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At least 1,027 records · Page 57

Evaluating Precision of Measured Radionuclide Ambient Air Concentrations

According to AIRNET – Quality Assurance Project Plan for the Radiological Air Sampling Network, SOP-5140, Revision 2 (to become EPC-CP-PIP-5140): “The regulation 40 CFR Part 61.93 requires that the system be able to readily detect a dose of 1.0 mrem above background. Following statistical principles and assuming 95% confidence for such a measurement, we require that 95% of all measurements must fall within two standard deviations of the mean. This represents the minimum acceptable precision for decision making.” An independent assessment of the Rad-NESHAP program completed in early 2019 found that no documentation existed proving that the Airnet data meets the precision defined above. Therefore, to address this particular finding, Airnet concentration data was pulled from the Environmental Information Management (EIM), a cloud-based database maintained by Locus Technologies, for analysis.

54 ENVIRONMENTAL SCIENCES↗

Atomic Oxygen Treatment for Non-Contact Removal of Organic Protective Coatings from Painting Surfaces

Current techniques for removal of varnish (lacquer) and other organic protective coatings from paintings involve contact with the surface. This contact can remove pigment, or alter the shape and location of paint on the canvas surface. A thermal energy atomic oxygen plasma, developed to simulate the space environment in low Earth orbit, easily removes these organic materials. Uniform removal of organic protective coatings from the surfaces of paintings is accomplished through chemical reaction. Atomic oxygen will not react with oxides so that most paint pigments will not be affected by the reaction. For paintings containing organic pigments, the exposure can be carefully timed so that the removal stops just short of the pigment. Color samples of Alizarin Crimson, Sap Green, and Zinc White coated with Damar lacquer were exposed to atomic oxygen. The lacquer was easily removed from all of the samples. Additionally, no noticeable change in appearance was observed after the lacquer was reapplied. The same observations were made on a painted canvas test sample obtained from the Cleveland Museum of Art. Scanning electron microscope photographs showed a slight microscopic texturing of the vehicle after exposure. However, there was no removal or disturbance of the paint pigment on the surface. It appears that noncontact cleaning using atomic oxygen may provide a viable alternative to other cleaning techniques. It is especially attractive in cases where the organic protective surface cannot be acceptably or safely removed by conventional techniques.

Rutledge, Sharon K.↗

BEAM DIAGNOSTICS USING BPM SIGNALS FROM INJECTED AND STORED BEAMS IN A STORAGE RING

Many modern light sources are operating in top-off injection mode or are being upgraded to top-off injection mode. The storage ring always has the stored beam and injected beam for top-off injection mode. So the BPM data is the mixture of both beam positions and the injected beam position cannot be measured directly. We propose to use dedicated wide band BPM electronics in the NSLS II storage ring to retrieve the injected beam trajectory with the singular value decomposition (SVD) method. The beam position monitor (BPM) has the capability to measure bunch-by-bunch beam position. Similar electronics can be used to measure the bunch-by-bunch beam current which is necessary to get the injection beam position. The measurement precision of current needs to be evaluated since button BPM sum signal has position dependence. The injected beam trajectory can be measured and monitored all the time without dumping the stored beam. We can adjust and optimize the injected beam trajectory to maximize the injection efficiency. We can also measure the storage ring acceptance by mapping the injected beam trajectory.

43 PARTICLE ACCELERATORS↗

Measurement of the Drell-Yan Cross Section in $pp$ Collisions at $\sqrt{s}=7$ TeV

The Drell-Yan differential cross section is measured in pp collisions at sqrt(s) = 7 TeV, from a data sample collected with the CMS detector at the LHC, corresponding to an integrated luminosity of 36 inverse picobarns. The cross section measurement, normalized to the measured cross section in the Z region, is reported for both the dimuon and dielectron channels in the dilepton invariant mass range 15-600 GeV. The normalized cross section values are quoted both in the full phase space and within the detector acceptance. The effect of final state radiation is also identified. The results are found to agree with theoretical predictions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Modeling material interfaces with hybrid adhesion method

A molecular dynamics simulation approach is presented to approximate layered material structures using discrete interatomic potentials through classical mechanics and the underlying principles of quantum mechanics. This method isolates the energetic contributions of the system into two pure material layers and an interfacial region used to simulate the adhesive properties of the diffused interface. The strength relationship of the adhesion contribution is calculated through small-scale separation calculations and applied to the molecular surfaces through an inter-layer bond criterion. By segregating the contributions into three regions and accounting for the interfacial excess energies through the adhesive surface bonds, it is possible to model each material with an independent potential while maintaining an acceptable level of accuracy in the calculation of mechanical properties. This method is intended for the atomistic study of the delamination mechanics, typically observed in thin-film applications. Therefore, the work presented in this paper focuses on mechanical tensile behaviors, with observations in the elastic modulus and the delamination failure mode. To introduce the hybrid adhesion method, we apply the approach to an ideal bulk copper sample, where an interface is created by disassociating the force potential in the middle of the structure. Various mechanical behaviors are compared to a standard EAM control model to demonstrate the adequacy of this approach in a simple setting. In addition, we demonstrate the robustness of this approach by applying it on (1) a Cu-Cu 2 O interface with interactions between two atom types, and (2) an Al-Cu interface with two dissimilar FCC lattices. These additional examples are verified against EAM and COMB control models to demonstrate the accurate simulation of failure through delamination, and the formation and propagation of dislocations under loads. Finally, the results conclude that by modeling the energy contributions of an interface using hybrid adhesion bonds, we can provide an accurate approximation method for studies of large-scale mechanical properties, as well as the representation of various delamination phenomena at the atomic scale.

36 MATERIALS SCIENCE↗

A COMPREHENSIVE ANALYSIS OF FERMI GAMMA-RAY BURST DATA. III. ENERGY-DEPENDENT T {sub 90} DISTRIBUTIONS OF GBM GRBs AND INSTRUMENTAL SELECTION EFFECT ON DURATION CLASSIFICATION

The durations (T {sub 90}) of 315 gamma-ray bursts (GRBs) detected with Fermi/GBM (8-1000 keV) up to 2011 September are calculated using the Bayesian Block method. We compare the T {sub 90} distributions between this sample and those derived from previous/current GRB missions. We show that the T {sub 90} distribution of this GRB sample is bimodal, with a statistical significance level comparable to those derived from the BeppoSAX/GRBM sample and the Swift/BAT sample, but lower than that derived from the CGRO/BATSE sample. The short-to-long GRB number ratio is also much lower than that derived from the BATSE sample, i.e., 1:6.5 versus 1:3. We measure T {sub 90} in several bands, i.e., 8-15, 15-25, 25-50, 50-100, 100-350, and 350-1000 keV, to investigate the energy-dependence effect of the bimodal T {sub 90} distribution. It is found that the bimodal feature is well observed in the 50-100 and 100-350 keV bands, but is only marginally acceptable in the 25-50 keV and 350-1000 keV bands. The hypothesis of bimodality is confidently rejected in the 8-15 and 15-25 keV bands. The T {sub 90} distributions in these bands are roughly consistent with those observed by missions with similar energy bands. The parameter T {sub 90} as a function of energy follows T-bar {sub 90}{proportional_to}E{sup -0.20{+-}0.02} for long GRBs. Considering the erratic X-ray and optical flares, the duration of a burst would be even longer for most GRBs. Our results, together with the observed extended emission of some short GRBs, indicate that the central engine activity timescale would be much longer than T {sub 90} for both long and short GRBs and the observed bimodal T {sub 90} distribution may be due to an instrumental selection effect.

79 ASTRONOMY AND ASTROPHYSICS↗

Parsec-scale Properties of Steep- and Flat-spectrum Extragalactic Radio Sources from a VLBA Survey of a Complete North Polar Cap Sample

We observed with the Very Long Baseline Array (VLBA) at 2.3 and 8.6 GHz a complete flux-density-limited sample of 482 radio sources with decl. > +75° brighter than 200 mJy at 1.4 GHz drawn from the NVSS catalog. A total of 34% of the sources show parsec-scale emission above the flux density detection limit of 30 mJy; their accurate positions and parsec-scale structure parameters are determined. Among all the sources detected at least at the shortest VLBA baselines, the majority, or 72%, have a steep single-dish spectrum. The fraction of the sources with a detectable parsec-scale structure is above 95% among the flat-spectrum objects and close to 25% among the steep-spectrum objects. We identified 82 compact steep-spectrum source candidates, which make up 17% of the sample; most of them are reported for the first time. The compactness and the brightness temperature of the sources in our sample show a positive correlation with single-dish and VLBA spectral indices. All the sources with a significant 8 GHz variability were detected by the VLBA snapshot observations, which independently confirmed their compactness. We demonstrated that 54% of the sources detected by the VLBA at 2.3 GHz in our sample have a steep VLBA spectrum. The compact radio emission of these sources is likely dominated by optically thin jets or mini-lobes, not by an opaque jet core. These results show that future VLBI surveys aimed at searching for new sources with parsec-scale structure should include not only flat-spectrum sources but also steep-spectrum ones in order to reach an acceptable level of completeness.

47 OTHER INSTRUMENTATION↗

The simultaneous determination of 20 trace elements in terrestrial, lunar and meteoritic material by radiochemical neutron activation analysis

A radiochemical neutron activation method has been developed and applied to determine the content of 20 trace elements (Ag, Au, Bi, Br, Cd, Co, Cs, Cu, Ga, Ge, In, Ir, Ni, Rb, Re, Sb, Te, Tl, and Zn) in 45 terrestrial, 230 lunar, and 70 meteoritic samples. Results obtained for the U.S.G.S. standard basalt BCR-1 indicate that the inherent precision for most elements is 10% or better. The values obtained for the trace elements investigated are compared to those previously reported in the literature. Data for Type I carbonaceous chondrites show their compositions to be far more uniform than previously supposed. The values obtained for several elements represent significant revisions in the accepted cosmic abundances. These new values include: Zn, 1250; Cd, 1.51; and Ir, 0.72 atoms/million Si atoms. Further results have provided insight into the meteoritic material and accretion of the moon, and give evidence of lunar highland vulcanism.

Keays, R. R.↗

Spectroscopy of neutral-colored QSO candidates

Spectroscopic observations of 21 QSO candidates are discussed; the candidates were taken mainly from sets of objects described as neutral colored that have been listed as possible identifications of radio sources. Candidate identifications are accepted for study without color discrimination (that is, neutral-colored and even reddish objects are examined) in the hope of removing possible bias against finding QSOs with z greater than approximately 3.5. The largest redshift among the objects described here, however, is z = 2.43. The observations therefore support the tentative conclusion that the decline in numbers of objects with z greater than approximately 3 among these samples is real.

Baldwin, J. A.↗

Parsec-scale Properties of Steep- and Flat-spectrum Extragalactic Radio Sources from a VLBA Survey of a Complete North Polar Cap Sample

We observed with the Very Long Baseline Array (VLBA) at 2.3 and 8.6 GHz a complete flux-density-limited sample of 482 radio sources with decl. > +75° brighter than 200 mJy at 1.4 GHz drawn from the NVSS catalog. A total of 34% of the sources show parsec-scale emission above the flux density detection limit of 30 mJy; their accurate positions and parsec-scale structure parameters are determined. Among all the sources detected at least at the shortest VLBA baselines, the majority, or 72%, have a steep single-dish spectrum. The fraction of the sources with a detectable parsec-scale structure is above 95% among the flat-spectrum objects and close to 25% among the steep-spectrum objects. We identified 82 compact steep-spectrum source candidates, which make up 17% of the sample; most of them are reported for the first time. The compactness and the brightness temperature of the sources in our sample show a positive correlation with single-dish and VLBA spectral indices. All the sources with a significant 8 GHz variability were detected by the VLBA snapshot observations, which independently confirmed their compactness. We demonstrated that 54% of the sources detected by the VLBA at 2.3 GHz in our sample have a steep VLBA spectrum. The compact radio emission of these sources is likely dominated by optically thin jets or mini-lobes, not by an opaque jet core. These results show that future VLBI surveys aimed at searching for new sources with parsec-scale structure should include not only flat-spectrum sources but also steep-spectrum ones in order to reach an acceptable level of completeness.

A V Popkov↗

TEMPORAL CORRELATIONS BETWEEN OPTICAL AND GAMMA-RAY ACTIVITY IN BLAZARS

We have been using the 0.76 m Katzman Automatic Imaging Telescope (KAIT) at Lick Observatory to optically monitor a sample of 157 blazars that are bright in gamma-rays being detected with high significance (≥10σ) in one year by the Large Area Telescope (LAT) on the Fermi Gamma-ray Space Telescope. We attempt to observe each source on a three-day cadence with KAIT, subject to weather and seasonal visibility. The gamma-ray coverage is essentially continuous. KAIT observations extend over much of the five-year Fermi mission for several objects, and most have >100 optical measurements spanning the last three years. These blazars (flat-spectrum radio quasars and BL Lac objects) exhibit a wide range of flaring behavior. Using the discrete correlation function (DCF), here we search for temporal relationships between optical and gamma-ray light curves in the 40 brightest sources in hopes of placing constraints on blazar acceleration and emission zones. We find strong optical-gamma-ray correlation in many of these sources at time delays of ∼1 to ∼10 days, ranging between –40 and +30 days. A stacked average DCF of the 40 sources verifies this correlation trend, with a peak above 99% significance indicating a characteristic time delay consistent with 0 days. These findings strongly support the widely accepted leptonic models of blazar emission. However, we also find examples of apparently uncorrelated flares (optical flares with no gamma-ray counterpart and gamma-ray flares with no optical counterpart) that challenge simple, one-zone models of blazar emission. Moreover, we find that flat-spectrum radio quasars tend to have gamma-rays leading the optical, while intermediate- and high-synchrotron peak blazars with the most significant peaks have smaller lags/leads. It is clear that long-term monitoring at high cadence is necessary to reveal the underlying physical correlation.

79 ASTRONOMY AND ASTROPHYSICS↗

Activity measurement of Fe 60 through the decay of Co 60 m and confirmation of its half-life

The half-life of the neutron-rich nuclide, 60Fe has been in dispute in recent years. A measurement in 2009 published a value of (2.62 ± 0.04) × 106 years, almost twice that of the previously accepted value from 1984 of (1.49 ± 0.27) × 106 years. This longer half-life was confirmed in 2015 by a second measurement, resulting in a value of (2.50 ± 0.12) × 106 years. All three half-life measurements used the grow-in of the γ-ray lines in 60Ni from the decay of the ground state of 60Co (t1/2=5.27 years) to determine the activity of a sample with a known number of 60Fe atoms. In contrast, the work presented here measured the 60Fe activity directly via the 58.6 keV γ-ray line from the short-lived isomeric state of 60Co (t1/2=10.5 minutes), thus being independent of any possible contamination from long-lived 60gCo. A fraction of the material from the 2015 experiment with a known number of 60Fe atoms was used for the activity measurement, resulting in a half-life value of (2.72 ± 0.16) × 106 years, confirming again the longer half-life. In addition, 60Fe/56Fe isotopic ratios of samples with two different dilutions of this material were measured with Accelerator Mass Spectrometry (AMS) to determine the number of 60Fe atoms. Combining this with our activity measurement resulted in a half-life value of (2.69 ± 0.28) × 106 years, again agreeing with the longer half-life.

Ostdiek, Karen M.↗

A simplified technique for delivering total body irradiation (TBI) with improved dose homogeneity

Purpose: Total body irradiation (TBI) with megavoltage photon beams has been accepted as an important component of management for a number of hematologic malignancies, generally as part of bone marrow conditioning regimens. The purpose of this paper is to present and discuss the authors' TBI technique, which both simplifies the treatment process and improves the treatment quality. Methods: An AP/PA TBI treatment technique to produce uniform dose distributions using sequential collimator reductions during each fraction was implemented, and a sample calculation worksheet is presented. Using this methodology, the dosimetric characteristics of both 6 and 18 MV photon beams, including lung dose under cerrobend blocks was investigated. A method of estimating midplane lung doses based on measured entrance and exit doses was proposed, and the estimated results were compared with measurements. Results: Whole body midplane dose uniformity of {+-}10% was achieved with no more than two collimator-based beam modulations. The proposed model predicted midplane lung doses 5% to 10% higher than the measured doses for 6 and 18 MV beams. The estimated total midplane doses were within {+-}5% of the prescribed midplane dose on average except for the lungs where the doses were 6% to 10% lower than the prescribed dose on average. Conclusions: The proposed TBI technique can achieve dose uniformity within {+-}10%. This technique is easy to implement and does not require complicated dosimetry and/or compensators.

61 RADIATION PROTECTION AND DOSIMETRY↗

Draft report on melt point as a function of composition for urania-based systems

This report documents the testing of a urania (UO 2.00 ) sample as a baseline and the attempt to determine the melt point associated with 4 compositions of urania-ceria and urania-neodymia pseudo binaries provided by ORNL, with compositions of 95/5, and 80/20 and of (U/Ce)O 2.00 and (U/Nd)O 2.00 in the newly developed ceramic melt point determination system. A redesign of the system using parts fabricated from tungsten was undertaken in order to help prevent contamination and tungsten carbide formation in the crucibles. The previously developed system employed mostly graphite parts that were shown to react with the sample containment black-body crucible leading to unstable temperature readings and crucible failure, thus the redesign. Measured melt point values of UO 2.00 and U 0.95 Ce 0.05 O 2.00 , U 0.80 Ce 0.20 O 2.00 , U 0.95 Nd 0.05 O 2.00 and U 0.80 Nd 0.20 O 2.00 were measured using a 2-color pyrometer. The value measured for UO 2.00 was consistent with the published accepted value 2845°C±25°C, although a wide range of values has been published by researchers and will be discussed later in the text. For comparison, values obtained from a published binary phase diagram of UO 2 -Nd 2 O 3 were used for comparison with our measure values. No literature melt point values for comparison with the measurements performed in this study were found for (U/Ce)O 2.00 in our stoichiometry range.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Initial Radiation of Nuclear Power Plant Components (CRADA NFE-17-06892 Final Report)

As advanced reactor concepts are developed, instrumentation and control (I&C) cables and sensors will play a significant role in assuring their operation is well understood, and safety-related process information can be collected reliably over the course of their design life. As a first step to develop acceptance criteria and define the limits of currently available nuclear I&C cable and sensor technology, a collaboration between Oak Ridge National Laboratory and Analysis and Measurement Services (AMS) Corporation was initiated under the Gateway for Accelerated Innovation in Nuclear (GAIN) Program. This collaborative effort focused on providing technical information related to the combined thermal and radiation aging of nuclear power plant (NPP) cables, companion NPP cable insulation samples, and two prototype temperature and two pressure sensors. This work was carried out using the instrumented gamma irradiation system that is part of the High Flux Isotope Reactor Gamma Irradiation Facility (HFIR GIF). This system provided the opportunity for the condition of the prototype sensors to be tracked during the irradiation in order to determine their functional limits with greater granularity when compared to a simple irradiation insertion at the HFIRGIF. Experimental assemblies for sensor irradiation were successfully completed, and sensor irradiation to accumulated dose of 3000 kGy at a rate of approximately 6 kGy/hr was carried out. Two prototype temperature assemblies were continuously monitored during exposure to 3000 kGy and found to have no observable degradation from the irradiation. Two pressure sensors were first irradiated to 1000 kGy. At which point, one of the sensors was found to operate normally; however, a second sensor failed the operability test. The operable pressure sensor output was then continuously monitored from 1000 kGy to 3000 kGy. The sensor output exhibited steady trendable drift versus the accumulated radiation dose. At the conclusion of the irradiation, the four test sensors were released for laboratory calibration checks. The calibration check of the temperature sensors found no significant change after irradiation compared to baseline measurements before irradiation; however, both pressure sensors failed the post-test calibration checks and both sensors were not functioning properly. These results will help inform sensor manufacturers and I&C design engineers of potential limitations of these types of sensors for use in high radiation environments associated with the compact configuration of new Small Modular Reactors (SMRs) such as NuScale’s reactor power module. Irradiations on NPP cables and companion samples were not completed due to programmatic delays, however a path forward that was based on lessons learned from this project was defined to accommodate future, comparable instrumented gamma irradiations at the HFIR GIF.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Self-consistent Color–Stellar Mass-to-light Ratio Relations for Low Surface Brightness Galaxies

The color–stellar mass-to-light ratio relation (CMLR) is a widely accepted tool for estimating the stellar mass (M {sub *}) of a galaxy. However, an individual CMLR tends to give distinct M {sub *} for a same galaxy when it is applied in different bands. Examining five representative CMLRs from the literature, we find that the difference in M {sub *} predicted in different bands from optical to near-infrared by a CMLR is 0.1 ∼ 0.3 dex. Based on a sample of low surface brightness galaxies that covers a wide range of color and luminosity, we therefore recalibrated each original CMLR in r, i, z, J, H, and K bands to give internally self-consistent M {sub *} for a same galaxy. The g–r is the primary color indicator in the recalibrated relations, which show little dependence on red (r–z) or near-infrared (J–K) colors. Additionally, the external discrepancies in the originally predicted γ {sub *} by the five independent CMLRs have been greatly reduced after recalibration, especially in the near-infrared bands, implying that the near-infrared luminosities are more robust in predicting γ {sub *}. For each CMLR, the recalibrated relations provided in this work could produce internally self-consistent M {sub *} from divergent photometric bands, and are extensions of the recalibrations from the Johnson–Cousin filter system by the pioneering work of McGaugh & Schombert to the filter system of the Sloan Digital Sky Survey.

79 ASTRONOMY AND ASTROPHYSICS↗

Polycyclic Aromatic Hydrocarbon Emission in Spitzer /IRS Maps. II. A Direct Link between Band Profiles and the Radiation Field Strength

We decompose the observed 7.7 μ m polycyclic aromatic hydrocarbon (PAH) emission complexes in a large sample of over 7000 mid-infrared spectra of the interstellar medium using spectral cubes observed with the Spitzer /IRS-SL instrument. In order to fit the 7.7 μ m PAH emission complex we invoke four Gaussian components, which are found to be very stable in terms of their peak positions and widths across all of our spectra, and subsequently define a decomposition with fixed parameters, which gives an acceptable fit for all the spectra. We see a strong environmental dependence on the interrelationships between our band fluxes—in the H ii regions all four components are intercorrelated, while in the reflection nebulae (RNs) the inner and outer pairs of bands correlate in the same manner as previously seen for NGC 2023. We show that this effect arises because the maps of RNs are dominated by emission from strongly irradiated photodissociation regions, while the much larger maps of H ii regions are dominated by emission from regions much more distant from the exciting stars, leading to subtly different spectral behavior. Further investigation of this dichotomy reveals that the ratio of two of these components (centered at 7.6 and 7.8 μ m) is linearly related to the UV-field intensity (log G {sub 0}). We find that this relationship does not hold for sources consisting of circumstellar material, which are known to have variable 7.7 μ m spectral profiles.

79 ASTRONOMY AND ASTROPHYSICS↗

Mineralogical diversity (spectral reflectance and Moessbauer data) in compositionally similar impact melt rocks from Manicouagan Crater, Canada

Meteoritic impacts under oxidizing surface conditions occur on both earth and Mars. Oxidative alteration of impact melt sheets is reported at several terrestrial impact structures including Manicouagan, West Clearwater Lake, and the Ries Basin. A number of studies have advocated that a significant fraction of Martian soil may consist of erosional products of oxidatively altered impact melt sheets. If so, the signature of the Fe-bearing mineralogies formed by the process may be present in visible and near infrared reflectivity data for the Martian surface. Of concern is what mineral assemblages form in impact melt sheets produced under oxidizing conditions and what their spectral signatures are. Spectral and Moessbauer data for 19 powder samples of impact melt rock from Manicouagan Crater are reported. Results show for naturally occurring materials that composite hematite-pyroxene bands have minima in the 910-nm region. Thus many of the anomalous Phobos-2 spectra, characterized by a shallow band minimum in the near-IR whose position varies between approximately 850 and 1000 nm, can be explained by assemblages whose endmembers (hematite and pyroxene) are accepted to be present on Mars. Furthermore, results show that a mineralogically diverse suite of rocks can be generated at essentially constant composition, which implies that variations in Martian surface mineralogy do not necessarily imply variations in chemical composition.

Morris, R. V.↗