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NASA NTRS2007

Observations of Lightning on Earth from the Lunar Surface

The NASA Optical Transient Detector (OTD) launched into a 70deg inclination orbit in April 1995 aboard the MicroLab-1 satellite and the Lightning Imaging Sensor (LIS) launched into a 35deg inclination orbit in November 1997 (and still operating today) aboard the Tropical Rainfall Measuring Mission have produced the most comprehensive global observations of lightning activity on Earth. The OTD collected data for 5-yr from an altitude of 740 km while the LIS, in its 10th year of operations, is still collecting data from its current altitude of 402 km. From these altitudes the OTD observes an individual storm within its field of view for approx.3 min and the LIS for approx.90 sec as the satellites orbit the earth. Figures 1-4 show the combined LIS/OTD distribution of lightning for day and night during the Northern Hemisphere warm season from April through August (Fig. 1,2) and the cool season from October through February (Fig. 3,4) as might be observed from the lunar surface (12-h daylight and 12-h nighttime observations). The day and night plots are for the twelve hour periods centered on local noon and midnight. The total viewtime of the global lightning activity is 200 hours or less, depending on latitude (Fig. 5). Most of the observed lightning occurs over the northern hemisphere land areas as reported in previous studies. More lightning activity is seen at the higher northern latitudes during the day. The greatest lightning maxima occurs in the southeastern US, during the day. The corresponding region at night shows much less lightning activity. In contrast, there is a maxima in lightning activity at night over the high Plains area of the U.S. This region had lower lightning rates during the daytime period. During the cold season, the southern hemisphere has significantly more lightning. The maxima in Central Africa is still present, and a secondary maxima is observed in South Africa. In South America, the maxima in Argentina occurs at night in association with large-scale mesoscale convective storm complexes. This is the region on the earth having the greatest frequency of extreme storms with flash rates exceeding 1000 flashes/min. daytime maxima is seen extending from Northern Argentina to Brazil. In the US., the Gulf of Mexico and the Gulf Coast states exhibit a maximum in lightning activity both day and night.

Goodman, S. J.↗

NASA NTRS2008

Seasonal Snow Extent and Snow Mass in South America using SMMR and SSM/I Passive Microwave Data (1979-2006)

Seasonal snow cover in South America was examined in this study using passive microwave satellite data from the Scanning Multichannel Microwave Radiometer (SMMR) on board the Nimbus-7 satellite and the Special Sensor Microwave Imagers (SSM/I) onboard Defense Meteorological Satellite Program (DMSP) satellites. For the period from 1979-2006, both snow cover extent and snow water equivalent (snow mass) were investigated during the coldest months (May-September), primarily in the Patagonia area of Argentina and in the Andes of Chile, Argentina and Bolivia, where most of the seasonal snow is found. Since winter temperatures in this region are often above freezing, the coldest winter month was found to be the month having the most extensive snow cover and usually the month having the deepest snow cover as well. Sharp year-to-year differences were recorded using the passive microwave observations. The average snow cover extent for July, the month with the greatest average extent during the 28-year period of record, is 321,674 km(exp 2). In July of 1984, the average monthly snow cover extent was 701,250 km(exp 2) the most extensive coverage observed between 1979 and 2006. However, in July of 1989, snow cover extent was only 120,000 km(exp 2). The 28-year period of record shows a sinusoidal like pattern for both snow cover and snow mass, though neither trend is significant at the 95% level.

Foster, J. L.↗

NASA NTRS2007

Seasonal Snow Extent and Snow Mass in South America Using SMMR and SSM/I Passive Microwave Data (1979-2003)

Seasonal snow cover in South America was examined in this study using passive microwave satellite data from the Scanning Multichannel Microwave Radiometer (SMMR) on board the Nimbus-satellite and the Special Sensor Microwave Imagers (SSM/I) on board Defense Meteorological Satellite Program (DMSP) satellites. For the period from 1979-2003, both snow cover extent and snow depth (snow mass) were investigated during coldest months (May-September), primarily in the Patagonia area of Argentina and in Chile. Most of the seasonal snow in South America is in the Patagonia region of Argentina. Since winter temperatures in this region are often above freezing, the coldest winter month was found to be the month having the most extensive snow cover and also usually the month having the deepest snow cover as well. Sharp year-to-year differences were recorded using the passive microwave observations. The average snow cover extent for July, the month with the greatest average snow extent during the 25-year period of record, is 320,700 km(exp 2). In July of 1984, the average monthly snow cover was 701,250 km(exp 2) - the most extensive coverage observed between 1979 and 2003. However, in July of 1989, snow cover extent was only 120 km(exp 2). The 25-year period of record shows a sinusoidal like pattern, though there appears to be no obvious trend in either increasing or decreasing snow extent or snow mass between 1979 and 2003.

Foster, J. L.↗

NASA NTRS2018

Early Results from the RELAMPAGO Lightning Mapping Array

In austral spring of 2018, an 11station NASA lightning mapping array (LMA) will be installed in the Cordoba region of Argentina, in support of GOES16/ 17 Geostationary Lightning Mapper (GLM) calibration and validation, as well as the Remote sensing of Electrification, Lightning, And Mesoscale/microscale Processes with Adaptive Ground Observations (RELAMPAGO) field campaign. This region of Argentina is well known for frequent, intense thunderstorms and severe weather. Lightning observations in storms that initiate, become severe, and grow upscale are expected to be obtained by GLM and the LMA during the LMA’s multimonth deployment. We hypothesize that, similar to the analogous U.S. High Plains, anomalously charged thunderstorms with frequent inverted lightning at low levels are common in this region, which may have implications for GLM detection efficiency. Deployment logistics and experimental approach will be explained, and some early results from the LMA (including comparison to GLM) will be presented.

Lang, Timothy↗

NASA NTRS2019

The RELAMPAGO Lightning Mapping Array: Preliminary Scientific Results and Application to GLM Calibration and Validation

During November 2018 through April 2019, an 11-station NASA lightning mapping array (LMA) was installed in the Cordoba region of Argentina, in support of GOES-16 Geostationary Lightning Mapper (GLM) calibration and validation, as well as the Remote sensing of Electrification, Lightning, And Mesoscale/microscale Processes with Adaptive Ground Observations (RELAMPAGO) field campaign. This region of Argentina is well known for frequent, intense thunderstorms and severe weather. The LMA was monitored remotely via the Internet throughout its deployment, but due to bandwidth limitations no real-time data were available. Custom GOES-16 imagery provided by NASA SPoRT assisted with monitoring of thunderstorm cases. Occasional site visits were done to obtain data disks, perform routine maintenance, and troubleshoot problems. During the deployment the network captured lightning in a variety of storm modes, including ordinary and severe multicells, supercells, and mesoscale convective systems. Many examples of normal-polarity thunderstorms, as well as a few examples of anomalously charged thunderstorms, were observed. Long (100+ km) horizontally stratified lightning flashes, as well as lightning in overshooting tops, also were frequently observed. Supporting research radar observations were available through January 2019, with operational radar coverage available after that time. Some cases featured supporting ABI meso scanning. This presentation will report on the LMA deployment in context with the RELAMPAGO field campaign, show results from some representative case studies, and will provide initial comparisons to GLM observations.

Lang, Timothy J.↗

NASA NTRSDate not supplied

Hail Storm Risk Assessment Using Space-Borne Remote Sensing Observations and Reanalyses

Much of the world is impacted by severe thunderstorms, but whether they become disasters depends upon resilience--our capacity to prepare, mitigate, respond, and recover. Hail is the costliest severe weather hazard for the insurance industry, generating ~70% of severe convective storm losses due to damage to assets such as homes, businesses, agriculture, and infrastructure. Most insurance companies do not reserve enough capital to cover catastrophes, so they acquire reinsurance. The reinsurance industry uses catastrophe models (CatModels) to statistically estimate risk to an insurer’s portfolio. Hail CatModels are developed with climatologies that define hailstorm frequency and severity. Hail-prone areas can be defined using hail reports from trained spotters, the media, and the general public. Extremely severe hail (2+ inch diameter) occurs nearly every day across the world. Weather radars can detect hail because hailstones strongly reflect microwave signals that they emit. However, hail climatologies are difficult to derive because hail covers small areas and there are neither hail reporting mechanisms (e.g. website or mobile app) nor radar networks in most places outside the US and Europe. This lack of ground truth on severe hail puts society and economies at risk. Hail is generated within storms by strong updrafts. These updrafts exhibit unique signatures in NASA and other agency satellite observations, offering new opportunities for hailstorm analysis. Geostationary (GEO) visible and infrared imagery has been collected for ~15-25 years across the world (region dependent) and methods have been developed at NASA Langley Research Center (LaRC) to detect hailstorm updrafts using GEO imagery. Climatological GEO updraft data has been used by Willis Towers Watson (WTW), a leader in catastrophe risk assessment for the insurance industry, and Karlsruhe Institute of Technology to develop CatModels over Europe and Australia. Hail can also be inferred with passive microwave imagery collected by low-Earth-orbiting sensors such as the GPM GMI, TRMM TMI, AMSR-E, AMSR-2, SSM/I, and SSMIS over the last 20+ years using methods developed at the Marshall Space Flight Center (MSFC). Hailstorms generate enhanced lightning flash rates that can be tracked using new GOES-R series GEO Lightning Mapping (GLM) imagery. Atmospheric reanalyses can be used to define favorable hailstorm environments for combination with the satellite-based storm detections. This presentation will describe a framework for developing continental to global hail climatologies and CatModels based on NASA satellite data and capabilities. This is a collaboration between LaRC and MSFC, WTW, and partners in Brazil, Argentina, and South Africa. This project seeks to mitigate hail disasters by aiding development of new satellite-based severe storm nowcasting tools by regional partners and developing climatologies to improve societal understanding of hail frequency. GEOO visible and infrared metrics of storm intensity, environmental conditions based on reanalyses, spotter hail reports and radar MESH observations are intercompared to quantify the detectability of hailstorms, and our ability to discriminate hailstorms from other severe storms. We are also maturing methods using land surface imaging satellite data (e.g. MODIS, Landsat, Sentinel 1 and 2) to identify hail damage to agriculture. Work with WTW will improve socioeconomic resilience through development of new CatModels. Southern Brazil, Uruguay, Paraguay, and Argentina feature some of the most intense thunderstorms on Earth. South America and South Africa are developing insurance markets of interest to WTW clients, and is similar to other regions routinely impacted by hail that do not have comprehensive hail reporting or radars to assess hailstorm frequency. Project datasets will be made available via online GIS-enabled tools developed at the LaRC Atmospheric Science Data Center (ASDC) which will visualize data and provide it in multiple formats for use in a wide range of open source and commercial tools.

Kristopher Michael Bedka↗

NASA NTRS2024

Interannual Lightning Variability within the TRMM LIS Dataset Using an ENSO Perspective

The Tropical Rainfall Measuring Mission (TRMM) Lightning Imaging Sensor (LIS) was used to investigate inter-annual variability of lightning from 1998-2014 within the 38° S – 38° N range. Previous studies have indicated that the El-Niño/Southern Oscillation (ENSO) phenomenon is one significant contributor to inter-annual lightning variability, potentially the dominant mechanism on the global scale. This period of 16 years contained four warm- (El Niño), eight cold- (La Niña), and four neutral-phase ENSO years based on the oceanic Niño index. Large magnitude lightning anomalies were found during the warm phase of ENSO, with mean warm-phase anomalies of > 10 Fl (1000 km) −2 min −1 in north-central Africa and Argentina. This includes a +35 Fl (1000 km) −2 min −1 anomaly in Argentina during the 2009 El Niño. In general, large-scale anomalies of thermodynamic properties and upper-atmospheric vertical motion coincided with the lightning anomalies observed in both Africa and South America. The anomaly over north-central Africa, however, was characterized by a 6-week shift in the annual lightning maximum with the warm phase, a result of the more complex environmental response to ENSO over the Sahel. The most consistent ENSO anomalies with appreciable lightning were found in southeastern Africa, northwestern Brazil, central Mexico, and the southern Red Sea. Of these, all but the Mexico region had enhanced lightning with the cold phase and suppressed lightning with the warm phase.

Austin G. Clark↗

NASA NTRSDate not supplied

Version 8 of the SMAP Level-4 Soil Moisture Data Assimilation Product

The NASA Soil Moisture Active Passive (SMAP) mission Level-4 Soil Moisture (L4_SM) product provides global, 9-km resolution, 3-hourly surface (0-5 cm) and root-zone (0-100 cm) soil moisture from April 2015 to present with a mean latency of 2.5 days from the time of observation. The product is based on the assimilation of SMAP L-band (1.4 GHz) brightness temperature (Tb) observations into the NASA Catchment land surface model as the model is driven with observations-based precipitation forcing. This presentation discusses the improvements in the forthcoming Version 8 of L4_SM, including updates in the precipitation forcing, the Catchment model parameters, and the L-band microwave radiative transfer model (mwRTM). The precipitation observations used in L4_SM Version 8 outside of North America and the high latitudes are from the latest (Version 7) NASA Integrated Multi-satellitE Retrievals for the Global Precipitation Measurement mission (IMERG) products. Moreover, occasionally excessive precipitation rates in earlier versions of L4_SM along certain longitudes in North America were eliminated by a bug fix in the precipitation corrections algorithm. The Catchment model in L4_SM Version 8 uses climatological snow albedo values based on observations from the Moderate Resolution Imaging Spectroradiometer, replacing the look-up table parameterization of earlier versions. Additionally, corrected soil parameters were implemented for a small region in Argentina that had erroneously been classified as peat because of an error in the ancillary soil data. Finally, the mwRTM in L4_SM Version 8 uses the Mironov soil mixing approach and updated values of the L-band scattering albedo, soil roughness, and vegetation opacity climatology obtained from the latest (Release 19) SMAP Level-2 dual-channel soil moisture retrieval product. During the development of L4_SM Version 8, the change in the mwRTM parameterization resulted in a reduced unbiased RMSE of surface soil moisture when verified against in situ measurements. It also reduced the standard deviation of the Tb observation-minus-forecast residuals by ~0.15 K, highlighting the importance of the mwRTM for successful data assimilation. The bug fixes in the precipitation corrections algorithm and the Catchment model soil parameters in the Argentina region result in locally large improvements of the simulated land surface states. In summary, the ongoing refinements of the L4_SM product continue to improve its science quality and performance for global soil moisture monitoring

Rolf Reichle↗

NASA NTRS2017

Unexpected Climatological Behavior of MLT Gravity Wave Momentum Flux in the Lee of the Southern Andes Hot Spot

The Southern Argentina Agile MEteor Radar (SAAMER), located at Tierra del Fuego (53.7degS, 67.7degW), has been providing near-continuous high-resolution measurements of winds and high-frequency gravity wave (GW) momentum fluxes of the mesopause region since May 2008. As SAAMER is located in the lee of the largest seasonal GW hot spot on Earth, this is a key location to study GWs and their interaction with large-scale motions. GW momentum flux climatologies are shown for the first time for this location and discussed in light of these unique dynamics. Particularly, the large eastward GW momentum fluxes during local winter are surprising, as these observations cannot be explained by the direct upward propagation of expected large-amplitude mountain waves (MWs) through the eastward stratospheric jet. Instead, these results are interpreted as secondary GWs propagating away from stratospheric sources over the Andes accompanying MW breaking over the Southern Andes.

Southern Argentina Agile MEteor Radar↗

DOE OSTI2024

Deployment and performance of a Low-Energy-Threshold Skipper-CCD inside a nuclear reactor

Charge Coupled Devices (CCD) are being used for reactor neutrino experiments and have already demonstrated their potential in constraining new physics models. The prospect of a Skipper-CCD experiment looking for standard and beyond standard model (BSM) physics in a nuclear reactor has been evaluated for different benchmark scenarios. Here, we report the first installation of a 2-g Skipper-CCD inside the containment building of a 2 GW th nuclear power plant and analyze its performance throughout its first 18 months of operation. The sensor was successfully deployed at Atucha II, in Argentina, 12 meters away from the center of the reactor core. We discuss the challenges involved in the commissioning of the detector and present data acquired during reactor ON and reactor OFF periods, with the sensor functioning with a sub-electron readout noise of 0.17 e - . Based on an exposure of 56.8 g day reactor ON and two reactor OFF data sets with a total exposure of 118.1 g day we characterize the system and evaluate the sensitivity to CEvNS. We achieved a background rate of 33 kdru and a low threshold of 45 eV ee . The ongoing efforts to improve sensitivities to CEvNS and BSM interaction are also discussed.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2023

Exploring sustainable electricity system development pathways in South America’s MERCOSUR sub-region

South America has abundant natural water and energy resources, and exploiting these resources to achieve a clean energy future is central to the continent’s economic and sustainable development objectives for the next several decades. Designing pathways to achieving this clean energy future requires better understanding the structural, techno-economic, and policy forces that may influence the future development of the electricity sector in the region. Here, we focus on an interconnected electricity system of five South American countries – Argentina, Brazil, Chile, Paraguay, and Uruguay – which represent major electricity generation, consumption, and trade dynamics in the region. We explore the implications of various forces that could shape the future composition of the power sector in the sub-region, including: evolving renewable energy cost and performance, natural gas prices, cross-border interconnection facilities, early retirement of installed hydropower, and different decarbonization goals. We use a model framework based on a power system planning platform (GridPath) to co-optimize investment and operations of generation, storage, and transmission facilities out to 2050. Our results in a Reference scenario indicate that the electricity system can maintain a relatively clean energy portfolio by leveraging existing hydropower capacity and integrating increasingly cost-competitive wind and solar power. However, dependence on natural gas in the region is likely to remain high. A low-carbon electricity system can cost-effectively be achieved through policy interventions (e.g., renewable portfolio standards) and by diversifying investments in wind, solar, battery storage, and some new hydropower capacity. We also find that existing hydropower is critical for maintaining reliable future grid operations. Enhanced regional electricity trade, mostly based on existing interconnection capacities with nominal investment in new transmission, can significantly benefit the clean energy transition in the region.

29 ENERGY PLANNING, POLICY, AND ECONOMY↗

DOE OSTI2023

Aperture size distribution, length, and preferential location of bed-parallel veins in shale

Bed-parallel, calcite-filled veins (BPVs) are common in shale formations, and although they have been widely described in other studies, little is known about their population aperture size distribution. To address this knowledge gap, we analyzed BPV sizes in outcrops and cores from the Vaca Muerta Formation, Neuquén Basin, Argentina; in two cores from the Marcellus Formation, Appalachian Basin, northeast Pennsylvania; and in one core from the Wolfcamp Shale, Delaware Basin, West Texas. Nine out of ten aperture size populations follow a negative exponential distribution, with one following a weak power law. Bed-parallel vein size distribution and intensity vary among formations and within the same shale. We define three groups of distributions: (1) Vaca Muerta outcrops, with the highest BPV intensity and the largest BPVs (cumulative frequency of 4.9 BPVs per meter [BPVs/m] for apertures 0.265 mm to 8.7 cm); (2) Vaca Muerta cores with a similar BPV intensity overall but with no apertures wider than 1.2 cm; and (3) Vaca Muerta, Wolfcamp, and Marcellus cores with the fewest BPVs (cumulative frequency up to 0.63 BPVs/m) and very few wider than 1 cm. Aperture and length in two outcrop data sets are weakly positively correlated and follow power laws with exponents of 0.44 and 0.49. Mechanical interfaces at boundaries between different lithologies exert a strong control on BPV location, with 65–75% of observed interfaces having BPVs along them. Only 25–30% of the BPVs occur at observed material interfaces, however, and unless subtle, unobserved mechanical layering is present, other factors must also control location. BPV intensity and organic richness (TOC) from Vaca Muerta well logs are correlated in some instances but not in others, indicating TOC is not always a good proxy for BPV location or intensity. Furthermore, these findings provide useful information for modeling of hydraulic fracture treatments where BPVs may influence development of the stimulated fracture network, for example by limiting height growth.

58 GEOSCIENCES↗

DOE OSTI2020

A 3-Year Sample of Almost 1,600 Elves Recorded Above South America by the Pierre Auger Cosmic-Ray Observatory

Elves are a class of transient luminous events, with a radial extent typically greater than 250 km, that occur in the lower ionosphere above strong electrical storms. We report the observation of 1,598 elves, from 2014 to 2016, recorded with unprecedented time resolution (100 ns) using the fluorescence detector (FD) of the Pierre Auger Cosmic-Ray Observatory. The Auger Observatory is located in the Mendoza province of Argentina with a viewing footprint for elve observations of 3∙10sup>6 km ₂, reaching areas above the Pacific and Atlantic Oceans, as well as the Córdoba region, which is known for severe convective thunderstorms. Primarily designed for ultrahigh energy cosmic-ray observations, the Auger FD turns out to be very sensitive to the ultraviolet emission in elves. The detector features modified Schmidt optics with large apertures resulting in a field of view that spans the horizon, and year-round operation on dark nights with low moonlight background, when the local weather is favorable. The measured light profiles of 18% of the elve events have more than one peak, compatible with intracloud activity. Within the 3-year sample, 72% of the elves correlate with the far-field radiation measurements of the World Wide Lightning Location Network. The Auger Observatory plans to continue operations until at least 2025, including elve observations and analysis. To the best of our knowledge, this observatory is the only facility on Earth that measures elves with year-round operation and full horizon coverage.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2020

New World Meteorological Organization Certified Megaflash Lightning Extremes for Flash Distance (709 km) and Duration (16.73 s) Recorded From Space

Identification and validation of atmospheric extremes are essential to monitoring climate change, to addressing engineering and safety concerns, and to promoting technological advancement. An international World Meteorological Organization evaluation committee has critically adjudicated and recommended acceptance of two lightning megaflash events (horizontal mesoscale lightning discharges of >100 km in length) as new global extremes using analysis of Geostationary Lightning Mapper data. The world's greatest extent for an individual lightning flash is a single flash that covered a horizontal distance of 709 ± 8 km (441 ± 5 mi) across parts of southern Brazil on 31 October 2018. Furthermore, the greatest duration for a single lightning flash is 16.730 ± 0.002 s from a flash that developed continuously over northern Argentina on 4 March 2019.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2020

Distinctive Signals in 1-min Observations of Overshooting Tops and Lightning Activity in a Severe Supercell Thunderstorm

This work examines a severe weather event that took place over central Argentina on December 11, 2018. The evolution of the storm from its initiation, rapid organization into a supercell, and eventual decay was analyzed with high-temporal resolution observations. This work provides insight into the spatio-temporal co-evolution of storm kinematics (updraft area and lifespan), cloud-top cooling rates, and lightning production that led to severe weather. The analyzed storm presented two convective periods with associated severe weather. An overall decrease in cloud-top local minima IR brightness temperature (MinIR10.3), increase in overshooting top area, and lightning jump (LJ) preceded both periods. LJs provided the highest lead time to the occurrence of severe weather, with the ground-based lightning networks providing the maximum warning time of around 30 min. Lightning flash counts from the Geostationary Lightning Mapper (GLM) were underestimated when compared to detections from ground-based lightning networks. Among the possible reasons for GLM’s lower detection efficiency were an optically dense medium located above lightning sources and the occurrence of flashes smaller than GLM’s footprint. The minimum MinIR provided the shorter warning time to severe weather occurrence. However, secondary minima in MinIR10.3 that preceded the absolute minima improved this warning time by more than 10 min. Furthermore, trends in MinIR10.3 for time scales shorter than 6 min revealed shorter cycles of fast cooling and warming, which provided information about the lifecycle of updrafts within the storm. The advantages of using observations with high-temporal resolution to analyze the evolution and intensity of convective storms are discussed.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2022

River Organic Carbon Fluxes Modulated by Hydrodynamic Sorting of Particulate Organic Matter

Rivers regulate the global carbon cycle by transferring particulate organic carbon (POC) from terrestrial landscapes to marine sedimentary basins, but the processes controlling the amount and composition of fluvially exported POC are poorly understood. We propose that hydrodynamic sorting processes modify POC fluxes during fluvial transit. We test this hypothesis by studying POC transported along a ~1,200 km reach of the Rio Bermejo, Argentina. Nanoscale secondary ion mass spectrometry revealed that POC was either fine, mineral-associated organic matter, or coarse discrete organic particles. Mineral-associated POC is more resistant to oxidation and has a lower particle settling velocity than discrete POC. Consequently, hydraulic sorting and downstream fining amplify the proportion of fine, mineral-associated POC from ~55% to ~78% over 1,220 km of downstream transit. This suggests that mineral-associated POC has a greater probability of export and preservation in marine basins than plant detritus, which may be oxidized to CO 2 during transit.

58 GEOSCIENCES↗

DOE OSTI2021

Ice Nucleating Particle Connections to Regional Argentinian Land Surface Emissions and Weather During the Cloud, Aerosol, and Complex Terrain Interactions Experiment

Abstract Here, we present a multi‐season study of ice‐nucleating particles (INPs) active via the immersion freezing mechanism, which took place in north‐central Argentina, a worldwide hotspot for mesoscale convective storms. INPs were measured untreated, after heating to 95°C, and after hydrogen peroxide digestion. No seasonal cycle of INP concentrations was observed. Heat labile INPs, which we define as “biological” herein, dominated the population active at −5 to −20°C, while non‐heat‐labile organic INPs (decomposed by peroxide) dominated at lower temperatures, from −20 to −28°C. Inorganic INPs (remaining after peroxide digestion), were minor contributors to the overall INP activity. Biological INP concentration active around −12°C peaked during rain events and under high relative humidity, reflecting emission mechanisms independent of the background aerosol concentration. The ratio of non‐heat‐labile organic and inorganic INPs was generally constant, suggesting they originated from the same source, presumably from regional arable topsoil based on air mass histories. Single particle mass spectrometry showed that soil particles aerosolized from a regionally common agricultural topsoil contained known mineral INP sources (K‐feldspar and illite) as well as a significant organic component. The INP activity observed in this study correlates well with agricultural soil INP activities from this and other regions of the world, suggesting that the observed INP spectra might be typical of many arable landscapes. These results demonstrate the strong influence of regional continental landscapes, emitting INPs of types that are not yet well represented in global models.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2022

The Amazon and La Plata River Basins as Moisture Sources of South America: Climatology and Intraseasonal Variability

Abstract Land‐atmosphere interactions are critical for precipitation (PPT) over South America where terrestrial evapotranspiration (ET) constitutes a significant fraction of moisture for rainfall over the ecologically and socio‐economically vital Amazon (AMZ) and La Plata (LPB) river basins. We quantify the contribution of ET from AMZ and LPB to PPT over the continent with a focus on the intraseasonal time scale. Using numerical water tracers embedded in the Weather Research and Forecasting model we track the moisture originating from the two basins. Our findings indicate that approximately 40% of annual rainfall over the eastern foothills of the Andes originates as AMZ ET, and nearly 30% of rainfall over northern Argentina originates as LPB ET. Analysis of moisture transport during both phases of the dominant intraseasonal oscillation pattern over South America reveals an intraseasonal “sloshing” of LPB moisture between the South Atlantic convergence zone (SACZ) and southeastern South America (SESA) regions. AMZ and LPB each supply approximately 6% of moisture for SACZ PPT during periods of intraseasonal enhancement (positive anomalies), highlighting the importance of moisture from the Atlantic Ocean. For the SESA region, LPB supplies 26% of the moisture for PPT during periods of intraseasonal enhancement while AMZ supplies 5%.

54 ENVIRONMENTAL SCIENCES↗