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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 109 records · Page 6

Hyperfine structure of excited states and quadrupole moment of Ne-21 using laser-induced line-narrowing techniques.

Observation results are presented on the optical hyperfine structure in Ne-21 obtained with the aid of laser-induced line-narrowing techniques. The output from a long stabilized single-mode 1.15-micron He-Ne laser focused into an external sample cell containing Ne-21 was used in implementing these techniques. Their applicability is demonstrated for optical hyperfine structure observation in systems whose features are ordinarily masked by Doppler broadening.

Ducas, T. W.↗

Observations of far-infrared transitions between excited states of OH

In observations of the Kleinmann-Low Nebula were detected of Orion 84.42 and 84.60 micron transitions between the P-2 sub 3/2 and Pi-2 sub 3/2 (J = 5/2) levels of OH with respective fluxes of 1.0 + or - 0.3 to the minus 17th power and 1.4 + or - 0.4 x 10 to the minus 17th power W cm/sq. When compared to 119 micron flux levels of OH and 153 micron flux levels of these radicals by Viscuso, these results suggest appreciable self-absorption of OH line radiation within the Nebula. It is probable that the CO emission due to the J = 31 yields 30 rotational transition at 84.411 micron makes a substantial contribution to the observed 84.42 micron flux, and that it also is at least partially absorbed at the 84.42 micron OH transition frequency. The 88.55 and 88.78 micron (J = 9/2 to 7/2) transitions of CH also were sought, but yielded only to upper limits of 3 x 10 to the minus 18th power W /sq cm each. A search of W3-IRS5 yields upper limits to the 84.42 micron OH and 87.19 micron CO (J = 30 to 29) transitions of 2 x 10 minus 18th power W cm/2.

Viscuso, P. J.↗

Observation of far-infrared transitions between excited states of OH

Spectra of the Kleinmann-Low nebula in Orion detected the 84.42 and 84.60 micron transitions between the 2Pi(3/2) J = 7/2 and 2Pi(3/2) J = 5/2 levels of OH with respective fluxes of 1 x 10 to the -17th and 1.4 x 10 to the -17th W/sq cm. When compared to the 119 micron flux levels of OH discussed by Watson (1982) and the 163 micron flux levels of OH by Viscuso et al. (1985), these results suggest appreciable self-absorption of OH line radiation within the nebula. The CO emission due to the J = 31 to 30 rotational transition at 84.411 microns makes a substantial contribution to the observed 84.22 micron flux, and is probably at least partially absorbed at the 84.42 micron OH transition frequency.

Viscuso, P. J.↗

Quantum chemistry and excited states: First investigations on pyrene-like molecules

Although the calculations are expected to be accurate within 10%, it follows then that there cannot be proposed unquestionable one-to-one attribution due to the density of the DIB's (Diffuse Interstellar Bands). Nevertheless, it has been shown that if one is interested in the experimental study of methyl-pyrene cations, for example, then, the most promising candidate is the 1-methyl isomer: this isomer has been investigated by d'Hendecourt and Leger (1993,1994) and their spectrum shows very striking features in very good agreement with both our calculations and a few DIB's. However, 1-methyl-pyrene cation is not the only product susceptible of being formed in this experiment, and further investigations are in progress to give a complete interpretations of the results. This preliminary report on pyrene-like molecules illustrates the role that theoretical calculations can ply in both the design and the interpretation of experiments.

Parisel, Olivier↗

Coherence Measurements for Excited to Excited State Transitions in Barium

Experimental studies concerning elastic and inelastic electron scattering by coherently ensembles of Ba (...6s6p (sub 1)P(sub 1)) atoms with various degrees of alignment will be described. An in-plane, linearly-polarized laser beam was utilized to prepare these target ensembles and the electron scattering signal as a function of polarization angle was measured for several laser geometries at fixed impact energies and scattering angles. From these measurements, we derived cross sections and electron-impact coherence parameters associated with the electron scattering process which is time reverse of the actual experimentally studied process. This interpretation of the experiment is based on the theory of Macek and Herte. The experimental results were also interpreted in terms of cross sections and collision parameters associated with the actual experimental processes. Results obtained so far will be presented and plans for further studies will be discussed.

Trajmar, S.↗