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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,063 records · Page 59
All sourcesNASA NTRSDOE OSTI
DOE OSTI2018

Preferential Charge Generation at Aggregate Sites in Narrow Band Gap Infrared Photoresponsive Polymer Semiconductors

Infrared organic photodetector materials are investigated using transient absorption spectroscopy, demonstrating that ultrafast charge generation assisted by polymer aggregation is essential to compensate for the energy gap law, which dictates that excited state lifetimes decrease as the band gap narrows. Short sub–picosecond singlet exciton lifetimes are measured in a structurally related series of infrared–absorbing copolymers that consist of alternating cyclopentadithiophene electron–rich “push” units and strong electron–deficient “pull” units, including benzothiadiazole, benzoselenadiazole, pyridalselenadiazole, or thiadiazoloquinoxaline. While the ultrafast lifetimes of excitons localized on individual polymer chains suggest that charge carrier generation will be inefficient, high detectivity for polymer:PC 71 BM infrared photodetectors is measured in the 0.6 < λ < 1.5 µm range. The photophysical processes leading to charge generation are investigated by performing a global analysis on transient absorption data of blended polymer:PC 71 BM films. In these blends, charge carriers form primarily at polymer aggregate sites on the ultrafast time scale (within our instrument response), leaving quickly decaying single–chain excitons unquenched. Lastly, the results have important implications for the further development of organic infrared optoelectronic devices, where targeting processes such as excited state delocalization over aggregates may be necessary to mitigate losses to ultrafast exciton decay as materials with even lower band gaps are developed.

36 MATERIALS SCIENCE↗
DOE OSTI2015

MULTI-MESSENGER ASTRONOMY OF GRAVITATIONAL-WAVE SOURCES WITH FLEXIBLE WIDE-AREA RADIO TRANSIENT SURVEYS

We explore opportunities for multi-messenger astronomy using gravitational waves (GWs) and prompt, transient low-frequency radio emission to study highly energetic astrophysical events. We review the literature on possible sources of correlated emission of GWs and radio transients, highlighting proposed mechanisms that lead to a short-duration, high-flux radio pulse originating from the merger of two neutron stars or from a superconducting cosmic string cusp. We discuss the detection prospects for each of these mechanisms by low-frequency dipole array instruments such as LWA1, the Low Frequency Array and the Murchison Widefield Array. We find that a broad range of models may be tested by searching for radio pulses that, when de-dispersed, are temporally and spatially coincident with a LIGO/Virgo GW trigger within a ∼30 s time window and ∼200–500 deg{sup 2} sky region. We consider various possible observing strategies and discuss their advantages and disadvantages. Uniquely, for low-frequency radio arrays, dispersion can delay the radio pulse until after low-latency GW data analysis has identified and reported an event candidate, enabling a prompt radio signal to be captured by a deliberately targeted beam. If neutron star mergers do have detectable prompt radio emissions, a coincident search with the GW detector network and low-frequency radio arrays could increase the LIGO/Virgo effective search volume by up to a factor of ∼2. For some models, we also map the parameter space that may be constrained by non-detections.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

Utilization of the LS-APGD microplasma/orbitrap-FTMS booster system for detection and isotopic analysis of neodymium nanoparticles

Detection and isotopic analysis of particle populations has seen rapid growth across several application areas, including environmental analysis, nuclear forensics, and food safety. The ability to characterize the particles' unique elemental and isotopic fingerprints could provide information related to formation, processing history, and transport. Regarding nuclear forensics, isotopic analysis of particles derived from diverse materials is often used as a tool to trace the origin and processing history. Mass spectrometric-based techniques currently used for particle population analysis often suffer from limited mass resolution, particularly when dealing with real-world samples that are affected by isobaric and polyatomic interferences from the matrix. To address these analytical challenges, we propose a novel method utilizing the liquid sampling-atmospheric pressure glow discharge (LS-APGD) microplasma ionization source coupled to an ultrahigh resolution Orbitrap mass spectrometer, further enhanced with the FTMS X2T Booster data acquisition and processing unit. The FTMS Booster enables acquisition of extended transient times of up to 3 s, significantly improving mass resolution, thereby reducing or even eliminating the need for prior separation of isobaric or polyatomic interferences. Additionally, the detection of low-abundance isotopes was improved by increasing the signal-to-noise (S/N) ratio. As proof of concept, this study demonstrates the feasibility of the LS-APGD/Orbitrap-FTMS X2T Booster platform for direct analysis using a suspension of well-characterized ∼120 nm neodymium particles. The quality of the isotope ratios values obtained from a few hundred particles were in good agreement with those obtained from homogeneous ionic solutions. These results highlight the potential of the LS-APGD/Orbitrap platform for rapid, accurate, and interference-resilient isotope ratio analysis of particle populations without the need for dissolution and subsequent chemical separations, offering significant advantages for nuclear forensics, safeguards, and environmental applications. The effort here also points to further paths forward, hopefully towards single particle (SP) analysis using microplasma ionization and the ultrahigh resolving power of the Orbitrap mass analyzer.

FTMS X2T booster↗
DOE OSTI2015

Spitzer point-source catalogs of ∼ 300,000 stars in seven nearby galaxies

We present Spitzer IRAC 3.6–8 μm and Multiband Imaging Photometer 24 μm point-source catalogs for seven galaxies: NGC 6822, M33, NGC 300, NGC 2403, M81, NGC 0247, and NGC 7793. The catalogs contain a total of ∼300,000 sources and were created by dual-band selection of sources with >3σ detections at both 3.6 and 4.5 μm. The source lists become significantly incomplete near m{sub 3.6}=m{sub 4.5}≃18. We complement the 3.6 and 4.5 μm fluxes with 5.8, 8.0, and 24 μm fluxes or 3σ upper limits using a combination of PSF and aperture photometry. This catalog is a resource as an archive for studying mid-infrared transients and for planning observations with the James Webb Space Telescope.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1994

Constraints on the luminosity function of gamma-ray bursts detected by BATSE

We have utilized the integral moment analysis technique of Horack & Emslie to extract information on the allowable form of the luminosity function for gamma-ray bursts observed by Burst and Transient Source Experiment (BATSE). Using the general properties of moments, we are able to derive constraints on the range of luminosity from which the gamma-ray bursts must be sampled. These constraints are independent of the form of the radial distribution of the gamma-ray bursts, and depend only on the assumptions that space is Euclidean and that the luminosity function phi(L) is distance independent. For power-law luminosity functions of the form phi(L) = A(sub 0)L(exp -alpha), we find that the range of luminosity from which 80% of the gamma-ray bursts must be sampled cannot exceed approximately 6.5, with a 3 sigma upper limit of 12-15, regardless of the value of alpha.

Horack, J. M.↗
DOE OSTI2017

Turbulent Magnetic Relaxation in Pulsar Wind Nebulae

We present a model for magnetic energy dissipation in a pulsar wind nebula. A better understanding of this process is required to assess the likelihood that certain astrophysical transients may be powered by the spin-down of a “millisecond magnetar.” Examples include superluminous supernovae, gamma-ray bursts, and anticipated electromagnetic counterparts to gravitational wave detections of binary neutron star coalescence. Our model leverages recent progress in the theory of turbulent magnetic relaxation to specify a dissipative closure of the stationary magnetohydrodynamic (MHD) wind equations, yielding predictions of the magnetic energy dissipation rate throughout the nebula. Synchrotron losses are self-consistently treated. To demonstrate the model’s efficacy, we show that it can reproduce many features of the Crab Nebula, including its expansion speed, radiative efficiency, peak photon energy, and mean magnetic field strength. Unlike ideal MHD models of the Crab (which lead to the so-called σ -problem), our model accounts for the transition from ultra to weakly magnetized plasma flow and for the associated heating of relativistic electrons. We discuss how the predicted heating rates may be utilized to improve upon models of particle transport and acceleration in pulsar wind nebulae. We also discuss implications for the Crab Nebula’s γ -ray flares, and point out potential modifications to models of astrophysical transients invoking the spin-down of a millisecond magnetar.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2013

Generation of THz transients by photoexcited single-crystal GaAs meso-structures

We report a sub-picosecond photoresponse and THz transient generation of GaAs single-crystal mesoscopic platelets excited by femtosecond optical pulses. Our structures were fabricated by a top-down technique, by patterning an epitaxial, 500-nm-thick GaAs film grown on top of an AlAs sacrificial layer and then transferring the resulting etched away 10 x 20-μm 2 platelets onto an MgO substrate using a micropipette. The freestanding GaAs devices, incorporated into an Au coplanar strip line, exhibited extremely low dark currents and ~0.4 % detection efficiency at 10 V bias. The all-optical, pump–probe carrier dynamics analysis showed that, for 800-nm-wavelength excitation, the intrinsic relaxation of photocarriers featured a 310-fs-wide transient with a 290 fs fall time. We have also carried out a femtosecond, timeresolved electro-optic characterization of our devices and recorded along the transmission line the electrical transients as short as ~600 fs, when the platelet was excited by a train of 100-fs-wide, 800-nm-wavelength optical laser pulses. The platelets have been also demonstrated to be very efficient generators of free-space propagating THz transients with the spectral bandwidth exceeding 2 THz.The presented performance of the epitaxial, freestanding GaAs meso-structured photodevices makes them uniquely suitable for THz-frequency optoelectronic applications, ranging from ultrafast photodetectors to THz-bandwidth optical-to-electrical transducers and photomixers.

42 ENGINEERING↗
DOE OSTI2024

The persistence of memory in ionic conduction probed by nonlinear optics

Predicting practical rates of transport in condensed phases enables the rational design of materials, devices and processes. This is especially critical to developing low-carbon energy technologies such as rechargeable batteries. For ionic conduction, the collective mechanisms, variation of conductivity with timescales and confinement, and ambiguity in the phononic origin of translation, call for a direct probe of the fundamental steps of ionic diffusion: ion hops. However, such hops are rare-event large-amplitude translations, and are challenging to excite and detect. Here we use single-cycle terahertz pumps to impulsively trigger ionic hopping in battery solid electrolytes. This is visualized by an induced transient birefringence, enabling direct probing of anisotropy in ionic hopping on the picosecond timescale. The relaxation of the transient signal measures the decay of orientational memory, and the production of entropy in diffusion. We extend experimental results using in silico transient birefringence to identify vibrational attempt frequencies for ion hopping. Using nonlinear optical methods, we probe ion transport at its fastest limit, distinguish correlated conduction mechanisms from a true random walk at the atomic scale, and demonstrate the connection between activated transport and the thermodynamics of information.

25 ENERGY STORAGE↗
DOE OSTI2026

Transient hydroperoxyalkyl intermediates (•QOOH) in isopentane oxidation. I. Conformer- and isomer-resolved infrared spectra

Transient carbon-centered hydroperoxyalkyl intermediates (•QOOH) in isopentane oxidation are characterized by infrared (IR) action spectroscopy under jet-cooled conditions with selective detection of hydroxyl (OH) radical products. Two distinct •QOOH isomers with radical sites at a primary carbon of one of the methyl groups (β-Me) or a secondary carbon (β-Et) of the ethyl group are identified by comparison with theoretically calculated IR absorption features for multiple conformers, including C–O, ethyl, and O–O torsions of the two isomers. Here, a master-equation analysis is developed and utilized to explore the conformational cooling process and the resultant conformer population distributions of the two isomers. Most of the IR features observed, including those in the strong fundamental and first overtone OH stretch regions as well as weaker combination bands involving OH stretch with torsion or OOH bend, are in good accord with computed anharmonic frequencies for the most populated conformers of the •QOOH_Et isomer. Relatively weak IR features most evident in the fundamental and first overtone OH stretch regions are ascribed to multiple conformers of the less stable •QOOH_Me isomer, along with a weak feature that is uniquely attributed to a combination band involving asymmetric CH 2 stretch and HCH bend of •QOOH_Me.

Chemical reaction jet spectroscopy↗
DOE OSTI2024

Development of Whole System Digital Twins for Advanced Reactors: Leveraging Graph Neural Networks and SAM Simulations

Here, in this work, we introduce a novel method to develop whole system digital twins (DTs) for advanced nuclear reactors. This method treats a complex reactor system as a heterogeneous graph: with the system components as different types of graph nodes and their physical interconnections as edges. Based on the heterogeneous graph, a graph neural network combining graph convolution and temporal node attention is developed as the DT, facilitating a comprehensive understanding of the system's dynamic behavior. By utilizing the System Analysis Module (SAM) code for simulating various operational transients, we develop a graph-based database that trains the DT. This DT is characterized by two primary functions: It can infer the entire system's status using sparse node information, and it can predict the progress of transients based on current and historical system information. Our approach is validated through case studies on the Experimental Breeder Reactor II (EBR-II) system and a generic Fluoride-salt-cooled High-temperature Reactor (gFHR), demonstrating the DT's accuracy in forecasting operational transients. The DT's rapid computation capabilities enhance its potential for supporting advanced reactor operations, offering benefits in intelligent simulation, autonomous control, and anomaly detection, paving the way for improved safety analysis and intelligent component health management for advanced reactor systems and reducing their operations and maintenance cost.

EBR-II↗
DOE OSTI2014

A COMPREHENSIVE X-RAY AND MULTIWAVELENGTH STUDY OF THE COLLIDING GALAXY PAIR NGC 2207/IC 2163

We present a comprehensive study of the total X-ray emission from the colliding galaxy pair NGC 2207/IC 2163, based on Chandra, Spitzer, and GALEX data. We detect 28 ultraluminous X-ray sources (ULXs), 7 of which were not detected previously because of X-ray variability. Twelve sources show significant long-term variability, with no correlated spectral changes. Seven sources are transient candidates. One ULX coincides with an extremely blue star cluster (B – V = –0.7). We confirm that the global relation between the number and luminosity of ULXs and the integrated star-formation rate (SFR) of the host galaxy also holds on local scales. We investigate the effects of dust extinction and age on the X-ray binary (XRB) population on subgalactic scales. The distributions of N {sub X} and L {sub X} are peaked at L {sub IR}/L {sub NUV} ∼ 1, which may be associated with an age of ∼10 Myr for the underlying stellar population. We find that approximately one-third of the XRBs are located in close proximity to young star complexes. The luminosity function of the XRBs is consistent with that typical for high-mass XRBs and appears unaffected by variability. We disentangle and compare the X-ray diffuse spectrum with that of the bright XRBs. The hot interstellar medium dominates the diffuse X-ray emission at E ≲ 1 keV and has a temperature kT=0.28{sub −0.04}{sup +0.05} keV and intrinsic 0.5-2 keV luminosity of 7.9×10{sup 40} erg s{sup −1}, a factor of ∼2.3 higher than the average thermal luminosity produced per unit SFR in local star-forming galaxies. The total X-ray output of NGC 2207/IC 2163 is 1.5×10{sup 41} erg s{sup −1}, and the corresponding total integrated SFR is 23.7 M {sub ☉} yr{sup –1}.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

The Simons Observatory: science goals and forecasts for the enhanced Large Aperture Telescope

We describe updated scientific goals for the wide-field, millimeter-wave survey that will be produced by the Simons Observatory (SO). Significant upgrades to the 6-meter SO Large Aperture Telescope (LAT) are expected to be complete by 2028, and will include a doubled mapping speed with 30,000 new detectors and an automated data reduction pipeline. In addition, a new photovoltaic array will supply most of the observatory's power. The LAT survey will cover about 60% of the sky at a regular observing cadence, with five times the angular resolution and ten times the map depth of the Planck satellite. The science goals are to: (1) determine the physical conditions in the early universe and constrain the existence of new light particles; (2) measure the integrated distribution of mass, electron pressure, and electron momentum in the late-time universe, and, in combination with optical surveys, determine the neutrino mass and the effects of dark energy via tomographic measurements of the growth of structure at redshifts z ≲ 3; (3) measure the distribution of electron density and pressure around galaxy groups and clusters, and calibrate the effects of energy input from galaxy formation on the surrounding environment; (4) produce a sample of more than 30,000 galaxy clusters, and more than 100,000 extragalactic millimeter sources, including regularly sampled AGN light-curves, to study these sources and their emission physics; (5) measure the polarized emission from magnetically aligned dust grains in our Galaxy, to study the properties of dust and the role of magnetic fields in star formation; (6) constrain asteroid regoliths, search for Trans-Neptunian Objects, and either detect or eliminate large portions of the phase space in the search for Planet 9; and (7) provide a powerful new window into the transient universe on time scales of minutes to years, concurrent with observations from the Vera C. Rubin Observatory of overlapping sky.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

A Search for Pulsars around Sgr A* in the First Event Horizon Telescope Data Set

In 2017 the Event Horizon Telescope (EHT) observed the supermassive black hole at the center of the Milky Way, Sagittarius A* (Sgr A*), at a frequency of 228.1 GHz (λ = 1.3 mm). The fundamental physics tests that even a single pulsar orbiting Sgr A* would enable motivate searching for pulsars in EHT data sets. The high observing frequency means that pulsars—which typically exhibit steep emission spectra—are expected to be very faint. However, it also negates pulse scattering, an effect that could hinder pulsar detections in the Galactic center. Additionally, magnetars or a secondary inverse Compton emission could be stronger at millimeter wavelengths than at lower frequencies. We present a search for pulsars close to Sgr A* using the data from the three most sensitive stations in the EHT 2017 campaign: the Atacama Large Millimeter/submillimeter Array, the Large Millimeter Telescope, and the IRAM 30 m Telescope. We apply three detection methods based on Fourier-domain analysis, the fast folding algorithm, and single-pulse searches targeting both pulsars and burst-like transient emission. We use the simultaneity of the observations to confirm potential candidates. No new pulsars or significant bursts were found. Being the first pulsar search ever carried out at such high radio frequencies, we detail our analysis methods and give a detailed estimation of the sensitivity of the search. We conclude that the EHT 2017 observations are only sensitive to a small fraction (≲2.2%) of the pulsars that may exist close to Sgr A*, motivating further searches for fainter pulsars in the region.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
NASA NTRS1988

Vacuum weathering of sulfur - Temperature effects and applications to Io

The effect of surface temperature on the initial transient and subsequent steady-state behavior of the vacuum-sublimation rate and the UV/visible spectral reflectance of frozen sulfur has been investigated. Surface temperature is found to be the dominant parameter controlling the rate of vacuum weathering of sulfur. The present results suggest that any freshly-frozen sulfur deposits on Io at typical Io hotspot temperatures should display major transient changes in color in a matter of hours to days. It is noted that these rapid changes in spectral reflectivity should be readily detectable by future high-resolution synotopic observations of Io spectrum in the UV/visible.

Nash, Douglas B.↗
NASA NTRS1994

Superhumps in cataclysmic binaries. 3: V795 Herculis

We report photometry of the cataclysmic variable V795 Herculis during 1990-1994. Comparison of recent with previously published data shows that the 2.78-hr periodicity has essentially disappeared; the amplitude has diminished by a factor of at least 10. In its place, there is a low-amplitude signal near the radial-velocity (orbital?) period of 2.60 hr. During 1983-1989, the star did show an obvious 2.78-hr signal. We study the published data on this signal, together with our own data under the (questionable) assumption that the signal still exists with an amplitude too small to survive the rigors of unbiased period detection. The data are really too sparse and too poorly distributed to decide the issue of phase stability. But since the photometric signal is transient and exceeds the likely orbital period by approximately 8%, the photometric waves are likely to be yet another example of 'superhumps', the phenomenon made famous by dwarf novae in superoutburst. At high frequencies, the star shows a quasi-periodic signal with P approximately 1160 s, and possibly also a stable signal with P = 1310.2 s (or 1330.4 s, the one-day alias). The beat period between these signals could be the orbital period, or that of the vanished superhump.

Patterson, Joseph↗
NASA NTRS1999

Analytical Assessment of a Gross Leakage Event Within the International Space Station (ISS) Node 2 Internal Active Thermal Control System (IATCS)

Results of the International Space Station (ISS) Node 2 Internal Active Thermal Control System (IATCS) gross leakage analysis are presented for evaluating total leakage flowrates and volume discharge caused by a gross leakage event (i.e. open boundary condition). A Systems Improved Numerical Differencing Analyzer and Fluid Integrator (SINDA/FLUINT) thermal hydraulic mathematical model (THMM) representing the Node 2 IATCS was developed to simulate system performance under steady-state nominal conditions as well as the transient flow effects resulting from an open line exposed to ambient. The objective of the analysis was to determine the adequacy of the leak detection software in limiting the quantity of fluid lost during a gross leakage event to within an acceptable level.

Holt, James M.↗
NASA NTRS2001

Analytical Assessment of a Gross Leakage Event Within the International Space Station (ISS) Node 2 Internal Active Thermal Control System (IATCS)

Results of the International Space Station (ISS) Node 2 Internal Active Thermal Control System (IATCS) gross leakage analysis are presented for evaluating total leakage flow rates and volume discharge caused by a gross leakage event (i.e. open boundary condition). A Systems Improved Numerical Differencing Analyzer and Fluid Integrator (SINDA85/FLUINT) thermal hydraulic mathematical model (THMM) representing the Node 2 IATCS was developed to simulate system performance under steady-state nominal conditions as well as the transient flow effect resulting from an open line exposed to ambient. The objective of the analysis was to determine the adequacy of the leak detection software in limiting the quantity of fluid lost during a gross leakage event to within an acceptable level.

Holt, James M.↗
NASA NTRS2006

Swift: Results from the first year of the mission

The Swift gamma-ray burst explorer was launched on Nov. 20,2004 from Cape Canaveral, Florida. The first instrument onboard became fully operational less than a month later. Since that time the Burst Alert Telescope (BAT) on Swift has detected more than one hundred gamma-ray bursts (GRBs), most of which have also been observed within two minutes by the Swift narrow-field instruments: the X-Ray Telescope (XRT) and the Ultra-Violet and Optical Telescope (UVOT). Swift trigger notices are distributed worldwide within seconds of the trigger through the Gamma-ray burst Coordinates Network (GCN) and a substantial fraction of GRBs have been followed up by ground and space-based telescopes, ranging in wavelength from radio to TeV. Results have included the first rapid localization of a short GRB and further validation of the theory that short and long bursts have different origins; detailed observations of the short-term power-law decay of burst afterglows leading to an improved understanding of the fireball model; and detection of the most distant GRB ever found. Swift is also a sensitive X-ray observatory with capabilities to monitor galactic and extragalactic transients on a daily basis, carry out the first all-sky hard X-ray survey since HEAO-1, and study in detail the spectra of X-ray transients. significant results, both in GRB science and in the search for and study of hard X-ray sources. In this talk I will provide a broad overview of the Swift mission and its most significant results, both in GRB science and in the search for and study of hard X-ray sources.

Krimm, H. A.↗