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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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NASA NTRS1992

The broad emission line and continuum variations of Seyfert galaxies. I - Time scales and amplitudes

Spectroscopic observations of 13 Seyfert 1 galaxies made from 1979 to 1984 at Palomar and Steward Observatories were analyzed for Balmer-line and optical continuum variability. The majority of the galaxies showed significant variations, particularly in the continuum. Typical peak-to-peak changes for H-beta and H-gamma integrated line fluxes were 100-200 percent, while the continua varied by 200-350 percent. In several cases, Balmer-line and continuum variations were found to be strongly correlated, as expected for photoionization by a central continuum source. However, these correlations were found to be highly nonlinear. Significant correlations were found between variability amplitude and global AGN properties such as luminosity. Moreover, a significant number of variations occurring on short time scales constrains the size of the broad-line region in Seyfert galaxies to about 90 lt-days across or less.

Rosenblatt, Edward I.↗

NASA NTRS1991

The electronic structure and second-order nonlinear optical properties of donor-acceptor acetylenes - A detailed investigation of structure-property relationships

A series of donor-acceptor acetylene compounds was synthesized in which systematic changes in both the conjugation length and the donor-acceptor strength were made. The effect of these structural changes on the spectroscopic and electronic properties of the molecules and, ultimately, on the measured second-order molecular hyperpolarizabilities (beta) was investigated. It was found that increases in the donor-acceptor strength resulted in increases in the magnitude of beta. For this class of molecules, the increase is dominated by the energy of the intramolecular charge-transfer transition, while factors such as the ground to excited-state dipole moment change and the transition-moment integral are much less important. Increasing the conjugation length from one to two acetylene linkers did not result in an increase in the value of beta; however, beta increased sharply in going from two acetylenes to three. This increase is attributed to the superposition of several nearly isoenergetic excited states.

Stiegman, A. E.↗

NASA NTRS1982

Recent advances in electromagnetic synthesis and analysis of dual-shaped reflector antennas

Dual-shaped reflectors have been used for many years. Thus, these reflectors have been used as high gain antennas on Voyagers 1 and 2. The objectives of the geometrical optics (GO) dual shaped synthesis are considered. Concerning the synthesis of dual shaped reflectors, it has been shown for circular symmetric reflectors that an exact GO solution can be found to the problem of transforming, by two reflections, any feed pattern into any aperture distribution. This problem involves solving two simultaneous nonlinear ordinary differential equations. The same approach for offset geometry leads to two simultaneous nonlinear partial differential equations. It is shown that these equations could also be integrated numerically, except that in general these equations are not total and therefore, in general, they do not have a 'smooth' solution. It is further shown that the offset partial differentials often very nearly form a total differential in many cases of practical importance.

Galindo-Israel, V.↗

DOE OSTI2026

A Compact Monolithic Electro-Optic Package for Quantum Microwave-to-Optical Transduction

We present a novel quantum transduction package that integrates a macroscopic electro-optic crystal into a compact, monolithic assembly designed for superconducting quantum processors. The device provides an efficient and scalable interface between microwave and optical domains while preserving cryogenic compatibility. We performed full-wave and quantum dynamical simulations to assess the performance of the hybrid system, focusing on the interaction between a transmon-based microwave cavity and the crystal’s and cavity low-frequency microwave mode. The transmon operates both as an ancilla for the QPU and as a nonlinear element enabling four-wave mixing between cavity and electro-optic crystal microwave fields. Our results indicate that this architecture can coherently mediate quantum information transfer from the cavity to the electro-optic mode, offering a promising platform for on-chip quantum transduction within superconducting quantum networks.

Reineri, Alessandro [Fermilab] (ORCID:000000016175↗

DOE OSTI2026

A Compact Monolithic Electro-Optic Package for Quantum Microwave-to-Optical Transduction

Reineri, Alessandro [Fermilab] (ORCID:000000016175↗

NASA NTRS1983

Integrated optical circuits for numerical computation

The development of integrated optical circuits (IOC) for numerical-computation applications is reviewed, with a focus on the use of systolic architectures. The basic architecture criteria for optical processors are shown to be the same as those proposed by Kung (1982) for VLSI design, and the advantages of IOCs over bulk techniques are indicated. The operation and fabrication of electrooptic grating structures are outlined, and the application of IOCs of this type to an existing 32-bit, 32-Mbit/sec digital correlator, a proposed matrix multiplier, and a proposed pipeline processor for polynomial evaluation is discussed. The problems arising from the inherent nonlinearity of electrooptic gratings are considered. Diagrams and drawings of the application concepts are provided.

Verber, C. M.↗

NASA NTRS2019

First Steps in the Creation of a Joint MISR/MODIS Ocean Color Atmospheric Correction Algorithm

We are creating a new algorithm that combines observations from MISR and MODIS (both on the NASA Terra spacecraft) to improve atmospheric correction and coverage for ocean color data products. The algorithm utilizes information rich, multi-angle MISR observations for atmospheric correction, applied to MODIS. Our goal is to produce atmospherically corrected Remote Sensing Reflectance from MODIS with enhanced coverage and accuracy, for input to downstream bio-optical ocean parameter retrieval algorithms.An important aspect of this work is the utilization of multi-angle views of the reflected ocean surface sun glint. Usually, such observations are avoided, since the intensity of the glint overwhelms any contribution from the ocean body. However, MISR's multi-angle observations see varying degrees of glint, which means they can be used to better determine aerosol optical properties (Kaufman et al., 2002, Ottaviani et al., 2013), and to identify surface wind speeds that govern the glint pattern. The latter could be utilized to replace the wind speeds taken from ancillary sources that are currently used to conservatively mask potential glint contamination in MODIS observations.To assess this capability, and to identify the appropriate parameterization, we present an analysis using the Generalized Nonlinear Retrieval Analysis (GENRA, Vukicevic et al., 2009) information content assessment. This technique is also easily modified to act as a Bayesian retrieval algorithm, for which initial results are discussed. Finally, we describe the status of integrating MISR data into the processing capabilities of the Ocean Biology Processing Group (OBPG) at NASA, and show the first ocean color vicarious calibration (Franz et al., 2007) of the MISR instrument.

Knobelspiesse, Kirk↗

DOE OSTI2026

Adaptive nonlinear wavefront shaping in layered TMDs

Two-dimensional transition metal dichalcogenides are promising candidates for nonlinear photonics applications, offering strong nonlinear susceptibility and compatibility with integrated platforms. Although considerable effort has been devoted to manipulating second harmonic generation in these materials, the dynamic control of nonlinear wavefronts remains largely unexplored. Metasurfaces have enabled significant progress in nonlinear beam engineering, yet their practical implementation is limited by low conversion efficiencies and restricted design flexibility. In this work, we employ feedback-based wavefront shaping using spatial light modulators to enhance SHG from pyramid-like WS 2 multilayer structures by over three orders of magnitude in selected spatial regions. This approach allows us to program nonlinear holograms and dynamically shape the SHG signal through phase-only modulation, opening new possibilities for nonlinear imaging, optical information processing, and data communication.

Mavian, Alex [Rensselaer Polytechnic Inst., Troy, ↗

NASA NTRS1995

Optical Computers and Space Technology

The rapidly increasing demand for greater speed and efficiency on the information superhighway requires significant improvements over conventional electronic logic circuits. Optical interconnections and optical integrated circuits are strong candidates to provide the way out of the extreme limitations imposed on the growth of speed and complexity of nowadays computations by the conventional electronic logic circuits. The new optical technology has increased the demand for high quality optical materials. NASA's recent involvement in processing optical materials in space has demonstrated that a new and unique class of high quality optical materials are processible in a microgravity environment. Microgravity processing can induce improved orders in these materials and could have a significant impact on the development of optical computers. We will discuss NASA's role in processing these materials and report on some of the associated nonlinear optical properties which are quite useful for optical computers technology.

Abdeldayem, Hossin A.↗

DOE OSTI2026

Multiresolution Quantum Chemistry: Nonlinear Response Properties at the Basis Set Limit

We benchmark the accuracy of Dunning correlation-consistent Gaussian basis sets for computing frequencydependent second-order hyperpolarizabilities relevant to second-harmonic generation (SHG), using multiresolution analysis (MRA) as a reference. Basis set errors are analyzed using a unit-sphere representation of the effective hyperpolarizability vector, enabling direct assessment of directional error structure. We introduce a relative RMS total error metric that integrates directional deviations over the unit sphere and complement it with signed projection errors that distinguish over- and underestimation. Unsupervised clustering based on these signed directional metrics reveals four distinct convergence behaviors across a set of 68 molecules. Unitsphere visualizations of representative systems show that basis set errors are often highly anisotropic and localized along specific bond directions, even when global error measures appear small. Doubly augmented basis sets consistently outperform singly augmented ones, and core-polarization functions are required for uniform convergence in second-row systems. Overall, this work demonstrates that directional analysis combined with clustering provides a robust framework for understanding basis set convergence in nonlinear optical response properties.

Basis sets↗

NASA NTRS2012

High Energy Laser Beam Propagation in the Atmosphere: The Integral Invariants of the Nonlinear Parabolic Equation and the Method of Moments

The method of moments is used to define and derive expressions for laser beam deflection and beam radius broadening for high-energy propagation through the Earth s atmosphere. These expressions are augmented with the integral invariants of the corresponding nonlinear parabolic equation that describes the electric field of high-energy laser beam to propagation to yield universal equations for the aforementioned quantities; the beam deflection is a linear function of the propagation distance whereas the beam broadening is a quadratic function of distance. The coefficients of these expressions are then derived from a thin screen approximation solution of the nonlinear parabolic equation to give corresponding analytical expressions for a target located outside the Earth s atmospheric layer. These equations, which are graphically presented for a host of propagation scenarios, as well as the thin screen model, are easily amenable to the phase expansions of the wave front for the specification and design of adaptive optics algorithms to correct for the inherent phase aberrations. This work finds application in, for example, the analysis of beamed energy propulsion for space-based vehicles.

Manning, Robert M.↗

NASA NTRS2021

Transmission Telescope Optical Dynamic Alignment

The Integrated Radio Optical Communication System (iROC) is designed to transmit data between Mars and Earth by means of radio waves at 32.67 GHz (Ka Band) and laser beam at 1550 nm, both transmitted via a combined teletenna. The iROC terminal will provide ‘beaconless’ operations to allow full function from the outer planets. In order to point without the aid of an uplink beacon, the proof of concept presented here is addressing the need for an accurate determination and control of the relative position of the laser beam with respect to a reference star. The experiment presented simulates a surrogate transmission telescope system in laboratory setting and presents the model used in the correction of the outgoing beam. The results of the model show a nonlinear dependence between the outgoing and the reference beam, indicating the necessity of a minimum of two metrology instruments placed along the optical system for increased pointing precision.

optical communication↗

DOE OSTI2025

Coherent Magnon–Photon Coupling in the Magnetic Semiconductor CrSBr

Magnon-based hybrid quantum systems are promising candidates for quantum interconnects and quantum sensors, and they offer a rich platform for exploring nonlinear magnonics and cavity–photon interactions. Two-dimensional (2D) van der Waals magnets provide a compact, atomically flat geometry that can be easily integrated into existing quantum circuits, such as superconducting resonators and qubits. Among various 2D magnets, the magnetic semiconductor CrSBr is particularly unique due to its strong spin–exciton, spin–lattice, and magnon–exciton interactions. In this work, we demonstrate coherent coupling between antiferromagnetic (AFM) magnons in CrSBr and microwave photons in a niobium-(Nb)-based-on-chip resonator. We tuned the magnon–photon coupling strength by changing the number of CrSBr flakes integrated into the Nb microwave photon resonators. Furthermore, this work demonstrates the first step toward integrating layered van der Waals 2D magnets into superconducting microwave circuits, with full access for microwave and optical probing.

Electromagnetic radiation↗

NASA NTRS1975

Infrared upconversion as a means of seeing in the dark

A new approach to seeing in the dark is described which is based on the principles of nonlinear optics employing a crystal such as lithium iodate. A nonlinear optical device capable of producing photons at higher frequencies from lower-frequency incident light is shown to upconvert infrared light directly into visible light. The major advantages of the infrared upconversion process is that it permits the infrared signal to be detected by photon-counting devices presently available for the visible spectral region, and that it can provide sensitivity to infrared radiation without the need for cryogenic cooling of the detector used. Early works on infrared upconversion are reviewed. The development of applications is discussed as to astronomical spectroscopy and infrared image upconversion involving either angular or positional resolution elements. The demonstration of infrared upconversion in rectangular waveguides of single-crystal GaAs by Anderson et al. (1971) indicates future possibilities in upconversion by the use of integrated optics devices.

Gurski, T. R.↗

NASA NTRS2020

Investigation Of Prandtl-Ishlinskii Hysteresis Compensation for Deep Space Optical Communications Pointing Control

This paper studies the simulated performance of the Deep Space Optical Communication (DSOC) laser downlink pointing control system that has a pointing requirement at the sub-microradian scale. To achieve the required pointing precision, the DSOC Flight Laser Transceiver (FLT) point-ahead mirror (PAM) employs piezoelectric actuators, which are widely used in precision applications due to their high motion resolution, rapid response, and high output forces. However, a piezoelectric actuator's performance is often limited by nonlinearities in their response, most significantly hysteresis. To study the effect of hysteresis on our simulated pointing performance, an invertible hysteresis model is developed using the Classical Prantdl-Ishlinskii (CPI) method. The simulation includes models of DSOC hardware and electronic system components based on key parameters (bias, frequency response, noise), with the hysteresis modeled in the PAM piezo actuator dynamics. A Proportional-Integral controller provides feedback with measurements from two potential sources: strain gauge sensors or a photon-counting camera. To compensate for hysteresis behavior, a feedforward inverse CPI hysteresis model is implemented in the control system. Two CPI models are built using different sampling methods (uniform sampling and cosine spacing) and controller performance is compared. For the maximum command range of ±400 μrad at 1 mHz, results show that the feedforward combined with feedback control reduces output tracking error by 50% or 58% (to 0.20 or 0.38 μrad) compared to feedback control alone (from 0.40 or 0.90 μrad), corresponding to the uniform-sampled and cosine-sampled CPI models, respectively.

Marinello, Lindsey A.↗

DOE OSTI2025

Giant Enhancement of Four-Wave Mixing by Doubly Zone-Folded Nonlocal Metasurfaces

Resonant optical metasurfaces hold promise for enhancing nonlinear optical signals and manipulating their fundamental properties. However, they rarely excel at amplifying signals from nonlinear processes with two incident pump beams, such as four-wave mixing (FWM) or sum-frequency generation. Frequency-mixing experiments impose challenging requirements for metasurface design due to the need to support multiple optical resonances with compatible field profiles at specified resonant wavelengths, often across a substantial spectral separation. Here, in this work, we introduce nonlocal ‘quadromer’ metasurfaces containing four nanostructures per unit cell as the key to unlocking configurable, multiresonant metasurfaces that enhance frequency-mixing processes. As a proof of concept, we experimentally demonstrate enhanced FWM using quadromer metasurfaces made of silicon and silicon-rich silicon nitride. The results are relevant for applications such as imaging of infrared light upconverted into the visible spectrum and the generation of quantum light via spontaneous FWM.

four-wave mixing↗

NASA NTRS1990

A parameterization for the shortwave transmissivity of stratiform water clouds based on empirical data and radiative transfer theory

Surface measurements of solar flux and total integrated liquid-water content, radiosonde data, and infrared satellite images are analyzed in conjunction with radiative transfer calculations to derive an empirical parameterization for the shortwave transmissivity of continental stratiform water clouds. The data were collected near Denver, Colorado, over a period of six years. A multiple reflection radiative transfer model is employed to estimate stratus cloud transmissivity in terms of the measurable liquid-water path (LWP). A nonlinear fit of estimated transmissivities to the corresponding observations of LWP yields close agreement with a previous, more complicated parameterization. The derived expression for cloud transmissivity is used to predict mean daily surface fluxes for 61 days during which periods of stratiform clouds were observed over the Denver area. A comparison between predicted and measured fluxes shows agreement to within + or - 4 percent, with best agreement for clouds of moderate optical thickness. Potential sources of error are identified with sensitivity studies.

Derr, V. E.↗

DOE OSTI2025

Resonant metasurface‐enabled quantum light sources for single‐photon emission and entangled photon‐pair generation

Light encodes information in multiple degrees of freedom (e.g., frequency, amplitude, and phase), enabling high‐speed, high‐bandwidth communication through fiber optics. Unlike classical light, quantum light (single or entangled photons) can transmit quantum states over long distances without loss of coherence, thereby coherently interconnecting quantum nodes for distributed quantum entanglement. Quantum light sources are critical for developing scalable quantum networks aimed at distributed quantum computing, quantum teleportation, and secure quantum communications. However, existing quantum light sources suffer from limited integrability, insufficient spectral and spatial tunability, and inefficiencies in achieving mass‐produced, deterministic, on‐demand quantum light generation. These limitations significantly hinder progress toward direct, on‐chip integration with quantum processing units and detectors – an essential step toward scalable quantum networks. Resonant metasurfaces that leverage photonic modes – such as Mie resonances, guided‐mode resonances, or symmetry‐protected bound states in the continuum – offer strong spatial and temporal confinement of electromagnetic fields, characterized by high quality factors and small mode volumes. These metasurfaces greatly enhance linear and nonlinear light‐matter interactions, making them ideal for efficient on‐chip quantum light generation and manipulation. Here, we describe recent advances in nanoscale quantum light sources and quantum photonic state manipulation enabled by resonant metasurfaces. We also provide an outlook on next‐generation miniaturized quantum light sources achievable through materials innovations in quantum emitters, the co‐design of resonant metasurfaces, and ultimately, the heterogeneous integration of emerging layered van der Waals materials with resonant metasurfaces.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗