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DOE OSTI2024

MEASUREMENT OF THE NEUTRON FLUENCE-RATES IN THE ADVANCED TEST REACTOR

The axial neutron fluence-rate distribution at the Advanced Test Reactor (ATR) is determined using a combination of pure nickel and cobalt-aluminium alloy dosimeter wires. Most irradiation programs at ATR need to know the fast neutron fluence-rate surrounding their experiment to correlate post-irradiation examination results with neutron dose. The activated dosimeter wires, which extend beyond the full fuelled region of the reactor core, are highly radioactive following the full cycle in ATR and must therefore be measured in the ATR canal. The system that is employed for these measurements is mechanical scanning mechanism is used to scan the activated wires across the face of a columnated shield and a NaI detector. This detector is not sufficiently calibrated to provide absolute activity measurements, therefore, the count-rate is recorded and normalized to the highest activity for that wire. Then, an approximately 3-mm long portion of the wire is removed from the highest activity region in the wire. The wires are then transferred, and an absolute activity measurement is made using a calibrated ionization chamber. These measurements are combined with corrections for decay, neutron energy spectrum, burnup, dosimeter composition, reactor power fluctuations, and reactor outages to determine the average axial neutron fluence-rate at various locations within ATR during the cycle.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

DOE OSTI2023

Development of a compact fast-neutron spectrometer for nuclear emergency response applications

We have developed a Compact Fast Neutron Spectrometer (CFNS) for passive assay of special nuclear material (SNM) through the observation of fast neutrons. The CFNS consists of eight organic glass scintillators (OGS) coupled to silicon photomultipliers and a waveform digitizer, which are integrated within a human-portable box. The CFNS determines the neutron energy profile by spectrum unfolding using the Maximum-Likelihood Expectation Maximization method. The detector acquisition system was optimized to have a dynamic range of up to 10 MeV neutron energy. Bulk special nuclear material (SNM) measurements from the National Criticality Experiments Research Center were analyzed for SNM validation/examination. Additionally, the results show that the CFNS can be used to distinguish between fission and (α, n) neutron emitters, regardless of intervening material type (Cu and polyethylene) and thickness, by taking the ratio of neutron counts at different regions in the unfolded energy spectrum. Additionally, by fitting an exponential curve to the unfolded energy spectrum of PuO 2 and Pu neutron emitters, the CFNS showed the ability of distinguishing between pure Pu oxide, pure Pu metal and mixed oxide-metal configurations.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2020

A search for optical and near-infrared counterparts of the compact binary merger GW190814

Here, we report on our observing campaign of the compact binary merger GW190814, detected by the Advanced LIGO and Advanced Virgo detectors on 2019 August 14. This signal has the best localization of any observed gravitational wave (GW) source, with a 90 per cent probability area of 18.5 deg 2 , and an estimated distance of ≈240 Mpc. We obtained wide-field observations with the Deca-Degree Optical Transient Imager (DDOTI) covering 88 per cent of the probability area down to a limiting magnitude of w = 19.9 AB. Nearby galaxies within the high probability region were targeted with the Lowell Discovery Telescope (LDT), whereas promising candidate counterparts were characterized through multicolour photometry with the Reionization and Transients InfraRed (RATIR) and spectroscopy with the Gran Telescopio de Canarias (GTC). We use our optical and near-infrared limits in conjunction with the upper limits obtained by the community to constrain the possible electromagnetic counterparts associated with the merger. A gamma-ray burst seen along its jet’s axis is disfavoured by the multiwavelength data set, whereas the presence of a burst seen at larger viewing angles is not well constrained. Although our observations are not sensitive to a kilonova similar to AT2017gfo, we can rule out high-mass (>0.1 M ⊙ ) fast-moving (mean velocity ≥0.3c) wind ejecta for a possible kilonova associated with this merger.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2024

Optically multiplexed neutron time-of-flight technique for inertial confinement fusion

Neutron time-of-flight (nTOF) detectors are crucial in diagnosing the performance of inertial confinement fusion (ICF) experiments, which implode targets of deuterium–tritium fuel to achieve thermonuclear conditions. These detectors utilize the fusion neutron energy spectrum to extract key measurements, including the hotspot ion temperature and fuel areal density. Previous work [Danly et al., Rev. Sci. Instrum. 94, 043502 (2023)] has demonstrated adding 1D spatial resolution to an nTOF-like detector using a neutron aperture and streak camera to measure the ion temperature profile of an ICF implosion. By contrast, the study presented herein explores modifying the 1D detector to use a fast photomultiplier tube (PMT) to validate the design of a 2D spatially resolved instrument based on reconstruction from 1D profiles. The modification would collect time-of-flight traces from separate scintillators in an imaging array with one PMT using optical fibers of varying lengths to time-multiplex the signals. This technique has been demonstrated in ride-along experiments on the OMEGA laser with 20 fiber-coupled scintillator channels connected to a Photek PMT210. Results provide constraints on the fiber lengths and PMT gating requirements to promote pulse fidelity throughout all channels. Calibration of the detector to fixed nTOFs can provide a preliminary estimate of the instrument response function (IRF), although measurement of the IRF is currently under way. These results suggest that nTOF signals can potentially be time-multiplexed with fibers so long as the design is strategic to mitigate signal-to-noise reduction, modal dispersion, and charge build-up in the PMT, which has implications beyond ion temperature imaging.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2023

Measurement of the 238 U( n,f ) prompt fission neutron spectrum from 10 keV to 10 MeV induced by neutrons with 1.5–20 MeV energy

With the recent emergence of fast nuclear reactors, there has been a corresponding increasing interest in 238 U-related nuclear data. However, while existing literature data span much of the energy ranges of interest for the prompt fission neutron spectrum (PFNS) for neutron-induced fission of 238U, most literature data sets are highly correlated, and thus new, independent measurements of this quantity are needed. In this work, we report the results of a new measurement of the 238 U PFNS at the Los Alamos Neutron Science Center for incident neutron energies from 1.5–20.0 MeV, and outgoing neutron energies of 0.01–10.0 MeV. With some notable exceptions, the present results generally agree with existing literature data, especially with regard to features relating to multichance fission and pre-equilibrium features in the PFNS, thus adding confidence to existing nuclear data evaluations and filling in gaps of knowledge at previously unmeasured incident neutron energies. This result is the third in a series of PFNS measurements by the Chi-Nu collaboration now spanning all three major actinides, 239 Pu, 235 U, and 238 U. Thus, for the first time, we report reliable experimental PFNS ratios and average PFNS energy comparisons for measurements of all three of these isotopes including accurate correlations between the different, but correlated experiments.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2026

Task Sharing of Proton Incorporation in Vertically Aligned Nanocomposite Triple Conductors: Growth, Structure, and Surface Exchange Kinetics

As protonic ceramic electrolysis cells emerge for efficient H 2 production, there is a need to develop air electrode materials enabling fast, durable steam splitting and proton incorporation. Single-phase triple conductors may fail to satisfy the myriad performance/stability requirements, and their critical charge-carriers (holes, oxygen vacancies, and protons) are in competition, limiting their concentrations. Instead, we propose task-sharing, vertically aligned nanocomposites (VANs), comprising a proton conductor (BaZr 0.9 Y 0.1 O 3-δ ) and a redox-active mixed ionic electronic conductor (Ce 0.9 Pr 0.1 O 2-δ ), that may enable rapid proton surface exchange at the solid–gas interface and transport along the solid–solid heterointerfaces. We grew VANs by pulsed laser deposition and investigated the interplay between their processing conditions, structure, and proton and oxygen surface exchange kinetics. We varied the substrate temperature, laser repetition rate, laser fluence, and processing oxygen pressure. The crystallinity and phases were characterized by grazing-incidence X-ray diffraction, and the strain and structural order as a function of depth were evaluated by angle-dependent synchrotron X-ray pair distribution function analysis. To evaluate the potential for interdiffusion, the formation energies of substitutional defects were simulated with density functional theory. Corresponding structural analysis and elemental mapping were performed by scanning/transmission electron microscopy, energy-dispersive X-ray spectroscopy, and electron energy-loss spectroscopy, indicating distinct nanoscale compositional regions with a hierarchical structure embedded in individual VANs columns and minimal interdiffusion across a bilayer film. Proton and oxygen surface exchange coefficients (k H , k O ) and polarization resistances were evaluated by electrical and optical relaxations and impedance spectroscopy of VAN-incorporated protonic ceramic electrochemical cells, respectively, at 400–500 °C, demonstrating values comparable to some of the best-known triple and mixed conductors.

36 MATERIALS SCIENCE↗

DOE OSTI2024

Fast ion studies in the extended high-performance high β P plasma on EAST

Comprehending and optimizing fast ion behaviors is critical for the enhancement of performance in Experimental Advanced Superconducting Tokamak (EAST). This study explores the potential benefits of several factors that can improve the fast ion confinement. First, experiments show the change in the direction of the NBI2 from counter-I p to co-I p leads to a significant reduction in fast ion losses. TRANSP/NUBEAM simulation and tomography results based on fast-ion D-alpha measurements reveal that after the neutral beam injection (NBI) upgrade, the beam ion prompt loss is reduced by approximately 50%. Second, the upgraded ion cyclotron resonant frequency (ICRF) antenna at the N-port features twice the coupling resistance of the original antennas at EAST. This improved ICRF power coupling has enhanced the synergistic heating effect of NBI + ICRF, where the ICRF wave field accelerates beam ions at the harmonics. Experiments demonstrate that NBI + ICRF synergistic not only enhances plasma neutron yield and β P , but also accelerates beam ions to hundreds of keV. Further, the electron density and the neutral beam voltage have been optimized to reduce the fast ion slowing-down time and beam ion losses. Experimental and simulation results indicate that increasing the electron density reduces beam ion losses and enhances the bootstrap current fraction. While higher beam voltage results in a slight decrease in beam power absorption, it can increase the fraction of bootstrap current. With the understanding of these optimization of fast ion confinement, experiments have demonstrated fully non-inductive operation at high density (n e /n G ∼ 0.67, β P ∼ 3.1, β N ∼ 2.1, H 98,y2 ∼ 1.2) even without the support of co-I p beam NBI2. This investigation presents a potential regime to enhance fast ion confinement and extend performance in the high β P plasma for future experiments.

EAST tokamak↗