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At least 1,063 records · Page 59

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DOE OSTI2017

A rapid method to extract Seebeck coefficient under a large temperature difference

The Seebeck coefficient is one of the three important properties in thermoelectric materials. Since thermoelectric materials usually work under large temperature difference in real applications, we propose a quasi-steady state method to accurately measure the Seebeck coefficient under large temperature gradient. Compared to other methods, this method is not only highly accurate but also less time consuming. It can measure the Seebeck coefficient in both the temperature heating up and cooling down processes. In this work, a Zintl material (Mg 3.15 Nb 0.05 Sb 1.5 Bi 0.49 Te 0.01 ) was tested to extract the Seebeck coefficient from room temperature to 573 K. Compared with a commercialized Seebeck coefficient measurement device (ZEM-3), there is ±5% difference between those from ZEM-3 and this method.

36 MATERIALS SCIENCE↗

DOE OSTI2024

The effect of temperature oscillations on energy storage rectification in harmonic systems

Abstract Rectification, the preferential transport of a current in one direction through a system, has garnered significant attention in molecules because of its importance for controlling thermal and electronic currents at the nanoscale. Here, we report the presence of energy storage rectification effects in a molecular chain. This phenomenon is generated by subjecting a harmonic molecular chain to an oscillating temperature gradient and showing that the energy absorption rate of the system depends on the direction of the gradient. We examine how the energy storage rectification ratios in the chain are affected by the oscillating gradient, asymmetry in the chain, and the system parameters. We find that energy storage rectification can be observed in harmonic lattice structures with time-dependent temperatures and that, correspondingly, anharmonicity is not required to generate this rectification mechanism in such systems.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2022

Predictive Large-Eddy Simulation of Supercritical-Pressure Reactive Flows in the Cold Ignition Regime

This report describes a one-year study performed under DOE sponsorship, continuing the investigation of high-pressure turbulent reactive flows. The interest is in the effect of the chemical species distribution in high-pressure turbulent flows in the presence of strong temperature gradients as would occur during reactions in realistic flows. The prime example of such flows are boundary layers in which the wall is at a lower temperature than that of the fluid, as would be the case in Diesel engines. Previous DOE BES work in the program further highlighted the importance of the boundary layer as a configuration for fundamental studies: soot formation in boundary layers is still a problem poorly understood and depends on the availability of particular chemical species at that location, and when boundary layer Large Eddy Simulations results were compared with measurements, the agreement was unfavorable, showing that this important ‘unit’ problem is not well understood. To understand this unit problem, modeling and Direct Numerical Simulations of this unit problem were conducted for the simplest possible multispecies system, that is a binary-species system. The results discovered a new phenomenon, that is, Soret effect induced uphill diffusion. The far-reaching implication is that through an imposed wall/fluid temperature difference it is possible to control the distribution of the species in the boundary layer. Because the results have been documented in one paper published in the refereed literature, and also in conference papers, this final report is in the form of an Executive Summary succinctly describing the results and putting them in perspective with respect to existing information. The refereed and conference papers published are individually listed as Appendices and attached to this report. One manuscript is still in progress and is thus not listed.

74 ATOMIC AND MOLECULAR PHYSICS↗

NASA NTRS1997

Nonlinear Transient Thermal Analysis by the Force-Derivative Method

High-speed vehicles such as the Space Shuttle Orbiter must withstand severe aerodynamic heating during reentry through the atmosphere. The Shuttle skin and substructure are constructed primarily of aluminum, which must be protected during reentry with a thermal protection system (TPS) from being overheated beyond the allowable temperature limit, so that the structural integrity is maintained for subsequent flights. High-temperature reusable surface insulation (HRSI), a popular choice of passive insulation system, typically absorbs the incoming radiative or convective heat at its surface and then re-radiates most of it to the atmosphere while conducting the smallest amount possible to the structure by virtue of its low diffusivity. In order to ensure a successful thermal performance of the Shuttle under a prescribed reentry flight profile, a preflight reentry heating thermal analysis of the Shuttle must be done. The surface temperature profile, the transient response of the HRSI interior, and the structural temperatures are all required to evaluate the functioning of the HRSI. Transient temperature distributions which identify the regions of high temperature gradients, are also required to compute the thermal loads for a structural thermal stress analysis. Furthermore, a nonlinear analysis is necessary to account for the temperature-dependent thermal properties of the HRSI as well as to model radiation losses.

Balakrishnan, Narayani V.↗

NASA NTRS1999

Climate Change and the Brewer-Dobson Circulation

Using GCM (General Circulation Model) simulations of the troposphere-stratosphere circulation in different climate regimes, the sensitivity of the Brewer-Dobson Circulation to climate change will be discussed. Included will be simulations of the stratosphere with increasing/doubled CO2 as done with different versions of the GISS (Goddard Institute for Space Studies) Global Climate Middle Atmosphere Model, with and without ozone response. To put the results in a broader perspective, stratospheric circulation changes from several paleoclimate simulations will also be presented, including the Last Glacial Maximum and the Paleocene, each with several different (plausible) latitudinal sea surface temperature gradients. Hence the climate changes investigated will include strong variations in baroclinic and topographic tropospheric planetary wave and gravity wave forcing, as well as global mean temperature and atmospheric CO2 levels. Results will be analyzed in terms of wave driving via E-P flux convergences and gravity wave effects, and will be shown to be strongly dependent on wave propagation characteristics.

Rind, David↗

NASA NTRS1999

Climate Change and the Brewer-Dobson Circulation

Using GCM simulations of the troposphere-stratosphere circulation in different climate regimes, the sensitivity of the Brewer-Dobson Circulation to climate change will be discussed. Included will be simulations of the stratosphere with increasing/doubled C02 as done with different versions of the GISS Global Climate Middle Atmosphere Model, with and without ozone response. To put the results in a broader perspective, stratospheric circulation changes from several paleoclimate simulations will also be presented, including the Last Glacial Maximum and the Paleocene, each with several different (plausible) latitudinal sea surface temperature gradients. Hence the climate changes investigated will include strong variations in baroclinic and topographic tropospheric planetary wave and gravity wave forcing, as well as global mean temperature and atmospheric C02 levels. Results will be analyzed in terms of wave driving via E-P flux convergences and gravity wave effects, and will be shown to be strongly dependent on wave propagation characteristics.

Rind, David↗

NASA NTRS2012

Quantitative Infrared Image Analysis Of Thermally-Thin Cellulose Surface Temperatures During Upstream and Downstream Microgravity Flame Spread from A Central Ignition Line

Surface view calibrated infrared images of ignition and flame spread over a thin cellulose fuel were obtained at 30 Hz during microgravity flame spread tests in the 10 second Japan Microgravity Center (JAMIC). The tests also used a color video of the surface view and color images of the edge view using 35 millimeter 1600 Kodak Ektapress film at 2 Hz. The cellulose fuel samples (50% long fibers from lumi pine and 50% short fibers from birch) were made with an area density of 60 grams per square meters. The samples were mounted in the center of a 12 centimeter wide by 16 centimeter tall flow duct that uses a downstream fan to draw the air through the flow duct. Samples were ignited after the experiment package was released using a straight hot wire across the center of the 7.5 centimeter wide by 14 centimeter long samples. One case, at 1 atmosphere 35%O2 in N2, at a forced flow of 10 centimeters per second, is presented here. In this case, as the test progresses, the single flame begins to separate into simultaneous upstream and downstream flames. Surface temperature profiles are evaluated as a function of time, and temperature gradients for upstream and downstream flame spread are measured. Flame spread rates from IR image data are compared to visible image spread rate data. IR blackbody temperatures are compared to surface thermocouple readings to evaluate the effective emissivity of the pyrolyzing surface. Preheat lengths are evaluated both upstream and downstream of the central ignition point. A surface energy balance estimates the net heat flux from the flame to the fuel surface along the length of the fuel.

Olson, Sandra L.↗

NASA NTRS2013

Quantitative Infrared Image Analysis Of Simultaneous Upstream and Downstream Microgravity Flame Spread over Thermally-Thin Cellulose in Low Speed Forced Flow

The effect of low velocity forced flow on microgravity flame spread is examined using quantitative analysis of infrared video imaging. The objective of the quantitative analysis is to provide insight into the mechanisms of flame spread in microgravity where the flame is able to spread from a central location on the fuel surface, rather than from an edge. Surface view calibrated infrared images of ignition and flame spread over a thin cellulose fuel were obtained along with a color video of the surface view and color images of the edge view using 35 mm color film at 2 Hz. The cellulose fuel samples were mounted in the center of a 12 cm wide by 16 cm tall flow duct and were ignited in microgravity using a straight hot wire across the center of the 7.5 cm wide by 14 cm long samples. Four cases, at 1 atm. 35%O2 in N2, at forced flows from 2 cm/s to 20 cm/s are presented here. This flow range captures flame spread from strictly upstream spread at low flows, to predominantly downstream spread at high flow. Surface temperature profiles are evaluated as a function of time, and temperature gradients for upstream and downstream flame spread are measured. Flame spread rates from IR image data are compared to visible image spread rate data. IR blackbody temperatures are compared to surface thermocouple readings to evaluate the effective emissivity of the pyrolyzing surface. Preheat lengths and pyrolysis lengths are evaluated both upstream and downstream of the central ignition point. A surface energy balance estimates the net heat flux from the flame to the fuel surface along the length of the fuel. Surface radiative loss and gas-phase radiation from soot are measured relative to the net heat feedback from the flame. At high surface heat loss relative to heat feedback, the downstream flame spread does not occur.

Olson, S. L.↗

DOE OSTI2025

Multiphase computational fluid dynamics modeling of reacting flows in absorption columns for carbon capture

First-principles derived computational fluid dynamics (CFD) simulations have been proposed as a fundamental tool for investigating solvent-based CO 2 absorption in packed columns due to their ability to accurately represent the underlying nonlinear, multiscale dynamics. Numerous studies have previously utilized such CFD simulations to investigate hydrodynamics of columns with structured and random packings by assessing the key hydrodynamic metrics such as the interfacial and wetted areas. While mapping such metrics for different conditions is essential to the optimization of absorption columns, it is not sufficient, as the CO 2 capture rate depends also on the coupled, nonlinear dynamics from the underlying chemical reaction kinetics, thermodynamics, and heat-transfer rates. In this work, we present detailed CFD simulation results augmented by incorporating the effects of interfacial physical mass transfer of CO 2 , heat release from chemical reaction kinetics, and thermophysical property variations from resulting temperature gradients. We demonstrate the applicability of the proposed approach in numerically assessing the performance of packed columns by evaluating key hydrodynamic quantities, CO 2 absorption rates, and temperature rise in a reference column with packings that are structurally similar to the Sulzer Mellapak™ 250.Y packing, for different solvent inflow velocities and temperatures. Predictions from simulation results are found to be consistent with the trends in experimental observations from the literature, suggesting that the predictive capabilities of the simulation framework can be leveraged to guide the future development of absorber-column designs and optimized process flowsheets.

Absorption columns↗

DOE OSTI2019

Controlling the Vapor Transport Crystal Growth of Hg 3 Se 2 I 2 Hard Radiation Detector Using Organic Polymer

The chalcohalide compound Hg 3 Se 2 I 2 with a defect anti-perovskite structure has been demonstrated to be a promising semiconductor for room temperature X- and gamma-ray detection. In this work, we use transport agents during the vapor growth of Hg 3 Se 2 I 2 crystals under gradient temperature profiles to dramatically improve the size and yield of Hg 3 Se 2 I 2 single crystals. Various growth conditions with combinations of organic polymer (polyethylene) with elemental Hg, Se, or 12 are compared. The largest single crystals (with size up to 7 x 5 x 3.5 mm 3 ) were obtained using both polyethylene and excess I-2 as the transport agents. The as-prepared detector devices based on these crystals have excellent photo response to a series of radiation sources, including low flux X-ray source, alpha particles, and gamma-rays. The X-ray induced photocurrent of Hg 3 Se 2 I 2 detectors is 3 orders of magnitude higher than the dark current, indicating excellent X-ray photosensitivity. Under Am-241 alpha particle source (5.5 MeV), the best energy resolution obtained is similar to 8.1%. The Hg 3 Se 2 I 2 device also shows improved detector performance under Co-57 and Cs-137 gamma-ray sources. The improved crystal growth and detector performance using this polymer additive during the vapor transport process further confirms the great potential for the development of Hg 3 Se 2 I 2 for radiation detection.

36 MATERIALS SCIENCE↗

DOE OSTI2022

The influence of recent and future climate change on spring Arctic cyclones

In recent decades, the Arctic has experienced rapid atmospheric warming and sea ice loss, with an ice-free Arctic projected by the end of this century. Cyclones are synoptic weather events that transport heat and moisture into the Arctic, and have complex impacts on sea ice, and the local and global climate. However, the effect of a changing climate on Arctic cyclone behavior remains poorly understood. This study uses high resolution (4 km), regional modeling techniques and downscaled global climate reconstructions and projections to examine how recent and future climatic changes alter cyclone behavior. Results suggest that recent climate change has not yet had an appreciable effect on Arctic cyclone characteristics. However, future sea ice loss and increasing surface temperatures drive large increases in the near-surface temperature gradient, sensible and latent heat fluxes, and convection during cyclones. The future climate can alter cyclone trajectories and increase and prolong intensity with greatly augmented wind speeds, temperatures, and precipitation. Such changes in cyclone characteristics could exacerbate sea ice loss and Arctic warming through positive feedbacks. The increasing extreme nature of these weather events has implications for local ecosystems, communities, and socio-economic activities.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1992

Effects of buoyancy-driven flow and thermal boundary conditions on physical vapor transport

A 2D numerical model was developed in order to ascertain if reduced gravity conditions are beneficial to physical vapor transport (PVT) and to determine its tolerance limits to residual accelerations. This was solved using the PHOENICS finite-volume code. Reduction of gravitational accelerations to less than 0.1 g0 was found to be sufficient to suppress buoyancy-driven convection to an extent that diffusion was the dominant transport mode, whence a greater uniformity in the growth rate could be obtained. It is shown that a uniform temperature gradient on the ampoule walls causes the vapor to be supersaturated throughout the ampoule, potentially resulting in undesirable nucleation at the walls. A 'hump' in the wall temperature profile can be used to avoid this. The prevailing transport conditions determine the size of the hump needed.

Nadarajah, Arunan↗

NASA NTRS2004

Direct Observation of Controlled Melting and Resolidification of Succinonitrile Mixtures in a Microgravity Environment

In support of the Pore Formation and Mobility Investigation (PFMI) direct observation of experiments on the controlled melting and subsequent resolidification of succinonitrile were conducted in the glovebox facility (GBX) of the International Space Station (ISS). Samples were prepared on ground by filling glass tubes, 1 cm ID and approximately 30 cm in length, with pure succinonitrile (SCN) and SCN-Water mixtures under 450 millibar of nitrogen. Experimental processing parameters of temperature gradient and translation speed, as well as camera settings, were remotely monitored and manipulated from the ground Telescience Center (TSC) at the Marshall Space Flight Center. Sample temperatures are monitored by six in situ thermocouples. Real time visualization during melt back revealed bubbles of different sizes initiating at the solid/liquid interface, their release, interactions, and movement into the temperature field ahead of them. Subsequent re-solidification examined planar interface breakdown and the transition to steady-state dendritic growth. A preliminary analysis of the observed phenomena and its implication to future microgravity experiments is presented and discussed.

Grugel, R. N.↗

NASA NTRS2000

Monitoring Geothermal Features in Yellowstone National Park with ATLAS Multispectral Imagery

The National Park Service (NPS) must produce an Environmental Impact Statement for each proposed development in the vicinity of known geothermal resource areas (KGRAs) in Yellowstone National Park. In addition, the NPS monitors indicator KGRAs for environmental quality and is still in the process of mapping many geothermal areas. The NPS currently maps geothermal features with field survey techniques. High resolution aerial multispectral remote sensing in the visible, NIR, SWIR, and thermal spectral regions could enable YNP geothermal features to be mapped more quickly and in greater detail In response, Yellowstone Ecosystems Studies, in partnership with NASA's Commercial Remote Sensing Program, is conducting a study on the use of Airborne Terrestrial Applications Sensor (ATLAS) multispectral data for monitoring geothermal features in the Upper Geyser Basin. ATLAS data were acquired at 2.5 meter resolution on August 17, 2000. These data were processed into land cover classifications and relative temperature maps. For sufficiently large features, the ATLAS data can map geothermal areas in terms of geyser pools and hot springs, plus multiple categories of geothermal runoff that are apparently indicative of temperature gradients and microbial matting communities. In addition, the ATLAS maps clearly identify geyserite areas. The thermal bands contributed to classification success and to the computation of relative temperature. With masking techniques, one can assess the influence of geothermal features on the Firehole River. Preliminary results appear to confirm ATLAS data utility for mapping and monitoring geothermal features. Future work will include classification refinement and additional validation.

Spruce, Joseph↗

NASA NTRS2022

The Influence of Recent and Future Climate Change on Spring Arctic Cyclones

Chelsea L Parker↗

DOE OSTI2017

Avalanches driven by pressure gradients in a magnetized plasma

The results are presented for a basic heat transport experiment involving an off-axis heat source in which avalanche events occur. The configuration consists of a long, hollow, cylindrical region of elevated electron temperature embedded in a colder plasma, and far from the device walls [Van Compernolle et al. Phys. Rev. E 91, 031102(R) (2015)]. The avalanche events are identified as sudden rearrangements of the pressure profile following the growth of fluctuations from ambient noise. The intermittent collapses of the plasma pressure profile are associated with unstable drift-Alfvén waves and exhibit both radial and poloidal dynamics. After each collapse, the plasma enters a quiescent phase in which the pressure profile slowly recovers and steepens until a threshold is exceeded, and the process repeats. The use of reference probes as time markers allows for the visualization of the 2D spatio-temporal evolution of the avalanche events. Avalanches are observed only for a limited combination of heating powers and magnetic fields. At higher heating powers, the system transits from the avalanche regime into a regime dominated by sustained drift-Alfvén wave activity. Here, this manuscript focuses on new results that illustrate the individual contributions to the avalanche process from density and temperature gradients in the presence of zero-order, sheared flows.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2026

Routes to high-performance operation in Wendelstein 7-X: turbulence suppression with shaping of the density profile

Steep density gradients generally lead to improved plasma performance in the neoclassically optimized stellarator W7-X. This is evident in the global energy confinement time as well as in the ion temperature and can be explained by a strong reduction of the ion temperature gradient turbulence. Such conditions can experimentally be realized by several methods: injection of cryogenic hydrogen pellets, appropriate combination of neutral beam and electron cyclotron resonance heating (ECRH) and, in some cases, with low power of ECRH after preconditioning of the first wall. The duration of the improved phases is determined by the ability to sustain the steep density gradient, by technical limitations of the involved systems and, eventually, by the plasma stability. This paper gives an overview of relevant experimental results and presents example discharges where the improved confinement conditions could be extended to multiple seconds: up to 4 s using neutral beam injection and from 14 to 40 s with steady state pellet injection. In these plasmas the turbulent thermal diffusivity is reduced by a factor of 3 to 4 in a broad radial range, which allows high ion temperatures of up to 3 keV at the densities of about 1.5 • 10 20 m −3 .

high performance plasma↗

DOE OSTI2018

High-Resolution Raman Measurements of Gradients at Interfaces

Fundamental investigations of non-equilibrium gas-liquid interfaces at elevated pressure will require knowledge of gas-phase boundary conditions affecting the interface structure. To assess the feasibility of applying one-dimensional imaging of spontaneous Raman scattering to resolve species and temperature gradients in the gas-phase boundary layer above a fluoroketone liquid surface, spectra of fluoroketone (1,1,1,2,2,4,5,5,5-nonafluoro-4-(trifluoromethyl)-3-pentanone) vapor in a carrier gas (N 2 or CO 2 ) are reported over the temperature range 300 K to 700 K. The measured Raman spectra show no detectable broadband interference from laser-induced fluorescence. Features of the fluoroketone Raman spectrum overlap the CO 2 spectrum, such that crosstalk corrections will be necessary for quantitative concentration measurements of CO 2 in mixtures. High-resolution Raman spectra in this overlap region, acquired over the same temperature range, will enable future development of temperature dependent spectral libraries for fluoroketone.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗