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At least 1,027 records · Page 57

Raman Wavelength Conversion in Ionic Liquids

Here, we explore the use of room-temperature ionic liquids (ILs) as Raman wavelength converters. ILs provide an engineerable framework to design suitable liquids for wavelength conversion over a broad spectral range, through careful selection of the molecular structures of the IL anions and cations so that specific characteristics can be obtained, such as a desirable Raman shift, low Brillouin scattering, and good optical transmission in the pump and Stokes wavelengths. Applying such criteria, we demonstrate that 1-ethyl-3-methylimidazolium dicyanamide (EMIM DCA) is an effective medium for conversion of 532-nm pulses from a Q-switched Nd :YAG laser to 603 nm. This corresponds to an approximate 2200 cm –1 shift, which can be used to generate mid-infrared radiation through subsequent difference frequency generation for optical pumping of CO 2 lasers. Threefold-higher Raman conversion efficiency is obtained in EMIM DCA compared with water under identical conditions in a proof-of-principle single-pass conversion setup, resulting in an efficient generation of multimillijoule, <6 ns duration, high-quality orange laser pulses in a wavelength region that is difficult to access at high energies. Consequently, we examine ILs representing two other classes of Raman-active functional groups and obtain conversion up to the fifth-order Stokes shift and first anti-Stokes shift. Through the tunable selection of their components and their useful dynamical properties, ILs provide a platform for efficient, simple, and alignment-tolerant high-energy Raman shifting with numerous industrial and technological applications.

74 ATOMIC AND MOLECULAR PHYSICS↗

Unifying femtosecond and picosecond single-pulse magnetic switching in Gd-Fe-Co

Many questions are still open regarding the physical mechanisms behind the magnetic switching in Gd-Fe-Co alloys by single optical pulses. Phenomenological models suggest a femtosecond scale exchange relaxation between sublattice magnetization as the driving mechanism for switching. The recent observation of thermally induced switching in Gd-Fe-Co by using both several picosecond optical laser pulse as well as electric current pulses has questioned this previous understanding. This has raised the question of whether or not the same switching mechanics are acting at the femtosecond and picosecond scales. In this work, we aim at filling this gap in the understanding of the switching mechanisms behind thermal single-pulse switching. To that end, we have studied experimentally thermal single-pulse switching in Gd-Fe-Co alloys, for a wide range of system parameters, such as composition, laser power, and pulse duration. We provide a quantitative description of the switching dynamics using atomistic spin dynamics methods with excellent agreement between the model and our experiments across a wide range of parameters and timescales, ranging from femtoseconds to picoseconds. Furthermore, we find distinct element-specific damping parameters as a key ingredient for switching with long picosecond pulses and argue that switching with pulse durations as long as 15 ps is possible due to a low damping constant of Gd. Our findings can be easily extended to speed up dynamics in other contexts where ferrimagnetic Gd-Fe-Co alloys have been already demonstrated to show fast and energy-efficient processes, e.g., domain-wall motion in a track and spin-orbit torque switching in spintronics devices.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

The Airborne Laser Ranging System - Its capabilities and applications

The Airborne Laser Ranging System is a proposed multibeam short pulse laser ranging system on board an aircraft. It simultaneously measures the distances between the aircraft and six laser retroreflectors (targets) deployed on the earth's surface. Depending on the host aircraft and terrain characteristics, the system can interrogate hundreds of targets distributed over an area as large as 60,000 sq. km in a matter of hours. Potentially, a total of 1.3 million individual range measurements can be made in a 6 hr flight. The precision of these range measurements is approximately 1 cm. These measurements are then used in a procedure which is basically an extension of trilateration techniques to derive the intersite vector between the laser ground targets. By repeating the estimation of the intersite vector, strain and strain rate errors can be estimated. These quantities are essential for crustal dynamic studies which include determination and monitoring of regional strain in the vicinity of active fault zones, land subsidence, and edifice building preceding volcanic eruptions.

Kahn, W. D.↗

Determining forest canopy characteristics using airborne laser data

A study is reported in which a profiling laser system flown at relatively low altitudes over a forested area was used to measure various forest canopy attributes, including tree heights. An analysis of the data obtained indicates that canopy closure is most strongly related to the penetration capability of the laser pulse, with the pulses attenuated more quickly in a dense canopy. Laser estimates of the average tree heights differ by less than 1 m from the photogrammetrically acquired values. It is concluded that the laser system is suitable for remotely sensing the vertical forest canopy profile. Elements of this profile are linearly related to crown closure and can be used to assess tree height.

Nelson, R.↗

Lunar observer laser altimeter

Understanding the global topography of the Moon is especially important for answering questions concerning lunar origin and evolution. Many outstanding problems in lunar science can be addressed with high resolution topographic data. The severe power, mass, size, and data-rate limitations imposed by the Lunar Geoscience Observer (LGO) and other Observer-class missions are major challenges for all instruments capable of measuring topography. A radar altimeter that meets these strict requirements could obtain a global prespective of lunar topography with a few kilometers spatial resolution and 10 m vertical resolution from a lunar orbit of 100 km. A prototype model is being constructed of the Lunar Observer Laser Altimeter (LOLA) capable of continuously measuring the range to the lunar surface with sub-meter vertical resolution within a 30 to 300 m diameter surface footprint. This same instrument is also designed to provide a direct measure of the surface height distribution in the footprint by waveform analysis of the backscattered laser pulse. Both these measurements are to be made in a continuous, nadir profile across the lunar surface from a 100 km orbit. The wavelength of the altimeter is 1064 nm. A short-pulse (2 nsec), diode-pumped Nd:YAG laser combined with a 25 cm diameter telescope, silicon avalanche photodiode detector, ranging electronics, and instrument computer was designed to make these measurements and meet all the requirements of the LGO mission.

Bufton, J. L.↗

Low-Temperature Rate Coefficients of C2H with CH4 and CD4 from 154 to 359 K

Rate coefficients for the reaction C2H + CH4 yields C2H2 + CH3 and C2H + CD4 yields C2HD + CD3 are measured over the temperature range 154-359 K using transient infrared laser absorption spectroscopy. Ethynyl radicals are produced by pulsed laser photolysis of C2H2 in a variable temperature flow cell, and a tunable color center laser probes the transient removal of C2H (Chi(exp 2) Sigma(+) (0,0,0)) in absorption. The rate coefficients for the reactions of C2H with CH4 and CD4 both show a positive temperature dependence over the range 154-359 K, which can be expressed as k(sub CH4) = (1.2 +/- 0.1) x 10(exp -11) exp((-491 +/- 12)/T) and k(sub CD4) = (8.7 +/- 1.8) x 10(exp -12) exp((-650 +/- 61)/T) cm(exp 3) molecule(exp -1) s(exp -1), respectively. The reaction of C2H + CH4 exhibits a significant kinetic isotope effect at 300 K of k(sub CH4)/k(sub CD4) = 2.5 +/- 0.2. Temperature dependent rate constants for C2H + C2H2 were also remeasured over an increased temperature range from 143 to 359 K and found to show a slight negative temperature dependence, which can be expressed as k(sub C2H2) = 8.6 x 10(exp -16) T(exp 1.8) exp((474 +/- 90)/T) cm(exp 3) molecule(exp -1) s(exp -1).

Opansky, Brian J.↗

Analysis of the Laser Propelled Lightcraft Vehicle

Advanced propulsion research and technology require launch and space flight technologies, which can drastically reduce mission costs. Laser propulsion is a concept in which energy of a thrust producing reaction mass is supplied via beamed energy from an off-board power source. A variety of laser/beamed energy concepts were theoretically and experimentally investigated since the early 1970's. During the 1980's the Strategic Defense Initiative (SDI) research lead to the invention of the Laser Lightcraft concept. Based upon the Laser Lightcraft concept, the U.S. Air Force and NASA have jointly set out to develop technologies required for launching small payloads into Low Earth Orbit (LEO) for a cost of $1.0M or $1000/lb to $ 100/lb. The near term objectives are to demonstrate technologies and capabilities essential for a future earth to orbit launch capability. Laser propulsion offers the advantages of both high thrust and good specific impulse, I(sub sp), in excess of 1000 s. Other advantages are the simplicity and reliability of the engine because of few moving parts, simpler propellant feed system, and high specific impulse. Major limitations of this approach are the laser power available, absorption and distortion of the pulsed laser beam through the atmosphere, and coupling laser power into thrust throughout the flight envelope, The objective of this paper is to assist efforts towards optimizing the performance of the laser engine. In order to accomplish this goal (1) defocusing of the primary optic was investigated using optical ray tracing and (2), time dependent calculations were conducted of the optically induced blast wave to predict pressure and temperature in the vicinity of the cowl. Defocusing of the primary parabolic reflector causes blurring and reduction in the intensity of the laser ignition site on the cowl. However, because of the caustic effect of ray-tracing optics the laser radiation still forms a well-defined ignition line on the cowl. The blast wave calculations show reasonable agreement with previously published calculations and recent detailed CFD computations.

Feikema, Douglas↗

Analysis of the Laser Lightcraft Vehicle

Advanced propulsion research and technology concepts require launch and space flight technologies, which can drastically reduce mission costs. Laser propulsion is a concept in which energy of a thrust producing reaction mass is supplied via beamed energy from an off-board power source. A variety of laser beamed energy concepts were theoretically and experimentally investigated since the early 1970's. During the 1980's the Strategic Defense Initiative (SDIO) research lead to the invention of the Laser Lightcraft concept. Based upon the Laser Lightcraft concept, the propulsion research center, TD 40, within the Space Transportation Directorate of NASA MSFC has set out to develop technologies required for launching small payloads into Earth Orbit for a cost of $1.0M or $1000/lb to $100/lb. The near term objectives are to demonstrate technologies and capabilities essential for a future earth to orbit launch capability. Laser propulsion offers the advantages of both high thrust and good specific impulse, I(sp) in excess of 1000 s(exp -1). Other advantages are the simplicity and reliability of the engine because of few moving parts; simplistic propellant feed system, and low specific fuel consumption as a result of high specific impulse. Major limitations of this approach are the laser power available, absorption and distortion of the pulsed laser beam through the atmosphere, and coupling laser power into thrust throughout the flight envelope. This summer's effort focused on performance of the laser engine, which included 1) optical ray tracing and 2), a time dependent calculation of the optically induced blast wave.

Feikema, Douglas A.↗

High Output Maximum Efficiency Resonator

A diode pumped, solid state laser is provided that can produce over 16 billion, 15 mJ, 10 ns Q-Switched laser pulses with a low measured decay rate. The laser can be integrated into a global biomass measuring instrument, and mounted on the International Space Station (ISS).

Stysley, Paul R.↗

Laser Sources for Generation of Ultrasound

Two laser systems have been built and used to demonstrate enhancements beyond current technology used for laser-based generation and detection of ultrasound. The first system consisted of ten Nd:YAG laser cavities coupled electronically and optically to permit sequential bursts of up to ten laser pulses directed either at a single point or configured into a phased array of sources. Significant enhancements in overall signal-to-noise ratio for laser ultrasound incorporating this new source system was demonstrated, using it first as a source of narrowband ultrasound and secondly as a phased array source producing large enhanced signal displacements. A second laser system was implemented using ultra fast optical pulses from a Ti:Sapphire laser to study a new method for making laser generated ultrasonic measurements of thin films with thicknesses on the order of hundreds of angstroms. Work by prior investigators showed that such measurements could be made based upon fluctuations in the reflectivity of thin films when they are stressed by an arriving elastic pulse. Research performed using equipment purchased under this program showed that a pulsed interferometric system could be used as well as a piezoreflective detection system to measure pulse arrivals even in thin films with very low piezoreflective coefficients.

Wagner, James W.↗

Tunable diode laser-pumped Tm,Ho:YLF laser operated in continuous-wave and Q-switched modes

Tunable continuous-wave and pulsed laser output was obtained from a Tm-sensitized Ho:YLiF4 crystal at subambient temperatures when longitudinally pumped with a diode laser array. A conversion efficiency of 42 percent and slope efficiency of approximately 60 percent relative to the absorbed pumped power have been achieved at a crystal temperature of 275 K. The emission spectrum was etalon tunable over a range of 16/cm centered at 2067 nm with fine tuning capability of the transition frequency with crystal temperature at measured rate of -0.03/cm/K. Output energies of 0.22 mJ per pulse and 22 ns pulse duration were recorded at Q-switch frequencies that correspond to an effective upper laser level lifetime of 6 ms, and a pulse energy extraction efficiency of 64 percent.

Mcguckin, B. T.↗

Remote sensing of atmospheric pressure and sea state using laser altimeters

Short-pulse multicolor laser ranging systems are currently being developed for satellite ranging applications. These systems use Q-switched pulsed lasers and streak-tube cameras to provide timing accuracies approaching a few picoseconds. Satellite laser ranging systems have been used to evaluate many important geophysical phenomena such as fault motion, polar motion and solid earth tides, by measuring the orbital perturbations of retroreflector equipped satellites. Some existing operational systems provide range resolution approaching a few millimeters. There is currently considerable interest in adapting these highly accurate systems for use as airborne and satellite based altimeters. Potential applications include the measurement of sea state, ground topography and atmospheric pressure. This paper reviews recent progress in the development of multicolor laser altimeters for use in monitoring sea state and atmospheric pressure.

Gardner, C. S.↗

Airborne bathymetric charting using pulsed blue-green lasers

Laboratory and airborne experiments have proven the feasibility and demonstrated the techniques of an airborne pulsed laser system for rapidly mapping coastal water bathymetry. Water depths of 10 plus or minus 0.25 m were recorded in waters having an effective attenuation coefficient of 0.175 m. A 2-MW peak power Nd:YAG pulsed laser was flown at an altitude of 600 m. An advanced system, incorporating a mirror scanner, a high pulsed rate laser, and a good signal processor, could survey coastal zones at the rate of several square miles per hour.

Kim, H. H.↗

Adaptive optics for laser power beaming

It has been proposed to use a high energy pulsed laser to beam power into space for satellites or a lunar base. The effects of atmospheric transmission are critical to such a system. Thermal blooming in the atmosphere can cause the beam to spread rapidly. Atmospheric turbulence can cause beam bending or beam spreading, resulting in the loss of transmitted energy that fails to hit the target receiver.

Leland, Robert P.↗

Relativistically Induced Transparency in Plasma (Final Research Report)

The major goal of this project was to study the process of relativistic transparency in plasmas. This process occurs when a very high intensity laser pulse interacts with a plasma. The electric field of the laser oscillates the electron speeds approaching the speed of light, increasing the effective mass of the electrons by the time-averaged Lorentz factor <γ>. The increase in the effective mass alters the critical density, the density at which the plasma becomes opaque to the electromagnetic wave of the laser. This project used experiments and particle-in-cell simulations to study this process in ultra-thin foil interactions. Experiments were performed through the LaserNetUS program on the Ohio State University laser system Scarlet. The transmitted and reflected light was studied as a function of the target thickness, the near-field profiles, the total energy and pulse duration were measured. Particle-in-cell simulations, using the OSIRIS code were used to model the interaction and better understand the dynamics. The results of both show current relativistic transparency theory is insufficient to predict the results, this is likely because the theories do not account for the laser energy absorption into the target and global plasma fields.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Towards critical and supercritical electromagnetic fields

Abstract The availability of ever stronger, laser-generated electromagnetic fields underpins continuing progress in the study and application of nonlinear phenomena in basic physical systems, ranging from molecules and atoms to relativistic plasmas and quantum electrodynamics. This raises the question: how far will we be able to go with future lasers? One exciting prospect is the attainment of field strengths approaching the Schwinger critical field ${E}_{\mathrm{cr}}$ in the laboratory frame, such that the field invariant ${E}^2-{c}^2{B}^2>{E}_{\mathrm{cr}}^2$ is reached. The feasibility of doing so has been questioned, on the basis that cascade generation of dense electron–positron plasma would inevitably lead to absorption or screening of the incident light. Here we discuss the potential for future lasers to overcome such obstacles, by combining the concept of multiple colliding laser pulses with that of frequency upshifting via a tailored laser–plasma interaction. This compresses the electromagnetic field energy into a region of nanometre size and attosecond duration, which increases the field magnitude at fixed power but also suppresses pair cascades. Our results indicate that laser facilities with peak power of tens of PW could be capable of reaching ${E}_{\mathrm{cr}}$ . Such a scenario opens up prospects for the experimental investigation of phenomena previously considered to occur only in the most extreme environments in the universe.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗