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At least 1,009 records · Page 56

Assessing residential PM 2.5 concentrations and infiltration factors with high spatiotemporal resolution using crowdsourced sensors

Building conditions, outdoor climate, and human behavior influence residential concentrations of fine particulate matter (PM 2.5 ). To study PM 2.5 spatiotemporal variability in residences, we acquired paired indoor and outdoor PM 2.5 measurements at 3,977 residences across the United States totaling >10,000 monitor-years of time-resolved data (10-min resolution) from the PurpleAir network. Time-series analysis and statistical modeling apportioned residential PM 2.5 concentrations to outdoor sources (median residential contribution = 52% of total, coefficient of variation = 69%), episodic indoor emission events such as cooking (28%, CV = 210%) and persistent indoor sources (20%, CV = 112%). Residences in the temperate marine climate zone experienced higher infiltration factors, consistent with expectations for more time with open windows in milder climates. Likewise, for all climate zones, infiltration factors were highest in summer and lowest in winter, decreasing by approximately half in most climate zones. Large outdoor–indoor temperature differences were associated with lower infiltration factors, suggesting particle losses from active filtration occurred during heating and cooling. Absolute contributions from both outdoor and indoor sources increased during wildfire events. Infiltration factors decreased during periods of high outdoor PM 2.5 , such as during wildfires, reducing potential exposures from outdoor-origin particles but increasing potential exposures to indoor-origin particles. Time-of-day analysis reveals that episodic emission events are most frequent during mealtimes as well as on holidays (Thanksgiving and Christmas), indicating that cooking-related activities are a strong episodic emission source of indoor PM 2.5 in monitored residences.

54 ENVIRONMENTAL SCIENCES↗

The First Swift Intensive AGN Accretion Disk Reverberation Mapping Survey

Swift intensive accretion disk reverberation mapping of four AGN yielded light curves sampled ∼200–350 times in 0.3–10 keV X-ray and six UV/optical bands. Uniform reduction and cross-correlation analysis of these data sets yields three main results: (1) The X-ray/UV correlations are much weaker than those within the UV/optical, posing severe problems for the lamp-post reprocessing model in which variations in a central X-ray corona drive and power those in the surrounding accretion disk. (2) The UV/optical interband lags are generally consistent with t μ l4 3 as predicted by the centrally illuminated thin accretion disk model. While the average interband lags are somewhat larger than predicted, these results alone are not inconsistent with the thin disk model given the large systematic uncertainties involved. (3) The one exception is the U band lags, which are on average a factor of ∼2.2 larger than predicted from the surrounding band data and fits. This excess appears to be due to diffuse continuum emission from the broad-line region (BLR). The precise mixing of disk and BLR components cannot be determined from these data alone. The lags in different AGN appear to scale with mass or luminosity. We also find that there are systematic differences between the uncertainties derived by JAVELIN versus more standard lag measurement techniques, with JAVELIN reporting smaller uncertainties by a factor of 2.5 on average. In order to be conservative only standard techniques were used in the analyses reported herein.

R. Edelson↗

First Results from Faint Infrared Grism Survey (Figs): First Simultaneous Detection of Ly Alpha Emission and Lyman Break From a Galaxy at Z =7.51

Galaxies at high redshifts provide a valuable tool to study cosmic dawn, and therefore it is crucial to reliably identify these galaxies. Here, we present an unambiguous and first simultaneous detection of both the Lyman-Alpha emission and the Lyman break from a z = 7.512 +/- 0.004 galaxy, observed in the Faint Infrared Grism Survey (FIGS). These spectra, taken with G102 grism on Hubble SpaceTelescope (HST), show a significant emission line detection (6 Sigma) in two observational position angles (PA), with Lyman-Alpha line flux of 1.06 +/- 0.19 x 10(exp -17) erg s(exp -1) cm(exp -2). The line flux is nearly a factor of four higher than in the archival MOSFIRE spectroscopic observations. This is consistent with other recent observations implying that ground-based near-infrared spectroscopy underestimates total emission line fluxes, and if confirmed, can have strong implications for reionization studies that are based on ground-based Lyman-Alpha measurements. A 4-Alpha detection of the NV line in one PA also suggests a weak Active Galactic Nucleus (AGN), and if confirmed would make this source the highest-redshift AGN yet found.These observations from the Hubble Space Telescope thus clearly demonstrate the sensitivity of the FIGS survey, and the capability of grism spectroscopy to study the epoch of reionization.

Faint Galaxy Z=7.51↗

The Gamma-Ray Pulsar Phenomenology in View of 3D Kinetic Global Magnetosphere Models

We develop kinetic plasma models of pulsar magnetospheres with magnetic-field-line-dependent plasma injection that reveal the importance of various magnetosphere regions in regulating the gamma-ray emission. We set different particle injection rates for the so-called open, closed, and separatrix zones. Moderate particle injection rates in open and closed zones ensure a global field structure close to the force-free one, while the dissipation occurs mainly in and around the equatorial current sheet. The particles injected in the separatrix zone affect the particle populations that enter the equatorial current sheet region and, therefore, the corresponding accelerating electric fields, particle energies, the spectral cutoff energy, and gamma-ray efficiency. The separatrix zone models reproduce the recently discovered fundamental plane of gamma-ray pulsars consistent with curvature radiation emission, the gamma-ray light-curve shapes, and the radio-lag vs. peak-separation correlation reported in the Fermi second pulsar catalog. The model beaming factors indicate that the pulsar total gamma-ray luminosities listed in the Fermi catalogs are overestimations of the actual ones. We find that the radiation reaction limited regime starts ceasing to govern the high-energy emission for spin-down powers less than 1034 erg/s. Our results also indicate that toward high magnetic inclination angles, the "Y point" around the rotational equator migrates well inside the light cylinder sparking additional peaks in the gamma-ray pulse profiles. We find that an equivalent enhanced particle injection beyond the Y point strengthens these features making the model gamma-ray light curves inconsistent with those observed.

Neutron stars↗

X-ray emission from supernova remnants MSH 14 - 63 and RCW 103

Electron-ion collisions, heavy element enrichment of emissions from reverse-shocked ejecta, abundances in the interstellar medium (ISM), the correspondence between the projected and measured age, ISM particle density, and distance, and classification factors for Type I or II supernovae are examined using a nonequilibrium ionization (NEI) model. The NEI model accounts for the absence of collisional ionization equilibrium and possibly thermal equilibrium between electrons and ions behind the shock fronts, and describes the emission spectra from ejecta and the shocked ISM. When applied to data from the SNR MSH 14 - 63 a non-Coulomb, ion-electron interaction is obtained that is consistent with a shocked ISM. For the SNR RCW 103, however, the processes behind the shock front are not discernable, although the elemental abundances will have solar values if the interactions are non-Coulomb. The age of RCW 103 must be approximated from physical data, as Chinese astronomers would not have been able to see the event from their position on earth two millenia ago.

Nugent, J. J.↗

Spatiotemporal dynamics of ecosystem fires and biomass burning-induced carbon emissions in China over the past two decades

Fire is a major type of disturbance that has important influences on ecosystem dynamics and carbon cycles. Yet our understanding of ecosystem fires and their carbon cycle consequences is still limited, largely due to the difficulty of large-scale fire monitoring and the complex interactions between fire, vegetation, climate, and anthropogenic factors. Here, using data from satellite-derived fire observations and ecosystem model simulations, we performed a comprehensive investigation of the spatial and temporal dynamics of China's ecosystem fire disturbances and their carbon emissions over the past two decades (1997–2016). Satellite-derived results showed that on average about 3.47 - 4.53 x 10 4 km 2 of the land was burned annually during the past two decades, among which annual burned forest area was about 0.81 - 1.25 × 10 4 km 2 , accounting for 0.33-0.51% of the forest area in China. Biomass burning emitted about 23.02 TgC per year. Compared to satellite products, simulations from the Energy Exascale Earth System Land Model (ELM) strongly overestimated China's burned area and fire-induced carbon emissions. Annual burned area and fire-induced carbon emissions were high for boreal forest in Northeast China's Daxing'anling region and subtropical dry forest in South Yunnan, as revealed by both the satellite product and the model simulations. Our results suggest that climate and anthropogenic factors play critical roles in controlling the spatial and seasonal distribution of China's ecosystem fire disturbances. Our findings highlight the importance of multiple complementary approaches in assessing ecosystem fire disturbance and its carbon consequences. Further studies are required to improve the methods of observing and modelling China's ecosystem fire disturbances, which will provide valuable information for fire management and ecosystem sustainability in an era when both human activities and the natural environment are rapidly changing.

54 ENVIRONMENTAL SCIENCES↗

Crack growth in single-crystal silicon

Crack growth in single-crystal silicon at room temperature in air was evaluated by double torsion (DT) load-relaxation method and monitored by acoustic emission (AE) technique. Both DT and AE methods indicated lack of subcritical crack growth in silicon. At the critical stress intensity factor, the crack front was found to be jumping several times in a 'mirror' region and then followed by fast crack growth in a 'hackle' region. Hackle marks were found to be associated with plastic deformation at the tip of the fast moving crack. No dislocation etch pits were found in the 'mirror' region, in which crack growth may result from interatomic bonds broken at the crack tip under stress without any plastic deformation. Acoustic emission appears to be spontaneously generated from both interatomic bonds broken and dislocation generation at the moving crack tip during the crack growth in single-crystal silicon.

Chen, C. P.↗

Version 2 of the global catalogue of large anthropogenic and volcanic SO 2 sources and emissions derived from satellite measurements

Sulfur dioxide (SO 2 ) measurements from the Ozone Monitoring Instrument (OMI), Ozone Mapping and Profiler Suite (OMPS), and TROPOspheric Monitoring Instrument (TROPOMI) satellite spectrometers were used to update and extend the previously developed global catalogue of large SO 2 emission sources. This version 2 of the global catalogue covers the period of 2005–2021 and includes a total of 759 continuously emitting point sources releasing from about 10 kt yr −1 to more than 4000 kt yr −1 of SO 2 , that have been identified and grouped by country and primary source origin: volcanoes (106 sources); power plants (477); smelters (74); and sources related to the oil and gas industry (102). There are several major improvements compared to the original catalogue: it combines emissions estimates from three satellite instruments instead of just OMI, uses a new version 2 of the OMI and OMPS SO 2 dataset, and updated consistent site-specific air mass factors (AMFs) are used to calculate SO 2 vertical column densities (VCDs). The newest TROPOMI SO 2 data processed with the Covariance-Based Retrieval Algorithm (COBRA), used in the catalogue, can detect sources with emissions as low as 8 kt yr −1 (in 2018–2021) compared to the 30 kt yr −1 limit for OMI. In general, there is an overall agreement within ±12 % in total emissions estimated from the three satellite instruments for large regions. For individual emission sources, the spread is larger: the annual emissions estimated from OMI and TROPOMI agree within ±13 % in 50 % of cases and within ±28 % in 90 % of cases. The version 2 catalogue emissions were calculated as a weighted average of emission estimates from the three satellite instruments using an inverse-variance weighting method. OMI, OMPS, and TROPOMI data contribute 7 %, 5 %, and 88 % to the average, respectively, for small (<30 kt yr −1 ) sources and 33 %, 20 %, and 47 %, respectively, for large (>300 kt yr −1 ) sources. The catalogue data show an approximate 50 % decline in global SO 2 emissions between 2005 and 2021, although emissions were relatively stable during the last 3 years. The version 2 of the global catalogue has been posted at the NASA global SO 2 monitoring website (https://doi.org/10.5067/MEASURES/SO2/DATA406, Fioletov et al., 2022).

volcanic↗

Observing soft X-ray line emission from the interstellar medium with X-ray calorimeter on a sounding rocket

For an X-ray calorimeter working at 0.1 K, the energy resolution ideally can be as good as one eV for a practical detector. A detector with a resolution of 17 eV FWHM at 6 keV has been constructed. It is expected that this can be improved by a factor of two or more. With X-ray calorimeters flown on a sounding rocket, it should be possible to observe soft X-ray line emission from the interstellar medium over the energy range 0.07 to 1 keV. Here, a preliminary design for an X-ray calorimeter rocket experiment and the spectrum which might be observed from an equilibrium plasma are presented. For later X-ray calorimeter sounding rocket experiments, it is planned to add an aluminum foil mirror with collecting area of about 400 sq cm to observe line features from bright supernova remnants.

Zhang, J.↗

Seasonal Controls of CO 2 and CH 4 Dynamics in a Temporarily Flooded Subtropical Wetland

Subtropical and tropical wetlands play a prominent role in the global carbon (C) cycle; yet factors that influence their C fluxes remain uncertain. We collected measurements from a temporarily flooded subtropical wetland over 3 years to investigate environmental drivers impacting CO 2 and CH 4 fluxes. The wetland was a sink of CO 2 (-469 to -380 g C-CO 2 · m -2 · year -1 ) and a source of CH 4 (25.1 to 32.1 g C-CH 4 · m -2 · year -1 ) to the atmosphere. Dry season CH 4 emissions represented 41 to 49% of the annual budget, reflecting the importance of continuous CH 4 flux measurements. Gross primary productivity (GPP) increased with temperature and radiation, and the influence of VPD on GPP varied with soil inundation. Higher water tables decreased Reco and increased GPP, and a higher GPP in turn lead to enhanced R eco likely through enhancements of GPP on autotrophic respiration. This suggests that the impact of the water table on R eco depends on the cancelling effects of hydrology and GPP. Emissions of CH 4 increased with soil temperature, water table, and GPP until soils were inundated at which point temperature and GPP became the main drivers. Water table and temperature influenced GPP and CH 4 fluxes, and increases in GPP directly enhanced CH 4 emissions. In addition to impacting C fluxes directly through water table depth, hydrology also determined the hierarchy of the dominance of factors controlling C fluxes and their response. The positive climate forcing of subtropical wetlands may be dictated by plant-mediated and climate interactions, with hydrological factors playing a major role in determining the greenhouse gas sink or source strength of subtropical wetlands.

54 ENVIRONMENTAL SCIENCES↗

Evidence for a Canonical GRB Afterglow Light Curve in the Swift/XRT Data

We present new observations of the early X-ray afterglows of the first 27 gamma-ray bursts (GRBs) detected with the Swift X-ray Telescope (XRT). The early X-ray afterglows show a canonical behavior, where the light curve broadly consists of three distinct power law segments. These power law segments are separated by two corresponding break times. On top of this canonical behavior of the early X-ray light curve, many events have superimposed X-ray flares, which are most likely caused by internal shocks due to long lasting sporadx activity of the central engine, up to several hours after the GRB. We find that the initial steep decay is consistent with it being the tail of the prompt emission: from photons that are radiated at large angles relative to our line of sight. The first break in the light curve takes place when the forward shock emission becomes dominant, with the intermediate shallow flux decay likely caused by the continuous energy injection into the external shock. When this energy injection stops, a second break is then observed in the light curve. This energy injection increases the energy of the afterglow shock by at least a factor of f greater than or approx. equal to 4, and augments the already severe requirements for the efficiency of the prompt gamma-ray emission.

Nousek, J. A.↗

Synchrotron emission from a cosmological jet as a model of gamma-ray bursts

The nonthermal rapidly varying spectra of gamma-ray bursts require relativistic beaming if the source is at a cosmological distance. Limits on the Lorentz factors and magnetic fields of extragalactic jet models of gamma-ray bursts are derived from the synchrotron source function, the position of the fundamental cyclotron resonance, the Thomson optical depth of radiating electrons, and the Thomson optical depth of electron-positron pairs created in photon-photon collisions of Compton upscattered radiation. The last of these constraints is the strongest, and it is satisfied by the observations if the jet's Lorentz factor is greater than 100. The limit from the position of the cyclotron fundamental requires a magnetic field strength below approximately 10 exp 10 G. Jet models producing observable cyclotron lines are allowed. The acceleration region in the burst must be separate from the emission region. The similarity of gamma-ray burst jet models to models of quasars and BL Lac objects suggest that if gamma-ray bursts are cosmological sources, they are a type of active galaxy.

Brainerd, J. J.↗

Diffuse continuum gamma rays from the Galaxy observed by COMPTEL

The diffuse Galactic continuum gamma-ray emission has been studied using the full Sky Survey from COMPTEL on the Compton Observatory CGRO. The diffuse emission appears to be visible in the whole 0.75-30 MeV range covered by the instrument, although a considerable contribution from unresolved point sources cannot be excluded. A correlation analysis using HI and CO surveys of the Galaxy is used to derive the Galactic emissivity spectrum, and this is consistent with a smooth continuation to the spectrum at higher energies derived by a similar analysis of COS-B data. The apparent conversion factor from integrated CO temperature to molecular hydrogen column density can also be determined from the correlation analysis. The value obtained is consistent with results from COS-B and other non-gamma-ray methods. Calculations of the emissivity spectrum from bremsstrahlung from a cosmic-ray electron spectrum based on propagation models are compared with the observations.

Strong, A. W.↗

The effects of fire on biogenic soil emissions of nitric oxide and nitrous oxide

Measurements of biogenic soil emissions of nitric oxide (NO) and nitrous oxide (N2O) before and after a controlled burn conducted in a chaparral ecosystem on June 22, 1987, showed significantly enhanced emissions of both gases after the burn. Mean NO emissions from heavily burned and wetted (to simulate rainfall) sites exceeded 40 ng N/sq m s, and increase of 2 to 3 compared to preburn wetted site measurements. N2O emissions from burned and wetted sites ranged from 9 to 22 ng N/sq m s. Preburn N2O emissions from these wetted sites were all below the detection level of the instrumentation, indicating a flux below 2 ng N/sq m s. The flux of NO exceeded the N2O flux from burned wetted sites by factors ranging from 2.7 to 3.4. These measurements, coupled with preburn and postburn measurements of ammonium and nitrate in the soil of this chaparral ecosystem and measurements of NO and N2O emissions obtained under controlled laboratory conditions, suggest that the postfire enhancement of NO and N2O emissions is due to production of these gases by nitrifying bacteria.

Levine, Joel S.↗

Understanding tungsten erosion during inter/intra-ELM periods in He-dominated JET-ILW plasmas

Tungsten erosion was quantified during inter/intra-ELM periods in He-dominated JET-ILW plasmas by optical emission spectroscopy. The intra-ELM tungsten sputtering in helium plasmas, which dominates the total W source, prevails by a factor of about 4 over inter-ELM sputtering in the investigated ELM frequency range from 90 Hz–120 Hz. He ions are mainly responsible for the W erosion during the ELMs in He plasmas. The strong in/out asymmetry of the ELM-induced W erosion is observed in He plasmas even at high ELM frequencies beyond 100 Hz. In Ohmic/L-mode plasmas and during the H-mode inter-ELM plasma phases both He 2+ and Be 2+ ionic species are major contributors to the W erosion. Their contribution depends on the electron temperature in the divertor: for T e > 15 eV both species cause significant W sputtering, for T e < 15 eV, B e 2+ ions are solely responsible for the W erosion. Tungsten erosion during in both inter and intra-ELM periods in He-dominated plasmas are significantly larger than in deuterium plasmas. It is 15–25 times larger during the inter-ELM phase and in L-mode discharges at T e = 25–30 eV. On the other hand, the ELM-induced W source is by a factor of 3 larger than in D plasmas.

36 MATERIALS SCIENCE↗

Voltage-dependent excitation dynamics in UV-absorbing organic photovoltaics with efficient charge transfer exciton emission

Intermolecular charge-transfer excitons play a central role in determining the performance of organic solar cells as their voltage-dependent formation, dissociation, and recombination dynamics contribute to photocurrent generation, radiative/nonradiative voltage losses, and photovoltaic fill factor. Here, we explore the properties of brightly-emitting wide energy gap (>2 eV) charge transfer excitons by measuring the voltage-dependent photoluminescence, photocurrent, and ultrafast pump–probe transient absorption spectra of organic solar cells employing five UV-absorbing donor molecules that differ only by the length of the oligophenylene or acene group at their core. We find that organic solar cells with a strong correlation between their voltage-dependent photocurrent and charge-transfer exciton photoluminescence have low photovoltaic fill factors as they require voltage to facilitate efficient charge-transfer exciton dissociation. In contrast, solar cells that are efficient can readily generate charges without an applied field and have a separate population of tightly-bound charge-transfer excitons that are responsible for emission. Furthermore, considering that the sum of all excitation loss rates (i.e., recombination and charge extraction) must be equal to the excitation generation rate in the steady state, these voltage-dependent data allow us to solve for the voltage-dependent fate of all excitations in the solar cells and estimate upper and lower bounds for geminate and non-geminate recombination, respectively.

14 SOLAR ENERGY↗

H I absorption limits and emission mapping for high-velocity clouds

Systematic emission and absorption surveys have been conducted for high-velocity H I in the direction of 63 bright continuum sources. High-velocity emisison is detected along 18 of these 63 directions with a threshold about a factor of 2 better than previous, much more extensive surveys. No high-velocity absorption was found in any of the directions. The sky distribution of the high-velocity emission and the column density distribution agree with larger surveys. Detailed emission maps in the vicinity of each continuum source show that the variations in column density within a high-velocity cloud are similar to the variations between high-velocity clouds. A previously discovered high-velocity cloud at high galactic latitude, in the direction of part of the Virgo Cluster of galaxies, was mapped. This small cloud is moving away from the galactic plane at v greater than 30 km/s and is probably not self-gravitating.

Colgan, Sean W. J.↗

Small- x factorization from effective field theory

We derive a factorization theorem that allows for resummation of small-x logarithms by exploiting Glauber operators in the soft collinear effective field theory. Our analysis is carried out for the hadronic tensor W μν in deep inelastic scattering, and leads to the definition of a new gauge invariant soft function S μν that describes quark and gluon emission in the central region. This soft function provides a new framework for extending resummed calculations for coefficient functions to higher logarithmic orders. Our factorization also defines impact factors by universal collinear functions that are process independent, for instance being identical in small-x DIS and Drell-Yan.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗