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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 109 records · Page 6

Terahertz field enhancement via coherent superposition of the pulse sequences after a single optical-rectification crystal

Terahertz electromagnetic pulses are frequently generated by optical rectification of femtosecond laser pulses. In many cases, the efficiency of this process is known to saturate with increasing intensity of the generation beam because of two-photon absorption. Here, we demonstrate two routes to reduce this effect in ZnTe(110) crystals and enhance efficiency, namely, by (i) recycling the generation pulses and by (ii) splitting each generation pulse into two pulses before pumping the crystal. In both methods, the second pulse arrives ∼1 ns after the first one, sufficiently long for optically generated carriers to relax. Enhancement is achieved by coherently superimposing the two resulting terahertz fields.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Large optical nonlinearity of ITO nanorods for sub-picosecond all-optical modulation of the full-visible spectrum

Optical nonlinearity induced by intense optical excitation of mobile electrons in metallic nanostructures can provide dynamic tuning of their electromagnetic response, which is potentially useful for all-optical information processing. Here we report on the sub-picosecond optical nonlinearity of indium tin oxide nanorod arrays (ITO-NRAs) following intraband, on-plasmon-resonance optical pumping, which enables modulation of the full-visible spectrum with large absolute change of transmission, favorable spectral tunability and beam-steering capability. We semi-quantitatively model the permittivity change, whose large amplitude stems from a significant electron redistribution under intraband pumping due to the low electron concentration. Further, we observe a transient response in the microsecond regime associated with the slow lattice cooling, which arises from the large aspect-ratio and low thermal conductivity of ITO-NRAs. Finally, our results demonstrate that all-optical control of the visible spectrum can be achieved by using heavily doped wide-bandgap semiconductors in their transparent regime with speed faster than that of noble metals.

36 MATERIALS SCIENCE↗

CSEM, Bottomhole Pressure, Salinity, and Flow-Rate Data Collected in Sep. 2020 for Proj. DE-FE0031785

This dataset consists of two directories: first directory named as EM for the controlled source electromagnetic (CSEM) survey data that are zipped per day for September 22, 23, 24, 25, and 27, 2020, and second directory named as "Bottomhole Pressure, Salinity, and Flow-Rate" for the simultaneous collection of bottomhole pressure and salinity and pump flow rate during the CSEM surveys.

CSEM↗

MAGNETICALLY SUSPENDED CANNED ROTOR PUMPS FOR THE INTEGRAL MOLTEN SALT REACTOR

This project developed a molten salt pump design for small modular reactors, concentrated solar, and Gen IV nuclear reactors with a magnetically levitated rotor that can operate at temperatures of up to 700 °C. This eliminates the need for rotating seals and roller element bearings which require maintenance and are prone to failure. The pump design is also more compact than existing molten salt pump designs which require long shafts to thermally isolate the electric motor. The aims of the project are to: 1) design and test the molten salt pump, 2) develop and test a high temperature position sensor needed for magnetic bearing control, and 3) develop and test high temperature coil fabrication methods for electric motor and magnetic bearing fabrication. To develop the high temperature coils, conductor materials were analyzed for oxidation, diffusion, cladding, and resistivity. Of the candidate conductor materials that met the requirements, silver was chosen. The long-term impact of radiation on silver resistivity was analyzed by developing a model of a generic molten salt fast reactor to model the conductor irradiation in worst case scenarios. The analysis showed that increased resistivity due to transmutation of silver decreases exponentially with the reactor reflector thickness. Different electrical insulation materials were tested and the final high temperature coils developed were able to withstand conductor to ground voltages up to 1800 V before insulation breakdown. Magnetic bearings require high-precision high-speed measurements of the rotor position to operate. Current commercial position sensors can only operate up to 550 °C so a novel position sensor was developed that can operate up to 800 °C. These sensors were also designed to measure the position of the metallic rotor through a thin metallic corrosion barrier that protects that coils, insulation, and magnetic cores so that the salt containment barrier does not have any penetrations. The high-temperature sensor was tested and had comparable performance to commercially available inductive position sensors. The sensor design and signal processing has led to several invention disclosures. The magnetically levitated molten salt pump design was completed and analyzed. The chloride salt test loop at Oak Ridge National Laboratory was chosen to test the pump and the pump hydraulics and power were designed for the test loop flow and pressure requirements. Classes of motor designs that do not utilize permanent magnetic were considered for the high-temperature motor. After extensive analysis of their performance, a synchronous reluctance motor was chosen for the pump. The design was refined and analyzed to optimize performance. The magnetic bearings were designed to meet the force and frequency requirements necessary to levitate the rotor and reject disturbances from rotor imbalance, motor forces, and hydraulic forces. Compliant mounts for the position sensors were designed that would not damage the ceramic sensor components and maintain sensor alignment over a wide temperature range. A thermal hydraulic analysis of the molten salt coolant flow used to cool the rotor and stator was performed to ensure that the maximum temperature in the rotor and stator will not exceed 725 °C. The corrosion barrier and casing were designed to maintain the salt fluid boundary by using compliant features to absorb large expansion mismatches due to different coefficients of thermal expansion (CTE). Finally, the salt drain and fill systems were designed along with the pump support structure, integration with the test loop, and thermal insulation and heating. Corrosion barrier fabrication experiments were performed to assess using laser cladding to apply a sub-millimeter corrosion barrier to the surface of a Fe-Co-V magnetic core material. The cladding method showed minimal mixing between materials at their interface and withstood temperature cycling without damage to the cladding. The technology commercialization is focused on the high-temperature position sensors and there has been significant interest from the nuclear industry in utilizing these sensors along with some interest from the aerospace industry. The project also led to a research collaboration with a fusion energy industrial partner to study barriers to scaling the pump design from the kW size to the MW size. This research collaboration will also study methods to create high-temperature coils that have conductor to ground breakdown voltages above 5 kV. The successful development of high-temperature electromagnetic coils and high-temperature position sensors greatly increases the temperature limits for electromagnetic devices that don’t rely on permanent magnets. This includes electric motors, magnetic bearings, linear actuators, rotary position and velocity sensing, actuated valves, and generators to name a few. This will fill a current need in molten salt reactors, concentrated solar, and fusion energy for these critical peripheral devices needed for practical reactor designs that do not currently have commercial solutions.

Hines, J Wesley↗

Femtosecond photocurrents at the FeRh/Pt interface

Femtosecond laser excitations of FeRh/Pt bilayers launch an ultrafast pulse of electric photocurrents in the Pt-layer and subsequently result in the emission of electromagnetic radiation in the THz spectral range. Analysis of the THz emission as a function of the polarization of the femtosecond laser pulse, external magnetic field, sample temperature, and sample orientation shows that the photocurrent can emerge due to vertical spin pumping and photo-induced inverse spin–orbit torque at the FeRh/Pt interface. Additionally, the vertical spin pumping from FeRh into Pt does not depend on the polarization of light and originates from ultrafast laser-induced demagnetization of the ferromagnetic phase of FeRh. The photo-induced inverse spin–orbit torque at the FeRh/Pt interface can be described in terms of a helicity-dependent effect of circularly polarized light on the magnetization of the ferromagnetic FeRh and the subsequent generation of a photocurrent.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Magnetic dynamics with Weyl fermions

Transport of charge and valley (axial) degrees of freedom coupled to order-parameter dynamics in magnetic Weyl semimetals is studied in the framework of nonequilibrium thermodynamics. In addition to the established valley-related transport anomalies that are rooted in band-structure topology, we construct dissipative couplings between the three dynamic constituents of the system driven out of equilibrium by electromagnetic perturbations. We show how the valley degree of freedom mediates an effective coupling between the charge and magnetic sectors of the system, through a combination of the chiral anomaly, on the electric side, and the Onsager-paired valley torque and pumping, on the magnetic side. This work complements previous studies of magnetic Weyl semimetals by a more systematic analysis of collective dissipation. We discuss several concrete examples of the valley-mediated current-driven magnetic instabilities and charge pumping, and extend the theory to the antiferromagnetic case.

36 MATERIALS SCIENCE↗

Stimulated Raman back scattering of extraordinary electromagnetic waves from periodically magnetized nanoparticle lattice

Stimulated Raman back scattering of extraordinary electromagnetic waves from the nanoparticle lattice is investigated in the presence of the static magnetic field. In the context of macroscopic theory, dispersion relation and growth rate of extraordinary mode for different values of static magnetic field and lattice parameters are derived and analyzed. It is found that when the static magnetic field is off, dispersion relation has two branches. These branches are related to the plasmonic and body wave branches of the plane polarized wave. Low frequency branch of the pump wave is not involved in the instability while the other branch is not stable, and the growth rate of Raman back scattered wave has one peak. If the electrons have cyclotron frequency by static magnetic field, dispersion has three branches. These branches are related to the plasmonic and body wave branches of left and right hand circularly polarized waves. In this situation, it is found that low frequency lower branch of the pump wave is stable while other branches are not stable, and the growth rate of Raman back scattered wave has three peaks. Numerical study of growth rate in various cyclotron frequencies shows that the growth rate increases and the instability band width decreases with increasing static magnetic field.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Control of light polarization using optically spin-injected vertical external cavity surface emitting lasers

We fabricated and characterized an optically pumped (100)-oriented InGaAs/GaAsP multiple quantum well Vertical External Cavity Surface Emitting Laser (VECSEL). The structure is designed to allow the integration of a Metal-Tunnel-Junction ferromagnetic spin-injector for future electrical injection. We report here the control at room temperature of the electromagnetic field polarization using optical spin injection in the active medium of the VECSEL. The switching between two highly circular polarization states had been demonstrated using an M-shaped extended cavity in multi-modes lasing. This result witnesses an efficient spin-injection in the active medium of the LASER.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Organic Vacuum Pump Fluids for the Vacuum Pumping of Fusion Power Plants

Vacuum pumps are the heart of the fusion fuel cycle, but most currently proposed pumping technologies are not capable of handling the required flow rates and vacuum pressures. Oil-containing vacuum pumps can readily meet the flow requirements, but vacuum fluids will degrade in fusion-relevant environments due to contact with tritium and exposure to high-energy radiation. Here, in this study, we describe a methodology to screen vacuum fluid candidates and purify these candidate fluids post oxidation, post exposure to deuterium, and post exposure to gamma radiation (<7.5 MGy) to simulate a process in which vacuum fluids can be recovered and regenerated during the fusion fuel cycle. A series of oils, including a highly purified mineral oil, phenyl silicone oil, and a polyphenyl ether, are shown to be suitable candidates for vacuum pumping. Additionally, we describe a simple purification methodology to remove oxidized functionalities and the associated isotopologues induced by contact with deuterium from the candidate vacuum fluids This purification methodology can also be applied to radiological damage with moderate effect. Finally, we demonstrate that the sorbents can be regenerated through electromagnetic microwave digestion.

oxidation↗

Nonlinear fluid simulation study of stimulated Raman and Brillouin scatterings in shock ignition

Here, we developed a new nonlinear fluid laser-plasma-instability code ( FLAME ) using a multi-fluid plasma model combined with full electromagnetic wave equations. The completed one-dimensional version of FLAME was used to study laser-plasma instabilities in shock ignition. The simulations results showed that absolute stimulated Raman scattering (SRS) modes growing near the quarter-critical surface were saturated by Langmuir-wave Decay Instabilities (LDI) and pump depletion. The ion-acoustic waves from LDI acted as seeds of Stimulated Brillouin Scattering, which displayed a bursting pattern and caused strong pump depletion. Re-scattering of SRS at the 1/16th-critical surface was also observed in a high temperature case. These results largely agreed with the corresponding Particle-in-Cell simulations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Ultrahigh-resolution spectroscopy with atomic or molecular dark resonances: Exact steady-state line shapes and asymptotic profiles in the adiabatic pulsed regime

Exact and asymptotic line shape expressions are derived from the semiclassical density matrix representation describing a set of closed three-level {Lambda} atomic or molecular states including decoherences, relaxation rates, and light shifts. An accurate analysis of the exact steady-state dark-resonance profile describing the Autler-Townes doublet, the electromagnetically induced transparency or coherent population trapping resonance, and the Fano-Feshbach line shape leads to the linewidth expression of the two-photon Raman transition and frequency shifts associated to the clock transition. From an adiabatic analysis of the dynamical optical Bloch equations in the weak field limit, a pumping time required to efficiently trap a large number of atoms into a coherent superposition of long-lived states is established. For a highly asymmetrical configuration with different decay channels, a strong two-photon resonance based on a lower states population inversion is established when the driving continuous-wave laser fields are greatly unbalanced. When time separated resonant two-photon pulses are applied in the adiabatic pulsed regime for atomic or molecular clock engineering, where the first pulse is long enough to reach a coherent steady-state preparation and the second pulse is very short to avoid repumping into a new dark state, dark-resonance fringes mixing continuous-wave line shape properties and coherent Ramsey oscillations are created. Those fringes allow interrogation schemes bypassing the power broadening effect. Frequency shifts affecting the central clock fringe computed from asymptotic profiles and related to the Raman decoherence process exhibit nonlinear shapes with the three-level observable used for quantum measurement. We point out that different observables experience different shifts on the lower-state clock transition.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Study of second harmonic generation by high power laser beam in magneto plasma

This paper examines the problem of nonlinear generation of second harmonic of a high power laser pulse propagating in magnetized plasma. The propagation of strong laser beam is proposed in the direction perpendicular to a relatively weak static magnetic field. The laser pulse is taken to be linearly polarized, with the orientation of its electric field that corresponds to an ordinary electromagnetic wave. Besides the standard ponderomotive nonlinearity, the appropriate wave equation also contains the nonlinearity that arises from the relativistic electron jitter velocities. During its propagation, the laser beam gets filamented on account of relativistic and pondermotive nonlinearities present in the plasma. The generated plasma wave gets coupled into the filamentary structures of the pump beam. Due to the expected presence of the beam filamentation, the work has been carried out by considering modified paraxial approximation (i.e., beyond the standard paraxial approximation of a very broad beam). It is found that the power of the plasma wave is significantly affected by the magnetic field strength in the presence of both relativistic and pondermotive nonlinearities. It is investigated that the second harmonic generation is also considerably modified by altering the strength of magnetic field. To see the effect of static magnetic field on the harmonic generation, a key parameter, i.e., the ratio of the cyclotron frequency {omega}{sub c}=eB{sub 0}/mc over the laser frequency {omega}{sub 0} has been used, where c is the velocity of light, m and e are the mass and charge of the electron and B{sub 0} is the externally applied magnetic field.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Theory of stimulated and spontaneous axion scattering.

We present a theory for nonlinear, resonant excitation of dynamical axions by counterpropagating electromagnetic waves in materials that break both 𝒫 and 𝒯 symmetries. We show that dynamical axions can mediate an exponential growth in the amplitude of the lower frequency (Stokes) beam. We also discuss spontaneous generation of a counterpropagating Stokes mode, enabled by resonant amplification of quantum and thermal fluctuations in the presence of a single pump laser. Remarkably, the amplification can be orders of magnitude larger than that obtained via stimulated Brillouin and Raman scattering processes, and can be modulated with the application of external magnetic fields, making stimulated axion scattering promising for optoelectronics applications.

Smith, M.↗

Negative Refraction in Time-Varying Strongly Coupled Plasmonic-Antenna–Epsilon-Near-Zero Systems

Time-varying metasurfaces are emerging as a powerful instrument for the dynamical control of the electromagnetic properties of a propagating wave. Here we demonstrate an efficient time-varying metasurface based on plasmonic nano-antennas strongly coupled to an epsilon-near-zero (ENZ) deeply subwavelength film. The plasmonic resonance of the metal resonators strongly interacts with the optical ENZ modes, providing a Rabi level spitting of ~30%. Optical pumping at frequency ω induces a nonlinear polarization oscillating at 2ω responsible for an efficient generation of a phase conjugate and a negative refracted beam with a conversion efficiency that is more than 4 orders of magnitude greater compared to the bare ENZ film. In this work, the introduction of a strongly coupled plasmonic system therefore provides a simple and effective route towards the implementation of ENZ physics at the nanoscale.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

CSEM, BHP, Salinity, Flow-Rate, Fiber, and Tilt Data Collected in Jan. 2022 for Proj. DE-FE0031785

This dataset consists of four directories: first directory named as EM for the controlled source electromagnetic (CSEM) survey data that are zipped per day for January 18-21, 22, 23, 24, 25, 26, 27, 28, 29, 30, and 31, 2022; second directory named as "Fiber" for the fiber optic slow-strain and microseismic data that are zipped per well; the third file that contains bottomhole pressure (BHP) and salinity and pump flow rate data during the CSEM surveys; and the fourth file that contained tiltmeter data.

CSEM↗

Center for the Study of Plasma Microturbulence

We have discovered a possible "natural fueling" mechanism in tokamak fusion reactors using large scale gyrokinetic turbulence simulation. In the presence of a heat flux dominated tokamak plasma, cold ions naturally pinch radially inward. If cold DT fuel is introduced near the edge using shallow pellet injection, the cold fuel will pinch inward, at the expense of hot helium ash going radially outward. By adjusting the cold DT fuel concentration, the core DT density profiles can be maintained. We have also shown that cold source ions from edge recycling of cold neutrals are pinched radially inward. This mechanism may be important for fully understanding the edge pedestal buildup after an ELM crash. Work includes benchmarking the gyrokinetic turbulence codes in the electromagnetic regime. This includes cyclone base case parameters with an increasing plasma beta. The code comparisons include GEM, GYRO and GENE. There is good linear agreement between the codes using the Cyclone base case, but including electromagnetics and scanning the plasma beta. All the codes have difficulty achieving nonlinear saturation as the kinetic ballooning limit is approached. GEM does not saturate well when beta gets above about 1/2 of the ideal ballooning limit. We find that the lack of saturation is due to the long wavelength k{sub y} modes being nonlinearly pumped to high levels. If the fundamental k{sub y} mode is zeroed out, higher values of beta nonlinearly saturate well. Additionally, there have been studies to better understand CTEM nonlinear saturation and the importance of zonal flows. We have continued our investigation of trapped electron mode (TEM) turbulence. More recently, we have focused on the nonlinear saturation of TEM turbulence. An important feature of TEM is that in many parameter regimes, the zonal flow is unimportant. We find that when zonal flows are unimportant, zonal density is the dominant saturation mechanism. We developed a simple theory that agrees with the simulation and predicts zonal density generation and feedback stabilization of the most unstable mode even in the absence of zonal flow. We are using GEM to simulate NSTX discharges. We have also done verification and validation on DIII-D. Good agreement with GYRO and DIII-D flux levels were reported in the core region.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Reactor Power Level Estimation by Fusing Multi-Modal Sensor Measurements

Estimates of the power level of a nuclear reactor based on measurements from an independent monitoring sensor system can help in the compliance verification of its declared operations. We present a three-level fusion method to estimate the power level of a nuclear reactor using features derived from infrared, electromagnetic, and acoustic sensor measurements collected in proximity to the reactor. Based on a simplified analytical model of the secondary coolant system of the reactor, we identify partial regression functions of the power level in terms of the temperature difference between inlet and outlet of coolant pipes, and the activity levels of four fans and four pumps, which are estimated as features from the sensor measurements. The power level estimator employs a combination of aggregate and complementary fusion steps at three levels to incorporate the multi-modal features in a structure that reflects the secondary cooling system and its partial regression functions. Using the measurements from a test campaign at an operational reactor, we show that this estimator achieves 3.47% or lower root mean square error under 5-fold cross validation. More generally, these results illustrate a progressive reduction in estimation error as additional modalities are appropriately incorporated, and that the fuser outperforms single modality features and their sub-combinations.

Rao, Nageswara↗