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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 109 records · Page 6
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DOE OSTI2025

Elucidating Processes Controlling Arctic Atmospheric Aerosol Sources, Aging, and Mixing States (Final Report)

Atmospheric aerosols play critical roles in the Earth’s energy budget, directly by scattering or absorbing solar and terrestrial radiation and indirectly by serving as seeds (nuclei) for cloud droplet and ice crystal formation and by depositing on snow and ice surface, thereby changing the surface albedo. These effects are dependent on aerosol particle size and chemical composition and impact the hydrological cycle as well. This project provided single-particle size and chemical composition measurements across the entire annual cycle in the high Arctic and in the Alaskan Arctic during fall – winter, addressing the most significant gaps in Arctic aerosol observational data. These needs were based on recent rapid sea ice loss across the entire Arctic, as well as the major annual delays in sea ice freeze-up during fall in the Chukchi Sea and increased wintertime sea ice fracturing in the Beaufort Sea, both off the North Slope of Alaska. Two DOE Atmospheric Radiation Measurement (ARM) field campaigns were conducted for atmospheric aerosol sampling. The Aerosols during the Polar Utqiagvik Night (APUN – ‘snow on ground’ in Iñupiaq) ARM field campaign at Utqagivik, Alaska was conducted from Oct. 28 – Dec. 22, 2018. Aerosol sizing instrumentation and a single-particle mass spectrometer were successfully deployed for size-resolved number concentration measurements and measurements of individual particle size and chemical composition, respectively. These results show the influence of locally-produced sea spray aerosol, with high cloud-forming potential, due to delayed sea ice freeze-up in the fall. During the 2019‐2020 international Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition, daily atmospheric aerosol particles were collected aboard the German icebreaker Polarstern in the Central Arctic from Nov. 2019 – Oct. 2020. Sea salt aerosol and marine organics were observed year-round during MOSAiC with varying morphologies and sources. These findings are important because most Arctic models do not include a sea spray aerosol source, despite this source increasing with declining sea ice extent. In addition to collecting new samples and data, this project also conducted further analysis of previously collected single-particle chemical composition measurements within the North Slope of Alaska oil fields and at Utqiaġvik, AK, during Aug. – Sep. 2015 and 2016 field campaigns. This work resulted in the discovery of chemical reactions of oil field combustion emissions occurring within fog droplets across the North Slope of Alaska and forming secondary aerosol, showing the impact of Arctic oil field emissions beyond black carbon aerosol and greenhouse gases. In addition, the distribution of chemical species across the aerosol population within the oil fields was quantified, using these data and a previously development framework. We also presented the first ambient evidence of the collision of two atmospheric particles resulting in formation of an organic-coated ammonium sulfate particle of marine origin, which has implications for cloud formation with declining sea ice extent. Overall, this project has elucidated connections between seawater biogeochemistry, resource extraction activities, atmospheric composition, clouds, and the energy budget of the Arctic region. The results of this project are expected to improve weather and sea ice forecasting for security and development in the Arctic and beyond.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1971

Climatology of Urban-regional Systems

Urbanized areas have come to be significant if not dominant components of many regional land surfaces. They represent perhaps the most dramatic recent change man has made in his environment - a change that may well burgeon in the foreseeable future as greater percentages of world populations crowd into metropolitan areas. The climate of urban-regional systems is involved because temperature, air, and pollutants added to the air are significant aspects of this change. During the past two years, substantial progress has been made in the application of remote sensing techniques to the study of urban climatology by programs jointly sponsored by NASA and the United States Geological Survey. The initial effort has endeavored with considerable success to map terrestrial radiation emission or the general thermal state of the land surface with the aid of imaging radiometers (mechanical-optical scanners).

Pease, R. W.↗
NASA NTRS1974

The GISS model of the global atmosphere

A description and numerical results are presented for a global atmospheric circulation model developed at the Goddard Institute for Space Studies (GISS). The model version described is a 9-level primitive-equation model in sigma coordinates. It includes a realistic distribution of continents, oceans and topography. Detailed calculations of energy transfer by solar and terrestrial radiation make use of cloud and water vapor fields calculated by the model. The model hydrologic cycle includes two precipitation mechanisms: large-scale supersaturation and a parameterization of subgrid-scale cumulus convection. Results are presented both from a comparison of the 13th to the 43rd days (January) of one integration with climatological statistics, and from five short-range forecasting experiments. In the extended integration, the near-equilibrium January-mean model atmosphere exhibits an energy cycle in good agreement with observational estimates, together with generally realistic zonal mean fields of winds, temperature, humidity, transports, diabatic heating, evaporation, precipitation, and cloud cover.

Somerville, R. C. J.↗
NASA NTRS1975

The correlation of Skylab L-band brightness temperatures with antecedent precipitation

The S194 L-band radiometer flown on the Skylab mission measured terrestrial radiation at the microwave wavelength of 21.4 cm. The terrain emissivity at this wavelength is strongly dependent on the soil moisture content, which can be inferred from antecedent precipitation. For the Skylab data acquisition pass from the Oklahoma panhandle to southeastern Texas on 11 June 1973, the S194 brightness temperatures are highly correlated with antecedent precipitation from the preceding eleven day period, but very little correlation was apparent for the preceding five day period. The correlation coefficient between the averaged antecedent precipitation index values and the corresponding S194 brightness temperatures between 230 K and 270 K, the region of apparent response to soil moisture in the data, was -0.97. The equation of the linear least squares line is given.

Mcfarland, M. J.↗
NASA NTRS1975

The correlation of Skylab L-band brightness temperatures with antecedent precipitation

The S194 L-band radiometer flown on the Skylab mission measured terrestrial radiation at the microwave wavelength of 21.4 cm. The terrain emissivity at this wavelength is strongly dependent on the soil moisture content, which can be inferred from antecedent precipitation. For the Skylab data acquisition pass from the Oklahoma panhandle to southeastern Texas on 11 June 1973, the S194 brightness temperatures are highly correlated with antecedent precipitation from the preceding eleven day period, but very little correlation was apparent for the preceding five day period. The correlation coefficient between the averaged antecedent precipitation index values and the corresponding S194 brightness temperatures between 230 K and 270 K, the region of apparent response to soil moisture in the data, was -0.97. The equation of the linear least squares line fitted to the data was: API (cm) = 31.99 -0.114 TB (K), where API is the antecedent precipitation index and TB is the S194 brightness temperature.

Mcfarland, M. J.↗
NASA NTRS1976

Estimates of the climatic impact of aerosols produced by Space Shuttles, SST's, and other high flying aircraft

Solar and terrestrial radiative transfer calculations are performed to evaluate the effect of additional aerosols (sulfuric acid, aluminum oxide) produced by aircraft and Space Shuttles flying through the stratosphere on the global heat balance. The results are presented by plotting the dependence of various quantities of interest as a function of the change in the optical depth of the stratosphere at a reference wavelength of 0.55 micron. Perturbation optical depths that will result from the amount of emission expected from supersonic transports (SSTs) and Space Shuttles over the next several decades are determined. The magnitude and importance of the surface temperature change resulting from the added aerosols are assessed. The effect of added aerosols on ozone destruction is evaluated. It is shown that the aerosols produced by SSTs, other high flying aircraft, and Space Shuttles over the next several decades would not seriously alter the climate. However, the effect of SSTs is sufficiently close to the threshold limit, which requires reevaluation as new data are available.

Pollack, J. B.↗
NASA NTRS1977

Atmospheric model development in support of SEASAT. Volume 3: Prediction models

As part of the SEASAT program of NASA, a set of four hemispheric, atmospheric models are developed. The four models use a polar stereographic grid in the horizontal and a sigma coordinate in the vertical. Conservation forms of the difference equations are integrated using either a fifteen or four minute time step on a 381 km or 127 km grid (at 60 deg N) for the 63 x 63 or 187 x 187 models respectively. A nonlinear pressure smoother is used along with momentum and temperature diffusion to help control computational noise. The horizontal boundary conditions are insulated slippery walls. Centered time differencing with time averaging of the pressure gradient force term in the momentum equations is used. Robert time filtering on of the temperature and moisture solutions is used for computational stability. The moisture and heat source/sink terms are modeled. Terms representing evaporation and large scale condensation, sensible heat exchange, parameterized cumulus convection and precipitation, and solar and terrestrial radiation are included. Initialization of the models is based on a pattern conservation technique to obtain objective analysis of the state parameter structure from the surface to 50 mb.

Wellck, R. E.↗
NASA NTRS1978

Properties of the stratospheric aerosol layer studied with a one-dimensional computer model

Aerosol particle effects are often neglected in theoretical studies of stratospheric phenomena. In reality, the particulate matter normally found above the tropopause may influence the terrestrial radiation balance, catalyze heterogeneous chemical interactions, and serve as a tracer of atmospheric motions. The paper proposes a one-dimensional model of the stratospheric aerosol layer, and it is used to compare aerosol theory with observational data. The model considers gaseous sulfur photochemistry and the physical aerosol processes of nucleation, coagulation, sedimentation, and diffusion. Calculations of the effects on the aerosol layer of stratospheric injections of aluminum oxide particles by Space Shuttle engines and of sulfur dioxide molecules by volcanic activity are performed. The relation between measured aerosol variability and changes in stratospheric air temperatures and vertical transport rates are discussed.

Turco, R. P.↗
NASA NTRS1991

Remote sensing of Earth's atmosphere and surface using a digital array scanned interferometer: A new type of imaging spectrometer

The capabilities of the digital array scanned interferometer (DASI) class of instruments for measuring terrestrial radiation fields over the visible to mid-infrared are evaluated. DASI's are capable of high throughput, sensitivity and spectral resolution and have the potential for field-of-view spatial discrimination (an imaging spectrometer). The simplicity of design and operation of DASI's make them particularly suitable for field and airborne platform based remote sensing. The long term objective is to produce a versatile field instrument which may be applied toward a variety of atmospheric and surface studies. The operation of DASI and its advantages over other spectrometers are discussed.

Hammer, Philip D.↗
NASA NTRS1982

NASA Experiment on Tropospheric-Stratospheric Water Vapor Transport in the Intertropical Convergence Zone

The following six papers report preliminary results obtained from a field experiment designed to study the role of tropical cumulo-nimbus clouds in the transfer of water vapor from the troposphere to the stratosphere over the region of Panama. The measurements were made utilizing special NOAA enhanced IR satellite images, radiosonde-ozonesondes and a NASA U-2 aircraft carrying. nine experiments. The experiments were provided by a group of NASA, NOAA, industry, and university scientists. Measurements included atmospheric humidity, air and cloud top temperatures, atmospheric tracer constituents, cloud particle characteristics and cloud morphology. The aircraft made a total of eleven flights from August 30 through September 18, 1980, from Howard Air Force Base, Panama; the pilots obtained horizontal and vertical profiles in and near convectively active regions and flew around and over cumulo-nimbus towers and through the extended anvils in the stratosphere. Cumulo-nimbus clouds in the tropics appear to play an important role in upward water vapor transport and may represent the principal source influencing the stratospheric water vapor budget. The clouds provide strong vertical circulation in the troposphere, mixing surface air and its trace materials (water vapor, CFM's sulfur compounds, etc.) quickly up to the tropopause. It is usually assumed that large scale mean motions or eddy scale motions transport the trace materials through the tropopause and into the stratosphere where they are further dispersed and react with other stratospheric constituents. The important step between the troposphere and stratosphere for water vapor appears to depend upon the processes occurring at or near the tropopause at the tops of the cumulo-nimbus towers. Several processes have been sugested: (1) The highest towers penetrate the tropopause and carry water in the form of small ice particles directly into the stratosphere. (2) Water vapor from the tops of the cumulonimbus clouds is transported somehow through the tropopause, the vapor pressure being controlled by the temperature at the tops of the clouds; the dryness of the stratosphere could be explained if most of the transport occurs in connection with very high clouds in regions with very high and cold tropopause. (3) Cumulo-nimbus anvils act as terrestrial-radiation shields allowing the ice particle temperatures near cloud tops to cool radiatively below the supersaturation point; this cooling would cause a vapor deposition on the ice particles which will settle out and thus act as water scavengers. The experiment was designed to collect information on these detailed physical processes near and above the tropopause in order to assess their importance and the role they play in controlling stratospheric water vapor humidity.

Page, William A.↗
NASA NTRS1994

Atmospheric Aerosols

Aerosols, defined as particles and droplets suspended in air, are always present in the atmosphere. They are part of the earth-atmosphere climate system, because they interact with both incoming solar and outgoing terrestrial radiation. They do this directly through scattering and absorption, and indirectly through effects on clouds. Submicrometer aerosols usually predominate in terms of number of particles per unit volume of air. They have dimensions close to the wavelengths of visible light, and thus scatter radiation from the sun very effectively. They are produced in the atmosphere by chemical reactions of sulfur-, nitrogen- and carbon-containing gases of both natural and anthropogenic origins. Light absorption is dominated by particles containing elemental carbon (soot), produced by incomplete combustion of fossil fuels and by biomass burning. Light-scattering dominates globally, although absorption can be significant at high latitudes, particularly over highly reflective snow- or ice-covered surfaces. Other aerosol substances that may be locally important are those from volcanic eruptions, wildfires and windblown dust.

Pueschel, R. F.↗
NASA NTRS1998

Stratospheric Aerosol Measurements

Stratospheric aerosols affect the atmospheric energy balance by scattering and absorbing solar and terrestrial radiation. They also can alter stratospheric chemical cycles by catalyzing heterogeneous reactions which markedly perturb odd nitrogen, chlorine and ozone levels. Aerosol measurements by satellites began in NASA in 1975 with the Stratospheric Aerosol Measurement (SAM) program, to be followed by the Stratospheric Aerosol and Gas Experiment (SAGE) starting in 1979. Both programs employ the solar occultation, or Earth limb extinction, techniques. Major results of these activities include the discovery of polar stratospheric clouds (PSCs) in both hemispheres in winter, illustrations of the impacts of major (El Chichon 1982 and Pinatubo 1991) eruptions, and detection of a negative global trend in lower stratospheric/upper tropospheric aerosol extinction. This latter result can be considered a triumph of successful worldwide sulfur emission controls. The SAGE record will be continued and improved by SAGE III, currently scheduled for multiple launches beginning in 2000 as part of the Earth Observing System (EOS). The satellite program has been supplemented by in situ measurements aboard the ER-2 (20 km ceiling) since 1974, and from the DC-8 (13 km ceiling) aircraft beginning in 1989. Collection by wire impactors and subsequent electron microscopic and X-ray energy-dispersive analyses, and optical particle spectrometry have been the principle techniques. Major findings are: (1) The stratospheric background aerosol consists of dilute sulfuric acid droplets of around 0.1 micrometer modal diameter at concentration of tens to hundreds of monograms per cubic meter; (2) Soot from aircraft amounts to a fraction of one percent of the background total aerosol; (3) Volcanic eruptions perturb the sulfuric acid, but not the soot, aerosol abundance by several orders of magnitude; (4) PSCs contain nitric acid at temperatures below 195K, supporting chemical hypotheses implicating manmade fluorocarbons as cause of the --'ozone hole'; (5) The current soot loading is too small to be of environmental (radiative and chemical) consequence. However, the fractal nature of soot distinguishes it aerodynamically and radiatively from sulfuric acid droplets such that its stratospheric residence time is longer, mainly because of vertical transport against gravity due to gravito-photophoretic forces. Thus it may accumulate and become of environmental concern in the future.

Pueschel, Rudolf, F.↗
NASA NTRS2011

Biological Based Risk Assessment for Space Exploration

Exposures from galactic cosmic rays (GCR) - made up of high-energy protons and high-energy and charge (HZE) nuclei, and solar particle events (SPEs) - comprised largely of low- to medium-energy protons are the primary health concern for astronauts for long-term space missions. Experimental studies have shown that HZE nuclei produce both qualitative and quantitative differences in biological effects compared to terrestrial radiation, making risk assessments for cancer and degenerative risks, such as central nervous system effects and heart disease, highly uncertain. The goal for space radiation protection at NASA is to be able to reduce the uncertainties in risk assessments for Mars exploration to be small enough to ensure acceptable levels of risks are not exceeded and to adequately assess the efficacy of mitigation measures such as shielding or biological countermeasures. We review the recent BEIR VII and UNSCEAR-2006 models of cancer risks and their uncertainties. These models are shown to have an inherent 2-fold uncertainty as defined by ratio of the 95% percent confidence level to the mean projection, even before radiation quality is considered. In order to overcome the uncertainties in these models, new approaches to risk assessment are warranted. We consider new computational biology approaches to modeling cancer risks. A basic program of research that includes stochastic descriptions of the physics and chemistry of radiation tracks and biochemistry of metabolic pathways, to emerging biological understanding of cellular and tissue modifications leading to cancer is described.

Cucinotta, Francis A.↗