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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 109 records · Page 6
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Theory of resonant x-ray scattering with ultrafast intense pulses

Here, we present a time-dependent Schrödinger equation approach within a nonrelativistic quantum electrodynamics framework to investigate resonant x-ray scattering driven by intense x-ray pulses. This method enables us to explore how coherent x-ray electron dynamics influence scattering signals from Ne + . We account for both resonance fluorescence and elastic scattering channels, while also considering competing photoionization and inner-shell decay processes. By computing the angular distribution and energy spectrum of scattered photons, we uncover interference effects between elastic scattering and resonance fluorescence pathways. Notably, this interference results in a small asymmetry in the energy spectrum. We discuss the experimental potential for detecting signatures of interference. Our findings demonstrate that the x-ray Rabi dynamics can be used to control scattering responses and provide insights into interference mechanisms and scattering efficiency in high-intensity x-ray regimes.

Venkatesh, Akilesh [Argonne National Laboratory (A↗
DOE OSTI2023

Search for Higgs Boson and Observation of $Z$ Boson through Their Decay into a Charm Quark-Antiquark Pair in Boosted Topologies in Proton-Proton Collisions at $\sqrt{s}$ = 13 TeV

A search for the standard model (SM) Higgs boson ($H$) produced with transverse momentum ($p_T$) greater than 450 GeV and decaying to a charm quark-antiquark ($c\bar{c}$) pair is presented. The search is performed using proton-proton collision data collected at $\sqrt{s} = 13$ TeV by the CMS experiment at the LHC, corresponding to an integrated luminosity of 138 fb$^{-1}$. Boosted $H \to c\overline{c}$ decay products are reconstructed as a single large-radius jet and identified using a deep neural network charm tagging technique. The method is validated by measuring the $Z \to c\bar{c}$ decay process, which is observed in association with jets at high $p_T$ for the first time with a signal strength of $1.00^{+0.17}_{-0.14}$ (syst)$\pm 0.08$ (theo) $\pm 0.06$ (stat), defined as the ratio of the observed process rate to the SM expectation. The observed (expected) upper limit on $\sigma (H){\cal B}(H \to c\overline{c})$ is set at 47 (39) times the SM prediction at 95\%confidence level.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Cold freeze out of superheavy dark matter and Hubble tension

We present a unified framework, the "X miracle", in which dark matter consists of superheavy, nonthermal X particles whose relic abundance is determined not by the conventional weak-scale, semi-relativistic ("hot") freeze-out of WIMPs, but by annihilation or decay occurring within the smallest and earliest gravitationally bound objects. Unlike thermal WIMPs, which decouple at velocities of order 0.3c with relic abundance ρ∞ set by weak-scale interactions, X particles are produced nonthermally with an initial overabun dance ρ ini >> ρ ∞ . They become nonrelativistic extremely early, redshift to ultra-cold velocities, allowing collapse into compact bound structures characterized by a novel quantum gravitational scale, r X = 4$\hbar$ 2 $/Gm^3_X$ = 10 −13 m $\hbar$$/m_Xc$, much larger than the Compton wavelength. The framework predicts a particle mass of 10 12 GeV and an enhanced cross section of 10 −21 m 3 /s. Overlapping particle wavefunctions in these compact structures drive annihilation or decay into additional radiation, leading to a "cold" freeze-out that converts most of ρ ini into radiation while leaving a relic density ρ ∞ . Solutions to the Boltzmann equation indicate that an extreme ("big") depletion, with only one particle in a billion surviving, yields an additional radiation contribution $ΔN_{eff}$ ≈ 0.4, which could help alleviate the Hubble tension. For particles of 10 12 GeV, the scenario predicts a dark coupling constant α X = 0.09 that is responsible for an instanton-induced decay process, consistent with current UHECR bounds. Early collapse at 10 −6 s may release binding energy as high-frequency (100kHz) gravitational waves or ultralight GUT-scale axions (10 −9 eV). Superheavy sterile neutrinos provide a natural particle realization, linking dark matter to neutrino mass and baryogenesis. If gravitationally produced, this framework favors high-scale inflation and effi cient reheating. The "X miracle" thus demonstrates that dark matter need not be weak-scale: gravitational dynamics can control freeze-out and evolution, producing multi-messenger observational signatures in UHECRs, axions, gravitational waves, and small-scale structures.

Xu, Zhijie Jay [Pacific Northwest National Laborat↗
DOE OSTI2021

Conjugated-linker dependence of the photophysical properties and electronic structure of chlorin dyads

The synthesis, photophysical properties and electronic structure of seven new chlorin dyads and associated benchmark monomers are described. Each dyad contains two identical chlorins linked at the macrocycle β-pyrrole 13-position. The extent of electronic communication between chlorin constituents depends on the nature of the conjugated linker. The communication is assessed by modification of prominent ground-state absorption and redox properties, rate constants and yields of excited-state decay processes, and molecular-orbital characteristics. Relative to the benchmark monomers, the chlorin dyads in toluene exhibit a substantial bathochromic shift of the long-wavelength absorption band (30 nm average), two-fold increased radiative rate constant [average (10 ns) -1 vs. (22 ns) -1 ], reduced singlet excited-state lifetimes (average 5.0 ns vs. 8.2 ns), and increased fluorescence quantum yields (average 0.56 vs. 0.42). The excited-state lifetime and fluorescence yield for the chlorin dyad with a benzothiadiazole linker are reduced substantially in benzonitrile vs. toluene due largely to ~25-fold accelerated internal conversion. The results aid design strategies for molecular architectures that may find utility in solar-energy conversion and photomedicine.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Studies of surface adsorbate electronic structure and femtochemistry at the fundamental length and time scales. Final report

The electronic structure and ultrafast (10-15 s-femtosecond timescale) electron dynamics were investigated for clean and atom/molecule covered metal surfaces. The studies were performed by scanning tunneling microscopy (STM) to measure the structure of adsorbed atoms and molecules on metal surfaces, and to investigate their electronic properties. The electronic structure of the observed molecular networks was calculated by electronic structure theory in collaboration with Prof. Jin Zhao, who is a long-time collaborator, a Professor at the University of Science and Technology of China, and holds an Adjunct Professorship at the University of Pittsburgh. We also investigated the electronic properties of C60 molecules when they are templated by corrugated black phosphorous surfaces. We found unexpected charge delocalization that is enabled by the templating. This research was done in collaboration with Professor Min Feng at the Wuhan University, and who also holds an Adjunct Professorship at the University of Pittsburgh. Moreover, the electronic structure and electron dynamics in metal surfaces were investigated by time-resolved photoemission electron spectroscopy. The focus of ultrafast spectroscopy has been on the plasmonic response of silver surfaces. One direction has been to develop multidimensional (energy, momentum, and time) photoelectron spectroscopy of the coherent response of solid surfaces. This method was applied to study the collective electron excitations known generally as plasmons, which screen optical fields from penetration into metals. Although this collective response has been known for more than 60 years and is used extensively to deposit optical energy into metals, how this happens is poorly known. We investigated the plasmonic response of silver at the point where the dielectric response passes through zero and bulk plasmon is excited by light. We discovered that the plasmon excitation decays by exciting electrons from the Fermi level of a metal, which is contrary to what is believed in the plasmonic science community. This research has been performed in collaboration with Dr. Marcel Reutzel, who was a postdoctoral fellow working on this research at the University of Pittsburgh, and now has a faculty position at the University of Göttingen in Germany. Prof. Branko Gumhalter from the Institute of Physics in Zagreb contributed on the theory of plasmonic decay processes. Furthermore, we investigated the Floquet engineering of electronic bands in metals leading to multiphoton photoemission and above threshold photoemission. Finally, we demonstrated that it is possible to change the electronic structure of metals by application of optical fields. Our studies indicated that this happens on subfemtosecond time scale and could potentially be used in ultrafast information processing and quantum computation. Related document information

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

Quantum Information Science in High Energy Physics at the Large Hadron Collider (Final Report-QuantISED)

We pursue scientific research at the interface of High Energy Physics and Quantum Information Science. This includes studies of thermal radiation and quantum entanglement in high-energy collisions at the Large Hadron Collider (LHC), with special emphasis on entanglement entropy and the Higgs boson. This project has also been extended to include quantum entanglement and charged current weak interactions using Fermilab results. And most recently, we have begun tests of the temporal entanglement using LHC data. Collider experiments such as proton-proton collisions at the LHC yield hadrons that exhibit an exponential behavior at low transverse momenta. This surprising behavior is seen in data from both the ATLAS and CMS collaborations. We attribute this phenomenon to quantum entanglement between the regions in the nucleon wave function. The exponential component to the transverse momentum distribution is a result of thermal radiation that is akin to Hawking or Unruh radiation that should exist at the event horizon of astrophysical black holes and neutron stars. The Principal Investigator, in collaboration with a theoretical physicist at Stony Brook University and Brookhaven National Laboratory, and with Yale University students, has shown evidence for this thermal radiation in several production and decay processes in the ATLAS and CMS data, and its connection to entanglement entropy (O.K. Baker and D.E Kharzeev, Phys. Rev. D 98, 054007 (2018)), including even the Higgs boson sector. Interestingly, this thermal behavior is also seen in momentum distributions of charged current weak interactions according to our studies. These findings suggest a deep connection between quantum entanglement (entanglement entropy) and thermalization in both hadron collisions at the energy frontier and neutrino scattering at the intensity frontier. We have confirmed the proposed relation between the effective temperature and the hard-scattering scale at lower energies using the most recent LHC data for the following systems: Higgs bosons, top quarks, and charged hadrons. Additionally, we have results for hadron production in neutrino scattering from nuclei using Fermilab weak interaction data. This study is carried out using data from the MINERvA collaboration. In those cases where entanglement is expected, there is an exponential component to the momentum distribution, while this component is absent in those processes where no entanglement is expected. This research thus tests the hypothesis about a link between quantum entanglement and thermalization in strong and weak interactions. See Phys Lett B 811, 135948 (2020). We also initiated research applying a quantum search algorithm (Grover's Algorithm) to LHC data. This quantum algorithm was used to show how rare events in LHC data can be searched for in large, unsorted databases, with quadratic speedup compared to classical search algorithms on classical computers. See "Application of a Quantum Search Algorithm to High- Energy Physics Data at the Large Hadron Collider", arXiv:2010.00649 [quant-ph].

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

A new aerial approach for quantifying and attributing methane emissions: implementation and validation

Methane (CH 4 ) is a powerful greenhouse gas that is produced by a diverse set of natural and anthropogenic emission sources. Biogenic methane sources generally involve anaerobic decay processes such as those occurring in wetlands, melting permafrost, or the digestion of organic matter in the guts of ruminant animals. Thermogenic CH 4 sources originate from the breakdown of organic material at high temperatures and pressure within the Earth's crust, a process which also produces more complex trace hydrocarbons such as ethane (C 2 H 6 ). Here, we present the development and deployment of an uncrewed aerial system (UAS) that employs a fast (1 Hz) and sensitive (1–0.5 ppb s -1 ) CH 4 and C 2 H 6 sensor and ultrasonic anemometer. The UAS platform is a vertical-takeoff, hexarotor drone (DJI Matrice 600 Pro, M600P) capable of vertical profiling to 120 m altitude and plume sampling across scales up to 1 km. Simultaneous measurements of CH 4 and C 2 H 6 concentrations, vector winds, and positional data allow for source classification (biogenic versus thermogenic), differentiation, and emission rates without the need for modeling or a priori assumptions about winds, vertical mixing, or other environmental conditions. The system has been used for direct quantification of methane point sources, such as orphan wells, and distributed emitters, such as landfills and wastewater treatment facilities. With detectable source rates as low as 0.04 and up to ~1500 kg h -1 , this UAS offers a direct and repeatable method of horizontal and vertical profiling of emission plumes at scales that are complementary to regional aerial surveys and localized ground-based monitoring.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Thermal modeling of three lakes within the continuous permafrost zone in Alaska using the LAKE 2.0 model

Abstract. Lakes in the Arctic are important reservoirs of heat with much lower albedo in summer and greater absorption of solar radiation than surrounding tundra vegetation. In the winter, lakes that do not freeze to their bed have a mean annual bed temperature >0 ∘C in an otherwise frozen landscape. Under climate warming scenarios, we expect Arctic lakes to accelerate thawing of underlying permafrost due to warming water temperatures in the summer and winter. Previous studies of Arctic lakes have focused on ice cover and thickness, the ice decay process, catchment hydrology, lake water balance, and eddy covariance measurements, but little work has been done in the Arctic to model lake heat balance. We applied the LAKE 2.0 model to simulate water temperatures in three Arctic lakes in northern Alaska over several years and tested the sensitivity of the model to several perturbations of input meteorological variables (precipitation, shortwave radiation, and air temperature) and several model parameters (water vertical resolution, sediment vertical resolution, depth of soil column, and temporal resolution). The LAKE 2.0 model is a one-dimensional model that explicitly solves vertical profiles of water state variables on a grid. We used a combination of meteorological data from local and remote weather stations, as well as data derived from remote sensing, to drive the model. We validated modeled water temperatures with data of observed lake water temperatures at several depths over several years for each lake. Our validation of the LAKE 2.0 model is a necessary step toward modeling changes in Arctic lake ice regimes, lake heat balance, and thermal interactions with permafrost. The sensitivity analysis shows us that lake water temperature is not highly sensitive to small changes in air temperature or precipitation, while changes in shortwave radiation and large changes in precipitation produced larger effects. Snow depth and lake ice strongly affect water temperatures during the frozen season, which dominates the annual thermal regime of Arctic lakes. These findings suggest that reductions in lake ice thickness and duration could lead to more heat storage by lakes and enhanced permafrost degradation.

Clark, Jason A. (ORCID:0000000248105261)↗
NASA NTRS1974

Mercury - Does its atmosphere contain water

The atmosphere of Mercury, like that of the moon, is maintained in an extremely tenuous minimum state by weak solar wind accretion and radioactive decay processes, and depleted by strong removal mechanisms. Unlike the moon, it has a high daytime surface temperature that promotes the production of water vapor, which may be the dominant atmospheric constituent derived from solar wind protons.

Thomas, G. E.↗
NASA NTRS1974

The protons and electrons trapped in the Jovian dipole magnetic field region and their interaction with Io

Detailed analysis of electrons equal to or greater than 3 MeV and of protons 0.5 to 1.8 MeV and equal to or greater than 35 MeV for both the inbound and the outbound passes of the Pioneer 10 spacecraft. Conclusive evidence is obtained that the trapped radiation in Jupiter's inner magnetosphere is maintained and supplied by inward diffusion from the outer regions of the trapped radiation zone. It is shown that the time required for isotropization of an anisotropic flux by pitch angle scattering inside L approximately equal to 6 is long in comparison with the time required for particles to diffuse inward from L approximately equal to 6 to L approximately equal to 3, that the high-energy protons were not injected at high energies by the Crand (cosmic ray albedo neutron decay) process but were accelerated in the magnetosphere of Jupiter, and that the main conclusions of this analysis are unaffected by use of either the D sub 1 or the D sub 2 magnetic field models. Theoretical studies of the capture of trapped electrons and protons by Io have been carried out, and it is found that the probability of capture by Io depends strongly upon the particle species and kinetic energy.

Simpson, J. A.↗
NASA NTRS1977

Microchannel plate life tests

The behavior of the gain of a microchannel plate (MCP) during operation of the latter at moderate output currents was investigated. The total charge per unit area, Q, extracted from the MCP is shown to be the relevant quantity for evaluating MCP performance. The shape of the gain versus Q curve provides information on the gain decay process. Long periods of stable gain, frequently exhibited by channeltrons, were not observed in the present experiment.

Sandel, B. R.↗
NASA NTRS1982

Three-dimensional flow field in the tip region of a compressor rotor passage. II - Turbulence properties

The turbulence properties in the annulus wall region of an axial flow compressor rotor was measured using a triaxial, hot-wire probe rotating with the rotor. The flow was surveyed across the entire passage at five axial locations (leading edge, 1/4 chord, 1/2 chord, 3/4 chord, and the trailing edge location) and at six radial locations in a low-speed compressor rotor. The data derived include all three components of turbulence intensity and three components of turbulence stress. A comprehensive interpretation of the data with emphasis on features related to rotation, leakage flow, annulus wall boundary layer, and blade boundary layer interactions is included. All the components of turbulent intensities and stresses are found to be high in the leakage-flow mixing region. The radial component of intensities and stresses is found to be much higher than the corresponding streamwise components. The turbulent spectra clearly reveal the decay process of the inlet-guide-vane wake within the rotor passage.

Lakshminarayana, B.↗
NASA NTRS1984

Thermal metamorphism of Si2O3 - (A circumstellar dust analog)

The thermal behavior of Si2O3, the metastable condensate from SiO vapor,has been studied experimentally. Si2O3 and its successor, amorphous quartz, have previously been shown to have infrared spectral features similar to some that appear in the spectra of grains in oxygen-rich circumstellar regions. Thermal annealing experiments show that only one Si2O3 decay process operates over the range between 750-1000 K. This process is a unimolecular disproportionation. The rate of this transformation can be expressed as k/hr = 10 to the 9th exp (-40 kcal/mole/RT). By using this rate constant, it is found that a significant fraction of freshly nucleated circumstellar grains can survive passage through a typical circumstellar shell virtually unaltered in structure. It is emphasized that this is only the first in a series of laboratory experiments intended to study the metamorphism of newly condensed circumstellar material ejected into the interstellar medium. Grains similar to these might have been incorporated into the primitive solar nebula, provided that they could also survive passage through the general interstellar medium.

Nuth, J. A.↗
NASA NTRS1987

The plasma wave environment of an auroral arc. III - VLF hiss

Auroral hiss in the vicinity of a quiet arc is studied by comparing the data obtained from a sounding rocket with predictions of the convective beam amplification (CBA) model of auroral hiss generation. It is concluded that the VLF auroral hiss observed by the payload appears to have been natural in origin. The CBA model produces predicted hiss spectra that are in good agreement with the data. The hiss intensity above the ionosphere was greater equatorward of the arc than within the arc; this pattern appears to be the result of emission geometry and refraction. Hiss intensity was not found to be better correlated with 0.1-0.7 keV fluxes than with more energetic electrons. No evidence is found for a three-wave parametric decay process. The data are consistent with a weak hiss source located at an altitude of 110-120 km.

Bering, E. A.↗
NASA NTRS1987

Diversity and similarity of comets

The evolution of comets from an early stage where they were all similar, to the later diversity is reviewed. The elemental abundances of all pristine comets are likely to be primitive, that is in solar abundance ratios for all elements including C, N, O, S, but with the exception of H (and assumedly He and Ne) that are severely depleted. The solid phase was originally in very fine grains, typically 0.1 micron or less, eventually sintered into larger grain clusters. The volatile phase contains H, C, N, O, and S molecules frozen in the pores of the grain clusters; cosmic ray plus solar irradiation changes the volatile to refractory ratio of the crust. Differences in dust tails, in plasma tails, in photometry between young and old comets, and in the variable carbon depletion of the gas phase seem to be induced by the decay processes.

Delsemme, A. H.↗