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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 109 records · Page 6
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Optical Bound States in the Continuum Enabled by Magnetic Resonances Coupled to a Mirror

Dielectric metasurfaces made of high refractive index and low optical loss materials have emerged as promising platforms to achieve high-quality factor modes enabling strong light–matter interaction. Bound states in the continuum have shown potential to demonstrate narrow spectral resonances but often require asymmetric geometry and typically feature strong polarization dependence, complicating fabrication and limiting practical applications. Here, we introduce a novel approach for designing high-quality bound states in the continuum using magnetic dipole resonances coupled to a mirror. The resulting metasurface has simple geometric parameters requiring no broken symmetry. To demonstrate the unique features of our photonic platform we show a record-breaking third harmonic generation efficiency from the metasurface benefiting from the strongly enhanced electric field at high-quality resonances. Our approach mitigates the shortcomings of previous platforms with simple geometry enabling facile and large-area fabrication of metasurfaces paving the way for applications in optical sensing, detection, quantum photonics, and nonlinear devices.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2024

Laboratory Study of Magnetic Reconnection in Lunar-relevant Mini-magnetospheres

Abstract Mini-magnetospheres are small ion-scale structures that are well suited to studying kinetic-scale physics of collisionless space plasmas. Such ion-scale magnetospheres can be found on local regions of the Moon, associated with the lunar crustal magnetic field. In this paper, we report on the laboratory experimental study of magnetic reconnection in laser-driven, lunar-like ion-scale magnetospheres on the Large Plasma Device at the University of California, Los Angeles. In the experiment, a high-repetition rate (1 Hz), nanosecond laser is used to drive a fast-moving, collisionless plasma that expands into the field generated by a pulsed magnetic dipole embedded into a background plasma and magnetic field. The high-repetition rate enables the acquisition of time-resolved volumetric data of the magnetic and electric fields to characterize magnetic reconnection and calculate the reconnection rate. We notably observe the formation of Hall fields associated with reconnection. Particle-in-cell simulations reproducing the experimental results were performed to study the microphysics of the interaction. By analyzing the generalized Ohm’s law terms, we find that the electron-only reconnection is driven by kinetic effects through the electron pressure anisotropy. These results are compared to recent satellite measurements that found evidence of magnetic reconnection near the lunar surface.

Astronomy & Astrophysics↗
DOE OSTI2024

Mechanical Design of the Interaction Region Dipole B1pF for Electron Ion Collider

Here, the Electron-Ion Collider (EIC), planned for construction at Brookhaven National Laboratory, will consist of two intersecting beams of intense electrons and high-energy protons or heavier atomic nuclei. The collider will need many demanding components, including high field superconducting magnets for the Interaction Region (IR). It has been decided that a prototype of one such magnet, the B1pF dipole, shall be built, to validate design choices common to all Rutherford cable dipole and quadrupole IR magnets. B1pF is one of several high field magnets in the interaction region whose design is based on the 15.1 mm wide NbTi cable, a cable like the one used in the main dipole coil of the Large Hadron Collider (LHC) at CERN. The current design is based on a single layer coil with an inner diameter of 300 mm and magnetic length of ~3 m which generates a magnetic field at the center of the magnet of about 3.7 T at a current of ~11 kA at design. This paper presents the mechanical design of the B1pF dipole magnet, and the R&D effort associated with the development of the prototype, including tests for successfully winding and curing coils of the needed configuration into proper structural and magnetic elements, and including a multilayer magnetic return yoke which meets field requirements while providing an initial reduced structure suitable for operational testing in an existing test facility.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2025

Spin Squeezing with Itinerant Magnetic Dipoles

Entanglement can improve the measurement precision of quantum sensors beyond the shot noise limit. Neutral atoms, the basis of some of the most precise and accurate optical clocks and interferometers, do not naturally exhibit the all-to-all interactions traditionally used to generate such entangled states. On the other hand, these systems exhibit exceedingly high degrees of experimental control over parameters such as temperature, spatial entropy, and itinerancy. In this work, we investigate spin squeezing in a highly coherent itinerant system of neutral atoms with magnetic dipole-dipole interactions. We achieve 7.1 dB of metrologically useful squeezing using finite-range spin-exchange interactions in an erbium quantum gas microscope, and we demonstrate that introducing atomic motion, realizing a dipolar 𝑡−𝐽 model, protects the spin sector coherence at low fillings, significantly improving the achievable spin squeezing in a 2D dipolar system. This work’s protocol can be implemented with most neutral atoms, opening the door to quantum-enhanced metrology in other itinerant dipolar systems, such as molecules or optical lattice clocks, and serves as a novel method for studying itinerant quantum magnetism with long-range interactions.

Atomic, optical & lattice clocks↗
DOE OSTI2024

Precision Measurements of the Neutron Magnetic Form Factor to High Momentum Transfer using Durand's Method

Protons and neutrons, collectively known as nucleons, along with electrons, constitute the funda- mental building blocks of the visible universe. Understanding their internal structure is crucial for addressing key scientific questions about our origin and existence. Elastic electron-nucleon scatter- ing provides insights into the spatial distributions of charge and current within nucleons through their electromagnetic form factors. Accurate knowledge of these form factors over a broad range of Q2, the squared four-momentum transfer in the scattering process, reveals details about the nucleon’s internal structure. However, high-Q2 data of the nucleon electromagnetic form factor is scarce due to the challenges associated with such measurements. This thesis reports preliminary results from high-precision measurements of the neutron magnetic form factor (Gn M ) to unprecedented Q2 using Durand’s method, also known as the “ratio” method. Systematic errors are greatly reduced by extracting Gn M from the ratio of neutron-coincident (D(e, e'n)) to proton-coincident (D(e, e'p)) quasi-elastic electron scattering from deuteron. The scattered electrons were detected in the BigBite spectrometer, which features multiple Gas Elec- tron Multiplier (GEM) layers with large active area for high-precision tracking at very high rates. Simultaneous nucleon detection was performed by the Super BigBite spectrometer, which utilizes a dipole magnet with large solid angle acceptance at forward angles and a novel hadron calorimeter with very high and comparable detection efficiencies for both protons and neutrons. This setup could handle very high luminosity, making high-Q2 measurements feasible. Data were collected at five Q2 points: 3, 4.5, 7.4, 9.9, and 13.6 (GeV/c)2. Preliminary results are reported for all, with the lowest two Q2 points in good agreement with existing world data, while the higher points significantly extend the Q2 range in which Gn M is known accurately. The precision of the highest Q2 point is expected to remain unmatched for years to come.

Datta, Provakar↗
DOE OSTI2024

Polycaprolactone‐Based Zinc Ink for High Conductivity Transient Printed Electronics and Antennas

Abstract Distributed sensors and electronics can be used in agriculture to optimize crop management and improve environmental outcomes. Electronic devices in these outdoor spaces require medium to long range (>1m) wireless communication of data over several weeks or months, which in turn requires high conductivity (1 × 10 5 Sm −1 ) antennas. Printed bioinert or ecoresorbable conductors, comprising carbon, magnesium, or zinc fillers, typically exhibit conductivity on the order of 10–1000 Sm −1 and lifetimes from a few hours to a few days. A print‐based fabrication process for chemically treated zinc traces, which achieves conductivity of up to 6 × 10 5 Sm −1 is reported here. The ink formulation uses a non‐water‐soluble soil biodegradable polycaprolactone binder. The ink and printing processes reported here led to stable conductive traces that are used in ultra high frequency radio frequency identification (UHF‐RFID) folded dipole antennas operating at 915 MHz. The conductivity of the printed traces is maintained for over 70 days in ambient environments when traces are protected by a biodegradable beeswax encapsulation layer.

Baumbauer, Carol L.↗
DOE OSTI2022

A coupled vacancy diffusion-dislocation dynamics model for the climb-glide motion of jogged screw dislocations

Here, we develop a novel model to study the climb/glide motion of jogged screw dislocations within the discrete dislocation dynamics (DDD) framework. We present results for the dependence of the climb velocity on the applied stress and on the jog size and distribution statistics. We show that the model predictions are consistent with experimental data in both γ-TiAl and Zircaloy-4. The ranges of the applied stress and jog spacing that determine the dominance of one of three dislocation mechanisms are identified. These are the jog dragging, dipole dragging, and dipole bypass mechanisms, respectively. The overall dislocation motion in the jog dragging regime is composed of glide of screw segments and climb of jogs, controlling the plastic strain and the creep rate, respectively. Based on current simulations and on a detailed examination of the predicted jog heights compared to experiments, we advance the hypothesis that a combination of jog dragging and dipole bypass mechanisms is necessary to reproduce the high creep rate observed in some experiments.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Measurement of nuclear interaction cross sections towards neutron-skin thickness determination

The accuracy of reaction theories used to extract properties of exotic nuclei from scattering experiments is often unknown or not quantified, but of utmost importance when, e.g., constraining the equation of state of asymmetric nuclear matter from observables as the neutron-skin thickness. In order to test the Glauber multiple-scattering model, the total interaction cross section of 12 C on carbon targets was measured at initial beam energies of 400, 550, 650, 800, and 1000 MeV/nucleon. The measurements were performed during the first experiment of the newly constructed R 3 B (Reaction with Relativistic Radioactive Beams) experiment after the start of FAIR Phase-0 at the GSI/FAIR facility with beam energies of 400, 550, 650, 800, and 1000 MeV/nucleon. The combination of the large-acceptance dipole magnet GLAD and a newly designed and highly efficient Time-of-Flight detector enabled a precise transmission measurement with several target thicknesses for each initial beam energy with an experimental uncertainty of ±0.4%. A comparison with the Glauber model revealed a discrepancy of around 3.1% at higher beam energies, which will serve as a crucial baseline for the model-dependent uncertainty in future fragmentation experiments.

Astronomy & Astrophysics↗
DOE OSTI2023

Towards critical and supercritical electromagnetic fields

Abstract The availability of ever stronger, laser-generated electromagnetic fields underpins continuing progress in the study and application of nonlinear phenomena in basic physical systems, ranging from molecules and atoms to relativistic plasmas and quantum electrodynamics. This raises the question: how far will we be able to go with future lasers? One exciting prospect is the attainment of field strengths approaching the Schwinger critical field ${E}_{\mathrm{cr}}$ in the laboratory frame, such that the field invariant ${E}^2-{c}^2{B}^2>{E}_{\mathrm{cr}}^2$ is reached. The feasibility of doing so has been questioned, on the basis that cascade generation of dense electron–positron plasma would inevitably lead to absorption or screening of the incident light. Here we discuss the potential for future lasers to overcome such obstacles, by combining the concept of multiple colliding laser pulses with that of frequency upshifting via a tailored laser–plasma interaction. This compresses the electromagnetic field energy into a region of nanometre size and attosecond duration, which increases the field magnitude at fixed power but also suppresses pair cascades. Our results indicate that laser facilities with peak power of tens of PW could be capable of reaching ${E}_{\mathrm{cr}}$ . Such a scenario opens up prospects for the experimental investigation of phenomena previously considered to occur only in the most extreme environments in the universe.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2022

Contrasting Climatic Trends of Atmospheric River Occurrences Over East Asia

Atmospheric rivers (ARs) are increasingly recognized as a major driver of hydrological cycles, and are projected to increase around the world under a changing climate. However, the long-term trends of ARs over East Asia (EA) remains less elucidated. Here we fill the gap by developing a longest-ever archive of EA ARs, and examine its role in determining spatiotemporal precipitation variability over EA. We find contrasting changes in AR occurrences, with more frequent ARs in low latitudes but less in high latitudes during the period 1950-2020. The “dipole” pattern of decadal changes in AR occurrences is dictated by atmospheric dynamics (i.e., winds) in the north but thermodynamics (i.e., moisture) in the south. The reduced AR occurrences explain 49% of decreased annual precipitation in northern China, while more AR-related precipitation is observed in southern China. Furthermore, our results provide new insights into regional hydroclimate over EA by connecting it with large-scale weather systems.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

HTS Dipole Magnet Model for the Persistent Current Operation

Recent advances in the fabrication of high-temperature superconducting (HTS) coils allow the design of superconducting accelerator magnets that work in a persistent current mode. Many various, rather low-field magnets in particle accelerators operate in the DC current mode. Fermilab designed, fabricated, and tested an HTS dipole magnet model that has 20-mm air gap and a magnetic field up to 0.5 T. The magnet has a primary copper coil that for a short period pumps the energy in the short-circuited secondary HTS coil. Here, the current paper presents the design, fabrication, and testing of this magnet at liquid-nitrogen temperature.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

Electric and magnetic dipole strength in 112,114,116,118,120,124 Sn

Background: There is renewed interest in electric dipole strength distributions for a variety of reasons including the extraction of the dipole polarizability related to properties of the symmetry energy and a measure for the neutron skin thickness, understanding the structure of low-energy $\textit{E}$1 strength in nuclei with neutron excess, and establishing the systematics of the isovector giant dipole resonance (IVGDR). Inelastic proton scattering at energies of a few hundred MeV and very forward angles including 0° has been established as a tool for the study of electric and magnetic dipole strength distributions in nuclei. Purpose: The present work aims at a systematic investigation of the electric and magnetic dipole strength distributions in the chain of stable even-mass tin isotopes. Methods: Inelastic proton scattering experiments were performed at the Research Center for Nuclear Physics, Osaka, with a 295-MeV beam covering laboratory angles 0°–6° and excitation energies 6–22 MeV. Cross sections due to $\textit{E}$1 and $\textit{M}$1 excitations were extracted with a multipole decomposition analysis (MDA) and then converted to reduced transition probabilities with the “virtual photon method” for $\textit{E}$1 and the “unit cross section method” for $\textit{M}$1 excitations, respectively. Including a theory-aided correction for the high-excitation-energy region not covered experimentally, the electric dipole polarizability was determined from the $\textit{E}$1 strength distributions. Results: In this work, total photoabsorption cross sections derived from the $\textit{E}$1 and $\textit{M}$1 strength distributions show significant differences compared to those from previous ($\textit{γ, xn}$) experiments in the energy region of the IVGDR. The widths of the IVGDR deduced from the present data with a Lorentz parametrization show an approximately constant value of about 4.5 MeV in contrast to the large variations between isotopes observed in previous work. The IVGDR centroid energies are in good correspondence to expectations from empirical systematics of their mass dependence. Furthermore, a study of the dependence of the IVGDR energies on bulk matter properties is presented. The $\textit{E}$1 strengths below neutron threshold show fair agreement in this work with results from ($\textit{γ, γ'}$) experiments on 112,116,120,124 Sn in the energy region between 6 and 7 MeV, where also isoscalar $\textit{E}$1 strength was found for 124 Sn. At higher excitation energies, large differences are observed, pointing to a different nature of the excited states with small ground-state branching ratios. The isovector spin-$\textit{M}$1 strengths exhibit a broad distribution between 6 and 12 MeV in all studied nuclei. Conclusions: The present results contribute to the solution of a variety of nuclear structure problems including the systematics of the energy and width of the IVGDR, the structure of low-energy $\textit{E}$1 strength in nuclei, new constraints to energy density functionals (EDFs) aiming at a systematic description of the dipole polarizability across the nuclear chart, from which properties of the symmetry energy can be derived, and the systematics of the isovector spin-$\textit{M}$1 strength in heavy nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Relative-Humidity Dependence of Electrochemically Active Surface Area in Porous Carbon Catalyst Layers

Polymer-electrolyte fuel cells (PEFCs) utilize porous catalyst layers (CLs) formed of carbon supports on which Pt particles are deposited and ionomer films are distributed. Carbon supports themselves have varying degrees of porosity, where high-surface-area carbon (HSC) supports possess nanometer-sized interior pores that are suitable for Pt nanoparticle deposition but prevent deleterious ionomer penetration. However, this requires protons to transport through water pathways inside the pores. To understand the generation of such pathways, we examine the various mechanisms of water uptake by PEFC CLs, and the subsequent impact of water uptake on Pt utilization through developing a multiphysics model of the water wetting phenomena as a function of relative humidity. The model details water uptake via ionomer absorption, capillary condensation in the hydrophilic pores, and surface adsorption using molecular potential that account for various water and surface dipole interactions. The results quantify how mesoporous carbons with highly hydrophilic pores increase Pt utilization through the development of wetted layers, which at the same time enable optimized gas-transport pathways. It also demonstrates the impact of pore-size distribution (PSD) and physical and chemical parameters on the water uptake phenomena, allowing for future CL particle and structure optimization.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Photodetachment spectroscopy and resonant photoelectron imaging of cryogenically cooled 1-pyrenolate

We report an investigation of the 1-pyrenolate anion (PyO - ) and the 1-pyrenoxy radical (PyO) using photodetachment spectroscopy and resonant photoelectron imaging of cryogenically-cooled anions. The electron affinity of PyO is measured to be 2.4772(4) eV (19,980 ± 3 cm -1 ) from high-resolution photoelectron spectroscopy. Photodetachment spectroscopy reveals a dipole-bound state (DBS) for PyO - 280 cm-1 below the detachment threshold, as well as a broad and intense valence excited state (shape resonance) 1,077 cm-1 above the detachment threshold. The shape resonance with an excitation energy of 21,055 cm -1 is due to excitation of an electron from the highest occupied molecular orbital of PyO - to its lowest unoccupied molecular orbital in the continuum. Twenty-nine vibrational levels of the DBS are observed, including twenty-seven above-threshold vibrational levels (vibrational Feshbach resonances). Twenty-seven resonant photoelectron spectra are obtained by tuning the detachment laser to the vibrational Feshbach resonances, resulting in highly non-Franck-Condon photoelectron spectra and rich vibrational information. In total, the frequencies of twenty-one vibrational modes are obtained for the PyO radical by the combination of the photodetachment and resonant photoelectron spectroscopy, including thirteen out-of-plane bending modes.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

Singlet magnetism in intermetallic UGa 2 unveiled by inelastic x-ray scattering

Using high resolution tender x-ray resonant inelastic scattering and hard x-ray nonresonant inelastic scattering beyond the dipole limit we were able to detect electronic excitations in intermetallic UGa 2 that are highly atomic in nature. Analysis of the spectral lineshape reveals that the local 5⁢ƒ 2 configuration characterizes the correlated nature of this ferromagnet. The orientation and directional dependence of the spectra indicate that the ground state is made of the Γ 1 singlet and/or Γ 6 doublet symmetry. With the ordered moment in the ab plane, we infer that the magnetism originates from the higher lying Γ 6 doublet being mixed with the Γ 1 singlet due to intersite exchange, qualifying UGa 2 to be a true quantum magnet. The ability to observe atomic excitations is crucial to resolve the ongoing debate about the degree of localization versus itineracy in U intermetallics.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2025

Magnetic and Mechanical Analysis of Bi-2212 Rutherford Cable in a Cos-Theta Sub-Scale Dipole Coil

The U.S. Magnet Development Program (US-MDP) explores high-field accelerator magnets compatible with operational conditions beyond the limits of Nb$_3$Sn technology. The ongoing R&D High-Temperature Superconductors (HTS) suggests using Bi$_2$Sr$_2$CaCu$_2$O$_{8-x}$ (Bi-2212) as superconducting element. Bi-2212 Rutherford cables maintain a high critical current (I$_C$) when exposed to a large external magnetic field. However, Bi-2212 exhibits an oversensitive stress-strain response when subject to large Lorentz forces. This paper reports on the magnetic and mechanical analysis of the Bi-2212 cosine-theta insert being developed at Fermilab for a hybrid magnet composed of two external layers of Nb$_3$Sn and two internal layers of Bi-2212. We performed a FEM analysis of the insert to estimate the HTS stress state in the coil's strands under magnetic and mechanical loads.

43 PARTICLE ACCELERATORS↗
DOE OSTI2024

Development and test of a large-aperture Nb3Sn cos-theta dipole coil with stress management

The stress-managed cos-theta (SMCT) coil is a new concept which was proposed and is being developed at Fermilab in the framework of US Magnet Development Program (US-MDP) for high-field and/or large-aperture accelerator magnets based on low-temperature and high-temperature superconductors. A 120-mm aperture two-layer Nb3Sn SMCT dipole coil has been developed at Fermilab to demonstrate and test the SMCT concept including coil design, fabrication technology and performance. The first SMCT demo coil was fabricated and assembled with 60-mm aperture Nb3Sn coil inside a dipole mirror configuration and tested separately and in series with the insert coil. This paper summarizes the design, parameters, and quench performance of the 120-mm aperture SMCT coil in a dipole mirror configuration.

43 PARTICLE ACCELERATORS↗