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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 109 records · Page 6
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Impact of Aerosol and Cloud on the Solar Energy Potential over the Central Gangetic Himalayan Region

We examine the impact of atmospheric aerosols and clouds on the surface solar radiation and solar energy at Nainital, a high-altitude remote location in the central Gangetic Himalayan region (CGHR). For this purpose, we exploited the synergy of remote-sensed data in terms of ground-based AERONET Sun Photometer and satellite observations from the MODerate Resolution Imaging Spectroradiometer (MODIS) and the Meteosat Second Generation (MSG), with radiative transfer model (RTM) simulations and 1 day forecasts from the Copernicus Atmosphere Monitoring Service (CAMS). Clouds and aerosols are one of the most common sources of solar irradiance attenuation and hence causing performance issues in the photovoltaic (PV) and concentrated solar power (CSP) plant installations. The outputs of RTM results presented with high accuracy under clear, cloudy sky and dust conditions for global horizontal (GHI) and beam horizontal irradiance (BHI). On an annual basis the total aerosol attenuation was found to be up to 105 kWh m –2 for the GHI and 266 kWh m –2 for BHI, respectively, while the cloud effect is much stronger with an attenuation of 245 and 271 kWh m –2 on GHI and BHI. The results of this study will support the Indian solar energy producers and electricity handling entities in order to quantify the energy and financial losses due to cloud and aerosol presence.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Multiphase outflows in post-starburst E+A galaxies - II. A direct connection between the neutral and ionized outflow phases

ABSTRACT Post-starburst E+A galaxies are systems that hosted a powerful starburst that was quenched abruptly. Simulations suggest that these systems provide the missing link between major merger ULIRGs and red and dead ellipticals, where AGN feedback is responsible for the expulsion or destruction of the molecular gas. However, many details remain unresolved and little is known about AGN-driven winds in this short-lived phase. We present spatially resolved IFU spectroscopy with MUSE/VLT of SDSS J124754.95-033738.6, a post-starburst E+A galaxy with a recent starburst that started 70 Myr ago and ended 30 Myr ago, with a peak SFR of $\sim 150\, \mathrm{M_{\odot }\,yr^{ -1}}$. We detect disturbed gas throughout the entire field of view, suggesting triggering by a minor merger. We detect fast-moving multiphased gas clouds, embedded in a double-cone face-on outflow, which are traced by ionized emission lines and neutral NaID emission and absorption lines. We find remarkable similarities between the kinematics, spatial extents, and line luminosities of the ionized and neutral gas phases, and propose a model in which they are part of the same outflowing clouds, which are exposed to both stellar and AGN radiation. Our photoionization model provides consistent ionized line ratios, NaID absorption optical depths and EWs, and dust reddening. Using the model, we estimate, for the first time, the neutral-to-ionized gas mass ratio (about 20), the sodium neutral fraction, and the size of the outflowing clouds. This is one of the best ever observed direct connections between the neutral and ionized outflow phases in AGN.

Baron, Dalya↗
DOE OSTI2021

Estimating Surface Solar Irradiance Using Meteosat-8 Satellite for India and Surrounding Regions (2017-2019)

Using the Physical Solar Model, Version 3 (PSM V3), the National Renewable Energy Laboratory—in collaboration with the University of Wisconsin, the National Oceanic and Atmospheric Administration, and Solar Consulting Services—produced modeled surface solar irradiance based on Meteosat-8 satellite cloud information. PSM V3 implements a physics-based radiative transfer approach to model surface solar irradiance using cloud properties processed from raw satellite data and ancillary data such as aerosol optical depth and precipitable water vapor from the Modern-Era Retrospective Analysis for Research and Applications, Version 2 (MERRA-2). Further, the modeled surface solar irradiance was validated using 10 high-quality ground measurement data from the Baseline Surface Radiation Network. The modeled data showed good correlation with the ground measurement, and the overall uncertainty is less than 35% for all validation locations. Because of the satellite viewing geometry, the Indian and European locations demonstrated higher uncertainties than the African locations, where the Meteosat-8 satellite has a more nadir viewing geometry. Further, instruction on how to access the data is provided.

14 SOLAR ENERGY↗
DOE OSTI2025

Impact of host climate model on contrail cirrus effective radiative forcing estimates

Estimates of aviation effective radiative forcing (ERF) indicate that contrail cirrus is currently its largest contributor, although with a substantial associated uncertainty of ∼ 70 %. Here, we implement the contrail parameterisation developed for the Community Atmosphere Model (CAM) in the UK Met Office Unified Model (UM), allowing us to compare, for the first time, the impact of key features of the host climate model on contrail cirrus ERF. We find that differences in background humidity between the models result in the UM-simulated contrail fractions being 2 to 3 times larger than in CAM. Additionally, the models show contrasting responses in overall global cloud fraction, with contrails increasing the total cloud fraction in the UM and decreasing it in CAM. Differences in the complexity of the cloud microphysics schemes lead to significant differences in simulated changes to cloud ice water content due to aviation. After compensating for the unrealistically low contrail optical depth in the UM, we estimate the 2018 contrail cirrus ERF to be 40.8 mW m−2 in the UM, compared to 60.1 mW m−2 in CAM. These values highlight the substantial uncertainty in contrail cirrus ERF due to differences in microphysics and radiation schemes between the two models. We also find a factor-of-8 uncertainty in contrail cirrus ERF due to existing uncertainty in contrail cirrus optical depth. Future research should focus on better representing microphysical and radiative contrail characteristics in climate models and on improved observational constraints.

Zhang, Weiyu [University of Leeds (United Kingdom)↗
DOE OSTI2024

Quantifying the impacts of marine aerosols over the southeast Atlantic Ocean using a chemical transport model: implications for aerosol–cloud interactions

The southeast Atlantic region, characterized by persistent stratocumulus clouds, has one of the highest uncertainties in aerosol radiative forcing and significant variability across climate models. In this study, we analyze the seasonally varying role of marine aerosol sources and identify key uncertainties in aerosol composition at cloud-relevant altitudes over the southeast Atlantic using the GEOS-Chem chemical transport model. We evaluate simulated aerosol optical depth (AOD) and speciated aerosol concentrations against those collected from ground observations and aircraft campaigns such as LASIC, ORACLES, and CLARIFY, conducted during 2017. The model consistently underestimates AOD relative to AERONET, particularly at remote locations like Ascension Island. However, when compared with aerosol mass concentrations from aircraft campaigns during the biomass burning period, it performs adequately at cloud-relevant altitudes, with a normalized mean bias (NMB) between -3.5 % (CLARIFY) and -7.5 % (ORACLES). At these altitudes, in the model, organic aerosols (63 %) dominate during the biomass burning period, while sulfate (41 %) prevails during austral summer, when dimethylsulfide (DMS) emissions peak in the model. Our findings indicate that marine sulfate can account for up to 69 % of total sulfate during the high-DMS period. Sensitivity analyses indicate that refining DMS emissions and oxidation chemistry may increase sulfate aerosol produced from marine sources, highlighting that there remains large uncertainty as to the role of DMS emissions in the marine boundary layer. Additionally, we find marine primary organic aerosol emissions may substantially increase total organic aerosol concentrations, particularly during austral summer. This study underscores the imperative need to refine marine emissions and their chemical transformations, as aerosols from marine sources are a major component of total aerosols at cloud-relevant altitudes and may impact uncertainties in aerosol radiative forcing over the southeast Atlantic.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Changes in Aerosols, Meteorology, and Radiation in the Southeastern U.S. Warming Hole Region during 2000 to 2019

Abstract Surface air temperatures in the southeastern United States that did not change from the climatological mean from 1900 to 2000 have increased since the year 2000. Analyzed herein are factors modulating the surface air temperatures in the region for a 20-yr period (2000–19) using space- and surface-based observations, and output from a reanalysis model. The 20-yr period is segregated into two decades, 2000–09 and 2010–19, corresponding to different tropospheric chemical regimes. Changes in seasonal and decadal averages are examined. The later decade experienced higher average surface air temperatures with significant warming during summer and fall seasons. Decadal and seasonal averages of cloud properties, column water vapor, rain rates, and top-of-atmosphere outgoing longwave radiation did not exhibit statistically significant differences between the two decades. The region experienced strong warm and moist advection during the winter months and very weak advection during the summer months. The later decade exhibited higher low-level moisture advection during the winter months than the earlier decade with insignificant changes in the temperature advection between the two decades. The later decade had significantly lower aerosol dry and liquid water mass during all seasons, along with lower aerosol optical depth, higher single scattering albedo, and lower top-of-the-atmosphere outgoing shortwave radiation during cloud-free conditions in the summer season. Collectively, these results suggest that changes in the aerosol direct radiative forcing are responsible for warming during summer months that experience weak advection and highlight seasonal differences in the temperature controlling mechanisms in the region.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

High-Spectral Resolution Lidar (HSRL) Instrument Handbook

High-spectral-resolution lidar (HSRL) systems provide vertical profiles of optical depth, backscatter cross-section, depolarization, and backscatter phase function. All HSRL measurements are calibrated by reference to molecular scattering, which is measured at each point in the lidar profile. Like the Raman lidar (RL), but unlike simple backscatter lidars such as the micropulse lidar (MPL), this enables the HSRL to measure backscatter cross-sections and optical depths without prior assumptions about the scattering properties of the atmosphere. The depolarization observations allow robust discrimination between ice and water clouds. Rigorous error estimates can be computed for all measurements. A very narrow angular field of view reduces multiple scattering contributions. The small field of view, coupled with a narrow optical bandwidth, nearly eliminates noise due to scattered sunlight. The laser transmitter is a diode-pumped, frequency-doubled Nd:YAG laser. Narrow-band, single-frequency operation is provided by injection seeding with a single-frequency, cw-diode-pumped diode laser. The main laser cavity is maintained in resonance with the seed laser by adjusting the cavity length to minimize the time between the Q-switch trigger and the emission of the laser pulse. The emission wavelength is tuned via temperature control of the seed laser crystal and is locked to line #1109 of the iodine absorption spectra. Locking is accomplished by minimizing the transmission through a 2-cm-long iodine absorption cell. Use of a high-repetition-rate laser and expansion of the transmitted beam through a 400-mm telescope reduces the transmitted energy density to eye-safe levels. It is possible to look directly into the output beam without hazard. The receiver and transmitter use the same afocal telescope, simplifying the maintenance of stable alignment of the transmitter and receiver although the angular FOV is only 100 μrad. The small FOV and the 4-kHz repetition rate also limit the near-field signal strength, making it possible to record continuous profiles that start at an altitude of ~100 m and extend to 30 km using photon counting detectors. The small FOV also suppresses multiple scattering contributions.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Optical Properties of Individual Tar Balls in the Free Troposphere

Tar balls are brown carbonaceous particles, highly viscous, spherical, amorphous, and light absorbing. They are believed to form in biomass burning smoke plumes during transport in the troposphere. Tar balls are believed to have a significant impact on the Earth’s radiative balance, but due to poorly characterized optical properties, this impact is highly uncertain. Here, we investigate the chemical composition and optical properties of individual tar balls transported in the free troposphere to the Climate Observatory “Ottavio Vittori” on Mt. Cimone, Italy (2165 meters above sea level) using multi-modal micro-spectroscopy. Our results show that tar balls contributed 50% of carbonaceous particles by number in the size range from 0.25 to 1.8 µm. Of those tar balls, 16% were inhomogeneously mixed with other constituents. Using electron energy loss spectroscopy, we retrieved the complex refractive index from 200 to 1200 nm for both inhomogeneously and homogeneously mixed tar balls. We found no significant difference in the average refractive index of inhomogeneously and homogenously mixed tar balls (1.40 - 0.03i, and 1.36 - 0.03i at 550 nm, respectively). Furthermore, we estimated the top of the atmosphere radiative forcing using the Santa Barbara DISORT Atmospheric Radiative Transfer model (SBDART) and found that a layer of only tar balls with an optical depth of 0.1 above vegetation would exert a positive radiative forcing ranging from 2.8 Wm-2 (on a clear sky day) to 9.5 Wm-2 (when clouds are below the aerosol layer). In conclusion, understanding the optical properties of tar balls can help reduce uncertainties associated with the contribution of biomass-burning aerosol in current climate models.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

EPCAPE-Partitioning Thrust-Los Alamos National Laboratory (EPCAPE-PT-LANL) Field Campaign Report

Coastal cities offer a unique environment for studying aerosol-cloud interactions and the effects of urban emissions on aerosol and cloud properties. As part of the U.S. Department of Energy Atmospheric Radiation Measurement (ARM)’s Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE), the Partitioning Thrust by Los Alamos National Laboratory (EPCAPE-PT-LANL) was conducted to complement the science goals of EPCAPE and add additional in-depth measurements of aerosols and clouds at Mt. Soledad. Our campaign focused on measuring the physical, optical, and chemical properties of aerosols, trace gases, and their interactions within marine stratocumulus clouds in La Jolla, California (see Figure 1).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Exploring the Constraints on Simulated Aerosol Sources and Transport across the North Atlantic with Island-Based Sun Photometers

Atmospheric aerosol over the North Atlantic Ocean impact regional clouds and climate. In this work, we use a set of sun photometer observations of Aerosol Optical Depth (AOD) located on the Graciosa and Cape Verde islands, along with the GEOS-Chem chemical transport model to investigate the sources of these aerosol and their transport over the North Atlantic Ocean. At both locations, the largest simulated contributor to aerosol extinction is the local source of sea-salt aerosol. In addition to this large source, we find that signatures consistent with long-range transport of anthropogenic, biomass burning, and dust emissions are apparent throughout the year at both locations. Model simulations suggest that this signal of long-range transport in AOD is more apparent at higher elevation locations; the influence of anthropogenic and biomass burning aerosol extinction is particularly pronounced at the height of Pico Mountain, near the Graciosa Island site. Using a machine learning approach, we further show that simulated observations at these three sites (near Graciosa, Pico Mountain, and Cape Verde) can be used to predict the simulated background aerosol imported into cities on the European mainland, particularly during the local winter months, highlighting the utility of background AOD monitoring for understanding downwind air quality.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Tropical Cirrus in Global Storm-Resolving Models. Part II: Cirrus Life Cycle and Top-of-Atmosphere Radiative Fluxes

Cirrus clouds of various thicknesses and radiative characteristics extend over much of the tropics, especially around deep convection. They are difficult to observe due to their high altitude and sometimes small optical depths. They are also difficult to simulate in conventional global climate models, which have coarse grid spacings and simplified parameterizations of deep convection and cirrus formation. We investigate the representation of tropical cirrus in global storm-resolving models (GSRMs), which have higher spatial resolution and explicit convection and could more accurately represent cirrus cloud processes. This study uses GSRMs from the DYnamics of the Atmospheric general circulation Modeled On Non-hydrostatic Domains (DYAMOND) project. The aggregate life cycle of tropical cirrus is analyzed using joint albedo and outgoing longwave radiation (OLR) histograms to assess the fidelity of models in capturing the observed cirrus cloud populations over representative tropical ocean and land regions. The proportions of optically-thick deep convection, anvils, and cirrus vary across models and are portrayed in the vertical distribution of cloud cover and top-of-atmosphere radiative fluxes. Model differences in cirrus populations, likely driven by subgrid processes such as ice microphysics, dominate over regional differences between convectively-active tropical land and ocean locations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Characterization of the aerosol vertical distributions and their impacts on warm clouds based on multi-year ARM observations

Aerosol vertical distribution plays a crucial role in cloud development and thus precipitation since both aerosol indirect and semi-direct effects significantly depend on the relative position of aerosol layer in reference to cloud, but its precise influence on cloud remains unclear. In this study, we integrated multi-year Raman Lidar measurements of aerosol vertical profiles from the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) facility with available Value-Added Products of cloud features to characterize aerosol vertical distributions and their impacts on warm clouds over the continental and marine ARM atmospheric observatories, i.e., Southern Great Plains (SGP) and Eastern North Atlantic (ENA). A unimodal seasonal distribution of aerosol optical depths (AODs) with a peak in summer is found at upper boundary layer over SGP, while a bimodal distribution is observed at ENA for the AODs at lower levels with a major winter-spring maximum. The diurnal mean of upper-level AOD at SGP shows a maximum in the early evening. According to the relative positions of aerosol layers to clouds we further identify three primary types of aerosol vertical distribution, including Random, Decreasing, and Bottom. It is found that the impacts of aerosols on cloud may or may not vary with aerosol vertical distribution depending on environmental conditions, as reflected by the wide variations of the relations between AOD and cloud properties. For example, as AOD increases, the liquid water paths (LWPs) tend to be reduced at SGP but enhanced at ENA. The relations of cloud droplet effective radius with AOD largely depend on aerosol vertical distributions, particularly showing positive values in the Random type under low-LWP condition (<50gm -2 ). In conclusion, the distinct features of aerosol-cloud interactions in relation to aerosol vertical distribution are likely attributed to the continental-marine contrast in thermodynamic environments and aerosol conditions between SGP and ENA.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Constraining the Twomey effect from satellite observations: issues and perspectives

Abstract. The Twomey effect describes the radiative forcing associated with a change in cloud albedo due to an increase in anthropogenic aerosol emissions. It is driven by the perturbation in cloud droplet number concentration (ΔNd, ant) in liquid-water clouds and is currently understood to exert a cooling effect on climate. The Twomey effect is the key driver in the effective radiative forcing due to aerosol–cloud interactions, but rapid adjustments also contribute. These adjustments are essentially the responses of cloud fraction and liquid water path to ΔNd, ant and thus scale approximately with it. While the fundamental physics of the influence of added aerosol particles on the droplet concentration (Nd) is well described by established theory at the particle scale (micrometres), how this relationship is expressed at the large-scale (hundreds of kilometres) perturbation, ΔNd, ant, remains uncertain. The discrepancy between process understanding at particle scale and insufficient quantification at the climate-relevant large scale is caused by co-variability of aerosol particles and updraught velocity and by droplet sink processes. These operate at scales on the order of tens of metres at which only localised observations are available and at which no approach yet exists to quantify the anthropogenic perturbation. Different atmospheric models suggest diverse magnitudes of the Twomey effect even when applying the same anthropogenic aerosol emission perturbation. Thus, observational data are needed to quantify and constrain the Twomey effect. At the global scale, this means satellite data. There are four key uncertainties in determining ΔNd, ant, namely the quantification of (i) the cloud-active aerosol – the cloud condensation nuclei (CCN) concentrations at or above cloud base, (ii) Nd, (iii) the statistical approach for inferring the sensitivity of Nd to aerosol particles from the satellite data and (iv) uncertainty in the anthropogenic perturbation to CCN concentrations, which is not easily accessible from observational data. This review discusses deficiencies of current approaches for the different aspects of the problem and proposes several ways forward: in terms of CCN, retrievals of optical quantities such as aerosol optical depth suffer from a lack of vertical resolution, size and hygroscopicity information, non-direct relation to the concentration of aerosols, difficulty to quantify it within or below clouds, and the problem of insufficient sensitivity at low concentrations, in addition to retrieval errors. A future path forward can include utilising co-located polarimeter and lidar instruments, ideally including high-spectral-resolution lidar capability at two wavelengths to maximise vertically resolved size distribution information content. In terms of Nd, a key problem is the lack of operational retrievals of this quantity and the inaccuracy of the retrieval especially in broken-cloud regimes. As for the Nd-to-CCN sensitivity, key issues are the updraught distributions and the role of Nd sink processes, for which empirical assessments for specific cloud regimes are currently the best solutions. These considerations point to the conclusion that past studies using existing approaches have likely underestimated the true sensitivity and, thus, the radiative forcing due to the Twomey effect.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

A Lagrangian analysis of pockets of open cells over the southeastern Pacific

Abstract. Pockets of open cells (POCs) have been shown to develop within closed-cell stratocumulus (StCu), and a large body of evidence suggests that the development of POCs result from changes in small-scale processes internal to the boundary layer rather than large-scale forcings. Precipitation is widely viewed as a key process important to POC development and maintenance. In this study, GOES-16 satellite observations are used in conjunction with MERRA-2 winds to track and compare the microphysical and environmental evolution of two populations of closed-cell StCu selected by visual inspection over the southeastern Pacific Ocean: one group that transitions to POCs and another comparison group (CLOSED) that does not. The high spatiotemporal resolution of the new GOES-16 data allows for a detailed examination of the temporal evolution of POCs in this region. We find that POCs tend to develop near the coast, last tens of hours, are larger than 104 km2, and often (88 % of cases) do not re-close before they exit the StCu deck. Most POCs are observed to form at night and tend to exit the StCu during the day when the StCu is contracting in area. Relative to the CLOSED trajectories, POCs have systematically larger effective radii, lower cloud drop number concentrations, a comparable conditional in-cloud liquid water path, and a higher frequency of more intense precipitation. Meanwhile, no systematic environmental differences other than boundary layer height are observed between POC and CLOSED trajectories. Interestingly, there are no differences in reanalysis aerosol optical depth between both sets of trajectories, which may lead one to the interpretation that differences in aerosol concentrations are not influencing POC development or resulting in a large number that re-close. However, this largely depends on the reanalysis treatment of aerosol–cloud interactions, and the product used in this study has no explicit handling of these important processes. These results support the consensus view regarding the importance of precipitation on the formation and maintenance of POCs and demonstrate the utility of modern geostationary remote sensing data in evaluating the POC life cycle.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Cloud drop number concentrations over the western North Atlantic Ocean: seasonal cycle, aerosol interrelationships, and other influential factors

Cloud drop number concentrations (N d ) over the western North Atlantic Ocean (WNAO) are generally highest during the winter (DJF) and lowest in summer (JJA), in contrast to aerosol proxy variables (aerosoloptical depth, aerosol index, surface aerosol mass concentrations, surface cloud condensation nuclei (CCN) concentrations) that generally peak inspring (MAM) and JJA with minima in DJF. Using aircraft, satellite remote sensing, ground-based in situ measurement data, and reanalysis data, we characterize factors explaining the divergent seasonal cycles and furthermore probe into factors influencing N d on seasonal timescales. The results can be summarized well by features most pronounced in DJF, including features associated with cold-air outbreak (CAO) conditions such as enhanced values of CAO index, planetary boundary layer height (PBLH),low-level liquid cloud fraction, and cloud-top height, in addition to winds aligned with continental outflow. Data sorted into high- and low-N d days in each season, especially in DJF, revealed that all of these conditions were enhanced on the high-N d days, including reduced sea level pressure and stronger wind speeds. Although aerosols may be more abundant in MAM and JJA, the conditions needed to activate those particles into cloud droplets are weaker than in colder months, which is demonstrated by calculations of the strongest (weakest) aerosol indirect effects in DJF (JJA) based on comparing N d to perturbations in four different aerosol proxy variables (total and sulfate aerosol optical depth, aerosol index, surface mass concentration of sulfate). We used three machine learning models and up to 14 input variables to infer about most influential factors related to N d for DJF and JJA, with the best performance obtained with gradient-boosted regression tree (GBRT) analysis. The model results indicated that cloud fraction was the most important input variable, followed by some combination (depending on season) of CAO index and surface mass concentrations of sulfate and organic carbon. Future work is recommended to further understand aspects uncovered here such as impacts of free tropospheric aerosol entrainment on clouds, degree of boundary layer coupling, wet scavenging, and giant CCN effects on aerosol–N d relationships, updraft velocity, and vertical structure of cloud properties such as adiabaticity that impact the satellite estimation of N d .

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Ground-based Transmission Spectroscopy with VLT FORS2: Evidence for Faculae and Clouds in the Optical Spectrum of the Warm Saturn WASP-110b

We present a ground-based optical transmission spectrum for the warm Saturn-mass exoplanet WASP-110b from two transit observations made with the FOcal Reducer and Spectrograph on the Very Large Telescope. The spectrum covers the wavelength range from 4000–8333 Å, which is binned in 46 transit depths measured to an averaged precision of 220 parts per million (ppm) over an averaged 80 Å bin for a Vmag = 12.8 star. The measured transit depths are unaffected by a dilution from a close A-type field dwarf, which was fully resolved. The overall main characteristic of the transmission spectrum is an increasing radius with wavelength and a lack of the theoretically predicted pressure-broadened sodium and potassium absorption features for a cloud-free atmosphere. We analyze archival high-resolution optical spectroscopy and find evidence for low to moderate activity of the host star, which we take into account in the atmospheric retrieval analysis. Using the AURA retrieval code, we find that the observed transmission spectrum can be best explained by a combination of unocculted stellar faculae and a cloud deck. Transmission spectra of cloud-free and hazy atmospheres are rejected at a high confidence. With a possible cloud deck at its terminator, WASP-110b joins the increasing population of irradiated hot-Jupiter exoplanets with cloudy atmospheres observed in transmission.

47 OTHER INSTRUMENTATION↗
DOE OSTI2024

Influence of covariance of aerosol and meteorology on co-located precipitating and non-precipitating clouds over the Indo-Gangetic Plain

Aerosol–cloud–precipitation interaction (ACPI) plays a pivotal role in the global and regional water cycle and the earth's energy budget; however, it remains highly uncertain due to the different underlying physical mechanisms. Therefore, this study aims to systematically analyze the effects of aerosols and meteorological factors on ACPI in the co-located precipitating clouds (PCs) and non-precipitating clouds (NPCs) in winter and summer seasons by employing the long-term (2001–2021) retrievals from the Moderate Resolution Imaging Spectroradiometer (MODIS) and Tropical Rainfall Measuring Mission (TRMM) coupled with the National Center for Environmental Prediction/National Center for Atmospheric Research (NCEP/NCAR) reanalysis-II datasets over the Indo-Gangetic Plain (IGP). The results exhibit a decadal increase in aerosol optical depth (AOD) over Lahore (5.2 %), Delhi (9 %), Kanpur (10.7 %), and Gandhi College (22.7 %) and a decrease over Karachi (-1.9 %) and Jaipur (-0.5 %). The most stable meteorology with high values of lower-tropospheric stability (LTS) is found in both seasons over Karachi. In the summer season, the occurrence frequency of clouds is high (74 %) over Gandhi College, 60 % of which are PCs. Conversely, the lowest number of PCs is found over Karachi. Similarly, in the winter season, the frequency of cloud occurrence is low over Karachi and high over Lahore and Gandhi College. The analysis of cloud top pressure (CTP) and cloud optical thickness (COT) indicates high values of cloud fraction (CF) for thick and high-level clouds over all study areas except Karachi. The microphysical properties such as cloud effective radius (CER) and cloud droplet number concentration (CDNC) bear high values (CER ≳ 15 µm and CDNC ≳ 50 cm -3 ) for both NPCs and PCs in summer. The AOD–CER correlation is good (weak) for PCs (NPCs) in winter. Similarly, the sensitivity value of the first indirect effect (FIE) is high (ranging from 0.2 ± 0.13 to 0.3 ± 0.01 in winter and from 0.19 ± 0.03 to 0.32 ± 0.05 in summer) for PCs and low for NPCs. The sensitivity value for the second indirect effect (SIE) is relatively higher (such as 0.6 ± 0.14 in winter and 0.4 ± 0.04 in summer) than FIE. Sensitivity values of the aerosol-cloud interaction (ACI) are low (i.e., -0.06 ± 0.09) for PCs in summer. Furthermore, the precipitation rate (PR) exhibits high values in the summer season, primarily due to the significant contribution from optically thick clouds with lower CDNC (≲ 50 cm -3 ) and larger CER and the intermediate contribution from optically thick clouds with higher CDNC ( ≳ 50 cm -3 ).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Understanding processes that control dust spatial distributions with global climate models and satellite observations

Dust aerosol is important in modulating the climate system at local and global scales, yet its spatiotemporal distributions simulated by global climate models (GCMs) are highly uncertain. In this study, we evaluate the spatiotemporal variations of dust extinction profiles and dust optical depth (DOD) simulated by the Community Earth System Model version 1 (CESM1) and version 2 (CESM2), the Energy Exascale Earth System Model version 1 (E3SMv1), and the Modern-Era Retrospective analysis for Research and Applications version 2 (MERRA-2) against satellite retrievals from Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), Moderate Resolution Imaging Spectroradiometer (MODIS), and Multi-angle Imaging SpectroRadiometer (MISR). We find that CESM1, CESM2, and E3SMv1 underestimate dust transport to remote regions. E3SMv1 performs better than CESM1 and CESM2 in simulating dust transport and the northern hemispheric DOD due to its higher mass fraction of fine dust. CESM2 performs the worst in the Northern Hemisphere due to its lower dust emission than in the other two models but has a better dust simulation over the Southern Ocean due to the overestimation of dust emission in the Southern Hemisphere. DOD from MERRA-2 agrees well with CALIOP DOD in remote regions due to its higher mass fraction of fine dust and the assimilation of aerosol optical depth. The large disagreements in the dust extinction profiles and DOD among CALIOP, MODIS, and MISR retrievals make the model evaluation of dust spatial distributions challenging. Our study indicates the importance of representing dust emission, dry/wet deposition, and size distribution in GCMs in correctly simulating dust spatiotemporal distributions.

54 ENVIRONMENTAL SCIENCES↗