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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 109 records · Page 6

Optimization of a dry, mixed nuclear fuel storage array for nuclear criticality safety - 14339

A dry storage array of used nuclear fuel at the Idaho National Laboratory contains a mixture of more than twenty different types of research and test reactor fuels. Significant neutronic interaction occurs between fuel canisters within this large storage arrangement of 636 fuel storage canisters. Nuclear criticality safety is maintained primarily by moderation control and through control of neutron interaction and leakage provided by the credited geometry. Over the nearly forty years of operation the collected fuels are now arranged in a configuration that does not minimize the system neutron multiplication factor (k{sub eff}). This creates a concern since the entire remaining facility storage capacity cannot be utilized without exceeding the system minimum subcritical state (k{sub safe}) for ensuring nuclear criticality safety. This work determines a more optimal arrangement for the stored fuels with a goal to minimize the system k{sub eff}, but also with a minimum of potential fuel canister relocation movements. The ultimate goal is to establish a solution for this multiple-objective optimization problem by finding the Pareto Front for maximum k{sub eff} reduction versus the number of canister relocations. The process first required additional analysis of the array by Monte-Carlo neutron transport codes (specifically, MCNP) to gain a greater understanding of the interaction characteristics of the disparate fuel types. Some stored fuels are composed of primarily metallic and oxide components that provide very little inherent moderation, while other fuel types contain graphite or zirconium-hydride which can contribute a significant amount of moderation. These factors cause a complex relationship within a fuel arrangement with respect to thermal utilization and axial leakage probability. The new MCNP analysis was utilized to develop a simplified spreadsheet-based empirical model which simulates the array k{sub eff} result. This empirical model was benchmarked against additional MCNP calculations for various arrangements and then employed in the optimization analysis. A Tabu metaheuristic and stochastic approximation optimization was applied to the empirical model with the optimization function to minimize the array k{sub eff}. The optimization algorithm interrogated the empirical model to determine the optimal rearrangement for up to sixty canister movements. The Pareto Front was found, which shows that a limited number of canister relocation movements could allow the existing thirty-one empty array positions to be filled with common research reactor fuels while also yielding a reduction in the overall array k{sub eff} relative to the current arrangement. This will impart an improvement in the facility utilization while also offering an enhancement in the safety margin. The reduction in array reactivity has been confirmed by a final set of MCNP calculations with the proposed new arrangements. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Color Transparency and Light-Front Holographic QCD

Color transparency, the reduction of initial-state or final-state interactions in coherent nuclear processes, is a natural prediction of QCD (quantum chromodynamics) provided that small-sized or point-like configurations (PLCs) are formed in high-momentum transfer, high-energy, semi-exclusive processes. I use the Frankfurt-Miller-Strikman criteria for the existence of PLCs to show that the wave functions of light-front holographic QCD, as currently formulated, do not contain a PLC.

Miller, Gerald A. (ORCID:0000000324433639)↗

Change of Nuclear Configurations in the Neutrinoless Double-β Decay of 130 Te → 130 Xe and 136 Xe → 136 Ba

The change in the configuration of valence protons between the initial and final states in the neutrinoless double-beta decay of Te-130 -> Xe-130 and of Xe-136 -> Ba-136 has been determined by measuring the cross sections of the (d,He-3) reaction with 101-MeV deuterons. Together with our recent determination of the relevant neutron configurations involved in the process, a quantitative comparison with the latest shell-model and interacting-boson-model calculations reveals significant discrepancies. These are the same calculations used to determine the nuclear matrix elements governing the rate of neutrinoless double-beta decay in these systems.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Concept of Very-Asymmetric lepton Collider for dark matter search

Accelerator-based searches for dark matter are aiming for high sensitivity and need an experimental setup with high luminosity. This field of research is often called intensity frontier physics. One of the best motivated portals of interaction between dark matter and ordinary matter is a dark photon which could be observed as a resonance in the invariant mass of the decay products. Electron–positron collisions are known to be the cleanest interaction for such a study. In this paper we propose a scheme for a collider which allows for a luminosity of a few orders of magnitude higher than could be obtained in a conventional symmetric collider and with a few times higher accessible mass than is possible using a positron beam and a fixed target approach. The key concept is based on asymmetric energies: a high-energy circulating positron beam and a low-energy high-intensity electron beam, and optimization of the beam interaction region. We present here a configuration of a collision region of 10 MeV electron and 4 GeV positron beams.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

On the nonadiabatic collisional quenching of OH(A) by H 2 : a four coupled quasi-diabatic state description

A four-state diabatic potential energy matrix (DPEM), H d , for the description of the nonadiabatic quenching of OH(A 2 Σ + ) by collisions with H 2 is reported. The DPEM is constructed as a fit to adiabatic energies, energy gradients, and derivative couplings obtained exclusively from multireference configuration interaction wave functions. A four-adiabatic-electronic-state representation is used in order to describe all energetically accessible regions of the nuclear coordinate space. Partial permutation-inversion symmetry is incorporated into the representation. Here, the fit is based on electronic structure data at 42 882 points, described by over 1.6 million least squares equations with a root mean square (mean unsigned) error of 178(83) cm –1 . Comparison of ab initio and H d determined minima, saddle points, and energy minimized points on C 2v , C s , C ∞v , and C 1 (noncoplanar) portions of two conical intersection seams are used to establish the accuracy of the H d .

74 ATOMIC AND MOLECULAR PHYSICS↗

Scrape-off layer plasma and neutral characteristics and their interactions with walls for FNSF

Simulations of the heat flux on plasma facing components from exhausting core plasma are reported for two possible Fusion Nuclear Science Facility (FNSF) divertor configurations. One configuration utilizes divertor plates strongly inclined with respect to the poloidal magnetic flux surfaces like that planned for ITER and results in a partially detached divertor-plasma. The second configuration has divertor plates orthogonal to the flux surfaces, which leads to a fully detached divertor-plasma if the width of the divertor region is sufficient. Both configurations use scrape-off layer impurity seeding to yield an acceptable peak heat flux of ~10 MW/m 2 or smaller on the divertor plates and chamber walls. The roles of recycled hydrogenic atoms and molecules are investigated and distribution of sputtering tungsten throughout the edge region modeled. Furthermore, the simulations are performed with the UEDGE 2D transport code to model both plasma and neutral components with supplementary neutral modeling performed with the DEGAS 2 Monte Carlo code.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Structured ground states of randomly interacting bosons

Bosonic degrees of freedom and their emergence as part of complex quantum many-body dynamics, symmetries, collective behavior, clustering, and phase transitions play an important role in modern studies of quantum systems. In this paper, we present a systematic study of many-boson systems governed by random interactions. Our findings show that ground states of randomly interacting bosons are not random, being dominated by a few collective configurations containing condensates of clusters.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Effective many-body interactions in reduced-dimensionality spaces through neural network models

Accurately describing properties of challenging problems in physical sciences often requires complex mathematical models that are unmanageable to tackle head on. Therefore, developing reduced-dimensionality representations that encapsulate complex correlation effects in many-body systems is crucial to advance the understanding of these complicated problems. However, a numerical evaluation of these predictive models can still be associated with a significant computational overhead. To address this challenge, in this paper we discuss a combined framework that integrates recent advances in the development of active-space representations of coupled cluster (CC) downfolded Hamiltonians with neural network approaches. The primary objective of this effort is to train neural networks to eliminate the computationally expensive steps required for evaluating hundreds or thousands of Hugenholtz diagrams, which correspond to multidimensional tensor contractions necessary for evaluating a many-body form of downfolded effective Hamiltonians. Using small molecular systems (the H 2 O and HF molecules) as examples, we demonstrate that training neural networks employing effective Hamiltonians for a few nuclear geometries of molecules can accurately interpolate or extrapolate their forms to other geometrical configurations characterized by different intensities of correlation effects. We also discuss differences between effective interactions that define CC downfolded Hamiltonians with those of bare Hamiltonians defined by Coulomb interactions in the active spaces. Published by the American Physical Society 2024

97 MATHEMATICS AND COMPUTING↗

Feasibility study of full-reactor gas core demonstration test

Separate studies of nuclear criticality, flow patterns, and thermodynamics for the gas core reactor concept have all given positive indications of its feasibility. However, before serious design for a full scale gas core application can be made, feasibility must be shown for operation with full interaction of the nuclear, thermal, and hydraulic effects. A minimum sized, and hence minimum expense, test arrangement is considered for a full gas core configuration. It is shown that the hydrogen coolant scattering effects dominate the nuclear considerations at elevated temperatures. A cavity diameter of somewhat larger than 4 ft (122 cm) will be needed if temperatures high enough to vaporize uranium are to be achieved.

Kunze, J. F.↗

A radioluminescent nuclear battery using volumetric configuration: 63 Ni solution/ZnS:Cu,Al/InGaP

Energy dense power sources are critical to the development of compact, remote sensors for terrestrial and space applications. Nuclear batteries using β - -emitting radioisotopes possess energy densities 1000 times greater than chemical batteries. Their power generation is a function of β - flux saturation point relative to the planar (2D) configuration, β - range, and semiconductor converter. An approach to increase power density in a beta-photovoltaic (β-PV) nuclear battery is described. By using volumetric (3D) configuration, the radioisotope, nickel-63 ( 63 Ni) in a chloride solution was integrated in a phosphor film (ZnS:Cu,Al) where the β - energy is converted into optical energy. The optical energy was converted to electrical energy via an indium gallium phosphate (InGaP) photovoltaic (PV) cell, which was optimized for low light illumination and closely matched to radioluminescence (RL) spectrum. With 15 mCi of 63 Ni activity, the 3D configuration energy values surpassed 2D configuration results. The highest total power conversion efficiency ($η_t$) of 3D configuration was 0.289% at 200 µm compared 0.0638% for 2D configuration at 50 µm. The highest electrical power and ηt for the 3D configuration were 3.35 nW e /cm 2 at an activity of 30 mCi and 0.289% at an activity of 15 mCi, respectively. By using 3D configuration, the interaction space between the radioisotope source and scintillation material increased, allowing for significant electrical energy output, relative to the 2D configuration. These initial results represent a first step to increase nuclear battery power density from microwatts to milliwatts per 1000 cm 3 with the implementation of higher energy β - sources.

25 ENERGY STORAGE↗

Adjustment of Non-linear Interaction Parameters for Relativistic Mean Field Approach by Using Artificial Neural Networks

The relativistic mean field (RMF) model with a small number of adjusted parameters has been used successfully in the last thirty years for predictions of various ground-state nuclear properties of nuclei. In this model, Dirac and Klein–Gordon like equations obtained from application of variation principle on phenomenological Lagrangian density are solved iteratively for calculations of nuclear properties of nuclei. For this purpose, parameters such as masses of considered mesons, nucleon–meson coupling constants, and self-couplings of mesons are needed and they are fitted from experimental data. Some parameter sets for RMF model introduced to correct predictions of nuclear properties of nuclei cover nuclidic chart. Besides Artificial Neural Network (ANN) method is used successfully in many field of science as in nuclear physics. ANN is known as a very powerful tool that are used when standard techniques fail to estimate the correlation between the variables. In the present study, ANN method has been employed to check its understanding capability of relations between RMF model parameters and their predictions on the ground-state binding energies of some spherical nuclei. Understanding capability of ANN method for these relations of considered nuclei has been found well. Based on this success, new non-linear parameter set for RMF model called DEFNE by us have been produced by using ANN method. Furthermore, predictions of RMF model with DEFNE parameter set for ground-state binding energies and charge radii of nuclei cover nuclidic chart have been found as in agreement with the available experimental data.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Emergence of an island of extreme nuclear isomerism at high excitation near 208 Pb

Metastable states with $T_{1/2}$ = 8(2) ms in 205Bi and $T_{1/2}$ = 0.22(2) ms in 204 Pb, with ≈ 8 MeV excitation energy and angular momentum ≥ 22 $\hbar$, have been established. These represent, by up to two orders of magnitude, the longest-lived nuclear states above an excitation energy of 7 MeV, ever identified in the nuclear chart. Additionally, the half-life of the 10.17 MeV state in 206 Bi has been determined to be 0.027(2) ms, the next highest value in this highly excited regime. These observations indicate the emergence of an island of extreme nuclear isomerism arising from core-excited configurations at high excitation in the vicinity of the doubly closed-shell nucleus 208 Pb. These results are expected to provide discriminating tests of the effective interactions used in current large-scale shell-model calculations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Nuclear structure and band mixing in Pt 194

We introduce a two-particle, two-hole mixed configuration scheme to fit E2 strengths for the 0 ↔ 2, 2 ↔ 4, and 4 ↔ 6 transitions in 194 Pt. The interaction includes two sets of pairing operators, {S ± (t), S 0 (t)} (t = s, d). Solutions within this framework are used to analyze energy spectra, E2 transitions, and band-mixing features of the model. The results confirm that mixing is small and similar for J = 2, 4, and 6, with the calculated energies and transition matrix elements in excellent agreement with experimental data.

190 ≤ A ≤ 219↗

Proton decays in 16 Ne and 18 Mg and isospin-symmetry breaking in carbon isotopes and isotones

We report that proton-rich nuclei possess unique properties in the nuclear chart. Due to the presence of both continuum coupling and Coulomb interaction, phenomena such as halos, Thomas-Ehrman shift, and proton emissions can occur. Relevant experimental data are difficult to obtain, so that theoretical calculations are needed to understand nuclei at drip lines and to guide experimentalists. In particular, the 16 Ne and 18 Mg isotopes are supposed to be one-proton and/or two-proton emitting nuclei, but associated experimental data are either incomplete or even unavailable. Consequently, we performed Gamow shell model calculations of carbon isotones bearing A = 15 - 18 . Isospin-symmetry breaking occurring in carbon isotones and isotopes is also discussed. It is hereby shown that the mixed effects of continuum coupling and Coulomb interaction at drip lines generate complex patterns in isospin multiplets. Added to that, it is possible to determine the one-proton and two-proton widths of 16 Ne and 18 Mg . Obtained decay patterns are in agreement with those obtained in previous experimental and theoretical works. Moreover, to our knowledge, this is the first theoretical calculation of binding energy and partial decay widths of 18 Mg in a configuration interaction picture.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Simulating the absorption spectra of helium clusters (N = 70, 150, 231, 300) using a charge transfer correction to superposition of fragment single excitations

Simulations of the n = 2 absorption spectra of HeN(N = 70, 150, 231, 300) clusters are reported, with nuclear configurations sampled by path integral molecular dynamics. The electronic structure is treated by a new approach, ALMO-CIS+CT, which is a formulation of configuration interaction singles (CIS) based on absolutely localized molecular orbitals (ALMOs). The method generalizes the previously reported ALMO-CIS model [K. D. Closser et al. J. Chem. Theory Comput. 11, 5791 (2015)] to include spatially localized charge transfer (CT) effects. It is designed to recover large numbers of excited states in atomic and molecular clusters, such as the entire n = 2 Rydberg band in helium clusters. ALMO-CIS+CT is shown to recover most of the error caused by neglecting charge transfer in ALMO-CIS and has comparable accuracy to standard CIS for helium clusters. For the n = 2 band, CT stabilizes states towards the blue edge by up to 0.5 eV. ALMO-CIS+CT retains the formal cubic scaling of ALMO-CIS with respect to system size. With improvements to the implementation over that originally reported for ALMO-CIS, ALMO-CIS+CT is able to treat helium clusters with hundreds of atoms using modest computing resources. Here, a detailed simulation of the absorption spectra associated with the 2s and 2p bands of helium clusters up to 300 atoms is reported, using path integral molecular dynamics with a spherical boundary condition to generate atomic configurations at 3 K. The main features of experimentally reported fluorescence excitation spectra for helium clusters are reproduced.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Borehole Disposal: Update on the Science, Technology, and Potentially Suitable Radioactive Wastes - 20170

A recent Special Issue of the Energies Journal on Deep Borehole Disposal of Nuclear Waste has delivered a timely update on the science and technology of borehole disposal and the types of radioactive wastes it could potentially accommodate. The Special Issue papers discuss (i) circumstances under which a national waste management programme might wish to consider deep borehole disposal [1], (ii) a status report of deep borehole disposal options in Germany [2], (iii) the use of deep horizontal drill-holes in sedimentary, metamorphic or igneous rocks for disposal of spent nuclear fuel and high-level radioactive waste [3], (iv) the analysis of corrosion performance of engineered barrier systems [4], (v) a review of the potential cementing systems suitable for deep borehole disposal [5], (vi) the thermal evolution around heat-generating waste for a wide range of material properties and disposal configurations [6], (vii) a geochemical analysis of deep brines focussed on fluid-rock interactions [7], (viii) post-closure performance assessment calculations for deep borehole disposal of Cs/Sr capsules [8], and (ix) an example safety case for deep borehole disposal of nuclear wastes [9]. This paper provides an overview of the main findings from these publications and highlights some of the technological and scientific challenges that need to be overcome when developing a deep borehole disposal concept. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Electromagnetic properties of low-lying states in neutron-deficient Hg isotopes: Coulomb excitation of 182 Hg, 184 Hg, 186 Hg and 188 Hg

The neutron-deficient mercury isotopes serve as a classical example of shape coexistence, whereby at low energy near-degenerate nuclear states characterized by different shapes appear. The electromagnetic structure of even-mass 182-188 Hg isotopes was studied using safe-energy Coulomb excitation of neutron-deficient mercury beams delivered by the REX-ISOLDE facility at CERN. The population of 0 + 1,2 , 2 + 1,2 and 4 + 1 states was observed in all nuclei under study. Reduced E2 matrix elements coupling populated yrast and non-yrast states were extracted, including their relative signs. These are a sensitive probe of shape coexistence and may be used to validate nuclear models. The experimental results are discussed in terms of mixing of two different configurations and are compared with three different model calculations: the Beyond Mean Field model, the Interacting Boson Model with configuration mixing and the General Bohr Hamiltonian. Partial agreement with experiment was observed, hinting to missing ingredients in the theoretical descriptions.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

The electron affinity of the uranium atom

The results of a combined experimental and computational study of the uranium atom are presented with the aim of determining its electron affinity. Experimentally, the electron affinity of uranium was measured via negative ion photoelectron spectroscopy of the uranium atomic anion, U – . Computationally, the electron affinities of both thorium and uranium were calculated by conducting relativistic coupled-cluster and multi-reference configuration interaction calculations. The experimentally determined value of the electron affinity of the uranium atom was determined to be 0.309 ± 0.025 eV. The computationally predicted electron affinity of uranium based on composite coupled cluster calculations and full four-component spin–orbit coupling was found to be 0.232 eV. Predominately due to a better convergence of the coupled cluster sequence for Th and Th – , the final calculated electron affinity of Th, 0.565 eV, was in much better agreement with the accurate experimental value of 0.608 eV. In both scenarios, the ground state of the anion corresponds to electron attachment to the 6d orbital.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗