 for Terra and June 24, 2002 for Aqua. A comprehensive set of remote sensing algorithms for cloud masking and the retrieval of cloud physical and optical properties has been developed by members of the MODIS atmosphere science team. The archived products from these algorithms have applications in climate change studies, climate modeling, numerical weather prediction, as well as fundamental atmospheric research. In addition to an extensive cloud mask, products include cloud-top properties (temperature, pressure, effective emissivity), cloud thermodynamic phase, cloud optical and microphysical parameters (optical thickness, effective particle radius, water path), as well as derived statistics. We will describe the various cloud properties being analyzed on a global basis from both Terra and Aqua. These include the latitudinal distribution of cloud optical and radiative properties of both liquid water and ice clouds, as well as joint histograms of cloud optical thickness and effective radius for selected geographical locations around the world.

King, Michael D.↗

NASA NTRS1992

Lidar Studies of Extinction in Clouds in the ECLIPS Project

The Experimental Cloud Lidar Pilot Study (ECLIPS) project has now had two active phases in 1989 and 1991. A number of laboratories around the world have taken part in the study. The observations have yielded new data on cloud height and structure, and have yielded some useful new information on the retrieval of cloud optical properties, together with the uncertainties involved. Clouds have a major impact on the climate of the earth. They have the effect of reducing the mean surface temperature from 30 C for a cloudless planet to a value of about 15 C for present cloud conditions. However, it is not at all certain how clouds would react to a change in the planetary temperature in the event of climate change due to a radiative forcing from greenhouse gases. Clouds both reflect out sunlight (negative feedback) and enhance the greenhouse effect (positive feedback), but the ultimate sign of cloud feedback is unknown. Because of these uncertainties, campaigns to study clouds intensely were initiated. The International Satellite Cloud Climatology (ISCPP) and the FIRE Campaigns (cirrus and stratocumulus) are examples. The ECLIPS was set up similarly to the above experiments to obtain information specifically on cloud base, but also cloud top (where possible), optical properties, and cloud structure. ECLIPS was designed to allow as many laboratories as possible globally to take part to get the largest range of clouds. It involves observations with elastic backscatter lidar, supported by infrared fluxes at the ground and radiosonde data, as basic instrumentation. More complex experiments using beam filter radiometers, solar pyranometers, and satellite data and often associated with other campaigns were also encouraged to join ECLIPS. Two periods for observation were chosen, Sep. - Dec. 1989 and Apr. - Jul. 1992 into which investigators were requested to fit 30 days of observations. These would be either continuous, or arranged to coincide with NOAA satellite overpasses to obtain AVHRR data. The distribution of the ECLIPS international effort as in 1991 is shown. The main gaps in the global distribution are in the tropics and the Southern Hemisphere.

Martin, C.↗

DOE OSTI2013

ON THE EFFECTS OF OPTICALLY THICK GAS (DISKS) AROUND MASSIVE STARS

Numerical simulations have shown that the often cited radiation pressure barrier to accretion onto massive stars can be circumvented, when the radiation field is highly anisotropic in the presence of a circumstellar accretion disk with high optical depth. Here, these studies of the so-called flashlight effect are expanded by including the opacity of the innermost dust-free but potentially optically thick gas regions around forming massive stars. In addition to frequency-dependent opacities for the dust grains, we use temperature- and density-dependent Planck and Rosseland mean opacities for the gas. The simulations show that the innermost dust-free parts of the accretion disks are optically thick to the stellar radiation over a substantial fraction of the solid angle above and below the disk's midplane. The temperature in the shielded disk region decreases faster with radius than in a comparison simulation with a lower constant gas opacity, and the dust sublimation front is shifted to smaller radii. The shielding by the dust-free gas in the inner disk thus contributes to an enhanced flashlight effect, which ultimately results in a smaller opening angle of the radiation pressure driven outflow and in a much longer timescale of sustained feeding of the circumstellar disk by the molecular cloud core. We conclude that it is necessary to properly account for the opacity of the inner dust-free disk regions around forming massive stars in order to correctly assess the effectiveness of the flashlight effect, the opening angle of radiation pressure driven outflows, and the lifetime and morphological evolution of the accretion disk.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2013

Study of Mechanisms of Aerosol Indirect Effects on Glaciated Clouds: Progress during the Project (Final Technical Report)

This 3-year project has studied how aerosol pollution influences glaciated clouds. The tool applied has been an 'aerosol-cloud model'. It is a type of Cloud-System Resolving Model (CSRM) modified to include 2-moment bulk microphysics and 7 aerosol species, as described by Phillips et al. (2009, 2013). The study has been done by, first, improving the model and then performing sensitivity studies with validated simulations of a couple of observed cases from ARM. These are namely the Tropical Warm Pool International Cloud Experiment (TWP-ICE) over the tropical west Pacific and the Cloud and Land Surface Interaction Campaign (CLASIC) over Oklahoma. During the project, sensitivity tests with the model showed that in continental clouds, extra liquid aerosols (soluble aerosol material) from pollution inhibited warm rain processes for precipitation production. This promoted homogeneous freezing of cloud droplets and aerosols. Mass and number concentrations of cloud-ice particles were boosted. The mean sizes of cloud-ice particles were reduced by the pollution. Hence, the lifetime of glaciated clouds, especially ice-only clouds, was augmented due to inhibition of sedimentation and ice-ice aggregation. Latent heat released from extra homogeneous freezing invigorated convective updrafts, and raised their maximum cloud-tops, when aerosol pollution was included. In the particular cases simulated in the project, the aerosol indirect effect of glaciated clouds was twice than of (warm) water clouds. This was because glaciated clouds are higher in the troposphere than water clouds and have the first interaction with incoming solar radiation. Ice-only clouds caused solar cooling by becoming more extensive as a result of aerosol pollution. This 'lifetime indirect effect' of ice-only clouds was due to higher numbers of homogeneously nucleated ice crystals causing a reduction in their mean size, slowing the ice-crystal process of snow production and slowing sedimentation. In addition to the known indirect effects (glaciation, riming and thermodynamic), new indirect effects were discovered and quantified due to responses of sedimentation, aggregation and coalescence in glaciated clouds to changing aerosol conditions. In summary, the change in horizontal extent of the glaciated clouds ('lifetime indirect effects'), especially of ice-only clouds, was seen to be of higher importance in regulating aerosol indirect effects than changes in cloud properties ('cloud albedo indirect effects').

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2013

Study of Mechanisms of Aerosol Indirect Effects on Glaciated Clouds: Progress during the Project (Final Technical Report)

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2016

Cirrus Heterogeneity Effects on Cloud Optical Properties Retrieved with an Optimal Estimation Method from MODIS VIS to TIR Channels.

This study presents preliminary results on the effect of cirrus heterogeneities on top-of-atmosphere (TOA) simulated radiances or reflectances for MODIS channels centered at 0.86, 2.21, 8.56, 11.01 and 12.03 micrometers , and on cloud optical properties retrieved with a research-level optimal estimation method (OEM). Synthetic cirrus cloud fields are generated using a 3D cloud generator (3DCLOUD) and radiances/reflectances are simulated using a 3D radiative transfer code (3DMCPOL). We find significant differences between the heterogeneity effects on either visible and near-infrared (VNIR) or thermal infrared (TIR) radiances. However, when both wavelength ranges are combined, heterogeneity effects are dominated by the VNIR horizontal radiative transport effect. As a result, small optical thicknesses are overestimated and large ones are underestimated. Retrieved effective diameter are found to be slightly affected, contrarily to retrievals using TIR channels only.

MODIS↗

NASA NTRS1989

Consequences of a conductive boundary on the local cloud. I - No dust

Using boundary conditions appropriate to the Local Cloud embedded in the Local Bubble, the evaporation of the cloud is modeled assuming steady flow. Included in the model are the effects of radiative cooling and nonequilibrium ionization structure in the interface, and pressure support and heat conduction inhibition due to the magnetic field. The soft X-ray and EUV emission from the interface are calculated and compared with observations. It is found that the emission in the softest X-ray band, the Be band, is harder than that calculated for an equilibrium, normal abundance, 10 to the 6th K plasma. Column densities of C IV, N V, O VI, Si IV, and Si III in the interface are calculated. The column density for O VI is found to be very close to observed values for nearby stars, while all others are too small to contribute significantly to observed values. The ionization of the Local Cloud due to radiation from the interface is calculated. It is found that a significant amount of ionizing radiation is produced, dominating all other known sources. The hardness of the emission, however, results in ionization of helium as well as hydrogen. Thus, the type of boundary modeled cannot explain the ionization of the very local interstellar medium inferred from solar backscatter measurements.

Slavin, Jonathan D.↗

DOE OSTI2026

Final report: Insights from ARM observations into aerosol processing and transport by extratropical cyclones and aerosol effects on cyclone clouds

This project advanced understanding of aerosol–cloud interactions in extratropical cyclones using observations from the Atmospheric Radiation Measurement (ARM) Eastern North Atlantic (ENA) observatory and ACE-ENA field campaigns, along with satellite datasets and numerical modeling. We have quantified the susceptibility of frontal clouds to aerosols, showing that this susceptibility is similar to that in non-frontal clouds despite substantial (factor 2) differences in droplet concentrations between these cloud types, and also significant differences in cloud albedo. A key finding was that Aitken-mode (here, 60-100nm diameter) aerosols play a disproportionately important role in droplet activation in frontal clouds, and concentrations of these particles are frequently strongly biased in climate models. Activation of aerosols depends strongly on updraft speeds, and via collaboration with Argonne National Laboratory we contributed to quantifying these better with the ARM radar wind profiler at the ENA site. Our studies in the North Atlantic have analogs in the Southern Ocean, and to draw these out we examined data from the MARCUS and SOCRATES field campaigns. We identified new particle formation within extratropical cyclones as a potentially important source of cloud condensation nuclei in these pristine marine environments. By combining ARM observations with perturbed parameter ensemble simulations, we demonstrated that surface observations can effectively constrain aerosol–cloud adjustments and reduce uncertainty in simulated cloud liquid water path responses by approximately 15%, yielding stronger constraints on historical aerosol cooling effects. The work further established precipitation processes as a dominant control on aerosol–cloud interactions and Earth system predictability.

Gordon, Hamish [Department of Chemical Engineering↗

DOE OSTI2026

Atmospheric Composition and Radiative Forcing Effects due to UN International Ship Emissions Regulations (ACRUISE) Field Campaign Report

Aerosols, or atmospheric particulates, are long known to be able to seed clouds and modify their characteristics (e.g., cloud brightness, coverage, lifetime). However, the impact of aerosols on clouds is highly complex and non-linear. As a result, aerosol-cloud interaction remains the largest uncertainty in our understanding of the Earth’s radiative balance and in any future climate projections. Aerosols are also a principal component of air pollution and are known to adversely affect respiratory and cardiovascular health.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2016

Fingerprints of a riming event on cloud radar Doppler spectra: observations and modeling

In this paper, Radar Doppler spectra measurements are exploited to study a riming event when precipitating ice from a seeder cloud sediment through a supercooled liquid water (SLW) layer. The focus is on the "golden sample" case study for this type of analysis based on observations collected during the deployment of the Atmospheric Radiation Measurement Program's (ARM) mobile facility AMF2 at Hyytiälä, Finland, during the Biogenic Aerosols – Effects on Clouds and Climate (BAECC) field campaign. The presented analysis of the height evolution of the radar Doppler spectra is a state-of-the-art retrieval with profiling cloud radars in SLW layers beyond the traditional use of spectral moments. Dynamical effects are considered by following the particle population evolution along slanted tracks that are caused by horizontal advection of the cloud under wind shear conditions. In the SLW layer, the identified liquid peak is used as an air motion tracer to correct the Doppler spectra for vertical air motion and the ice peak is used to study the radar profiles of rimed particles. A 1-D steady-state bin microphysical model is constrained using the SLW and air motion profiles and cloud top radar observations. The observed radar moment profiles of the rimed snow can be simulated reasonably well by the model, but not without making several assumptions about the ice particle concentration and the relative role of deposition and aggregation. In conclusion, this suggests that in situ observations of key ice properties are needed to complement the profiling radar observations before process-oriented studies can effectively evaluate ice microphysical parameterizations.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS2010

Multiyear Statistics of 2-D Shortwave Radiative Effects at Three ARM Sites

This study examines the importance of horizontal photon transport effects, which are not considered in the 1-D calculations of solar radiative heating used by most atmospheric dynamical models. In particular, the paper analyzes the difference between 2-D and 1-D radiative calculations for 2-D vertical cross-sections of clouds that were observed at three sites over 2- to 3-year periods. The results show that 2-D effects increase multiyear 24-hour average total solar absorption by about 4.1 W/sq m, 1.2 W/sq m, and 0.3 W/sq m at a tropical, mid-latitude, and arctic site, respectively. However, 2-D effects are often much larger than these average values, especially for high sun and for convective clouds. The results also reveal a somewhat unexpected behavior, that horizontal photon transport often enhances solar heating even for oblique sun. These findings underscore the need for fast radiation calculation methods that can allow atmospheric dynamical simulations to consider the inherently multidimensional nature of shortwave radiative processes.

Varnai, Tamas↗