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Results for “Carbon dioxide removal technology”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 109 records · Page 6
All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

CRADA Number NFE-22-09333 with Holocene Climate Corporation (CRADA Final Report:)

Holocene Climate Corporation has developed and scaled up a novel technology for Direct Air Capture (DAC) that is based on cutting-edge research initiated at Oak Ridge National Laboratory (ORNL). According to the IPCC, carbon dioxide capture from the air and its sequestration are necessary to keep global temperature rise below 1.5°C by 2050. DAC is a viable and practical way to reach this goal. DAC can happen anywhere in the world, takes up a fraction of the land of forests, and along with the sequestration of CO 2 , provides permanent and verifiable removal of carbon from the atmosphere. The proposed project aimed to facilitate knowledge transfer from ORNL to Holocene focusing on (i) the synthesis of the ORNL patented material which builds the cornerstone of the DAC technology, and (ii) required analytical methods needed to conduct crystallization bench-scale experimentation and technology development. Furthermore, ORNL conducted research centered around CO 2 absorption using an air-liquid contacting structure with an aqueous amino acid solution. The achievements under this project comprise successful knowledge transfer from ORNL to the entire Holocene team to jump-start their internal R&D and technological development activities.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Bioenergy pathways within United States net-zero CO 2 emissions scenarios in the Energy Modeling Forum 37 study

The Energy Modeling Forum 37 study is organized around carbon dioxide (CO 2 ) mitigation scenarios reaching net-zero CO 2 emissions by 2050 in the United States. Here, this paper summarizes the potential contribution of bioenergy use in the electric power, transportation, industrial, and buildings sectors toward meeting that target based on model results. Thirteen modeling teams reported bioenergy consumption in the Reference and Net Zero scenarios. Consumption of bioenergy increased over time in the Reference scenario, from an average across models of 3.2 exajoules (EJ) in 2020 to 3.8 EJ in 2050. Average bioenergy consumption in 2050 increased further to 7.3 EJ in the Net Zero scenario. All scenarios that reach net-zero emissions required some form of carbon dioxide removal to offset emissions that are difficult to reduce. Carbon dioxide removal using bioenergy with CO 2 capture and storage (BECCS) varies widely across models, up to 1000 Mt CO 2 in 2050. Some models rely instead on direct air carbon capture and storage (DACCS), up to 2200 Mt CO 2 , and others use a combination of BECCS and DACCS. Model results show a strong inverse relationship between the amounts of BECCS and DACCS deployed. All modeling teams assumed a carbon sink from land use, land use change, and forestry, further offsetting a portion of emissions from fossil fuels and industry that are expensive to eliminate. Bioenergy consumption in 2050 decreased by an average of 1.5 EJ across eight models in a Net Zero+ scenario relative to the Net Zero scenario, due in part to a lower equilibrium carbon price resulting from optimistic cost assumptions for all energy technologies.

09 BIOMASS FUELS↗
DOE OSTI2025

Direct Air Capture Using Aqueous Amino Acid Solvents in a Crossflow Absorber

Carbon dioxide (CO 2 ) is the most abundant of all greenhouse gases (GHGs). CO 2 levels in the atmosphere are 50% higher than in the preindustrial era, trapping heat. CO 2 removal from the atmosphere by direct air capture (DAC) is needed to achieve the internationally agreed global temperature goals. The most common CO 2 capture technology is absorption by aminebased solvents in packed columns. Amino acid solutions have recently gained attention due to their advantages over traditional amine solvents. To be implemented effectively, DAC industrial processes need to handle large airflow rates in separation absorbers. The large air and solvent flow rates preclude the use of countercurrent columns due to high-pressure drops and the occurrence of flooding. Crossflow air−liquid absorbers are used to handle large air and liquid volumes due to their lower-pressure drop. The objective of this work is to study the influence of crossflow absorber geometric parameters and operating conditions on product formation and process efficiency. An already derived theoretical model for countercurrent absorbers has been modified to simulate the operation of a crossflow DAC absorber. The predictive model was implemented into a computer code that was used to study the efficiency of the processes as geometric equipment dimensions and operating parameters vary. Practical suggestions are made to design more efficient DAC processes.

Absorption↗
DOE OSTI2025

Dehydration Membrane Reactor for Production of Valuable Chemicals from CO 2 and H 2

GTI Energy and partners have been developing a technology for production of liquefied petroleum gas (LPG) from carbon dioxide (CO 2 ) and hydrogen (H 2 ) using a novel catalytic membrane reactor. The reactor contains a bi-functional catalyst for methanol synthesis and LPG synthesis, resulting in LPG production in a single reactor. A transformational dehydration membrane is used to remove water in situ, shifting the thermodynamic equilibrium towards product formation. As a result, CO 2 conversion as high as 90.2% and LPG yield as high as 60.5% were obtained at 300°C and 20 bara in the membrane reactor, which significantly exceed the literature results of the traditional reactors

03 NATURAL GAS↗
DOE OSTI2025

Filer City Biomass Carbon Removal and Storage (BiCRS) Net-Negative Study

NorthStar Clean Energy Company (NorthStar) conducted the Filer City Biomass Carbon Removal and Storage (BiCRS) Net-Negative Study to develop a conceptual design and cost estimate for retrofitting the TES Filer City Station with post-combustion carbon capture technology in Mainstee Michigan. The Filer City BiCRS Net-Negative Study allowed NorthStar and team to confirm the commercial feasibility of a post-combustion carbon capture system applied to biomass-fired boilers. At the time of the study, there were no operating facilities in the world with carbon capture applied to flue gas from woody biomass as proposed for Filer City. Due to the solvent-agnostic nature of B&W’s SolveBright™ technology, the team determined that multiple amines, both traditional and proprietary, would be capable of 95% CO 2 capture efficiency with the steam available from Filer City’s existing boilers after modifications to burn 100% biomass. Based on the cost estimates produced, NorthStar can now confirm the Filer City BiCRS Project is economically viable with a combination of tax credits available from the Inflation Reduction Act of 2022 and high-quality Carbon Dioxide Removal Credits sold on the Voluntary Carbon Market. The Filer City BiCRS project is uniquely positioned to become one of the first projects to capture and sequester large volumes of CO 2 from a biogenic source, removing existing CO 2 from the atmosphere. The unlimited version of the Filer City Biomass Carbon Removal and Storage (BiCRS) Net-Negative Study Final Technical Report is attached.

01 COAL, LIGNITE, AND PEAT↗
DOE OSTI2025

Wind-Driven Direct Air Capture System Using 3D Printed, Passive, Amine-Loaded Contactors (WEDAC)

This project advanced the development of a novel wind-driven direct air capture (WEDAC) system for removing carbon dioxide (CO 2 ) from the atmosphere. Our research focused on combining passive air contact with electrothermal desorption using specially designed carbon fiber modules, aiming to provide a scalable, low-cost, and energy-efficient alternative to conventional carbon capture systems.

36 MATERIALS SCIENCE↗
DOE OSTI2019

The effect of wood composition and supercritical CO 2 extraction on charcoal production in ferroalloy industries

This work demonstrates that the integration of supercritical carbon dioxide extraction with slow pyrolysis is an effective method for the production of value-added chemicals and charcoal that is an attractive alternative to coke for industry. Integration of technologies is key for the development of holistic biorefineries that exploit all parts of the biomass feedstock and generate little or ideally no waste. In fact, the use of waste or low valued wood fractions is attractive due to their plentiful abundance and lack of exploitation. Supercritical carbon dioxide has been demonstrated to be effective at the removal of over half of extractives from low quality wood and forestry wastes, which can account for up to 11 wt %, of the dried biomass in waste needles. High extractive yields by supercritical carbon dioxide extraction illustrates the potential of utilizing low quality wood as an alternative feedstock for the sustainable production of value-added chemicals. We report high yields of steroids and derivatives, terpenes and other plant metabolites were obtained in the extracts of needles, branches and bark. Importantly, supercritical carbon dioxide extraction had little impact neither on the physical properties of original wood nor on the yield of solid charcoal. This indicates that extraction by supercritical carbon dioxide can be used as a method for adding further value to the process by removal of bio-based chemicals, whilst still maintaining the yield of the solid fuel product. Moreover, the heat treatment temperature and supercritical carbon dioxide extraction had a significant impact on the tar yields during pyrolysis, leading to an increase in naphthalene, polycyclic aromatic hydrocarbons, aromatic and phenolic fractions with greater temperature. These results are promising as they show that the charcoal obtained from this renewable feedstock could be used as an alternative to fossil-based coke in applications including ferroalloy industries.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2026

Removal of Calcium and Silica from Simulated Blowdown Water Using CO 2 -Assisted Magnesium Electrocoagulation

Blowdown water from various industries and cooling facilities contains high concentrations of calcium (Ca), magnesium (Mg), silica, and corrosion inhibitors, which render the water unsuitable for discharge into surface water and wastewater treatment plants. Electrocoagulation (EC) is effective at removing Ca and silica. Here, in this study, Mg-alloy electrodes EC resulted in ∼91% silica removal at a 5400 C/L charge loading. Ca removal, however, was only 31%. To enhance Ca removal, carbon dioxide (CO 2 ) containing gas was introduced. CO 2 addition formed carbonate ions, which reacted with Ca/Mg ions to generate carbonate precipitates. Introducing 5% and 14% CO 2 , simulating natural gas-fired and coal-fired flue gas, enhanced Ca removal to 38% and 47%, respectively. Pure CO 2 facilitated 70% Ca removal, more than two times higher than that without CO 2 , while maintaining high silica removal. FTIR, XRD, and SEM-EDS analyses confirmed enhanced Ca/Mg carbonate formation upon CO 2 . In situ Raman spectroscopy was employed to monitor carbonate-ions formation. The results demonstrated carbonate-ions removal through Ca-carbonate formation after CO 2 addition. A techno-economic assessment showed that recycled electrode materials and flue gas lead to ∼3 times lower cost compared with conventional silica/Ca removal through chemical coagulation, softening, or membrane filtration. The study demonstrated that CO 2 addition removes high concentrations of Ca and silica ions from wastewaters at a competitive cost.

blowdown water↗
DOE OSTI2024

Capturing carbon dioxide from air with charged-sorbents

Emissions reduction and greenhouse gas removal from the atmosphere are both necessary to achieve net-zero emissions and limit climate change. There is thus a need for improved sorbents for the capture of carbon dioxide from the atmosphere, a process known as direct air capture. In particular, low-cost materials that can be regenerated at low temperatures would overcome the limitations of current technologies. In this work, we introduce a new class of designer sorbent materials known as ‘charged-sorbents’. These materials are prepared through a battery-like charging process that accumulates ions in the pores of low-cost activated carbons, with the inserted ions then serving as sites for carbon dioxide adsorption. We use our charging process to accumulate reactive hydroxide ions in the pores of a carbon electrode, and find that the resulting sorbent material can rapidly capture carbon dioxide from ambient air by means of (bi)carbonate formation. Unlike traditional bulk carbonates, charged-sorbent regeneration can be achieved at low temperatures (90–100 °C) and the sorbent’s conductive nature permits direct Joule heating regeneration using renewable electricity. Given their highly tailorable pore environments and low cost, we anticipate that charged-sorbents will find numerous potential applications in chemical separations, catalysis and beyond.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Technical and Community Foundations for High-Integrity CDR MRV Standards (Final Report)

The goal of this project (hereafter referred to as the “umbrella project”) was to establish cross-cutting technical foundations for carbon dioxide removal (CDR) accounting decisions. These cross-cutting and science driven technical foundations are necessary to increase trust in standards-setting and protocol development. According to key stakeholders in the industry, establishment of trusted standards is necessary to unlock and catalyze investment in the CDR industry as well as commercialization and deployment of verified, accepted high quality CDR technologies. Additionally, our umbrella project served as the lead coordinator of the cohort of three additional CDR pathway-focused projects funded under this award. In this role, we brought together the project teams to share insights, industry feedback, and approaches to CDR accounting standards development.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2026

The Potential and Cost of Carbon Dioxide Removal Using Direct Air Capture with Land-Based Wind and Utility-Scale Photovoltaics

The rapid deployment of direct air capture and storage (DACS) is critical for achieving emission targets, necessitating precise evaluation of the scale and cost of carbon dioxide removal. This study examines the availability of land, electricity generation, and geologic CO 2 storage within the United States, estimating a technical potential for low-temperature, adsorbent-based DACS to remove approximately 9 gigatonnes of CO 2 annually. By 2050, a substantial portion of this removal could be achieved at net-removed costs below $\$$300/tonneCO 2 , though costs are highly variable depending on factors such as facility scale, construction expenses, climate-dependent productivity and heating efficiency, and geologic storage conditions. In the short term, DACS deployment will help identify key research priorities for advancing technology and reducing removal costs. Concurrently, there is an urgent need for scientifically robust and standardized frameworks for monitoring, reporting, and verifying DACS performance across both established and emerging technologies and energy sources.

Carbon capture↗
DOE OSTI2024

Field Validation of a Pilot-scale Black Liquor Membrane for Water Removal at Ahlstrom-Munksjö Paper Mill in Mosinee, WI

Project Background: The Industrial Technology Validation (ITV) program aims to identify and demonstrate the performance of new, emerging, and underutilized technologies in the industrial sector to help inform decisions towards accelerating commercialization and deployment. Pulp and paper is considered one of the most energy-intensive industries in the manufacturing sector. There are several methodologies for converting wood into pulp in the paper-making industry. The kraft process is a chemical method for producing wood pulp. The kraft process generates black liquor as a byproduct of pulp production. Traditionally, water is evaporated from the liquor by a set of multi-effect evaporators (MEEs), which concentrate weak black liquor (WBL) into strong black liquor (SBL) to support efficient combustion in a recovery boiler. Concentrating black liquor is an energy-intensive step in recovering pulping chemicals and generating high-pressure steam from dissolved wood solids. About 7% of pulp and paper energy usage, or nearly 164 trillion Btu, is used to remove water from black liquor in U.S. kraft pulp mills per year. The U.S. DOE’s IEDO is interested in the black liquor membrane technology evaluated in this report because it offers the potential for a more energy-efficient and less carbon-intensive kraft pulping process across 99 kraft pulp mills in 24 states (Agenda 2020 Technology Alliance 2016). This ITV project validates an innovative black liquor membrane technology for kraft pulp mills to understand its impact and benefits. Via Separations is a technology vendor that developed a graphene oxide membrane system to remove water from WBL before entering the evaporator set. High-pressure positive displacement (HPR) pumps move the black liquor through membranes that separate water and create a more concentrated black liquor. The vendor claims their pre-commercial technology reduces evaporator steam consumption by dewatering WBL before entering the evaporators. They also claim their technology has non-energy benefits such as enhanced soap collection and improved pulp throughput. This evaluation focuses on validating the energy and carbon dioxide (CO 2 e) emissions benefits associated with the membrane system.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗
DOE OSTI2024

Potential of U.S. Marine and Offshore Wind Energy to Power Marine Carbon Dioxide Removal

The goal of this project was to provide a preliminary feasibility assessment of powering different marine carbon dioxide removal (mCDR), carbon capture (mCC), and carbon sequestration (mCS) strategies with marine energy. The investigation focused on methods with clear power requirements at sea beyond monitoring such as artificial upwelling, deep ocean storage, electrochemical (eChem) mCDR and mCC, offshore microalgae cultivation, and seaweed farming and sinking. The project found that eChem mCDR powered by marine energy and offshore wind energy available in the United States could meet global CDR scales needed by 2040 and 2050 to limit warming to 1.5 degrees C by 2100 and marine energy alone could greatly contribute to reaching scales needed by 2040. Note that this preliminary estimate assumes that it is possible to harvest all the marine and offshore wind resources available in the United States with existing technology options. Though the biological methods were limited in scale they still hold promise in developing carbon negative fuels and products which can reduce emissions in the short term.

afforestation↗
DOE OSTI2025

Biomanufacturing from gaseous C1 feedstocks: A perspective on opportunities and challenges

Single-carbon (C1) substrates including carbon dioxide, carbon monoxide, and methane are abundantly available from natural and anthropogenic sources and present potential feedstocks for biomanufacturing. Utilizing these C1 gas feedstocks in bioprocesses for sustainable production of chemicals and fuels could prove pivotal in removing excess carbon from the atmosphere. This perspective describes the spectrum and sources of CO2, CO, and CH4 and examines emerging opportunities in microbial bioconversion and bioelectrochemical processes for these feedstocks. We discuss existing challenges in bioprocess development that currently restrict the commercialization of C1 biomanufacturing technologies. We detail different aerobic and anaerobic bioconversion approaches for C1 feedstocks employing pure and mixed cultures and examine the suitability of each scenario for producing specific molecules. Beyond strain engineering and bioprocess constraints, we address often overlooked factors that limit the development of efficient and reliable bioprocesses, including technology availability for research and safety considerations. We then discuss and recommend the necessary safety features and technological research tools for developing fast, safe, and efficient bioprocesses using gaseous feedstocks to support the scale-up and commercialization of C1 biomanufacturing technologies. This perspective provides an overview of the current scientific and industrial state of the art and offers insights into future technological needs that must be addressed to realize the potential of biomanufacturing from gaseous feedstocks. Synopsis: C1 gases offer a sustainable feedstock for biomanufacturing of fuels and chemicals. This work analyzes bioconversion methods, challenges, and safety considerations, and emphasizes the need for improved technology to enable commercialization.

Biomanufacturing↗
DOE OSTI2023

Initial Systems-Level Assessment of a Distributed Direct Air Capture System Concept at the Urban-scale (UrbanDAC)

Direct Air Capture (DAC) systems offer a promising solution for mitigating global carbon emissions by directly removing ambient carbon dioxide (CO 2 ) from the atmosphere. While future DAC facilities are typically envisioned as being large and centralized, small-scale systems present an alternative approach with advantages such as adaptability and lower uptake costs. By harnessing waste heat from the built environment, such small-scale systems become distributed DAC at the urban scale (UrbanDAC) that benefit from existing urban infrastructure, while presenting challenges such as identifying eligible buildings and sustainable transportation and storage of captured CO 2 . Collaborating with engineering experts and developers of a DAC unit that can be co-located with cooling towers of existing commercial buildings, this study explores the systems-level implications of UrbanDAC using a geographically explicit multi-decision criteria analysis (MCDA) framework. By considering various infrastructure and environmental factors, network analysis and geospatial techniques are applied to identify optimal building candidates for distributed DAC units within Knoxville, Tennessee, USA, as a representative mid-size city. The selected outputs of the MCDA are used to explore a scenario that assumes a CO 2 collection and transport route for 20 high-ranking candidate buildings; total carbon emissions, EV energy consumption, and net carbon dioxide removal (CDR) are then calculated. Results suggest that the spatial variation of optimal candidates between thriving commercial areas is an important planning consideration. Examining the feasibility of UrbanDAC at an urban planning level provides valuable insights into the barriers and enabling conditions for CDR in cities, where the vast majority of CO 2 emissions are produced, and supports decision-making processes for the implementation of decarbonization initiatives. Through this initial assessment, this research acts as a pilot study for an emerging technology that highlights the importance of distributed DAC technologies in addressing climate change and emphasizes the need for further research and exploration in this domain.

32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗
DOE OSTI2020

Na + -gated water-conducting nanochannels for boosting CO 2 conversion to liquid fuels

Robust, gas-impeding water-conduction nanochannels that can sieve water from small gas molecules such as hydrogen (H 2 ), particularly at high temperature and pressure, are desirable for boosting many important reactions severely restricted by water (the major by-product) both thermodynamically and kinetically. Identifying and constructing such nanochannels into large-area separation membranes without introducing extra defects is challenging. We found that sodium ion (Na + )–gated water-conduction nanochannels could be created by assembling NaA zeolite crystals into a continuous, defect-free separation membrane through a rationally designed method. Highly efficient in situ water removal through water-conduction nanochannels led to a substantial increase in carbon dioxide (CO 2 ) conversion and methanol yield in CO 2 hydrogenation for methanol production.

Science & Technology - Other Topics↗
DOE OSTI2021

High-efficiency catalytic reduction of residual oxygen for purification of carbon dioxide streams from high-pressure oxy-combustion systems

Pressurized oxy-combustion is a promising technology for carbon capture, utilization, and storage. For the captured CO 2 to be used for enhanced oil recovery or stored in geological formations, flue gas impurities, including residual O 2 in the CO 2 stream, must be purified to meet the purity specifications. A catalytic approach to reducing residual O 2 with CH 4 was investigated in this study. Five CoMn- and Cu-based catalysts were synthesized or acquired, and a reverse-flow fixed-bed reactor was used to assess their performance for O 2 removal from a simulated oxy-combustion flue gas at 15 bar. The impacts of the operating parameters on O 2 removal, such as temperature, gas hourly space velocity, O 2 /CH 4 ratio, and gas pressure, were investigated. Among the tested catalysts, the two CoMn catalysts were superior in both activity and selectivity, with the reaction lighting off at about 350 °C and achieving 99% O 2 removal at about 500 °C. Finally, the kinetics of the catalytic reaction is discussed, and the Mars–van Krevelen redox mechanism is deemed valid for describing the reaction pathway for the top-performing CoMn catalysts. The catalytic reaction was determined to be first order in CH 4 and zero order in O 2 under the test conditions.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗