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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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NASA NTRS2007

Identification of Stratospheric Waves in Ozone in the Tropics from OMI High Spectral Resolution Measurements

Previous studies using Total Ozone Mapping Spectrometer (TOMS) measurements have identified several types of tropical waves in the stratosphere. These waves include Kelvin waves, mixed Rossby-gravity waves, equatorial Rossby waves, and global normal modes. All of these detected waves occur when their zonal phase speeds are opposite the zonal winds in the low-mid stratosphere associated with the Quasi-biennial Oscillation (QBO). Peak-to-peak amplitudes in all cases are typically 5 DU. While total ozone data from TOMS is sensitive in detecting these tropical waves, they provide each day only a single horizontal cross-sectional map. The high spatial and spectral resolution of the Aura Ozone Monitoring Instrument (OMI) provides a unique means to evaluate 3D structure in these waves including their propagation characteristics. Ozone profiles retrieved from OMI radiances for wavelengths 270-310 nm are utilized to examine the nature of these wave disturbances extending from the lower to upper stratosphere.

Ziemke, J. R.↗
NASA NTRS2007

What You Need to Know About the OMI NO2 Data Product for Air Quality Studies

The standard nitrogen dioxide (NO2) data product, produced from measurements by the Ozone Monitoring Instrument (OMI), are publicly available online from the NASA GESDISC facility. Important data fields include total and tropospheric column densities, as well as collocated data for cloud fraction and cloud top height, surface albedo and snow/ice coverage, at the resolution of the OMI instrument (12 km x 26 km, at nadir). The retrieved NO2 data have been validated, principally under clear-sky conditions. The first public-release version has been available since September 2006. An improved version of the data product, which includes a number of new data fields, and improved estimates of the retrieval uncertainties will be released by the end of 2007. This talk will describe the standard NO2 data product, including details that are essential for the use of the data for air quality studies. We will also describe the principal improvements with the new version of the data product.

Celarier, E. A.↗
NASA NTRS2010

Application of OMI Observations to a Space-Based Indicator of NOx and VOC Controls on Surface Ozone Formation

We investigated variations in the relative sensitivity of surface ozone formation in summer to precursor species concentrations of volatile organic compounds (VOCs) and nitrogen oxides (NOx) as inferred from the ratio of the tropospheric columns of formaldehyde to nitrogen dioxide (the "Ratio") from the Aura Ozone Monitoring Instrument (OMI). Our modeling study suggests that ozone formation decreases with reductions in VOCs at Ratios less than 1 and NOx at Ratios greater than 2; both NOx and VOC reductions may decrease ozone formation for Ratios between 1 and 2. Using this criteria. the OMI data indicate that ozone formation became: 1. more sensitive to NOx over most of the United States from 2005 to 2007 because of the substantial decrease in NOx emissions, primarily from stationary sources, and the concomitant decrease in the tropospheric column of NO2. and 2. more sensitive to NOx with increasing temperature, in part because emissions of highly reactive, biogenic isoprene increase with temperature, thus increasing the total VOC reactivity. In cities with relatively low isoprene emissions (e.g .. Chicago). the data clearly indicate that ozone formation became more sensitive to NOx from 2005 to 2007. In cities with relatively high isoprene emissions (e.g ., Atlanta), we found that the increase in the Ratio due to decreasing NOx emissions was not obvious as this signal was convolved with variations in the Ratio associated with the temperature dependence of isoprene emissions and, consequently, the formaldehyde concentration.

Duncan, Bryan N.↗
NASA NTRS2011

DISCOVER-AQ: An Overview and Initial Comparisons of NO2 with OMI Observations

The first deployment of the Earth Venture -1 DISCOVER-AQ (Deriving Information on Surface conditions from Column and Vertically Resolved Observations Relevant to Air Quality) project was conducted during July 2011 in the Baltimore-Washington region. Two aircraft (a P-3B for in-situ sampling and a King Air for remote sensing) were used along with an extensive array of surface-based in-situ and remote sensing instrumentation. Fourteen flight days were accomplished by both aircraft and over 250 profiles of trace gases and aerosols were performed by the P-3B over surface air quality monitoring stations, which were specially outfitted with sunphotometers and Pandora UV/Vis spectrometers. The King Air flew with the High Spectral Resolution Lidar for aerosols and the ACAM UV/Vis spectrometer for trace gases. This suite of observations allows linkage of surface air quality with the vertical distributions of gases and aerosols, with remotely-sensed column amounts observed from the surface and from the King Air, and with satellite observations from Aura (OMI and TES), GOME-2, MODIS and GOES. The DISCOVER-AQ data will allow determination of under what conditions satellite retrievals are indicative of surface air quality, and they will be useful in planning new satellites. In addition to an overview of the project, a preliminary comparison of tropospheric column NO2 densities from the integration of in-situ P-3B observations, from the Pandoras and ACAM, and from the new Goddard OMI NO2 algorithm will be presented.

Pickering, Kenneth↗
NASA NTRS2012

A New Retrieval Algorithm for OMI NO2: Tropospheric Results and Comparisons with Measurements and Models

Nitrogen oxides (NOx =NO+NO2) are important atmospheric trace constituents that impact tropospheric air pollution chemistry and air quality. We have developed a new NASA algorithm for the retrieval of stratospheric and tropospheric NO2 vertical column densities using measurements from the nadir-viewing Ozone Monitoring Instrument (OMI) on NASA's Aura satellite. The new products rely on an improved approach to stratospheric NO2 column estimation and stratosphere-troposphere separation and a new monthly NO2 climatology based on the NASA Global Modeling Initiative chemistry-transport model. The retrieval does not rely on daily model profiles, minimizing the influence of a priori information. We evaluate the retrieved tropospheric NO2 columns using surface in situ (e.g., AQS/EPA), ground-based (e.g., DOAS), and airborne measurements (e.g., DISCOVER-AQ). The new, improved OMI tropospheric NO2 product is available at high spatial resolution for the years 200S-present. We believe that this product is valuable for the evaluation of chemistry-transport models, examining the spatial and temporal patterns of NOx emissions, constraining top-down NOx inventories, and for the estimation of NOx lifetimes.

Swartz, W. H.↗
NASA NTRS2016

Interpreting the Ultraviolet Aerosol Index Observed with the OMI Satellite Instrument to Understand Absorption by Organic Aerosols: Implications for Atmospheric Oxidation and Direct Radiative Effects

Satellite observations of the ultraviolet aerosol index (UVAI) are sensitive to absorption of solar radiation by aerosols; this absorption affects photolysis frequencies and radiative forcing. We develop a global simulation of the UVAI using the 3-D chemical transport model GEOSChem coupled with the Vector Linearized Discrete Ordinate Radiative Transfer model (VLIDORT). The simulation is applied to interpret UVAI observations from the Ozone Monitoring Instrument (OMI) for the year 2007. Simulated and observed values are highly consistent in regions where mineral dust dominates the UVAI, but a large negative bias (-0.32 to -0.97) exists between simulated and observed values in biomass burning regions. We determine effective optical properties for absorbing organic aerosol, known as brown carbon (BrC), and implement them into GEOS-Chem to better represent observed UVAI values over biomass burning regions. The inclusion of absorbing BrC decreases the mean bias between simulated and OMI UVAI values from -0.57 to -0.09 over West Africa in January, from -0.32 to +0.0002 over South Asia in April, from -0.97 to -0.22 over southern Africa in July, and from -0.50 to +0.33 over South America in September. The spectral dependence of absorption after including BrC in the model is broadly consistent with reported observations for biomass burning aerosol, with absorbing Angstrom exponent (AAE) values ranging from 2.9 in the ultraviolet (UV) to 1.3 across the UV-Near IR spectrum. We assess the effect of the additional UV absorption by BrC on atmospheric photochemistry by examining tropospheric hydroxyl radical (OH) concentrations in GEOS-Chem. The inclusion of BrC decreases OH by up to 30% over South America in September, up to 20% over southern Africa in July, and up to 15% over other biomass burning regions. Global annual mean OH concentrations in GEOS-Chem decrease due to the presence of absorbing BrC, increasing the methyl chloroform lifetime from 5.62 to 5.68 years, thus reducing the bias against observed values. We calculate the direct radiative effect (DRE) of BrC using GEOS-Chem coupled with the radiative transfer model RRTMG (GC-RT). Treating organic aerosol as containing more strongly absorbing BrC changes the global annual mean all-sky top of atmosphere (TOA) DRE by +0.03Wm(exp -2) and all-sky surface DRE by -0.08Wm(exp -2). Regional changes of up to +0.3Wm(exp -2) at TOA and down to -1.5Wm(exp -2) at the surface are found over major biomass burning regions.

Air Pollution↗
NASA NTRS2016

A Ten-Year Global Record of Absorbing Aerosols Above Clouds from OMI's Near-UV Observations

Aerosol-cloud interaction continues to be one of the leading uncertain components of climate models, primarily due to the lack of an adequate knowledge of the complex microphysical and radiative processes associated with the aerosol-cloud system. The situations when aerosols and clouds are found in the same atmospheric column, for instance, when light-absorbing aerosols such as biomass burning generated carbonaceous particles or wind-blown dust overlay low-level cloud decks, are commonly found over several regional of the world. Contrary to the cloud-free scenario over dark surface, for which aerosols are known to produce a net cooling effect (negative radiative forcing) on climate, the overlapping situation of absorbing aerosols over cloud can potentially exert a significant level of atmospheric absorption and produces a positive radiative forcing at top-of-atmosphere. The magnitude of direct radiative effects of aerosols above cloud depends directly on the aerosol loading, microphysical-optical properties of the aerosol layer and the underlying cloud deck, and geometric cloud fraction. We help in addressing this problem by introducing a novel product of optical depth of absorbing aerosols above clouds retrieved from near-UV observations made by the Ozone Monitoring Instrument (OMI) on board NASA's Aura platform. The presence of absorbing aerosols above cloud reduces the upwelling radiation reflected by cloud and produces a strong 'color ratio' effect in the near-UV region, which can be unambiguously detected in the OMI measurements. Physically based on this effect, the OMACA algorithm retrieves the optical depths of aerosols and clouds simultaneously under a prescribed state of atmosphere. The algorithm architecture and results from a ten-year global record including global climatology of frequency of occurrence and above-cloud aerosol optical depth, and a discussion on related future field campaigns are presented.

Ozone Monitoring Instrument↗
NASA NTRS2016

Solar Spectral Irradiance Variability in Cycle 24: Model Predictions and OMI Observations

Utilizing the excellent stability of the Ozone Monitoring Instrument (OMI), we characterize both short-term (solar rotation) and long-term (solar cycle) changes of the solar spectral irradiance (SSI) between 265-500 nanometers during the ongoing Cycle 24. We supplement the OMI data with concurrent observations from the GOME-2 (Global Ozone Monitoring Experiment - 2) and SORCE (Solar Radiation and Climate Experiment) instruments and find fair-to-excellent agreement between the observations and predictions of the NRLSSI2 (Naval Research Laboratory Solar Spectral Irradiance - post SORCE) and SATIRE-S (the Naval Research Laboratory's Spectral And Total Irradiance REconstruction for the Satellite era) models.

Sun↗
NASA NTRS2018

Mission Operations Working Group (MOWG) Report to the OMI Science Team

This PowerPoint presentation will discuss Aura's current spacecraft and OMI insturment status, highlight anyperformance trends and impacts to OMI operations, identify any operational changes and express concerns or potential process improvements. Reviewed by Eric Moyer, ESMO Deputy Project Manager.

Aura Mission Status↗
NASA NTRS2019

Learning from GES DISC's MLS and OMI Data Users: Metrics Matter

It has been over 15 years since Aura research satellite launched in 2004 to observe the Earth's ozone layer, air quality, and climate from four different instruments - the High Resolution Dynamics Limb Sounder (HIRDLS), the Microwave Limb Sounder (MLS), the Ozone Monitoring Instrument (OMI), and the Tropospheric Emission Spectrometer (TES). Observations from the Aura mission have established a concrete understanding of the changing chemistry of our atmosphere.The NASA Goddard Earth Sciences Data and Information Services Center (GES DISC) is the official archive and distribution center for the HIRDLS, MLS, and OMI instruments. This presentation will report metrics of data usage and services on these instruments. Key to GES DISC's mission to provide better data support is gaining a better understanding of our users' needs and behaviors as they discover, access and utilize these data. We will summarize the users' needs from these instruments based on user inquiry information collected over the Aura mission lifetime and present findings from this ensemble metrics.

Metrics↗
NASA NTRS2019

Lightning NOx Production in the Tropics as Determined Using OMI NO2 Retrievals and WWLLN Stroke Data

Nitrogen oxide (NOx) production by lightning in the tropics is estimated using tropospheric NOx amounts (LNOx*) over deep convective grid boxes derived from OMI (Ozone Monitoring Instrument) nitrogen dioxide (NO2) slant columns and detection efficiency adjusted WWLLN (World Wide Lightning Location Network) flashes. The lightning NOx production efficiency (LNOx PE) in the tropics is determined for the austral and boreal summers of 2007 to 2011 by regressing regional mean daily values of LNOx* for individual seasons against daily flash totals during flash windows prior to the OMI overpass. LNOx PE is determined to be approximately two times larger over marine locations than over continental locations possibly because marine flashes are more energetic. Overall, the mean LNOx PE for the tropics is calculated to be 170 ± 100 mol per flash with values over the tropical Pacific (low flash rate region) being largest. The main contributors to uncertainties in PE are uncertainties in WWLLN flash detection efficiency, upper tropospheric NOx lifetime in the near field of convection, and air mass factor biases.

Dale J. Allen↗
NASA NTRS2020

Synergistic Use of Hyperspectral UV-Visible OMI and Broadband Meteorological Imager MODIS Data for a Merged Aerosol Product

The retrieval of optimal aerosol datasets by the synergistic use of hyperspectral ultraviolet(UV)–visible and broadband meteorological imager (MI) techniques was investigated. The Aura Ozone Monitoring Instrument (OMI) Level 1B (L1B) was used as a proxy for hyperspectral UV–visible instrument data to which the Geostationary Environment Monitoring Spectrometer (GEMS) aerosol algorithm was applied. Moderate-Resolution Imaging Spectroradiometer (MODIS) L1B and dark target aerosol Level 2 (L2) data were used with a broadband MI to take advantage of the consistent time gap between the MODIS and the OMI. First, the use of cloud mask information from the MI infrared (IR) channel was tested for synergy. High-spatial-resolution and IR channels of the MI helped mask cirrus and sub-pixel cloud contamination of GEMS aerosol, as clearly seen in aerosol optical depth (AOD) validation with Aerosol Robotic Network (AERONET) data. Second, dust aerosols were distinguished in the GEMS aerosol-type classification algorithm by calculating the total dust confidence index (TDCI) from MODIS L1B IR channels. Statistical analysis indicates that the Probability of Correct Detection (POCD) between the forward and inversion aerosol dust models (DS) was increased from 72% to 94% by use of the TDCI for GEMS aerosol-type classification, and updated aerosol types were then applied to the GEMS algorithm. Use of the TDCI for DS type classification in the GEMS retrieval procedure gave improved single-scattering albedo (SSA) values for absorbing fine pollution particles (BC) and DS aerosols. Aerosol layer height (ALH) retrieved from GEMS was compared with Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) data, which provides high-resolution vertical aerosol profile information. The CALIOP ALH was calculated from total attenuated backscatter data at 1064 nm, which is identical to the definition of GEMS ALH. Application of the TDCI value reduced the median bias of GEMS ALH data slightly. The GEMS ALH bias approximates zero, especially for GEMS AOD values of>~0.4 and GEMS SSA values of<~0.95.Finally, the AOD products from the GEMS algorithm and MI were used in aerosol merging with the maximum-likelihood estimation method, based on a weighting factor derived from the standard deviation of the original AOD products. With the advantage of the UV–visible channel in retrieving aerosol properties over bright surfaces, the combined AOD products demonstrated better spatial data availability than the original AOD products, with comparable accuracy. Furthermore, pixel-level error analysis of GEMS AOD data indicates improvement through MI synergy.

aerosol↗
NASA NTRS2019

Midlatitude Lightning NOx Production Efficiency Inferred From OMI and WWLLN Data

Oxides of nitrogen are critical trace gases in the troposphere and are precursors for nitrate aerosol and ozone, which is an important pollutant and greenhouse gas. Lightning is the major source of NOx(NO + NO2) in the mid-to upper troposphere. We estimate the production efficiency (PE) of lightning NOx (LNOx) using satellite data from the Ozone Monitoring Instrument (OMI) and the ground-based WorldWide Lightning Location Network (WWLLN) in three northern midlatitude, primarily continental regions that include much of North America, Europe and East Asia. Data were obtained over 5 boreal summers, 2007 –2011 and comprise the largest number of midlatitude convective events to date for estimating the LNOx PE with satellite NO2and ground-based lightning measurements. In contrast to some previous studies, the algorithm assumes no minimum flash-rate threshold and estimates freshly produced LNOxby subtracting a background of aged NOx estimated from the OMI dataset itself. We infer an average value of 180 ± 100 moles LNOx produced per lightning flash. We also show evidence of a dependence of PE on lightning flash rate and find an approximate empirical power function relating moles LNOxto flashes. PE decreases by an order of magnitude for a 2-order of magnitude increase in flash rate. This phenomenon has not been reported in previous satellite LNOxstudies but is consistent with ground-based observations suggesting an inverse relationship between flash rate and size.

LNOx↗
NASA NTRSDate not supplied

Has NO(2) in Metropolitan Areas Returned to Pre-COVID-19 Levels as Measured by OMI Satellite Data?

Nitrogen oxides (NOx = NO + NO2) are primarily emitted through the combustion of fossil fuels, such as automobiles and power plants. NOx can contribute to chemical reactions that produce ozone and fine particulate matter (PM2.5) pollution. Using tropospheric vertical column density (TVCD) NO2 data from satellite hyperspectral instruments, such as the Ozone Monitoring Instrument (OMI) on board NASA’s EOS Aura satellite, one can monitor changes in NO2 pollution during “black-swan” events, such as mobility restrictions during COVID-19 lockdowns. Our OMI team has created the Global Nitrogen Dioxide Monitoring Home Page (https://so2.gsfc.nasa.gov/no2/no2_index.html ) where we display NO2 TVCD time series, animated maps, and COVID-specific NO2 anomalies comparing to a pre-COVID five-year average for 317 cities and regions around the world. During the pandemic as a result of the widespread lockdowns, many areas saw low NO2 anomalies superimposed on the natural weather related NO2 changes, such as seasonal NO2 cycle. Has NO2 levels returned to pre-Covid-19 levels in large metropolitan areas? We analyze NO2 time series from March through September for the years 2020-2023 using as a reference the average NO2 from 2015-2019 for those months. We will present data from selected cities that represent all countries.

Keith D Evans↗
NASA NTRS2013

Impact of NO2 Profile Shape in OMI Tropospheric NO2 Retrievals

Nitrogen oxides (NOx NO + NO2) are key actors in air quality and climate change. Tropospheric NO2 columns from the nadir-viewing satellite sensors have been widely used to understand sources and chemistry of NOx. We have implemented several improvements to the operational algorithm developed at NASA GSFC and retrieved tropospheric NO2 columns. We present tropospheric NO2 validation studies of the new OMI Standard Product version 2.1 using ground-based and in-situ aircraft measurements. We show how vertical profile of scattering weight and a-priori NO2 profile shapes, which are taken from chemistry-transport models, affect air mass factor (AMF) and therefore tropospheric NO2 retrievals. Users can take advantage of scattering weights information that is made available in the operational NO2 product. Improved tropospheric NO2 data retrieved using thoroughly evaluated high spatial resolution NO2 profiles are helpful to test models.

OMI↗
NASA NTRS2014

Satellite Monitoring Over the Canadian Oil Sands: Highlights from Aura OMI and TES

Satellite remote sensing provides a unique perspective for air quality monitoring in and around the Canadian Oil Sands as a result of its spatial and temporal coverage. Presented are Aura satellite observations of key pollutants including nitrogen dioxide (NO2), sulfur dioxide (SO2), carbon monoxide (CO), ammonia (NH3), methanol (CH3OH), and formic acid (HCOOH) over the Canadian Oil Sands. Some of the highlights include: (i) the evolution of NO2 and SO2 from the Ozone Monitoring Instrument (OMI), including comparisons with other nearby sources, (ii) two years of ammonia, carbon monoxide, methanol, and formic acid observations from 240 km North-South Tropospheric Emission Spectrometer (TES) transects through the oils sands, and (iii) preliminary insights into emissions derived from these observations.

NO2↗
NASA NTRS2015

Estimates of Power Plant NOx Emissions and Lifetimes from OMI NO2 Satellite Retrievals

Isolated power plants with well characterized emissions serve as an ideal test case of methods to estimate emissions using satellite data. In this study we evaluate the Exponentially-Modified Gaussian (EMG) method and the box model method based on mass balance for estimating known NOx emissions from satellite retrievals made by the Ozone Monitoring Instrument (OMI). We consider 29 power plants in the USA which have large NOx plumes that do not overlap with other sources and which have emissions data from the Continuous Emission Monitoring System (CEMS). This enables us to identify constraints required by the methods, such as which wind data to use and how to calculate background values. We found that the lifetimes estimated by the methods are too short to be representative of the chemical lifetime. Instead, we introduce a separate lifetime parameter to account for the discrepancy between estimates using real data and those that theory would predict. In terms of emissions, the EMG method required averages from multiple years to give accurate results, whereas the box model method gave accurate results for individual ozone seasons.

Emissions inventory↗
NASA NTRS2014

Exploring NASA OMI Level 2 Data With Visualization

Satellite data products are important for a wide variety of applications that can bring far-reaching benefits to the science community and the broader society. These benefits can best be achieved if the satellite data are well utilized and interpreted, such as model inputs from satellite, or extreme events (such as volcano eruptions, dust storms, etc.).Unfortunately, this is not always the case, despite the abundance and relative maturity of numerous satellite data products provided by NASA and other organizations. Such obstacles may be avoided by allowing users to visualize satellite data as images, with accurate pixel-level (Level-2) information, including pixel coverage area delineation and science team recommended quality screening for individual geophysical parameters. We present a prototype service from the Goddard Earth Sciences Data and Information Services Center (GES DISC) supporting Aura OMI Level-2 Data with GIS-like capabilities. Functionality includes selecting data sources (e.g., multiple parameters under the same scene, like NO2 and SO2, or the same parameter with different aggregation methods, like NO2 in OMNO2G and OMNO2D products), user-defined area-of-interest and temporal extents, zooming, panning, overlaying, sliding, and data subsetting, reformatting, and reprojection. The system will allow any user-defined portal interface (front-end) to connect to our backend server with OGC standard-compliant Web Mapping Service (WMS) and Web Coverage Service (WCS) calls. This back-end service should greatly enhance its expandability to integrate additional outside data-map sources.

Level 2↗