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NASA NTRS1982

Photometry and polarimetry of Titan - Pioneer 11 observations and their implications for aerosol properties

Pioneer 11 measurements of Titan's limb darkening and polarization at red and blue wavelengths are refined, and the integrated disk brightness measurements at phase angles from 22 to 96 deg, over which Titan's phase coefficient averages about 0.014 magnitudes/deg in both colors, are reduced. Comparisons of the data with vertically homogeneous multiple scattering models indicate that the single-scattering phase functions of the aerosols in both colors are flat at scattering angles between 80 and 150 deg, with a small peak at larger scattering angles. Although a vertically homogeneous model in which particles are assumed to scatter as spheres cannot simultaneously match the polarization observations of both colors for any refractive index, observed polarizations are most sensitive to the particle properties near optical depth 1/2 in each color. Models based on single scattering by spheres can therefore be successful over a range of refractive indices, if the size of the particles increases with depth and if the cross section of the particles increases sufficiently rapidly with decreasing wavelength.

Tomasko, M. G.↗

NASA NTRSDate not supplied

X-ray and Multiwavelength Polarization of Mrk 501 Since 2022

We present multiwavelength polarization measurements for the luminous blazar Mrk 501 over a 14-month period. The 2 to 8 keV X-ray polarization was measured with the Imaging X-ray Polarimetry Explorer (IXPE) with six 100-ks observations spanning from March 2022 to June 2023. Each IXPE observation was accompanied with simultaneous X-ray data from NuSTAR, Swift/XRT, or XMM-Newton. Complementary optical polarization measurements were also available in the B,V,R,I, J bands as well as radio polarization measurements from 4.85 GHz to 225.5 GHz. Over the six IXPE observations, we find small to no variability in the X-ray polarization degree and angle with IXPE except for the most recent observation in June 2023 with slightly elevated polarization degree at ~3 sigma above the average of the other five observations. The optical and radio measurements show no apparent correlations to the X-ray polarization properties. This is consistent with the energy-stratified shock scenario established from the first two IXPE observations in which the polarized optical and radio emission is likely from different spatial regions than the polarized X-ray emission.

AGN↗

NASA NTRSDate not supplied

X-ray and Multiwavelength Polarization of Mrk 501 in 2022-2023

AGN↗

NASA NTRS1991

Non-contact temperature measurement

Three methods for noncontact temperature measurement are presented. Ideal gas thermometry is realized by using laser-induced fluorescence to measure the concentration of mercury atoms in a Hg-Ar mixture in the vicinity of hot specimens. Emission polarimetry is investigated by measuring the spatially resolved intensities of polarized light from a hot tungsten sphere. Laser polarimetry is used to measure the optical properties, emissivity, and, in combination with optical pyrometry, the temperature of electromagnetically levitated liquid aluminum. The precision of temperature measurements based on the ideal gas law is + or - 2.6 percent at 1500-2000 K. The polarized emission technique is found to have the capability to determine optical properties and/or spectral emissivities of specimens over a wide range of wavelengths with quite simple instruments.

Nordine, Paul C.↗

DOE OSTI2024

Circularly Polarized Attosecond Pulses Enabled by an Azimuthal Phase and Polarization Grating

High-harmonic generation (HHG) is an extreme nonlinear optical process that can map the properties of an infrared driving laser beam onto short wavelength attosecond pulse trains. However, current techniques for generating circularly polarized high harmonics for probing magnetic materials and chiral systems have limitations: two-color collinear counter-rotating driving lasers result in a low cutoff photon energy, while single-color non-collinear counter-rotating schemes suffer from low conversion efficiency. In this work, we generate circularly polarized attosecond pulse trains by using a structured laser driver which has a rotating polarization and phase grating along the azimuthal coordinate. Furthermore, our experimental and numerical results demonstrate the production of left and right circularly polarized harmonics, which naturally separate upon propagation. Our approach uses a single laser color in a collinear geometry, that can be scaled for high efficiency. Simulations show this scheme can extend into the soft x-ray region when driven by mid-infrared driving lasers, while preserving the same high phase-matching cutoff photon energy as for linearly-polarized high harmonics.

attosecond science↗

NASA NTRS2017

Water-Leaving Contribution to Polarized Radiation Field Over Ocean

The top-of-atmosphere (TOA) radiation field from a coupled atmosphere-ocean system (CAOS) includes contributions from the atmosphere, surface, and water body. Atmo-spheric correction of ocean color imagery is to retrieve water-leaving radiance from the TOA measurement, from which ocean bio-optical properties can be obtained. Knowledge of the ab-solute and relative magnitudes of water-leaving signal in the TOA radiation field is important for designing new atmospheric correction algorithms and developing retrieval algorithms for new ocean biogeochemical parameters. In this paper we present a systematic sensitivity study of water-leaving contribution to the TOA radiation field, from 340 nm to 865 nm, with polarization included. Ocean water inherent optical properties are derived from bio-optical models for two kinds of waters, one dominated by phytoplankton (PDW) and the other by non-algae particles (NDW). In addition to elastic scattering, Raman scattering and fluorescence from dissolved organic matter in ocean waters are included. Our sensitivity study shows that the polarized reflectance is minimized for both CAOS and ocean signals in the backscattering half plane, which leads to numerical instability when calculating water leaving relative contribution, the ratio between polarized water leaving and CAOS signals. If the backscattering plane is excluded, the water-leaving polarized signal contributes less than 9% to the TOA polarized reflectance for PDW in the whole spectra. For NDW, the polarized water leaving contribution can be as much as 20% in the wavelength range from 470 to 670 nm. For wavelengths shorter than 452 nm or longer than 865 nm, the water leaving contribution to the TOA polarized reflectance is in general smaller than 5% for NDW. For the TOA total reflectance, the water-leaving contribution has maximum values ranging from 7% to 16% at variable wavelengths from 400 nm to 550 nm from PDW. The water leaving contribution to the TOA total reflectance can be as large as 35%for NDW, which is in general peaked at 550 nm. Both the total and polarized reflectances from water-leaving contributions approach zero in the ultraviolet and near infrared bands. These facts can be used as constraints or guidelines when estimating the water leaving contribution to the TOA reflectance for new atmospheric correction algorithms for ocean color imagery.

inelastic scatterin↗

NASA NTRS2005

The Solar Ultraviolet Magnetograph Investigation: Polarization Properties

This paper will describe the objectives of the Marshall Space Flight Center (MSFC) Solar Ultraviolet Magnetograph Investigation (SUMI) and the optical components that have been developed to meet those objectives. A sounding rocket payload is being developed to test the feasibility of magnetic field measurements in the Sun s transition region. This paper will review the scientific measurements that will be made by the SUMI sounding rocket program, and the optics have been optimized for simultaneous measurements of two magnetic lines formed in the transition region (CIV at 1550 A and MgII at 2800 A). Finally, this paper will concentrate on the polarization properties of the SUM1 polarimeter and toroidal varied-line-space gratings.

West, E. A.↗

NASA NTRS2018

Polarization Ray Tracing and Polarization Aberration Compensation in Reflective Astronomical Telescopes

Assessing and optimizing polarization performance in the context of ray-based optical design can be challenging. We describe an approach to this problem that decouples polarization effects from optical system geometry for reflective systems. Each surface's polarization properties are parameterized in terms of their impact on retardance and diattenuation in the small angle-of-incidence limit, separating polarization assessment from the task of coating design. A low-resolution ray trace of the system is adequate to determine ray geometry at each interface, which can then be interpolated to rapidly evaluate net Jones Matrix pupil functions. Coating behavior can be easily varied using the ellipsometric parameters to investigate impacts and compensation. Desired values of these parameters can then be specified as constraints in coating design. Investigation with candidate telescope optical designs for LUVOIR show baseline root-mean-square wavefront errors in the nm range for the on-diagonal Jones matrix component, and throughputs of tens of parts per million. Promising possibilities for compensation using a purpose-designed coating on the secondary mirror are discussed, which reduce the on-diagonal wavefront error by a factor 20, with accompanying but more modest reductions in coupling into off-diagonal terms.

Sabatke, Derek↗

DOE OSTI2020

Engineered optical fibers and uses thereof

A system comprises an electromagnetic radiation source, a polarizing element, a mode converter, an optical fiber, and a measurement device. The polarizing element receives electromagnetic radiation produced by the electromagnetic radiation source and outputs linearly-polarized electromagnetic radiation having a linear polarization angle θ1. The mode converter converts the linearly-polarized electromagnetic radiation to an orbital angular momentum (OAM) mode of linearly-polarized electromagnetic radiation with topological charge Li. The OAM mode of linearly-polarized electromagnetic radiation is a superposition of first and second OAM modes with topological charges Li and opposite circular polarizations. The optical fiber supports propagation of the first and second OAM modes with an absolute effective index difference Δneff greater than or equal to 5×10−5, such that linearly-polarized electromagnetic radiation with linear polarization angle θ2 is emitted by the optical fiber. The measurement device is configured to determine a property of the electromagnetic radiation based on the polarization angle θ2.

Ramachandran, Siddharth↗

NASA NTRS1978

Zodiacal light as an indicator of interplanetary dust

The most striking feature of the night sky in the tropics is the zodiacal light, which appears as a cone in the west after sunset and in the east before sunrise. It is caused by sunlight scattered or absorbed by particles in the interplanetary medium. The zodiacal light is the only source of information about the integrated properties of the whole ensemble of interplanetary dust. The brightness and polarization in different directions and at different colors can provide information on the optical properties and spatial distribution of the scattering particles. The zodiacal light arises from two independent physical processes related to the scattering of solar continuum radiation by interplanetary dust and to thermal emission which arises from solar radiation that is absorbed by interplanetary dust and reemitted mainly at infrared wavelengths. Attention is given to observational parameters of zodiacal light, the methods of observation, errors and absolute calibration, and the observed characteristics of zodiacal light.

Weinberg, J. L.↗

NASA NTRS1999

Overview of Photonic Materials for Application in Space Environments

Future space systems will he based on components evolving from the development and refinement of new and existing photonic materials. Optically based sensors, inertial guidance, tracking systems, communications, diagnostics, imaging and high speed optical processing are but a few of the applications expected to widely utilize photonic materials. The response of these materials to space environment effects (SEE) such as spacecraft charging, orbital debris, atomic oxygen, ultraviolet irradiation, temperature and ionizing radiation will be paramount to ensuring successful space applications. The intent of this paper is to, address the latter two environments via a succinct comparison of the known sensitivities of selected photonic materials to the temperature and ionizing radiation conditions found in space and enhanced space environments Delineation of the known temperature and radiation induced responses in LiNbO3, AlGaN, AlGsAs,TeO2, Si:Ge, and several organic polymers are presented. Photonic materials are realizing rapid transition into applications for many proposed space components and systems including: optical interconnects, optical gyros, waveguide and spatial light modulators, light emitting diodes, lasers, optical fibers and fiber optic amplifiers. Changes to material parameters such as electrooptic coefficients, absorption coefficients, polarization, conductivity, coupling coefficients, diffraction efficiencies, and other pertinent material properties examined for thermo-optic and radiation induced effect. Conclusions and recommendations provide the reader with an understanding of the limitations or attributes of material choices for specific applications.

Taylor, E. W.↗

NASA NTRS1985

Optical and radio properties of X-ray selected BL Lacertae objects

The eight BL Lac objects from the HEAO 1 A-2 all-sky survey and from the Einstein medium-sensitivity survey (MSS) form a flux-limited complete X-ray selected sample. The optical and radio properties of the MSS BL Lac objects are presented and compared with those of the HEAO 1 A-2 sample and with those of radio-selected BL Lac objects. The X-ray selected BL Lac objects possess smaller polarized fractions and less violent optical variability than radio-selected BL Lac objects. These properties are consistent with the substantial starlight fraction seen in the optical spectra of a majority of these objects. This starlight allows a determination of definite redshifts for two of four MSS BL Lac objects and a probable redshift for a third. These redshifts are 0.2, 0.3, and 0.6. Despite the differences in characteristics between the X-ray selected and radio-selected samples, it is concluded that these eight objects possess most of the basic qualities of BL Lac objects and should be considered members of that class. Moreover, as a class, these X-ray selected objects have the largest ratio of X-ray to optical flux of any active galactic nuclei yet discovered.

Stocke, J. T.↗

NASA NTRS2001

Retrieval of Polar Stratospheric Cloud Microphysical Properties from Lidar Measurements: Dependence on Particle Shape Assumptions

A retrieval algorithm has been developed for the microphysical analysis of polar stratospheric cloud (PSC) optical data obtained using lidar instrumentation. The parameterization scheme of the PSC microphysical properties allows for coexistence of up to three different particle types with size-dependent shapes. The finite difference time domain (FDTD) method has been used to calculate optical properties of particles with maximum dimensions equal to or less than 2 mu m and with shapes that can be considered more representative of PSCs on the scale of individual crystals than the commonly assumed spheroids. Specifically. these are irregular and hexagonal crystals. Selection of the optical parameters that are input to the inversion algorithm is based on a potential data set such as that gathered by two of the lidars on board the NASA DC-8 during the Stratospheric Aerosol and Gas Experiment 0 p (SAGE) Ozone Loss Validation experiment (SOLVE) campaign in winter 1999/2000: the Airborne Raman Ozone and Temperature Lidar (AROTEL) and the NASA Langley Differential Absorption Lidar (DIAL). The 0 microphysical retrieval algorithm has been applied to study how particle shape assumptions affect the inversion of lidar data measured in leewave PSCs. The model simulations show that under the assumption of spheroidal particle shapes, PSC surface and volume density are systematically smaller than the FDTD-based values by, respectively, approximately 10-30% and approximately 5-23%.

Reichardt, J.↗

NASA NTRS2021

Validation of the aerosol optical property products derived by the GRASP/Component approach from multi-angular polarimetric observations

The multi-angle polarimetric satellite observations are helpful for improving the retrievals of aerosol parameters. However, practical applications of polarization technology are still limited because of complexity of measurement and interpretation of polarimetric observations. In this study, we analyze the performance of a new component approach developed in the frame of the Generalized Retrieval of Atmosphere and Surface Properties (GRASP) algorithm. In addition to aerosol optical properties including particle size distribution, non-sphericity and index of refraction that are commonly derived from multi-angle radiance and polarization measurements, the GRASP/Component approach also provides some information about aerosol composition. Specifically, in this approach aerosol is modeled as an internal mixture of several components with distinctly different chemical compositions and known refractive indices. The approach is intended not only to provide additional insight on aerosol composition but also to improve retrieval of basic aerosol optical properties. This study presents comprehensive validation and evaluation of Aerosol Optical Depth (AOD), Ångstrom exponent (AE), fine mode AOD (AODF), coarse mode AOD (AODC), and single scattering albedo (SSA) as retrieved by the GRASP/Component approach. The GRASP/Component products include aerosol retrievals using two different aerosol component mixing rules, i.e., Maxwell-Garnett (MG) effective medium approximation and a simple Volume- Weighted averaging (VW). The differences between the results obtained using these two assumptions are also discussed. The obtained results show that the aerosol optical property products of GRASP/Component approach have good agreement with the ground-based AERONET measurements, which is comparable to other PARASOL/ GRASP approaches. Specifically, the AOD retrieved by GRASP/Component approach show high correlation and nearly no bias both over land and ocean, as compared with AERONET. The more detailed aerosol properties such as AE, AODF, AODC and SSA also show one of the best comparisons with AERONET. These improvements can probably be attributed to the use of the additional physical constraints on spectral dependence of the complex refractive index and the reduction of total number of aerosol parameters directly retrieved in the GRASP/Component approach. In addition, the choice of mixing rules had no significant effect on optical retrievals. With the exception of SSA, the results obtained based on the MG mixing rule were found to be slightly better over those obtained using VW mixing rule, especially for bias.

Brent N Holben↗

NASA NTRS1989

Interstellar circular polarization and the dielectric nature of dust grains

The implications of the observed relationship between the wavelength dependence of interstellar circular and linear polarization were reexamined. Mie theory calculations for grains with various optical constants demonstrate that any population of grains which matches the observed wavelength dependence of linear polarization also yields the correct cross-over wavelength of circular polarization. The coincidence of the peak wavelength of linear polarization and the cross-over of circular polarization is therefore independent of the optical constants of the grains and cannot be used as a critical constraint on grain properties. The observed relationship instead reflects a more fundamental connection between linear and circular polarization which was derived from the Kramers-Kronig relations by Shapiro (1975). Numerical results fully support Shapiro's conclusions and demonstrate that the apparent upper limit on the visual absorptivity of polarizing grains deduced from earlier Mie theory calculations (Martin, 1972) was spurious and resulted from a violation of the Kramers-Kronig relations in the assumed optical constants of the particles. The Kramers-Kronig interpretation of circular polarization can be used to place constraints on linear polarization outside the wavelength range in which it was observed. This approach was used to show that the peak observed in the visual is likely to be the only significant feature in the linear polarization curve, which therefore appears to be well approximated at all wavelengths by the Serkowski formula. A synthesis of available laboratory data was used to analyze the properties of dielectric core-mantel grains as the source of visual extinction and polarization.

Chlewicki, Grzegorz↗

DOE OSTI2023

Chiral Perovskite Nanoplatelets with Tunable Circularly Polarized Luminescence in the Strong Confinement Regime

Chiral perovskite nanocrystals have emerged as an interesting chiral excitonic platform that combines both structural flexibility and superior optoelectronic properties. Despite several recent demonstrations of optical activity in various chiral perovskite nanocrystals, efficient circularly polarized luminescence (CPL) with tunable energies remains a challenge. The chirality imprinting mechanism as a function of perovskite nanocrystal dimensionality remains elusive. Here, in this study, atomically thin inorganic perovskite nanoplatelets (NPLs) are synthesized with precise control of layer thickness and are functionalized by chiral surface ligands, serving as a unique platform to probe the chirality transfer mechanism at the organic/perovskite interface. It is found that chirality is successfully imprinted into mono-, bi-, and tri-layer inorganic perovskite NPLs, exhibiting tunable circular dichroism (CD) and CPL responses. However, chirality transfer decreases in thicker NPLs, resulting in decreased CD and CPL dissymmetry factors for thicker NPLs. Aided by large-scale first-principles calculations, it is proposed that chirality transfer is mainly mediated through a surface distortion rather than a hybridization of electronic states, giving rise to symmetry breaking in the perovskite lattice and spin-split conduction bands. The findings described here provide an in-depth understanding of chirality transfer and design principles for distorted-surface perovskites for chiral photonic applications.

36 MATERIALS SCIENCE↗

DOE OSTI2026

Hot-Carrier Photoluminescence in Low-Temperature CsSnI3 Nanocrystals

In the halide perovskites, the B-site metal lone-pairs electrons are strongly suspected to underpin many of the interesting properties of the inorganic halide perovskites. Recently, a stable low-temperature monoclinic polar phase was predicted for CsSnI3, opening the possibility of direct investigation of both these lone pair electrons and a ferroelectric distorted structure. To date there are no other reports of such a structure in CsSnI3, and a known low-temperature monoclinic structure in CsSnBr3 remains unexplored. We have found optical evidence of a transformation occurring around 240 K in CsSnI3 nanocrystals, with several changes in optical behavior below this transition point, including novel high-energy photoluminescene and new states in the transient absorption spectrum. We have successfully characterized the optical properties of this low-temperature phase and found evidence for a polar, monoclinic structure. Discovery of a stable monoclinic polar structure in the halide perovskites opens many new potential directions for further research and electronics applications.

14 SOLAR ENERGY↗

DOE OSTI2022

Visualization of Chiral Electronic Structure and Anomalous Optical Response in a Material with Chiral Charge Density Waves

Chiral materials have attracted significant research interests as they exhibit intriguing physical properties, such as chiral optical response, spin-momentum locking, and chiral induced spin selectivity. Recently, layered transition metal dichalcogenide 1T–TaS 2 has been found to host a chiral charge density wave (CDW) order. Nevertheless, the physical consequences of the chiral order, for example, in electronic structures and the optical properties, are yet to be explored. Here, we report the spectroscopic visualization of an emergent chiral electronic band structure in the CDW phase, characterized by windmill-shaped Fermi surfaces. Further, we uncover a remarkable chirality-dependent circularly polarized Raman response due to the salient in-plane chiral symmetry of CDW, although the ordinary circular dichroism vanishes. Chiral Fermi surfaces and anomalous Raman responses coincide with the CDW transition, proving their lattice origin. Our Letter paves a path to manipulate the chiral electronic and optical properties in two-dimensional materials and explore applications in polarization optics and spintronics.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗