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At least 109 records · Page 6

Report Summarizing Boiling Transition (Dryout) Testing of FeCrAl Cladding

Nuclear fuel and cladding in a light water reactor must maintain integrity under all normal operational and anticipated operational occurrences. In a Boiling Water Reactor (BWR) some Anticipated Operational Occurrences (AOOs) and Anticipated Transients Without SCRAM (ATWS) events have been known to result in cladding damage due to dryout with conventional Zircaloy-2 claddings. This work presents an assessment of commercially-fabricated, accident tolerant iron-chromium-aluminum (FeCrAl) alloy C26M cladding in such events with regard to the ballooning failure mode for unirradiated cladding In the severe accident test station (SATS), an experiment has been developed to gauge accident tolerance of fuel cladding materials under simulated cyclic dryout conditions. Thermal cycling from 300°C to 650°C was implemented on C26M and Zircaloy-2 tubes. The C26M tube did not fail after 54 cycles. The Zircaloy- 2 tube run under the same parameters as the C26M tube failed during the fourth cycle, consistent with expectations from the literature. Due to thermal gradients present in the furnace, both tubes experienced a maximum temperature at ~780°C. Due to differences in tube geometry, the hoop stress of the C26M tube was significantly higher than that of the Zircaloy-2 tube, 76 MPa at the maximum peak temperature compared to 55 MPa at burst, respectively. The cyclic dryout experiments show an increased performance of C26M over Zircaloy-2 under simulated conditions, an indication of C26M possessing superior high temperature oxidation resistance, mechanical properties and potentially resistance to fatigue.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Evaluation of an Accident Tolerant Fuel Leak in the Advanced Test Reactor

Accident Tolerant Fuels (ATF), which are nuclear fuel sources designed to withstand operational irregularities and incidents, have been a topic of interest in the nuclear industry for several decades. Interest in ATF technology surged following the 2011 accident at Fukushima Daiichi in Japan. At the Advanced Test Reactor (ATR), one of Idaho National Laboratory’s (INL) four operating nuclear reactors, the ATF program is a collaborative effort between the national laboratory and various stakeholders within the nuclear industry. This program focuses on the research and development of novel fuel compositions, cladding, and component materials with enhanced accident-resistant properties. During one of ATR’s 60-day operating cycles in 2024, the reactor experienced five unplanned shutdowns. Following the fifth shutdown, radiation monitors detected an increase in radiation levels coming from the loop piping. Subsequent water samples confirmed the cause was a leak of fission products from the ATF experiment, designated as ATF-2C. The source of the leak was identified as the instrumented section of the test train. The primary discussions in this presentation are 1) the design of the ATF test train, 2) the operating parameters leading up to and following the detection of the leak, and 3) the quantification and characterization of the released fission products.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Performance-based simulants for Hanford radioactive waste treatment process testing

Radioactive wastes from nuclear fuel processing are stored in large underground storage tanks at the Hanford Nuclear Reservation. Treatment and remediation require that waste feed from the storage tanks be delivered to the Hanford Tank Waste Treatment and Immobilization Plant continually for the duration of the treatment mission. Furthermore, the complex physical and chemical processes required for this mission, the significant scale, and the hazardous nature of the waste necessitate the use of simulants in process testing. A new class of simulants, “performance-based simulants,” has been developed to match the process performance of the simulant to actual waste performance data.

Hanford tank waste treatment↗

Application of Dynamical System Scaling for Accelerated Fuel Qualification Efforts

There are considerable ongoing research and testing campaigns to qualify new fuel designs such as metallic fuels for advanced reactor designs and the Accident Tolerant Fuel (ATF) campaign for light water reactors (LWR). The typical research and development lifecycle needed to qualify a nuclear fuel design, under ideal conditions, can take up to 20-25 years which limits the ability for new fuels to make fast deployments into commercial, test, and research reactors. While there are several efforts to accelerate nuclear fuel qualification through advanced modeling coupled with state-of-the-art experiments, there is not yet a framework to methodically quantify and rank distortions occurring in experimental test specimens needed to validate nuclear fuel performance codes. This study uses the Dynamical System Scaling (DSS) methodology to quantify transient scaling distortions that occur over experiment and simulated transients. DSS analysis metrics provide a researcher with several tools and information embedded within test data to identify dominant phenomena, associated timescales, and quantify a transient?s overall dynamic distortion. This is demonstrated with separate analyses of the SETH-C and CHF-SERTTA thermal-hydraulic experiments in the TREAT facility at Idaho National Laboratory. The outcome of this work is a scaling and data analysis approach to account for the influence a scaled fuel test specimen?s geometric and temporal distortions have on its ability to be representative of the full-scale design.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

High-burnup fuel stress analysis prior to and during a LOCA transient

High-burnup fuel fragmentation and pulverization have been experimentally observed during simulated loss-of-coolant accident (LOCA) transient testing of high-burnup (>62 GWd/tU) nuclear fuel. The cause of this phenomenon is generally accepted to be the formation of stresses arising from the off-normal conditions. However, the primary mechanism(s) contributing to the stress formation is/are still being debated. Leading hypotheses suggest that the concurrence of fission gas bubbles and high burnup structure on the pellet periphery (i.e., the rim) leave the fuel susceptible to pulverization. Other hypotheses suggest that pulverization is artificially inflated during externally heated tests that do not reproduce prototypic fuel stresses and radial temperature profiles as the fuel transitions from full-power nuclear heating to decay heating. This work performs finite element analyses of fuel pellet temperatures and macroscopic stresses prior to and during a LOCA transient to identify (1) operating conditions that may exacerbate the fuel pellet stress state, (2) differences in predicted stresses with nuclear vs. furnace heating, and (3) how fuel cracking impacts the subsequent stress state in the pellet fragments. Analyses predict that macroscopic transient fuel stresses resulting from constrained thermal expansion will remain below the fracture stress of fresh UO 2 once the fragment size reaches ~4 mm or less. Calculated fuel stresses from simulated LOCA tests performed with representative nuclear vs. electrical heating rates are shown to be equal within 5% and essentially unchanged for all times after the first 27 seconds of the transients. Because the fuel stresses do not change once the temperature profile becomes uniform, macroscopic transient stresses would be no different than those following a normal shutdown. Because pulverization of high burnup fuel does not occur prior to a LOCA test, pulverization of high burnup UO 2 cannot be initiated by differential thermal stresses.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Status of the Fuel Fragment Dispersal Studies at Oak Ridge National Laboratory

During a loss-of-coolant accident, a nuclear fuel rods undergo balloon and burst. High burnup fuel is known to fragment and pulverize leading to the potential for the fuel to disperse through the burst opening either during the initial burst or following the burst during the reflood event. This milestone summarizes the design and assembly of a system to study dispersal in a postburst event. Surrogate fuel material (HfO 2 , tungsten, and yttria-stabilized zirconia [YSZ]) dispersing from as-burst loss-of-coolant accident (LOCA) test specimens was extensively investigated, along with dispersal of actual nuclear fuel following a LOCA Severe Accident Test Station (SATS) test.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Status of the Fuel Fragment Dispersal Studies at Oak Ridge National Laboratory

During a loss-of-coolant accident, a nuclear fuel rods undergo balloon and burst. High burnup fuel is known to fragment and pulverize leading to the potential for the fuel to disperse through the burst opening either during the initial burst or following the burst during the reflood event. This milestone summarizes the design and assembly of a system to study dispersal in a postburst event. Surrogate fuel material (HfO2, tungsten, and yttria-stabilized zirconia [YSZ]) dispersing from as-burst loss-of-coolant accident (LOCA) test specimens was extensively investigated, along with dispersal of actual nuclear fuel following a LOCA Severe Accident Test Station (SATS) test. Surrogate material tests spanned a variety of burst geometries, particle types, particle size distributions, and rod oscillation loadings (frequency and amplitude combinations).

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Completion and Testing of a New High-Temperature Cell Holder to Support High Dose Rate Electron Beam Irradiations of Select Sulfur Chlorides (S2Cl2 and SOCl2) for Advanced Low Temperature Chlorination of Zirconium-based Used Nuclear Fuel Cladding

Short communication on the completion and testing of a new high-temperature cell holder to support high dose rate electron beam irradiations of select sulfur chlorides (S2Cl2 and SOCl2) for advanced low temperature chlorination of zirconium-based used nuclear fuel cladding.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

NRAD Program Presentation

This is a PowerPoint presentation highlighting the Idaho National Laboratory's Neutron Radiography Reactor, NRAD, programmatic capabilities, neutron radiography quality assurance requirements, and examples of resulting training, informational, and typical radiographic capabilities for nondestructive testing of irradiated nuclear reactor fuels.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

The MPACT 2020 Milestone: Safeguards and Security by Design of Future Nuclear Fuel Cycle Facilities.

The Materials Protection, Accounting, and Control Technologies (MPACT) campaign, within the U.S. Department of Energy Office of Nuclear Energy, has developed a Virtual Facility Distributed Test Bed for safeguards and security design for future nuclear fuel cycle facilities. The purpose of the Virtual Test Bed is to bring together experimental and modeling capabilities across the U.S. national laboratory and university complex to provide a one-stop-shop for advanced Safeguards and Security by Design (SSBD). Experimental testing alone of safeguards and security technologies would be cost prohibitive, but testbeds and laboratory processing facilities with safeguards measurement opportunities, coupled with modeling and simulation, provide the ability to generate modern, efficient safeguards and security systems for new facilities. This Virtual Test Bed concept has been demonstrated using a generic electrochemical reprocessing facility as an example, but the concept can be extended to other facilities. While much of the recent work in the MPACT program has focused on electrochemical safeguards and security technologies, the laboratory capabilities have been applied to other facilities in the past (including aqueous reprocessing, fuel fabrication, and molten salt reactors as examples). This paper provides an overview of the Virtual Test Bed concept, a description of the design process, and a baseline safeguards and security design for the example facility. Parallel papers in this issue go into more detail on the various technologies, experimental testing, modeling capabilities, and performance testing.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

EDS Analysis of FCCI in AFC-FAST Fuel Pins

The Advanced Fuel Campaign’s Fission Accelerated Steady-state Testing (FAST) program uses metallic fuel pins with small diameters to reach a desired burnup more quickly. This enables accelerated testing of advanced fuel designs and decreases the time between idea conception and commercial usage. Post-irradiation examination is critical in this process, especially with respect to the fuel-cladding chemical interactions (FCCI). In this work, energy dispersive X-ray spectroscopy (EDS) is used to track how elements from the fuel and fission products have diffused through the cladding. Elemental redistribution along the fuel-cladding interface is mapped and FCCI region thicknesses are measured. The correlations between geometry, temperature, burnup, and FCCI thickness are presented.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Progress Report on Mockup Irradiation Capsule Fuel Measurements at LANSCE

Irradiation tests are a key component of nuclear fuel development and identifying typical and atypical regions in the irradiated fuel volume relies on very few characterization techniques. The goal of the effort reported here is to provide complementary measurements adding to the available parameter space for post irradiation examination as well as to inform subsequent hot cell PIE examinations by identifying typical and atypical regions with respect to microstructure, tomographic data, or isotope densities. Pulsed neutrons, enabling diffraction as well as energy-resolved neutron imaging and neutron absorption resonance spectroscopy, offer unique capabilities for this purpose. Time-of-flight neutron diffraction has the potential to offer efficient, non-destructive and non-contact microstructural characterization of irradiated fuel specimen with spatial resolution of 1 mm 3 to 1 cm 3 while for energy-resolved neutron imaging (and by extension tomography) a resolution of 100 μm 3 was demonstrated. The potential results include crystallinity vs. amorphous volumes and microstructural information such as phase compositions, lattice strains (indicative of residual stresses or chemistry variations) and textures from the diffraction data as well as distances (e.g. pellet to cladding), cracks, and isotope densities of minor actinides, fission products as well as fission gas partial pressures e.g. in the plenum from energy resolved neutron imaging.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Accelerated Irradiation Testing and Post-Irradiation Characterization: U.S.-Based Capabilities for Advanced Nuclear Systems and Radioisotope Production

Irradiation experiments and post-irradiation examinations, together referred to as irradiation testing (IRT), are prerequisites for nuclear fuel and material qualification for the deployment of new and advanced reactors, as well as radioisotope production, thereby ensuring regulatory compliance. Qualified research and test reactors (RTRs) and testing facilities are essential to enable IRT to verify performance and safety under prototypical reactor conditions. In the past, qualification of new fuels or structural materials required about 20 years. Synergist strategies, advanced tools, and qualified methods are needed to greatly reduce this timeframe of IRT and radioisotope production. This study, termed accelerated-IRT, focuses on identifying gaps and leveraging U.S.-based RTRs and material testing capabilities, leveraging the preliminary evaluation and qualification of selected RTRs to provide a generic as well as specific-case solution paths forward, ensuring adherence to stringent regulatory standards. Furthermore, IRT and radioisotope production utilizing qualified RTRs necessarily includes modeling and simulation to support the design (i.e. neutronics, thermal, and structural aspects) and manufacturing of irradiation test specimens, vehicles, capsules, apparatuses, and flow loops. In addition, IRT can be improved by applying advanced manufacturing techniques and in-pile sensors and instrumentation, as discussed in this study.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

High-temperature irradiation-resistant thermocouple instability model for in-pile reactor use

This article presents an instability model for the high-temperature irradiation-resistant thermocouple (HTIR-TC). Here the term instability defines the superposition of both drift and inhomogeneity of TC thermoelements occurring simultaneously. The HTIR-TC is an advanced thermocouple (TC) that uses the refractory metals niobium and molybdenum as sensing thermoelements for generating electromotive force (EMF) in a field of neutrons and at temperatures upward of 1,600°C. In the Advanced Gas Reactor (AGR) 5/6/7 tests conducted at Idaho National Laboratory’s Advanced Test Reactor (ATR), the HTIR-TCs showed low to moderate instability throughout the life of the test. The instability model reveals that HTIR-TCs can, when the operating temperature of the reactor fuel is normal, maintain performance throughout an 18-month refueling cycle typical of nuclear power plants, reflecting an instability of less than ±1%. The HTIR-TC is also qualified for incorporation into a test fixture during the testing of new fuels.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Coupled chemical–CFD modeling of unsealed dry storage of advanced test reactor spent fuel

We report given the current lack of long-term disposal for spent nuclear fuel storage in the United States, the current inventory of advanced test reactor (ATR) fuel at Idaho National Laboratory (INL) is expected to be stored in a dry storage facility for an extended storage period. As part of an effort to understand the conditions during a 50-year period, a three-dimensional computational fluid dynamics (CFD) of the unsealed canisters packed with spent fuel in the storage facility was constructed, this CFD model is coupled with radiolytic chemical reactions associated with water vapor and other species. The coupled model is simulated over a range of sensitivity parameters for the fuel decay heat, relative humidity, and oxyhydroxide film thickness for undried and fully-dried fuel. The most important parameter was the initial fuel decay heat. Over the range of cases, the hydrogen and nitric acid concentrations are low enough no significant impact is expected.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Estimation of post-burst vibration-induced fuel dispersal thresholds following LOCA-simulant testing

The nuclear industry intends to increase burnup past the regulatory limit of 62 GWd/MTU, and to be successful, the dispersal behavior of fragmented high-burnup fuel during loss-of-coolant accidents must be better understood. Part of this behavior is fuel fragmentation, relocation, and dispersal. This work reports on testing concerning the dispersal of fuel from rods following burst and pressure blowdown through the burst. The Fuel Relocation Induced by Accident Recovery (FRIAR) system was used to examine surrogate material and pre-burst cladding specimens to evaluate the effects of vibrational loading, mixture composition, and burst size on post-burst dispersal. Vibrational loading resulted in maximum dispersal around 15 Hz when the loading was performed with peak-to-peak oscillation amplitudes at 0.5 and 1 mm. Here, under this aggressive vibrational loading, dispersal was found to become significant as burst widths increased to approximately 5 mm and larger. However, below 4 mm widths, little material dispersed out of the opening, even at 1 mm amplitudes and for more dispersive mixtures (smaller average fragments). At and above 7 mm widths, dispersal was rapid for all mixtures. Finally, dispersal in the threshold region (4–5 mm wide bursts) strongly depended on the mixture. For mixtures with large fragments, dispersal was minimized to a few fragments, as the large fragments proved to be effective at minimizing dispersal. Conversely, mixtures with smaller fragments showed increased dispersal in this region.

Burst geometry↗

MFC Transient Testing and Fuel Fabrication Capabilities

MFC Transient Testing Capabilities and Fuel Fabrication capabilities are summarized in this slide deck. Slides are included for TREAT and TREAT capabilities, EFF, FASB, FMF, ZPPR, AFF, and the Fuels Fabrication Modernization Capability. First use of this slide deck is for presentation at Westinghouse Electric Corporation, but there will be other uses later.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Post-irradiation 1600°C Heating Test of AGR-1 UCO Fuel Kernels

The Advanced Gas Reactor Fuel Development and Qualification (AGR) Program was established to perform research and development on tristructural isotropic (TRISO) coated-particle fuel to support deployment of high temperature gas-cooled reactors (HTGRs) . This talk will discuss the results from a post-irradiation heating test of five individual fuel kernels extracted from four TRISO fuel particles that were deconsolidated from an irradiated AGR-1 fuel compact.

heating test↗