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At least 1,063 records · Page 59

Design and Testing of a Prototype Electrodynamic Regolith Conveyor for Lunar ISRU

NASA’s Swamp Works Electrostatics and Surface Physics Laboratory (ESPL) is developing a 4-phaseelectrodynamic regolith conveyor (ERC) that could convey regolith without the risk of rotating or vibratory actuation, which could jam or require regular maintenance due to the abrasive nature of lunar regolith. Another goal of electrodynamic conveying is the reduction of conveying power, which is important considering the limited capacity of early-stage lunar power systems. The current state of the art(SOA) for lunar regolith conveying is based on recent NASA system studies for oxygen production plants. These plant designs require conveying rates around 100 kg/hr, to produce 10 mT/yr of oxygen from the regolith. To accomplish this, conventional augers and vibratory spiral conveyors have been identified as the SOA or the leading candidates due to their extensive use in the terrestrial material handling industry. At NASA KSC, the use of dynamic electric fields, generated by alternating high voltage on electrodes, has been developed as a dust mitigation solution known as the Electrodynamic Dust Shield (EDS). The EDS is being developed for lenses, solar panels, radiators, fabric and seals and is scheduled for a technology demonstration mission on the Moon in 2023. ESPL researchers have shown the ability to move thin layers (~ a few mm) of dust with mW of power. In Academia, researchers have shown the ability to electrodynamically convey regolith up to ~1 kg/hr with a 4-phase EDS and electromagnetically convey particles that would suggest a lunar regolith conveying rate of ~25 kg/hr. This paper will describe the design and testing of a prototype ERC that could scale to support transporting regolith at ISRU relevant flow rates.

Aaron D S Olson↗

Spent nuclear fuel recycling with plasma reduction and etching

A method of extracting uranium from spent nuclear fuel (SNF) particles is disclosed. Spent nuclear fuel (SNF) (containing oxides of uranium, oxides of fission products (FP) and oxides of transuranic (TRU) elements (including plutonium)) are subjected to a hydrogen plasma and a fluorine plasma. The hydrogen plasma reduces the uranium and plutonium oxides from their oxide state. The fluorine plasma etches the SNF metals to form UF 6 and PuF 4 . During subjection of the SNF particles to the fluorine plasma, the temperature is maintained in the range of 1200-2000 deg K to: a) allow any PuF 6 (gas) that is formed to decompose back to PuF 4 (solid), and b) to maintain stability of the UF 6 . Uranium (in the form of gaseous UF 6 ) is easily extracted and separated from the plutonium (in the form of solid PuF 4 ). The use of plasmas instead of high temperature reactors or flames mitigates the high temperature corrosive atmosphere and the production of PuF 6 (as a final product). Use of plasmas provide faster reaction rates, greater control over the individual electron and ion temperatures, and allow the use of CF 4 or NF 3 as the fluorine sources instead of F 2 or HF.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Development of CFD Flow Analysis for Nuclear Facility Ventilation Systems

Understanding and modeling of particulate transport has importance related to safety in ventilated environments that contain hot cells, gloveboxes, and fume hoods. In particular, good modeling of the airflow in these spaces is required to understand areas of stagnation where particles drop out of the free stream and accumulate. This accumulation of particulate can cause either contamination and/or higher than acceptable local dose levels. It is known that multiple sites across the DOE complex take credit for hot cells, gloveboxes, and/or hoods in their safety basis for providing a defense-in-depth benefit for both onsite and offsite releases. By providing confinement of radioactive materials, such features serve to reduce direct doses to facility workers and mitigate the consequences to the environment due to an uncontrolled release. Each of these features has access points that interface with the personnel space. Understanding how air flow behaves at these access points is of great interest to those performing hazard analysis. Computational Fluid Dynamics (CFD) can be used to analyze and model the flows in hot cells and glove boxes as a way to confirm operation. While CFD capability continues to advance, there are still important modeling assumptions that are left to the analyst's discretion. These are most notably the choice of the turbulence models, mesh structure, and wall boundary condition assumptions used in the model. In this work, we apply CFD in modeling airflow through an occupiable work area of the Alpha Gamma Hot Cell Facility (AGHCF) at Argonne National Laboratory (ANL). This modeling is then compared to field test data to both inform and verify the modeling assumptions. Based on the results of field tests, modeling assumptions and boundary conditions are refined and the process is repeated until the results are found to be reliable with a high level of confidence.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Effect of Quartz Aperture Covers on the Fluid Dynamics and Thermal Efficiency of Falling Particle Receivers

Falling particle receivers are an emerging technology for use in concentrating solar power systems. In this paper, quartz half-shells are investigated for use as full or partial aperture covers to reduce receiver thermal losses. Quartz half-shell aperture covers offer the ability to minimally interfere with incoming solar radiation from the heliostat field while obstructing thermal radiation and advection from leaving the receiver cavity. The fluid dynamics and heat transfer of a receiver subdomain and surrounding air are modeled using ANSYS®FLUENT We compare the percentage of total incident solar power lost due to conduction through the receiver walls, advective losses through the aperture, and radiation exiting the aperture. Contrary to expected outcomes, results show that quartz aperture covers can increase radiative losses and result in modest to nonexistent reductions in advective losses. The increased radiative losses are driven by elevated quartz half-shell temperatures and have the potential to be mitigated by active cooling and/or material selection. Quartz half-shell total transmissivity was measured experimentally using a radiometer and the National Solar Thermal Test Facility heliostat field with values up to 0.97 ± 0.01. Quartz half-shell aperture covers did not yield expected efficiency gains in numerical results due to increased radiative losses, but efficiency improvement in some numerical results and the performance of quartz half-shells subject to concentrated solar radiation suggest that quartz half-shell aperture covers should be investigated further.

14 SOLAR ENERGY↗

Ion motion in the wake driven by long particle bunches in plasmas

In this paper, we explore the role of the background plasma ion motion in self-modulated plasma wakefield accelerators. We employ Dawson's plasma sheet model to derive expressions for the transverse plasma electric field and ponderomotive force in the narrow bunch limit. We use these results to determine the on-set of the ion dynamics and demonstrate that the ion motion could occur in self-modulated plasma wakefield accelerators. Simulations show the motion of the plasma ions can lead to the early suppression of the self-modulation instability and of the accelerating fields. The background plasma ion motion can nevertheless be fully mitigated by using plasmas with heavier plasmas.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Layout and performance of HPK prototype LGAD sensors for the High-Granularity Timing Detector

The High-Granularity Timing Detector is a detector proposed for the ATLAS Phase II upgrade. The detector, based on the Low-Gain Avalanche Detector (LGAD) technology, will cover the pseudo-rapidity region of 2.4 < |n| < 4.0 with two end caps on each side and a total area of 6.4 m 2 . The timing performance can be improved by implanting an internal gain layer that can produce signals with a fast rising edge. It significantly improves the signal-to-noise ratio. The required average timing resolution per track for a minimum ionizing particle is 30 ps at the start and 50 ps at the end of the HL-LHC operation. This is achieved with several layers of LGAD. The innermost region of the detector would accumulate a 1MeV neutron-equivalent fluence up to 2.5 10 15 n eq /cm 2 including a safety factor of 1.5 before being replaced during the scheduled shutdowns. The addition of this new detector is expected to play an important role in the mitigation of high pile-ups at the HL-LHC. The layout and performance of the various versions of LGAD prototypes produced by Hamamatsu (HPK) have been studied by the ATLAS Collaboration. The breakdown voltages, depletion voltages, inter-pad gaps, collected charge as well as the time resolution have been measured and the production yield of large size sensors has been evaluated.

47 OTHER INSTRUMENTATION↗

Experimental Considerations in Long-Baseline Neutrino Oscillation Measurements

Long-baseline neutrino oscillation experiments, which are among the largest neutrino experiments in the world, have extensive physics programs to make precision measurements of three-flavor oscillation parameters, search for physics beyond the Standard Model, and study neutrinos from astrophysical sources. In this article, experimental considerations, including oscillation phenomenology, detector and experiment design, and analysis strategies, are described, with a focus on the three-flavor oscillation measurements. Current and future experiments are discussed, and significant sources of systematic uncertainty, along with mitigation strategies, are emphasized as control of systematic uncertainty is critical for success in precise measurement of long-baseline oscillation parameters. This article is structured as a primer for those new to this area of experimental work.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Current Control for Scorpius

There is a need to control the current produced by the Scorpius injector. Reduced beam current aids beam transport, reduces instability growth, mitigates spot-size enlargement due to beam-target interactions, and reduces reflections caused by beam loading of the cells. A method for reducing beam current without major impact on operations or major hardware replacement has been explored through simulations, the results of which are presented.

43 PARTICLE ACCELERATORS↗

2x2 Demonstrator High-Coverage Light Readout System in a Novel LArTPC

DUNE is a long-baseline Liquid Argon Time Projection Chamber (LArTPC) neutrino oscillation experiment. Its near detectors, located at Fermi National Laboratory, will constrain systematic errors on far detector measurements. The 2x2 Demonstrator, a novel proof of concept prototype for the ND LArTPC, has a modular TPC design that mitigates event pileup in a high-occupancy nearline beam environment, further aided by a native 3D pixelated charge readout and a 30% coverage, low profile light readout. This will be the first large-scale LArTPC to utilize pixels in place of wire planes

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Pickup Specifications for Crab Cavity Noise Feedback Pickup

The Electron-Ion Collider will employ crab cavities to compensate for the significant 25 mrad crossing angle, leading to an order of magnitude increase in luminosity. The crab cavity Radio Frequency system will inject low levels of noise to the crabbing field, generating transverse emittance growth and potentially limiting luminosity lifetime. A novel dedicated feedback system acting through the crab cavities has been proposed to mitigate emittance growth. The perfor mance of the noise feedback will largely depend on its pickup precision. In this note we present pickup specifications to achieve the required performance.

43 PARTICLE ACCELERATORS↗

Capacity Fade and Its Mitigation in Li-Ion Cells with Silicon-Graphite Electrodes

In this study we scrutinize the causes for capacity fade in lithium-ion cells containing silicongraphite (Si-Gr) blends in the negative electrode and examine approaches for minimizing this fade. The causal mechanisms are inferred from data obtained by electrochemistry, microscopy, spectroscopy and thermogravimetry techniques. The presence of SiOxFy signals in the Si-Gr electrode, LixPOyFz compounds in the electrolyte, and SiO2 species on the NCM523 positive electrode, highlight the crucial role of hydrolytically generated HF, which accelerates the degradation of Si particles. The hydrolysis could result from residual moisture in the current electrode fabrication process, which uses aqueous binders. Water can also be released when silanol groups on the Si nanoparticles react with HF to form Si-F compounds. We note that the primary cause of capacity fade in the full cells is the loss of solid electrolyte interphase (SEI) integrity resulting from volume changes in Si particles during electrochemical cycling. Adding fluoroethylene carbonate (FEC) to the conventional electrolyte slows capacity fade through the formation of a cross linked polymer with elastomeric properties. Further gains in cell longevity are possible by excluding water during electrode fabrication, using hydrolytically stable lithium salts, and adopting electrolyte systems that provide more elasticity to the SEI layers.

fluoroethylene carbonate↗

Mitigating Voltage Fade in Cathode Materials by Improving the Atomic Level Uniformity of Elemental Distribution

Li-rich and Mn-rich (LMR) layered structured materials are very promising cathodes for high-energy lithium-ion batteries. However, their fundamental structure and voltage fading mechanisms are far from being well understood. Here we report the first evidence on the reduced voltage and energy fade of LMR cathode by improving the atomic level spatial distribution of the chemical species. LMR cathode (Li[Li0.2Ni0.2M0.6]O2) prepared by co-precipitation and sol-gel methods are dominated by R-3m phase and show significant Ni-segregation at the surface of the particles. They exhibit large voltage-fade and fast capacity degradation. In contrast, LMR cathode prepared by hydrothermal assisted method is dominated by C2/m phase and minimal Ni-segregation. It also demonstrates much smaller voltage-fade and excellent capacity retention. The fundamental correlation between the atomic level spatial distribution of the chemical species and the functional stability of the materials found in this work also guide the design of other functional materials with enhanced stabilities.

Cation mixing↗

Tuning Cation (Dis)Order in Cr‐Based Li‐Excess Oxide Cathode Materials to Improve Li+ Transport Properties

Abstract Li‐excess disordered rocksalts (DRXs) hold promise as next‐generation cathodes for Li‐ion batteries due to their high capacity and energy density, along with the potential to eliminate the need for Co and Ni. However, due to their low Li + diffusivity, DRXs need to be pulverized into nanoparticles to achieve high performance. Herein, a new strategy for overcoming this limitation is demonstrated, involving the design of as‐synthesized partially disordered oxides with a structure that lies between ordered layered and fully disordered, exhibiting a varying degree of local (dis)order. This unique structure activates new Li + diffusion channels, improving percolation and transport properties. This strategy allows a large content of Li + to be accessed in material with large, micron‐sized particles through highly reversible Cr 3+/6+ and O redox, yielding a first discharge capacity of 286 mAh g −1 (881 Wh kg −1 ). The Li + percolation network is further improved by substituting Ti with a mixture of multiple metals, which appears to locally decrease the migration barrier through lattice distortion. Proper tuning of the chemical composition, especially the content of metals with empty d orbitals, is established as a crucial factor for controlling the degree of disorder and mitigating voltage fade and hysteresis growth upon cycling.

Moździerz, Maciej↗

Quantifying gas generation from slurries used in fabrication of Si-containing electrodes for lithium-ion cells

The high capacity of silicon motivates its use as anode material for Li-ion batteries. While such Si-based electrodes are typically processed from aqueous slurries, elemental silicon is highly susceptible to hydrolysis, yielding flammable hydrogen gas as a byproduct. This gassing can present numerous safety and quality concerns for scaling up of the production. In this study we describe a method to quantify the volume of gases generated using the Archimedes principle. We show that the gas volumes are affected by various factors, which include the characteristics of the electrode slurry and attributes (particle size, surface coatings) of the silicon powders. A catalytic effect on gas evolution is observed when a lithiated polycarboxylate binder is present in the solution. On the other hand, negligible gas generation is observed in electrode slurries containing the N -methyl-2-pyrrolidone (NMP) solvent, which could be considered as an alternative to the water-based processes presently under consideration. Lastly, our study can be used as a guide for the development of slurry mixtures that can mitigate the safety concerns associated with the silicon-electrode fabrication process.

25 ENERGY STORAGE↗

Progress with Long-Range Beam-Beam Compensation Studies for High Luminosity LHC

Long-range beam-beam (LRBB) interactions can be a source of emittance growth and beam losses in the LHC during physics and will become even more relevant with the smaller '* and higher bunch intensities foreseen for the High Luminosity LHC upgrade (HL-LHC), in particular if operated without crab cavities. Both beam losses and emittance growth could be mitigated by compensat-ing the non-linear LRBB kick with a correctly placed current carrying wire. Such a compensation scheme is currently being studied in the LHC through a demonstration test using current-bearing wires embedded into col-limator jaws, installed either side of the high luminosity interaction regions. For HL-LHC two options are considered, a current-bearing wire as for the demonstrator, or electron lenses, as the ideal distance between the particle beam and compensating current may be too small to allow the use of solid materials. This paper reports on the ongoing activities for both options, covering the progress of the wire-in-jaw collimators, the foreseen LRBB experiments at the LHC, and first considerations for the design of the electron lenses to ultimately replace material wires for HL-LHC.

43 PARTICLE ACCELERATORS↗

Multipole approximation of special nonlinear magnets for the IOTA ring

All existing focusing optics for accelerators are built to be "linear", i.e. the transverse focusing force is proportional to the particle displacement from the closed orbit. Such approach is used in order to make trajectories stable in the entire area of phase space, because the potential describing linear focusing is integrable and does not produce chaotic motion. Technically, the needed field is achieved with the help of dipole and quadrupole magnets. But the linear motion is unstable to perturbations in the focusing fields and excludes any betatron tune spread over particle's energy, which is beneficial for the beam stability. Moreover, the focusing strength depends on the particle's energy deviation from the designed one. These undesired effects are usually suppressed by the addition of non- linear elements, such as sextupoles and octupoles. Unfortunately, these additions make focusing potential nonintegrabe, leading to the limitation of stable phase space area. Recent research showed, that there exist non-linear potentials that, nevertheless, are fully integrable [1, 2]. Thus, there is an opportunity to create stable non-linear focusing optics that provides high betatron tune spread and mitigate magnetic field errors. This approach is to be implemented in electron storage ring called Integrable Optics Test Accelerator (IOTA) at Fermilab [3]. The main goal is to show the possibility to implement the nonlinear integrable system in a realistic accelerator design. Development of a magnet, which creates exact non-linear potential, is a technically complicated task, that takes much time and efforts. However, it is possible to expand the non- linear potential into superposition of multipoles of even orders (i.e quadrupole, octupole, etc.). Though this series is not convergent in the entire space, a few low order terms can be used to model the true potential in some limited area. In turn, each of the multipole potentials can be generated by speci ed electrical current in PCB coiled on the surface of storage ring's vacuum tube. Such approach is much cheaper than the creation of a magnet of solid iron with high current coil and faster than the development of \exact" non-linear magnet, but it can help identify some features of non-linear integrable optics application. The goal of this research work is to find analytically the angular distribution of electrical current on the surface of the vacuum tube, which creates inside it multipole potential with given parameters. Hereafter, there is the task to develop a model of flexible printed circuit board (PCB), which could be coiled around the vacuum tube in order to provide the desired current distribution.

Vorobev, Viktor↗

Analysis of MIR-18 results for physical and biological dosimetry: radiation shielding effectiveness in LEO

We compare models of radiation transport and biological response to physical and biological dosimetry results from astronauts on the Mir space station. Transport models are shown to be in good agreement with physical measurements and indicate that the ratio of equivalent dose from the Galactic Cosmic Rays (GCR) to protons is about 3/2:1 and that this ratio will increase for exposures to internal organs. Two biological response models are used to compare to the Mir biodosimetry for chromosome aberration in lymphocyte cells; a track-structure model and the linear-quadratic model with linear energy transfer (LET) dependent weighting coefficients. These models are fit to in vitro data for aberration formation in human lymphocytes by photons and charged particles. Both models are found to be in reasonable agreement with data for aberrations in lymphocytes of Mir crew members: however there are differences between the use of LET dependent weighting factors and track structure models for assigning radiation quality factors. The major difference in the models is the increased effectiveness predicted by the track model for low charge and energy ions with LET near 10 keV/micrometers. The results of our calculations indicate that aluminum shielding, although providing important mitigation of the effects of trapped radiation, provides no protective effect from the galactic cosmic rays (GCR) in low-earth orbit (LEO) using either equivalent dose or the number of chromosome aberrations as a measure until about 100 g/cm 2 of material is used.

Flight Experiment↗

Cross-beam energy transfer saturation by ion trapping-induced detuning

The performance of direct-drive inertial confinement fusion implosions relies critically on the coupling of laser energy to the target plasma. Cross beam energy transfer (CBET), the resonant exchange of energy between intersecting laser beams mediated by ponderomotively driven ion-acoustic waves (IAW), inhibits this coupling by scattering light into unwanted directions. Furthermore, the variety of beam intersection angles and varying plasma conditions in an implosion results in IAWs with a range of phase velocities. Here we show that CBET saturates through a resonance detuning that depends on the IAW phase velocity and that results from trapping-induced modifications to the ion distribution functions. For smaller phase velocities, the modifications to the distribution functions can rapidly thermalize in the presence of mid-Z ions, leading to a blueshift in the resonant frequency. For larger phase velocities, the modifications can persist, leading to a redshift in the resonant frequency. Ultimately, these results may reveal pathways towards CBET mitigation and inform reduced models for radiation hydrodynamics codes to improve their predictive capability.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗