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At least 109 records · Page 6

A two-dimensional model simulation of the EL Chichon volcanic eruption cloud

Using a two-dimensional model of sulfate photochemistry, transport, and aerosol microphysics, a 2-year period following the eruptions of El Chichon have been simulated. Present calculations suggest that the residence time of the cloud in the stratosphere exceeds 2 years. The model reproduces the observed optical depth, lidar backscatter, and infrared extinction coefficients, if about 10 megatonnes of SO2 are injected. The major deficiency of the model is a somewhat too rapid transport.

Capone, L. A.↗

Remote Marine Aerosol: A Characterization of Physical, Chemical and Optical Properties and their Relation to Radiative Transfer in the Troposphere

Our research effort is focused on improving our understanding of aerosol properties needed for optical models for remote marine regions. This includes in-situ and vertical column optical closure and involves a redundancy of approaches to measure and model optical properties that must be self consistent. The model is based upon measured in-situ aerosol properties and will be tested and constrained by the vertically measured spectral differential optical depth of the marine boundary layer, MBL. Both measured and modeled column optical properties for the boundary layer, when added to the free-troposphere and stratospheric optical depth, will be used to establish spectral optical depth over the entire atmospheric column for comparison to and validation of satellite derived radiances (AVHRR).

Clarke, Antony D.↗

Radiative Forcing of the Pinatubo Aerosol as a Function of Latitude and Time

We present calculations of the radiative forcing of the Mt. Pinatubo aerosols as a function of latitude and time after the eruption and compare the results with GOES satellite data. The results from the model indicate that the net effect of the aerosol was to cool the earth-atmosphere system with the most significant radiative effect in the tropics (corresponding to the location of the tropical stratospheric reservoir) and at latitudes greater than 60 deg. The high-latitude maximum is a combined effect of the high-latitude peak in optical depth (Trepte et al 1994) and the large solar zenith angles. The comparison of the predicted and measured net flux shows relatively good agreement, with the model consistently under predicting the cooling effect of the aerosol.

Bergstrom, R. W.↗

Radiative Forcing of the Pinatubo Aerosol as a Function of Latitude and Time

We present calculations of the radiative forcing of the Mt. Pinatubo aerosols as a function of latitude and time after the eruption and compare the results with GOES satellite data. The results from the model indicate that the net effect of the aerosol was to cool the earth-atmosphere system with the most significant radiative effect in the tropics (corresponding to the location of the tropical stratospheric reservoir) and at latitudes greater than 60 degrees. The high-latitude maximum is a combined effect of the high-latitude peak in optical depth (Trepte et al 1994) and the large solar zenith angles. The comparison of the predicted and measured net flux shows relatively good agreement, with the model consistently under predicting the cooling effect of the aerosol.

Bergstrom, Robert W.↗

Measurement of stratospheric aerosol on Saturn using an eclipse of Titan

Measurements of the aerosol content in the Saturn atmosphere made during an eclipse of Titan by Saturn are presented. Observations of the ingress of Titan into the shadow of Saturn on December 20.08, 1979 were made by the 74-in telescope at Kottamia Station in Egypt at an effective wavelength of 6728 A with FWHM of 1000 A. The deviation of the observed light curve after a satellite darkening of 3 mag from that predicted for a clear Saturn atmosphere is interpreted in terms of an aerosol layer decreasing in extinction coefficient from a base altitude 5 km below the planetary tropopause to an altitude of up to 75 km above the tropopause. For an aerosal layer extending to 75 km above the tropopause calculations reveal possible optical depths ranging from 0.020 to 0.050. The range of the optical depth is comparable to that of the Jupiter atmosphere, and suggests that similar processes may be responsible for the stratospheric haze on both planets.

Smith, D. W.↗

Tropopause Laminar Cirrus and Its Role in the Lower Stratosphere Total Water Budget

Laminar cirrus are thin, extensive, isolated layers of ice clouds frequently observed in the tropical tropopause layer. Widespread laminar cirrus significantly affects tropical tropopause layer total water and thermal budget. In this study, we extract laminar cirrus from the Cloud‐Aerosol Lidar with Orthogonal Polarization Level 1 attenuated total backscatter images for January 2009, in order to characterize statistical properties of laminar cirrus cloud length, base, thickness, optical depth, and layer partial ice water path. These characteristics are used to develop an algorithm identifying laminar cirrus automatically from the Cloud‐Aerosol Lidar with Orthogonal Polarization Level 2 layer product for 2008–2017. The nearly 10‐year records reveal that tropopause laminar cirrus occurrence (30–40% of total cirrus) is strongly anticorrelated with the tropopause temperatures in that colder tropopause in frequent (super)saturation during boreal winter favors in situ formation of clouds. Interannually, anomalously warmer troposphere temperature (ΔT), easterly shear of the quasi‐biennial oscillation, and stronger upwelling branch of the Brewer‐Dobson circulation enhance laminar cirrus formation via cooling of the tropopause. The tropopause laminar cirrus carries ~0.05 mg/m(exp 3) (~0.5 ppmv) of ice water content during boreal winter and <0.01 mg/m(exp 3) during summer, which is anticorrelated with the seasonal variations of water vapor (H2O) observed by the Microwave Lime Sounder, indicating a temperature‐regulated partition between vapor and ice. Interannually, in cirrus‐rich region 1 ppmv decrease in H2O corresponds to 0.2–0.3 ppmv increase in ice water content. Frequently situated in (super)saturated air, tropopause laminar cirrus are likely to survive multiple lifecycles of the sublimation‐deposition processes, and may contribute up to 10% to the total water budget in the lower stratosphere. Satellites constantly observe thin, isolated, extensive layer of cirrus around the tropopause. The so‐called “laminar” cirrus occurrence and their ice amount are strongly regulated by temperature, such that colder temperatures favor more frequent (super)saturation, which results in more frequent laminar cirrus with more ice amount and therefore less water vapor. In this study we analyze laminar cirrus and water vapor from the Cloud‐Aerosol Lidar with Orthogonal Polarization and Microwave Lime Sounder observations, and hypothesize that laminar cirrus could act as an important transient water storage and contribute to the total water budget in the lower stratosphere.

Tao Wang↗

Observation of El Chichon volcanic aerosols by the solar backscattered ultraviolet (SBUV) experiment

The Solar Backscatter Ultraviolet Experiment (SBUV) aboard the Nimbus-7 satellite identified large amounts of SO2 in the tropical stratosphere on April 15, 1982, 11 days after major eruption of the El Chichon volcano in southern Mexico. It is shown in the present study that the backscattered ultraviolet radiances measured by the SBUV experiment have been strongly affected by the presence of stratospheric volcanic cloud from the El Chichon eruptions. Both SO2 and aerosol amounts present in the volcanic cloud have been mapped on the basis of an analysis of the radiances measured by the SBUV and TOMS (Total Ozone Mapping Spectrometer) experiments. It is estimated that a volcanic cloud of optical depths as small as 0.03 can be detected using SBUV, provided the cloud reaches the middle atmosphere. Lower-altitude clouds have progressively smaller effects on the radiances as well as on the ozone profile derived from them and are therefore harder to detect.

Bhartia, P. K.↗

Chapter 10 - Remote Sensing Measurements of Aerosol Properties

Satellite instruments have proven especially capable at monitoring the quantity of airborne particles in columns of atmosphere, globally. This chapter describes the principles of satellite measurements and retrieval algorithms, and surveys current instruments and their capabilities. We outline the issues associated with retrieval algorithms, such as surface characterization and aerosol proximity to clouds, and the challenges with interpretation of the results. The relationship between measured aerosol properties and climate-relevant aerosol properties simulated in models is outlined, as well as how measurements are used to evaluate models. Most space-based aerosol instruments are passive sensors that measure reflected sunlight at multiple wavelengths, some at multiple viewing angles. A few are active sensors that send out their own laser light and measure the returned signal. Except when clouds are present, the excess amount of light scattered back to space, beyond that expected from the surface and atmospheric gas, is attributed to aerosol. Satellite measurements are used in many ways in aerosol research. They often provide the only method for monitoring hazardous phenomena such as major wildfire and volcanic eruption plumes, especially in remote areas. Stable, long-term, near-global-scale satellite data records make it possible to identify regional and global aerosol trends. Aerosol radiative effects on climate can be quantified on a near-global scale and used to estimate the strength of aerosol–radiation and aerosol–cloud interactions as well as to evaluate climate model simulations of these interactions. Aerosol-type mapping from satellite imagery is helpful for source attribution, model validation, and to constrain particle light-absorption properties that are essential for radiative forcing calculations. The range of aerosol properties retrieved from satellite observations has grown considerably since the first global estimates of aerosol optical depth (τ a) over ocean were made in the late 1970s. Methods for retrieving particle size and light-absorption properties were explored in the 1990s using multispectral, multi-angle observations, and polarization in visible and near-infrared wavelengths. Sensitivity to particle light absorption, primarily from black or brown carbon content, improved with the inclusion of UV channels, and sensitivity to very thin aerosol layers in the upper troposphere and lower stratosphere was advanced with the use of limb-sounding instruments and active sensors. There are limitations to every measurement technique, including satellite aerosol remote sensing. For wide-swath, passive instruments, aerosol retrievals near clouds can present substantial challenges as far as 15 km away due to cloud-scattered light contaminating the signal. In nearly all cases, retrievals over bright snow and ice surfaces are precluded because surface reflectance uncertainties can overwhelm the aerosol signal. Similarly, meteorological cloud is identified and masked out where possible. Data from passive sensors also lack vertical resolution except those that view toward the limb or where multi-angle imagery is acquired over plumes from wildfires, erupting volcanoes, and wind-blown dust. Yet, passive sensors provide vastly more coverage than the active instruments that mitigate these issues. Particle microphysical information is qualitative from all remote sensing techniques, relying on proxies to infer particle composition, hygroscopicity, and the amount of light-absorbing material. Further, particles smaller than about 200 nm diameter cannot be distinguished from atmospheric gas molecules with remote sensing, which hinders studies of cloud condensation nuclei and their effects on clouds. Most satellite instruments dedicated to aerosol observations are in low-Earth, near-polar, sun-synchronous orbits, which means they cross the equator at the same local time each day. Most are set on cycles that repeat approximately every 16 days, which makes it difficult to monitor aerosol evolution locally. Geostationary satellites make it possible to observe changes occurring from minutes to hours over regions up to 8000 km in size, but lack coverage of high latitudes, and often provide more limited constraints on aerosol properties. Ground-truth data are vital for satellite aerosol-retrieval validation. The AErosol RObotic NETwork (AERONET) of sun photometers was created in 1993 and has become an established global network of over 350 instruments for validating satellite measurements. The network, as well as global networks of ground-based lidars, solar flux radiometers and other sun photometers, are widely used for evaluating global satellite retrievals and model simulations. NASA's Earth Observing System (EOS) program beginning in 1999 led to improvements in reliability, spatial resolution, and spectral resolution (and hence, to improved particle size discrimination and light absorption properties). Satellite payloads include advanced broad-swath and multi-angle imagers, along with the first space-based active sensor focused largely on long-term aerosol monitoring. Since about 2002, Europe's SENTINEL and operational meteorological satellite fleets are also providing sustained aerosol observations, with planned continuation until at least 2030. Satellite remote sensing instruments offer valuable data for evaluating aerosol representations in global climate models. They have been used to assess aerosol optical and physical properties, trends and distributions, and are applied increasingly as direct model constraints in data assimilation to create global aerosol reanalysis products. Aerosol optical depth is the most common quantity adopted for routine model evaluation, including multiwavelength data to loosely constrain particle-size distributions. These evaluations of multiple models have revealed general biases in their regional aerosol amounts and seasonal patterns of transport and removal. Although satellite measurements have near-global coverage, substantial errors can be introduced into the model observation comparison unless attention is paid to spatial and temporal collocation, cloud screening, subgrid-scale variability, and measurement uncertainties that vary with retrieval conditions.

aerosol properties↗

Constraining the Global, Cloud-Free Reflected Solar Radiation Flux (RSRF) with Earth Observing System (EOS) Instruments

Variations in the top-of-atmosphere reflected solar radiation flux, and in the factors that determine its value, are among the most important diagnostic indicators of changes in Earth's energy balance. Data from the MISR (Multi-angle Imaging SpectroRadiometer), MODIS (Moderate-resolution Imaging Spectroradiometer), SAGE-3 (Stratospheric Aerosol and Gas Experiment), and CERES (Clouds and Earth's Radiant Energy System), all of which are spacecraft instruments scheduled for launch in 1999, will each constrain pieces of the RSRF budget. Prior to launch, we are performing studies to determine the sensitivity of these instruments to key factors that influence the cloud-free RSRF: aerosol optical depth, aerosol scattering properties, and surface visible bidirectional reflectance distribution function (BRDF). We are also assessing the ability of the aggregate of instruments to constrain the overall RSRF budget under natural conditions over the globe. Consider the MISR retrieval of aerosols: according to simulations over cloud-free, calm ocean, for pure particles with natural ranges of optical depth, particle size, and indices of refraction, MISR can retrieve column aerosol optical depth for all but the darkest particles, to an uncertainty of at most 0.05 or 20%, whichever is larger, even if the particle properties are poorly known. For one common particle type, soot, constraints on the optical depth over dark ocean are very poor. The simulated measurements also allow us to distinguish spherical from non-spherical particles, to separate two to four compositional groups based on indices of refraction, and to identify three to four distinct size groups between 0. 1 and 2.0 microns characteristic radius at most latitudes. Based on these results, we expect to distinguish air masses containing different aerosol types, routinely and globally, with multiangle remote sensing data. Such results far exceed current satellite aerosol retrieval capabilities, which provide only total optical depth for assumed particle properties; the new information will complement in situ data, which give details about aerosol size and composition locally. In addition, our team is using climatologies that reflect the constraints each instrument is expected to provide, along with ERBE (Earth Radiation Budget Experiment) data and a radiative transfer code, to study overall sensitivity to RSRF, helping us prepare for similar studies with new data from the EOS-era instruments.

Kahn, Ralph↗

Technical Note: A Time-Dependent I(sub 0) Correction for Solar Occultation Instruments

Solar occultation has proven to be a reliable technique for the measurement of atmospheric constituents in the stratosphere. NASA's Stratospheric Aerosol and Gas Experiments (SAGE, SAGE II, and SAGE III) together have provided over 25 years of quality solar occultation data, a data record which has been an important resource for the scientific exploration of atmospheric composition and climate change. Herein, we describe an improvement to the processing of SAGE data that corrects for a previously uncorrected short-term timedependence in the calibration function. The variability relates to the apparent rotation of the scanning track with respect to the face of the sun due to the motion of the satellite. Correcting for this effect results in a decrease in the measurement noise in the Level 1 line-of-sight optical depth measurements of approximately 40% in the middle and upper stratospheric SAGE II and III where it has been applied. The technique is potentially useful for any scanning solar occultation instrument, and suggests further improvement for future occultation measurements if a full disk imaging system can be included.

Burton, Sharon P.↗

Twenty years of balloon-borne tropospheric aerosol measurements at Laramie, Wyoming

The paper examines the tropospheric aerosol record obtained over the period 1971 to 1990, during which high-altitude balloons with optical particle counters were launched at Laramie, Wyoming, in a long-term study of the stratospheric sulfate aerosol layer. All aerosol particle size ranges display pronounced seasonal variations, with the condensation nuclei concentration and the optically active component showing a summer maximum throughout the troposphere. Mass estimates, assuming spherical sulfate particles, indicate an average column mass between altitudes of 2.5 and 10 km of about 4 and 16 mg/sq m in winter and summer, respectively. Calculated optical depths vary between 0.01 and 0.04 from winter to summer; the estimated mass scattering cross section is about 3 sq m/g throughout the troposphere. There is evidence for a decreasing trend of 1.6-1.8 percent/yr in the optically active tropospheric aerosol over the past 20 yr, which may be related to a similar reduction in SO2 emission in the U.S. over this period.

Hofmann, David J.↗

Assessment of the atmospheric impact of volcanic eruptions

The dominant global impact of volcanic activity is likely to be related to the effects of volcanic gases on the Earth's atmosphere. Volcanic gas emissions from individual volcanic arc eruptions are likely to cause increases in the stratospheric optical depth that result in surface landmass temperature decline of 2 to 3 K for less than a decade. Trachytic and intermediate magmas are much more effective in this regard than high-silica magmas, and may also lead to extensive ozone depletion due to effect of halogens and magmatic water. Given the assumed relationship between arc volcanism and subduction rate, and the relatively small variation in global spreading rates in the geologic record, it is unlikely that the rates of arc volcanism have varied greatly during the Cenozoic. Hotspot related basaltic fissure eruptions in the subaerial environment have a higher mass yield of sulfur, but lofting of the valcanic aerosol to levels above the tropopause is required for a climate impact. High-latitude events, such as the Laki 1783 eruption can easily penetrate the tropopause and enter the stratosphere, but formation of a stratospheric volcanic aerosol form low-latitude effusive basaltic eruptions is problematical, due to the elevated low-latitude tropopause. Due to the high sulfur content of hotspot-derived basaltic magmas, their very high mass eruption rates and the episodic behavior, hotspots must be regarded as potentially major modifiers of Earth's climate through the action of their volcanic volatiles on the chemistry and physics of the atmosphere.

Sigurdsson, H.↗

Satellite and aircraft measurements of stratospheric aerosol particles

Data on the characteristics of the stratospheric aerosol as measured with sensors on the SAM II and SAGE I satellites and with ground-based and airborne lidar are discussed. Emphasis is placed on the impact of the El Chichon eruptions. The volcanic cloud was tracked to an altitude of 30 km, and was observed to travel around the earth in 3 weeks. The maximum stratospheric loading is estimated at 12 Mtons, which increased the stratospheric optical depth to 0.15-2.0 at the peak period. The particulate loading was predicted to lower the Northern Hemisphere average temperatures by 0.4-0.5 C in 1984-85.

Mccormick, M. P.↗

Aerosol Absorption Effects in the TOMS UV Algorithm

The availability of global long-term estimates of surface UV radiation is very important, not only for preventive medicine considerations, but also as an important tool to monitor the effects of the stratospheric ozone recovery expected to occur in the next few decades as a result of the decline of the stratospheric chlorine levels. In addition to the modulating effects of ozone and clouds, aerosols also affect the levels of UV-A and W-B radiation reaching the surface. Oscillations in surface W associated with the effects of aerosol absorption may be comparable in magnitude to variations associated with the stratospheric ozone recovery. Thus, the accurate calculation of surface W radiation requires that both the scattering and absorption effects of tropospheric aerosols be taken into account. Although absorption effects of dust and elevated carbonaceous aerosols are already accounted for using Aerosol Index technique, this approach does not work for urban/industrial aerosols in the planetary boundary layer. The use of the new TOMS long-term global data record on UV aerosol absorption optical depth, can improve the accuracy of TOMS spectral UV products, by properly including the spectral attenuation effects of carbonaceous, urban/industrial and mineral aerosols. The TOMS data set on aerosol properties will be discussed, and results of its use in the TOMS surface W algorithm will be presented.

Torres, O.↗

A determination of the infrared optical depth of the El Chichon volcanic cloud

Infrared transmission spectra of the atmosphere above 11-km altitude were obtained in December 1982 and April/May 1983 from a NASA Convair 990 aircraft. The observations on the first flight series encompassed low and middle latitudes in the Northern Hemisphere, while the observations on the second series covered a wide range of latitudes in both hemispheres. These data have been analyzed to derive the optical depth of the El Chichon volcanic cloud at a wavelength of 8.4 microns. These data imply that concentrated sulfuric acid was the dominant source of aerosol extinction in the 8- to 12-microns window region of the earth's atmosphere and that the volume modal particle radius equalled 0.6 + or - 0.1 mu at the time of the observations. At these times, the volcanic particles produced a significant warming of the lower stratosphere and had a nontrivial impact on the radiation budget of the troposphere and ground in the Northern Hemisphere.

Pollack, James B.↗

Aerosol-Induced Changes of Convective Cloud Anvils Produce Strong Climate Warming

The effect of aerosol on clouds poses one of the largest uncertainties in estimating the anthropogenic contribution to climate change. Small human-induced perturbations to cloud characteristics via aerosol pathways can create a change in the top-of-atmosphere radiative forcing of hundreds of Wm(exp-2) . Here we focus on links between aerosol and deep convective clouds of the Atlantic and Pacific Intertropical Convergence Zones, noting that the aerosol environment in each region is entirely different. The tops of these vertically developed clouds consisting of mostly ice can reach high levels of the atmosphere, overshooting the lower stratosphere and reaching altitudes greater than 16 km. We show a link between aerosol, clouds and the free atmosphere wind profile that can change the magnitude and sign of the overall climate radiative forcing. We find that increased aerosol loading is associated with taller cloud towers and anvils. The taller clouds reach levels of enhanced wind speeds that act to spread and thin the anvi1 clouds, increasing areal coverage and decreasing cloud optical depth. The radiative effect of this transition is to create a positive radiative forcing (warming) at top-of-atmosphere. Furthermore we introduce the cloud optical depth (r), cloud height (Z) forcing space and show that underestimation of radiative forcing is likely to occur in cases of non homogenous clouds. Specifically, the mean radiative forcing of towers and anvils in the same scene can be several times greater than simply calculating the forcing from the mean cloud optical depth in the scene. Limitations of the method are discussed, alternative sources of aerosol loading are tested and meteorological variance is restricted, but the trend of taller clouds; increased and thinner anvils associated with increased aerosol loading remains robust through all the different tests and perturbations.

Koren, I.↗

A physical model of Titan's clouds

A physical model of the formation and growth of aerosols in the atmosphere of Titan has been constructed in light of the observed correlation between variations in Titan's albedo and the sunspot cycle. The model was developed to fit spectral observations of deep methane bands, pressures, temperature distributions, and cloud structure, and is based on a one-dimensional physical-chemical model developed to simulate the earth's stratospheric aerosol layer. Sensitivity tests reveal the model parameters to be relatively insensitive to particle shape but sensitive to particle density, with high particle densities requiring larger aerosol mass production rates to produce compatible clouds. Solution of the aerosol continuity equations for particles of sizes 13 A to about 3 microns indicates the importance of a warm upper atmosphere and a high-altitude mass injection layer, and the production of aerosols at very low aerosol optical depths. Limits are obtained for the chemical production of aerosol mass and the eddy diffusion coefficient, and it is found that an increase in mass input causes a decrease in mean particle size.

Toon, O. B.↗

Cloud Statistics for NASA Climate Change Studies

The Principal Investigator participated in two field experiments and developed a global data set on cirrus cloud frequency and optical depth to aid the development of numerical models of climate. Four papers were published under this grant. The accomplishments are summarized: (1) In SUCCESS (SUbsonic aircraft: Contrail & Cloud Effects Special Study) the Principal Investigator aided weather forecasters in the start of the field program. A paper also was published on the clouds studied in SUCCESS and the use of the satellite stereographic technique to distinguish cloud forms and heights of clouds. (2) In SHEBA (Surface Heat Budget in the Arctic) FIRE/ACE (Arctic Cloud Experiment) the Principal Investigator provided daily weather and cloud forecasts for four research aircraft crews, NASA's ER-2, UCAR's C-130, University of Washington's Convert 580, and the Canadian Atmospheric Environment Service's Convert 580. Approximately 105 forecasts were written. The Principal Investigator also made daily weather summaries with calculations of air trajectories for 54 flight days in the experiment. The trajectories show where the air sampled during the flights came from and will be used in future publications to discuss the origin and history of the air and clouds sampled by the aircraft. A paper discussing how well the FIRE/ACE data represent normal climatic conditions in the arctic is being prepared. (3) The Principal Investigator's web page became the source of information for weather forecasting by the scientists on the SHEBA ship. (4) Global Cirrus frequency and optical depth is a continuing analysis of global cloud cover and frequency distribution are being made from the NOAA polar orbiting weather satellites. This analysis is sensitive to cirrus clouds because of the radiative channels used. During this grant three papers were published which describe cloud frequencies, their optical properties and compare the Wisconsin FM Cloud Analysis to other global cloud data such as the International Satellite Cloud Climatology Program (ISCCP) and the Stratospheric Aerosol and Gas Experiment (SAGE). A summary of eight years of HIRS data will be published in late 1998. Important information from this study are: 1) cirrus clouds cover most of the earth, 2) they are found about 40% of the time globally, 3) in the tropics cirrus cloud frequencies are even higher, from 80-100%, 4) there is slight evidence that cirnis cloud cover is increasing in the northern hemisphere at about 0.5% per year, and 5) cirrus clouds have an average infrared transmittance of about 40% of the terrestrial radiation. (5) Global Cloud Frequency Statistics published on the Principal Investigator's web page have been used in the planning of the future CRYSTAL experiment and have been used for refinements of a global numerical model operated at the Colorado State University.

Wylie, Donald P.↗