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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 109 records · Page 6
All sourcesNASA NTRSDOE OSTI
DOE OSTI2016

Synchrotron X-ray microbeam diffraction measurements of full elastic long range internal strain and stress tensors in commercial-purity aluminum processed by multiple passes of equal-channel angular pressing

Synchrotron X-ray microbeam diffraction was used to measure the full elastic long range internal strain and stress tensors of low dislocation density regions within the submicrometer grain/subgrain structure of equal-channel angular pressed (ECAP) aluminum alloy AA1050 after 1, 2, and 8 passes using route B C . This is the first time that full tensors were measured in plastically deformed metals at this length scale. The maximum (most tensile or least compressive) principal elastic strain directions for the unloaded 1 pass sample for the grain/subgrain interiors align well with the pressing direction, and are more random for the 2 and 8 pass samples. The measurements reported here indicate that the local stresses and strains become increasingly isotropic (homogenized) with increasing ECAP passes using route BC. The average maximum (in magnitude) LRISs are -0.43 σ a for 1 pass, -0.44 σ a for 2 pass, and 0.14 σ a for the 8 pass sample. Furthermore, these LRISs are larger than those reported previously because those earlier measurements were unable to measure the full stress tensor. Significantly, the measured stresses are inconsistent with the two-component composite model.

36 MATERIALS SCIENCE↗
DOE OSTI2015

Investigation of specimen size effects by in-situ microcompression of equal channel angular pressed copper

Here, micropillar compression testing was implemented on Equal Channel Angular Pressed copper samples ranging from 200 nm to 10 µm in side length in order to measure the mechanical properties yield strength, first load drop during plastic deformation at which there was a subsequent stress decrease with increasing strain, work hardening, and strain hardening exponent. Several micropillars containing multiple grains were investigated in a 200 nm grain sample. The effective pillar diameter to grain size ratios, D/d , were measured to be between 1.9 and 27.2. Specimens having D/d ratios between 0.2 and 5 were investigated in a second sample that was annealed at 200 °C for 2 h with an average grain size of 1.3 µm. No yield strength or elastic modulus size effects were observed in specimens in the 200 nm grain size sample. However work hardening increases with a decrease in critical ratios and first stress drops occur at much lower stresses for specimens with D/d ratios less than 5. For comparison, bulk tensile testing of both samples was performed, and the yield strength values of all micropillar compression tests for the 200 nm grained sample are in good agreement with the yield strength values of the tensile tests.

36 MATERIALS SCIENCE↗
DOE OSTI2016

Description of alpha decay and cluster radioactivity in the dinuclear system model

A unified description of cluster radioactivity and α-decay of cold nuclei in the dinuclear system model is proposed. Quantum dynamical fluctuations along the charge (mass) asymmetry coordinate determine the spectroscopic factor, and tunneling along the relative distance coordinate determines the penetrability of the barrier of the nucleus–nucleus interaction potential. A new method for calculating the spectroscopic factor is proposed. The hindrance factors for the orbital angular momentum transfer are studied. A potential reason for the half-life to deviate from the Geiger–Nuttall law in α-decays of neutron-deficient nuclei {sup 194,} {sup 196}Rn is found. The fine structure of α-decays of U and Th isotopes is predicted and characterized. The model is used to describe α-decays from the rotational band of even–even nuclei. The known half-lives in the regions of “lead” and “tin” radioactivities are reproduced well, and the most probable cluster yields are predicted. The cluster decay of excited nuclei is discussed. The relation of cluster radioactivity to spontaneous fission and highly deformed nuclear states is analyzed.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2017

Radiation instability of equal channel angular extruded T91 at ultra-high damage levels

Although several studies have shown that nano-grained alloys have higher radiation resistance than coarse-grained variants, with dense grain boundary structures acting as defect sinks to remove damage, the present study shows the failure of severe deformation to suppress void swelling in T91 alloy at ultra-high damage levels. Fe self-ion irradiation up to 1000 peak dpa produced significantly more swelling in extruded T91 than conventional T91 at 475 °C. Dramatic radiation-enhanced grain growth was observed in the extruded T91, manifested in two rapid grain growth stages. One stage occurs at a relatively low damage level, and the other at a higher damage level beyond 750 peak dpa. The second rapid growth stage is correlated with void swelling and starts at the end of the swelling incubation period. The study suggests that the defect sink properties of the growing grain boundaries under a coarsening process are different from that of stable boundary configurations. When void swelling becomes significant and voids act as a biased sink for vacancies, the growing grain boundaries act as a biased sink for interstitials, leading to rapid growth at higher damage levels.

36 MATERIALS SCIENCE↗
DOE OSTI2025

Gamma Decay of the 154 Sm Isovector Giant Dipole Resonance: Smekal-Raman Scattering as a Novel Probe of Nuclear Ground-State Deformation

𝛾 decays of the isovector giant dipole resonance (IVGDR) of the deformed nucleus 154 Sm were measured using 2$^{+}_{1}$-Smekal-Raman and elastic scattering of linearly polarized, quasimonochromatic photon beams. The two scattering processes were disentangled through their distinct angular distributions. Their branching ratio and cross sections were determined at six excitation energies covering the 154 Sm IVGDR. Both agree with the predictions of the geometrical model for the IVGDR and confirm 𝛾 decay as an observable sensitive to the structure of the resonance. Consequently, the data place strong constraints on the nuclear shape, including the degree of triaxiality. The derived 154 Sm shape parameters 𝛽 = 0.2925⁢(25) and 𝛾 = 5.0⁢(15)° agree well with other measurements and recent Monte Carlo shell-model calculations.

150 ≤ A ≤ 189↗
DOE OSTI2018

54 Fe neutron elastic and inelastic scattering differential cross sections from 2–6 MeV

Measurements of neutron elastic and inelastic scattering cross sections from 54 Fe were performed for nine incident neutron energies between 2 and 6 MeV. Measured differential scattering cross sections are compared to those from previous measurements and the ENDF, JENDL, and JEFF data evaluations. TALYS calculations were performed and modifications of the default parameters are found to better describe the experimental cross sections. A spherical optical model treatment is generally adequate to describe the cross sections in this energy region; however, in 54 Fe the direct coupling is found to increase suddenly above 4 MeV and requires an increase in the DWBA deformation parameter by approximately 25%. Furthermore, this has little effect on the elastic scattering differential cross sections but makes a significant improvement in both the strength and shape of the inelastic scattering angular distribution, which are found to be very sensitive to the size and extent of the surface absorption region.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2016

Microstructure characterization of LAE442 magnesium alloy processed by extrusion and ECAP

The magnesium alloy LAE442 was processed by extrusion and equal channel angular pressing (ECAP) to achieve ultrafine grained microstructure. Detailed characterization of the microstructure was performed by scanning electron microscope, electron back scattered diffraction (EBSD) and transmission electron microscope. The initial, as-cast, microstructure consisted of large grains of ~ 1 mm. The grain refinement due to the processing by severe plastic deformation led to a decrease of the average grain size to ~ 1.7 μm after the final step of ECAP. A detailed characterization of secondary phases showed the precipitation of Al{sub 11}RE{sub 3}, Al{sub 2}Ca and Al{sub 10}RE{sub 2}Mn{sub 7} intermetallic phases. X-ray diffraction measurements proved that Li is dissolved within the magnesium matrix in the as-cast condition. Newly formed Al{sub 3}Li phase was observed after ECAP. The texture formation due to the extrusion and ECAP was different from that in the other magnesium alloys due to the activation of non-basal slip systems as a result of the decrease of the c/a ratio. - Highlights: • Combined extrusion and equal channel angular pressing results in significant grain refinement by factor 1000 approximately. • Al{sub 11}RE{sub 3}, Al{sub 2}Ca and Al{sub 10}RE{sub 2}Mn{sub 7} secondary phases are present in the as-cast material while Li was dissolved in the Mg matrix. • Extrusion and ECAP have no effect on the composition of the secondary phases but they influence strongly their distribution. • Texture evolution is affected by decrease of c/a ratio due to the presence of Li and resulting activation of non-basal slip.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Modeling the dynamic response of rock masses with multiple compliant fluid saturated joint sets—Part I: Mesoscale simulations

Recently a mesoscale model was developed that includes thermomechanically consistent constitutive equations with dissipation due to porous compaction, inelastic distortional deformation rate, and slipping on persistent dry joint surfaces. In this Part I of a two-part paper, we describe enhancements of the mesoscale model which include: normal compliance with hysteresis, non-persistent joints with finite area, joint sets with angular deviation, and the weakening effect of fluid pressure in the joints. Examples study the influences of these effects on average strength. These computationally expensive simulations are used to inspire functional forms in a continuum model, described in Part II, which is needed for large scale simulations of real applications.

42 ENGINEERING↗
DOE OSTI2019

Effect of ECAP Die Angles on Microstructure Mechanical Properties and Corrosion Behavior of AZ80 Mg Alloy

In this article, the effect of channel angles on material properties was investigated during equal channel angular pressing of AZ80 magnesium alloy using processing route R at 325 °C processing temperature. Channel angles of 90° and 110° and common corner angle 30° have been considered for this study. It has been revealed that the channel angle has a significant influence on deformation homogeneity, microhardness, ultimate tensile strength, ductility and corrosion behavior of Mg alloys. Investigation with reference to as-received AZ80 Mg alloy indicates 18.47% improvement in UTS and 76.07% enhancement in ductility after processing through 3P-90° and 2P-110° ECAP, respectively. Also, the corrosion rate reduces to 89.47% after processing the sample with 3P-110° ECAP die.

36 MATERIALS SCIENCE↗
DOE OSTI2019

A New Approach for Consolidation of Pure Magnesium Powder Using an Integrated Severe Plastic Deformation Route

In this paper, a new approach using a novel severe plastic deformation route is presented for consolidation and processing of a high-density and ultrafine-grained pure magnesium. Pure magnesium particles were successfully consolidated at 400 °C into a sufficiently dense bulk material using a new combined method including cyclic extrusion compression, equal channel angular pressing (ECAP) and conventional extrusion. The grain refinement, consolidation behavior and mechanical properties were deeply investigated. Results showed that the as-consolidated material had a fine grain structure with excellent tensile strength and ductility compared to as-cast and as-ECAPed specimens. Vickers microhardness increased from 38.75 to 52.58 during the process. Porosity also reduced considerably from 12.55 to 1.2% during the process which led to a dense bulk material. Results indicate that the introduced method is a promising and effective process for producing strong bulk materials from metal powders.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Chiral-like doublet band structure and octupole correlations in 104 Ag

The nature of the yrast negative-parity band and its chiral-like partner band in 104 Ag is investigated experimentally and theoretically. Lifetimes of states in the negative-parity yrast band and positive-parity band based on the 4424-keV level are measured using Doppler shift attenuation technique. Lifetimes of three more states have been determined along with the upper limit for the lifetime of the highest observed yrast states. Further, lifetimes known from earlier studies are determined with better precision. The level scheme of 104 Ag has also been extended with the addition of new enhanced E1 transitions linking the positive-parity band based on the 4424-keV levels and the yrast negative-parity and its partner band. B(E1) and/or B(E1)/B(M1) values for the transitions from the positive-parity band to the yrast and its partner band have been determined for the first time; these suggest strong octupole correlation between the positive-parity and the negative-parity bands. Here, calculations based on the triaxial projected shell model (TPSM) and covariant density functional theory (CDFT) have been performed to unravel the intrinsic structures of the partner band and the excited positive-parity band. TPSM calculations predict that doublet bands have significant angular momentum contributions along the three principle axes, suggesting that bands could have chiral symmetry breaking origin. The CDFT calculations predict a π(g 9/2 ) -1 Ⓧν(h 11/2 )(g 7/2 ,d 5/2 ) 2 aligned quasiparticle configuration for the negative-parity doublet bands with deformation parameters β≈0.20 and γ≈5°. The partner band could be interpreted as a chiral vibration mode built on top of the yrast band. The excited positive-parity band is predicted to have aligned four quasiparticle configurations, namely, π(g 9/2 ) -1 Ⓧν(h 11/2 ) 2 (g 7/2 ,d 5/2 ) 1 . Further, these calculations predict significant octupole softness in 104 Ag which could be the reason for enhanced E1 transitions between the four quasiparticle positive-parity bands and the doublet negative-parity bands.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Non-Synchronous Rotation on Europa Driven by Ocean Currents

It has been suggested that the ice shell of Jupiter's moon Europa may drift non-synchronously due to tidal torques. Here we argue that torques applied by the underlying ocean are also important and can result in non-synchronous rotation. The resulting spin rate can be slightly slower than the synchronous angular rate that would have kept the same point of the ice shell facing Jupiter. We develop an ice shell rotation model, driven by ocean stress calculated using a high-resolution state-of-the-art ocean general circulation model, and take into account the viscoelastic deformation of the ice shell. We use the ice shell model results together with observed limits on the ice shell drift speed to constrain ice shell parameters such as effective viscosity, which is currently uncertain by at least four orders of magnitude. Our results suggest, at best, sluggish ice shell convection. Depending on the relaxation time scale of the ice shell and on the ocean currents, the ice shell may exhibit negligible drift, constant drift, or oscillatory drift superimposed on random fluctuations. The expected rotation rate exceeds ~30 m/yr; future spacecraft observations can be used to test these predictions and yield insight into the properties of the ice shell and underlying ocean.

15 GEOTHERMAL ENERGY↗
DOE OSTI2018

Sierra/RKPM: Current State and Applications

The Reproducing Kernel Particle Method (RKPM), a meshfree method, has been implemented in Sandia's Sierra/Solid Mechanics in a collaboration between Sandia and the University of California San Diego's Center for Extreme Events Research (UCSD/CEER). Meshfree methods, like RKPM, have an advantage over mesh-based methods, like the Finite Element Method (FEM), in applications where achieving or maintaining a quality mesh becomes burdensome or impractical. For example, using FEM for problems with very large deformations will result in poor element Jacobians which causes problems with the parametric mapping. RKPM constructs the approximation functions in the physical domain, circumventing the parametric mapping issue. Also, reconstructing the approximation functions at very large deformations is straight-forward. RKPM has an advantage over traditional meshfree methods such as Smoothed-Particle Hydrodynamics (SPH) due to its ability to reproduce linear or higher-order functions exactly. This removes the tensile instabilities that are present in SPH and allows preservation of angular momentum. The point of this memo is to explore the capabilities and limitations of the current implementation by testing it on three different applications: 1) a quasi-static ductile shearing problem 2) a dynamic concrete panel perforation problem and 3) a set of dynamic metal panel perforation problems. In summary, areas where RKPM appears to be a promising alternative to current methods have been identified. Also, outstanding inefficiencies and issues (bugs) with code are noted, ways to improve the capabilities using material from literature are mentioned and areas deserving of new research are highlighted.

42 ENGINEERING↗
DOE OSTI2025

Origin of the Low-Energy Enhancement of the γ-Ray Strength Function

The low-energy enhancement (LEE) in γ-ray strength functions has been experimentally identified in a large number of nuclei during the past two decades; however, the origin of the enhancement is not fully understood. Building on previous theoretical work, we investigate the LEE and its relation to the scissors mode (SM) with an independent theoretical approach. We apply a novel angular-momentum-projected shell-model method that explicitly endows degrees of freedom to describe the scissors motion. Taking the recently measured γ-ray strength functions in Neodymium isotopes as examples, we find that the LEE arises from a quasi-free scissors motion appearing only in weakly-deformed nuclei, which can be viewed as an approximate free-rotation of neutrons with respect to protons. This leads us to propose a new type of collective motion, scissors rotation, to contrast the scissors vibration widely known in well-deformed nuclei. The observed LEE is naturally interpreted as the first evidence for this collective excitation mode.

Collective models↗
DOE OSTI2026

Lifetimes of low-lying levels in 158 Gd

The low-lying structure of the well-deformed nucleus 158 Gd has been revisited to elucidate the nature of the low-lying states in 158 Gd. Earlier (p, t) studies identified numerous 0 + states below 4.3 MeV, prompting questions about whether these states correspond to collective vibrations or shape coexistence. New and previously reported (n, n' γ) measurements are combined, including γ-γ coincidences, excitation functions, and angular distributions, to extract lifetimes and transition probabilities for 44 excited states up to 2.7 MeV, including 32 previously unmeasured levels. Our results confirm or revise γ-ray placements and provide detailed transition strengths, revealing both weakly collective and strongly enhanced B(E2) and B(E1) transition probabilities. In particular, a tentative 0 + state at 2437.8 keV exhibits a strong interband B(E2) transition, which may be a candidate for a possible two-phonon (ββ) excitation. Systematic comparisons with neighboring Gd isotopes, Hartree–Fock–Bogoliubov, and interacting-boson model predictions suggest that the first excited 0 + state in 158 Gd is predicted to be a β-vibration, although it is weakly collective.

158Gd↗
DOE OSTI2026

In situ quantification of fracture slip induced by hydraulic injections in a deep borehole: A comparison of two different borehole techniques

In situ measurements of fracture deformation during fluid injection are rare, yet essential for understanding the mechanical response of fractured rock. In this study, we evaluate the reliability of two methods by comparing their slip vector estimates: high-resolution borehole acoustic televiewer images captured before and after injection tests, and displacement data from a three-component borehole deformation probe recorded during the injections. Acoustic televiewer images capture only final in-plane displacement, whereas three-component borehole deformation measurements provide full 3D, transient fracture movement. Four injection tests in a fractured granitic rock mass along an inclined borehole at the Bedretto Underground Laboratory (Switzerland), beneath more than 1100 m of overburden, were analyzed. The two methods yielded consistent kinematics and comparable slip magnitudes, typically in the range of 0.2 – 0.6 mm. Angular differences between estimated slip directions ranged from 0.2° to 28°. For two test intervals with pre-existing fractures optimally oriented for slip, the measured slip vectors agreed with forward-modeled slip vectors based on the regional in situ stress field, supporting the Wallace–Bott hypothesis. Measurable shear displacement was identified in two test intervals containing fractures oriented nearly perpendicular to the least principal stress, including a newly formed hydraulic fracture. This demonstrates that even fractures unfavorably oriented for slip can undergo shear due to local stress perturbations around an inclined borehole.

Acoustic televiewer↗
DOE OSTI2023

Hexadecapole strength in the rare isotopes 74,76 Kr

In the Ge-Sr mass region, isotopes with neutron number N ≤ 40 are known to feature rapid shape changes with both nucleon number and angular momentum. To gain new insights into their structure, inelastic proton scattering experiments in inverse kinematics were performed on the rare isotopes 74,76 Kr. This work focuses on observables related to the J π = $4$$^{+}_{1}$ states of the Kr isotopes and, in particular, on the hexadecapole degree of freedom. By performing coupled-channels calculations, hexadecapole deformation parameters β 4 were determined for the J π = $4$$^{+}_{1}$ states of 74,76 Kr from inelastic proton scattering cross sections. Two possible coupled-channels solutions were found. A comparison to predictions from nuclear energy density functional theory, employing both non-relativistic and relativistic functionals, clearly favors the large, positive β 4 solutions. These β 4 values are unambiguously linked to the well deformed prolate configuration. Given the β 2 - β 4 trend, established in this work, it appears that β 4 values could provide a sensitive measure of the nuclear shell structure.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

Annual Continuation And Progress Report For Low-Energy Nuclear Physics Research At Lawrence Livermore National Laboratory

(I)In this project, the Beta-­decay Paul Trap, an open-­geometry RFQ ion trap that can be instrumented with sophisticated radiation detection arrays, is used for precision β-­decay studies. Measurements of β-­decay angular correlations, which are sensitive to exotic particles and other phenomena beyond the Standard Model (SM) of particle physics that may occur at the TeV-­energy scale, are being performed by taking advantage of the favorable properties of the mirror 8 Li and 8 B β ± decays and the benefits afforded by using trapped ions. By detecting the β and two α particles emitted in these decays, the complete kinematics can be reconstructed. This allows a simultaneous measurement of the β-­n, β-­n-­α, and β-α correlations and a determination of the neutrino energy and momentum event by event. In addition, the 8 B neutrino spectrum, of great interest in solar neutrino oscillation studies, can be determined in a new way. Beta-­delayed neutron spectroscopy is also being performed on neutron-­rich isotopes by studying the β-­decay recoil ions that emerge from the trap with high efficiency, good energy resolution, and practically no backgrounds. This novel technique is being used to study isotopes of mass-­number A~130 in the vicinity of the N=82 neutron magic number to help understand the rapid neutron-­capture process (r-­process) that creates many of the heavy isotopes observed in the cosmos. (II)A year-long CHICO2 campaign at ANL/ATLAS together with GRETINA included a total of 10 experiments, seven with the radioactive beams from CARIBU and three with stable beams, with 82 researchers involved from 27 institutions worldwide. CHICO2 performed flawlessly during this long campaign with achieved position resolution matching to that of GRETINA, which greatly enhances the sensitivity in the study of nuclear γ-­ray spectroscopy. This can be demonstrated in our results on 144 Ba and 146 Ba where the octupole deformation is evident from the measured B(E3; 3 - →0 + ) strengths that significantly greater than the theoretical predictions. We anticipate that CHICO2 will continue to be a viable charged-­particle detector for the research need of the low-­energy nuclear physics community.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗