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At least 1,045 records · Page 58

Sub-Sampled Imaging for STEM: Maximising Image Speed, Resolution and Precision Through Reconstruction Parameter Refinement

Sub-sampling during image acquisition in scanning transmission electron microscopy (STEM) has been shown to provide a means to increase the overall speed of acquisition while at the same time providing an efficient means to control the dose, dose rate and dose overlap delivered to the sample. In this paper, we discuss specifically the parameters used to reconstruct sub-sampled images and highlight their effect on inpainting using the beta-process factor analysis (BPFA) methodology. The selection of the main control parameters can have a significant effect on the resolution, precision and sensitivity of the final inpainted images, and here we demonstrate a method by which these parameters can be optimised for any image in STEM. As part of this paper, we also provide a link to open source code and a tutorial on its use, whereby these parameters can be tested for any datasets. When coupled with the hardware necessary to rapidly sub-sample images in STEM, this approach can have significant implications for imaging beam sensitive materials and dynamic processes.

47 OTHER INSTRUMENTATION↗

Formation of Benzene and Naphthalene through Cyclopentadienyl-Mediated Radical–Radical Reactions

Resonantly stabilized free radicals (RSFRs) have been contemplated as fundamental molecular building blocks and reactive intermediates in molecular mass growth processes leading to polycyclic aromatic hydrocarbons (PAHs) and carbonaceous nanoparticles on Earth and in deep space. Here, by combining molecular beams and computational fluid dynamics simulations, we provide compelling evidence on the formation of benzene via the cyclopentadienyl-methyl reaction and of naphthalene through the cyclopentadienyl self-reaction, respectively. These systems offer benchmarks for the conversion of a five-membered ring to the 6π-aromatic (benzene) and the generation of the simplest 10π-PAH (naphthalene) at elevated temperatures. These results uncover molecular mass growth processes from the “bottom up” via RSFRs in high temperature circumstellar environments and combustion systems expanding our fundamental knowledge of the organic, hydrocarbon chemistry in our universe.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Electrostatic and aerodynamic forced vibrations of a thin flexible electrode: Quasi-periodic vs. chaotic oscillations

In this paper, transverse vibrations of an electrostatically actuated thin flexible cantilever perturbed by low-speed air flow are studied using both experiments and numerical modeling. In the experiments, the dynamic characteristics of the cantilever are studied by supplying a DC voltage with an AC component for electrostatic forcing and a constant uniform air flow around the cantilever system for aerodynamic forcing. A range of control parameters leading to stable vibrations are established using a dimensionless operating parameter that is the ratio of the induced and the free stream velocities. Numerical results are validated with experimental data. Assuming the amplitude of vibrations are small, then a non-linear dynamic Euler-Bernoulli beam equation with viscous damping and gravitational effects is used to model the equation of motion. Aerodynamic forcing is modelled as a temporally sinusoidal and uniform force acting perpendicular to the beam length. The forcing amplitude is found to be proportional to the square of the air flow velocity. Numerical results strongly agree with the experiments predicting accurate vibration amplitude, displacement frequency, and quasi-periodic displacement of the cantilever tip.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Deterministic scattering of relativistic electron beams by off-resonant circularly polarized electromagnetic waves

A mechanism is presented whereby relativistic electron beams localized in phase space are deterministically scattered by coherent circularly polarized electromagnetic waves without stochastic processes. It is shown via an exact single-particle analysis that the condition for maximal scattering is an off-resonant condition, contrary to previous kinetic analyses that predict maximal diffusion or interaction at exact resonance or its harmonics. The mechanism, verified by single-particle simulations, enables a fast, nonlinear redistribution of the beam particles. A possible application of this mechanism to runaway electron suppression is presented.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Development of a wide bandwidth heterodyne dispersion interferometer for electron density measurement of atmospheric pressure plasmas

One of the challenges of electron density measurements of an atmospheric pressure plasma (APP) with a laser interferometer is the significant and unwanted phase shift caused by changes in the neutral gas density. These unwanted phase shifts can be mitigated and plasma density measured using an interferometer architecture called a dispersion interferometer (DI). A DI is composed of two nonlinear orientation patterned GaAs crystals for frequency doubling and measures the phase shift induced by a plasma in the interference signal between two second-harmonic beams. Measurement of plasma dynamics or a short plasma pulse in less than a millisecond is enabled with heterodyne detection in a DI using an acousto-optic cell with a frequency of 40 MHz. This heterodyne DI (HDI) is targeted to measure APPs in an electron density range of 10 20 –10 24 m −3 . Finally, the HDI achieves a line-integrated density resolution of 2 × 10 15 m −2 (a phase resolution of 0.005°) with a time constant of 1 μs using ensemble averaging techniques.

atmospheric pressure plasma↗

Precise determination of the deuteron spin structure at low to moderate Q 2 with CLAS and extraction of the neutron contribution

In this study, we present the final results for the deuteron spin structure functions obtained from the full data set collected with Jefferson Lab's CLAS in 2000-2001. Polarized electrons with energies of 1.6, 2.5, 4.2 and 5.8 GeV were scattered from deuteron ( 15 ND 3 ) targets, dynamically polarized along the beam direction, and detected with CLAS. From the measured double spin asymmetry, the virtual photon absorption asymmetry A d 1 and the polarized structure function g d 1 were extracted over a wide kinematic range (0.05 GeV2 < Q2 < 5 GeV2 and 0.9 GeV < W < 3 GeV). We use an unfolding procedure and a parametrization of the corresponding proton results to extract from these data the polarized structure functions A n 1 and g 1 n of the (bound) neutron, which are so far unknown in the resonance region, W < 2 GeV. We compare our final results, including several moments of the deuteron and neutron spin structure functions, with various theoretical models and expectations as well as parametrizations of the world data. The unprecedented precision and dense kinematic coverage of these data can aid in future extractions of polarized parton distributions, tests of perturbative QCD predictions for the quark polarization at large x, a better understanding of quark-hadron duality, and more precise values for higher-twist matrix elements in the framework of the Operator Product Expansion.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Determination of the proton spin structure functions for 0.05 < Q 2 < 5 GeV 2 using CLAS

In this work, we present the results of our final analysis of the full data set of g$p\atop{1}$ (Q 2 ), the spin structure function of the proton, collected using CLAS at Jefferson Laboratory in 2000–2001. Polarized electrons with energies of 1.6, 2.5, 4.2, and 5.7 GeV were scattered from proton targets ( 15 NH 3 dynamically polarized along the beam direction) and detected with CLAS. From the measured double spin asymmetries, we extracted virtual photon asymmetries A$p\atop{1}$ and A$p\atop{2}$ and spin structure functions g$p\atop{1}$ and g$p\atop{2}$ over a wide kinematic range (0.05 GeV 2 < Q 2 < 5 GeV 2 and 1.08 GeV < W < 3 GeV) and calculated moments of g$p\atop{1}$. We compare our final results with various theoretical models and expectations, as well as with parametrizations of the world data. Lastly, our data, with their precision and dense kinematic coverage, are able to constrain fits of polarized parton distributions, test pQCD predictions for quark polarizations at large x, offer a better understanding of quark-hadron duality, and provide more precise values of higher twist matrix elements in the framework of the operator product expansion.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Rheology of concentrated fiber suspensions with a load-dependent friction coefficient

Here we investigate the effects of fiber aspect ratio, roughness, flexibility, and volume fraction on the rheology of concentrated suspensions in a steady shear flow using direct numerical simulations. We model the fibers as inextensible continuous flexible slender bodies with the Euler-Bernoulli beam equation governing their dynamics suspended in an incompressible Newtonian fluid. The fiber dynamics and fluid flow coupling is achieved using the immersed boundary method. In addition, the fiber surface roughness might lead to interfiber contacts, resulting in normal and tangential forces between the fibers, which follow Coulomb’s law of friction. The surface roughness is modeled as hemispherical protrusions on the fiber surfaces. Their deformation results in a normal load-dependent friction coefficient. Our simulations accurately predict the experimentally observed shear thinning in fiber suspensions. Furthermore, we find that the suspension viscosity η increases with increasing the volume fraction, roughness, fiber rigidity, and aspect ratio. The increase in η is the macroscopic manifestation of a similar increase in the microscopic contact contribution to the total stress with these parameters. In addition, we observe positive and negative first N 1 and second N 2 normal stress differences, respectively, with |N 2 | < |N 1 |, in agreement with previous experiments. Last, we propose a modified Maron-Pierce law to quantify the reduction in the jamming volume fraction by increasing the fiber aspect ratio and roughness. Our results and analysis establish the use of fiber surface tribology to tune the suspension flow behavior.

42 ENGINEERING↗

High-viscosity injector-based pink-beam serial crystallography of microcrystals at a synchrotron radiation source

Since the first successful serial crystallography (SX) experiment at a synchrotron radiation source, the popularity of this approach has continued to grow showing that third-generation synchrotrons can be viable alternatives to scarce X-ray free-electron laser sources. Synchrotron radiation flux may be increased ∼100 times by a moderate increase in the bandwidth (`pink beam' conditions) at some cost to data analysis complexity. Here, we report the first high-viscosity injector-based pink-beam SX experiments. The structures of proteinase K (PK) and A 2A adenosine receptor (A 2A AR) were determined to resolutions of 1.8 and 4.2 Å using 4 and 24 consecutive 100 ps X-ray pulse exposures, respectively. Strong PK data were processed using existing Laue approaches, while weaker A 2A AR data required an alternative data-processing strategy. This demonstration of the feasibility presents new opportunities for time-resolved experiments with microcrystals to study structural changes in real time at pink-beam synchrotron beamlines worldwide.

36 MATERIALS SCIENCE↗

Modeling Variable-Impedance, Magnetically Insulated, Transmission Lines

Coupling generator current to electron-beam loads and dynamic-inductance loads (z pinches) is greatly improved with low-inductance vacuum transmission lines. Typically, magnetically insulated transmission lines (MITLs) utilize nearly constant impedance geometries where the minimum impedance (anode-cathode gap) is limited by electron loss during the setup of magnetic insulation. Constant-impedance MITL designs are not optimized for low inductance (Zτ) when given a constraint on vacuum electron flow. We describe the design and the modeling of MITLs that have a nonconstant impedance. The baseline variable-impedance MITL designs are based on equilibrium vacuum-electron flow models [1] that are incorporated into the Screamer circuit code [2]. Such designs satisfy the MITL limits in the areal density of the loss current and have magnetically insulated flow that is stable everywhere along the MITL. Different MITL designs are then modeled analytically and with a 2-D particle-in-cell computer code in order to quantify subtle electron losses driven by changes to the vacuum impedance as a function of distance along the transmission line. We present a variable-impedance MITL design that delivers more current with a lower inductance than found in constant-impedance MITL designs.

47 OTHER INSTRUMENTATION↗

Verification of R-matrix calculations for charged-particle reactions in the resolved resonance region for the 7 Be system

R-matrix theory is used to present nuclear reactions in the resolved resonance region. It uses information on bound states and low energy resonances to accurately parametrize cross sections on the resonances as well as the non-resonant background. Since the seminal work of Lane and Thomas (1958), the method has been widely used to analyze experimental cross-section data in a broad range of fields spanning nuclear reaction dynamics, nuclear astrophysics, ion beam analysis and their applications. Different R-matrix codes have been developed and used in these different applications with very little communication among the developers or practitioners on the capabilities, achievements or limitations of the codes. A limited comparison among three R-matrix codes on neutron-induced reactions was performed by the International Atomic Energy Agency (IAEA) International Evaluation of Neutron Cross Section Standards project (2007). Since then, significant progress has been made in their implementation of the R-matrix algorithms, and R-matrix codes have enhanced capabilities. In this paper we introduce, for the first time, the results of a comprehensive effort to verify the most widely used R-matrix codes in the various fields of nuclear science and applications: AMUR, AZURE2, CONRAD, EDA, FRESCO, GECCCOS, and SAMMY. In addition to the description of the capabilities of the codes and their specifications, we discuss the results of a joint exercise which was coordinated by the International Atomic Energy Agency. The aim of the exercise was to compare calculations of charged-particle reaction cross sections for the light composite system 7Be. The calculations were performed by the codes using identical input R-matrix parameters and other specifications and were limited to charged-particle channels.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Centrality dependence of charged jet production in p–Pb collisions at $\sqrt{s_\mathrm{NN}}$ = 5.02 TeV

Measurements of charged jet production as a function of centrality are presented for p–Pb collisions recorded at $\sqrt{s_\mathrm{NN}}$= 5.02 TeV with the ALICE detector. Centrality classes are determined via the energy deposit in neutron calorimeters at zero degree, close to the beam direction, to minimise dynamical biases of the selection. The corresponding number of participants or binary nucleon–nucleon collisions is determined based on the particle production in the Pb-going rapidity region. Jets have been reconstructed in the central rapidity region from charged particles with the anti-k T algorithm for resolution parameters R = 0.2 and R = 0.4 in the transverse momentum range 20 to 120 GeV/c. The reconstructed jet momentum and yields have been corrected for detector effects and underlying-event background. In the five centrality bins considered, the charged jet production in p–Pb collisions is consistent with the production expected from binary scaling from pp collisions. The ratio of jet yields reconstructed with the two different resolution parameters is also independent of the centrality selection, demonstrating the absence of major modifications of the radial jet structure in the reported centrality classes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Dark Field Proton Radiography (Los Alamos LDRD Report)

Proton radiography at LANL (pRad) takes advantage of the high flux, high proton energy, and flexible timing structure of LANSCE's 800-MeV proton beam to visualize dense, dynamic systems under extreme strain. With recent needs identified for the development of the W93, the pRad team has been actively searching for ways to increase the facility's radiographic capabilities. Recently, we discovered that utilizing two magnetic lenses (one upstream and one downstream of the object), and specific combinations of collimator choices within the two lenses, that the signal-to-noise ratio was improved by more than a factor of two. However, we did not fully understand the mechanism, and found that results did not match forward modeling predictions. This work specifically sought to implement an engineering solution to solve this problem, through the development of an actuated collimator that reduced the time required to swap collimator settings from a typical 4-8 hours, to less than 30 seconds. This allowed, in combination with a unique multi-material, multi-resolution stepwedge, to acquire an unprecedently enormous dataset, with in total 24 collimation combinations, and multiple diffuser settings and pulse patterns, equivalent to almost a full run cycle's worth of data in a few days. This massive dataset is currently being harnessed to make a fully-predictive, ultra-fast Python-based model of the system, to dial in specific settings for any future experiments that fully optimize that radiographic sensitivity to the material of interest.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Electron dynamics and energy conversion in O-type linear-beam devices.

A general nonlinear interaction theory is used to investigate the effects of transverse fields (i.e., radial circuit fields and radial space-charge fields) in traveling-wave amplifiers for a variety of beam-focusing conditions. Magnetic focusing fields which are periodic or tapered (increased) with distance along the device are considered in addition to uniform magnetic fields. Results are presented for Brillouin flow and near-Brillouin flow, and the minimum magnetic field strength required to effectively constrain the electron beam is determined as a function of the operating parameters for the various focusing systems. Confined flow is also examined for the uniform-field case in order to have a basis of comparison from which the effects of radial motion of the beam electrons can be determined. The results indicate the importance of transverse effects and further yield information on the stability of strongly modulated cylindrical electron beams.-

Detweiler, H. K.↗

Nonlinear dynamics; Proceedings of the International Conference, New York, NY, December 17-21, 1979

Papers were presented on turbulence, ergodic and integrable behavior, chaotic maps and flows, chemical and fully developed turbulence, and strange attractors. Specific attention was given to measures describing a turbulent flow, stochastization and collapse of vortex systems, a subharmonic route to turbulent convection, and weakly nonlinear turbulence in a rotating convection layer. The Korteweg-de Vries and Hill equations, plasma transport in three dimensions, a horseshoe in the dynamics of a forced beam, and the explosion of strange attractors exhibited by Duffing's equation were also considered.

Helleman, R. H. G.↗

Impact dynamics research on composite transport structures

The experimental and analytical efforts being undertaken to investigate the response of composite and aluminum structures under crash loading conditions were reviewed. A Boeing 720 airplane was used in the controlled-impact demonstration test. Energy absorption of composite materials, the tearing of fuselage skin panels, the friction and abrasion behavior of composite skins, and the crushing behavior and dynamic response of composite beams were among the topics addressed.

Carden, H. D.↗