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Exploring the Production of NOx by Lightning and Its Impact on Tropospheric Ozone
Our quantitative understanding of free tropospheric (FT) chemistry is quite poor. State-of-the-art regional air quality models (e.g., US EPA's CMAQ) perform very poorly in simulating FT chemistry, with Uniform ozone around 70 ppb throughout the FT in summer, while ozonesonde data show much higher levels of ozone and much spatial-temporal structure. Such models completely neglect lightning-NOx (LNOx) emissions (the most significant source of NOx in the FT), and also contain large uncertainties in the specifications of intercontinental transport, stratosphere-troposphere exchange (STE) and PBLFT exchange (PFTE). Global air chemistry models include LNOx, but in very crude fashion, with the frequency and distribution of lightning being based on modeled cloud parameters (hence large uncertainty), lightning energetics being assumed to be constant for all flashes (literature value, while in reality there is at least a two-orders of magnitude variability from flash-to-flash), and the production of NOx in the surrounding heated air, per Joule of heating, being assumed to be constant also (literature value, while in fact it is a non-linear function of the dissipated heat and local air density, p). This situation is commonly blamed on paucity of pertinent observational data, but for the USA, there is now a wealth of surface- and satellite-based data of lightning available to permit much improved observation-based estimation of LNOx emissions. In the FT, such NOx has a long residence time, and also the ozone production efficiency from NOx there is considerably higher than in the PBL. It is, therefore, of critical importance in FT chemistry. This paper will describe the approach and data products of an ongoing NSSTC project aimed at a much-improved quantification of not only LNOx production on the scale of continental USA based on local and regional lightning observations, but also of intercontinental transport, STE and PFTE, all in upgraded simulations of tropospheric transport and chemistry. In our approach for LNOx, (a) we utilize continuous observed lightning information from the NLDN ground network and from satellite imagers (OTD and LIS) to quantify lightning frequency and distribution at the spatial-temporal scales of models such as CMAQ; (b) we develop new methodologies to quantify flash-specific lightning energy dissipation as heat (epsilon) using data from the research-grade lightning measurement facility at NASA-KSC, and to parameterize epsilon based on regional lightning monitoring data (ground- and satellite-based); and, (c) we develop a new parameterization of NOx production as a function of epsilon and rho. Based on such observation-based information, we are working to develop a gridded, episodic LNOx emissions inventory for the USA for use in models like CMAQ. We are also developing approaches for global(MOZART)- regional(CMAQ) chemistry coupling to improve intercontinental transport and STE. Finally, we are developing new methodologies for assimilation of satellite-observed (GOES) clouds into meteorological modeling (MM5), to improve PFTE and to optimize co-location of cloud convection and observed lightning. We will incorporate these improvements in CMAQ simulations over the USA to better understand FT processes and chemistry, and its impact on ground-level ozone.
Long-Term Trends in Aerosols, Low Clouds, and Large-Scale Meteorology Over the Western North Atlantic From 2003 to 2020
Here, a continuous decrease in aerosols over the Western North Atlantic Ocean (WNAO) on a decadal timescale provides a long-term benchmark to evaluate how various natural and anthropogenic processes affect the manifestation of aerosol-cloud interactions in this region. Furthermore, the WNAO serves as a natural laboratory with diverse aerosol sources, marine boundary layer clouds more variable than those in marine stratocumulus deck regions, and unique flow regimes established by the Gulf Stream and the semi-permanent Bermuda High. We investigate how satellite-retrieved macrophysical and microphysical properties of low clouds and the surface shortwave irradiance changed from 2003 to 2020, in tandem with this aerosol decrease. The decadal changes in large-scale meteorology related to the North Atlantic Oscillation (NAO) are also examined. We find a reduction in low-cloud optical thickness, accompanied by fewer and larger cloud droplets, yet observe no significant changes in low-cloud fraction and liquid water path. Despite the reduction in low-cloud optical thickness together with aerosol decrease, a corresponding increase in the trends of surface shortwave irradiance, also known as surface brightening, is lacking. This absence of brightening is potentially related to concomitant changes found in large-scale meteorology associated with NAO—Bermuda High strengthening, sea surface warming, and atmospheric moistening— as well as an increase in high-level cloud fraction that can counteract the surface brightening. Ultimately, our findings suggest that spatial patterns of decadal meteorological variability introduce complexities in the surface cloud radiative effect over the WNAO, thereby complicating the isolation and examination of aerosol-cloud interactions.
Investigation of Meteorological Conditions Associated with Aircraft Icing in Layer-Type Clouds for 1947-48 Winter
Rotating-cylinder measurements of the icing conditions encountered in flight during the winter of 1947-48 are presented. Liquid water content, drop size, and temperature data are shown to be consistent with previously measured conditions and with proposed maximum icing conditions in supercooled layer-type clouds. Cumulative frequency graphs of meteorological parameters indicate the frequency with which various icing conditions have been encountered in the Great Lakes area and surrounding states.
Long-Term Trends in Aerosols, Low Clouds, and Large-scale Meteorology over the Western North Atlantic from 2003 to 2020
A continuous decrease of aerosol over the western North Atlantic Ocean (WNAO) on decadal timescales provides a long-term experiment to evaluate how other natural and anthropogenic processes affect the manifestation of aerosol-cloud interactions in this region. Furthermore, the WNAO is a natural laboratory with diverse aerosol sources, marine boundary layer clouds that are more variable than marine stratocumulus deck regions, and unique flow regimes set up by the Gulf Stream and semi-permanent Bermuda High. We investigate how satellite-retrieved macrophysical and microphysical properties of low clouds and the surface shortwave irradiance changed from 2003 to 2020, in tandem with this aerosol decrease. The decadal changes in large-scale meteorology relating to the North Atlantic Oscillation (NAO) are also examined. We find no significant changes in low-cloud fraction but a widespread reduction in low-cloud optical depth attributed to fewer and larger cloud droplets with almost no change in cloud liquid water path. Despite robust signals in low-cloud optical properties together with aerosol decrease, a corresponding increase in the surface shortwave irradiance trends, also called surface brightening, is lacking. This absence of brightening is potentially due to concomitant changes found in large-scale meteorology associated with NAO— a Bermuda High strengthening, sea surface warming, and atmospheric moistening— as well as an increase in high cloud fraction that can counteract the surface brightening. Ultimately, our findings suggest that spatial patterns in the decadal meteorological variability, likely set up by NAO, contribute more to the surface cloud radiative effect over the WNAO than aerosol-cloud interactions.
A study of a non-deepening tropical disturbance.
Nondeepening synoptic scale tropical disturbance showing dependence on in situ development and decay in upper troposphere
Low-Level Cloud Variability over the Equatorial Cold Tongue in Observations and Models
A fourth paper now in press is, Low-level cloud variability over the equatorial cold tongue in observations and models, by D. K. Mansbach and J. R. Norris (2007, J. Climate). This study examined cloud and meteorological observations from satellite, surface, and reanalysis datasets and fount that monthly anomalies in low-level cloud amount and near-surface temperature advection are strongly negatively correlated on the southern side of the equatorial Pacific cold tongue. This inverse correlation occurs independently of relationships between cloud amount and sea surface temperature (SST) or lower tropospheric static stability (LTS) and the combination of advection plus SST or LTS explains significantly more interannual cloud variability in a multilinear regression than does SST or LTS alone. Warm anomalous advection occurs when the equatorial cold tongue is well defined and the southeastern Pacific trade winds bring relatively warm air over colder water. Ship meteorological reports and soundings show that the atmospheric surface layer becomes stratified under these conditions, thus inhibiting the upward mixing of moisture needed to sustain cloudiness against subsidence and entrainment drying. Cold anomalous advection primarily occurs when the equatorial cold tongue is weak or absent and the air-sea temperature difference is substantially negative. These conditions favor a more convective atmospheric boundary layer, greater cloud amount, and less frequent occurrence of clear sky. Examination of output from global climate models developed by the Geophysical Fluid Dynamics Laboratory (GFDL) and the National Center for Atmospheric Research (NCAR) indicates that both models generally fail to simulate the cloud-advection relationships observed on the northern and southern sides of the equatorial cold tongue. Although the GFDL atmosphere model does reproduce the expected signs of cloud-advection correlations when forced with prescribed historical SST variations, it does not consistently do so when coupled to an ocean model. The NCAR model has difficulty reproducing the observed correlations in both atmosphere-only and coupled versions. This suggests that boundary layer cloud parameterizations could be improved through better representation of the effects of advection over varying SST.
A Study of Meteorological Conditions Associated With Noctilucent Clouds
Temperature measurements were obtained in the upper stratosphere and mesosphere between 50 and 95 km with passive inflatable falling spheres launched on small meteorological rockets as part of the DROPPS (Distribution and Role of Particles in the Polar Summer Mesosphere) program. Temperatures of the neutral atmosphere have been combined with similar measurements obtained during 1991 and 1993. Temperatures were found to change monatonically with altitude except during the Nocticulent Clouds (NLC) occurrences during DROPPS. The temperature lapse rate changed between 5 July 1999, 2313 UTC and 6 July 1999, 0209 UTC; this included a lowering of the altitude of minimum temperature by about 5 km. Furthermore, winds backed from a northeasterly direction to a northwesterly direction. Whether the change in temperature observed is a result of advection related to the changes of the wind field due to advection. Comparisons will also concentrate on the meteorological conditions during the NLC event during DROPPS and earlier 1991 and 1993 NLC'S.
A calculation of percentage area covered by convective clouds from moisture convergence
Calculation of percentage area covered by convective clouds from moisture convergence
Retrieval of nonprecipitating liquid water cloud parameters from microwave data - A simulation study
A new microwave algorithm, analogous to the IR 'radiance-ratioing' method of Eyre and Menzel (1989) is developed to retrieve the height and 'effective' fraction (defined as the product of the emissivity times the actual physical fractional coverage) of nonprecipitating water clouds using various pairs of the 20 microwave channels planned for the Advanced Microwave Sounding Unit (AMSU), an instrument slated to fly on polar-orbiting satellites beginning in 1994. The results of a simulation study are presented to provide some insights into the potentials of this technique using different AMSU channel combinations. This study suggests that the use of the oxygen channels 3 and 5 and water vapor channels 19 and 20 will produce the most accurate retrievals of liquid water cloud parameters and the highest percentage of good-quality retrievals over a range of meteorological and cloud conditions.
A Surface Radiation Balance Data Set from Siple Dome in West Antarctica for Atmospheric and Climate Model Evaluation
A field campaign at Siple Dome in West Antarctica during the austral summer 2019-2020 offers an opportunity to evaluate climate model performance, particularly cloud microphysical simulation. Over Antarctic ice sheets and ice shelves, clouds are a major regulator of the surface energy balance, and in the warm season their presence occasionally induces surface melt that can gradually weaken an ice shelf structure. This dataset from Siple Dome, obtained using transportable and solar-poweredequipment, includes surface energy balance measurements, meteorology and cloud remote sensing. To demonstrate how these data can be used to evaluate model performance, comparisons are made with meteorological reanalysis known to give generally good performance over Antarctica (ERA5). Surface albedo measurements show expected variability with observed cloud amount, and can be used to evaluate a model's snowpack parameterization. One case study discussed involves a squall with northerly winds, during which ERA5 fails to produce cloud cover throughout one of the days. A second case study illustrates how shortwave spectroradiometer measurements that encompass the 1.6-micron atmospheric window reveal cloud phase transitions associated with cloud lifecycle. Here, continuously precipitating mixed-phase clouds become mainly liquid water clouds from local morning through the afternoon, not reproduced by ERA5. We challenge researchers to run their various regional or global models in a manner that has the large-scale meteorology follow the conditions of this field campaign, compare cloud and radiation simulations with this Siple Dome dataset, and potentially investigate why cloud microphysical simulations or other model components might produce discrepancies with these observations.
A Surface Radiation Balance Dataset from Siple Dome in West Antarctica for Atmospheric and Climate Model Evaluation
Abstract A field campaign at Siple Dome in West Antarctica during the austral summer 2019/20 offers an opportunity to evaluate climate model performance, particularly cloud microphysical simulation. Over Antarctic ice sheets and ice shelves, clouds are a major regulator of the surface energy balance, and in the warm season their presence occasionally induces surface melt that can gradually weaken an ice shelf structure. This dataset from Siple Dome, obtained using transportable and solar-powered equipment, includes surface energy balance measurements, meteorology, and cloud remote sensing. To demonstrate how these data can be used to evaluate model performance, comparisons are made with meteorological reanalysis known to give generally good performance over Antarctica (ERA5). Surface albedo measurements show expected variability with observed cloud amount, and can be used to evaluate a model’s snowpack parameterization. One case study discussed involves a squall with northerly winds, during which ERA5 fails to produce cloud cover throughout one of the days. A second case study illustrates how shortwave spectroradiometer measurements that encompass the 1.6- μ m atmospheric window reveal cloud phase transitions associated with cloud life cycle. Here, continuously precipitating mixed-phase clouds become mainly liquid water clouds from local morning through the afternoon, not reproduced by ERA5. We challenge researchers to run their various regional or global models in a manner that has the large-scale meteorology follow the conditions of this field campaign, compare cloud and radiation simulations with this Siple Dome dataset, and potentially investigate why cloud microphysical simulations or other model components might produce discrepancies with these observations. significance statement Antarctica is a critical region for understanding climate change and sea level rise, as the great ice sheets and the ice shelves are subject to increasing risk as global climate warms. Climate models have difficulties over Antarctica, particularly with simulation of cloud properties that regulate snow surface melting or refreezing. Atmospheric and climate-related field work has significant challenges in the Antarctic, due to the small number of research stations that can support state-of-the-art equipment. Here we present new data from a suite of transportable and solar-powered instruments that can be deployed to remote Antarctic sites, including regions where ice shelves are most at risk, and we demonstrate how key components of climate model simulations can be evaluated against these data.
The Potential Impact of Satellite-Retrieved Cloud Parameters on Ground-Level PM2.5 Mass and Composition
Satellite-retrieved aerosol optical properties have been extensively used to estimate ground-level fine particulate matter (PM2.5) concentrations in support of air pollution health effects research and air quality assessment at the urban to global scales. However, a large proportion, approximately 70%, of satellite observations of aerosols are missing as a result of cloud-cover, surface brightness, and snow-cover. The resulting PM2.5 estimates could therefore be biased due to this non-random data missingness. Cloud-cover in particular has the potential to impact ground-level PM2.5 concentrations through complex chemical and physical processes. We developed a series of statistical models using the Multi-Angle Implementation of Atmospheric Correction (MAIAC) aerosol product at 1 km resolution with information from the MODIS cloud product and meteorological information to investigate the extent to which cloud parameters and associated meteorological conditions impact ground-level aerosols at two urban sites in the US: Atlanta and San Francisco. We find that changes in temperature, wind speed, relative humidity, planetary boundary layer height, convective available potential energy, precipitation, cloud effective radius, cloud optical depth, and cloud emissivity are associated with changes in PM2.5 concentration and composition, and the changes differ by overpass time and cloud phase as well as between the San Francisco and Atlanta sites. A case-study at the San Francisco site confirmed that accounting for cloud-cover and associated meteorological conditions could substantially alter the spatial distribution of monthly ground-level PM2.5 concentrations.
Analysis and Preliminary Design of an Optical Instrument for the Measurement of Drop Size and Free-water Content of Clouds
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Icing zones in a warm front system with general precipitation
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Near-Surface Meteorology During the Arctic Summer Cloud Ocean Study (ASCOS): Evaluation of Reanalyses and Global Climate Models.
Atmospheric measurements from the Arctic Summer Cloud Ocean Study (ASCOS) are used to evaluate the performance of three atmospheric reanalyses (European Centre for Medium Range Weather Forecasting (ECMWF)- Interim reanalysis, National Center for Environmental Prediction (NCEP)-National Center for Atmospheric Research (NCAR) reanalysis, and NCEP-DOE (Department of Energy) reanalysis) and two global climate models (CAM5 (Community Atmosphere Model 5) and NASA GISS (Goddard Institute for Space Studies) ModelE2) in simulation of the high Arctic environment. Quantities analyzed include near surface meteorological variables such as temperature, pressure, humidity and winds, surface-based estimates of cloud and precipitation properties, the surface energy budget, and lower atmospheric temperature structure. In general, the models perform well in simulating large-scale dynamical quantities such as pressure and winds. Near-surface temperature and lower atmospheric stability, along with surface energy budget terms, are not as well represented due largely to errors in simulation of cloud occurrence, phase and altitude. Additionally, a development version of CAM5, which features improved handling of cloud macro physics, has demonstrated to improve simulation of cloud properties and liquid water amount. The ASCOS period additionally provides an excellent example of the benefits gained by evaluating individual budget terms, rather than simply evaluating the net end product, with large compensating errors between individual surface energy budget terms that result in the best net energy budget.
Stereoscopic observations from meteorological satellites
Stereo cloud top height measurements, accurate to within + or - 500 m, have been performed using operational weather satellites. The stereo has been demonstrated using various combinations of GEO and LEO satellites, and the use of synthetic stereo was considered. Stereo can be done over most of the earth (60 deg S to 60 deg N) during the day; at higher latitudes and at night, stereo can be done using two LEOs if the proper coincidences occur. The usefulness of stereo cloud top height measurements has been demonstrated by many studies of convective storm cloud systems. Recommendations relating to short, medium, and long term planning regarding stereo observations from meteorological satellites are outlined.
Sunlight-absorbing aerosol amplifies the seasonal cycle in low-cloud fraction over the southeast Atlantic
Abstract. The mean altitude of the smoke loading over the southeast Atlantic moves from the boundary layer in July to the free troposphere by October. This study details the month-by-month changes in cloud properties and the large-scale environment as a function of the biomass burning aerosol loading at Ascension Island (8∘ S, 14.5∘ W) from July to October, based on island measurements, satellite retrievals, and reanalysis. In July and August, the smoke loading predominantly varies within the boundary layer. During both months, the low-cloud fraction is less and is increasingly cumuliform when more smoke is present, with the exception of a late morning boundary layer deepening that encourages a short-lived cloud development. The meteorology varies little, suggesting aerosol–cloud interactions explain the cloudiness changes. September marks a transition month during which midlatitude disturbances can intrude into the Atlantic subtropics, constraining the free tropospheric aerosol closer to the African coast. Stronger boundary layer winds on cleaner days help deepen, dry, and cool much of the marine boundary layer compared to that on days with high smoke loadings, with stratocumulus reducing everywhere but at the northern deck edge. The September free troposphere is better mixed on smoky days compared to October. Longwave cooling rates, generated by a sharp water vapor gradient at the aerosol layer top, encourage a small-scale vertical mixing that could help maintain the well-mixed smoky September free troposphere. The October meteorology primarily varies as a function of the strength of the free tropospheric winds advecting aerosol offshore. The free tropospheric aerosol loading is less than in September, and the moisture variability is greater. Low-level clouds increase and are more stratiform in October when the smoke loadings are higher. The increased free tropospheric moisture can help sustain the clouds through a reduction in evaporative drying during cloud-top entrainment. Enhanced subsidence above the coastal upwelling region, increasing cloud droplet number concentrations, may further prolong cloud lifetime through microphysical interactions. Reduced subsidence underneath stronger free tropospheric winds at Ascension Island supports slightly higher cloud tops during smokier conditions. Overall, the monthly changes in the large-scale aerosol and moisture vertical structure act to amplify the seasonal cycle in low-cloud amount and morphology. This is climatically important, as cloudiness changes dominate changes in the top-of-atmosphere radiation budget.