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At least 991 records · Page 55

Multi-GeV FFA beam transport test at CEBAF

Jefferson National Lab plans an upgrade project to reach 22 GeV high polarization electron beam by using Fixed Field Alternating-gradient (FFA) magnets. The utilization of the FFA magnets for 10-22 GeV beam energy range is unexampled, therefore those magnets need an experimental validation before their full installation to form an arc in the Continuous Electron Beam Accelerator Facility (CEBAF). For this reason, JLAB is also considering the design of an FFA magnet test bench, i.e. a half or full FFA cell, that would be deployed in the current CEBAF in order to serve as the highest energy demonstration for the FFA field uniformity, permanent magnet resiliency with the beam as well as enabling beam optics measurements with the 5-11 GeV range highly polarized beams which closely resembles the full energy range of the 22 GeV upgrade. In this report, we present the status of the planned beamline for the FFA beam transport test at CEBAF.

Accelerator Physics↗

High power beta electron device - Beyond betavoltaics

Developing watt level power sources with beta emitting radioisotopes has been limited by the inability to utilize high energy (> 100 KeV) beta emitters at high radioisotope loadings without damaging the energy conversion materials. A new type of beta electron power source is described that removes those restrictions. This approach contains the radioisotope in a beta transparent titanium tube and confines beta electrons emitted through the tube wall to spiral trajectories around the tube with an axial magnetic field. The confined beta electrons dissipate energy though multiple interactions with surrounding excimer precursor gas atoms to efficiently generate photons. Photovoltaic cells convert the photons to electrical power. Since the beta electrons dissipate energy in the excimer precursor gas, the device can be loaded with more than 10 13 Bq of radioisotope to generate 100 milliwatt to watt levels of electrical power without damaging the device materials or degrading its performance. Furthermore, the power source can use a variety of beta radioisotopes and scales by stacking the devices.

30 DIRECT ENERGY CONVERSION↗

Transport of 12 GeV positron beams at Ce+BAF

Jefferson Lab (JLab) is developing a concept to upgrade the Continuous Electron Beam Accelerator Facility (CEBAF) to additionally deliver spin-polarized continuous-wave positron beams for its nuclear physics program users (Ce+BAF 12 GeV). The concept involves repurposing the Low Energy Recirculator Facility (LERF) at JLab as a dual injector, first producing 100-300 MeV spin-polarized electron beams which are subsequently used for the generation and formation of 123 MeV continuous-wave positron beams. The positron beams are transported to CEBAF and injected for acceleration up to 12 GeV, tailored to the requirements of its four experimental halls. Given the higher emittance of the secondary positron beams, the CEBAF optics are optimized for low dispersion and low beta functions to enhance transmission within the Ce+BAF acceptance limits and with an R56 to manage the positron beams bunch length and energy spread. Potential bottlenecks are being investigated through both optical modeling and measurements using an electron beam, as well as degraded electron beams, to map the 6d acceptance of CEBAF as it is today. This presentation shares preliminary results from multi-particle tracking simulations of the positron beam up to 12 GeV, including spatial, momentum, and spin characteristics, and explores the feasibility of delivering beams simultaneously to multiple experimental halls via extraction optics.

Accelerator Physics↗

Light‐driven Transformation of Carbon Monoxide into Hydrocarbons using CdS@ZnS : VFe Protein Biohybrids

Enzymatic Fisher-Tropsch (FT) process catalyzed by vanadium (V)-nitrogenase can convert carbon monoxide (CO) to longer-chain hydrocarbons (>C2) under ambient conditions, although this process requires high-cost reducing agent(s) and/or the ATP-dependent reductase as electron and energy sources. Using visible light-activated CdS@ZnS (CZS) core-shell quantum dots (QDs) as alternative reducing equivalent for the catalytic component (VFe protein) of V-nitrogenase, we first report a CZS : VFe biohybrid system that enables effective photo-enzymatic C−C coupling reactions, hydrogenating CO into hydrocarbon fuels (up to C4) that can be hardly achieved with conventional inorganic photocatalysts. Surface ligand engineering optimizes molecular and opto-electronic coupling between QDs and the VFe protein, realizing high efficiency (internal quantum yield >56 %), ATP-independent, photon-to-fuel production, achieving an electron turnover number of >900, that is 72 % compared to the natural ATP-coupled transformation of CO into hydrocarbons by V-nitrogenase. The selectivity of products can be controlled by irradiation conditions, with higher photon flux favoring (longer-chain) hydrocarbon generation. The CZS : VFe biohybrids not only can find applications in industrial CO removal for high-value-added chemical production by using the cheap, renewable solar energy, but also will inspire related research interests in understanding the molecular and electronic processes in photo-biocatalytic systems.

Chemistry↗

FreeDam – A webtool for free-electron laser-induced damage in femtosecond X-ray crystallography

Over the last decade X-ray free-electron laser (XFEL) sources have been made available to the scientific community. One of the most successful uses of these new machines has been protein crystallography. When samples are exposed to the intense short X-ray pulses provided by the XFELs, the sample quickly becomes highly ionized and the atomic structure is affected. Here we present a webtool dubbed FreeDam based on non-thermal plasma simulations, for estimation of radiation damage in free-electron laser experiments in terms of ionization, temperatures and atomic displacements. The aim is to make this tool easily accessible to scientists who are planning and performing experiments at XFELs.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Chemically assisted ion beam etching of polycrystalline and (100)tungsten

A chemically assisted ion-beam etching technique is described which employs an ion beam from an electron-bombardment ion source and a directed flux of ClF3 neutrals. This technique enables the etching of tungsten foils and films in excess of 40 microns thick with good anisotropy and pattern definition over areas of 30 sq mm, and with a high degree of selectivity. (100) tungsten foils etched with this process exhibit preferred-orientation etching, while polycrystalline tungsten films exhibit high etch rates. This technique can be used to pattern the dispenser cathode surfaces serving as electron emitters in traveling-wave tubes to a controlled porosity.

Garner, Charles↗

Double core hole valence-to-core x-ray emission spectroscopy: A theoretical exploration using time-dependent density functional theory

With the help of newly developed X-ray free-electron laser (XFEL) sources, creating double core holes (DCHs) simultaneously at the same or different atomic sites in a molecule has now become possible. DCH X-ray emission is a new form of X-ray nonlinear spectroscopy that can be studied with a XFEL. Here in this paper, we computationally explore the metal K-edge valence-to-core (VtC) X-ray emission spectroscopy (XES) of metal/metal and metal/ligand DCH states in a series of transition metal complexes with time-dependent density functional theory. The simulated DCH VtC-XES signals are compared with conventional single core hole (SCH) XES signals. The energy shifts and intensity changes of the DCH emission lines with respect to the corresponding SCH-XES features are fingerprints of the coupling between the second core hole and the occupied orbitals around the DCHs that contain important chemical bonding information of the complex. The difference between delocalized/localized core hole models on DCH VtC-XES is also briefly discussed. We theoretically demonstrate that DCH XES provides subtle information on the local electronic structure around metal centers in transition metal complexes beyond conventional linear XES. In conclusion, our predicted changes from calculations between SCH-XES and DCH-XES features should be detectable with modern XFEL sources.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Design of a microbunched electron cooler energy recovery linac

Microbunched electron Cooling (MBEC), a type of Coherent electron Cooling (CeC), is a possible way to cool high energy protons; such an electron cooler can be driven by an energy recovery linac (ERL). The beam parameters of this design are based on cooling 275 and 100 GeV protons at the Electron-Ion Collider (EIC), requiring 150 and 55 MeV electrons, respectively. If implemented, a high energy cooler would serve to increase the average luminosity of the collider by mitigating the emittance growth caused by various processes. This ERL is designed to deliver a bunch charge of 1 nC, an average current of 100 mA, and strict requirements on the transverse emittance, slice energy spread, and longitudinal distribution profile. This paper covers the current state of the design.

Accelerator Physics↗

Biomonitoring of Air Pollution in Bosnia and Herzegovina Using Epiphytic Lichen Hypogymnia physodes

The aim of the study was to assess heavy metals (Cd, Cr, Cu, Fe, Mn, Ni, Pb and Zn) air pollution in Bosnia and Herzegovina by using a lichen, Hypogymnia physodes. Metal content was determined by flame atomic absorption spectrometry (FAAS) and was between very high naturality or alteration to middle naturality or alteration. Strong correlations between Cr and Ni confirmed mainly anthropogenic sources. The scanning electron microscopy and energy dispersive X-ray spectroscopy (SEM/EDS) analysis of C, O, Na, Mg, Al, Si, P, S, Cl, K, Ca, V, Co, As, Sn, Sb, Hg and Bi were performed on the lichen surface and hyphae of the transplanted samples. Despite significant damage to tissue and cell integrity, the recurrent presence of particulate matter in lichen indicates the considerable presence of dust in the urban atmosphere which, according to chemical composition, may be due to anthropogenic and natural sources such as soil.

54 ENVIRONMENTAL SCIENCES↗

Time evolution of the distribution function for stochastically heated relativistic electrons in a laser field of picosecond duration

We report a numerical analysis of the stochastic acceleration of electrons, stipulated by a random change in the phase of the force acting on the electron. The main source of randomness is the random spatial distribution of electromagnetic fields in the focal region of multimode laser radiation. A typical frequency of the random phase change corresponding to the maximum impact of the effect under consideration lies in the range of (0.25–0.5)ν (ν is the radiation frequency of a neodymium laser). A wave packet model convenient for calculations taking into account the radiative transitions of the neodymium ion is proposed. The dependence of the average energy of relativistic electrons on the flux density in the range of 10{sup 15}–10{sup 18} W cm{sup -2} is calculated. The time dependence of the average electron energy during the laser pulse in the form of approximating formulas is constructed. The typical time for the development of stochastic heating of electrons is determined. It is found that the stochastic acceleration process weakly depends on the laser pulse duration, when the latter exceeds several hundred periods of the electromagnetic wave. (interaction of laser radiation with matter. laser plasma)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Positron-electron pairs in astrophysics; Proceedings of the Workshop, Greenbelt, MD, January 6-8, 1983

Astrophysical sources of positron-electron-pair annihilation radiation are characterized in reviews and reports of observational and theoretical investigations. Topics examined include gamma-ray lines from solar flares, gamma-ray bursts, pulsars, the Galactic center, active galaxies, and physical processes in relativistic and magnetized plasmas. Spectra, historgrams, graphs, and diagrams are provided.

Burns, M. L.↗

Performance of GaAs and silicon concentrator cells under 1 MeV electron irradiation

Gallium arsenide concentrator cells from three sources and silicon concentrator cells from one source were exposed to 1 MeV electrons at fluences up to 1 x 10 to the 15th electrons per square cm. Performance data were taken after several fluences, at two temperatures (25 and 80 C), and at concentration levels from 1 to about 150X AM0. Data at one sun and 25 C were taken with an X-25 xenon lamp solar simulator. Data at concentrations were taken using a pulsed solar simulator with the assumption of a linear relationship between short-circuit current and irradiance. The cells are 5 mm x 5 mm with a 4 mm diameter illuminated area.

Curtis, H. B.↗

Correcting x ray spectra obtained from the AXAF VETA-I mirror calibration for pileup, continuum, background and deadtime

The VETA-I mirror was calibrated with the use of a collimated soft X-ray source produced by electron bombardment of various anode materials. The FWHM, effective area and encircled energy were measured with the use of proportional counters that were scanned with a set of circular apertures. The pulsers from the proportional counters were sent through a multichannel analyzer that produced a pulse height spectrum. In order to characterize the properties of the mirror at different discrete photon energies one desires to extract from the pulse height distribution only those photons that originated from the characteristic line emission of the X-ray target source. We have developed a code that fits a modeled spectrum to the observed X-ray data, extracts the counts that originated from the line emission, and estimates the error in these counts. The function that is fitted to the X-ray spectra includes a Prescott function for the resolution of the detector a second Prescott function for a pileup peak and a X-ray continuum function. The continuum component is determined by calculating the absorption of the target Bremsstrahlung through various filters correcting for the reflectivity of the mirror and convolving with the detector response.

Chartas, G.↗

Correcting X-ray spectra obtained from the AXAF VETA-I mirror calibration for pileup, continuum, background and deadtime

The VETA-I mirror was calibrated with the use of a collimated soft X-ray source produced by electron bombardment of various anode materials. The FWHM, effective area and encircled energy were measured with the use of proportional counters that were scanned with a set of circular apertures. The pulsers from the proportional counters were sent through a multichannel analyzer that produced a pulse height spectrum. In order to characterize the properties of the mirror at different discrete photon energies one desires to extract from the pulse height distribution only those photons that originated from the characteristic line emission of the X-ray target source. We have developed a code that fits a modeled spectrum to the observed X-ray data, extracts the counts that originated from the line emission, and estimates the error in these counts. The function that is fitted to the X-ray spectra includes a Prescott function for the resolution of the detector a second Prescott function for a pileup peak and a X-ray continuum function. The continuum component is determined by calculating the absorption of the target Bremsstrahlung through various filters, correcting for the reflectivity of the mirror and convolving with the detector response.

Chartas, G.↗

Stimulated X-ray Raman and Absorption Spectroscopy of Iron–Sulfur Dimers

Iron–sulfur complexes play an important role in biological processes such as metabolic electron transport. A detailed understanding of the mechanism of long-range electron transfer requires knowledge of the electronic structure of the complexes, which has traditionally been challenging to obtain, either by theory or by experiment, but the situation has begun to change with advances in quantum chemical methods and intense free electron laser light sources. We compute the spectra for stimulated X-ray Raman spectroscopy (SXRS) and absorption spectroscopy of homovalent and mixed-valence [2Fe–2S] complexes, using the ab initio density matrix renormalization group algorithm. The simulated spectra show clear signatures of the theoretically predicted dense low-lying excited states within the d–d manifold. Finally, the difference in spectral intensity between the absorption-active and Raman-active states provides a potential mechanism to selectively excite states by a proper tuning of the excitation pump, to access the electronic dynamics within this manifold.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Counterstreaming solar wind halo electron events on open field lines?

Counterstreaming solar wind halo electron events have been identified as a common 1 AU signature of coronal mass ejection events, and have generally been interpreted as indicative of closed magnetic field topologies, i.e., magnetic loops or flux ropes rooted at both ends in the Sun, or detached plasmoids. In this paper we examine the possibility that these events may instead occur preferentially on open field lines, and that counterstreaming results from reflection or injection behind interplanetary shocks or from mirroring from regions of compressed magnetic field farther out in the heliosphere. We conclude that neither of these suggested sources of counterstreaming electron beams is viable and that the best interpretation of observed counterstreaming electron events in the solar wind remains that of passage of closed field structures.

Gosling, J. T.↗

Automated tracking of the Florida manatee (Trichechus manatus)

The electronic, physical, biological and environmental factors involved in the automated remote tracking of the Florida manatee (Trichechus manatus) are identified. The current status of the manatee as an endangered species is provided. Brief descriptions of existing tracking and position locating systems are presented to identify the state of the art in these fields. An analysis of energy media is conducted to identify those with the highest probability of success for this application. Logistic questions such as the means of attachment and position of any equipment to be placed on the manatee are also investigated. Power sources and manateeborne electronics encapsulation techniques are studied and the results of a compter generated DF network analysis are summarized.

Michelson, R. C.↗