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At least 109 records · Page 6

Performance of large-scale 6 Li-doped pulse-shape discriminating plastic scintillators

A 6 Li-doped plastic scintillator with pulse-shape discrimination capabilities, commercially identified as EJ -299-50, has been developed and produced at the kilogram-scale. A total of 44 bars of dimensions 5.5 cm x 5.5 cm x 50 cm of this material have been characterized. Optical properties like light output and effective attenuation length have been found to be comparable to 6 Li-doped liquid scintillators. Further, the scintillator EJ -299-50 shows good neutron detection capabilities with an effective efficiency for capture on 6 Li of approximately 85%. Stability tests performed on two formulation variations showed no intrinsic degradation in the material or optical properties during several months of observations.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND

The scintillator surface detector of the Pierre Auger observatory

Data collected so far by the Pierre Auger Observatory have enabled major advances in ultra-high energy cosmic ray physics and demonstrated that improved determination of masses of primary cosmic-ray particles, preferably on an event-by-event basis, is necessary for understanding their origin and nature. Improvement in primary mass measurements was the main motivation for the upgrade of the Pierre Auger Observatory, called AugerPrime. As part of this upgrade, scintillator detectors are added to the existing water-Cherenkov surface detector stations. By making use of the differences in detector response to the electromagnetic particles and muons between scintillator and water-Cherenkov detectors, the electromagnetic and muonic components of cosmic-ray air showers can be disentangled. Since the muonic component is sensitive to the primary mass, such combination of detectors provides a powerful way to improve primary mass composition measurements over the original Auger surface detector design. In this paper, the so-called Scintillator Surface Detectors are discussed, including their design characteristics, production process, testing procedure and deployment in the field.

Detector design and construction technologies and

Ionospheric S4 Scintillations From GNSS Radio Occultation (RO) at Slant Path

Ionospheric scintillation can significantly degrade the performance and the usability of space‐based communication and navigation signals. Characterization and prediction of ionospheric scintillation can be made from the Global Navigation Satellite System (GNSS) radio occultation (RO) technique using the measurement from a deep slant path where the RO tangent height (ht) is far below the ionospheric sources. In this study, the L–band S4 from the RO measurements at ht = 30 km is used to infer the amplitude scintillation on the ground. The analysis of global RO data at ht = 30 km shows that sporadic–E (Es), equatorial plasma bubbles (EPBs), and equatorial spread–F (ESF) produce most of the significant S4 enhancements, although the polar S4 is generally weak. The enhanced S4 is a strong function of local time and magnetic dip angle. The Es–induced daytime S4 tends to have a negative correlation with the solar cycle at low latitudes but a positive correlation at high latitudes. The nighttime S4 is dominated by a strong semiannual variation at low latitudes.

GPS radio occultation

Light output and neutron detection efficiency of boron-based neutron scintillator screens for neutron imaging

Recent research has explored the development of boron-based neutron scintillator screens, which potentially offer improved spatial resolution and neutron capture efficiency compared to traditional lithium-based screens. This work builds upon previous efforts to improve boron-based neutron scintillators by assessing a newer generation of boron-based scintillator screens fabricated using different compositions and fabrication approaches compared to previous generations of screens. Some of the test screens exhibit higher light output than previous efforts and higher neutron capture efficiency than lithium-based screens. This paper describes the current state of screen development, measurement results for the most recent generation of screens, and future activities.

46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN

Enhanced Neutron and γ-Ray Detection via 6 Li Substitution in Undoped and Tl-Doped Zero-Dimensional Perovskite Cs 3 Cu 2 I 5 Scintillators

Radiation detectors are crucial in a wide variety of research and commercial applications, such as oil and gas exploration, medical imaging, nuclear nonproliferation, and homeland security. Neutron and gamma-ray detectors are fundamental components in portal monitors at ports and border crossings, bolstering national security against radiological threats. This study presents a dual-mode scintillator, undoped and Tl-doped 6 Li-Cs 3 Cu 2 I 5 , and demonstrates its potential as a promising material for simultaneous thermal neutron and gamma-ray detection. We explore the Bridgman growth of both undoped and thallium doped Li → Cu and Li → Cs substitutional systems with various Li doping levels and assess their impact on scintillation properties. Under 662 keV gamma-ray excitation, the undoped crystals had light yields up to 35,900 ph/MeV, with energy resolutions down to 4.5%. The Tl-doped crystals performed better than the undoped crystals with light yields peaking at 65,900 ph/MeV and energy resolutions as low as 3.5%. When exposed to a moderated 252 Cf excitation source, our crystals had light yields between 102,900 and 167,200 photons per thermal neutron capture, with a full energy thermal neutron peak reaching 3 MeV in gamma equivalent energy. Pulse shape discrimination studies reveal well-separated gamma and neutron events, resulting in Figure-Of-Merit (FOM) as high as 3.7. Furthermore, these findings highlight the potential of Li-doped Cs 3 Cu 2 I 5 as a viable candidate for next-generation dual-mode scintillators.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH

Nonlinear light-output calibration of the oxygenated xylene scintillators used in OMEGA neutron time-of-flight spectrometers

Neutron time-of-flight (nTOF) spectrometers are essential instruments for measuring and evaluating the performance of inertial confinement fusion implosions. The neutron spectrometers utilized for the OMEGA laser include two liquid-based scintillators, each consisting of a large volume filled with xylene that is coupled to four photomultiplier tubes. Analysis of the signal from these detectors requires detailed knowledge of the scintillator’s light output, which is needed to fit the nTOF spectrum, from which the neutron energy spectrum is informed. The light output is nonlinearly proportional to the neutron energy, which, in turn, affects the interpretation of the neutron energy spectrum from a TOF signal. A recent campaign on OMEGA was performed to calibrate the xylene detectors and infer the shape of the light-output curve. The campaign utilized materials with increasing Z placed in the OMEGA target chamber to initiate scattering events with the 14 MeV fusion neutrons. This process leads to the production of backscatter neutrons of varying energies that appear as peaks in the nTOF data. Simulations using a neutron transport code were combined with the measured deuterium–tritium neutron yields to calculate the expected backscattered neutron yields from the well-known scattering cross sections of each material. Furthermore, the neutron-energy dependent light output of the scintillator inferred from the experiment is compared to the light-output curve simulated with a neutron transport code for the following neutron energies: 1.5, 2.5, 6, and 14 MeV.

47 OTHER INSTRUMENTATION

Scintillation light detection in polycrystalline diamond using single photon detectors

Here, this study investigates the scintillation properties of polycrystalline diamond for particle detection applications, particularly in neutron and alpha radiation environments. Polycrystalline diamonds provide a cost-effective alternative to monocrystalline diamonds while retaining essential detection properties. Photoluminescence measurements were performed to analyze emission spectra, revealing distinct characteristics based on impurity content and crystallinity. Scintillation responses were assessed using Silicon Photomultipliers (SiPMs), demonstrating the capability of polycrystalline diamond powders to respond to alpha irradiation, albeit with reduced resolution compared to traditional scintillators. A prototype neutron detector was developed by combining diamond powder with neutron-sensitive 6 LiF, and its performance was evaluated through experimental testing and Geant4 simulations. The findings indicate that polycrystalline diamond-based detectors can achieve significant detection efficiency while remaining insensitive to gamma radiation, offering potential for portable neutron detection applications.

47 OTHER INSTRUMENTATION

Detection of uranium-photofission neutrons with a 4 He scintillation detector

The use of photon active interrogation to detect special nuclear material has held significant theoretical promise, as the interrogating source particles, photons, are fundamentally different from one of the main signatures of special nuclear material: neutrons produced in nuclear fission. However, neutrons produced by photonuclear reactions in the accelerator target, collimator, and environment can obscure the fission neutron signal. These (γ, n) neutrons could be discriminated from fission neutrons by their energy spectrum, but common detectors sensitive to the neutron spectrum, like organic scintillators, are typically hampered by the intense photon background characteristic of photon-based active interrogation. In contrast, high-pressure 4 ⁢He-based scintillation detectors are well-suited to photon active interrogation, as they are similarly sensitive to fast neutrons and can measure their spectrum, but show little response to gamma rays. Here, in this work, a photon active interrogation system utilizing a 4 ⁢He scintillation detector and a 9 MeV linac-bremsstrahlung x-ray source was experimentally evaluated. The detector was shown to be capable of operating in intense gamma-ray environments and detecting photofission neutrons from 238 ⁢U when interrogated by this x-ray source. The photofission neutrons show clear spectral separation from (γ, n) neutrons produced in lead, a common shielding material.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND

Next-generation neutron detection using a 6 Li glass scintillator composite

Neutron detectors are crucial in fundamental science, nuclear security, safeguards, and civil applications. 3 He-filled gas proportional counters are the gold standard for thermal neutron detection, prized for their efficiency, neutron/gamma discrimination, and stability; however, the scarcity of 3 He has prompted the search for alternatives. Here, we introduce a neutron detector design based on a scintillating composite consisting of 6 Li glass scintillator particles dispersed in an organic matrix. A detector consisting of this scintillating composite, photomultiplier tubes (PMTs) for optical detection, and electronics for reading out the PMT signal in both pulse and current modes was prototyped and characterized using various neutron and gamma sources. The prototype achieves a measured intrinsic detection efficiency of 6.70 ± 0.01%, a die-away time of 10.3 ± 0.1 μs, a negligible gamma misidentification probability, and response linearity up to at least 3.7 × 10 6 incident neutrons/s established via a cross-calibration technique. This detector holds the potential to outperform traditional 3 He-gas-based neutron detection systems, offering a viable alternative amidst the ongoing 3 He shortage and promising advancements in neutron detection technology.

47 OTHER INSTRUMENTATION

Scintillating glass for precision calorimetry in nuclear physics

High-performance scintillator materials are needed for particle identification and measurements of energy and momentum of electromagnetic particles in modern nuclear physics experiments. As an example, the US Electron-Ion Collider, a unique collider with diverse physics topics, requires electromagnetic calorimetry enabling high-quality electron identification and detection in the momentum range of 0.3 to tens of GeV. The highest resolution in electromagnetic calorimeters can be provided by homogeneous materials, e.g., lead tungstate crystals. Inorganic glass scintillators have been investigated as an attractive and cost-effective alternative to crystals, that is also easier and faster to manufacture in mass production. In this paper, we discuss progress in the fabrication and characterization of recent scintillating glass samples on both test bench and beam tests. Further, the results are well-reproduced by simulation and are discussed in the context of the Electron-Ion Collider experimental requirements and bench-marked against lead tungstate crystals.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS

Technology Transfer from Fermi Research Alliance to Itasca Plastics for the purpose of Commercializing Scintillator Material

Researchers at the Fermi National Accelerator Laboratory (Fermilab) developed extruded plastic scintillator in the late 1990s, which was first used in the D-Zero experiment. Extruded plastic scintillator is currently produced at Fermilab and is used in particle detectors worldwide. The purpose of this CRADA is to transfer the knowledge related to the Fermilab extrusion process to Itasca Plastics, Inc. (Itasca Plastics). Much of this knowledge is contained in documentation that is in the public domain, although it is distributed over several communications (papers, conference records, etc.) and over several years. Under this CRADA Fermilab will assemble the information, provide it to Itasca Plastics and provide limited consulting to complete the knowledge transfer. If the transfer is successful, Itasca Plastics will be able to establish a U.S. commercial manufacturing capability for extruded scintillator material that can be used for high energy physics and commercial applications.

36 MATERIALS SCIENCE

Field Test Report Neutron Scintillator Array Dry Storage Cask Scanner FY2024

During two weeks of Field Testing at the Idaho National Laboratory INTEC Cask Farm in July and August 2024, the LLNL Dry Storage Cask Scanner Array was lifted on top of an MC-10 dry storage fuel cask and operated to acquire neutron and gamma-ray data from the 24 fuel bundle positions. Neutron and gamma-ray data acquisition scans across the top of the cask of varying dwell times were performed July 15-18, 2024 and August 19-22, 2024 to evaluate the ability of the scanner data to reveal asymmetries in the fuel positions that reflect asymmetries in the MC-10 cask fuel bundle loading. The MC-10 cask 24 position fuel bundle loading at the INTEC Cask Farm is well documented, including the locations of six empty fuel bundle positions. This loading presents an opportunity to test the ability of the scanner system to detect diversion of spent fuel bundles as well as to validate the MC-10 cask MCNP modeling. The cask scanner array consists of six Stilbene crystal scintillator detectors and a linear actuator frame that moves the six detectors across the MC-10 dry storage cask to obtain data above each of the 24 fuel bundle positions. The detectors are connected to a pulse-shape discrimination data acquisition system capable of generating separate neutron and gamma-ray spectra for each detector and for each scan position. From the prior single detector Field Test in 2021 and iteration with MCNP modeling, the neutron and gamma-ray data were analyzed in multiple energy regions to identify an analysis method that would provide the strongest and most consistent signature of the asymmetric MC-10 cask fuel loading1 . From both the 2021 Field Test and the current Field Test results, the neutron capture gamma-ray count rate around 2.2 MeV provides the strongest signature of the asymmetric MC-10 cask fuel loading and has qualitative agreement with MCNP calculations. Counting all gamma-rays produces a similar signature. Neutrons emerging from the cask top are moderated and captured by the hydrogen in the polyethylene moderator and scintillator detector, producing a 2.2 MeV gamma ray which is seen in the scintillator gamma-ray spectrum. The count rate in the 2.2 MeV gamma-ray region is ~50 c/s, which is ~1000x higher than the ~0.05 n/s rate in the > 4MeV neutron region, and ~50x greater than the ~1 n/s rate in the neutrons > 500 keV region. Analysis of the 2.2 MeV neutron-capture Compton-scattered gamma-rays produces a statistically significant signature of the INTEC Cask Farm MC-10 asymmetric fuel loading. MCNP simulations indicate that the average neutron energy spectrum offers the potential to detect a large asymmetry from several missing bundles as well as individual missing fuel bundles. Testing this feature will require measurements on a cask with single missing elements.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS

Scintillating Bubble Chambers for Rare Event Searches

The Scintillating Bubble Chamber (SBC) collaboration is developing liquid-noble bubble chambers to detect sub-keV nuclear recoils, allowing the search for low-mass (GeV-scale) dark matter and coherent elastic neutrino-nucleus scattering from low-energy (MeV-scale) neutrinos. The scintillating bubble chamber detectors benefit from the energy reconstruction that the scintillation signal gives in addition to the superior electron-recoil insensitivity that bubble chambers naturally provide. The high level of superheat achievable in noble liquids while being electron-recoil insensitive allows for lower nuclear recoil thresholds than in existing freon-based bubble chambers, potentially reaching the 100 eV threshold desired for reactor CEvNS measurements. To validate this lower threshold, the SBC collaboration is constructing two 10 kg detectors that are functionally identical. The SBC-LAr10, which is being commissioned at Fermilab, is intended for engineering and calibration research and has additional possibilities in assessing coherent elastic neutrino-nucleus scattering in argon. SBC-SNOLAB, the second detector for a low-background dark matter search, will be run at SNOLAB underground.

Pyda, Daniel [Unlisted, US]

Analysis of scintillation light dependence on liquid Argon purity

Previous studies have investigated the correlation between impurity concentrations in Liquid Argon (LAr) and the temporal evolution of either the slow scintillation decay time or the light yield. These impurities typically consist of various molecular species. Electronegative contaminants directly affect electron drift and photon production, while other molecules, such as nitrogen (N_2),can influence LAr scintillation properties without necessarily affecting electron lifetime. Many current and future neutrino and dark-matter experiments use LAr detectors. This study aims to evaluate the measured electron lifetimes in relation to the timing characteristics of the scintillation light signal in the SBN ICARUS detector at Fermi National Accelerator Laboratory. The ICARUS experiment consists of two cryostats that have shown some discrepancies in the measured electron lifetime over the years. In particular, this study addresses the use of data collected under varying purity conditions in the two cryostats.

Saia, Clara [Catania Astrophys. Observ.]

Dual Readout in Homogenous Inorganic Scintillators for Precision Calorimeters

Homogeneous inorganic scintillator-based calorimeters are the gold standard for electromagnetic energy resolution, but often degrade the hadronic energy resolution achievable at colliders. By incorporating the dual readout technique, we seek to improve the hadronic energy resolution of these calorimeters through the measurement and separation of the scintillation and Cherenkov light in hadronic showers. In April 2024, CalVision performed single-crystal tests using the electron test beam at DESY. Using a single delay line technique for waveform analysis, sufficient cerenkov light can be extracted to fully capitalize on the dual readout technique. This talk will present the results of PWO, BGO, BSO, PbF2, and two novel scintillating glasses.

Anderson, Thomas [Virginia U.]

Scintillator Manufacture

This paper will be a literature review of composite scintillators, and their applications in neutron detection. Due to the shortage of 3 He, the traditional medium for neutron detection, new materials need to be explored for this purpose. Composite scintillating particle materials can serve as a solution to replace 3 He, offering faster response times, and all-solid-state form factors for diversified applications in the field. This project will include manufacturing Europium (Eu) and Sodium (Na) doped LiCaAlF 6 (LiCAF) scintillating particles for neutron detection.

36 MATERIALS SCIENCE

A brief review of ionospheric scintillation fading effects as observed in NASA satellite tracking and data acquisition networks.

Discussion of some results of the effects of ionospheric irregularities on NASA satellite tracking and data acquisition operations. Ionospheric scintillation fading produced by irregularities has been observed at 136 MHz (vhf), 400 MHz (uhf), 1550 MHz (L-band) and 1700 to 2200 MHz (S-band). Details of these observations are presented. Vhf scintillation effects are evident in both auroral and equatorial regions. Fading effects decrease with increasing radio frequency in the auroral region. The same frequency dependence for fading is not observed in the equatorial region. Although there is a seasonal and diurnal character to scintillation in the equatorial region, fading effects are usually more severe than in the auroral region for a given radio frequency. Space diversity measurements indicate that reasonable solutions for vhf telemetry problems are available for either region. Space diversity should provide a solution for microwave frequencies as well. Ionospheric fading amplitude for 1700 MHz is relatively small in the auroral region. In the equatorial region amplitude fading levels for 1550-MHz signals from ATS-5 are often much larger than expected. Observations of the Apollo Lunar Surface Experiment Package (ALSEP) operating at 2300 MHz observed near the geomagnetic equator show fading peaks in excess of 15 dB.

Golden, T. S.

Velocity of the solar wind as determined from interplanetary scintillations.

The method of smooth perturbations is used to derive the equations for interplanetary scintillation in a (statistically) spherically symmetric solar wind with constant wind velocity. The expressions, valid in the limit of small scintillation index, are used to discuss the relation between the radial wind velocity and the observed projected velocity of the scintillation pattern. It is found that the pattern velocity is systematically less than the wind velocity by a substantial fraction, depending on the radial variation of the density fluctuations. If the fluctuations fall off as 1/r-squared the correction is 18 percent, whereas if the fluctuations are proportional to 1/r the correction is 57 percent. The effects may be even more severe if the solar wind is not spherically symmetric.

Jokipii, J. R.