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At least 109 records · Page 6

Tethered balloon-borne profile measurements of atmospheric properties in the cloudy atmospheric boundary layer over the Arctic sea ice during MOSAiC: Overview and first results

The tethered balloon-borne measurement system BELUGA (Balloon-bornE moduLar Utility for profilinG the lower Atmosphere) was deployed over the Arctic sea ice for 4 weeks in summer 2020 as part of the Multidisciplinary drifting Observatory for the Study of Arctic Climate expedition. Using BELUGA, vertical profiles of dynamic, thermodynamic, aerosol particle, cloud, radiation, and turbulence properties were measured from the ground up to a height of 1,500 m. BELUGA was operated during an anomalously warm period with frequent liquid water clouds and variable sea ice conditions. Three case studies of liquid water phase, single-layer clouds observed on 3 days (July 13, 23, and 24, 2020) are discussed to show the potential of the collected data set to comprehensively investigate cloud properties determining cloud evolution in the inner Arctic over sea ice. Simulated back-trajectories show that the observed clouds have evolved within 3 different air masses (“aged Arctic,” “advected over sea ice,” and “advected over open ocean”), which left distinct fingerprints in the cloud properties. Strong cloud top radiative cooling rates agree with simulated results of previous studies. The weak warming at cloud base is mostly driven by the vertical temperature profile between the surface and cloud base. In-cloud turbulence induced by the cloud top cooling was similar in strength compared to former studies. From the extent of the mixing layer, it is speculated that the overall cloud cooling is stronger and thus faster in the warm oceanic air mass. Larger aerosol particle number concentrations and larger sizes were observed in the air mass advected over the sea ice and in the air mass advected over the open ocean.

Arctic↗

Normalized vertical ice mass flux profiles from vertically pointing 8-mm-wavelength Doppler radar

During the FIRE 2 (First International Satellite Cloud Climatology Project Regional Experiment) project, NOAA's Wave Propagation Laboratory (WPL) operated its 8-mm wavelength Doppler radar extensively in the vertically pointing mode. This allowed for the calculation of a number of important cirrus cloud parameters, including cloud boundary statistics, cloud particle characteristic sizes and concentrations, and ice mass content (imc). The flux of imc, or, alternatively, ice mass flux (imf), is also an important parameter of a cirrus cloud system. Ice mass flux is important in the vertical redistribution of water substance and thus, in part, determines the cloud evolution. It is important for the development of cloud parameterizations to be able to define the essential physical characteristics of large populations of clouds in the simplest possible way. One method would be to normalize profiles of observed cloud properties, such as those mentioned above, in ways similar to those used in the convective boundary layer. The height then scales from 0.0 at cloud base to 1.0 at cloud top, and the measured cloud parameter scales by its maximum value so that all normalized profiles have 1.0 as their maximum value. The goal is that there will be a 'universal' shape to profiles of the normalized data. This idea was applied to estimates of imf calculated from data obtained by the WPL cloud radar during FIRE II. Other quantities such as median particle diameter, concentration, and ice mass content can also be estimated with this radar, and we expect to also examine normalized profiles of these quantities in time for the 1993 FIRE II meeting.

Orr, Brad W.↗

Possible fossil H2O liquid-ice interfaces in the Martian crust

The extensive chaotic and fretted terrains in the equatorial regions of Mars are explained on the basis of the vertical distribution of H2O liquid and ice which once existed in the crust. This account assumes that below the permafrost containing water ice, there was a second zone in which liquid water resided for at least a time. Diagenetic alteration and cementation characterized the material in the subpermafrost zone; above, pristine fragmented material with various ice concentrations was found. Later, the ice-laden zone was stripped away by a number of erosional processes, exposing the former ice-liquid water interface.

Soderblom, L. A.↗

Radar-Based Bayesian Estimation of Ice Crystal Growth Parameters within a Microphysical Model

The potential for polarimetric Doppler radar measurements to improve predictions of ice microphysical processes within an idealized model–observational framework is examined. In an effort to more rigorously constrain ice growth processes (e.g., vapor deposition) with observations of natural clouds, a novel framework is developed to compare simulated and observed radar measurements, coupling a bulk adaptive-habit model of vapor growth to a polarimetric radar forward model. Bayesian inference on key microphysical model parameters is then used, via a Markov chain Monte Carlo sampler, to estimate the probability distribution of the model parameters. The statistical formalism of this method allows for robust estimates of the optimal parameter values, along with (non-Gaussian) estimates of their uncertainty. To demonstrate this framework, observations from Department of Energy radars in the Arctic during a case of pristine ice precipitation are used to constrain vapor deposition parameters in the adaptive habit model. The resulting parameter probability distributions provide physically plausible changes in ice particle density and aspect ratio during growth. A lack of direct constraint on the number concentration produces a range of possible mean particle sizes, with the mean size inversely correlated to number concentration. Consistency is found between the estimated inherent growth ratio and independent laboratory measurements, increasing confidence in the parameter PDFs and demonstrating the effectiveness of the radar measurements in constraining the parameters. Furthermore, the combined Doppler and polarimetric observations produce the highest-confidence estimates of the parameter PDFs, with the Doppler measurements providing a stronger constraint for this case.

54 ENVIRONMENTAL SCIENCES↗

Biological enhancement of cloud droplet concentrations observed off East Antarctica

Abstract The impact that biogenic emissions have on aerosol-cloud interactions across the Southern Ocean is poorly quantified. Here we use satellite and ship observations during austral summer to study these interactions. We present observational evidence that biogenic aerosols increase cloud condensation nuclei and cloud droplet number concentrations over the Southern Ocean off East Antarctica, coinciding with very low concentrations of ice-nucleating particles and higher occurrences of supercooled liquid-containing low-level clouds.

Mallet, Marc D.↗

A Numerical Evaluation of Icing Effects on a Natural Laminar Flow Airfoil

As a part of CFD code validation efforts within the Icing Branch of NASA Glenn Research Center, computations were performed for natural laminar flow (NLF) airfoil, NLF-0414. with 6 and 22.5 minute ice accretions. Both 3-D ice castings and 2-D machine-generated ice shapes were used in wind tunnel tests to study the effects of natural ice is well as simulated ice. They were mounted in the test section of the Low Turbulence Pressure Tunnel (LTPT) at NASA Langley that the 2-dimensionality of the flow can be maintained. Aerodynamic properties predicted by computations were compared to data obtained through the experiment by the authors at the LTPT. Computations were performed only in 2-D and in the case of 3-D ice, the digitized ice shape obtained at one spanwise location was used. The comparisons were mainly concentrated on the lift characteristics over Reynolds numbers ranging from 3 to 10 million and Mach numbers ranging from 0.12 to 0.29. WIND code computations indicated that the predicted stall angles were in agreement with experiment within one or two degrees. The maximum lift values obtained by computations were in good agreement with those of the experiment for the 6 minute ice shapes and the minute 3-D ice, but were somewhat lower in the case of the 22.5 minute 2-D ice. In general, the Reynolds number variation did not cause much change in the lift values while the variation of Mach number showed more change in the lift. The Spalart-Allmaras (S-A) turbulence model was the best performing model for the airfoil with the 22.5 minute ice and the Shear Stress Turbulence (SST) turbulence model was the best for the airfoil with the 6 minute ice and also for the clean airfoil. The pressure distribution on the surface of the iced airfoil showed good agreement for the 6 minute ice. However, relatively poor agreement of the pressure distribution on the upper surface aft of the leading edge horn for the 22.5 minute ice suggests that improvements are needed in the grid or turbulence models.

Chung, James J.↗

Arctic Impact Identification with Less Data Using Variable Relationships: An Exploratory Express LDRD project.

Regional impacts from sea ice loss can be challenging to separate from internal climate variability, potentially requiring thousands of ensemble members. East Asian wintertime cooling has been linked to sea ice loss from present day conditions in the Polar Amplification Model Intercomparison Project with these large ensemble counts. This cooling is theorized to arise from a strengthened Siberian High and East Asian Jet response. The strengthened Siberian High can be detected with one fifth the ensemble members needed for the East Asian wintertime cooling in a single model. We thus hypothesize that leveraging relationships between multiple variables in a conditional pathways-based approach would reduce the number of required ensemble members to conclusively attribute East Asian wintertime cooling to future sea ice concentrations. In all analyzed cases, confidence was increased when evaluating sea ice loss’s responsibility for the joint effects of East Asian cooling, East Asian Jet strengthening, and Siberian High strengthening over just East Asian cooling. However, we were not able to confidently attribute future East Asian wintertime cooling to sea ice loss in a single model. We found that significant intra-ensemble variability within single Earth System Models (ESMs) produced highly uncertain forcing response models upon which attribution results were undermined. We were able to show that ensemble mean seasonally averaged metrics from multiple ESMs greatly improved the accuracy of the forcing response linear models and exposed the necessity of all three steps in the pathway (sea ice area, Siberian High pressure, and East Asian Jet speed) for accurate prediction of East Asian wintertime cooling. Although all three steps were necessary, East Asian wintertime cooling possesses a large dependence on the Siberian High pressure, which weakens the confidence associated with overall strong joint-attribution comparing present day and future scenarios. We believe transitioning the pathway nodes to relative changes between the Siberian High and Aleutian Low as well as between the midlatitude westerlies and subtropical jet in the East Asianj Jet region may be able to produce significant attribution more fully dependent upon all three steps. Ultimately, this research demonstrates the simple extensibility of conditional pathways-based attribution to sea ice loss forcing on the Earth system.

54 ENVIRONMENTAL SCIENCES↗

Radar-Based Bayesian Estimation of Ice Crystal Growth Parameters within a Microphysical Model

The potential for polarimetric Doppler radar measurements to improve predictions of ice microphysical processes within an idealized model–observational framework is examined. In an effort to more rigorously constrain ice growth processes (e.g., vapor deposition) with observations of natural clouds, a novel framework is developed to compare simulated and observed radar measurements, coupling a bulk adaptive-habit model of vapor growth to a polarimetric radar forward model. Bayesian inference on key microphysical model parameters is then used, via a Markov chain Monte Carlo sampler, to estimate the probability distribution of the model parameters. The statistical formalism of this method allows for robust estimates of the optimal parameter values, along with (non-Gaussian) estimates of their uncertainty. To demonstrate this framework, observations from Department of Energy radars in the Arctic during a case of pristine ice precipitation are used to constrain vapor deposition parameters in the adaptive habit model. The resulting parameter probability distributions provide physically plausible changes in ice particle density and aspect ratio during growth. A lack of direct constraint on the number concentration produces a range of possible mean particle sizes, with the mean size inversely correlated to number concentration. Consistency is found between the estimated inherent growth ratio and independent laboratory measurements, increasing confidence in the parameter PDFs and demonstrating the effectiveness of the radar measurements in constraining the parameters. The combined Doppler and polarimetric observations produce the highest-confidence estimates of the parameter PDFs, with the Doppler measurements providing a stronger constraint for this case.

Robert S. Schrom↗

Mesoscale simulations of the November 25-26 and December 5-6 cirrus cases using the RAMS model

The Regional Atmospheric Modeling System (RAMS), developed at Colorado State University, was used during the First ISCCP (International Satellite Cloud Climatology Project) Regional Experiment (FIRE) 2 (13 Nov. through 6 Dec. 1991) to provide real time forecasts of cirrus clouds. Forecasts were run once a day, initializing with the 0000 UTC dataset provided by NOAA (Forecast Systems Laboratory (FSL) Mesoscale Analysis and Prediction System (MAPS)). In order to obtain better agreement with observations, a second set of simulations were done for the FIRE 2 cases that occurred on 25-26 Nov. and 5-6 Dec. In this set of simulations, a more complex radiation scheme was used, the Chen/Cotton radiation scheme, along with the nucleation of ice occurring at ice supersaturations as opposed to nucleation occurring at water supersaturations that was done in the actual forecast version. The runs using these more complex schemes took longer wall clock time (7-9 hours for the actual forecasts as compared to 12-14 hrs for the runs using the more complex schemes) however, the final results of the simulations were definitely improved upon. Comparisons between these two sets of simulations are given. Now underway are simulations of these cases using a closed analytical solution for the auto-conversion of ice from a pristine ice class (sizes less than about 50 microns in effective diameter) to a snow class (effective diameters on the order of several hundred microns). This solution is employed along with a new scheme for the nucleation of ice crystals due to Meyers et al and Demott et al. The scheme is derived assuming complete gamma distributions for both the pristine and snow classes. The time rate of change of the number concentration and mass mixing-ratio of each distribution is found by calculating either the flux of crystals that grow beyond a certain critical diameter by vapor deposition in an ice supersaturated regime or by calculating the flux of crystals that evaporate to sizes below that same critical effective diameter.

Harrington, J. L.↗

Cloud Processing of Aerosol during SAIL Field Campaign Report

Globally, on average, the release rate of aerosols from clouds is estimated to be about 6,000 Tg/yr and an aerosol particle is estimated to experience about three cloud cycles. Cloud processing of aerosol produces aerosols that have dramatically different physicochemical properties compared to their original form. Cloud processing may transform particles to efficient cloud condensation nuclei (CCN) or ice nucleating particles (INP) that can further participate in cloud formation. We investigated cloud processing of aerosol during the U.S. Department of Energy (DOE)’s Atmospheric Radiation Measurement (ARM) Surface Atmosphere Integrated Field Laboratory (SAIL) field campaign using multi-modal offline analysis techniques available at DOE’s Environmental Molecular Sciences Laboratory (EMSL). The main scientific aim of this project was to understand the processes that transform aerosols (chemically, and physically), and influence aerosol-cloud interactions. Aerosol particles undergo significant modifications due to warm (cloud droplets) and cold cloud (ice crystals) processing. Cloud processing of aerosol has important effects on the atmospheric aerosol number and mass concentration, size distribution, phase separation, and chemical composition.

54 ENVIRONMENTAL SCIENCES↗

Aerosol-Ice Formation Closure Pilot Study (AEROICSTUDY) Field Campaign Report

The aerosol-ice formation closure pilot study (AEROICESTUDY) was a field campaign conducted at the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility at the Southern Great Plains (SGP) observatory from October 7 to 28, 2019. The purpose of this campaign was to test a field observational approach for conducting an aerosol-ice formation closure study. In other words, the goal was to predict the number of ice nucleating particles (INPs) from the measurements of physical and chemical aerosol properties and compare those to measured INP number concentrations. This project was motivated by the fact that the aerosol community has widely conducted aerosol radiative closure, aerosol-cloud condensation nuclei (CCN), and CCN-droplet closure studies to test the physical models and parameterizations that cloud-resolving and climate models rely on to perform reliable simulations of the Earth system and energy budget. However, very few closure studies related to INPs have been conducted, and to our knowledge, none using robust, size-resolved, ambient aerosol composition measurements as model inputs.

aerosol-ice formation↗

Aerosol-Ice Formation Closure Pilot Study (AEROICESTUDY) Field Campaign Report

The aerosol-ice formation closure pilot study (AEROICESTUDY) was a field campaign conducted at the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility at the Southern Great Plains (SGP) observatory from October 7 to 28, 2019. The purpose of this campaign was to test a field observational approach for conducting an aerosol-ice formation closure study. In other words, the goal was to predict the number of ice nucleating particles (INPs) from the measurements of physical and chemical aerosol properties and compare those to measured INP number concentrations. This project was motivated by the fact that the aerosol community has widely conducted aerosol radiative closure, aerosol-cloud condensation nuclei (CCN), and CCN-droplet closure studies to test the physical models and parameterizations that cloud-resolving and climate models rely on to perform reliable simulations of the Earth system and energy budget. However, very few closure studies related to INPs have been conducted, and to our knowledge, none using robust, size-resolved, ambient aerosol composition measurements as model inputs

AEROICESTUDY↗

Evaluating the Performance of Single and Double Moment Microphysics Schemes During a Synoptic-Scale Snowfall Event

Increases in computing resources have allowed for the utilization of high-resolution weather forecast models capable of resolving cloud microphysical and precipitation processes among varying numbers of hydrometeor categories. Several microphysics schemes are currently available within the Weather Research and Forecasting (WRF) model, ranging from single-moment predictions of precipitation content to double-moment predictions that include a prediction of particle number concentrations. Each scheme incorporates several assumptions related to the size distribution, shape, and fall speed relationships of ice crystals in order to simulate cold-cloud processes and resulting precipitation. Field campaign data offer a means of evaluating the assumptions present within each scheme. The Canadian CloudSat/CALIPSO Validation Project (C3VP) represented collaboration among the CloudSat, CALIPSO, and NASA Global Precipitation Measurement mission communities, to observe cold season precipitation processes relevant to forecast model evaluation and the eventual development of satellite retrievals of cloud properties and precipitation rates. During the C3VP campaign, widespread snowfall occurred on 22 January 2007, sampled by aircraft and surface instrumentation that provided particle size distributions, ice water content, and fall speed estimations along with traditional surface measurements of temperature and precipitation. In this study, four single-moment and two double-moment microphysics schemes were utilized to generate hypothetical WRF forecasts of the event, with C3VP data used in evaluation of their varying assumptions. Schemes that incorporate flexibility in size distribution parameters and density assumptions are shown to be preferable to fixed constants, and that a double-moment representation of the snow category may be beneficial when representing the effects of aggregation. These results may guide forecast centers in optimal configurations of their forecast models for winter weather and identify best practices present within these various schemes.

Molthan, Andrew L.↗

Observations of Fog-Aerosol Interactions Over Central Greenland

Supercooled fogs can have an important radiative impact at the surface of the Greenland Ice Sheet, but they are difficult to detect and our understanding of the factors that control their lifetime and radiative properties is limited by a lack of observations. This study demonstrates that spectrally resolved measurements of downwelling longwave radiation can be used to generate retrievals of fog microphysical properties (phase and particle effective radius) when the fog visible optical depth is greater than ~0.25. For 12 cases of fog under otherwise clear skies between June and September 2019 at Summit Station in central Greenland, nine cases were mixed-phase. The mean ice particle (optically-equivalent sphere) effective radius was 24.0 ± 7.8 µm, and the mean liquid droplet effective radius was 14.0 ± 2.7 µm. These results, combined with measurements of aerosol particle number concentrations, provide evidence supporting the hypotheses that (a) low surface aerosol particle number concentrations can limit fog liquid water path, (b) fog can act to increase near-surface aerosol particle number concentrations through enhanced mixing, and (c) multiple fog events in quiescent periods gradually deplete near-surface aerosol particle number concentrations.

54 ENVIRONMENTAL SCIENCES↗

Tethered balloon-borne observations of thermal-infrared irradiance and cooling rate profiles in the Arctic atmospheric boundary layer

Clouds play an important role in controlling the radiative energy budget of the Arctic atmospheric boundary layer. To quantify the impact of clouds on the radiative heating or cooling of the lower atmosphere and of the surface, vertical profile observations of thermal-infrared irradiances were collected using a radiation measurement system carried by a tethered balloon. We present 70 profiles of thermal-infrared radiative quantities measured in summer 2020 during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition and in autumn 2021 and spring 2022 in Ny-Ålesund, Svalbard. Measurements are classified into four groups: cloudless, low-level liquid-bearing cloud, elevated liquid-bearing cloud, and elevated ice cloud. Cloudless cases display an average radiative cooling rate of about —2 K d—1 throughout the atmospheric boundary layer. Instead, low-level liquid-bearing clouds are characterized by a radiative cooling up to —80 K d—1 within a shallow layer at cloud top, while no temperature tendencies are identified underneath the cloud layer. Radiative transfer simulations are performed to quantify the sensitivity of radiative cooling rates to cloud microphysical properties. In particular, cloud top cooling is strongly driven by the liquid water path, especially in optically thin clouds, while for optically thick clouds the cloud droplet number concentration has an increased influence. Additional radiative transfer simulations are used to demonstrate the enhanced radiative importance of the liquid relative to ice clouds. To analyze the temporal evolution of thermal-infrared radiation profiles during the transitions from a cloudy to a cloudless atmosphere, a respective case study is investigated.

54 ENVIRONMENTAL SCIENCES↗

Aerosol-Ice Formation Closure Pilot Study (AEROICSTUDY) Field Campaign Report

The aerosol-ice formation closure pilot study (AEROICESTUDY) was a field campaign conducted at the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility at the Southern Great Plains (SGP) observatory from October 7 to 28, 2019. The purpose of this campaign was to test a field observational approach for conducting an aerosol-ice formation closure study. In other words, the goal was to predict the number of ice nucleating particles (INPs) from the measurements of physical and chemical aerosol properties and compare those to measured INP number concentrations. This project was motivated by the fact that the aerosol community has widely conducted aerosol radiative closure, aerosol-cloud condensation nuclei (CCN), and CCN-droplet closure studies to test the physical models and parameterizations that cloud-resolving and climate models rely on to perform reliable simulations of the Earth system and energy budget. However, very few closure studies related to INPs have been conducted, and to our knowledge, none using robust, size-resolved, ambient aerosol composition measurements as model inputs.

54 ENVIRONMENTAL SCIENCES↗

ETO lidar studies of cirrostratus altocumulogenitus: Another role for supercooled liquid water in cirrus cloud formation

Cirrus clouds have traditionally been viewed as cold, wispy, or stratiform ice clouds, typically displaying optical phenomena such as haloes. A composition entirely of hexagonal ice crystals, of one habit or another could only have a transitory existence in cirrus, since the concentrations of ice nuclei (IN) measured by various techniques (at the surface or in the lower troposphere) indicate an enormous number of IN that should be active at cirrus cloud temperatures. In light of recent instrumental aircraft and polarization lidar studies of cirrus clouds, it is clear that highly supercooled cloud droplets can sometimes be a component of cirrus clouds. It remains to be determined if supercooled liquid water (SLW) is present abundantly enough in cirrus to play a significant role in earth's radiance balance, or is merely a curious, infrequent occurrence. To help evaluate this issue, the UH polarization lidar FIRE Extended Time Observation (ETO) of cirrus clouds are being utilized to compile, among other parameters, a climatological record of SLW clouds associated with and within cirrus.

Sassen, Kenneth↗

Data report on variations in the composition of sea ice during MIZEX/East'83 with the Nimbus-7 SMMR

Data acquired with the scanning multichannel microwave radiometer (SMMR) on board the Nimbus-7 satellite for a six-week period including the 1983 MIZEX in Fram Strait were analyzed with the use of a previously developed procedure for calculating sea ice concentration, multiyear fraction, and ice temperature. These calculations can compared with independent observations made on the surface and from aircraft in order to check the validity of the calculations based on SMMR data. The calculation of multiyear fraction, which was known earlier to be invalid near the melting point of sea ice, was of particular interest during this period. The indication of multiyear ice was found to disappear a number of times, presumably corresponding to freeze/thaw cycles which occurred in this time period. Both grid-print maps and grey-scale images of total sea ice concentration and multiyear sea ice fraction for the entire period are included.

Gloersen, P.↗