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DIAL with heterodyne detection including speckle noise: Aircraft/shuttle measurements of O3, H2O, and NH3 with pulsed tunable CO2 lasers

Atmospheric trace constituent measurements with higher vertical resolution than attainable with passive radiometers are discussed. Infrared differential absorption lidar (DIAL), which depends on Mie scattering from aerosols, has special advantages for tropospheric and lower stratospheric applications and has great potential importance for measurements from shuttle and aircraft. Differential absorption lidar data reduction involves comparing large amplitude signals which have small differences. The accuracy of the trace constituent concentration inferred from DIAL measurements depends strongly on the errors in determining the amplitude of the signals. Thus, the commonly used SNR expression (signal divided by noise in the absence of signal) is not adequate to describe DIAL measurement accuracy and must be replaced by an expression which includes the random coherent (speckle) noise within the signal. A comprehensive DIAL computer algorithm is modified to include heterodyne detection and speckle noise. Examples for monitoring vertical distributions of O3, H2O, and NH3 using a ground-, aircraft-, or shuttle-based pulsed tunable CO2 laser DIAL system are given.

Brockman, P.↗

Toward an improved global network for determination of tropospheric ozone climatology and trends

Current data on ozone variability on daily, monthly, annual, and interannual time scales were used for a standard trend-prediction analysis. Using the results of this analysis, together with a quantitative theory that defines the 'effectively sampled region' for an observing station, a definition was developed for a global network capable of determining ozone climatology and ozone trends with uncertainties not above 1 percent per year at the 95 percent confidence level. The definition indicates a need for at least a doubling of the present number of stations; the areas where more stations are most needed include the oceans, most of Asia, Africa, and South America. It is pointed out that differential absorption lidar ozone instruments have the potential for far more frequent measurements of ozone vertical profiles and, hence, potentially more accurate climatology and trend determinations than the ozonesondes; however, the differential-absorption lidar ozone measurements may produce a biased data set above the cloud base.

Prinn, Ronald G.↗

Advances in High Energy Solid-State Pulsed 2-Micron Lidar Development for Ground and Airborne Wind, Water Vapor and CO2 Measurements

NASA Langley Research Center has a long history of developing 2-micron lasers. From fundamental spectroscopy research, theoretical prediction of new materials, laser demonstration and engineering of lidar systems, it has been a very successful program spanning around two decades. Successful development of 2-micron lasers has led to development of a state-of-the-art compact lidar transceiver for a pulsed coherent Doppler lidar system for wind measurement with an unprecedented laser pulse energy of 250 millijoules in a rugged package. This high pulse energy is produced by a Ho:Tm:LuLiF laser with an optical amplifier. While the lidar is meant for use as an airborne instrument, ground-based tests were carried out to characterize performance of the lidar. Atmospheric measurements will be presented, showing the lidar's capability for wind measurement in the atmospheric boundary layer and free troposphere. Lidar wind measurements are compared to a balloon sonde, showing good agreement between the two sensors. Similar architecture has been used to develop a high energy, Ho:Tm:YLF double-pulsed 2-micron Integrated Differential Absorption Lidar (IPDA) instrument based on direct detection technique that provides atmospheric column CO2 measurements. This instrument has been successfully used to measure atmospheric CO2 column density initially from a ground mobile lidar trailer, and then it was integrated on B-200 plane and 20 hours of flight measurement were made from an altitude ranging 1500 meters to 8000 meters. These measurements were compared to in-situ measurements and National Oceanic and Atmospheric Administration (NOAA) airborne flask measurement to derive the dry mixing ratio of the column CO2 by reflecting the signal by various reflecting surfaces such as land, vegetation, ocean surface, snow and sand. The lidar measurements when compared showed a very agreement with in-situ and airborne flask measurement. NASA Langley Research Center is currently developing a triple-pulsed 2-micron Integrated Differential Absorption Lidar (IPDA) instrument for simultaneous measurement of water vapor and carbon-dioxide column density measurement from an air-borne platform. This presentation will give an overview of the 2 decades of 2-micron coherent and direction detection of laser/lidar development at NASA Langley Research Center and will present the ground and airborne wind and column CO2 measurement intercomparison with in-situ, balloon and flask measurements.

Singh, Upendra N.↗

Laser remote sensing of atmospheric ammonia using a CO2 lidar system

A CO2 differential-absorption lidar system has been used for the remote sensing of ammonia in the atmosphere. For CO2 lidar returns backscattered from topographic targets at ranges up to 2.7 km, the path-averaged sensitivity of the DIAL system was 5 ppb of NH3. Concentrations of atmospheric ammonia were found to vary during the day from undetectable levels (less than 5 ppb) to as high as 20 ppb, depending on temperature and humidity conditions.

Force, A. P.↗

The JPL Table Mountain and Mauna Loa Stratospheric Ozone Lidars

The development of a differential absorption lidar (DIAL) system for long-term measurements of stratospheric ozone and for potential inclusion in the Network for the Detection of Stratospheric Change (NDSC) began at JPL in 1986, concurrent with the first workshop that considered the priorities and appropriate measurement techniques for such a network. The DIAL system at the JPL Table Mountain Facility (TMF) was developed specifically to have characteristics suitable for longterm measurements as proposed for NDSC. Regular measurements of stratospheric ozone concentration profiles commenced in February 1988 and this system has been fully described elsewhere.

Mcdermid, I. Stuart↗

Lidar Measurements of Aerosol and Ozone Distributions During the 1992 Airborne Arctic Stratospheric Expedition

The LaRC airborne lidar system was operated from the ARC DC-8 aircraft during the 1992 Airborne Arctic Stratospheric Expedition (ASEE-2) to investigate the distribution of stratospheric aerosols and O3 across the Arctic vortex from Jan. to Mar. 1992. Monthly flights were made across the Arctic vortex from Anchorage, Alaska, to Stavanger, Norway, and then back to Bangor, Maine, and additional round-trip flights north into the vortex were made each month from either Stavanger or Bangor depending on the location of the vortex that month. The airborne lidar system uses the differential absorption lidar (DIAL) technique at laser wavelengths of 301.5 and 310.8 nm to measure O3 profiles above the DC-8 over the 12-25 km altitude range. Lidar measurements of aerosol backscatter and depolarization profiles over the 12-30 km altitude range are made simultaneously with the O3 measurements using infrared (IR) and visible (VIS) laser wavelengths of 603 and 1064 nm, respectively. The measurements of Pinatubo aerosols, polar stratospheric clouds, and O3 made with the airborne DIAL system during the AASE-2 expedition and to chemical and dynamical process that contribute to O3 depletion in the wintertime Arctic stratosphere.

Browell, E. V.↗

An Overview of the NASA ADM-Aeolus Cal/Val Test Flight Campaign

Lidars are uniquely capable of collecting high precision and high spatio-temporal observations that have been used for atmospheric process studies from the ground, aircraft, and space for over 30 years. The Atmospheric Dynamics Mission Aeolus (ADM-Aeolus), the first-ever spaceborne Doppler wind lidar, was developed by the European Space Agency and launched in August 2018. The ADM-Aeolus Atmospheric Laser Doppler Instrument (ALADIN) observes profiles of the component of the wind vector and aerosol optical properties along the instrument’s line-of-sight direction on a global scale. Two airborne lidar systems have been developed at NASA Langley Research Center in recent years that collect measurements in support of several NASA Earth Science Division focus areas. The Doppler Aerosol WiNd (DAWN) lidar measures vertical profiles of horizontal wind speed and direction. The High Altitude Lidar Observatory (HALO) measure high resolution profiles of atmospheric water vapor (WV) and aerosol and cloud optical properties. Though new space-based missions with advanced capabilities such as Aeolus are continuously being conceived and developed, there are limitations in terms of spatial and vertical detail and measurement precision that can be accomplished from space, thus airborne remote sensing observations like those from DAWN and HALO are required to fill these observational gaps as well as to calibrate and validate space-based measurements. Over a two-week period in April 2019 during their Aeolus Cal/Val Test Flight campaign, NASA conducted five research flights over the Eastern Pacific Ocean with the DC-8 aircraft to 1) demonstrate the DAWN Doppler wind lidar, HALO high spectral resolution lidar aerosol/cloud measurement and differential absorption lidar WV measurement capabilities across a range of atmospheric conditions, 2) demonstrate Aeolus Cal/Val flight strategies and compare DAWN and HALO measurements with Aeolus to gain an initial perspective of Aeolus performance, and 3) demonstrate how atmospheric dynamic processes can be resolved and better understood through simultaneous observations of wind, WV, and aerosol profile observations, coupled with numerical model and other remote sensing observations. This paper provides a brief description of the DAWN and HALO instruments, discusses the synergistic observations collected across a wide range of atmospheric conditions sampled during the DC-8 flights, and a summary of the validation of DAWN, HALO, and Aeolus observations and comparisons.

Kristopher M. Bedka↗

Novel Technique and Technologies for Active Optical Remote Sensing of Greenhouse Gases

The societal benefits of understanding climate change through identification of global carbon dioxide sources and sinks led to the desired NASA's active sensing of carbon dioxide emissions over nights, days, and seasons (ASCENDS) space-based missions of global carbon dioxide measurements. For more than 15 years, NASA Langley Research Center (LaRC) have developed several carbon dioxide active remote sensors using the differential absorption lidar (DIAL) technique operating at the two-micron wavelength. Currently, an airborne two-micron triple-pulse integrated path differential absorption (IPDA) lidar is under development. This IPDA lidar measures carbon dioxide as well as water vapor, the dominant interfering molecule on carbon dioxide remote sensing. Advancement of this triple-pulse IPDA lidar development is presented.

Singh, Upendra N.↗

Tropopause fold structure determined from airborne lidar and in situ measurements

Airborne differential absorption lidar and in situ data obtained during the April 20, 1984 flight experiment conducted over Nevada and California are analyzed. The O3 and aerosols profiles and in situ measurements reveal a 2.0-km-deep layer (with high O3 concentrations and enhanced aerosol backscattering) and a correlation of 0.8 between O3 and aerosol backscatter (with both values decreasing about 25 percent along the central axis of the fold). It is observed that the cold boundary of the fold has weaker gradients, larger-scale undulations, and more irregularity than the warm boundary. The potential vorticity distribution along the flight path was derived from radiosonde data. A positive correlation between the O3 mixing ratio and the potential vorticity values in the fold is detected; the average ratio between O3 and potential vorticity is 50.2 ppbv/10 to the -5th sq cm deg per g s.

Browell, E. V.↗

Correction function in the Lidar equation and the solution techniques for CO2 Lidar date reduction

For lidar systems with long laser pulses the unusual behavior of the near-range signals causes serious difficulties and large errors in reduction. The commonly used lidar equation is no longer applicable since the convolution of the laser pulse with the atmospheric parameter distributions should be taken into account. It is important to give more insight into this problem and find the solution techniques. Starting from the original equation, a general form is suggested for the single scattering lidar equation where a correction function Cr is introduced. The correction Function Cr(R) derived from the original equation indicates the departure from the normal lidar equation. Examples of Cr(R) for a coaxial CO2 lidar system are presented. The Differential Absorption Lidar (DIAL) errors caused by the differences of Cr(R) for H2O measurements are plotted against height.

Zhao, Y.↗

Rotational Raman Lidar for Lower Tropospheric Temperature Profiling

Accurate sensing of the tropospheric temperature profile is basically needed in meteorology and 3D mapping of the boundary layer atmospheric temperature over urban and industrial areas. Several temperature lidar techniques were investigated, including Differential Absorption Lidar (DIAL), rotational and vibrational Raman, Rayleigh and high resolution Rayleigh schemes. For the tropospheric applications, the rotational Raman scheme looks potentially advantageous, but several stringent technical problems still remain to be solved. Reported here are the continuing efforts of the system development of the rotational Raman lidar.

Kobayashi, Takao↗

Development of a Compact, Ground-Based Ozone DIAL System

We are developing a portable, eye-safe, ground-based ozone lidar instrument specialized for ozone differential absorption lidar (DIAL) measurements in the troposphere. This prototype instrument is intended to operate at remote field sites and to serve as the basic unit for future monitoring projects requiring multi-instrument networks, such as that proposed for the Global Tropospheric Ozone Project (GTOP). GTOP is currently being formulated by a scientific panel of the International Global Atmospheric Chemistry Project to meet its goal to better understand the processes that control the global distribution of tropospheric ozone. In order for the lidar to be widely deployed in networks, it must be fairly easy to use and maintain as well as being cost-competitive with ground station launching ozone sondes which operate several times a day. To achieve these goals, emphasis is placed upon the incorporation of: (1) all-solid state transmitters which can reliably produce 20-40 mJ pulses; (2) a highly efficient, narrow-bandpass receiver; (3) dual analog and photon-counting detector channels; and (4) flexible, user-friendly control software.

Chyba, T. H.↗

Development of a Portable, Ground-Based Ozone Lidar Instrument for Tropospheric Ozone Research and Educational Training

The objective of this project is to develop a portable, eye-safe, ground-based ozone lidar instrument specialized for ozone differential absorption lidar (DIAL) measurements in the troposphere. This prototype instrument is intended to operate at remote field sites and to serve as the basic unit for monitoring projects requiring multi-instrument networks, such as that discussed in the science plan for the Global Tropospheric Ozone Project (GTOP). This instrument will be based at HU for student training in lidar technology as well as atmospheric ozone data analysis and interpretation. It will be also available for off-site measurement campaigns and will serve as a test bed for further instrument development. Later development beyond this grant to extend the scientific usefulness of the instrument may include incorporation of an aerosol channel and upgrading the laser to make stratospheric ozone measurements. Undergraduate and graduate students have been and will be active participants in this research effort.

Chyba, Thomas↗

Development of a Portable, Ground-based Ozone Lidar Instrument for Tropospheric Ozone Research and Educational Training

The objective of this research project is to develop a portable, eye-safe, ground-based ozone lidar instrument specialized for ozone differential absorption lidar (DIAL) measurements in the troposphere. This research project directly supports the goal of NASA's Earth Science Enterprise to understand the distribution and budget of tropospheric ozone (objective 1.5 of the Earth Science Strategic Enterprise Plan, 1998-2002). It can participate in ground validation experiments for TES, a tropospheric ozone satellite mission due to be launched in 2002. It can also be utilized for correlative ground measurements in future GTE (Global Tropospheric Experiment) and space-based ozone lidar missions, such as ORACLE. Multiple ground-based ozone lidar systems would improve the data obtained through current ozone-sonde networks. This prototype instrument could to serve as the basic unit for these and other future monitoring projects requiring multi-instrument networks, such as that proposed for the Global Tropospheric Ozone Project (GTOP). GTOP is currently being formulated by a scientific panel of the International Global Atmospheric Chemistry Project to meet its goal to better understand the processes that control the global distribution of tropospheric ozone. In order for the lidar to be widely deployed in networks, it must be fairly easy to use and maintain as well as being cost-competitive with a ground station launching ozonesondes several times a day. A second 2-year grant to continue this effort with students participating in ground tests and system improvements has been awarded by the Office of Equal Employment Opportunities (OEOP). This project also supports existing NASA lidar missions through its development of advanced, compact lidar technology. Innovations in both transmitters and receivers have been made in this project. Finally, this system could be modified in the future to probe more deeply into the stratosphere. This could be accomplished by increasing the emitted energy or optimizing the wavelengths for this purpose. In addition to NASA, this system has applications to the EPA, NOAA, and the DOD. An AFOSR grant has been awarded based on the results of this effort to fund advanced transmitter development at medium (20-40 mJ) energies. A second proposal to the DOD with a letter of support from Air Force Research Laboratory, has been submitted to extend this uv laser technology to 100 mJ levels. Thus, this project has enabled students and faculty at Hampton University to begin to develop research efforts in support of the mission of the DOD. This instrument will be based at Hampton University (HU) to meet our educational goal to train students in lidar technology as well as atmospheric ozone data analysis and interpretation. It will be also available for off-site measurement campaigns and will serve as a test bed for further instrument development. Later development beyond this grant to extend the scientific usefulness of the instrument may include incorporation of an aerosol channel and upgrading the laser to make stratospheric ozone measurements. Seven undergraduates, three graduate students, and one postdoctoral. researcher (formerly an HU student) have been active participants in this research effort.

Chyba, Thomas↗

Development of Laser, Detector, and Receiver Systems for an Atmospheric CO2 Lidar Profiling System

A ground-based Differential Absorption Lidar (DIAL) is being developed with the capability to measure range-resolved and column amounts of atmospheric CO2. This system is also capable of providing high-resolution aerosol profiles and cloud distributions. It is being developed as part of the NASA Earth Science Technology Office s Instrument Incubator Program. This three year program involves the design, development, evaluation, and fielding of a ground-based CO2 profiling system. At the end of a three-year development this instrument is expected to be capable of making measurements in the lower troposphere and boundary layer where the sources and sinks of CO2 are located. It will be a valuable tool in the validation of NASA Orbiting Carbon Observatory (OCO) measurements of column CO2 and suitable for deployment in the North American Carbon Program (NACP) regional intensive field campaigns. The system can also be used as a test-bed for the evaluation of lidar technologies for space-application. This DIAL system leverages 2-micron laser technology developed under a number of NASA programs to develop new solid-state laser technology that provides high pulse energy, tunable, wavelength-stabilized, and double-pulsed lasers that are operable over pre-selected temperature insensitive strong CO2 absorption lines suitable for profiling of lower tropospheric CO2. It also incorporates new high quantum efficiency, high gain, and relatively low noise phototransistors, and a new receiver/signal processor system to achieve high precision DIAL measurements.

Ismail, Syed↗

Lidar system analysis for measurement of atmospheric species

Several important aspects of lidar are discussed, which pertain to a system analysis of the applicability of certain types of lidar to specific measurement objectives. The differential absorption lidar (DIAL) technique is emphasized. A brief treatment of the DIAL technique is followed by a discussion of the comparison of DIAL with other lidar measurement techniques. Sensitivity expressions are presented for DIAL with either direct or coherent (heterodyne) detection systems. A treatment of the fundamental similarities and differences in using the UV and IR spectral regions for species measurements, such as backscattering properties, spectral characteristics of the absorbing species, and factors relevant to the optimization of the DIAL measurement accuracy, is also included. Finally, results obtained from an existing ground-based DIAL system used to measure water vapor profiles are briefly discussed.

Menzies, R. T.↗

LASE measurements of convective boundary layer development during SGP97

The Southern Great Plains 1997 (SGP97) field experiment was conducted in Oklahoma during June-July 1997 to validate the models used for computing remote soil moisture using measurements by microwave radiometers. One of the objectives of SGP97 was to examine the effect of soil moisture on the evolution of the Atmospheric Boundary Layer (ABL) and clouds over the Southern Great Plains (SGP) during the warm season. The LASE (Lidar Atmospheric Sensing Experiment) airborne DIAL (Differential Absorption Lidar) system, which was flown autonomously on the NASA ER-2 aircraft during previous missions, was reconfigured to fly on the NASA P3 research aircraft. During SGP97 LASE was used to study the morning evolution of the ABL, particularly as manifested in the development of the convective boundary layer, and to study the influence of soil moisture variations on the development of ABL. The ABL development is strongly influenced by the surface energy budget, which is in turn influenced by soil moisture, mesoscale meteorology, clouds, and solar insolation. LASE data acquired during this mission are being used to study the ABL water vapor budget, the development of the ABL, spatial and temporal variabilities in the ABL, and the meteorological factors that influence the ABL development. This field experiment also permitted comparisons of LASE water vapor measurements with water vapor profiles acquired by radiosondes launched at the DOE (Department of Energy) Atmospheric Radiation Measurement (ARM) Southern Great Plain (SGP) site and at NASA/Wallops Flight Facility, as well as with measurements from other SGP97 aircraft.

Ismail, Syed↗

Retrieval of Polar Stratospheric Cloud Microphysical Properties from Lidar Measurements: Dependence on Particle Shape Assumptions

A retrieval algorithm has been developed for the microphysical analysis of polar stratospheric cloud (PSC) optical data obtained using lidar instrumentation. The parameterization scheme of the PSC microphysical properties allows for coexistence of up to three different particle types with size-dependent shapes. The finite difference time domain (FDTD) method has been used to calculate optical properties of particles with maximum dimensions equal to or less than 2 mu m and with shapes that can be considered more representative of PSCs on the scale of individual crystals than the commonly assumed spheroids. Specifically. these are irregular and hexagonal crystals. Selection of the optical parameters that are input to the inversion algorithm is based on a potential data set such as that gathered by two of the lidars on board the NASA DC-8 during the Stratospheric Aerosol and Gas Experiment 0 p (SAGE) Ozone Loss Validation experiment (SOLVE) campaign in winter 1999/2000: the Airborne Raman Ozone and Temperature Lidar (AROTEL) and the NASA Langley Differential Absorption Lidar (DIAL). The 0 microphysical retrieval algorithm has been applied to study how particle shape assumptions affect the inversion of lidar data measured in leewave PSCs. The model simulations show that under the assumption of spheroidal particle shapes, PSC surface and volume density are systematically smaller than the FDTD-based values by, respectively, approximately 10-30% and approximately 5-23%.

Reichardt, J.↗