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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 109 records · Page 6
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Single-Particle Photoluminescence and Dark-Field Scattering during Charge Density Tuning

Single-particle spectroelectrochemistry provides optical insight into understanding physical and chemical changes occurring on the nanoscale. While changes in dark-field scattering during electrochemical charging are well understood, changes to the photoluminescence of plasmonic nanoparticles under similar conditions are less studied. Here, we use correlated single-particle photoluminescence and dark-field scattering to compare their plasmon modulation at applied potentials. We find that changes in the emission of a single gold nanorod during charge density tuning of intraband photoluminescence can be attributed to changes in the Purcell factor and absorption cross section. Lastly, modulation of interband photoluminescence provides an additional constructive observable, giving promise for establishing dual channel sensing in spectroelectrochemical measurements.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Towards the optimization of direct laser acceleration

Experimental measurements using the OMEGA EP laser facility demonstrated direct laser acceleration (DLA) of electron beams to (505 ± 75) MeV with (140 ± 30) nC of charge from a low-density plasma target using a 400 J, picosecond duration pulse. Similar trends of electron energy with target density are also observed in self-consistent two-dimensional particle-in-cell simulations. The intensity of the laser pulse is sufficiently large that the electrons are rapidly expelled from along the laser pulse propagation axis to form a channel. The dominant acceleration mechanism is confirmed to be DLA and the effect of quasi-static channel fields on energetic electron dynamics is examined. A strong channel magnetic field, self-generated by the accelerated electrons, is found to play a comparable role to the transverse electric channel field in defining the boundary of electron motion.

43 PARTICLE ACCELERATORS↗
DOE OSTI2020

Fermi-liquid theory and divergences of the two-particle irreducible vertex in the periodic Anderson lattice

Here we analyze the divergences of the irreducible vertex function in dynamical mean field theory, which may indicate either a nonphysical breakdown of the perturbation theory or a response to some physical phenomenon. To investigate this question, we construct a quasiparticle vertex from the diverging irreducible vertex functions. This vertex describes the scattering between quasiparticles and quasiholes in a Fermi liquid. We show that the quasparticle vertex does not diverge in the charge channel, wherein the irreducible vertex does diverge; and we show that the quasiparticle vertex does diverge in the spin channel, wherein the irreducible vertex does not diverge. This divergence occurs at the Mott transition, wherein the Fermi-liquid theory breaks down. Both the half filled Hubbard and Anderson lattices are investigated. In general, our results support that the divergences of the irreducible vertex function do not indicate a nonphysical failure of the perturbation theory. Instead, the divergences are the mathematical consequence of inverting a matrix (the local charge susceptibility) which accumulates increasingly negative diagonal elements as the Hubbard interaction suppresses charge fluctuations. Indeed, we find that the first divergences of the irreducible vertex in both Hubbard and Anderson lattices occurs near the maximum magnitude of the (negative) vertex-connected part of the charge susceptibility.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Electrochemical reactivity of atomic and molecular species under solid-state confinement

The nanoconfinement of electrochemically-active guest species in host solid state electrode materials provides opportunities to tune mass transport between the bulk electrolyte and inner surface of the electrode, enhance electron-transfer rates, and/or improve the stability and dispersion of active material. Here, this review summarizes recent experimental and theoretical electrochemical studies of three types of nanoconfined guest species: (1) ion adsorption of electrolyte ions, (2) confined redox-active molecules, and (3) electrocatalytic reactions of confined ions/solvents and catalytic particles. The examples discussed in this review illustrate how the confinement of guest species within enclosed spaces with nanoscale dimensions – such as pores, pockets, channels, and interlayers – can lead to improved electrochemical performance.

25 ENERGY STORAGE↗
DOE OSTI2026

Ion transport through reconfigurable nanoparticle-surfactant stabilized droplet interface bilayers

Despite their adaptability and mechanical stability, Pickering emulsions based on the interfacial assembly of colloidal particles have not found use in iontronics, since the dense interfacial packing of micron-sized particles precludes functional connectivity between two droplets. In this work, we introduce a chemically reconfigurable droplet interface bilayer (DIB) platform based on the interfacial assembly of nanoparticle-surfactants (NPSs) that enables spontaneous or field-induced formation of ion-conducting nanochannels, eliminating the need of ionophores or nanochannel-forming proteins. These nanoscopic channels emerge from packing defects in the jammed interfacial assemblies of the charged NPSs and support size and charge selective, hysteretic ion transport governed by interfacial electrostatics and dimensional constraints. The NPS-DIBs show short-term and long-term plasticity, hallmarks of neuromorphic behavior, that are mediated by the structural and chemical design of the bilayer. These assemblies establish a versatile, chemically tunable platform that couples soft-matter mechanics with interfacial ionic functionality, offering a robust foundation for soft iontronic systems.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Recovery of coincident frequency domain multiplexed detector pulses using sequential deconvolution

Multiplexing of radiation detector signals into a single channel significantly reduces the need for a large number of digitizer channels, which reduces the cost and the power consumption of a data acquisition system. We previously demonstrated frequency domain multiplexing by convolution using a prototype system that multiplexed two EJ-309 organic scintillators signals into a single channel. Each detector pulse was converted to a damped sinusoid which was then combined into a single channel. The combined signal was digitized and the original detector signal was recovered from the damped sinusoid by deconvolution. In this paper, we demonstrate the recovery of multiple detector signals that arrive during the same digitized record via a new sequential deconvolution method. Here, when two detectors produce signals in the same digitized record and their pulses do not overlap in time, we found that the charge, arrival time, and particle type can be estimated fairly precisely for the first pulse, but the second pulse exhibits substantial degradation in the precision of the estimated charge and arrival time. When the pulses overlap in time, we demonstrate both theoretically and experimentally that the part of the first pulse that does not overlap with the second can be recovered accurately, so the arrival time and amplitude of the first pulse can be estimated fairly precisely, but not the charge or particle type. None of these quantities can be estimated precisely for the second pulse when the two pulses overlap.

47 OTHER INSTRUMENTATION↗
DOE OSTI2026

A 24-channel ultra-low-noise preamplifier for dN/dx measurements with drift tube detectors

Cluster counting $(dN/dx)$ is a promising method to enhance particle identification for gaseous detectors, especially in next-generation collider experiments like the FCC-ee, where good $π/K$ separation over a broad momentum range is essential. However, its implementation in large-scale systems has been limited by the challenging requirements for high-resolution signal amplification and readout. This paper presents a 24-channel ultra-low-noise preamplifier board designed for drift tube detectors to enable $dN/dx$ measurements. The three-stage amplification topology employs SiGe transistors and integrates dedicated noise-minimization techniques, achieving a charge gain of 21.11 mV/fC from 0.3 fC to 50 fC, a bandwidth of 542 MHz, and a voltage gain of 47.8 dB. The measured voltage noise density is 0.35 nV/$\sqrt{\textrm{Hz}}$ , surpassing most of the state-of-the-art preamplifiers for gaseous and silicon detectors. Validation tests conducted on the sMDT chambers at the CERN Proton Synchrotron test beam facility demonstrate that the proposed design meets the stringent preamplifier requirements for implementing the $dN/dx$ method in drift-tube detector systems, achieving an equivalent noise charge of 0.14 fC and a signal-to-noise ratio of 73 when operated with a He:iC 4 H 10 (90:10) gas mixture. The design also shows promise for broader application in other gaseous or semiconductor detectors.

Drift tube detector↗
DOE OSTI2025

Search for emerging jets in pp collisions at $\sqrt{s} = 13.6$ TeV with the ATLAS experiment

A search for emerging jets is presented using 51.8 fb −1 of proton–proton collision data at $\sqrt{s} = 13.6$ TeV, collected by the ATLAS experiment during 2022 and 2023. The search explores a hypothetical dark sector featuring ‘dark quarks’ that are charged under a confining gauge group and couple to the standard model (SM) via a new mediator particle. These dark quarks undergo showering and hadronisation within the dark sector, forming long-lived dark mesons that decay back into SM particles. This results in jets that contain multiple displaced vertices known as emerging jets. The analysis targets events with pairs of emerging jets, produced either through a vector mediator, Z′, in the s-channel, or a scalar mediator, Φ, in the t-channel. No significant excess over the SM background is observed. Assuming a dark pion proper decay length between 5 mm and 50 mm, Z′ mediator masses between 600 GeV and 2550 GeV are excluded for quark and dark quark coupling values of 0.01 and 0.1, respectively. For a quark dark-quark coupling of 0.1, Φ mediator masses between 600 GeV and 1375 GeV are excluded. These results represent the first direct search targeting emerging jet pair production via a Z′ mediator, as well as the first study of emerging jet production mediated by a scalar particle exchanged in the t-channel.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

First Observation of the β3αp Decay of 13 O via β-Delayed Charged-Particle Spectroscopy

The β-delayed proton decay of 13 O has previously been studied, but the direct observation of β-delayed 3⁢α⁢p decay has not been reported. Rare 3⁢α⁢p events from the decay of excited states in 13 N* provide a sensitive probe of cluster configurations in 13 N*. To measure the low-energy products following β-delayed 3⁢αp decay, the Texas Active Target (TexAT) time projection chamber was employed using the one-at-a-time β-delayed charged-particle spectroscopy technique at the Cyclotron Institute, Texas A&M University. A total of 1.9 × 10 5 13 O implantations were made inside the TexAT time projection chamber. Furthermore, a total of 149 3⁢αp events were observed, yielding a β-delayed 3⁢αp branching ratio of 0.078(6)%. Four previously unknown α-decaying excited states were observed in 13 N at 11.3, 12.4, 13.1, and 13.7 MeV decaying via the 3⁢α + p channel.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

A mechanism of defect-enhanced phase transformation kinetics in lithium iron phosphate olivine

Abstract Antisite defects are a type of point defect ubiquitously present in intercalation compounds for energy storage applications. While they are often considered a deleterious feature, here we elucidate a mechanism of antisite defects enhancing lithium intercalation kinetics in LiFePO 4 by accelerating the FePO 4 → LiFePO 4 phase transformation. Although Fe Li antisites block Li movement along the [010] migration channels in LiFePO 4 , phase-field modeling reveals that their ability to enhance Li diffusion in other directions significantly increases the active surface area for Li intercalation in the surface-reaction-limited kinetic regime, which results in order-of-magnitude improvement in the phase transformation rate compared to defect-free particles. Antisite defects also promote a more uniform reaction flux on (010) surface and prevent the formation of current hotspots under galvanostatic (dis)charging conditions. We analyze the scaling relation between the phase boundary speed, Li diffusivity and particle dimensions and derive the criteria for the co-optimization of defect content and particle geometry. A surprising prediction is that (100)-oriented LiFePO 4 plates could potentially deliver better performance than (010)-oriented plates when the Li intercalation process is surface-reaction-limited. Our work suggests tailoring antisite defects as a general strategy to improve the rate performance of phase-changing battery compounds with strong diffusion anisotropy.

36 MATERIALS SCIENCE↗
DOE OSTI2025

The imaging Time-of-Propagation detector at Belle II

Here, we report on the construction, operation, and performance of the Time-of-Propagation detector with imaging used for the Belle II experiment running at the Super-KEKB e + e - collider. This detector is located in the central barrel region and uses Cherenkov light to provide particle identification among hadrons. The Cherenkov light is radiated in highly polished bars of synthetic fused silica (quartz) and transported to the ends of the bars via total internal reflection. One bar end is instrumented with finely segmented micro-channel-plate photomultiplier tubes to record the light, while the other end has a mirror attached to reflect the photons back to the instrumented end. Both the propagation times and hit positions of the Cherenkov photons are measured; these depend on the Cherenkov angle and together provide good discrimination among charged pions, kaons, and protons with momenta up to around 4 GeV/ c . To date, the detector has been used to record and analyze almost 600 fb −1 of Belle II data.

43 PARTICLE ACCELERATORS↗
DOE OSTI2025

HRPPD photosensors for RICH detectors with a high resolution timing capability

Recently, a new version of DC-coupled High Rate Picosecond Photodetectors (DC-HRPPDs) substantially re-designed for use at the Electron-Ion Collider (EIC) has been developed. A first batch of seven “EIC HRPPDs” was manufactured in early 2024. These HRPPDs are DC-coupled photosensors based on Micro-Channel Plates (MCPs) that have an active area of 104 mm by 104 mm, 32 × 32 direct readout pixel array at a pitch of 3.25 mm, peak quantum efficiency in excess of 30%, exceptionally low dark count rates and timing resolution of 15–20 ps for a single photon detection. As such, these photosensors are very well suited for Ring Imaging CHerenkov (RICH) detectors that can additionally provide high resolution timing capability, especially in a configuration where a detected charged particle passes through the sensor window, which produces a localized flash containing a few dozens of Cherenkov photons in it.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Edge mode percolation and equilibration in the topological insulator cadmium arsenide

Two-dimensional topological insulators can feature one-dimensional charge transport via edge modes, which offer a rich ground for studying exotic quasi-particles and for quantum materials applications. In this work, we use lateral junction devices, defined by nanoscale finger gates, to study edge mode transport in the two-dimensional topological insulator Cd 3 As 2 . The finger gate can be tuned to transmit an integer number of quantum Hall edge modes and exhibits full equilibration in the bipolar regime. When the Fermi level of the channel crosses a Landau level, reflected modes percolate through the channel, resulting in an anomalous conductance peak. The device does not fully pinch off when the channel is tuned into the topological gap, which is a sign of remnant modes in the channel. These modes are expected from band inversion, while residual bulk conduction associated with the disorder potential may also play a role.

36 MATERIALS SCIENCE↗
DOE OSTI2026

Pandora-based muon neutrino disappearance search in the SBN program with 1muonNp quasi-elastic like channel

The Short-Baseline Neutrino (SBN) program at Fermilab aims to perform a definitive search for light sterile neutrinos using multiple liquid argon time projection chamber detectors. We present the status of an analysis of muon neutrino charged-current interactions in two SBN detectors (SBND and ICARUS), selecting fully contained events with one muon and at least one proton in the final state, inspired by the recent ICARUS standalone results. This topology-driven selection reduces dependence on neutrino interaction cross-section modeling while preserving high statistics and good neutrino energy resolution, enabled by robust reconstruction and particle identification. Fully contained events enable precise kinematic reconstruction and support relative measurements between detectors, directly addressing the core goals of the SBN program. A detailed evaluation of systematic uncertainties is currently underway, with the objective of reducing the dominant systematics to the percent level. The current status of this analysis, with a particular focus on the event selection performance, will be presented in this poster.

Artero Pons, Maria [Padua U.; INFN, Padua]↗
DOE OSTI2025

Characterization of the optical model of the T2K 3D segmented plastic scintillator detector unit cube

The magnetized near detector (ND280) of the T2K long-baseline neutrino oscillation experiment has been recently upgraded aiming to satisfy the requirement of reducing the systematic uncertainty from measuring the neutrino–nucleus interaction cross section, which is the largest systematic uncertainty in the search for leptonic charge-parity symmetry violation. A key component of the upgrade is SuperFGD, a 3D segmented plastic scintillator detector made of approximately 2,000,000 optically-isolated 1 cm 3 cubes. The SuperFGD cube unit shows promising optical performance, including a high light yield of about 40 photoelectrons (p.e.) per channel, a low cube-to-cube crosstalk rate below 3%, and a sub-nanosecond time resolution of 0.96 ns. By combining tracking and stopping power measurements of final state particles, this novel detector enables precise 3D-imaging of GeV neutrino interactions with reduced systematic uncertainties. A detailed Geant4 based optical simulation of the SuperFGD building block, i.e. a plastic scintillating cube read out by three wavelength shifting fibers, has been developed and validated with the different datasets collected in various beam tests. In this manuscript the description of the optical model as well as the comparison with data are reported.

Neutrino oscillations↗
DOE OSTI2019

Near-threshold incoherent pion photoproduction on the deuteron with final-state interaction effects

Highlights: • Incoherent pion photoproduction on the deuteron near threshold is investigated including rescattering effects. • For the first time, polarization observables are predicted near threshold. • The influence of NN-FSI effect is moderate in the π{sup 0}-production. • πN-rescattering has a noticeable contribution only in the π{sup 0}-production. • The unpolarized cross sections have a satisfactory agreement with experiment and other theories. - Abstract: Incoherent pion photoproduction on the deuteron γd→πNN is investigated in the energy region E{sub γ}{sup thr}≤E{sub γ}≤ 160 MeV. The model applied contains the amplitudes of the impulse approximation as well as the NN and πN rescattering in the final state. For the elementary γN→πN amplitude, the unitary isobar MAID-2007 model is used. This model is parameterized in terms of invariant amplitudes and allows one to give a more reliable description of the threshold region. The half-off-shell NN and πN scattering amplitudes are obtained from separable representations of realistic NN and πN interactions, respectively. For the first time, numerical results for the linear photon asymmetry Σ, vector T{sub 11} and tensor T{sub 2M} (M=0,1,2) deuteron spin asymmetries for the reactions γd→π{sup −}pp, γd→π{sup +}nn, and γd→π{sup 0}np are presented. In addition, results for the unpolarized differential and total cross sections are given. We found that the influence of NN rescattering is moderate in both charged-and neutral-pion production channels, whereas πN rescattering is almost negligible in the charged-pion production channels which is not the case in neutral-pion production since a noticeable contribution is obtained. The calculated results for unpolarized differential and total cross sections are compared with the available experimental data and other theoretical models, and a satisfactory agreement is obtained.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Charged Current Single Pion Production on SBND

The Short Baseline Neutrino (SBN) program at Fermilab is designed to provide precise measurements of neutrino oscillations using 3 Liquid Argon Time Projection Chambers (LArTPC) built along Fermilab's Booster Neutrino Beam (BNB). The Short Baseline Near Detector (SBND), located at only 110 m from the BNB target, will precisely characterize the neutrino flux before oscillations take place, thanks to its unprecedented neutrino interaction statistics. Due to its proximity to the neutrino production target, the detector expects over a million neutrino interactions annually, which will open the possibility of exploring exclusive channels of neutrino interactions. This poster will show SBND’s capabilities of exploring Muon Neutrino Charged Current Single Pion production, for which previous measurements in Argon were limited by statistics. The poster will introduce the relevance of this process for neutrino Physics, the unique possibilities of SBND and a preliminary event selection using SBND's current reconstruction tools.

43 PARTICLE ACCELERATORS↗
DOE OSTI2025

Unexpected Breakdown of Collinear Factorisation at Leading Twist in Exclusive π 0 γ Photoproduction Due to Glauber Pinch

We demonstrate the breakdown of collinear factorisation for the exclusive photoproduction at leading twist of a pair, sensitive to both quark and gluon GPD channels. For the very first time in the case of an exclusive process, we demonstrate the breakdown of collinear factorisation through soft-to-collinear Glauber exchanges. We show that the amplitude fails to factorise due to the presence of a Glauber pinch, which has the same power counting as the standard collinear pinch. The Glauber pinch that occurs here is peculiar, since the mechanism that produces it involves two-loop integrals. This is corroborated by an explicit calculation of the gluon GPD channel to pair photoproduction, which leads to a divergent amplitude already at leading twist-2 and at leading order in . On the other hand, for processes where the gluon GPD channel is forbidden, for example when the outgoing meson is a charged pion or a rho meson, collinear factorisation works without any issues.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗