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At least 109 records · Page 6

Application of Shear Plate Interferometry to Jet Diffusion Flame Temperature Measurements

The recent ban on the production of bromotrifluoromethane (CF3Br) because of its high stratospheric ozone depletion potential has led to interest in finding alternative agents for fire extinguishing applications. Some of the promising alternatives are fluorinated hydrocarbons. A clear understanding of the effects of CF3Br and alternative chemical suppressants on diffusion flames is therefore necessary in the selection of alternative suppressants for use in normal and microgravity. The flame inhibition effects of halogen compounds have been studied extensively in premixed systems. The effect of addition of halocarbons (carbon-halogen compounds) to diffusion flames has been studied experimentally in coflow configurations and in counterflow gaseous and liquid-pool flames. Halogenated compounds are believed to inhibit combustion by scavenging hydrogen radicals to form the relatively unreactive compound HF, or through a catalytic recombination cycle involving HBr to form H2. Comparisons between halogens show that bromine inhibition is significantly more effective than chlorine or fluorine. Although fluorinated compounds are only slightly more effective inhibitors on a mass basis than nitrogen, they are more effective on a volume basis and are easily stored in liquid form. The objectives of this study are (a) to determine the stability limits of laminar jet diffusion flames with respect to inhibitor concentration in both normal and microgravity, and (b) to investigate the structure of halocarbon-inhibited flames. In the initial phase of this project, visual diagnostics were used to observe the structure and behavior of normal and microgravity flames. The initial observations showed significant changes in the structure of the flames with the addition of halocarbons to the surrounding environment, as discussed below. Furthermore, the study established that the flames are more stable relative to the addition of halocarbons in microgravity than in normal gravity. Visual diagnostics of flames are, however, necessarily limited to detection of radiative emission in the visible range, and offer only qualitative information about the nature of the processes in the flame. In particular, the study sought to understand the structure of the inhibitor-perturbed flames with regard to temperature and species concentration in the outer region of the flame. Whereas thermocouple measurements can be used in ground based studies, their implementation in drop-tower rigs is limited. A possible approach to determine the temperature field around the flame is to use interferometric techniques. The implementation and testing of a shear-plate interferometry technique is described below.

VanDerWege, Brad A.↗

Premixed Flame-Vortex Interactions Imaged in Microgravity

A unique experiment makes it now possible to obtain detailed images in microgravity showing how an individual vortex causes the wrinkling, stretching, area increase, and eventual extinction of a premixed flame. The repeatable, controllable flame-vortex interaction represents the fundamental building block of turbulent combustion concepts. New information is provided that is central to turbulent flame models, including measurements of all components of flame stretch, strain, and vorticity. Simultaneous measurements of all components of these quantities are not possible in fully turbulent flames but are possible in the present axisymmetric, repeatable experiment. Advanced PIV diagnostics have been used at one-g and have been developed for microgravity. Numerical simulations of the interaction are being performed at NRL. It is found that microgravity conditions greatly augment the flame wrinkling process. Flame area and the amplitude of wrinkles at zero-g are typically twice that observed at one-g. It is inferred that turbulent flames in microgravity could have larger surface area and thus propagate significantly faster than those in one-g, which is a potential safety hazard. A new mechanism is identified by PIV images that shows how buoyancy retards flame wrinkling at one-g; buoyancy produces new vorticity (due to baroclinic torques) that oppose the wrinkling and the stretch imposed by the original vortex. Microgravity conditions remove this stabilizing mechanism and the amplitude of flame wrinkling typically is found to double. Microgravity also increases the flame speed by a factor of 1.8 to 2.2. Both methane and propane-air flames were studied at the NASA Lewis drop tower. Results indicate that it is important to add buoyancy to models of turbulent flames to simulate the correct flame wrinkling, stretch and burning velocity.

Driscoll, J. F.↗

Dynamics and Structure of Weakly-Strained Flames In Normal- and Micro-Gravity

Strained laminar flames have been systematically studied, as the understanding of their structure and dynamic behavior is of relevance to turbulent combustion. Most of these studies have been conducted in opposed-jet, stagnation-type flow configurations. Flame studies in stagnation flows also allow for the determination of fundamental flame properties such as laminar flame speeds and extinction states that can be also conveniently modeled in detail. Studies at high strain rates are important in quantifying and understanding the response of vigorously-burning flames under conditions in which the transport time scales become comparable to the chemical time scales. Studies of weakly-strained flames can be of particular interest for all stoichiometries. For example, the laminar flame speeds for any equivalence ratio, phi, can be accurately determined by using the counterflow technique only if measurements are obtained at very low strain rates. Furthermore, near-limit flames can be only stabilized by weak strain rates. Previous studies have shown that weakly-burning flames are particularly sensitive to chain mechanisms, thermal radiation, and unsteadiness. The stabilization and study of weakly-strained flames is complicated by the presence of buoyancy that can render the flames unstable to the point of extinction. Such instabilities are caused either by the induced natural convection or the fact that higher density fluid can find itself on top of a lower density fluid. Thus, the use of microgravity (mu-g) becomes essential in order to provide meaningful insight into this important combustion regime. In view of the foregoing considerations, the main objectives of the program are to: (1) Experimentally determine the laminar flame speed at near-zero strain rates; (2) Experimentally determine the extinction limits of near-limit flames; (3) Experimentally determine the response of near-limit flames to unsteadiness and heat loss; (4) Introduce Digital Particle Image Velocimetry (DPIV) in microgravity; (5) Conduct detailed numerical simulations of the experiments; and (6) Provide physical insight into the underlying physico-chemical mechanisms.

Zhang, Hai↗

Flame Spread Along Free Edges of Thermally Thin Samples in Microgravity

The effects of imposed flow velocity on flame spread along open edges of a thermally thin cellulosic sample in microgravity are studied experimentally and theoretically. In this study, the sample is ignited locally at the middle of the 4 cm wide sample and subsequent flame spread reaches both open edges of the sample. The following flame behaviors are observed in the experiments and predicted by the numerical calculation; in order of increased imposed flow velocity: (1) ignition but subsequent flame spread is not attained, (2) flame spreads upstream (opposed mode) without any downstream flame, and (3) the upstream flame and two separate downstream flames traveling along the two open edges (concurrent mode). Generally, the upstream and downstream edge flame spread rates are faster than the central flame spread rate for an imposed flow velocity of up to 5 cm/s. This is due to greater oxygen supply from the outer free stream to the edge flames than the central flames, For the upstream edge flame, the greater oxygen supply results in a flame spread rate that is nearly independent of, or decreases gradually, with the imposed flow velocity. The spread rate of the downstream edge, however, increases significantly with the imposed flow velocity.

Mell, W. E.↗

Spot Radiative Ignition and Subsequent Three Dimensional Flame Spread Over Thin Cellulose Fuels

Spontaneous radiative ignition and transition to flame spread over thin cellulose fuel samples was studied aboard the USMP-3 STS-75 Space Shuttle mission, and in three test series in the 10 second Japan Microgravity Center (JAMIC). A focused beam from a tungsten/halogen lamp was used to ignite the center of the fuel sample while an external air flow was varied from 0 to 10 cm/s. Non-piloted radiative ignition of the paper was found to occur more easily in microgravity than in normal gravity. Ignition of the sample was achieved under all conditions studied (shuttle cabin air, 21%-50% O2 in JAMIC), with transition to flame spread occurring for all but the lowest oxygen and flow conditions. While radiative ignition in a quiescent atmosphere was achieved, the flame quickly extinguished in air. The ignition delay time was proportional to the gas-phase mixing time, which is estimated using the inverse flow rate. The ignition delay was a much stronger function of flow at lower oxygen concentrations. After ignition, the flame initially spread only upstream, in a fan-shaped pattern. The fan angle increased with increasing external flow and oxygen concentration from zero angle (tunneling flame spread) at the limiting 0.5 cm/s external air flow, to 90 degrees (semicircular flame spread) for external flows at and above 5 cm/s, and higher oxygen concentrations. The fan angle was shown to be directly related to the limiting air flow velocity. Despite the convective heating from the upstream flame, the downstream flame was inhibited due to the 'oxygen shadow' of the upstream flame for the air flow conditions studied. Downstream flame spread rates in air, measured after upstream flame spread was complete and extinguished, were slower than upstream flame spread rates at the same flow. The quench regime for the transition to flame spread was skewed toward the downstream, due to the augmenting role of diffusion for opposed flow flame spread, versus the canceling effect of diffusion at very low cocurrent flows.

Olson, Sandra L.↗

Structure and Early Soot Oxidation Properties of Laminar Diffusion Flames

Soot is an important unsolved problem of combustion science because it is present in most hydrocarbon-fueled flames and current understanding of the reactive and physical properties of soot in flame environments is limited. This lack of understanding affects progress toward developing reliable predictions of flame radiation properties, reliable predictions of flame pollutant emission properties and reliable methods of computational combustion, among others. Motivated by these observations, the present investigation extended past studies of soot formation in this laboratory, to consider soot oxidation in laminar diffusion flames using similar methods. Early work showed that O2 was responsible for soot oxidation in high temperature O2-rich environments. Subsequent work in high temperature flame environments having small O2 concentrations, however, showed that soot oxidation rates substantially exceeded estimates based on the classical O2 oxidation rates of Nagle and Strickland-Constable and suggests that radicals such as O and OH might be strong contributors to soot oxidation for such conditions. Neoh et al. subsequently made observations in premixed flames, supported by later work, that showed that OH was responsible for soot oxidation at these conditions with a very reasonable collision efficiency of 0.13. Subsequent studies in diffusion flames, however, were not in agreement with the premixed flame studies: they agreed that OH played a dominant role in soot oxidation in flames, but found collision efficiencies that varied with flame conditions and were not in good agreement with each other or with Neoh et al. One explanation for these discrepancies is that optical scattering and extinction properties were used to infer soot structure properties for the studies that have not been very successful for representing the optical properties of soot. Whatever the source of the problem, however, these differences among observations of soot oxidation in premixed and diffusion flames clearly must be resolved. Motivated by these findings, the present study undertook measurements of soot and flame properties within the soot oxidation region of some typical laminar diffusion flames and exploited the new measurements to identify soot oxidation mechanisms for these conditions. Present considerations were limited to the early stages of soot oxidation (carbon consumption less than 70%) where reactions at the surface of primary soot particles dominate the process, rather than the later stages when particle porosity and internal particle oxidation become important as discussed by Neoh et al.

El-Leathy, A. M.↗

Large Lewis No. Edge-Flame Instabilities

Edge-flames play an important role in a number of microgravity investigations, and in the general study of flames. Examples include the candle-flame experiments carried out on board both the Space Shuttle and the Mir Space Station; the flame-spread-over-liquid work carried out by H. Ross and W. Sirignano amongst others and lifted turbulent diffusion flames. In all of these configurations a local two-dimensional flame structure can be identified which looks like a flame-sheet with an edge, and these structures exhibit dynamical behavior which characterizes them and distinguishes them from ad hoc 2D flame structures. Edge-flames can exist in both a non-premixed context (edges of diffusion flames) and in a premixed context (edges of deflagrations), but the work reported here deals with the edges of diffusion flames. It is particularly relevant, we believe, to oscillations that have been seen in both the candle-flame context, and the flame-spread-over-liquid context. These oscillations are periodic edge-oscillations (in an appropriate reference frame), sans oscillation of the trailing diffusion flame. It is shown that if the Lewis number of the fuel is sufficiently large (the Lewis number of the oxidizer is taken to be 1), and the Damkohler number is sufficiently small, oscillating-edge solutions can be found. Oscillations are encouraged by an on-edge convective flow and the insertion of a cold probe, discouraged by an off-edge convective flow. In the present work, the nature of these oscillations is examined in more depth, using a variety of numerical strategies.

Buckmaster, J.↗

Stability of Enclosed Laminar Flames Studied in Microgravity

In practical combustion systems, the flame is often anchored at the inlet where the fuel is injected into an air duct. This type of system is found in powerplant combustors, gas turbine combustors, and the jet engine afterburner. Despite its successful use, this configuration is vulnerable to adverse flow conditions that can cause the flame to literally lift off from the inlet or even blowout. Poor flame stability is, of course, unwanted, especially where safety has a high priority. Our understanding of the mechanisms that control flame stability is incomplete in part because the interaction of buoyant (i.e., gravity-induced) convection makes it difficult to interpret normal-gravity results. However, a comparison of normal-gravity and microgravity results can provide a clear indication of the influence of forced and buoyant flows on flame stability. Therefore, a joint microgravity study on the stability of Enclosed Laminar Flames (ELF) was carried out by researchers at The University of Iowa and the NASA Lewis Research Center. The microgravity tests were conducted in the Microgravity Glovebox (MGBX), during the STS-87 space shuttle mission in late 1997, using hardware designed and produced at Lewis. The primary objective of the ELF investigation was to determine the mechanisms controlling the stability of round, laminar, gas-jet diffusion flames in a coflow air duct. The study specifically focused on the effect of buoyancy on the flame characteristics and velocities at the lift-off, reattachment, and blowout of the flame. When the fuel or air velocity is increased to a critical value, the flame base abruptly jumps downstream, and the flame is said to have reached its lift-off condition. Flow conditions are such that the flame cannot be maintained at the burner rim despite the presence of both fuel and oxygen. When the velocity is further increased, the flame eventually extinguishes at its blowout condition. In contrast, if the velocity is reduced, the flame base eventually returns to anchor at the burner rim, at a velocity lower than that of lift-off, indicating a hysteresis effect.

Stocker, Dennis P.↗

The Effect of Reduced Pressure on the Characteristics of Spreading Flames

Flame spread over solid fuels is a canonical problem in fire science, due to its direct implications on material flammability and importance in fire development. In a microgravity environment, such as onboard a spacecraft, flames can behave very differently than on Earth. This is concerning for spaceflight life safety, especially in higher-oxygen environments. Due to the difficulties associated with microgravity testing, low-pressure environments have been proposed as an alternative to approximately replicate the burning behavior of solid fuels observed in reduced gravity conditions because of similar diffusion and heat transfer mechanisms. However, the roles played by gravity and pressure on flame length, standoff distance, and flame spread rate vary with the burning configuration. In concurrent flame spread, the buoyant flow enhances the spread rate by bringing the flame closer to the fuel surface and increasing the heating of the solid fuel. In opposed flame spread, the sample is preheated by the flame ahead of the flame leading edge, which is strongly affected by the surrounding flow field. In this work, we consider flames spreading over thin cotton samples in both downward (opposed) and upward (concurrent) configurations to investigate the effect of pressure (30-100 kPa) on flame characteristics, such as spread rate and standoff distance. A small forced flow is induced upward so that the flames are exposed to a mixed (forced and free) flow. By reducing pressure, flames become less bright, their standoff distance increases, and their spread rates decrease similar to what is observed in low-gravity environments. These results could in help understanding the differences between flames spreading at low pressure and low gravity environments for these similar, yet very different, spreading configurations. They could also provide more information about potential Earth-based flammability testing of materials for spacecraft applications.

fire safety↗

The effect of reduced pressure on the characteristics of spreading flames

Flame spread over solid fuels is a canonical problem in fire science, due to its direct implications on material flammability and importance in fire development. In a microgravity environment, such as onboard a spacecraft, flames can behave very differently than on Earth. This is concerning for spaceflight life safety, especially in higher-oxygen environments. Due to the difficulties associated with microgravity testing, low-pressure environments have been proposed as an alternative to approximately replicate the burning behavior of solid fuels observed in reduced gravity conditions because of similar diffusion and heat transfer mechanisms. However, the roles played by gravity and pressure on flame length, standoff distance, and flame spread rate vary with the burning configuration. In concurrent flame spread, the buoyant flow enhances the spread rate by bringing the flame closer to the fuel surface and increasing the heating of the solid fuel. In opposed flame spread, the sample is preheated by the flame ahead of the flame leading edge, which is strongly affected by the surrounding flow field. In this work, we consider flames spreading over thin cotton samples in both downward (opposed) and upward (concurrent) configurations to investigate the effect of pressure (30-100 kPa) on flame characteristics, such as spread rate and standoff distance. A small forced flow is induced upward so that the flames are exposed to a mixed (forced and free) flow. By reducing pressure, flames become less bright, their standoff distance increases, and their spread rates decrease similar to what is observed in low-gravity environments. These results could in help understanding the differences between flames spreading at low pressure and low gravity environments for these similar, yet very different, spreading configurations. They could also provide more information about potential Earth-based flammability testing of materials for spacecraft applications.

fire safety↗

A Computational and Experimental Study of Coflow Laminar Methane/Air Diffusion Flames: Effects of Fuel Dilution, Inlet Velocity, and Gravity

The influences of fuel dilution, inlet velocity, and gravity on the shape and structure of laminar coflow CH4-air diffusion flames were investigated computationally and experimentally. A series of nitrogen-diluted flames measured in the Structure and Liftoff in Combustion Experiment (SLICE) on board the International Space Station was assessed numerically under microgravity (mu g) and normal gravity (1g) conditions with CH4 mole fraction ranging from 0.4 to 1.0 and average inlet velocity ranging from 23 to 90 cm/s. Computationally, the MC-Smooth vorticity-velocity formulation was employed to describe the reactive gaseous mixture, and soot evolution was modeled by sectional aerosol equations. The governing equations and boundary conditions were discretized on a two-dimensional computational domain by finite differences, and the resulting set of fully coupled, strongly nonlinear equations was solved simultaneously at all points using a damped, modified Newton's method. Experimentally, flame shape and soot temperature were determined by flame emission images recorded by a digital color camera. Very good agreement between computation and measurement was obtained, and the conclusions were as follows. (1) Buoyant and nonbuoyant luminous flame lengths are proportional to the mass flow rate of the fuel mixture; computed and measured nonbuoyant flames are noticeably longer than their 1g counterparts; the effect of fuel dilution on flame shape (i.e., flame length and flame radius) is negligible when the flame shape is normalized by the methane flow rate. (2) Buoyancy-induced reduction of the flame radius through radially inward convection near the flame front is demonstrated. (3) Buoyant and nonbuoyant flame structure is mainly controlled by the fuel mass flow rate, and the effects from fuel dilution and inlet velocity are secondary.

flames↗

An Experimental and Theoretical Study of Radiative Extinction of Diffusion Flames

In a recent paper on 'Observations of candle flames under various atmospheres in microgravity' by Ross et al., it was found that for the same atmosphere, the burning rate per unit wick surface area and the flame temperature were considerably reduced in microgravity as compared with normal gravity. Also, the flame (spherical in microgravity) was much thicker and further removed from the wick. It thus appears that the flame becomes 'weaker' in microgravity due to the absence of buoyancy generated flow which serves to transport the oxidizer to the combustion zone and remove the hot combustion products from it. The buoyant flow, which may be characterized by the strain rate, assists the diffusion process to execute these essential functions for the survival of the flame. Thus, the diffusion flame is 'weak' at very low strain rates and as the strain rate increases the flame is initially 'strengthened' and eventually it may be 'blown out'. The computed flammability boundaries of T'ien show that such a reversal in material flammability occurs at strain rates around 5 sec. At very low or zero strain rates, flame radiation is expected to considerably affect this 'weak' diffusion flame because: (1) the concentration of combustion products which participate in gas radiation is high in the flame zone; and (2) low strain rates provide sufficient residence time for substantial amounts of soot to form which is usually responsible for a major portion of the radiative heat loss. We anticipate that flame radiation will eventually extinguish this flame. Thus, the objective of this project is to perform an experimental and theoretical investigation of radiation-induced extinction of diffusion flames under microgravity conditions. This is important for spacecraft fire safety.

Atreya, Arvind↗

On the Structure and Stabilization Mechanisms of Planar and Cylindrical Premixed Flames

The configurational simplicity of the stationary one-dimensional flames renders them intrinsically attractive for fundamental flame structure studies. The possibility and fidelity of studies of such flames on earth, however, have been severely restricted by the unidirectional nature of the gravity vector. To demonstrate these complications, let us first consider the premixed flame. Here a stationary, one-dimensional flame can be established by using the flat-flame burner. We next consider nonpremixed flames. First it may be noted that in an unbounded gravity-free environment, the only stationary one-dimensional flame is the spherical flame. Indeed, this is a major motivation for the study of microgravity droplet combustion, in which the gas-phase processes can be approximated to be quasi-steady because of the significant disparity between the gas and liquid densities for subcritical combustion. In view of the above considerations, an experimental and theoretical program on cylindrical and spherical premixed and nonpremixed flames in microgravity has been initiated. For premixed flames, we are interested in: (1) assessing the heat loss versus flow divergence as the dominant stabilization mechanism; (2) determining the laminar flame speed by using this configuration; and (3) understanding the development of flamefront instability and the effects of the flame curvature on the burning intensity.

Eng, James A.↗

Candle flames in microgravity

The candle flame in both normal and microgravity is non-propagating. In microgravity, however, the candle flame is also non-convective where (excepting Stefan flow) pure diffusion is the only transport mode. It also shares many characteristics with another classical problem, that of isolated droplet combustion. Given their qualitatively similar flame shapes and the required heat feedback to condensed-phase fuels, the gas-phase flow and temperature fields should be relatively similar for a droplet and a candle in reduced gravity. Unless the droplet diameter is maintained somehow through non-intrusive replenishment of fuel, the quasi-steady burning characteristics of a droplet can be maintained for only a few seconds. In contrast, the candle flame in microgravity may achieve a nearly steady state over a much longer time and is therefore ideal for examining a number of combustion-related phenomena. In this paper, we examine candle flame behavior in both short-duration and long-duration, quiescent, microgravity environments. Interest in this type of flame, especially 'candle flames in weightlessness', is demonstrated by very frequent public inquiries. The question is usually posed as 'will a candle flame burn in zero gravity', or, 'will a candle burn indefinitely (or steadily) in zero gravity in a large volume of quiescent air'. Intuitive speculation suggests to some that, in the absence of buoyancy, the accumulation of products in the vicinity of the flame will cause flame extinction. The classical theory for droplet combustion with its spherically-shaped diffusion flame, however, shows that steady combustion is possible in the absence of buoyancy if the chemical kinetics are fast enough. Previous experimental studies of candle flames in reduced and microgravity environments showed the flame could survive for at least 5 seconds, but did not reach a steady state in the available test time.

Dietrich, D. L.↗

Influence of Buoyant Convection on the Stability of Enclosed Laminar Flames

Enclosed diffusion flames are commonly found in practical combustion systems, such as the power-plant combustor, gas turbine combustor, and jet engine after-burner. In these systems, fuel is injected into a duct with a co-flowing or cross-flowing air stream. In combustors, this flame is anchored at the burner (i.e., fuel jet inlet) unless adverse conditions cause the flame to lift off or blow out. Investigations of burner stability study the lift off, reattachment, and blow out of the flame. There have been numerous studies of flame stability. Relatively few studies have investigated the stability of flames with an oxidizer co-flow, compared with the number of studies on (nearly) free jet diffusion flames. The air flow around the fuel jet can significantly alter the lift off, reattachment and blow out of the jet diffusion flame. In normal gravity, however, the effects of the air flow on flame stability are often complicated by the presence of buoyant convection. A comparison of normal-gravity and microgravity flames can provide clear indication of the influence of forced and buoyant flows on the flame stability. The overall goal of the Enclosed Laminar Flames (ELF) research, described at the following URL site: http://zeta.lerc.nasa.gov/expr/elf.htm, is to improve our understanding of the effects of buoyant convection on the structure and stability of co-flow diffusion flames.

Brooker, John E.↗

A Theory of Oscillating Edge Flames

It has been known for some years that when a near-limit flame spreads over a liquid pool of fuel, the edge of the flame can oscillate relative to a frame moving with the mean speed. Each period of oscillation is characterized by long intervals of modest motion during which the edge gases radiate like those of a diffusion flame, punctuated by bursts of rapid advance during which the edge gases radiate like those in a deflagration. Substantial resources have been brought to bear on this issue within the microgravity program, both experimental and numerical. It is also known that when a near-asphyxiated candle-flame burns at zero gravity, the edge of the (hemispherical) flame can oscillate violently prior to extinction. Thus a web-surfer, turning to the NASA web-site at http://microgravity.msfc.nasa.gov, and following the trail combustion science/experiments/experimental results/candle flame, will find photographs and a description of candle burning experiments carried out on board both the Space-shuttle and the Russian space station Mir. A brief report can also be found in the proceedings of the Fourth Workshop. And recently, in a third microgravity program, the leading edge of the flame supported by injection of ethane through the porous surface of a plate over which air is blown has been found to oscillate when conditions are close to blow-off. A number of important points can be made with respect to these observations: It is the edge itself which oscillates, advancing and retreating, not the diffusion flame that trails behind the edge; oscillations only occur under near limit conditions; in each case the Lewis number of the fuel is significantly larger than 1; and because of the edge curvature, the heat losses from the reacting edge structure are larger than those from the trailing diffusion flame. We propose a general theory for these oscillations, invoking Occam's 'Law of Parsimony' in an expanded form, to wit: The same mechanism is responsible for the oscillations in all three experiments; and no new mechanism is invoked (Occam's original 'Razor'). Such a strategy eliminates Marangoni effects as the source, for these are absent in the second and third experiments. And it eliminates arguments that point to numerically predicted gas eddies as the source, a new mechanism, unelucidated. Indeed, we hypothesize that the essential driving mechanism for the instability is a combination of large Lewis number and heat losses from the reacting structure near the flame edge. Instabilities driven by these mechanisms are commonplace in 1D configurations. Chemical reactor theory, for example, leads to system responses which mimic the response of the candle flame - steady flame, oscillations, extinction. In a combustion context, oscillating instabilities were first reported for diffusion flames in a theoretical study by Kirkby and Schmitz, and here also the instabilities are associated with near-extinction conditions, large Lewis numbers, and heat losses. And deflagrations will oscillate if the Lewis number is large enough, oscillations that are exacerbated when heat losses are present, whether global or to a surface.

Buckmaster, J.↗

Quantitative Studies on the Propagation and Extinction of Near-Limit Premixed Flames under Normal- and Micro-gravity

Strained laminar flames have been systematically studied, as the understanding of their structure and dynamic behavior is of relevance to turbulent combustion.. Most of these studies have been conducted in opposed-jet, stagnation-type flow configurations. Studies at high strain rates are important in quantifying and understanding the response of vigorously burning flames and determine extinction states. Studies of weakly strained flames can be of particular interest for all stoichiometries. For example, the laminar flame speeds, S(sup o)(sub u), can be accurately determined by using the counterflow technique only if measurements are obtained at very low strain rates. Furthermore, near-limit flames are stabilized by weak strain rates. Previous studies have shown that near-limit flames are particularly sensitive to chain mechanisms, thermal radiation, and unsteadiness. The stabilization and study of weakly strained flames is complicated by the presence of buoyancy that can render the flames unstable to the point of extinction. Thus, the use of microgravity (mu-g) becomes essential in order to provide meaningful insight into this important combustion regime. In our past studies the laminar flame speeds and extinction strain rates were directly measured at ultra-low strain rates. The laminar flame speeds were measured by having a positively strained planar flame undergoing a transition to a negatively strained Bunsen flame and by measuring the propagation speed during that transition. The extinction strain rates of near-limit flames were measured in mu-g. Results obtained for CH4/air and C3H8/air mixtures are in agreement with those obtained by Maruta et al.

Egolfopoulos, F. N.↗

Three-Dimensional Upward Flame Spreading in Partial-Gravity Buoyant Flows

Reduced-gravity environments have been used to establish low-speed, purely forced flows for both opposed- and concurrent-flow flame spread studies. Altenkirch's group obtained spacebased experimental results and developed unsteady, two-dimensional numerical simulations of opposed-flow flame spread including gas-phase radiation, primarily away from the flammability limit for thin fuels, but including observations of thick fuel quenching in quiescent environments. T'ien's group contributed some early flame spreading results for thin fuels both in opposed flow and concurrent flow regimes, with more focus on near-limit conditions. T'ien's group also developed two- and three-dimensional numerical simulations of concurrent-flow flame spread incorporating gas-phase radiative models, including predictions of a radiatively-induced quenching limit reached in very low-speed air flows. Radiative quenching has been subsequently observed in other studies of combustion in very low-speed flows including other flame spread investigations, droplet combustion and homogeneous diffusion flames, and is the subject of several contemporary studies reported in this workshop. Using NASA aircraft flying partial-gravity "parabolic" trajectories, flame spreading in purely buoyant, opposed-flow (downward burning) has been studied. These results indicated increases in flame spread rates and enhanced flammability (lower limiting atmospheric oxygen content) as gravity levels were reduced from normal Earth gravity, and were consistent with earlier data obtained by Altenkirch using a centrifuge. In this work, experimental results and a three-dimensional numerical simulation of upward flame spreading in variable partial-gravity environments were obtained including some effects of reduced pressure and variable sample width. The simulation provides physical insight for interpreting the experimental results and shows the intrinsic 3-D nature of buoyant, upward flame spreading. This study is intended to link the evolving understanding of flame spreading in purely-forced flows to the purely-buoyant flow environment, particularly in the concurrent flow regime; provide additional insight into the existence of steady flame spread in concurrent flows; and stimulate direct comparisons between opposed- and concurrent-flow flame spread. Additionally, this effort is intended to provide direct practical understanding applicable to fire protection planning for the habitable facilities in partial gravity environments of anticipated Lunar and Martian explorations.

Sacksteder, Kurt R.↗