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Improved Characterization of PSC Processes Derived from a Third-Generation CALIOP and MLS Detection and Composition Classification Algorithm

The new 3-year CloudSat and CALIPSO Science Team project described in this poster will use a unique combination of data from the Cloud-Aerosol LIdar with Orthogonal Polarization (CALIOP) instrument on CALIPSO and the Microwave Limb Sounder (MLS) on Aura, in conjunction with supporting meteorological information and detailed modeling studies, to advance our understanding of polar stratospheric cloud (PSC) processes and their role in ozone depletion. We will develop a third-generation (Gen3) PSC detection and composition algorithm that incorporates a new, more robust two-dimensional, multi-channel CALIOP feature detection scheme (2D-McDA). We will also devise and implement an improved two-dimensional PSC composition classification scheme that utilizes multiple parameters (e.g., CALIOP 532-nm parallel and perpendicular scattering ratios, CALIOP 1064-nm total scattering ratio, MLS HNO3 and H2O, ambient temperature, and temperature histories) in a Bayesian approach to determine the most likely PSC composition and help constrain solid PSC particle number density and size/shape. The combined CALIOP/MLS analyses will allow us to study in detail the full life cycle of PSCs and their resulting impact on gas-phase HNO3 and H2O, which should lead to improved parameterizations of PSC microphysics in global CCMs where detailed particle information is not available. The Gen3 CALIOP PSC algorithm will be a natural stepping-stone toward the analysis of data collected during future spaceborne lidar missions, such as NASA’s Atmosphere Observation System (AtmOS) mission currently scheduled for launch late in this decade. We will also investigate possible trends in PSC occurrence and composition over the entire CALIOP data record and through further comparisons with the Stratospheric Aerosol Measurement (SAM) II solar occultation PSC record from 1979-1989. Finally, we will validate the mountain-wave parameterization and PSC schemes used in the UM-UKCA (Unified Model coupled to the United Kingdom Chemistry and Aerosol module) chemistry-climate model through detailed comparisons with earlier CALIOP PSC data products and those developed under this proposal.

CALIPSO↗

Improved Characterization of PSC Processes Derived from a Third-Generation CALIOP and MLS Detection and Composition Classification Algorithm

The new 3-year CloudSat and CALIPSO Science Team project described in this poster will use a unique combination of data from the Cloud-Aerosol LIdar with Orthogonal Polarization (CALIOP) instrument on CALIPSO and the Microwave Limb Sounder (MLS) on Aura, in conjunction with supporting meteorological information and detailed modeling studies, to advance our understanding of polar stratospheric cloud (PSC) processes and their role in ozone depletion. We will develop a third-generation (Gen3) PSC detection and composition algorithm that incorporates a new, more robust two-dimensional, multi-channel CALIOP feature detection scheme (2D-McDA). We will also devise and implement an improved two-dimensional PSC composition classification scheme that utilizes multiple parameters (e.g., CALIOP 532-nm parallel and perpendicular scattering ratios, CALIOP 1064-nm total scattering ratio, MLS HNO3 and H2O, ambient temperature, and temperature histories) in a Bayesian approach to determine the most likely PSC composition and help constrain solid PSC particle number density and size/shape. The combined CALIOP/MLS analyses will allow us to study in detail the full life cycle of PSCs and their resulting impact on gas-phase HNO3 and H2O, which should lead to improved parameterizations of PSC microphysics in global chemistry-climate models (CCMs) where detailed particle information is not available. The Gen3 CALIOP PSC algorithm will be a natural stepping-stone toward the analysis of data collected during future spaceborne lidar missions, such as NASA’s Atmosphere Observation System (AOS) mission currently scheduled for launch late in this decade. We will also investigate possible trends in PSC occurrence and composition over the entire CALIOP data record and through further comparisons with the Stratospheric Aerosol Measurement (SAM) II solar occultation PSC record from 1979-1989. Finally, we will validate the mountain-wave parameterization and PSC schemes used in the UM-UKCA (Unified Model coupled to the United Kingdom Chemistry and Aerosol module) CCM through detailed comparisons with earlier CALIOP PSC data products and those developed under this proposal.

CALIPSO↗

Validation of UARS Microwave Limb Sounder Temperature and Pressure Measurements

The accuracy and precision of the Upper Atmosphere Research Satellite (UARS) Microwave Limb Sounder (MLS) atmospheric temperature and tangent-point pressure measurements are described. Temperatures and tangent- point pressure (atmospheric pressure at the tangent height of the field of view boresight) are retrieved from a 15-channel 63-GHz radiometer measuring O2 microwave emissions from the stratosphere and mesosphere. The Version 3 data (first public release) contains scientifically useful temperatures from 22 to 0.46 hPa. Accuracy estimates are based on instrument performance, spectroscopic uncertainty and retrieval numerics, and range from 2.1 K at 22 hPa to 4.8 K at 0.46 hPa for temperature and from 200 m (equivalent log pressure) at 10 hPa to 300 m at 0.1 hPa. Temperature accuracy is limited mainly by uncertainty in instrument characterization, and tangent-point pressure accuracy is limited mainly by the accuracy of spectroscopic parameters. Precisions are around 1 K and 100 m. Comparisons are presented among temperatures from MLS, the National Meteorological Center (NMC) stratospheric analysis and lidar stations at Table Mountain, California, Observatory of Haute Provence (OHP), France, and Goddard Spaceflight Center, Maryland. MLS temperatures tend to be 1-2 K lower than NMC and lidar, but MLS is often 5 - 10 K lower than NMC in the winter at high latitudes, especially within the northern hemisphere vortex. Winter MLS and OHP (44 deg N) lidar temperatures generally agree and tend to be lower than NMC. Problems with Version 3 MLS temperatures and tangent-point pressures are identified, but the high precision of MLS radiances will allow improvements with better algorithms planned for the future.

Fishbein, E. F.↗

A search for mountain waves in MLS stratospheric limb radiances fron the winter Northern Hemisphere: data analysis and global mountain wave modeling

Despite evidence from ground-based data that flow over mountains is a dominant source of gravity waves (GWs) for the Northern Hemisphere winter middle atmosphere, GW-related signals in global limb radiances from the Microwave Limb Sounder (MLS) on the Upper Atmosphere Research Satellite (UARS) have shown little direct evidence of mountain waves.

gravity waves dynamics general circulation global ↗

The Re-Analysis of Ozone Profile Data from a 41-Year Series of SBUV Instruments

In this study we present the validation of ozone profiles from a number of Solar Back Scattered Ultra Violet (SBUV) and SBUV/2 instruments that were recently reprocessed using an updated (Version 8.6) algorithm. The SBUV dataset provides the longest available record of global ozone profiles, spanning a 41-year period from 1970 to 2011 (except a 5-year gap in the 1970s) and includes ozone profile records obtained from the Nimbus-4 BUV and Nimbus-7 SBUV instruments, and a series of SBUV(/2) instruments launched on NOAA operational satellites (NOAA 09, 11, 14, 16, 17, 18, 19). Although modifications in instrument design were made in the evolution from the BUV instrument to the modern SBUV(/2) model, the basic principles of the measurement technique and retrieval algorithm remain the same. The long term SBUV data record allows us to create a consistent, calibrated dataset of ozone profiles that can be used for climate studies and trend analyses. In particular, we focus on estimating the various sources of error in the SBUV profile ozone retrievals using independent observations and analysis of the algorithm itself. For the first time we include in the metadata a quantitative estimate of the smoothing error, defined as the error due to profile variability that the SBUV observing system cannot inherently measure. The magnitude of the smoothing error varies with altitude, latitude, season and solar zenith angle. Between 10 and 1 hPa the smoothing errors for the SBUV monthly zonal mean retrievals are of the order of 1 %, but start to increase above and below this layer. The largest smoothing errors, as large as 15-20%, were detected in in the troposphere. The SBUV averaging kernels, provided with the ozone profiles in version 8.6, help to eliminate the smoothing effect when comparing the SBUV profiles with high vertical resolution measurements, and make it convenient to use the SBUV ozone profiles for data assimilation and model validation purposes. The smoothing error can also be minimized by combining layers of data, and we will discuss recommendations for this approach as well. The SBUV ozone profiles have been intensively validated against satellite profile measurements obtained from the Microwave Limb Sounders (MLS) (on board the UARS and AURA satellites), Stratospheric Aerosol and Gas Experiment (SAGE) and Michelson Interferometer for Passive Atmospheric Sounding (MIPAS). Also, we compare coincident and collocated SBUV ozone retrievals with observations made by ground-based instruments, such as microwave spectrometers, lidars, Umkehr instruments and balloon-borne ozonosondes. Finally, we compare the SBUV ozone profiles with output from the NASA GSFC GEOS-CCM model. In the stratosphere between 25 and 1 hPa the mean biases and standard deviations are within 5% for monthly mean ozone profiles. Above and below this layer the vertical resolution of the SBUV algorithm decreases and the effects of vertical smoothing should be taken into account. Though the SBUV algorithm has a coarser vertical resolution in the lower stratosphere and troposphere, it is capable of precisely estimating the integrated ozone column between the surface and 25 hPa. The time series of the tropospheric - lower stratospheric ozone column derived from SBUV agrees within 5% with the corresponding values observed by an ensemble of ozone sonde stations in North Hemisphere. Drift of the ozone time series obtained from each SBUV(/2) instrument relative to ground based and satellite measurements are evaluated and some features of individual SBUV(l2) instruments are discussed. In addition to evaluating individual instruments against independent observations, we also focus on the instrument to instrument consistency in the series. Overall, Version 8.6 ozone profiles obtained from two different SBUV(l2) instruments compare within a couple of percent during overlap periods and are consistently varying in time, with some exceptions. Some of the noted discrepancies might bssociated with ozone diurnal variations, since the difference in the local time of the observations for a pair of SBUV(l2) instruments could be several hours. Other issues include the potential short-term drift in measurements as the instrument orbit drifts, and measurements are obtained at high solar zenith angles (>85 ). Based on the results of the validation, a consistent, calibrated dataset of SBUV ozone profiles has been created based on internal calibration only.

Kramarova, Natalya↗

Arctic Ozone Depletion Observed by UARS MLS During the 1994-95 Winter

The Earth's northern hemisphere lower stratosphere was unusually cold in December 1995 and January 1995. Temperatures low enough for polar stratospheric cloud formation persisted until mid-March 1995, and the polar vortex was exceptionally strong throughout the winter. Previous and current Atmosphere Research Satellite (UARS) Microwave Limb Sounder (MLS) measurements indicating ozone depletion are given.

arctic↗

Validation of the Aura Microwave Limb Sounder middle atmosphere water vapor and nitrous oxide measurements

The quality of the version 2.2 (v2.2) middle atmosphere water vapor and nitrous oxide measurements from the Microwave Limb Sounder (MLS) on the Earth Observing System (EOS) Aura satellite is assessed. The impacts of the various sources of systematic error are estimated by a comprehensive set of retrieval simulations. Comparisons with correlative data sets from ground-based, balloon and satellite platforms operating in the UV/visible, infrared and microwave regions of the spectrum are performed. Precision estimates are also validated, and recommendations are given on the data usage. The v2.2 H2O data have been improved over v1.5 by providing higher vertical resolution in the lower stratosphere and better precision above the stratopause. The single-profile precision is ~0.2–0.3 ppmv (4–9%), and the vertical resolution is ~3–4 km in the stratosphere. The precision and vertical resolution become worse with increasing height above the stratopause. Over the pressure range 0.1–0.01 hPa the precision degrades from 0.4 to 1.1 ppmv (6–34%), and the vertical resolution degrades to ~12–16 km. The accuracy is estimated to be 0.2–0.5 ppmv (4–11%) for the pressure range 68–0.01 hPa. The scientifically useful range of the H2O data is from 316 to 0.002 hPa, although only the 82–0.002 hPa pressure range is validated here. Substantial improvement has been achieved in the v2.2 N2O data over v1.5 by reducing a significant low bias in the stratosphere and eliminating unrealistically high biased mixing ratios in the polar regions. The single-profile precision is ~13–25 ppbv (7–38%), the vertical resolution is ~4–6 km and the accuracy is estimated to be 3–70 ppbv (9–25%) for the pressure range 100–4.6 hPa. The scientifically useful range of the N2O data is from 100 to 1 hPa.

Atlas, E.↗

Effect of Convection on the Tropical Tropopause Layer over the Tropical Americas

Water vapor and ozone are the most important gases that regulate the radiative balance of the Tropical Tropopause Layer (TTL). Their radiative contribution dictates the height within the TTL and the rate at which air either ascends into the tropical stratosphere or subsides back to the tropical troposphere. The details of the mechanisms that control their concentration, however, are poorly understood. One of such mechanisms is convection that reaches into the TTL. ill this study, we will present evidence from space-borne observations of the impact that convection has on water vapor, ozone, and temperature in the TTL over the Tropical Americas where deep and overshooting convection have the highest frequency of occurrence in the tropics. We explore the effect of convective systems such as hurricanes during the 2005 season using the Microwave Limb Sounder (MLS) on Aura version 1.5 data and more recent tropical systems using the newly released version 2 data with higher vertical resolution. ill order to provide the horizontal extent and the vertical structure of the convective systems, we use data from the Moderate Resolution Imaging Spectroradiometer (MODIS) on Aqua, the Microwave Humidity Sensor (MHS) on NOAA~18, and CloudSat when available.

Pittman, Jasna↗

Study Pollution Impacts on Upper-Tropospheric Clouds with Aura, CloudSat, and CALIPSO Data

This viewgraph presentation reviews the impact of pollution on clouds in the Upper Troposphere. Using the data from the Aura Microwave Limb Sounder (MLS), CloudSat, CALIPSO the presentation shows signatures of pollution impacts on clouds in the upper troposphere. The presentation demonstrates the complementary sensitivities of MLS , CloudSat and CALIPSO to upper tropospheric clouds. It also calls for careful analysis required to sort out microphysical changes from dynamical changes.

radar↗

Ozone Vertical Profile Satellite Measurements by S-NPP OMPS, Aura MLS, and Sentinel-5P TROPOMI

NASA has been monitoring ozone variations from space since 1970 with the launch of the Backscatter Ultraviolet instrument (BUV) on Nimbus- 4. Ozone in the Earth’s stratosphere and troposphere plays a crucial role in protecting life from harmful solar UV radiation, and it also influences Earth’s climate. The vertical distribution of ozone is used in modeling forecasts, verifying model analysis and simulations, and improving the measurement of tropospheric ozone that is a toxic constituent of air pollution. The Microwave Limb Sounder (MLS) on the EOS Aura spacecraft has been monitoring long-term continuous stratosphere ozone vertical behaviors since 2004. The Ozone Mapper Profile Suite (OMPS) on the Suomi National Polar-orbiting Partnership (S-NPP) was launched in 2011. Two of its three instruments, the Limb Profiler (LP) and the Nadir Profiler (NP), are designed to map ozone profiles with full global coverage (~6 days for NP) and a high level of vertical accuracy (1-km reporting record for LP) in the stratosphere and upper troposphere. The TROPOspheric Monitoring Instrument (TROPOMI) on the Copernicus Sentinel-5 Precursor (S5P), launched in 2017, aims to retrieve ozone profiles in both the troposphere and up to top-of-atmosphere (TOA) by using UV radiation measurements in a spectral range of 270-320 nm. S5P/TROPOMI ozone profile products are planned to become available in April 2020. This presentation will concentrate on satellite ozone vertical profile data collections from OMPS and MLS which are archived at the NASA Goddard Earth Sciences Data and Information Services Center (GES DISC). TROPOMI ozone vertical profiles for the troposphere and to top-of-atmosphere will become available at NASA GES DISC in 2020. The presentation briefly explores their potential complementary usability in determining three-dimensional ozone global distributions with high temporal and spatial resolutions.

Zeng, Jian↗

Improved Understanding of the Modeled QBO Using MLS Observations and MERRA Reanalysis

The Quasi-Biennial Oscillation (QBO) dominates the variability of the tropical stratosphere on interannual time scales. The QBO has been shown to extend its influence into the chemical composition of this region through dynamical mechanisms. We have started our analysis using the realistic QBO internally generated by the Goddard Earth Observing System Version 5 (GEOS-5) general circulation model coupled to a comprehensive stratospheric and tropospheric chemical mechanism forced with observed sea surface temperatures over the past 33 years. We will show targeted comparisons with observations from NASAs Aura satellite Microwave Limb Sounder (MLS) and the Modern Era Retrospective-Analysis for Research and Applications (MERRA) reanalysis to provide insight into the simulation of the primary and secondary circulations associated with the QBO. Using frequency spectrum analysis and multiple linear regression we can illuminate the resulting circulations and deduce the strengths and weaknesses in their modeled representation. Inclusion of the QBO in our simulation improves the representation of the subtropical barriers and overall tropical variability. The QBO impact on tropical upwelling is important to quantify when calculating trends in sub-decadal scale datasets.

MERRA↗

GEOS Constituent Data Assimilation beyond Aura MLS: Assimilating NASA SAGE III/ISS profiles of stratospheric water vapor

Water vapor in the lower stratosphere is an important trace gas for atmospheric chemistry and radiative budget with direct impact on climate. During the last quarter of the 20th century, the Stratospheric Aerosol and Gas Experiment (SAGE) missions were crucial in monitoring the stratospheric ozone loss and the subsequent recovery as well as trends in water vapor linked to surface temperature trends. The SAGE III instrument aboard the International Space Station (ISS) continues the SAGE mission record, with high vertical resolution profiles of water vapor (and other constituents) since mid-2017. The NASA GEOS Earth system model has the capability to assimilate multi-constituents from ground and space-based instruments using the GEOS Constituent Data Assimilation System (CoDAS). Reanalysis products of stratospheric water vapor without data constraints are historically poor, and two recent reanalyses which assimilated stratospheric constituents observed by the Microwave Limb Sounder (MLS) improve the representation of stratospheric composition, including water vapor, when compared against independent observations. The MLS instrument is on NASA's Aura satellite which is expected to be decommissioned in the coming years. Here we demonstrate that while the number of solar occultation observations a day from SAGE III/ISS is about 1 % of the total number of profiles observed globally by MLS, the chemical timescales of water vapor in the lower stratosphere are long enough that the SAGE III/ISS data can provide a useful constraint on the assimilated product. Analyzed water vapor fields from assimilating only SAGE III/ISS water vapor profiles agree well with independent stratospheric observations, including when compared against the frost-point hygrometers at the three NOAA stations. Over the five-year period from 2017 through 2022, the analyzed water vapor using SAGE III/ISS captures many of the features seen with the assimilation of MLS observations. Note, this ability is reduced over regions where the SAGE III/ISS instrument provides infrequent or no observations (associated with the orbit of the ISS), as highlighted in the case study period following the eruption of the tropical underwater volcano Hunga Tonga in early 2022. Nevertheless, there is a clear benefit to the assimilation of stratospheric water vapor from SAGE III/ISS observations, allowing us to continue to monitor stratospheric composition for climate assessments following the impending loss of Aura.

K. Emma Knowland↗

GEOS Constituent Data Assimilation Beyond Aura MLS: Assimilating NASA SAGE III/ISS Profiles of Stratospheric Water Vapor

Water vapor in the lower stratosphere is an important trace gas for atmospheric chemistry and radiative budget with direct impact on climate. During the last quarter of the 20th century, the Stratospheric Aerosol and Gas Experiment (SAGE) missions were crucial in monitoring the stratospheric ozone loss and the subsequent recovery as well as trends in water vapor linked to surface temperature trends. The SAGE III instrument aboard the International Space Station (ISS) continues the SAGE mission record, with high vertical resolution profiles of water vapor (and other constituents) since mid-2017. The NASA GEOS Earth system model has the capability to assimilate multi-constituents from ground and space-based instruments using the GEOS Constituent Data Assimilation System (CoDAS). Reanalysis products of stratospheric water vapor without data constraints are historically poor, and two recent reanalyses which assimilated stratospheric constituents observed by the Microwave Limb Sounder (MLS) improve the representation of stratospheric composition, including water vapor, when compared against independent observations. The MLS instrument is on NASA's Aura satellite which is expected to be decommissioned in the coming years. Here we demonstrate that while the number of solar occultation observations a day from SAGE III/ISS is about 1 % of the total number of profiles observed globally by MLS, the chemical timescales of water vapor in the lower stratosphere are long enough that the SAGE III/ISS data can provide a useful constraint on the assimilated product. Analyzed water vapor fields from assimilating only SAGE III/ISS water vapor profiles agree well with independent stratospheric observations, including when compared against the frost-point hygrometers at the three NOAA stations. Over the five-year period from 2017 through 2022, the analyzed water vapor using SAGE III/ISS captures many of the features seen with the assimilation of MLS observations. Note, this ability is reduced over regions where the SAGE III/ISS instrument provides infrequent or no observations (associated with the orbit of the ISS), as highlighted in the case study period following the eruption of the tropical underwater volcano Hunga Tonga in early 2022. Nevertheless, there is a clear benefit to the assimilation of stratospheric water vapor from SAGE III/ISS observations, allowing us to continue to monitor stratospheric composition for climate assessments following the impending loss of Aura.

K. Emma Knowland↗

GEOS Constituent Data Assimilation Beyond Aura MLS: Assimilating NASA SAGE III/ISS Profiles of Stratospheric Water Vapor

Water vapor in the lower stratosphere is an important trace gas for atmospheric chemistry and radiative budget with direct impact on climate. During the last quarter of the 20th century, the Stratospheric Aerosol and Gas Experiment (SAGE) missions were crucial in monitoring the stratospheric ozone loss and the subsequent recovery as well as trends in water vapor linked to surface temperature trends. The SAGE III instrument aboard the International Space Station (ISS) continues the SAGE mission record, with high vertical resolution profiles of water vapor (and other constituents) since mid-2017. The NASA GEOS Earth system model has the capability to assimilate multi-constituents from ground and space-based instruments using the GEOS Constituent Data Assimilation System (CoDAS). Reanalysis products of stratospheric water vapor without data constraints are historically poor, and two recent reanalyses which assimilated stratospheric constituents observed by the Microwave Limb Sounder (MLS) improve the representation of stratospheric composition, including water vapor, when compared against independent observations. The MLS instrument is on NASA's Aura satellite which is expected to be decommissioned in the coming years. Here we demonstrate that while the number of solar occultation observations a day from SAGE III/ISS is about 1 % of the total number of profiles observed globally by MLS, the chemical timescales of water vapor in the lower stratosphere are long enough that the SAGE III/ISS data can provide a useful constraint on the assimilated product. Analyzed water vapor fields from assimilating only SAGE III/ISS water vapor profiles agree well with independent stratospheric observations, including when compared against the frost-point hygrometers at the three NOAA stations. Over the five-year period from 2017 through 2022, the analyzed water vapor using SAGE III/ISS captures many of the features seen with the assimilation of MLS observations. Note, this ability is reduced over regions where the SAGE III/ISS instrument provides infrequent or no observations (associated with the orbit of the ISS), as highlighted in the case study period following the eruption of the tropical underwater volcano Hunga Tonga in early 2022. Nevertheless, there is a clear benefit to the assimilation of stratospheric water vapor from SAGE III/ISS observations, allowing us to continue to monitor stratospheric composition for climate assessments following the impending loss of Aura.

K. Emma Knowland↗

Toric offset three-reflector antenna for the advanced microwave limb sounder

An advanced Microwave Limb Sounder (MLS), now in concept development for a potential future mission, is a space-borne heterodyne instrument to measure pressure, temperature, and atmospheric constituents from thermal emission between 120 and 2400 GHz. Previous MLS instruments used pencil-beam antennas sized to resolve N 1 vertical scale height. Current atmospheric models need better horizontal resolution than orbit spacing provides. To meet these needs, a new antenna concept combines the wide scan range of the parabolic torus with unblocked offset Cassegrain optics. The resulting system is diffraction-limited in the vertical plane but extremely astigmatic, with beamwidths 0.13~2.5. Nadir axis symmetry ensures that this Beam AspectRatio (BAR) is invariant over f33' of azimuth. The antenna can feed either an array of receivers or multiplexed low-noise receivers whose FOVs are swept by a small scanning mirror. We describe 3 stages of antenna design: First, using a paraxial-optics method, we choose conic profiles given vertical resolution orbit geometry, then develop the surfaces by nadir axis rotation, matching axisymmetric feeds to the BAR. A ray-trace program validates the design and generates alignment and deformation tolerances. Finally, a physical optics analysis verifies reflector surface currents and radiation patterns.

microwave↗

Constraining Middle Atmospheric Moisture in GEOS-5 Using EOS-MLS Observations

Middle atmospheric water vapor plays an important role in climate and atmospheric chemistry. In the middle atmosphere, water vapor, after ozone and carbon dioxide, is an important radiatively active gas that impacts climate forcing and the energy balance. It is also the source of the hydroxyl radical (OH) whose abundances affect ozone and other constituents. The abundance of water vapor in the middle atmosphere is determined by upward transport of dehydrated air through the tropical tropopause layer, by the middle atmospheric circulation, production by the photolysis of methane (CH4), and other physical and chemical processes in the stratosphere and mesosphere. The Modern-Era Retrospective analysis for Research and Applications (MERRA) reanalysis with GEOS-5 did not assimilate any moisture observations in the middle atmosphere. The plan is to use such observations, available sporadically from research satellites, in future GEOS-5 reanalyses. An overview will be provided of the progress to date with assimilating the EOS-Aura Microwave Limb Sounder (MLS) moisture retrievals, alongside ozone and temperature, into GEOS-5. Initial results demonstrate that the MLS observations can significantly improve the middle atmospheric moisture field in GEOS-5, although this result depends on introducing a physically meaningful representation of background error covariances for middle atmospheric moisture into the system. High-resolution features in the new moisture field will be examined, and their relationships with ozone, in a two-year assimilation experiment with GEOS-5. Discussion will focus on how Aura MLS moisture observations benefit the analyses.

Jin, Jianjun↗

Ground-Based Microwave Measurements of ClO and O3 Over Scott Base, Antarctica

We present measurements from a new microwave instrument that has been deployed at Scott Base, Antarctica, primarily to measure ClO. The new instrument allows for the extension of the time series of lower stratospheric ClO measurements begun in 1996 at this site, while some of the technical improvements offer the possibility of making additional measurements. We show measurements of ClO and O 3 in both the upper and lower stratosphere near both the fall and spring equinox and document the diurnal variations of these measurements throughout the season. The ground-based measurements are compared with Aura Microwave Limb Sounder (MLS) measurements, which are available twice per day, and with a NASA Goddard 2D model (GSFC2D) simulation. We show that, in agreement with the GSFC2D model diurnal variations, upper stratospheric ClO mixing ratios gradually increase throughout the daylight hours, while in the lower stratospheric austral spring, when heterogeneous chemistry associated with polar stratospheric clouds occurs, daily maximum ClO mixing ratios of near 2 ppbv occur near noon. We also show measurements of stratospheric O 3 , primarily in the upper stratosphere, which, while exhibiting a low bias of ∼15%–20% relative to Aura MLS, show temporal variations in good agreement with MLS.

stratospheric ozone↗

Mountain Waves in the Middle Atmosphere: Microwave Limb Sounder Observations and Analyses

Observations and analyses of mesoscale gravity waves in the stratosphere from the Upper Atmosphere Research Satellite (UARS) Microwave Limb Sounder (MLS) are summarized, with focus on global distribution of topography related wave activities. We found most of the orographical wave activities occur during the winter seasons over high latitude mountain ridges. In the northern hemisphere, the strongest waves are those over Scandinavia, Central Eurasia, and southern Greenland, whereas in the southern hemisphere, wave activities are outstanding over the Andes, New Zealand, and Antarctic rim;, MLS observations suggest that these orographic waves are located mostly on the down stream side of the mountain ridge with downward phase progression and have horizontal phase velocities opposite to the stratospheric jet-stream. Future studies using MLS data and numerical modeling will lead to better understanding of gravity wave effects on dynamics and chemistry in the middle atmosphere.

UPPER ATMOSPHERE↗