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At least 109 records · Page 6

Comparisons of Satellite Retrieval of Aerosol Properties from SeaWiFS and TOMS to the AERONET Measurements during ACE-Asia

The primary goal of the ACE (Aerosol Characterization Experiment)-Asia mission is to increase our understanding of how atmospheric aerosol particles over the Asian-Pacific region affect the Earth climate system. In support of the day-to-day flight planning of ACE-Asia, we built a near real-time system to provide satellite data from the polar-orbiting instruments Earth Probe TOMS (Total Ozone Mapping Spectrometer) (in the form of absorbing aerosol index) and SeaWiFS (Sea-Viewing Wide Field-of-View Sensor) (in the form of aerosol optical thickness and Angstrom exponent). The results were available via web access. These satellite data provide a 'big picture' of aerosol distribution in the region, which is complementary to the ground based measurements. In this paper, we will briefly discuss the algorithms used to generate these data. The retrieved aerosol optical thickness and Angstrom exponent from SeaWiFS will be compared with those obtained from various AERONET (Aerosol Robotic Network) sites over the Asian-Pacific region. The TOMS aerosol index will also be compared with AERONET aerosol optical thickness over different aerosol conditions. Finally, we will discuss the climate implication of our studies using the combined satellite and AERONET observations.

Hsu, Christina N.↗

Three Years of Airborne Observations During NASA Activate: A Statistical Summary of Chemical, Optical, and Microphysical Aerosol Properties Over the Western North Atlantic Ocean

Airborne observations are critical to understanding Earth’s climate system and surface-level air quality by providing both spatial and vertical information that is not possible through ground measurement networks or satellite observations. Airborne platforms allow assessments of long-range transport, vertical redistribution, boundary-layer dynamics, and cloud-aerosol-interactions that are critical to model evaluation and satellite validation. Still, the high cost and effort of aircraft operations can limit measurement campaigns to short, focused time periods. Multiple deployments are often necessary for seasonal comparisons, and results can be limited if target phenomenon are infrequent. Subsequent analyses typically focus on case studies, especially if deployment conditions are climatologically anomalous. The NASA ACTIVATE (Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment) mission was designed to overcome these limitations by operating semi-continuously over multiple months during multiple seasons. Flight plans were intentionally simple, repetitive, and systematic to provide a statistically robust dataset that could be utilized similarly to a ground-network. Here, we present an overview of three years (2020-2022) of aerosol measurements from the NASA HU-25 Falcon aircraft supporting the ACTIVATE mission. Data from 179 flights were considered, the majority of which were based at NASA Langley Research Center and flown locally over the Wester North Atlantic Ocean just east of Hampton, VA, USA. Airmass characteristics tended to transition from continental outflow near the coast to mostly marine over the open ocean. Seasonal, diurnal, spatial, and vertical trends in aerosol microphysical, optical, and chemical properties are discussed in the context of synoptic scale meteorology. Statistical benefits of the ACTIVATE sampling strategy are discussed with regard to future model evaluation.

Luke D Ziemba↗

Two-Channel Satellite Retrievals of Aerosol Properties: An Overview

In order to reduce current uncertainties in the evaluation of the direct and indirect effects of tropospheric aerosols on climate on the global scale, it has been suggested to apply multi-channel retrieval algorithms to the full period of existing satellite data. This talk will outline the methodology of interpreting two-channel satellite radiance data over the ocean and describe a detailed analysis of the sensitivity of retrieved aerosol parameters to the assumptions made in different retrieval algorithms. We will specifically address the calibration and cloud screening issues, consider the suitability of existing satellite data sets to detecting short- and long-term regional and global changes, compare preliminary results obtained by several research groups, and discuss the prospects of creating an advanced retroactive climatology of aerosol optical thickness and size over the oceans.

Mishchenko, Michael I.↗

Airborne Observations of Aerosol Properties in Southeast Asia: Overview of Emissions, Cloud Processing, and Long Range Transport during NASA CAMP2Ex

The Southwest Monsoon represents an important synoptic scale meteorological feature that modulates precipitation throughout Southeast Asia. In addition, southwesterly flow can funnel large amounts of biomass burning aerosol into heavily populated areas throughout the Philippines, mixing with urban emissions and representing a significant air quality issue. From a climate perspective, understanding interactions between these particles and clouds has important societal ramifications through frequent extreme periods of flood and drought. Here we present airborne observations made in support of the NASA CAMP2Ex (Cloud and Aerosol Monsoonal Processes-Philippines Experiment) mission aboard the Wallops Flight Facility P-3 research aircraft, based at Clark International Airport in the Luzon region of Northern Philippines. Nineteen research flights were conducted in August-October of 2019. An extensive suite of aerosol microphysical, optical, and chemical instrumentation was deployed, along with trace gas and remote sensing measurements, to characterize aerosol emissions and their vertical/spatial variability associated with moderately convective marine cloud systems in the region. Analysis will focus on characterizing disparate aerosol sources with respect to derived chemical and optical properties relevant to global circulation modeling. For example, higher than expected mass scattering efficiencies for aged biomass burning emissions, derived from a combination of nephelometer and aerosol mass spectrometer measurements, are attributed to increased particle size and decreased density. Results will also illustrate the evolution of aerosols from Indonesian agricultural biomass burning activities into the Philippines region, in comparison with urban emissions from the megacity Manila and transported air masses from mainland Asia.

Luke David Ziemba↗

Response to "Toward Unified Satellite Climatology of Aerosol Properties. 3. MODIS Versus MISR Versus AERONET"

A recent paper by Mishchenko et al. compares near-coincident MISR, MODIS, and AERONET aerosol optical depth (AOD) products, and reports much poorer agreement than that obtained by the instrument teams and others. We trace the reasons for the discrepancies primarily to differences in (1) the treatment of outliers, (2) the application of absolute vs. relative criteria for testing agreement, and (3) the ways in which seasonally varying spatial distributions of coincident retrievals are taken into account.

Kahn, Ralph A.↗

Response to Toward Unified Satellite Climatology of Aerosol Properties: MODIS versus MISR versus AERONET - 3

A recent paper by Mishchenko et al. compares near-coincident MISR, MODIS, and AERONET aerosol optical depth (AOD), and gives a much less favorable impression of the utility of the satellite products than that presented by the instrument teams and other groups. We trace the reasons for the differing pictures to whether known and previously documented limitations of the products are taken into account in the assessments. Specifically, the analysis approaches differ primarily in (1) the treatment of outliers, (2) the application of absolute vs. relative criteria for testing agreement, and (3) the ways in which seasonally varying spatial distributions of coincident retrievals are taken into account. Mishchenko et al. also do not distinguish between observational sampling differences and retrieval algorithm error. We assess the implications of the different analysis approaches, and cite examples demonstrating how the MISR and MODIS aerosol products have been applied successfully to a range of scientific investigations.

Kahn, Ralph A.↗

Toward Unified Satellite Climatology of Aerosol Properties. 3. MODIS Versus MISR Versus AERONET

We use the full duration of collocated pixel-level MODIS-Terra and MISR aerosol optical thickness (AOT) retrievals and level 2 cloud-screened quality-assured AERONET measurements to evaluate the likely individual MODIS and MISR retrieval accuracies globally over oceans and land. We show that the use of quality-assured MODIS AOTs as opposed to the use of all MODIS AOTs has little effect on the resulting accuracy. The MODIS and MISR relative standard deviations (RSTDs) with respect to AERONET are remarkably stable over the entire measurement record and reveal nearly identical overall AOT performances of MODIS and MISR over the entire suite of AERONET sites. This result is used to evaluate the likely pixel-level MODIS and MISR performances on the global basis with respect to the (unknown) actual AOTs. For this purpose, we use only fully compatible MISR and MODIS aerosol pixels. We conclude that the likely RSTDs for this subset of MODIS and MISR AOTs are 73% over land and 30% over oceans. The average RSTDs for the combined [AOT(MODIS)+AOT(MISR)]/2 pixel-level product are close to 66% and 27%, respectively, which allows us to recommend this simple blend as a better alternative to the original MODIS and MISR data. These accuracy estimates still do not represent the totality of MISR and quality-assured MODIS pixel-level AOTs since an unaccounted for and potentially significant source of errors is imperfect cloud screening. Furthermore, many collocated pixels for which one of the datasets reports a retrieval, whereas the other one does not may also be problematic.

Mishchenko, Michael I.↗

Remote Marine Aerosol Properties over the Western North Atlantic Ocean during NAAMES

The overarching goal of this postdoctoral project is: quantitatively assess and constrain the aerosol budgets in the remote North Atlantic marine boundary layer, under a wide range of aerosol emission sources, meteorological states to improve process-level understanding of marine aerosol-cloud interactions critical to adequately link observations and climate modelling.

Aerosol NAAMES↗

Dissipation of Mixed-Phase Arctic Clouds and Its Relationship to Aerosol Properties - Final Technical Report

The overarching objective of this project was to further our understanding of low-level Arctic cloud behavior in ultra-low aerosol concentration environments. To this end, we used a combination of modeling and analysis of DOE ARM datasets to understand the frequency of aerosol-limited cloud dissipation events, to understand the microphysical processes that lead to aerosol-limited dissipation, and to understand how above-cloud aerosol particles can work to maintain low-level clouds that exist in boundary layers with ultra-low aerosol concentrations. We found that aerosol-limited dissipation is unlikely to occur at the DOE long-term observation facilities at North Slope Alaska and Oliktok Point but possibly does occur at higher latitudes in the Arctic. At these higher latitudes, aerosol concentrations are frequently observed to be higher, often substantially higher, than in the boundary layer. These reservoirs can be sufficient to maintain low-level clouds. When they are insufficient, clouds appear to dissipate due to a depletion of liquid water through precipitation that is reinforced by a shutdown of the dynamical processes that support these clouds.

54 ENVIRONMENTAL SCIENCES↗

Measurements of aerosol properties needed to infer backscatter characteristics in support of the NASA Doppler Lidar program

During the first year two areas of work were emphasized, analysis of aerosol data to provide improved estimates of backscatter over the Pacific ocean and development of a global model for backscatter at different wavelengths and preparation and planning for the aircraft flights of the GLOVE program. Significant progress was made in each of these areas. The analytical work is a continuation of the GAMETAG analysis, and was directed toward the development of a backscatter model for the Pacific Oceanic free troposphere. This has included a further evaluation of relationships between the optical effects at different wavelengths, a comparison of modeled optical effects at differing temporal resolutions, and an investigation of the effects of sampling on the modeled results. An initial investigation of the predictability of 9 to 10 micrometers Beta values from other data sets as well as some preliminary comparisons of the modeling results with experimental data. The comparison of the optical effects was extended to make the comparisons for different sets of time bases between 1 and 20 minutes.

Patterson, E. M.↗

Modelling atmospheric aerosol backscatter at CO2 laser wavelengths. I - Aerosol properties, modeling techniques, and associated problems. II - Modeled values in the atmosphere. III - Effects of changes in wavelength and ambient conditions

The various methods of calculating the atmospheric aerosol backscattering function, beta(CO2), both from measured aerosol characteristics and from optical measurements made at other wavelengths, are discussed in detail, with limits placed on their accuracy. The most significant factor in determining beta(CO2) is found to be the aerosol size distribution and concentration; this should be known accurately for particle radii up to at least 1 micron for stratospheric particles and 5 microns for tropospheric particles. Results are then presented from the modeling of the aerosol backscattering function at a wavelength of 10.6 microns in the lowest 20 km of the atmosphere. It is found that beta(CO2) varies from 10 to the -6th per m per sr in the planetary boundary layer to less than 10 to the -11th per m per sr in the stratosphere. It is next shown that, with the exception of (NH4)2SO4-containing aerosols, whose size distributions have relatively large numbers of small particles, the variation of backscattering with CO2 wavelength is less than a factor of approximately 3. For such (NH4)2SO4 aerosol distributions, however, the variation of backscatter function with CO2 wavelengths between 9.1 and 11.1 microns may reach one order of magnitude.

Kent, G.S.↗