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DOE OSTI2020

A Guided Tour of ab initio Nuclear Many-Body Theory

Over the last decade, new developments in Similarity Renormalization Group techniques and nuclear many-body methods have dramatically increased the capabilities of ab initio nuclear structure and reaction theory. Ground and excited-state properties can be computed up to the tin region, and from the proton to the presumptive neutron drip lines, providing unprecedented opportunities to confront two- plus three-nucleon interactions from chiral Effective Field Theory with experimental data. In this contribution, I will give a broad survey of the current status of nuclear many-body approaches, and I will use selected results to discuss both achievements and open issues that need to be addressed in the coming decade.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2026

A New Window into the Baryon Cycle at Cosmic Noon with Line Intensity Mapping: Forecasts for auto- and cross-correlations in [CII]-158$μ$m, HI 21 cm, CO$_{J+1\rightarrow J}$, and H$α$ galaxies

Across the peak of cosmic star formation at $z\sim1-2$, inflow, processing, and feedback drive rapid changes in the spatial distribution and chemical composition of baryons in galaxies and surrounding reservoirs; this baryon cycle can be tomographically mapped by line intensity mapping (LIM) of atomic hydrogen, ionized carbon, and carbon monoxide. We present a simulation-based forecasting framework for detecting auto- and cross-power spectra between spectroscopic surveys of four such tracers at $z\sim0.5-1.7$ mapping the same deep field - TIM, EoRSpec/FYST, MeerKAT, & Euclid. We forward-model 3-D distributions for these tracers from magnetohydrodynamic simulations, directly capturing the two-halo, one-halo, and shot statistics without relying on analytical decompositions. We further detail a signal-to-noise formalism, tailored to LIM surveys with highly anisotropic geometries and Fourier-space coverage. We demonstrate that galaxy cross-correlations will be the dominant discovery channel for current-generation surveys. These instruments will detect the auto-spectra for CO and HI 21 cm and the CO $\times$ 21 cm cross-spectrum at modest S/N $\sim 1-10$, while placing upper limits on the [CII]-158$μ$m signals. [CII], CO, and HI LIM will be $\sim3-30\times$ ($0.5-1.5$ dex) more sensitive to cross-correlation with the Euclid survey, however, than their respective auto-correlations, constraining all three models of line emission at high significance (S/N $\sim 10-40$) within this decade. Finally, we formulate a staged instrumental trajectory with planned or reasonable improvements, including the as-proposed SKA-Mid. We forecast advancing the per-$k$-mode sensitivities of each auto-, galaxy-line, and line-line spectrum by several orders of magnitude, enabling new percent- and sub-percent level constraints on cosmology and the redshift evolution of star formation and the baryon cycle.

Agrawal, Shubh [Pennsylvania U., Dept. Math.]↗

DOE OSTI2021

DC Circuit Breakers: A Technology Development Status Survey

DC circuit breakers (DCCBs) play a significant role in obtaining the reliability and stability of DC power systems. Selective and fast isolating of faults minimizes the power supply outages to end electricity users and protects the power converters implemented in the DC system. During the last decades, DCCBs have been deeply investigated in industry and academia. There has been impressive progress in terms of efficiency, response time, power-density, lifetime, and electrical operating ratings. Introducing wide bandgap (WBG) devices further has motivated researchers to propose more efficient and novel topologies. This paper provides a point of reference and a background review for DCCBs from novel aspects, fulfilling absent parts in the literature. The elaborated subjects include current commutation circuitry, DCCBs trip-curves developments, newly added functions to DCCBs, as well as marketing analysis. The advancements of DCCBs are surveyed and development needs are recognized. This paper aims to identify the future research needs of DCCBs for emerging DC power systems.

42 ENGINEERING↗

DOE OSTI2025

Automated segmentation and analysis of point clouds of pier foundations using Pier Inspection and Evaluation Report (PIER)

Pier foundations are commonly used in locations with unstable soil or where other types of foundations are unsuitable or cost prohibitive. A pier foundation consists of vertical columns to support the structure and elevate it above the ground. Common materials for pier foundations include masonry, concrete, timber, and steel. The methods for accurate placement of pier foundations have remained relatively unchanged for decades. For simple installations, construction chalk lines are used to layout the locations of piers to ensure accurate placement and elevation. For more complex installations, surveying instruments operated by trained professionals are employed to accurately locate piers and assess correct elevation before construction. After installation, another survey may need to be performed to assess the quality of the as-built foundation. However, with the advent of terrestrial laser scanners (TLS), the means now exist for contractors to conduct their own assessments of as-built foundations. The major barrier preventing contractors from performing their own assessments of as-built foundation quality is the segmentation and analysis of point cloud data, a skill that often requires a trained user. The objective of this research is to develop a software tool (PIER: Pier Inspection and Evaluation Report) to enable automated segmentation and analysis of point clouds of pier foundations. In this paper, the automated segmentation and analysis algorithms are detailed. A mockup lay out of pier foundations was built using concrete masonry units, and the algorithms were tested to evaluate performance. Limitations of the current algorithms and future research direction are discussed.

Turki, Amine [ORNL]↗

DOE OSTI2022

Radio frequency sensing and its innovative applications in diverse sectors: A comprehensive study

Recent advancements in radio frequency (RF) sensing technology can be attributed to the development of the Internet of Things (IoT), healthcare, RF-identification, and communication applications. RF sensing is a multidisciplinary research field that requires expertise in computing, electronics, and electromagnetics to cover all system features, including protocol development, antenna design, sensor integration, algorithm formulation, interconnection, data, and analytics. The overarching aim of this work is to present detailed information about RF technologies and their innovations and application diversity from the novel work carried out at CSI Lab1, together in one platform with an extensive survey. This study presents state-of-the art applications and RF sensing that include W-Fi, radar, and SDR and RFID-based sensing. A comprehensive survey and study of the advantages and limitations of each non-contact technology is discussed. Additionally, open research gaps have been identified as well. Decades of knowledge and experience have been put to use to meet new challenges and demands. The development and study of RF systems, IoT, RFID sensing, and research and deployment activities, are briefly discussed. The emerging research projects with industry, institutional research centers, and academic studies are also addressed. Finally, an outline of identified potential future research areas is provided, emphasizing opportunities and challenges.

47 OTHER INSTRUMENTATION↗

DOE OSTI2020

A Rapid Sequential Separation Method for Determination of Actinides and TENORM in Fracking Wastes - 20223

With recent advances in unconventional drilling technology in the US and around the world, the risks of environmental contamination and exposure due to technologically enhanced naturally occurring radioactive materials (TENORM) from fracking wastes have also surfaced. Although the Permian Basin (southeastern New Mexico, western Texas) has long been a modest producer of oil, the advent of fracking technology a decade ago turned it into hot property for producers. A 2018 assessment of undiscovered, technically recoverable continuous oil and gas resources by the U.S. Geological Survey estimates an average 46.3 billion barrels of oil and 281 trillion cubic feet of gas. This is likely to increase the use of unconventional drilling and TENORM generation. TENORM concentrations in oil and gas exploration and production waste can be several hundred to several thousand times higher than background TENORM concentrations. Both the thorium and uranium decay chains contribute to airborne radionuclides arising from the radon gas escaping the ground and subsequently decaying as airborne particulates. Additionally, radon decay products {sup 210}Pb and {sup 210}Po can build up in scale on the internal surfaces of oil and gas handling pipes and in sludge in refineries, becoming potential inhalation and ingestion hazards for workers. Furthermore, southeastern NM is also home to world's only licensed and operating transuranic nuclear waste repository, the DoE's Waste Isolation Pilot Plant (WIPP). Plutonium isotopes ({sup 239+240}Pu) and {sup 241}Am, are expected to account for more than 99% of the total radioactivity scheduled for disposal in the WIPP repository. Thus, an improved understanding of the environmental fate and transport of TENORM, liberated by unconventional drilling, is essential to assess how best to protect individuals and the environment. In this context, accurate measurement of TENORM and actinides in environmental and biological samples is essential. In this presentation, a new sequential method for the separation and pre-concentration of actinides (Pu, Am, Np) and TENORM (Po, U and Th) derived from oil and gas exploration is proposed. The TEVA method involves a rapid co-precipitation step to remove matrix interferences from the samples, followed by plutonium oxidation state adjustment to Pu (IV) and an incubation period of ∼ 1 hour at 50-60 deg. C to allow the resultant Po (II) to oxidize into Po(IV). The polonium, neptunium, thorium and plutonium are then separated on a TEVA column, while americium and uranium are separated on a TRU column. After separation, the alpha counting source was prepared by micro-precipitation with copper sulfide (CuS) for polonium and neodymium fluoride (NdF{sub 3}) for actinides. The efficiency and reliability of the procedures were tested by analyzing filter, drinking water and frack sand samples. The method is simple, robust and can be performed quickly with excellent removal of interferences, high chemical recovery and very good alpha peak resolution. (authors)

07 ISOTOPE AND RADIATION SOURCES↗

DOE OSTI2025

Peeking into the next decade in large-scale structure cosmology with its Effective Field Theory

After the successful full-shape analyses of BOSS data using the Effective Field Theory of Large-Scale Structure, we investigate what upcoming galaxy surveys might achieve. We introduce a “perturbativity prior” that ensures that loop terms are as large as theoretically expected, which is effective in the case of a large number of EFT parameters. After validating our technique by comparison with already-performed analyses of BOSS data, we provide Fisher forecasts using the one-loop prediction for power spectrum and bispectrum for two benchmark surveys: DESI and MegaMapper. We find overall great improvements on the cosmological parameters. In particular, we find that MegaMapper (DESI) should obtain at least a 12σ (2σ) evidence for non-vanishing neutrino masses, bound the curvature Ω k to 0.0012 (0.012), and primordial inflationary non-Gaussianities as follows: f NL loc. to ± 0.26 (3.3), f NL eq. to ±16 (92), f NL orth. to ± 4.2 (27). Such measurements would provide much insight on the theory of Inflation. We investigate the limiting factor of shot noise and ignorance of the EFT parameters.

cosmological parameters from LSS↗

DOE OSTI2022

Topological Materials for Functional Optoelectronic Devices

The recent realization of topology as a mathematical concept in condensed matter systems has shattered Landau's widely accepted classification of phases by spontaneous symmetry breaking as he famously said, “a particular symmetry property exists or does not exist.” Topological materials (TMs) such as topological insulators and topological semimetals, are characterized by properties that depend on the topology of the band structure. Such dependence has drastic implications on the optical, electrical, and thermal properties of the material. Fundamental physics of TMs is currently under active research in condensed matter, materials science, and high energy physics. Here, recent advances in exploiting the unique properties of TMs to realize functional optoelectronic devices are surveyed. Current and future applications that are, or may be, enabled by their unique properties are discussed. Although many theoretical ideas have been proposed over the past decade or so on using TMs in optoelectronic applications, the focus will be on experimentally realized devices.

36 MATERIALS SCIENCE↗

DOE OSTI2022

A tale of a tail: a tidally disrupting ultra-diffuse galaxy in the M81 group

ABSTRACT We present the discovery of a giant tidal tail of stars associated with F8D1, the closest known example of an ultra-diffuse galaxy (UDG). F8D1 sits in a region of the sky heavily contaminated by Galactic cirrus and has been poorly studied since its discovery two decades ago. The tidal feature was revealed in a deep map of resolved red giant branch stars constructed using data from our Subaru Hyper Suprime-Cam survey of the M81 Group. It has an average surface brightness of μg ∼ 32 mag arcsec−2 and can be traced for over a degree on the sky (60 kpc at the distance of F8D1) with our current imagery. We revisit the main body properties of F8D1 using deep multiband imagery acquired with MegaCam on CFHT and measure effective radii of 1.7–1.9 kpc, central surface brightnesses of 24.7–25.7 mag, and a stellar mass of ∼7 × 107M⊙. Assuming a symmetric feature on the other side of the galaxy, we calculate that 30–36 per cent of F8D1’s present-day luminosity is contained in the tail. We argue that the most likely origin of F8D1’s disruption is a recent close passage to M81, which would have stripped its gas and quenched its star formation. As the only UDG that has so far been studied to such faint surface brightness depths, the unveiling of F8D1’s tidal disruption is important. It leaves open the possibility that many other UDGs could be the result of similar processes, with the most telling signatures of this lurking below current detection limits.

Žemaitis, Rokas (ORCID:0000000285660491)↗

DOE OSTI2022

Advanced Heterogeneous Integration Enabled by 3D Freestanding Membranes—From Material Growths to Applications

For the future of electronics such as bioelectronics, 3D integrated electronics, and bendable electronics, the need for flexibility and stackability of electronic products has substantially grown up. However, conventional wafer-based single-crystalline semiconductors cannot catch up with such trends because they are bound to thick rigid wafers such that they are neither flexible nor stackable. Although polymer-based organic electronic materials are more compatible as they are mechanically compliant and less costly than inorganic counterparts, their electronic/photonic performance is substantially inferior to that of single-crystalline inorganic materials. Such performance-mechanical compliance dilemma could be resolved by developing methods to obtain cheap, flexible, stackable, single-crystalline inorganic systems. Such dream electronic systems could be realized by producing single-crystalline freestanding membranes. For the past few decades, various layer transfer techniques (a.k.a layer liftoff techniques) have been developed to produce single-crystalline freestanding membranes. In today's talk, I will present the survey of the layer liftoff techniques and go over how these strategies unlock new ways of manufacturing advanced electronic systems. In addition, I will introduce unprecedented artificial heterostructure devices enabled by stacking of those freestanding 3D material membranes, e.g., the world's smallest vertically-stacked full-color micro-LEDs, the world's best multiferroic devices, chip-less wireless e-skin, and reconfigurable hetero-integrated chips with AI accelerators.

Kim, Jeehwan↗

DOE OSTI2022

Advanced Heterogeneous Integration Enabled by 3D Freestanding Membranes—From Material Growths to Applications

Kim, Jeehwan↗

DOE OSTI2022

HT Lyn and IR Lyn: Two Semi-detached-type Near-contact Binaries with Stable Orbital Period

Abstract We presented the first photometric and orbital period investigations for two near-contact binaries: HT Lyn and IR Lyn. The light-curves solutions derived from both our ground-based and various surveys’ observations suggested that HT Lyn and IR Lyn are two semi-detached-type near-contact binaries with the secondary and primary components filling the Roche lobe. Combining the eclipse timings derived from several surveys’ data and our observations with those reported in the literature, we modified the orbital periods and revealed that their orbital periods were stable for the last two decades. The absolute physical parameters were well determined by using the empirical relations and the Gaia-distance-based method. Similar to other near-contact binaries, the primary components of HT Lyn and IR Lyn are evolving at the main-sequence stage, while their less-massive secondary components show the over-sized and over-luminosity features and should be more evolved than their primary ones. Combining the stable orbital period with the semi-detached configurations, we infer that the two near-contact binaries may be just located in the critical phase and evolving from the current semi-detached phase to the detached or contact one.

Astronomy & Astrophysics↗

DOE OSTI2022

Estimating the impact of foregrounds on the future detection of Rayleigh scattering

Rayleigh scattering of the cosmic microwave background (CMB) by neutral hydrogen shortly after recombination leaves frequency-dependent imprints on intensity and polarization fluctuations. High signal-to-noise observations of CMB Rayleigh scattering would provide additional insight into the physics of recombination, including greater constraining power for parameters like the primordial helium fraction, the light relic density, and the sum of neutrino masses. However, such a measurement of CMB Rayleigh scattering is challenging due to the presence of astrophysical foregrounds, which are more intense at the high frequencies, where the effects of Rayleigh scattering are most prominent. Here we forecast the detectability of CMB Rayleigh scattering including foreground removal using blind internal linear combination methods for a set of near-future surveys. Furthermore, we show that atmospheric effects for ground-based observatories and astrophysical foregrounds pose a significant hindrance to detecting CMB Rayleigh scattering with experiments planned for this decade, though a high-significance measurement should be possible with a future CMB satellite.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2023

The SOUX AGN sample: optical/UV/X-ray SEDs and the nature of the disc

We use the SOUX sample of ~700 active galactic nucleus (AGN) to form average optical-ultraviolet (UV)-X-rays spectral energy distributions (SEDs) on a two-dimensional (2D) grid of M BH and L 2500 . We compare these with the predictions of a new AGN SED model, qsosed, which includes prescriptions for both hot and warm Comptonization regions as well as an outer standard disc. This predicts the overall SED fairly well for 7.5 < log(M BH /M ⊙ ) < 9.0 over a wide range in L/L Edd , but at higher masses the outer disc spectra in the model are far too cool to match the data. We create optical-UV composites from the entire Sloan Digital Sky Survey sample and use these to show that the mismatch is due to there being no significant change in spectral shape of the optical-UV continuum across several decades of M BH at constant luminosity. We show for the first time that this cannot be matched by standard disc models with high black hole spin. These apparently fit, but are not self-consistent as they do not include the General Relativistic effects for the emission to reach the observer. At high spin, increased gravitational redshift compensates for almost all of the higher temperature emission from the smaller inner disc radii. The data do not match the predictions made by any current accretion flow model. Either the disc is completely covered by a warm Comptonization layer whose properties change systematically with L/L Edd , or the accretion flow structure is fundamentally different to that of the standard disc models.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2020

Long-term Photometry and Orbital Period Change of the W UMa–type Binary v0599 Aur: Evidence of about 11 yr Magnetic-activity Cycle

Combining all available photometric data from various surveys and literature with our observations, we present 10 sets of light curves for the eclipsing binary V0599 Aur covering a timescale of 20 yr. During the last two decades, the O’Connell effect continuously varied and went through at least two flips between positive and negative effects. The photometric solutions from our two sets of multicolored light curves show that V0599 Aur is a W-type shallow contact binary with an active spot on the secondary. Its absolute parameters are determined by combining the Gaia distance with the photometric solutions. The period investigation reveals a secular decrease and a cyclic variation in its orbital period. The former mainly originates from the mass transfer from the more massive secondary to the less massive primary. The latter can be preferentially explained as a result of cyclic magnetic activity of the secondary, with three observational supports: (1) the existence and evolution of an active spot suggested by the long-term photometry, (2) periodic variation in both the O’Connell effect and relative luminosity, and (3) weak correlations between O’Connell effect/relative luminosity changes and cyclic period variation. Together with the cyclic period variation and its theoretical reasonability by Applegate’s mechanism, we suggest that the secondary of V0599 Aur is a solar-type magnetic-activity star with an approximately 11 yr active cycle. Furthermore, by combining the secular period decrease with the Roche-lobe model, we infer that V0599 Aur is evolving from the marginal contact state controlled by thermal relaxation oscillation theory to the overcontact state.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2022

The Time Domain Spectroscopic Survey: Changing-look Quasar Candidates from Multi-epoch Spectroscopy in SDSS-IV

Active galactic nuclei (AGN) can vary significantly in their rest-frame optical/UV continuum emission, and with strong associated changes in broad line emission, on much shorter timescales than predicted by standard models of accretion disks around supermassive black holes. Most such changing-look or changing-state AGN—and at higher luminosities, changing-look quasars (CLQs)—have been found via spectroscopic follow-up of known quasars showing strong photometric variability. The Time Domain Spectroscopic Survey of the Sloan Digital Sky Survey IV (SDSS-IV) includes repeat spectroscopy of large numbers of previously known quasars, many selected irrespective of photometric variability, and with spectral epochs separated by months to decades. Our visual examination of these repeat spectra for strong broad line variability yielded 61 newly discovered CLQ candidates. We quantitatively compare spectral epochs to measure changes in continuum and Hβ broad line emission, finding 19 CLQs, of which 15 are newly recognized. The parent sample includes only broad line quasars, so our study tends to find objects that have dimmed, i.e., turn-off CLQs. However, we nevertheless find four turn-on CLQs that meet our criteria, albeit with broad lines in both dim and bright states. We study the response of Hβ and Mg ii emission lines to continuum changes. The Eddington ratios of CLQs are low, and/or their Hβ broad line width is large relative to the overall quasar population. Repeat quasar spectroscopy in the upcoming SDSS-V black hole Mapper program will reveal significant numbers of CLQs, enhancing our understanding of the frequency and duty cycle of such strong variability, and the physics and dynamics of the phenomenon.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2024

Graphitic Carbon Nitride Quantum Dots (g‐C 3 N 4 QDs): From Chemistry to Applications

Since their emergence in 2014, graphitic carbon nitride quantum dots (g-C 3 N 4 QDs) have attracted much interest from the scientific community due to their distinctive physicochemical features, including structural, morphological, electrochemical, and optoelectronic properties. Owing to their desirable characteristics, such as non-zero band gap, ability to be chemically functionalized or doped, possessing tunable properties, outstanding dispersibility in different media, and biocompatibility, g-C 3 N 4 QDs have shown promise for photocatalysis, energy devices, sensing, bioimaging, solar cells, optoelectronics, among other applications. As these fields are rapidly evolving, it is very strenuous to pinpoint the emerging challenges of the g-C 3 N 4 QDs development and application during the last decade, mainly due to the lack of critical reviews of the innovations in the g-C 3 N 4 QDs synthesis pathways and domains of application. Herein, an extensive survey is conducted on the g-C 3 N 4 QDs synthesis, characterization, and applications. Scenarios for the future development of g-C 3 N 4 QDs and their potential applications are highlighted and discussed in detail. In conclusion, the provided critical section suggests a myriad of opportunities for g-C 3 N 4 QDs, especially for their synthesis and functionalization, where a combination of eco-friendly/single step synthesis and chemical modification may be used to prepare g-C 3 N 4 QDs with, for example, enhanced photoluminescence and production yields.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2024

Understanding piezocatalysis, pyrocatalysis and ferrocatalysis

The last decade has witnessed the emergence of the application of piezoelectric and ferroelectric materials for catalytic and photocatalytic applications that harness light, thermal and mechanical energy into chemical reactions. This article surveys the different concepts of pyro- and piezocatalysis and differences with respect to ferrocatalysis and switchable catalysis and delves into the current understanding of the mechanisms underlying piezocatalysis. The outlook for advancing in the surface science studies required for the design of new and better catalysts based on polar electromechanically active materials is discussed in the context of the state of the art experimental studies and potential future nanoscience developments.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗