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NASA NTRS1991

Reflectivities of uniform and broken layered clouds

Differences between the reflectivities of uniform layered clouds and of broken clouds taken from the same layers of the Californian coast were investigated using 1 km data obtained by the AVHRRs on the NOAA-9 and -10 satellites during the FIRE Marine Stratocumulus Intensive Field Observations (June 29 - July 18, 1987). The reflectivities are compared at 0.63 micron, where cloud droplets are nonabsorbing, and at 3.7 micron, where the cloud droplets absorb and the single-scattering albedo is about 0.9. It was found that, at visible wavelengths, the reflectivities of broken clouds were only 80-85 percent of those of the same clouds where they formed regions of extensive uniform layers. The radiation not reflected was transmitted to the surface. The results suggest that the presatellite estimates of the planetary albedo may be too large because they failed to allow for the effects of cloud boundaries on cloud reflectivities.

Coakley, James A., Jr.↗
NASA NTRS2008

Radiative Susceptibility of Cloudy Atmospheres to Droplet Number Perturbations: 2. Global analysis from MODIS

Global distributions of albedo susceptibility for areas covered by liquid clouds are presented for 4 months in 2005. The susceptibility estimates are based on expanded definitions presented in a companion paper and include relative cloud droplet number concentration (CDNC) changes, perturbations in cloud droplet asymmetry parameter and single-scattering albedo, atmospheric/surface effects, and incorporation of the full solar spectrum. The cloud properties (optical thickness and effective radius) used as input in the susceptibility calculations come from MODIS Terra and Aqua Collection 5 gridded data. Geographical distributions of susceptibility corresponding to absolute ( absolute cloud susceptibility ) and relative ( relative cloud susceptibility ) CDNC changes are markedly different indicating that the detailed nature of the cloud microphysical perturbation is important for determining the radiative forcing associated with the first indirect aerosol effect. However, both types of susceptibility exhibit common characteristics such as significant reductions when perturbations in single-scattering properties are omitted, significant increases when atmospheric absorption and surface albedo effects are ignored, and the tendency to decrease with latitude, to be higher over ocean than over land, and to be statistically similar between the morning and afternoon MODIS overpasses. The satellite-based susceptibility analysis helps elucidate the role of present-day cloud and land surface properties in indirect aerosol forcing responses. Our realistic yet moderate CDNC perturbations yield forcings on the order of 1-2 W/sq m for cloud optical property distributions and land surface spectral albedos observed by MODIS. Since susceptibilities can potentially be computed from model fields, these results have practical application in assessing the reasonableness of model-generated estimates of the aerosol indirect radiative forcing.

Oreopoulos, Lazaros↗
NASA NTRS2001

Effect of Aerosols on Cloud Field with Satellite-Derived Data and GCM Simulation

Numerical experiment was performed using an general circulation model (GCM) including aerosol indirect effect into water cloud and the simulated global distribution of cloud droplet radii was compared with the global distribution of cloud effective radii retrieved from Advanced Very High Resolution Radiometer (AVHRR). Comparisons of GCM calculation with AVHRR retrieval showed that our GCM generally can simulate the global characteristics of cloud droplet radii such as a land-sea contrast associated with difference of aerosol abundance and coastal region feature due to aerosol injection from adjacent continental area. AVHRR retrieval and GCM simulation, however, are turned out to show disagreement over tropical region. AVHRR retrieval may tend to overestimate droplet radii due to the contamination of signal by drizzles and ice particles, whereas our GCM does not treat aerosol indirect effect in deep convective clouds predominant over tropics. Over equatorial central Pacific, where satellite retrieval may suffer from statistical biases, satellite retrieval and GCM simulation are also found to be different. Keywords: aerosol indirect effect

Suzuki, Kentaroh↗
NASA NTRS2022

Measurement report: Closure Analysis of Aerosol–cloud Composition in Tropical Maritime Warm Convection

Cloud droplet chemical composition is a key observable property that can aid understanding of how aerosols and clouds interact. As part of the Clouds, Aerosols and Monsoon Processes – Philippines Experiment (CAMP2Ex), three case studies were analyzed involving collocated airborne sampling of relevant clear and cloudy air masses associated with maritime warm convection. Two of the cases represented a polluted marine background, with signatures of transported East Asian regional pollution, aged over water for several days, while the third case comprised a major smoke transport event from Kalimantan fires. Sea salt was a dominant component of cloud droplet composition, in spite of fine particulate enhancement from regional anthropogenic sources. Furthermore, the proportion of sea salt was enhanced relative to sulfate in rainwater and may indicate both a propensity for sea salt to aid warm rain production and an increased collection efficiency of large sea salt particles by rain in subsaturated environments. Amongst cases, as precipitation became more significant, so too did the variability in the sea salt to (non-sea salt) sulfate ratio. Across cases, nitrate and ammonium were fractionally greater in cloud water than fine-mode aerosol particles; however, a strong covariability in cloud water nitrate and sea salt was suggestive of prior uptake of nitrate on large salt particles. A mass-based closure analysis of non-sea salt sulfate compared the cloud water air-equivalent mass concentration to the concentration of aerosol particles serving as cloud condensation nuclei for droplet activation. While sulfate found in cloud was generally constrained by the sub-cloud aerosol concentration, there was significant intra-cloud variability that was attributed to entrainment – causing evaporation of sulfate-containing droplets –and losses due to precipitation. In addition, precipitation tended to promote mesoscale variability in the sub-cloud aerosol through a combination of removal, convective downdrafts, and dynamically driven convergence. Physical mechanisms exerted such strong control over the cloud water compositional budget that it was not possible to isolate any signature of chemical production/loss using in-cloud observations. The cloud-free environment surrounding the non-precipitating smoke case indicated sulfate enhancement compared to convective mixing quantified by a stable gas tracer; however, this was not observed in the cloud water (either through use of ratios or the mass closure), perhaps implying that the warm convective cloud timescale was too short for chemical production to be a leading-order budgetary term and because precursors had already been predominantly exhausted. Closure of other species was truncated by incomplete characterization of coarse aerosol (e.g., it was found that only 10 %–50% of sea salt mass found in cloud was captured during clear-air sampling) and unmeasured gasphase abundances affecting closure of semi-volatile aerosol species (e.g., ammonium, nitrate and organic) and soluble volatile organic compound contributions to total organic carbon in cloud water.

Ewan Crosbie↗
NASA NTRS1993

Low cloud investigations for project FIRE: Island studies of cloud properties, surface radiation, and boundary layer dynamics. A simulation of the reflectivity over a stratocumulus cloud deck by the Monte Carlo method

The radiation field over a broken stratocumulus cloud deck is simulated by the Monte Carlo method. We conducted four experiments to investigate the main factor for the observed shortwave reflectively over the FIRE flight 2 leg 5, in which reflectivity decreases almost linearly from the cloud center to cloud edge while the cloud top height and the brightness temperature remain almost constant through out the clouds. From our results, the geometry effect, however, did not contribute significantly to what has been observed. We found that the variation of the volume extinction coefficient as a function of its relative position in the cloud affects the reflectivity efficiently. Additional check of the brightness temperature of each experiment also confirms this conclusion. The cloud microphysical data showed some interesting features. We found that the cloud droplet spectrum is nearly log-normal distributed when the clouds were solid. However, whether the shift of cloud droplet spectrum toward the larger end is not certain. The decrease of number density from cloud center to cloud edges seems to have more significant effects on the optical properties.

Ackerman, Thomas P.↗
NASA NTRS2011

Simultaneous Retrieval of Aerosol and Cloud Properties During the MILAGRO Field Campaign

Estimation of Direct Climate Forcing (DCF) due to aerosols in cloudy areas has historically been a difficult task, mainly because of a lack of appropriate measurements. Recently, passive remote sensing instruments have been developed that have the potential to retrieve both cloud and aerosol properties using polarimetric, multiple view angle, and multi spectral observations, and therefore determine DCF from aerosols above clouds. One such instrument is the Research Scanning Polarimeter (RSP), an airborne prototype of a sensor on the NASA Glory satellite, which unfortunately failed to reach orbit during its launch in March of 2011. In the spring of 2006, the RSP was deployed on an aircraft based in Veracruz, Mexico, as part of the Megacity Initiative: Local and Global Research Observations (MILAGRO) field campaign. On 13 March, the RSP over flew an aerosol layer lofted above a low altitude marine stratocumulus cloud close to shore in the Gulf of Mexico. We investigate the feasibility of retrieving aerosol properties over clouds using these data. Our approach is to first determine cloud droplet size distribution using the angular location of the cloud bow and other features in the polarized reflectance. The selected cloud was then used in a multiple scattering radiative transfer model optimization to determine the aerosol optical properties and fine tune the cloud size distribution. In this scene, we were able to retrieve aerosol optical depth, the fine mode aerosol size distribution parameters and the cloud droplet size distribution parameters to a degree of accuracy required for climate modeling. This required assumptions about the aerosol vertical distribution and the optical properties of the coarse aerosol size mode. A sensitivity study was also performed to place this study in the context of future systematic scanning polarimeter observations, which found that the aerosol complex refractive index can also be observed accurately if the aerosol optical depth is larger than roughly 0.8 at a wavelength of (0.555 m).

Knobelspiesse, K.↗
NASA NTRS1980

Photographic measurement of droplet density

Density of cloud droplets in expansion chamber or static diffusion liquid chamber is measured with error of less than 3 percent by improved photographic technique. Precision is substantial advance over 10 percent accuracy limitation in methods used in past. Method should be useful in pollutant analysis, fine-particle research, and aerosol studies.

Yager, W. C.↗
NASA NTRS2017

Impacts of Solar-Absorbing Aerosol Layers on the Transition of Stratocumulus to Trade Cumulus Clouds

The effects of an initially overlying layer of solar-absorbing aerosol on the transition of stratocumulus to trade cumulus clouds are examined using large-eddy simulations. For lightly drizzling cloud the transition is generally hastened, resulting mainly from increased cloud droplet number concentration (Nc) induced by entrained aerosol. The increased Nc slows sedimentation of cloud droplets and shortens their relaxation time for diffusional growth, both of which accelerate entrainment of overlying air and thereby stratocumulus breakup. However, the decrease in albedo from cloud breakup is more than offset by redistributing cloud water over a greater number of droplets, such that the diurnal-average shortwave forcing at the top of the atmosphere is negative. The negative radiative forcing is enhanced by sizable longwave contributions, which result from the greater cloud breakup and a reduced boundary layer height associated with aerosol heating. A perturbation of moisture instead of aerosol aloft leads to a greater liquid water path and a more gradual transition. Adding absorbing aerosol to that atmosphere results in substantial reductions in liquid water path (LWP) and cloud cover that lead to positive short-wave and negative longwave forcings on average canceling each other. Only for heavily drizzling clouds is the breakup delayed, as inhibition of precipitation overcomes cloud water loss from enhanced entrainment. Considering these simulations as an imperfect proxy for biomass burning plumes influencing Namibian stratocumulus, we expect regional indirect plus semi-direct forcings to be substantially negative to negligible at the top of the atmosphere, with its magnitude sensitive to background and perturbation properties.

Zhou, Xiaoli↗
NASA NTRS2001

GCM Simulations of the Aerosol Indirect Effect: Sensitivity to Cloud Parameterization and Aerosol Burden

We describe the coupling of the Goddard Institute for Space Studies (GISS) general circulation model (GCM) to an online sulfur chemistry model and source models for organic matter and sea-salt that is used to estimate the aerosol indirect effect. The cloud droplet number concentration is diagnosed empirically from field experiment datasets over land and ocean that observe droplet number and all three aerosol types simultaneously; corrections are made for implied variations in cloud turbulence levels. The resulting cloud droplet number is used to calculate variations in droplet effective radius, which in turn allows us to predict aerosol effects on cloud optical thickness and microphysical process rates. We calculate the aerosol indirect effect by differencing the top-of-the-atmosphere net cloud radiative forcing for simulations with present-day vs. pre-industrial emissions. Both the first (radiative) and second (microphysical) indirect effects are explored. We test the sensitivity of our results to cloud parameterization assumptions that control the vertical distribution of cloud occurrence, the autoconversion rate, and the aerosol scavenging rate, each of which feeds back significantly on the model aerosol burden. The global mean aerosol indirect effect for all three aerosol types ranges from -1.55 to -4.36 W/sq m in our simulations. The results are quite sensitive to the pre-industrial background aerosol burden, with low pre-industrial burdens giving strong indirect effects, and to a lesser extent to the anthropogenic aerosol burden, with large burdens giving somewhat larger indirect effects. Because of this dependence on the background aerosol, model diagnostics such as albedo-particle size correlations and column cloud susceptibility, for which satellite validation products are available, are not good predictors of the resulting indirect effect.

Menon, Surabi↗
NASA NTRS2001

GCM Simulations of the Aerosol Indirect Effect: Sensitivity to Cloud Parameterization and Aerosol Burden

We describe the coupling of the Goddard Institute for Space Studies (GISS) general circulation model (GCM) to an online sulfur chemistry model and source models for organic matter and sea-salt that is used to estimate the aerosol indirect effect. The cloud droplet number concentration is diagnosed empirically from field experiment datasets over land and ocean that observe droplet number and all three aerosol types simultaneously; corrections are made for implied variations in cloud turbulence levels. The resulting cloud droplet number is used to calculate variations in droplet effective radius, which in turn allows us to predict aerosol effects on cloud optical thickness and microphysical process rates. We calculate the aerosol indirect effect by differencing the top-of-the-atmosphere net cloud radiative forcing for simulations with present-day vs. pre-industrial emissions. Both the first (radiative) and second (microphysical) indirect effects are explored. We test the sensitivity of our results to cloud parameterization assumptions that control the vertical distribution of cloud occurrence, the autoconversion rate, and the aerosol scavenging rate, each of which feeds back significantly on the model aerosol burden. The global mean aerosol indirect effect for all three aerosol types ranges from -1.55 to -4.36 W m(exp -2) in our simulations. The results are quite sensitive to the pre-industrial background aerosol burden, with low pre-industrial burdens giving strong indirect effects, and to a lesser extent to the anthropogenic aerosol burden, with large burdens giving somewhat larger indirect effects. Because of this dependence on the background aerosol, model diagnostics such as albedo-particle size correlations and column cloud susceptibility, for which satellite validation products are available, are not good predictors of the resulting indirect effect.

Menon, Surabi↗
NASA NTRS1975

The application of satellite data in the determination of ocean temperatures and cloud characteristics and statistics

The author has identified the following significant results. The major shortcoming of the data was the loss of the infrared radiances from the S191 spectrometer. The cloud thermodynamic phase determination procedure was derived and tested with the data collected by the S192 multispectral scanner. Results of the test indicate a large fraction of the data could be classified thermodynamically. An added bonus was the inclusion of snow in the classification approach. The conclusion to be drawn from this portion of the effort is that in most cases considered ice clouds, liquid water droplet clouds, and snow fields can be spectroscopically separated to a high degree of accuracy.

Curran, R. J.↗
NASA NTRS2014

NASA Glenn Propulsion Systems Lab: 2012 Inaugural Ice Crystal Cloud Calibration Procedure and Results

The inaugural calibration of the ice crystal and supercooled liquid water clouds generated in NASA Glenn's engine altitude test facility, the Propulsion Systems Lab (PSL) is reported herein. This calibration was in support of the inaugural engine ice crystal validation test. During the Fall of 2012 calibration effort, cloud uniformity was documented via an icing grid, laser sheet and cloud tomography. Water content was measured via multi-wire and robust probes, and particle sizes were measured with a Cloud Droplet Probe and Cloud Imaging Probe. The environmental conditions ranged from 5,000 to 35,000 ft, Mach 0.15 to 0.55, temperature from +50 to -35 F and relative humidities from less than 1 percent to 75 percent in the plenum.

ice clouds↗
NASA NTRS2000

Near-Global Survey of Cloud Column Susceptibilities Using ISCCP Data

A new parameter, cloud column susceptibility, is introduced to study the aerosol indirect effect. There are several advantages of this new parameter in comparison with the traditional cloud susceptibility. First, no assumptions about constant liquid water content and cloud layer thickness are required in calculations so that errors caused by these assumptions can be avoided. Second, no a priori knowledge of liquid water content is necessary in remote sensing, which makes global survey by satellite data possible even though liquid water content may change significantly. Third, this new parameter can deal with variations of cloud geometrical thickness during cloud-aerosol interactions, which are evidenced by Without assuming how cloud droplet size will respond to changes of number concentration, this new parameter describes the aerosol indirect effect more directly. It addresses the question of how cloud albedo changes with increasing column number concentrations of cloud droplets, which is resulted from cloud-aerosol interactions. In this study, two approaches are used to retrieve cloud column susceptibility by satellite data. The results of both approaches show a striking contrast of cloud column susceptibilities between continental and maritime. Between the two approaches, the one that uses no assumption of constant liquid water content leads to smaller, some times even negative, cloud column susceptibilities. This finding suggests that the aerosol indirect effect may be overestimated if the assumption of constant liquid water content is used in model studies.

Han, Qingyuan↗
NASA NTRS1989

The role of cloud microphysical processes in climate - An assessment from a one-dimensional perspective

A one-dimensional climate model with an interactive cloud formation and precipitation program is used to study the relationship between cloud microphysical processes and climate. It is shown that the rate of precipitation is directly proportional to the fourth power of the mean cloud particle radius. The effects of CO2 doubling on the climate are examined. It is suggested that smaller cloud droplets may be produced by condensation nuclei over the oceans, as a result of greenhouse warming and pollution over land. Larger cloud droplets could be caused by the removal of cloud-forming nuclei, resulting from enhance precipitation due to greenhouse perturbations.

Liou, Kuo-Nan↗
NASA NTRS2013

Saharan Dust Event Impacts on Cloud Formation and Radiation over Western Europe

We investigated the impact of mineral dust particles on clouds, radiation and atmospheric state during a strong Saharan dust event over Europe in May 2008, applying a comprehensive online-coupled regional model framework that explicitly treats particle-microphysics and chemical composition. Sophisticated parameterizations for aerosol activation and ice nucleation, together with two-moment cloud microphysics are used to calculate the interaction of the different particles with clouds depending on their physical and chemical properties. The impact of dust on cloud droplet number concentration was found to be low, with just a slight increase in cloud droplet number concentration for both uncoated and coated dust. For temperatures lower than the level of homogeneous freezing, no significant impact of dust on the number and mass concentration of ice crystals was found, though the concentration of frozen dust particles reached up to 100 l-1 during the ice nucleation events. Mineral dust particles were found to have the largest impact on clouds in a temperature range between freezing level and the level of homogeneous freezing, where they determined the number concentration of ice crystals due to efficient heterogeneous freezing of the dust particles and modified the glaciation of mixed phase clouds. Our simulations show that during the dust events, ice crystals concentrations were increased twofold in this temperature range (compared to if dust interactions are neglected). This had a significant impact on the cloud optical properties, causing a reduction in the incoming short-wave radiation at the surface up to -75Wm-2. Including the direct interaction of dust with radiation caused an additional reduction in the incoming short-wave radiation by 40 to 80Wm-2, and the incoming long-wave radiation at the surface was increased significantly in the order of +10Wm-2. The strong radiative forcings associated with dust caused a reduction in surface temperature in the order of -0.2 to -0.5K for most parts of France, Germany, and Italy during the dust event. The maximum difference in surface temperature was found in the East of France, the Benelux, and Western Germany with up to -1 K. This magnitude of temperature change was sufficient to explain a systematic bias in numerical weather forecasts during the period of the dust event.

Bangert, M.↗
NASA NTRS1985

Cloud Microphysics by Thermal Wave Methods

This experiments series is the first application of a low-gravity experimental technique to the study of cloud microphysics. The low-gravity environment is provided by the parabolic maneuver of NASA's KC-135 aircraft. The primary objective is to compare experimental observations of cloud droplet growth and evaporation in a convection free environment with a numerical model of the process. Beyond that, the work also involves the development and testing of low-gravity research techniques. In particular, passive methods of thermal control have been devised and used effectively. The study to date has shown that the method is particularly suitable for looking at interactions between adjoining portions of the cloud drop field and interactions of the drop field with a solid interface. After final analysis of the data, it is expected the results will shed light on the development of cloud droplet size spectra in natural clouds as well as the performance of certain types of cloud physics instrumentation, particularly continuous flow diffusion chambers and loud condensation nuclei counters.

Anderson, B. J.↗
NASA NTRS1990

Model test of CCN-cloud albedo climate forcing

Cloud condensation nuclei (CCN) influence cloud albedo through their effect on the cloud droplet size distribution. A number of studies have evaluated the climatic impact of the CCN-cloud albedo feedback, but all have assumed that cloud distributions, cloud thicknesses, and cloud liquid water contents would remain constant as the climate adjusted. This assumption has been tested using the Livermore version of the National Center for Atmospheric Research Community Climate Model. The results indicate that there are no significant compensating changes in cloud properties that would counteract the 1.7 percent global albedo increase resulting from a fourfold increase in marine CCN concentration. Furthermore, when ocean surface temperatures are decreased 4 C in a manner broadly consistent with the enhanced cloud albedos, an increase in cloud fraction of 3.5 percent and a reduction in cloud altitude are predicted, leading to a positive feedback from clouds that would imply a climate impact roughly double that calculated from cloud droplet size distribution change alone.

Ghan, S. J.↗
NASA NTRS2005

Clouds of Neptune and Uranus

We present results on the bases and concentrations of methane ice, ammonia ice, ammonium hydrosulfide-solid, water ice, and aqueous-ammonia solution (droplet) clouds of Neptune and Uranus, based on an equilibrium cloud condensation model. Due to their similar p-T structures, the model results for Neptune and Uranus are similar. Assuming 30-50x solar enhancement for the condensibles species, as expected from formation models, we find that the base of the droplet cloud is at the 370 bars for 30 solar, and at 500 bars for 50 solar cases. Despite this, entry probes need to be deployed to only 50-100 bars to obtain all the critical information needed to constrain models of the formation of these planets and their atmospheres.

Atreya, Sushil K.↗