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Nuclear Data Sheets for A=31

Nuclear spectroscopic information for the known nuclides of mass 31 (F, Ne, Na, Mg, Al, Si, P, S, Cl, Ar) has been evaluated. A useful source of many of the Adopted Levels for {sup 31}P and {sup 31}S is presented in Endt's evaluations (1998En04,1990En08,1978En02,1973EnVA), however all the adopted properties of levels and gamma rays have been re-evaluated in this work. The data sets for reactions and decays, including all available gamma–ray data, are based mostly on the original literature. The 31Mg nuclide is a prime candidate for the study of ‘island-of-inversion’ as its ground state and first excited state can only be explained by intruder orbitals in a deformed shell-model approach. {sup 31}S is of importance in astrophysics rp-process as a possible ‘bottleneck’ nuclide. There are no data available for excited states in {sup 31}F, {sup 31}Ne and {sup 31}Ar. No gamma transitions are known in {sup 31}Cl. For {sup 31}Na, only one excited state is known. The radioactive decay characteristics of {sup 31}F and {sup 31}Ne isotopes have not yet been investigated. The {sup 31}S and {sup 31}Mg nuclei are currently being pursued intensively by various experimental groups, including recent work by Nuclear Astrophysics group at McMaster, the results of which will soon become available.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

On-Site Inspection RadioIsotopic Spectroscopy (Osiris) System Development

We have designed and tested hardware and software for the acquisition and analysis of high-resolution gamma-ray spectra during on-site inspections under the Comprehensive Nuclear-Test-Ban Treaty (CTBT). The On-Site Inspection RadioIsotopic Spectroscopy—Osiris—software filters the spectral data to display only radioisotopic information relevant to CTBT on-site inspections, e.g.,132I. A set of over 100 fission-product spectra was employed for Osiris testing. These spectra were measured, where possible, or generated by modeling. The synthetic test spectral compositions include non-nuclear-explosion scenarios, e.g., a severe nuclear reactor accident, and nuclear-explosion scenarios such as a vented underground nuclear test. Comparing its computer-based analyses to expert visual analyses of the test spectra, Osiris correctly identifies CTBT-relevant fission product isotopes at the 95% level or better.The Osiris gamma-ray spectrometer is a mechanically-cooled, battery-powered ORTEC Transpec-100, chosen to avoid the need for liquid nitrogen during on-site inspections. The spectrometer was used successfully during the recent 2014 CTBT Integrated Field Exercise in Jordan. The spectrometer is controlled and the spectral data analyzed by a Panasonic Toughbook notebook computer. To date, software development has been the main focus of the Osiris project. In FY2016-17, we plan to modify the Osiris hardware, integrate the Osiris software and hardware, and conduct rigorous field tests to ensure that the Osiris system will function correctly during CTBT on-site inspections. The planned development will raise Osiris to technology readiness level TRL-8; transfer the Osiris technology to a commercial manufacturer, and demonstrate Osiris to potential CTBT on-site inspectors.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Benched: Upgrading and Updating the Los Alamos Benchmark Suite for the 21st Century [Slides]

The presentation begins by stating that most organizations make choices to handle specific things when preparing input files for validation, such as which elemental abundance data to use, how to decompose specific elements, and setting calculation precision. It also discusses the consequences, which include differing calculation results between different organizations for the same case, even when using the same code. This is illustrated by the intercomparison exercise and input files that are prepared by one organization and are not necessarily correct for another. The presentation explains that the Los Alamos Benchmark Suite is a centralized repository of high-quality benchmark models currently under development at LANL. The objectives of the new repository are to remain up to date with the latest ICSBEP revision, to have a formal review and revision process, to (eventually) be an open-source repository, and to provide new tools for improved input and output file generation and review.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

The Study of (n, 2n) Reaction Cross Sections for Ce and Nd Isotopes up to 20 MeV

Neutron cross section calculations for {sup 136}Ce(n, 2n){sup 135}Ce, {sup 138}Ce(n, 2n){sup 137}Ce, {sup 140}Ce(n, 2n){sup 139}Ce, {sup 142}Ce(n, 2n){sup 141}Ce, {sup 142}Nd(n, 2n){sup 141}Nd, {sup 144}Nd(n, 2n){sup 143}Nd, {sup 146}Nd(n, 2n){sup 145}Nd, {sup 148}Nd(n, 2n){sup 147}Nd, and {sup 150}Nd(n, 2n){sup 149}Nd were done in the incident energy range from 10 to 20 MeV. The calculations were performed using three codes TALYS-1.6 for two-component Exciton model, EMPIRE-3.2 Malta for Exciton model, and ALICE/ASH for the Geometry-Dependent Hybrid (GDH) model. The results of model calculations were compared with the available experimental data and also with the evaluated data in the TENDL-2015 (based on the modified TALYS code), ENDF/B-VII.1 libraries. The calculated cross section data were compared with the available experimental data obtained from EXFOR and also compared with semiempirical formulas around 14–15 MeV. The results of model calculation were found to be in good agreement with the experimental data given in literature and semiempirical data around 14–15MeV.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

TREAT neutronics analysis and design support, Part I: Multi-SERTTA

Experiment vehicle design is necessary in preparation for Transient Reactor Test (TREAT) facility restart and the resumption of transient testing to support Accident Tolerant Fuel (ATF) characterization and other future fuels testing requirements. Currently the most mature vehicle design is the Multi-SERTTA (Static Environments Rodlet Transient Test Apparatuses), which can accommodate up to four concurrent rodlet-sized specimens under separate environmental conditions. Robust test vehicle design requires neutronics analyses to support design development, optimization of the power coupling factor (PCF) to efficiently maximize energy generation in the test fuel rodlets, and experiment safety analyses. Calculations were performed to support analysis of a near-final design of the Multi-SERTTA vehicle, the design process for future TREAT test vehicles, and establish analytical practices for upcoming transient test experiments. Models of the Multi-SERTTA vehicle containing typical PWR-fuel rodlets were prepared and neutronics calculations were performed using MCNP6.1 with ENDF/B-VII.1 nuclear data libraries. Calculation of the PCF for reference conditions of a PWR fuel rodlet in clean water at operational temperature and pressure provided results between 1.10 and 1.73 W/g-MW depending on the location of the four Multi-SERTTA units with the stack. Basic changes to the Multi-SERTTA secondary vessel containment and support have minimal impact on PCF; using materials with less neutron absorption can improve expected PCF values, especially in the primary containment. An optimized balance is needed between structural integrity, experiment safety, and energy deposition in the experiment. Type of medium and environmental conditions within the primary vessel surrounding the fuel rodlet can also have a significant impact on resultant PCF values. The estimated reactivity insertion worth into the TREAT core is impacted more by the primary and secondary Multi-SERTTA vehicle structure with the experiment content and contained environment having a near negligible impact on overall system reactivity. Additional calculations were performed to evaluate the peak-to-average assembly powers throughout the TREAT core, as well as the nuclear heat generation for the various structural components of the Multi-SERTTA assembly. Future efforts include the evaluation of flux collars to shape the PCF for individual Multi-SERTTA units during an experiment such as to achieve uniformity in test unit environmental conditions impacted by the non-uniform axial flux/power profile of TREAT. Upon resumption of transient testing, experimental results from both the Multi-SERTTA and Multi-SERTTA-CAL will be compared against calculational results and methods for further optimization and design strategies. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Fission with Exotic Nuclei (Abbreviated Report)

Nuclear fission is a key mechanism involved in the synthesis of heavy elements in the Cosmos and is the primary explanation for the stability of superheavy elements. Nevertheless, our knowledge of fission remains extremely fragmented. Most experiments have been conducted only on a tiny number of stable actinide nuclei and are often incomplete, leading to gaps in our basic understanding of the process. For many radioactive isotopes, basic fission data such as the charge or mass distribution of the fragments is unknown. These gaps cannot always be filled by simulation alone. Common fission models contain too many free parameters and lack predictive power. In contrast, the fundamental theory of fission under development at LLNL is much more predictive, but its current computational cost is too high to be used extensively for data evaluations. A unique window of opportunity to resolve these limitations has recently opened: the U.S. nuclear science community is ramping up major experimental programs at the Facility for Rare Isotope Beams (FRIB, the DOE flagship facility in low-energy nuclear science), and techniques from machine learning have shown great potential to simplify the use of a fundamental, quantum-mechanical theory of fission. This project has two components. On the experimental side, we acquired and deployed at the HIGS facility a new dual Frisch-Grid ionization chamber to measure correlated fragment-mass, kinetic energy, and angular distributions of fission fragments from induced fission. This new device was used to perform measurements of charge, mass and total kinetic energy of fission fragments in the photofission of 238 U and eight gamma-ray beam energies between 6.2 and 13 MeV, which allowed extracting high-precision independent yields for this reaction. The device was also used to perform measurements of the same quantities in the neutron-induced fission of 234 U with monoenergetic beams of energy between 5 and 8 MeV. In parallel, we collaborated with a team at Commissariat à l’énergie atomique et aux énergies alternatives (CEA) to perform a series of measurements of fission yields in inverse kinematics for the two isotopes of 236 U and 240 Pu. The experiment took place at the Grand Accélérateur National d’Ions Lourds in France in June 2023. The deployment of the VAMOS spectrometer with a new array called PISTA allowed determining the excitation energy of the fissioning system within 1 Mega-electronvolts. The second component of the project involved using deep neural networks to build fast and reliable emulators of our current fission models. In an invited paper published in Frontier in Physics, we showed that autoencoders could successfully compress nuclear wavefunctions in nuclear density functional theory. We achieved a dimensionality reduction of the order of two orders of magnitude while keeping the error in the total energy to less than 0.01%. In a second paper submitted to Physical Review Letters in June 2023 with our collaborators at CEA, we showed that variational autoencoders can learn the collective degrees of freedom driving the fission process.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Active Time-Domain Reflectometry for Unattended Safeguards Systems FY15 Report

The International Atomic Energy Agency (IAEA) continues to expand its use of unattended measurement systems. An increasing number of systems and an expanding family of instruments create challenges in terms of deployment efficiency and the implementation of data authentication measures. In collaboration with the IAEA, tamper-indicating measures to address data-transmission authentication challenges with unattended safeguards systems are under investigation. Pacific Northwest National Laboratory (PNNL) is studying the viability of active time-domain reflectometry (TDR) along two parallel but interconnected paths: (1) swept-frequency TDR as the highly flexible, laboratory gold standard to which field-deployable options can be compared, and (2) a low-cost commercially available spread-spectrum TDR technology as one option for field implementation. This report describes PNNL’s FY15 progress in the viability study including: an overview of the TDR methods under investigation; description of the testing configurations and mock tampering scenarios; results from a preliminary sensitivity comparison of the two TDR methods; demonstration of a quantitative metric for estimating field performance that acknowledges the need for high detection probability while minimizing false alarms. FY15 progress reported here sets the stage for a rigorous comparison of the candidate TDR methods, over a range of deployment scenarios and perturbing effects typical of IAEA unattended monitoring systems.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Environmental Cracking and Irradiation Resistant Stainless Steels by Additive Manufacturing

Metal additive manufacturing (AM), or metal 3D printing is an emergent advanced manufacturing method that can create near net shape geometries directly from computer models. This technology can provide the capability to rapidly fabricate complex parts that may be required to enhance the integrity of reactor internals components. Such opportunities may be observed during a plant refueling outage and AM parts can be rapidly custom designed, manufactured and deployed within the outage interval. Additive manufacturing of stainless steel (SS) components can add business benefits on fast delivery on repair hardware, installation tooling, new design prototypes tests, etc. For the nuclear industry, the supply chain is always an issue for reactor service. AM can provide through-life supply chain (40-60 years) for high-value low-volume components. In the meantime, the capability of generating complex geometries and functional gradient materials will improve the performance, reduce the overall component cost, plant asset management cost and increase the plant reliability by the improvement in materials performance in nuclear environments. While extensive work has been conducted regarding additively manufacturing of austenitic SS parts, most efforts focused only on basic attributes such as porosity, residual stress, basic tensile properties, along with components yield and process monitoring. Little work has been done to define and evaluate the material requirements for nuclear applications. Technical gaps exist, which limit this technology adoption in the nuclear industry, which includes high manufacturing cost, unknown risks, limited nuclear related data, lack of specification and qualification methods, and no prior business experience. The main objective of this program was to generate research data to address all these technical gaps and establish a commercial practice to use AM technology in the nuclear power industry. The detailed objectives are listed as follows: (1) Evaluate nuclear related properties of AM 316L SS, including microstructure, tensile properties, impact toughness, stress corrosion cracking (SCC), corrosion fatigue (CF), irradiation effects, and irradiation assisted stress corrosion cracking (IASCC). (2) Understand the correlations among laser processing, heat treatment, microstructure and SCC/irradiation properties; (3) Optimize and improve the manufacturing process to achieve enhanced nuclear application properties; (4) Fabricate, evaluate, qualify and test a prototype reactor component to demonstrate the commercial viability and cost benefit; (5) Create regulatory approval path and commercialization plans for the production of a commercial reactor component.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Validation and Testing of ENDF/B-VII Decay Data

The nuclear decay library developed for the ORIGEN code was upgraded from ENDF/B-VI.8 to -VII.0 and released in the SCALE nuclear modeling and simulation code system in 2011. Experience with the ENDF/B-VII.0 library identified serious errors and performance issues in the evaluated decay sublibrary. Initially, errors were identified in the decay scheme for the 238U series, leading to large discrepancies in the gamma emission rate for uranium. Further testing of the fission product decay data revealed significant performance issues with ENDF/B-VII.0 relative to the previous release of ENDF/B-VI. To address the performance issues, the decay data library in SCALE was upgraded to ENDF/B-VII.1 and released as an update for users in 2013. This paper describes the practical impact of the ENDF/B-VII.0 decay data performance issues on common code applications, and the validation and testing performed on the updated ORIGEN libraries developed from the ENDF/B-VII.1 sublibrary.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Draft Rules for Alloy 617 Creep-Fatigue Design Using an EPP+SMT Approach

The report describes an improved new creep-fatigue design method for structural components in high temperature nuclear service. The new method uses an integrated elastic-perfectly plastic (EPP) analysis and Simplified Model Test (SMT) approach that greatly simplifies the design process by avoiding the separate evaluation of creep and fatigue damages and eliminating the requirement of stress classification. The report includes draft design rules, presented in a format compatible with an ASME nuclear Code Case, as well as a commentary on the rules and the validation of the rules using pressurized SMT (p-SMT) test data. Areas of potential improvement have been identified for further evaluation. The report also develops EPP+SMT design charts for Alloy 617 at temperatures between 800°C and 950°C by extrapolating high strain range, short hold test data to low strain range and long hold times, typical for structural components in high temperature nuclear service. The design charts are currently limited to 10,000 cycles to avoid excessive extrapolation outside the test database. More robust alternate extrapolation procedures will be considered in future work. The report includes several verification problems comparing the new EPP+SMT design method with current ASME creep-fatigue design methods. The comparison demonstrates that the EPP+SMT method significantly reduces the over-conservatism in current methods. Finally, the report includes a fully-documented sample problem with multiple load cases detailing the application of proposed EPP+SMT design rules.

36 MATERIALS SCIENCE↗

Updates to the HTR-PROTEUS HALEU Benchmark Using Modern Analysis Methodologies

The HTR-PROTEUS IRPhEP Handbook benchmarks represent some of the highest quality benchmarks available for systems with TRISO-HALEU fuel, graphite pebbles, graphite reflector, and high neutron leakage. Nevertheless, significant variability in computed eigenvalue results was encountered in HTR-PROTEUS configurations that are relevant for transportation configurations. The team will investigate the source of these variabilities in the original benchmark. In addition, the team will investigate the HTR-PROTEUS subcritical measurements, kinetics data, and potential criticality effects from the introduction of hydrogen in the system (water ingress). The project will generate a benchmark evaluation of additional HTR-PROTEUS measurements that can significantly increase the value of these criticality benchmarks in testing nuclear codes and data to support transportation validation needs for industry and the U.S. NRC.

22 - GENERAL STUDIES OF NUCLEAR REACTORS↗

U.S. Efforts in Support of Examinations at Fukushima Daiichi - November 2025 Meeting Notes

Fifteen years have passed since the March 11, 2011, the Great East Japan Earthquake (GEJE) triggered a tsunami that inundated the Fukushima Daiichi Nuclear Power Station (Daiichi or 1F) and led to severe accidents in multiple units at the plant. During these fifteen years since these events, Daiichi forensics examinations and evaluations have revealed many insights for enhancing the safety of nuclear power plants worldwide. However, uncertainties remain regarding the events after the GEJE. Additional Daiichi forensics information is required to inform future Decontamination and Decommissioning (D&D) activi- ties conducted by the plant owner, Tokyo Electric Power Company Holdings, Incorporated (TEPCO Hold- ings). This forensics information also has important implications for the safety and operation of U.S. commercial nuclear power plants. A collaborative U.S. and Japanese effort, which includes approximately 50 experts in reactor safety and plant operations, was initiated in 2014 by the Department of Energy Office of Nuclear Energy (U.S. DOE-NE) to identify Daiichi examination needs and evaluate recent Daiichi examination data to address these needs. This collaborative effort, which is beneficial to the U.S. and Japan, continues as Japan moves forward with D&D activities.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Guideline for Performing Systematic Approach to Evaluate and Qualify Legacy Documents that Support Advanced Reactor Technology Activity

The establishment of a systematic process for the evaluation of historic technology information for use in advanced reactor licensing is described. Efforts are underway to recover and preserve Experimental Breeder Reactor II and Fast Flux Test Facility historical data. These efforts have generally emphasized preserving information from data-acquisition systems and hard-copy reports and entering it into modern electronic formats suitable for data retrieval and examination. The guidance contained in this document has been developed to facilitate consistent and systematic evaluation processes relating to quality attributes of historic technical information (with focus on sodium-cooled fast reactor (SFR) technology) that will be used to eventually support licensing of advanced reactor designs. The historical information may include, but is not limited to, design documents for SFRs, research-and-development (R&D) data and associated documents, test plans and associated protocols, operations and test data, international research data, technical reports, and information associated with past U.S. Nuclear Regulatory Commission (NRC) reviews of SFR designs. The evaluation process is prescribed in terms of SFR technology, but the process can be used to evaluate historical information for any type of advanced reactor technology. An appendix provides a discussion of typical issues that should be considered when evaluating and qualifying historical information for advanced reactor technology fuel and source terms, based on current light water reactor (LWR) requirements and recent experience gained from Next Generation Nuclear Plant (NGNP).

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Formatting and V&V of Consistent 238,240−24 2Pu $\overline{v}_p$ Evaluated Mean Values and Covariances

This report is in answer to the Nuclear Criticality Safety Program FY24 quarter 4 milestone that requires: “Format and V&V nu-bar means and covariances” for 238,240-242 Pu average prompt fission neutron multiplicities, $\overline{ν}$ p , that were obtained by a consistent evaluation leveraging the fission-event generator CGMF and a detailed uncertainty quantification of experimental data. It is described how nuclear data mean values and covariances were formatted using ENDFtk. Implementing the new 238,240-242 Pu $\overline{ν}$ p into the ENDF/B-VIII.1β 4 library leads to only small overall changes in criticality values of the Jezebel, Dirty Jezebel, Jupiter-001, Jupiter-002, EUCLID 3x2 and EUCLID 8x1 critical assemblies. Simulated k eff uncertainties due to $\overline{ν}$ p covariances change only little if cross-isotope covariances are considered or not for those assemblies with low percentage content of minor Pu isotopes. However, for the Dirty Jezebel critical assembly, that has a sizeable 240 Pu and non-negligible 241 Pu content, the simulated k eff uncertainties due to considering or neglecting cross-isotope $\overline{ν}$ p covariances is 443 versus 374 pcm.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

FISPACT-II: An Advanced Simulation System for Activation, Transmutation and Material Modelling

Fispact-II is a code system and library database for modelling activation-transmutation processes, depletion-burn-up, time dependent inventory and radiation damage source terms caused by nuclear reactions and decays. The Fispact-II code, written in object-style Fortran, follows the evolution of material irradiated by neutrons, alphas, gammas, protons, or deuterons, and provides a wide range of derived radiological output quantities to satisfy most needs for nuclear applications. It can be used with any ENDF-compliant group library data for nuclear reactions, particle-induced and spontaneous fission yields, and radioactive decay (including but not limited to TENDL-2015, ENDF/B-VII.1, JEFF-3.2, JENDL-4.0u, CENDL-3.1 processed into fine-group-structure files, GEFY-5.2 and UKDD-16), as well as resolved and unresolved resonance range probability tables for self-shielding corrections and updated radiological hazard indices. The code has many novel features including: extension of the energy range up to 1 GeV; additional neutron physics including self-shielding effects, temperature dependence, thin and thick target yields; pathway analysis; and sensitivity and uncertainty quantification and propagation using full covariance data. The latest ENDF libraries such as TENDL encompass thousands of target isotopes. Nuclear data libraries for Fispact-II are prepared from these using processing codes PREPRO, NJOY and CALENDF. These data include resonance parameters, cross sections with covariances, probability tables in the resonance ranges, PKA spectra, kerma, dpa, gas and radionuclide production and energy-dependent fission yields, supplemented with all 27 decay types. All such data for the five most important incident particles are provided in evaluated data tables. The Fispact-II simulation software is described in detail in this paper, together with the nuclear data libraries. The Fispact-II system also includes several utility programs for code-use optimisation, visualisation and production of secondary radiological quantities. Included in the paper are summaries of results from the suite of verification and validation reports available with the code.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗