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At least 109 records · Page 6
All sourcesNASA NTRSDOE OSTI
NASA NTRS2014

Ticosonde CFH at Costa Rica: A Seasonal Climatology of Tropical UT-LS Water Vapor and Inter-Comparisons with MLS and CALIPSO

Balloon sonde measurements of tropical water vapor using the Cryogenic Frostpoint Hygrometer were initiated in Costa Rica in July 2005 and have continued to the present day. Over the nine years through July 2014, the Ticosonde program has launched 174 CFH payloads, representing the longest-running and most extensive single-site balloon dataset for tropical water vapor. In this presentation we present a seasonal climatology for water vapor and ozone at Costa Rica and examine the frequency of upper tropospheric supersaturation with comparisons to cloud fraction and cloud ice water content observations from the Cloud Aerosol Lidar with Orthogonal Polarization (CALIOP) on the CALIPSO mission. We then make a critical comparison of these data to water vapor measurements from the MLS instrument on board Aura in light of recently published work for other sites. Finally, we examine time series of 2-km altitude averages in the upper troposphere-lower stratosphere at Costa Rica in light of anomalies and trends seen in various large-scale indices of tropical water vapor.

water vapor↗
NASA NTRS2016

Impact of MODIS SWIR Band Calibration Improvements on Level-3 Atmospheric Products

The spectral reflectance measured by the MODIS reflective solar bands (RSB) is used for retrieving many atmospheric science products. The accuracy of these products depends on the accuracy of the calibration of the RSB. To this end, the RSB of the MODIS instruments are primarily calibrated on-orbit using regular solar diffuser (SD) observations. For lambda < 0.94 microns the SDs on-orbit bi-directional reflectance factor (BRF) change is tracked using solar diffuser stability monitor (SDSM) observations. For lambda > 0.94 microns, the MODIS Characterization Support Team (MCST) developed, in MODIS Collection 6 (C6), a time-dependent correction using observations from pseudo-invariant earth-scene targets. This correction has been implemented in C6 for the Terra MODIS 1.24 micron band over the entire mission, and for the 1.375 micron band in the forward processing. As the instruments continue to operate beyond their design lifetime of six years, a similar correction is planned for other short-wave infrared (SWIR) bands as well. MODIS SWIR bands are used in deriving atmosphere products, including aerosol optical thickness, atmospheric total column water vapor, cloud fraction and cloud optical depth. The SD degradation correction in Terra bands 5 and 26 impact the spectral radiance and therefore the retrieval of these atmosphere products. Here, we describe the corrections to Bands 5 (1.24 microns) and 26 (1.375 microns), and produce three sets (B5, B26 correction on/on, on/off, and off/off) of Terra-MODIS Level 1B (calibrated radiance product) data. By comparing products derived from these corrected and uncorrected Terra MODIS Level 1B (L1B) calibrations, dozens of L3 atmosphere products are surveyed for changes caused by the corrections, and representative results are presented. Aerosol and water vapor products show only small local changes, while some cloud products can change locally by > 10%, which is a large change.

Calibration↗
NASA NTRS2020

Differences in Tropical High Clouds Among Reanalyses: Origins and Radiative Impacts

We examine differences among reanalysis highcloud products in the tropics, assess the impacts of these differences on radiation budgets at the top of the atmosphere and within the tropical upper troposphere and lower stratosphere (UTLS), and discuss their possible origins in the context of the reanalysis models. We focus on the ERA5 (fifthgeneration European Centre for Medium-range Weather Forecasts – ECMWF – reanalysis), ERA-Interim (ECMWF Interim Reanalysis), JRA-55 (Japanese 55-year Reanalysis), MERRA-2 (Modern-Era Retrospective Analysis for Research and Applications, Version 2), and CFSR/CFSv2 (Climate Forecast System Reanalysis/Climate Forecast System Version 2) reanalyses. As a general rule, JRA-55 produces the smallest tropical high-cloud fractions and cloud water contents among the reanalyses, while MERRA-2 produces the largest. Accordingly, long-wave cloud radiative effects are relatively weak in JRA-55 and relatively strong in MERRA-2. Only MERRA-2 and ERA5 among the reanalyses produce tropical-mean values of outgoing long-wave radiation (OLR) close to those observed, but ERA5 tends to underestimate cloud effects, while MERRA-2 tends to overestimate variability. ERA5 also produces distributions of longwave, short-wave, and total cloud radiative effects at the top of the atmosphere that are very consistent with those observed. The other reanalyses all exhibit substantial biases in at least one of these metrics, although compensation between the long-wave and short-wave effects helps to constrain biases in the total cloud radiative effect for most reanalyses. The vertical distribution of cloud water content emerges as a key difference between ERA-Interim and other reanalyses. Whereas ERA-Interim shows a monotonic decrease of cloud water content with increasing height, the other reanalyses all produce distinct anvil layers. The latter is in better agreement with observations and yields very different profiles of radiative heating in the UTLS. For example, whereas the altitude of the level of zero net radiative heating tends to be lower in convective regions than in the rest of the tropics in ERAInterim, the opposite is true for the other four reanalyses. Differences in cloud water content also help to explain systematic differences in radiative heating in the tropical lower stratosphere among the reanalyses. We discuss several ways in which aspects of the cloud and convection schemes impact the tropical environment. Discrepancies in the vertical profiles of temperature and specific humidity in convective regions are particularly noteworthy, as these variables are directly constrained by data assimilation, are widely used, and feed back to convective behaviour through their relationships with thermodynamic stability.

High Clouds↗
NASA NTRSDate not supplied

Examining the Feasibility of Detailed Decomposition of Radiative Flux Anomalies to Cloud Changes

This presentation will explore the degree to which radiative flux anomalies in the last two decades seen by CERES can be interpreted as the result of changes in particular cloud types. A study of this kind is potentially enabled by the new CERES FlxByCldTyp (FBCT) product which provides combined Terra and Aqua daytime 1°-regional gridded daily and monthly top-of-the-atmosphere radiative fluxes and associated MODIS-derived cloud properties stratified by Cloud Top Pressure (CTP) and Cloud Optical Thickness (TAU), i.e., arrays of cloud properties and radiative fluxes resolved in CTP-TAU bins. It has been shown (Sun et al. 2022) that the FBCT time series of global flux anomalies tracks closely its SSF1deg and EBAF counterparts, indicating that these three products provide fluxes of consistent stability for interannual variability studies. We are thus in position to examine whether CERES regional or global radiative fluxes anomalies and trends are driven by changes in certain elements of FBCT flux arrays corresponding to particular cloud types. Anomalies in flux array elements will in turn be investigated in terms of cloud property variations within the CTP-TAU bins where the biggest flux anomalies are encountered. We will essentially seek to obtain the relative contributions to the anomalies of binned all-sky fluxes of changes in cloud fraction within cloud types and of changes in their overcast fluxes modulated by other cloud properties. Such an analysis holds great promise of unveiling the root causes of cloud-driven changes in the planetary radiation budget of the last two decades.

cloud↗
NASA NTRS2023

A Cloud Detection Neural Network for Above-Aircraft Clouds Using Airborne Cameras

We introduce a method convolutional neural networks to detect the presence of clouds in airborne camera images. We quantify the performance of this Cloud Detection Neural Network (CDNN) using human-labeled validation data where we report a 96% accuracy in detecting clouds in testing datasets for both Zenith- viewing and Forward-viewing models. We assess our performance by comparing the flight-averaged cloud fraction of zenith and forward CDNN retrievals, with that of the prototype hyperspectral total-diffuse Sunshine Pyranometer (SPN-S) instrument’s cloud optical depth data. Comparison of the CDNN with the SPN-S on time specific intervals resulted in 93% accuracy for the zenith- viewing CDNN and 84% for the forward- viewing CDNN. The comparison of the CDNNs with the SPN-S on flight-averaged cloud fraction resulted in an agreement of 0.15 for the Forward CDNN and 0.07 for the Zenith CDNN. We then quantify the ability of the CDNN to identify the presence of clouds above the aircraft using a forward- looking camera mounted inside the aircraft cockpit compared to the use of an All- Sky upward-looking camera that is mounted outside the fuselage on top of the aircraft. We present results from the CDNN based on airborne imagery from the NASA Aerosol Cloud Meteorology Interactions Over the Western Atlantic Experiment (ACTIVATE) and the Clouds, Aerosol and Monsoon Processes- Philippines Experiment (CAMP2Ex). For CAMP2Ex 53% of flight dates had above- aircraft cloud fraction above 50%, while for ACTIVATE 52% and 54% of flight dates observed above-aircraft cloud fraction above 50% for 2020 and 2021, respectively.

Joseph D Nied↗
NASA NTRSDate not supplied

Role of Arctic Low Clouds in the Arctic Climate System: Isolating the Surface Type Influence on Arctic Low-Clouds

Interactions between sea ice and clouds represent a mechanism through which sea ice influences climate. Understanding the cloud response to the rapidly changing Arctic surface properties is necessary for improving climate simulations and projection of future change inside and outside the Arctic. Towards the goal of understanding the cloud response to sea ice, we composite cloud properties for ice-free, marginal ice zone (MIZ), and ice-covered surfaces during MIZ crossing events to analyze the cloud property differences between surface types. Restricting the analysis to MIZ crossing events enables the isolation of the sea ice effect on clouds from meteorological factors. We find larger cloud fraction and total water concentration below ~1.5 km over ice-free relative to ice-covered surfaces during non-summer months. During summer, the results suggest larger cloud fraction and total water concentration over ice-free surfaces, however differences do not exceed observational uncertainty. Cloud property differences are linked to atmospheric thermodynamic profile differences, namely ice-free surfaces are warmer, moister, less stable, and have more positive surface turbulent fluxes than ice-covered surfaces. Ice-free minus ice-covered cloud property differences scale with surface temperature differences and are only found in the presence of a surface temperature difference. Our results suggest a 0.02 cloud fraction and 0.005 g m 3 total water concentration increase (~5%) at the level of maximum cloud fraction between 2000-2021 due to the observed Arctic sea ice decline in fall, corresponding to ~2 Wm 2 increase in the net surface radiative flux supporting a positive sea ice-cloud radiative feedback in fall and winter and a negative sea ice-cloud radiative feedback in spring. We propose an updated conceptual model where the average surface type influence on cloud properties is mediated by surface temperature differences between ice-free and ice-covered surfaces.

Arctic climate↗
NASA NTRS2023

Comparison of Clouds and Cloud Feedback between AMIP5 and AMIP6

We examine the changes in clouds and cloud feedback between Phase 5 (AMIP5) and Phase 6 (AMIP6) of the Atmospheric Model Intercomparison Project. Each model is perturbed by uniformly increasing the sea surface temperature by 4 K. The simulated cloud fraction, the perturbed states and cloud radiative kernels are used to derive cloud feedback in the shortwave (SW), longwave (LW) and their sum (Net). Compared to AMIP5, the cloud fraction in AMIP6 increases by 9.1%, while the perturbation leads to a 0.25% decrease. The Net cloud feedback at the top of the atmosphere (TOA) is almost double (174%). Statistical tests support that this change is mainly due to an increase in the surface SW cloud feedback caused by optically thick, middle and low clouds. The contribution of the atmospheric Net component (12%) stems from the increase in the atmospheric LW cloud feedback, likely to play a role in weakening (strengthening) the northward (southward) meridional atmospheric energy transport, while the opposite is true for the surface LW and Net cloud feedback in the meridional oceanic energy transport. The substantial increase in cloud feedback at the TOA primarily contributes to the higher climate sensitivity. The cloud feedback spread in AMIP6 is comparable to that in AMIP5.

Clouds↗
NASA NTRS2022

Assessment of Two Stochastic Cloud Subcolumn Generators Using Observed Fields of Vertically Resolved Cloud Extinction

We evaluate two stochastic subcolumn generators used in GCMs to emulate subgrid cloud variability enabling comparisons with satellite observations and simulations of certain physical processes. Our evaluation necessitated the creation of a reference observational dataset that resolves horizontal and vertical cloud variability. The dataset combines two CloudSat cloud products that resolve two-dimensional cloud optical depth variability of liquid, ice, and mixed phase clouds when blended at ~200 m vertical and ~ 2 km horizontal scales. Upon segmenting the dataset to individual “scenes”, mean profiles of the cloud fields are passed as input to generators that produce scene-level cloud subgrid variability. The assessment of generator performance at the scale of individual scenes and in a mean sense is largely based on inferred joint histograms that partition cloud fraction within predetermined combinations of cloud top pressure –cloud optical thickness ranges. Our main finding is that both generators tend to underestimate optically thin clouds, while one of them also tends to overestimate some cloud types of moderate and high optical thickness. Associated radiative flux errors are also calculated by applying a simple transformation to the cloud fraction histogram errors, and are found to approach values almost as high as 3 Wm-2 for the cloud radiative effect in the shortwave part of the spectrum.

cloud variability↗
NASA NTRS1976

A single field of view method for retrieving tropospheric temperature profiles from cloud-contaminated radiance data

An iterative method is presented to retrieve single field of view (FOV) tropospheric temperature profiles directly from cloud-contaminated radiance data. A well-defined temperature profile may be calculated from the radiative transfer equation (RTE) for a partly cloudy atmosphere when the average fractional cloud amount and cloud-top height for the FOV are known. A cloud model is formulated to calculate the fractional cloud amount from an estimated cloud-top height. The method is then examined through use of simulated radiance data calculated through vertical integration of the RTE for a partly cloudy atmosphere using known values of cloud-top height(s) and fractional cloud amount(s). Temperature profiles are retrieved from the simulated data assuming various errors in the cloud parameters. Temperature profiles are retrieved from NOAA-4 satellite-measured radiance data obtained over an area dominated by an active cold front and with considerable cloud cover and compared with radiosonde data. The effects of using various guessed profiles and the number of iterations are considered.

Hodges, D. B.↗
NASA NTRS2016

Saharan Dust as a Causal Factor of Significant Cloud Cover Along the Saharan Air Layer in the Atlantic Ocean

The tropical Atlantic is frequently affected by Saharan dust intrusions. Based on MODIS cloud fraction (CF) data during the ten-year study period, we found that these dust intrusions contribute to significant cloud cover along the Saharan Air Layer (SAL). Below the temperature inversion at the SAL's base, the presence of large amounts of settling dust particles, together with marine aerosols, produces meteorological conditions suitable for the formation of shallow stratocumulus clouds. The significant cloud fraction along the SAL together with clouds over the Atlantic Inter-tropical Convergence Zone contributes to the 20% hemispheric CF asymmetry between the tropical North and South Atlantic. This leads to the imbalance in strong solar radiation, which reaches the sea surface between the tropical North and South Atlantic, and, consequently, affects climate formation in the tropical Atlantic. Therefore, despite the fact that, over the global ocean, there is no noticeable hemispheric asymmetry in cloud fraction, over the significant area such as the tropical Atlantic the hemispheric asymmetry in CF takes place. Saharan dust is also the major contributor to hemispheric aerosol asymmetry over the tropical Atlantic. The NASA GEOS-5 model with aerosol data assimilation was used to extend the MERRA reanalysis with five atmospheric aerosol species (desert dust, sulfates, organic carbon, black carbon, and sea-salt). The obtained ten-year (2002 - 2012) MERRA-driven aerosol reanalysis dataset (aka MERRAero) showed that, over the tropical Atlantic, dust and carbonaceous aerosols were distributed asymmetrically relative to the equator, while other aerosol species were distributed more symmetrically.

CF↗
NASA NTRS2005

Antarctica Cloud Cover for October 2003 from GLAS Satellite Lidar Profiling

Seeing clouds in polar regions has been a problem for the imagers used on satellites. Both clouds and snow and ice are white, which makes clouds over snow hard to see. And for thermal infrared imaging both the surface and the clouds cold. The Geoscience Laser Altimeter System (GLAS) launched in 2003 gives an entirely new way to see clouds from space. Pulses of laser light scatter from clouds giving a signal that is separated in time from the signal from the surface. The scattering from clouds is thus a sensitive and direct measure of the presence and height of clouds. The GLAS instrument orbits over Antarctica 16 times a day. All of the cloud observations for October 2003 were summarized and compared to the results from the MODIS imager for the same month. There are two basic cloud types that are observed, low stratus with tops below 3 km and high cirrus form clouds with cloud top altitude and thickness tending at 12 km and 1.3 km respectively. The average cloud cover varies from over 93 % for ocean and coastal regions to an average of 40% over the East Antarctic plateau and 60-90% over West Antarctica. When the GLAS monthly average cloud fractions are compared to the MODIS cloud fraction data product, differences in the amount of cloud cover are as much as 40% over the continent. The results will be used to improve the way clouds are detected from the imager observations. These measurements give a much improved understanding of distribution of clouds over Antarctica and may show how they are changing as a result of global warming.

Spinhirne, J. D.↗
NASA NTRS2021

Global Daytime Variability of Clouds from DSCOVR/EPIC Observations

Knowledge of the daytime variability of cloud fraction is pivotal for the accurate determination of the atmosphere's energy balance. Yet, polar orbiting satellites are unable to fully capture daytime variability and individual geostationary satellites only provide measurements for portions of the Earth. In addition, diurnal cloud fraction variations analyzed with General Circulation Models provide results that cannot be reconciled with observations in many situations. Here we show that the Earth Polychromatic Imaging Camera (EPIC) aboard the DSCOVR satellite presents a unique opportunity to examine changes in daytime global cloud fraction resolved at one-hour frequency. For the first time, we characterize the global daytime variability of clouds with a single sensor, presenting evidence that the fraction of liquid clouds reaches its maximum over continental areas and its minimum over ocean around noon. We compare our results with previous global and regional studies and examine implications for the Earth's energy budget.

cloud fraction↗
NASA NTRS2016

Study of the Effect of Temporal Sampling Frequency on DSCOVR Observations Using the GEOS-5 Nature Run Results: Cloud Coverage - Part II

This is the second part of a study on how temporal sampling frequency affects satellite retrievals in support of the Deep Space Climate Observatory (DSCOVR) mission. Continuing from Part 1, which looked at Earth's radiation budget, this paper presents the effect of sampling frequency on DSCOVR-derived cloud fraction. The output from NASA's Goddard Earth Observing System version 5 (GEOS-5) Nature Run is used as the "truth". The effect of temporal resolution on potential DSCOVR observations is assessed by subsampling the full Nature Run data. A set of metrics, including uncertainty and absolute error in the subsampled time series, correlation between the original and the subsamples, and Fourier analysis have been used for this study. Results show that, for a given sampling frequency, the uncertainties in the annual mean cloud fraction of the sunlit half of the Earth are larger over land than over ocean. Analysis of correlation coefficients between the subsamples and the original time series demonstrates that even though sampling at certain longer time intervals may not increase the uncertainty in the mean, the subsampled time series is further and further away from the "truth" as the sampling interval becomes larger and larger. Fourier analysis shows that the simulated DSCOVR cloud fraction has underlying periodical features at certain time intervals, such as 8, 12, and 24 h. If the data is subsampled at these frequencies, the uncertainties in the mean cloud fraction are higher. These results provide helpful insights for the DSCOVR temporal sampling strategy.

GEOS-5↗
NASA NTRS1984

Solar reflection from interacting and shadowing cloud elements

An attempt is made to relate the reflection from a broken cloud field to that from a plane parallel cloud of the same optical properties by using Monte Carlo simulations for a very simple model of an array of regularly spaced, infinitely long bar clouds. Reflection from the array is represented by an effective cloud fraction, and it is shown that for many cases this may be obtained by treating the cloud elements to be noninteracting azimuthally symmetric reflectors. The effective cloud fraction is a function of solar zenith angle, the aspect ratio of the individual cloud elements, and the normal or zenith cloud fraction of the array. Model computations for reflection from an array of randomly distributed identical cylinders are also presented as an example of a possible application of this technique.

HARSHVARDHAN↗
NASA NTRS1994

11 micrometer emissivities and droplet radii for marine stratocumulus

The results of a new multispectral infrared retrieval scheme for obtaining fractional cloud cover and 11 micrometer emissivity with those of the spatial coherence method which obtains fractional cloud cover assuming that the clouds are opaque at infrared wavelengths. Both methods are applied to 4-km NOAA advanced very high resolution radiometer global area coverage data for 250-km-scale regions containing single-layered marine stratocumulus off the coast of South America. The average 11 micrometer emissivity for low level clouds is found to be between 0.70 and 0.85. The low emissivity is evidently due to the thinning of clouds at their edges. Semitransparent cloud edges evidently make up a substantial portion of the area covered by such clouds. This result indicates that cloud cover obtained using the spatial coherence method is underestimated by 0.1 to 0.2, as has been claimed in a previous study. The fractional cloud cover for the ensemble of 250-km-scale regions studied here increased slightly from 0.60 for daytime observations to 0.63 for nighttime observations. The 11 micrometer emissivity also increased slightly, but about half of the increase was related to the increase in cloud cover and a decrease in the relative area covered by cloud edge material. Presumably, the other half was due to an increase in cloud liquid water. Cloud height showed no significant change. The average effective droplet radius increased from 9.3 micrometers for daytime observations to 10.2 micrometers at night.

Luo, Gang↗
NASA NTRS2014

The Atmospheric Infrared Sounder Version 6 Cloud Products

The version 6 cloud products of the Atmospheric Infrared Sounder (AIRS) and Advanced Microwave Sounding Unit (AMSU) instrument suite are described. The cloud top temperature, pressure, and height and effective cloud fraction are now reported at the AIRS field-of-view (FOV) resolution. Significant improvements in cloud height assignment over version 5 are shown with FOV-scale comparisons to cloud vertical structure observed by the CloudSat 94 GHz radar and the Cloud-Aerosol LIdar with Orthogonal Polarization (CALIOP). Cloud thermodynamic phase (ice, liquid, and unknown phase), ice cloud effective diameter D(sub e), and ice cloud optical thickness (τ) are derived using an optimal estimation methodology for AIRS FOVs, and global distributions for 2007 are presented. The largest values of tau are found in the storm tracks and near convection in the tropics, while D(sub e) is largest on the equatorial side of the midlatitude storm tracks in both hemispheres, and lowest in tropical thin cirrus and the winter polar atmosphere. Over the Maritime Continent the diurnal variability of tau is significantly larger than for the total cloud fraction, ice cloud frequency, and D(sub e), and is anchored to the island archipelago morphology. Important differences are described between northern and southern hemispheric midlatitude cyclones using storm center composites. The infrared-based cloud retrievals of AIRS provide unique, decadal-scale and global observations of clouds over portions of the diurnal and annual cycles, and capture variability within the mesoscale and synoptic scales at all latitudes.

infrared instruments↗
NASA NTRS2017

Effects of Surface BRDF on the OMI Cloud and NO2 Retrievals: A New Approach Based on Geometry-Dependent Lambertian Equivalent Reflectivity (GLER) Derived from MODIS

The Ozone Monitoring Instrument (OMI) cloud and NO2 algorithms use a monthly gridded surface reflectivity climatology that does not depend upon the observation geometry. In reality, reflection of incoming direct and diffuse solar light from land or ocean surfaces is sensitive to the sun sensor geometry. This dependence is described by the bidirectional reflectance distribution function (BRDF). To account for the BRDF, we propose to use a new concept of geometry-dependent Lambertian equivalent reflectivity (GLER). Implementation within the existing OMI cloud and NO2 retrieval infrastructure requires changes only to the input surface reflectivity database. GLER is calculated using a vector radiative transfer model with high spatial resolution BRDF information from MODIS over land and the Cox Munk slope distribution over ocean with a contribution from water-leaving radiance. We compare GLER and climatological LER at 466 nm, which is used in the OMI O2-O2cloud algorithm to derive effective cloud fractions. A detailed comparison of the cloud fractions and pressures derived with climatological and GLERs is carried out. GLER and corresponding retrieved cloud products are then used as input to the OMI NO2 algorithm. We find that replacing the climatological OMI-based LERs with GLERs can increase NO2 vertical columns by up to 50 % in highly polluted areas; the differences include both BRDF effects and biases between the MODIS and OMI-based surface reflectance data sets. Only minor changes to NO2 columns (within 5 %) are found over unpolluted and overcast areas.

MODIS BRDF OMI clouds NO2 GLER↗
NASA NTRS2017

Accounting for the Effects of Surface BRDF on Satellite Cloud and Trace-Gas Retrievals: A New Approach Based on Geometry-Dependent Lambertian-Equivalent Reflectivity Applied to OMI Algorithms

Most satellite nadir ultraviolet and visible cloud, aerosol, and trace-gas algorithms make use of climatological surface reflectivity databases. For example, cloud and NO2 retrievals for the Ozone Monitoring Instrument (OMI) use monthly gridded surface reflectivity climatologies that do not depend upon the observation geometry. In reality, reflection of incoming direct and diffuse solar light from land or ocean surfaces is sensitive to the sun-sensor geometry. This dependence is described by the bidirectional reflectance distribution function (BRDF). To account for the BRDF, we propose to use a new concept of geometry-dependent Lambertian equivalent reflectivity (LER). Implementation within the existing OMI cloud and NO2 retrieval infrastructure requires changes only to the input surface reflectivity database. The geometry-dependent LER is calculated using a vector radiative transfer model with high spatial resolution BRDF information from the Moderate Resolution Imaging Spectroradiometer (MODIS) over land and the Cox-Munk slope distribution over ocean with a contribution from water-leaving radiance. We compare the geometry-dependent and climatological LERs for two wavelengths, 354 and 466 nm, that are used in OMI cloud algorithms to derive cloud fractions. A detailed comparison of the cloud fractions and pressures derived with climatological and geometry-dependent LERs is carried out. Geometry-dependent LER and corresponding retrieved cloud products are then used as inputs to our OMI NO2 algorithm. We find that replacing the climatological OMI-based LERs with geometry-dependent LERs can increase NO2 vertical columns by up to 50% in highly polluted areas; the differences include both BRDF effects and biases between the MODIS and OMI-based surface reflectance data sets. Only minor changes to NO2 columns (within 5 %) are found over unpolluted and overcast areas.

Lambert-equivalent reflectivity↗