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DOE OSTI2022

Ultrafast carrier dynamics in terahertz photoconductors and photomixers: beyond short-carrier-lifetime semiconductors

Abstract Efficient terahertz generation and detection are a key prerequisite for high performance terahertz systems. Major advancements in realizing efficient terahertz emitters and detectors were enabled through photonics-driven semiconductor devices, thanks to the extremely wide bandwidth available at optical frequencies. Through the efficient generation and ultrafast transport of charge carriers within a photo-absorbing semiconductor material, terahertz frequency components are created from the mixing products of the optical frequency components that drive the terahertz device – a process usually referred to as photomixing. The created terahertz frequency components, which are in the physical form of oscillating carrier concentrations, can feed a terahertz antenna and get radiated in case of a terahertz emitter, or mix with an incoming terahertz wave to down-convert to DC or to a low frequency photocurrent in case of a terahertz detector. Realizing terahertz photoconductors typically relies on short-carrier-lifetime semiconductors as the photo-absorbing material, where photocarriers are quickly trapped within one picosecond or less after generation, leading to ultrafast carrier dynamics that facilitates high-frequency device operation. However, while enabling broadband operation, a sub-picosecond lifetime of the photocarriers results in a substantial loss of photoconductive gain and optical responsivity. In addition, growth of short-carrier-lifetime semiconductors in many cases relies on the use of rare elements and non-standard processes with limited accessibility. Therefore, there is a strong motivation to explore and develop alternative techniques for realizing terahertz photomixers that do not rely on these defect-introduced short-carrier-lifetime semiconductors. This review will provide an overview of several promising approaches to realize terahertz emitters and detectors without short-carrier-lifetime semiconductors. These novel approaches utilize p-i-n diode junctions, plasmonic nanostructures, ultrafast spintronics, and low-dimensional materials to offer ultrafast carrier response. These innovative directions have great potentials for extending the applicability and accessibility of the terahertz spectrum for a wide range of applications.

36 MATERIALS SCIENCE↗
DOE OSTI2014

SU-E-J-46: Development of a Compton Camera Prototype for Online Range Verification of Laser-Accelerated Proton Beams

Purpose: Development of a photon detection system designed for online range verification of laser-accelerated proton beams via prompt-gamma imaging of nuclear reactions. Methods: We develop a Compton camera for the position-sensitive detection of prompt photons emitted from nuclear reactions between the proton beam and biological samples. The detector is designed to be capable to reconstruct the photon source origin not only from the Compton scattering kinematics of the primary photon, but also to allow for tracking of the Compton-scattered electrons. Results: Simulation studies resulted in the design of the Compton camera based on a LaBr{sub 3}(Ce) scintillation crystal acting as absorber, preceded by a stacked array of 6 double-sided silicon strip detectors as scatterers. From the design simulations, an angular resolution of ≤ 2° and an image reconstruction efficiency of 10{sup −3} −10{sup −5} (at 2–6 MeV) can be expected. The LaBr{sub 3} crystal has been characterized with calibration sources, resulting in a time resolution of 273 ps (FWHM) and an energy resolution of about 3.8% (FWHM). Using a collimated (1 mm diameter) {sup 137}Cs calibration source, the light distribution was measured for each of 64 pixels (6×6 mm{sup 2}). Data were also taken with 0.5 mm collimation and 0.5 mm step size to generate a reference library of light distributions that allows for reconstructing the interaction position of the initial photon using a k-nearest neighbor (k-NN) algorithm developed by the Delft group. Conclusion: The Compton-camera approach for prompt-gamma detection offers promising perspectives for ion beam range verification. A Compton camera prototype is presently being developed and characterized in Garching. Furthermore, an arrangement of, e.g., 4 camera modules could even be used in a ‘gamma-PET’ mode to detect delayed annihilation radiation from positron emitters in the irradiation interrupts (with improved performance in the presence of an additional third (prompt) photon (as in 10C and 14O). This work was supported by the DFG Cluster of Excellence MAP (Munich-Centre for Advanced Photonics)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2012

Spreader-Bar Radiation Detection System Enhancements: A Modeling and Simulation Study

An investigation of radiation detectors on crane-mounted platforms was performed to understand the limitations and optimal capability of these types of systems. Crane-mounted systems are primarily focused on crane-mounted radiation detector systems, where the detectors are mounted on a spreader-bar platform. Spreader bars are attached with cables to a crane at seaports to load and unload containers from cargo ships. The bars can spread from 20 feet to 53 feet using hydraulics, allowing a single bar to move a variety of container lengths. Spreader-bars are also used on straddle carriers, which move containers around the laydown yard in the port. Spreader bar radiation detection (SBRD) systems are commercially available from at least two companies. These systems employ a set of spectroscopic sensors placed on the underside of a gantry crane and held near the top of a cargo container for detection. These systems have been previously tested and some issues and limitations observed. Radiation detectors mounted on spreader-bars are single sided systems (observing cargo only from the top) and it is therefore challenging to obtain the same sensitivity as double-sided systems (for example, portal monitors) especially when considering the possible amounts of intervening cargo that could be present. The approximately exponential attenuation of gamma rays in intervening dense cargo presents an inherent limitation to detection. However, SBRD systems hold detectors closer to the container, have a longer dwell time, and may have lower background (over the ship); all of these aspects help mitigate the single-sided issue. In addition, there are operational considerations that make spreader-bar radiation systems attractive. These include scanning for radiation during other operations (loading, unloading or container movement) which minimizes additional time for scanning, incorporating the radiation detection into existing equipment to minimize initial cost, and in the case of ship unloading, scanning the containers before reaching the laydown yard. This study is focused on researching optimized configurations of SBRD systems, including number of detectors, locations, and best use of detector data, to determine a reasonable limit on the capability of these types of systems. The results will help support decisions on where and how these systems might be effectively deployed, and could be used for future specification development for SBRD acquisition. The next phase of this research and investigation into SBRD systems and quantification of the possible improved capability with an enhanced SBRD is the focus of this report. Supporting this investigation, detailed models of an enhanced SBRD system were created using a 3D radiation transport code, and models were run to simulate the data from sources and background for a realistic cargo-loading port environment. The enhanced SBRD had increased detector material (numbers of detectors) compared to the commercial systems, with a distribution providing more uniform coverage. Measurements using small industrial sources were made with an enhanced SBRD system developed by Sandia National Laboratory to support model validation to establish credibility for the simulations of these threat and background scenarios. A significant simulation effort was undertaken to simulate sources of interest within a 40-foot cargo container. In order to estimate the performance of a generalized SBRD system in scenarios including background and cargo, a highly enriched uranium (HEU) test source (with 3x10 -8 232 U by weight) within a wood cargo model was simulated for a 40-foot cargo container. This source was placed at a variety of locations, and the flux from the source was multiplied as necessary to create estimated minimal detectable quantities (MDQ) figures for various quantities of HEU. Simulated data sets were produced corresponding to a complete container offloading scenario for a large number of statistical realizations. Significant work was performed on both the algorithm development and the container cargo distributions entering the US, and the result of this modeling, validation, and simulation effort was a set of estimates of the performance of a variety of radiation detection algorithms in this cargo-screening environment. In the case of algorithms, a variety of contemporary radiation detection and identification approaches were employed, and the optimal approaches to selecting time and location subsets of detector data were explored. In all cases, algorithm performance was compared, and the best approaches were suggested along with the best expected performance from the enhanced SBRD. In general, template-matching schemes employing a limited set of regression parameters tend to provide best results. The improvements of an enhanced SBRD with increased detector material and improved algorithms result in an effective MDQ of 10 kg of HEU in ~50 percent of the imported cargo in 40-foot containers, assuming a random source location. This is approximately two times the capability of the estimated performance of the commercial systems. For an MDQ of the 10 kg HEU source located in the worst location (bottom of the 40-foot container), the volume of cargo scanned drops to 10% for the enhanced SBRD, again a factor of two or more larger than the commercial systems. Enhancing the SBRD systems by adding more detectors, providing a more uniform coverage, and incorporating more advanced algorithms will result in a significant increase in capability. Although this investigation provided some indication of the performance capabilities of an enhanced SBRD system, additional work is needed to estimate the capability for other container configurations, such as the 20 and 45 foot containers. Since the 20-foot container weight limit is similar to the 40-foot, more dense cargo is typically shipped in 20-foot containers. This will result in a smaller percentage of cargo scanned for the 20-foot containers (for a particular source quantity) compared to the 40-foot containers. In addition to other configuration, other source material needs to be investigated to understand the capabilities for the entire threat space, where only HEU is considered in this work.

crane-mounted↗
DOE OSTI2019

High Energy Micron Scale Pixel Hybrid Detector

The objective of this technology development project has been to fabricate and characterize a new X-ray area image sensor innovation designed for high efficiency detection and imaging of hard X-rays (>20 KeV) with micron scale pixel resolution. A key technology component consists of a monolithic hybrid X-ray detector built by layering an amorphous Selenium X-ray photoconductor film directly deposited on a small pitch (7.8μm) CMOS active pixel readout array. A specific goal of this work is to provide a new detector tool to researchers working with synchrotron light sources, to extend the depth of exploration into nanoscale structures, and do so cost effectively. Early generation X-ray imaging detector tools fail to provide adequate resolving power and efficiency at high energies and our innovation provides a solution. A majority of proposed phase I tasks were completed. Those tasks included, in collaboration with KA Imaging, successful fabrication of specified a-Se layers on a 1Mpixel CMOS readout array to create the direct hybrid X-ray imaging array, packaging of the imaging array, assembly of electronics into a shielded detector box, loading user interface software for camera control and image capture, and performing initial (no X-ray) detector evaluation at Farrier Microengineering facilities. After initial tests, extensive testing using the X-ray beam line 1-BM source at Argonne National Laboratory Advanced Photon Source(ANL-APS) was performed. Imaging performance studies were conducted at multiple X-ray beam energies. Studies included X-ray response vs. X-ray energy, vs. applied detector field strength (HV), response linearity vs. integration time, MTF vs. beam energy, image lag measurements, and micron scale resolution pattern target imaging. This high energy micron scale X-ray detection technology is a first of a kind to be evaluated at the ANL-APS and is supported by Dr. Antonino Miceli, head of the detector physics group. Accomplishments include the first successful demonstration of a 1Mpix amorphous Selenium on CMOS readout direct hybrid X-ray imaging detector at a DOE sponsored National Laboratory. Modeled performance predictions were confirmed, proving micron scale resolution as well as an order of magnitude increase in conversion efficiency over conventional scintillator detector performance. A discovery of evidence of propagation-based phase contrast edge enhancement was unplanned and will be exploited in future experiments. This phase 1 technology demonstration verifies the efficacy of proposed high energy micron scale pixel X-ray hybrid a-Se imaging array products. The new detector products will cost effectively replace early generation detector technologies that currently fail to address increasing demand for tools to study nano structures and physical processes at high X-ray energies above 20keV. For example, current systems for transmission X-ray microscopy have low efficiency and available large pixel (~55µm) direct detectors do not offer sufficient resolution for Bragg fringe imaging at high energies. This detector innovation will solve these inadequacies. The new detector technology will compete in a $50M scientific X-ray detector market, growing at 6%, and will benefit Microtomography(µCT), X-ray diffractometry (XRD), Coherent Diffraction Imaging (CDI) applications. One application specified by Dr. Miceli at ANL is the 3D reconstruction of compact crystals at high energies requires small pixel high efficiency X-ray detectors. Farrier Microengineering, working with colleagues at KA Imaging and the University of Waterloo, successfully achieved the critical objectives of the Phase I proposal. We have proven the technical feasibility of this innovation by building and successfully testing a 1Mpixel a-Se/CMOS hybrid direct X-ray imaging array. Our commercialization roadmap of detector products will be implemented during a phase II project. We will demonstrate a migration of the technology to larger detector array sizes, improved temporal performance with detector layer engineering, and improved environmental and operational stability. Manufacturability and cost effectiveness are key objectives and product designs will leverage current state of the art CMOS wafer fabrication quality and volume manufacturing economics.

36 MATERIALS SCIENCE↗
DOE OSTI2022

High Temperature Optocoupler for 3D High Density Power Modules

The goal of this proposed research is to develop a reliable high-temperature optocouplers, which can operate at 250°C with at least ten-year lifetime, and replace isolation transforms as the galvanic isolation solution for the 3D integration of high density power modules. The electrification of future transportations (i.e., electric vehicles) will continuously drive the demand for high density power modules. Optocouplers (i.e., packaged light emitter and detector) as a promising candidate to replace bulky isolation transformers are highly desirable to facilitate the continuous scale-down of gate driver circuitry that will lead to 3D high density power modules and achieve disruptive performance in terms of thermal management, power density, power efficiency, reliability and operating environments. However, regular semiconductor optoelectronic materials and devices have significant difficulty functioning in the harsh environments designated for high density power module usage (such as operation at high temperatures). Ultimately, it is not the intrinsic properties of power devices that prevent their use at higher temperatures, but rather the low voltage electronics needed to drive them and the packaging that surrounds them. The typical operating temperature for optocouplers is only up to 100°C, due to the limitations of light emitting diode (LED) devices inside and packaging materials. A systematic characterization methodology will be developed to analyze the performance, lifetime and reliability of LED devices and distinguish multiple failure mechanisms at high temperatures. An original methodology of “design for reliability” will be developed to design the optoelectronic devices with high reliability and long lifetime at high temperatures. A new architecture of high temperature high reliable optocouplers will be developed, fabricated and demonstrated with continuous operating at 250°C. The development of efficient, reliable high density 3D power modules is the foundation for energy efficiency and energy reliability. Enabled with advanced 3D integration and packaging technologies, high density power module solutions can achieve much more superior performance over the conventional discrete solutions in terms of efficiency, thermal management and power density. The proposed concept of high temperature optocouplers as the galvanic isolation solution for high density power modules will bring together interdisciplinary research involving the wide bandgap materials, optoelectronics, high reliable device design, electronics packaging and power modules. A streamline of skilled personnel would be trained including graduate and undergraduate students, local engineers and scientists which are in great demand to both academia and optoelectronics industry. The proposed research topics, such as, solid state lighting and high temperature device reliability, are currently of major interest at the Department of Energy, in particular, Sandia National Laboratories. This project can enhance collaborations between the University of Arkansas (UA) and Sandia National Laboratories. The findings of the proposed research are expected to be integrated into high density 3-D power modules at the Engineering Research Center for Power Optimization for Electro-Thermal Systems (POETS).

42 ENGINEERING↗
DOE OSTI2020

First on-line detection of radioactive fission isotopes produced by laser-accelerated protons

Abstract The on-going developments in laser acceleration of protons and light ions, as well as the production of strong bursts of neutrons and multi- $$\hbox {MeV}$$ MeV photons by secondary processes now provide a basis for novel high-flux nuclear physics experiments. While the maximum energy of protons resulting from Target Normal Sheath Acceleration is presently still limited to around $$100 \, \hbox {MeV}$$ 100 MeV , the generated proton peak flux within the short laser-accelerated bunches can already today exceed the values achievable at the most advanced conventional accelerators by orders of magnitude. This paper consists of two parts covering the scientific motivation and relevance of such experiments and a first proof-of-principle demonstration. In the presented experiment pulses of $$200 \, \hbox {J}$$ 200 J at $$\approx \, 500 \, \hbox {fs}$$ ≈ 500 fs duration from the PHELIX laser produced more than $$10^{12}$$ 10 12 protons with energies above $$15 \, \hbox {MeV}$$ 15 MeV in a bunch of sub-nanosecond duration. They were used to induce fission in foil targets made of natural uranium. To make use of the nonpareil flux, these targets have to be very close to the laser acceleration source, since the particle density within the bunch is strongly affected by Coulomb explosion and the velocity differences between ions of different energy. The main challenge for nuclear detection with high-purity germanium detectors is given by the strong electromagnetic pulse caused by the laser-matter interaction close to the laser acceleration source. This was mitigated by utilizing fast transport of the fission products by a gas flow to a carbon filter, where the $$\upgamma$$ γ -rays were registered. The identified nuclides include those that have half-lives down to $$39 \, \hbox {s}$$ 39 s . These results demonstrate the capability to produce, extract, and detect short-lived reaction products under the demanding experimental condition imposed by the high-power laser interaction. The approach promotes research towards relevant nuclear astrophysical studies at conditions currently only accessible at nuclear high energy density laser facilities.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2017

Solar Living House Final Technical Report

The Solar Living House is a high-performance solar-powered dwelling designed by a team of faculty and students from the University of Florida, in collaboration with Santa Fe College, the National University of Singapore, and Alachua Habitat for Humanity. The project was designed in accordance with the Solar Decathlon 2015, a research, design, education, and outreach program developed by the U.S. Department of Energy (DOE). The Solar Living House is fundamentally a house for living, centered on people and the activities of daily life while quietly introducing advanced design, construction, and engineering technologies. The 993 square-foot two-bedroom one-bath home was designed to embrace and frame an exterior courtyard space. This courtyard acts as an extension of the interior living spaces, maximizing the spatial potentials of a modest building footprint and introducing natural light into the primary living spaces of the house. Research Outcomes: The Solar Living House advances work on high-performance buildings through three principal technological innovations: wet/dry modular construction, a building automation system, and solar dehumidification systems. Wet / Dry Modular Construction: The house is designed as a series of five modules, including one that is designated as the “wet core.” The wet core consolidates the mechanical systems and bathroom into a single module to reduce plumbing runs, efficiency losses, and on-site construction time. The other four modules are designed to eliminate interior load bearing walls to allow for maximum flexibility in the reconfiguring of the space over time. The modules are designed to meet the structural challenges of both Florida’s hurricanes and California’s earthquakes. Building Automation System: The house is equipped with an integrated building automation system, allowing the houses environmental systems, lights, security systems, and smoke detectors to be programmed, monitored, and controlled through any mobile or computing device. These systems allow for more precise calibrations of temperature/humidity/lighting to correspond with user needs and preferences, minimizing energy losses with economical night- or day-time setbacks. Solar Dehumidification System: The most significant technological innovation in the Solar Living House is the solar thermal dehumidification system. This system generates hot water through two rooftop-mounted evacuated tube solar thermal collectors. The hot water is used to continually dry a regenerative solid desiccant material, typically white silica gel. The solid desiccant is used to adsorb moisture and humidity from the air without additional mechanical cooling. This strategy allows humidity to be modulated independently of air temperature, providing greater thermal comfort and reducing the opportunity for the growth of mold spores within the house while also reducing the overall energy consumption of the HVAC system. Economic Feasibility: The team set aggressive goals for affordability, targeting a construction cost of $138,710. An independent professional cost estimator determined the overall project costs, as designed, would be $333,799, or $336.15 per square foot of finished floor area. This is more than 2.4 times the target construction cost. By comparison, the average construction cost for a home in the United States in 2015 was $289,415, or $103.29 per square foot of finished floor area. Following work on the Solar Living House, team leaders incorporated many of its objectives into a net-zero energy home on a site in Gainesville, Florida. This site-built home avoided many of the constraints and complications of modular construction necessitated by the Solar Decathlon, allowing it to be built for a much more modest budget. This two-bedroom two bath 1,800 square foot home was constructed for $135.39 per square foot, including active photovoltaic solar systems, careful attention to continuous air barriers, increased insulation levels, and permanent site constructions. This project suggest that high-performance buildings can be realized for more modest budgets. Public Benefits: Work on the Solar Living House and Solar Decathlon 2015 offered our student team unparalleled learning opportunities. Because of the duration of the project, a number of students participated at different points in their education, from first year undergraduates all the way through to advanced graduate students. The opportunity for collaboration with students and faculty from the National University of Singapore was also extraordinary, allowing for a sharing of technical knowledge and cultural exchange. The wider public has benefited from this work as its findings have been shared through public presentations and publications. It serves as a useful stepping stone along the path towards affordable, high-performance buildings.

14 SOLAR ENERGY↗
DOE OSTI2024

Axions beyond Gen 2

The QCD (Quantum ChromoDynamics) axion emerged as one of the best-motivated dark matter candidates. In 2018, the Axion Dark Matter eXperiment (ADMX), one of the U.S. Department of Energy’s “Gen 2” flagship dark-matter projects, demonstrated first sensitivity to the highly plausible “DFSZ” dark matter axion couplings over a small frequency range. We anticipate this development marks the first step in constructing yet more powerful experiments that can explore large swaths of the axion parameter space at high sensitivity and result in a discovery. But, realizing this requires advances in both our understanding of the theory and experiment design. Between 25 January and 27 January 2021, the “Axions Beyond Gen 2 Workshop” was held, where selected members of the community discussed our broad understanding of the QCD axion and charted a course for future experiments having sensitivity and mass reach well beyond the current “Gen 2” experiments. These proceedings are summaries of the topics presented and discussed.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2012

Nevada National Security Site: Site-Directed Research and Development (Fiscal Year 2011 Annual Report)

This fiscal year 2011 annual report of the Site-Directed Research and Development program, the 10th anniversary edition, recognizes a full decade of innovative R&D accomplishments in support of the Nevada National Security Site (NNSS). Last year the NNSS itself was renamed to reflect a diversifying mission, and our R&D program has contributed significantly to shape emerging missions that will continue to evolve. New initiatives in stockpile stewardship science, nonproliferation, and treaty verification and monitoring have had substantial successes in FY 2011, and many more accomplishments are expected. SDRD is the cornerstone on which many of these initiatives rest. Historically supporting our main focus areas, SDRD is also building a solid foundation for new, and non-traditional, emerging national security missions. The program continues its charter to advance science and technology for a broad base of agencies including the U.S. Department of Energy (DOE), U.S. Department of Defense (DoD), U.S. Department of Homeland Security (DHS), and many others.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗
DOE OSTI2018

Measurement of the Negative Pion and Positive Kaon Total Hadronic Cross Sections on Argon at the LArIAT Experiment

The Liquid Argon Time Projection Chamber (LArTPC) represents one of the most advanced experimental technologies for physics at the Intensity Frontier due to its full 3D-imaging, excellent particle identication and precise calorimetric energy reconstruction. By deploying a LArTPC in a dedicated calibration test beam line at Fermilab, LArIAT (Liquid Argon In A Testbeam) aims to experimentally calibrate this technology in a controlled environment and to provide physics results key to the neutrino oscillation physics and proton decay searches of the Short Baseline Neutrino (SBND, MicroBooNE, ICARUS) and Long Baseline Neutrino programs (DUNE). LArIAT's physics program entails a vast set of topics with a particular focus on the study of nuclear eects such as pion and kaon characteristic interaction modes. This thesis presents two measurements performed for the rst time: the measure- ment of the negative pion total hadronic cross section on argon in the 100-1050 MeV kinetic energy range and the measurement of the positive kaon total hadronic cross section on argon in the 100-650 MeV kinetic energy range. The analyses devised for these measurements use both the core elements of LArIAT: beamline and LArTPC. The rst step in each analysis is the development of an event selection based on beam- line and TPC information geared towards the identication of the hadron of interest. We then proceed to match the beamline candidate to a suitable TPC track. Finally, we apply the \thin slice method" technique and measure the cross section, correcting for background contamination and detector eects. The thin slice technique is a new method to measure hadron-argon cross sections possible only due to the combination of the tracking and calorimetry capability of the LArTPC technology. Albeit never on argon, the hadronic cross section of pions has been extensively measured before on lighter and heavier dierent elements in thin target experiments, leading to solid predictions for measurements on argon. Through the use of a dierent technique, our measurement of the negative pion total hadronic cross section on argon is in general agreement with the predictions by the Geant4 Bertini Cascade model which are based on data from thin target experiments. On the contrary, cross section measurements for kaons are extremely scarce, thus more dicult to model. Our measurement of the positive kaon total hadronic cross section on argon is mostly in tension with the Geant4 prediction over the explored range of energies and provides new experimental data to properly compare existing interaction models. This thesis also reports two ancillary detector physics measurements necessary for the cross section analyses: the measurements of the LArIAT electric eld and calorimetry constants. We developed a technique to measure the LArIAT electric eld using cathode-anode piercing tracks with cosmic data. We applied a new technique for the measurement of the calorimetry calibration constants based on the particles' momentum measurement. The negative pion and the positive kaon total hadronic cross measurements are the rst physics results of the LArIAT experiment and will be the basis for the future LArIAT measurements of pion and kaon cross sections in the exclusive channels. The outcome of these measurements will ultimately enable to quantify and reduce the systematic associated with the hadronic interaction models in neutrino-argon interactions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Discovering Elusive Dynamics Across Frontiers (Final Technical Report)

Profound puzzles, such as the nature of dark matter, the origins of the electroweak scale, the mechanism behind the small neutrino mass, and the strong CP problem, suggested new physics beyond the Standard Model and drove the particle physics program in search of the associated new particles. Despite extensive searches, conventional realizations of new physics have not yet provided conclusive evidence. This raised the serious possibility that new dynamics might be more elusive, perhaps due to a richer gauge and matter structure than previously considered. Notably, the existence of dark matter and advancements in understanding the naturalness problem urged exploration into sectors with complex gauge and matter structures. Through experiments like the LHC, DUNE, and small-scale experiments, the robust US HEP program played a critical role in pursuing these well-motivated but under-explored scenarios for new physics. I explored these physics opportunities in depth, focusing on novel searches and significant improvements in parameter space coverage. The elusive dynamics revealed rich information about the underlying theory and were essential in identifying observable opportunities. Understanding the observable consequences required a deep comprehension of the theory, which I also developed. The proposal included essential components aimed at coherently increasing our knowledge in well-motivated elusive dynamics models. Through research on high-quality axions, composite neutrinos, the Higgs boson as a portal to hidden strong dynamics, and new scalar potentials to generate alternative electroweak phase transitions, I focused on identifying new signatures and parameter regions in plausible elusive dynamics models. The exploration emphasized generic possibilities motivated by broad classes of elusive dynamics models. These signatures were not effectively probed previously due to various challenges such as triggering, background suppression, or experimental design. My research involved close interaction with experimental colleagues to overcome these difficulties, leveraging new theoretical and experimental possibilities. These efforts included identifying new observables such as timing information and substructure in calorimetries, new multiple-hit techniques, new scattering events, and new resonance searches in liquid argon detectors. This work created a positive feedback loop: theory and experimental work inspired each other, revealing new exciting opportunities that supported both programs.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Hydrogen Detection Strategies to Support H2@SCALE - The NREL Sensor Laboratory

Hydrogen represents a major pathway to decarbonize and stabilize the national and international energy industry and select manufacturing markets. To facilitate the development of hydrogen markets, the US Department of Energy initiated H2@Scale to bring together stakeholders to advance affordable hydrogen production, transport, storage, and utilization to increase revenue opportunities in multiple energy sectors. One major impediment to hydrogen implementation is cost. To expedite the use of hydrogen in energy and other markets, the United States announced in 2021 the Hydrogen Shot, which seeks to reduce the cost of clean hydrogen by 80% to $1 per 1 kilogram in 1 decade ("1 1 1"). As the cost of hydrogen drops, new applications will emerge that will require unique configurations of existing equipment and infrastructure, and eventually lead to advances in the generation and utilization of hydrogen. As the hydrogen economy expands, sensors and detection methods will need to adapt to changing infrastructure demands to address the primary targets of health & safety, emissions monitoring, and process control. The NREL Sensor Laboratory is playing a pivotal role in advancing the use of hydrogen sensors and detection methodologies in each of these categories to support DOE's mission for safe and efficient utilization in emerging markets. Health & safety monitors are required to ensure that operators and facilities can react to unintended hydrogen releases, either as GH2, LH2, or as a constituent of blends (e.g., natural gas or ammonia). Current detection methodologies focus on safety applications to detect near its lower flammable limit (4 vol %), and typically include point sensors in applications such as fixed or mobile detectors (e.g., personal gas monitors). Methodologies amenable for area detection include acoustic, emerging optical imaging methods, and flame detectors. Comparable detection strategies can be utilized for emissions monitoring and quantization, however few methods can simultaneously cover both low (emissions) and high (health & safety) levels. Deployment of emission level detectors will be required to 1) reduce product loss through small but potentially significant leaks from an environmental or cost perspective, 2) reduce downtime of high demand systems by early identification of eminent system failures (leaks through pump or compressor seals indicative of impending failure), and 3) address potential emission monitoring requirements that may be set by regulating bodies. The first two points should be adopted by industry to reduce the cost-of-goods-sold. The third main category for hydrogen detection relates to process control and may be advantageous for many existing applications. Two main applications are emerging. For example, the purity requirements for hydrogen that is dispensed from refueling systems for hydrogen fuel cell electric vehicles (FCEV) is rigorously regulated by the Standard SAE J2719, which prescribes maximum allowable levels of multiple impurities in the hydrogen fuel and must be verified by a regulatory body. Hydrogen contaminant detectors (HCD) integrated to the fueling station can assure this compliance. HCDs must be able operate in 100% H2 backgrounds and be able to distinguish between multiple contaminants at low ppm to low ppb levels. Secondly, as a strategy to decarbonize the natural gas grid, there are proposals to blend hydrogen with natural gas. This blending will affect transport applications (pipeline infrastructure), stationary combustion systems (turbines), and consumer and commercial appliances. In the short-term, hydrogen levels up to 20% are proposed. Variations in the hydrogen level can have dramatic impact on the combustion process and on the potential response of safety sensors. These mixtures may be regulated so that the concentration at a delivery point must be monitored with high precision. However, routine maintenance may introduce background gases such as ambient air (with water) or maintenance gases (introduced with welding processes or adhesive outgassing.) Therefore, the detection methodology must be robust enough to recover or respond to various contaminants. Several reviews can be found in literature addressing sensing and detection technologies, including their limitations and applications. However, for most applications, limitations can be alleviated by combining various detection techniques either through system integration or implementation of machine learning methods (artificial intelligence). In this presentation, we will discuss several applications, highlight their current approach for hydrogen detection, and suggest detection strategies to supplement their limitations.

ENERGY STORAGE,HYDROGEN↗
DOE OSTI2016

An advanced materials irradiation facility for materials and fuels irradiations at the high flux isotope reactor

The High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory (ORNL) is a pressurized, light-water-cooled and -moderated, beryllium-reflected, 85 MW research reactor fueled by Highly enriched {sup 235}U. The Materials Irradiation Facility (MIF) at HFIR) is one of the two experimental platforms in the US that can host fully instrumented and monitored experiments in a high-neutron-flux environment. The unique advantage of instrumented capsules is that the researcher can monitor and acquire in situ data and change capsule operating conditions in real time during the irradiation. Recently ORNL funded a Laboratory-Directed Research and Development (LDRD) project to strategically enhance the capabilities of MIF and provide researchers with a more flexible experimental platform. MIF comprises 4 systems: a gas supply system, a supervisory control system, an effluent system, and a standard gas routing system. The first 3 systems have common functionality for all types of experiments. The gas routing system provides the correct gases and gas mixtures for individual experiments and is unique to each experiment. MIF improvements include an updated and more sophisticated experiment monitoring system, a modular design allowing easier addition of simultaneous experiments, and features that allow rapid incorporation of additional instrumentation. The new design is both modular and re-configurable. It calls for a standard gas routing system module that can be configured with software to allow for easy expansion to multiple experiments. The ability to monitor the effluent activity during fissile material irradiation is a much needed enhancement for detecting fuel failures or determining fission product release. A gamma-ray spectrometry will be installed in a bypass gas line off the effluent main stream. The gas will flow through the detector for continuous detection of the particles of interest.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2025

Energy-resolved neutron imaging and diffraction including grain orientation mapping using event camera technology

Time-of-flight neutron diffraction and energy-resolved imaging each provide unique perspectives into material properties. Neutron diffraction is useful for assessing microstructural parameters such as phase composition, texture, and dislocation densities, though it typically provides averaged data over the sampled volume. Energy-resolved imaging, on the other hand, offers both spatial and spectral information by detecting Bragg edges and neutron absorption resonances, which enables detailed mapping of microstructure and isotopic composition. When combined, these techniques have the potential to enrich our understanding of material behavior across different scales, enhancing our understanding of complex materials. Traditionally, these modalities are conducted on separate instruments, which is time-consuming and poses challenges for data integration. Here, we report the integration of the LumaCam, an event-mode energy-resolved neutron imaging camera with the HIPPO time-of-flight diffractometer at LANSCE. This integration enables simultaneous diffraction and imaging across the full spectrum, with analysis optimized for diffraction and Bragg-edge imaging in the thermal range (0.45–10 Å) and resonance imaging in the epithermal range (0.5–3000 eV), facilitating comprehensive multi-modal analysis. We demonstrate its capabilities through case studies, including spatial mapping of grain orientations in a steel sample and accurate thickness estimations for irregular samples including a depleted uranium cylinder and a natural silver-containing mineral specimen. The combined setup enhances real-time sample alignment and provides comprehensive data for crystal structure, texture, and isotopic composition analysis. This approach opens new possibilities for advanced applications in nuclear engineering, archaeology, and materials science.

36 MATERIALS SCIENCE↗
DOE OSTI2018

The LiteBIRD Satellite Mission: Sub-Kelvin Instrument

Inflation is the leading theory of the first instant of the universe. Inflation, which postulates that the universe underwent a period of rapid expansion an instant after its birth, provides convincing explanation for cosmological observations. Recent advancements in detector technology have opened opportunities to explore primordial gravitational waves generated by the inflation through “B-mode” (divergent-free) polarization pattern embedded in the cosmic microwave background anisotropies. If detected, these signals would provide strong evidence for inflation, point to the correct model for inflation, and open a window to physics at ultra-high energies. LiteBIRD is a satellite mission with a goal of detecting degree-and-larger-angular-scale B-mode polarization. LiteBIRD will observe at the second Lagrange point with a 400 mm diameter telescope and 2622 detectors. It will survey the entire sky with 15 frequency bands from 40 to 400 GHz to measure and subtract foregrounds. The US LiteBIRD team is proposing to deliver sub-Kelvin instruments that include detectors and readout electronics. A lenslet-coupled sinuous antenna array will cover low-frequency bands (40–235 GHz) with four frequency arrangements of trichroic pixels. An orthomode-transducer-coupled corrugated horn array will cover high-frequency bands (280–402 GHz) with three types of single frequency detectors. The detectors will be made with transition edge sensor (TES) bolometers cooled to a 100 milli-Kelvin base temperature by an adiabatic demagnetization refrigerator. The TES bolometers will be read out using digital frequency multiplexing with Superconducting QUantum Interference Device (SQUID) amplifiers. Up to 78 bolometers will be multiplexed with a single SQUID amplifier. Lastly, we report on the sub-Kelvin instrument design and ongoing developments for the LiteBIRD mission.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2017

NASA's Orgins Space Telescope Mission and Its Synergies with SOFIA

The Origins Space Telescope (OST) is the mission concept for the Far Infrared Surveyor, a study in development by NASA in preparation for the 2020 Astronomy and Astrophysics Decadal Survey. The science program that has been selected to drive the OST performance requirements is broad, covering four main themes: Charting the Rise of Metals, Dust, and the First Galaxies; Unveiling the Growth of Black Holes and Galaxies Over Cosmic Time; Tracing the Signatures of Life and the Ingredients of Habitable Worlds; and Characterizing Small Bodies in the Solar System. The OST telescope itself will have a primary mirror diameter of 8-15 m (depending on the launch vehicle that is selected), will be diffraction-limited at 40m, and will be actively cooled to approximately 5K. Five science instruments have been base-lined for the observatory: a heterodyne instrument covering 150-500 m with a spectral resolving power of R1e7; a low-spectral resolution (R500) spectrometer covering 35-500 m; a high-spectral resolution (R1e5) spectrometer covering 50-500 m; a far-infrared imager (R15) covering 35-500m; and a mid-infrared imagerspectrometer (R15-500) covering 6-40m. In addition to having a vastly higher sensitivity than the corresponding SOFIA instrumentation that will allow more detailed follow-up of SOFIAs discoveries, the OST mission will be configured to provide efficient large-area mapping, which will further complement SOFIAs science capabilities by providing new targets for study by SOFIA. Furthermore, new SOFIA instruments can provide an excellent testbed for the advanced far-infrared detector technologies what will be required to achieve the anticipated OST performance.

Mission↗
DOE OSTI2026

SEARCHING FOR MESONIC DARK MATTER WITH THE HEAVY PHOTON SEARCH EXPERIMENT

Several highly-sensitive astrophysical experiments over the past couple of decades have demonstrated that the current abundance of visible Standard Model matter cannot explain galactic rotation curves, the expansion history of the Universe, or the apparent warping of light in empty space. Instead, one finds strong agreement with this body of experimental results upon positing the existence of an invisible particulate field, dark matter. Namely, a cold, weakly interacting dark matter component can explain all these phenomena. A number of accelerator-based experiments have been developed to search for the weak couplings/interactions of these particles, many of them concentrating on particle models with masses of tens to thousands of GeV. A relatively new, well-motivated model is a dark sector coupled to the Standard Model via a dark photon. The current abundance of dark matter can be obtained if one assumes that dark matter is coupled to light by a MeV to GeV particle with a U(1) symmetry. The parameter space of these models remains largely unexplored because they are difficult to probe experimentally. In this thesis, I analyze data from the Heavy Photon Search (HPS) detector, whose two detector halves closely surround the electron beam, providing acceptance to far-forward boosted interactions. This forward acceptance to highly boosted particles yields unprecedented sensitivity to MeV-scale invariant masses. I exhaustively optimize the offline reconstruction of the HPS detector. Each reconstruction object, from Silicon Vertex Tracker hits to tracks, is studied to maximize acceptance of dark matter events. I then use the 2021 run data to search for one model of dark-photon-mediated matter, the Strongly Interacting Massive Particle (SIMP). SIMP models provide self-interacting dark matter candidates that can form bound states resembling dark mesons. HPS can detect SIMPs through the decay of a dark vector boson (either a dark ¿ or ¿) into e+e- pairs. I obtain exclusion contours for SIMPs using both an optimized cuts-based selection and a machine-learning-based selection, advancing our knowledge of the nature of dark matter.

O'Dwyer, Rory [Stanford Univ., CA (United States).↗
NASA NTRS1989

Advanced technology satellite demodulator development

Ford Aerospace has developed a proof-of-concept satellite 8 phase shift keying (PSK) modulation and coding system operating in the Time Division Multiple Access (TDMA) mode at a data range of 200 Mbps using rate 5/6 forward error correction coding. The 80 Msps 8 PSK modem was developed in a mostly digital form and is amenable to an ASIC realization in the next phase of development. The codec was developed as a paper design only. The power efficiency goal was to be within 2 dB of theoretical at a bit error rate (BER) of 5x10(exp 7) while the measured implementation loss was 4.5 dB. The bandwidth efficiency goal was 2 bits/sec/Hz while the realized bandwidth efficiency was 1.8 bits/sec/Hz. The burst format used a preamble of only 40 8 PSK symbol times including 32 symbols of all zeros and an eight symbol unique word. The modem and associated special test equipment (STE) were fabricated mostly on a specially designed stitch-weld board although a few of the highest rate circuits were built on printed circuit cards. All the digital circuits were ECL to support the clock rates of from 80 MHz to 360 MHz. The transmitter and receiver matched filters were square-root Nyquist bandpass filters realized at the 3.37 GHz i.f. The modem operated as a coherent system although no analog phase locked (PLL) loop was employed. Within the budgetary constraints of the program, the approach to the demodulator has been proven and is eligible to proceed to the next phase of development of a satellite demodulator engineering model. This would entail the development of an ASIC version of the digital portion of the demodulator, and MMIC version of the quadrature detector, and SAW Nyquist filters to realize the bandwidth efficiency.

Ames, Stephen A.↗