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At least 109 records · Page 6

Generalized symmetry in dynamical gravity

We explore generalized symmetry in the context of nonlinear dynamical gravity. Our basic strategy is to transcribe known results from Yang-Mills theory directly to gravity via the tetrad formalism, which recasts general relativity as a gauge theory of the local Lorentz group. By analogy, we deduce that gravity exhibits a one-form symmetry implemented by an operator U α labeled by a center element α of the Lorentz group and associated with a certain area measured in Planck units. The corresponding charged line operator W ρ is the holonomy in a spin representation ρ, which is the gravitational analog of a Wilson loop. The topological linking of U α and W ρ has an elegant physical interpretation from classical gravitation: the former materializes an exotic chiral cosmic string defect whose quantized conical deficit angle is measured by the latter. We verify this claim explicitly in an AdS-Schwarzschild black hole background. Notably, our conclusions imply that the standard model exhibits a new symmetry of nature at scales below the lightest neutrino mass. More generally, the absence of global symmetries in quantum gravity suggests that the gravitational one-form symmetry is either gauged or explicitly broken. The latter mandates the existence of fermions. Finally, we comment on generalizations to magnetic higher-form or higher-group gravitational symmetries.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Two-Dimensional Uranyl Borates: From Conventional to Extreme Synthetic Conditions: Two-Dimensional Uranyl Borates: From Conventional to Extreme Synthetic Conditions

A systematic investigation of uranyl borates under different synthetic conditions resulted in five new 2D compounds, namely, (H 3 O)[(UO 2 )(BO 3 )], Li[(UO 2 )(BO 3 )] · (H 2 O), α-K 4 [(UO 2 ) 5 (BO 3 ) 2 O 4 ], β-K 4 [(UO 2 ) 5 (BO 3 ) 2 O 4 ] and K 2.5 [(UO 2 ) 5 (BO 3 ) 2 O 2.5 (OH) 1.5 ] · (H 2 O) 2.5 . (H 3 O)[(UO 2 )(BO 3 )] and Li[(UO 2 )(BO 3 )] · (H 2 O) were obtained from hydrothermal reactions at 220 °C using the same mineralizer. Both materials possess the uranophane sheet topology with different symmetry of the unit cells. In the structure of (H 3 O)[(UO 2 )(BO 3 )] and Li[(UO 2 )(BO 3 )] · (H 2 O), UO 7 pentagonal bipyramids share edges and vertexes with four BO 3 planar triangles. α-K 4 [(UO 2 ) 5 (BO 3 ) 2 O 4 ] and β-K 4 [(UO 2 ) 5 (BO 3 ) 2 O 4 ] are polytypes. α-K 4 [(UO 2 ) 5 (BO 3 ) 2 O 4 ] was synthesized from a high-temperature solid-state reaction under ambient pressure; whereas β-K 4 [(UO 2 ) 5 (BO 3 ) 2 O 4 ] was obtained from a high-temperature/high-pressure (HT/HP) reaction. Both structures have an identical anion topology, but β-K 4 [(UO 2 ) 5 (BO 3 ) 2 O 4 ] crystallizes in space group with higher symmetry. In K 2.5 [(UO 2 ) 5 (BO 3 ) 2 O 2.5 (OH) 1.5 ] · (H 2 O) 2.5 , which was obtained from a hydrothermal reaction, UO 7 polyhedra share vertexes and edges with two independent BO 3 triangles, forming the most complex uranyl borate layers among all five compounds. The different synthetic routes, novel topologies, thermal behavior and Raman spectra are discussed.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Transverse spin in the light-ray OPE

We study a product of null-integrated local operators O 1 and O 2 on the same null plane in a CFT. Such null-integrated operators transform like primaries in a fictitious d – 2 dimensional CFT in the directions transverse to the null integrals. We give a complete description of the OPE in these transverse directions. The terms with low transverse spin are light-ray operators with spin J 1 + J 2 – 1. The terms with higher transverse spin are primary descendants of light-ray operators with higher spins J 1 + J 2 – 1 + n, constructed using special conformally-invariant differential operators that appear precisely in the kinematics of the light-ray OPE. As an example, the OPE between average null energy operators contains light-ray operators with spin 3 (as described by Hofman and Maldacena), but also novel terms with spin 5, 7, 9, etc. These new terms are important for describing energy two-point correlators in non-rotationally-symmetric states, and for computing multi-point energy correlators. We check our formulas in a non-rotationally-symmetric energy correlator in N = 4 SYM, finding perfect agreement.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Chiral electronic excitations in the quasi-two-dimensional Rashba system BiTeI

The optical transitions between spin-polarized bands of the quasi-two-dimensional Rashba system BiTeI are investigated using polarization-resolved resonant Raman spectroscopy. We detect chiral excitations between states with opposite helicity and compare spectra to calculations within a three-band model. Using the resonant Raman excitation profile, we deduce the Rashba parameters and band gaps of the higher conduction bands near the Fermi level, and compare the parameters to values obtained by ab initio density functional theory.

36 MATERIALS SCIENCE↗

Pion gravitational form factors in the QCD instanton vacuum. I

The pion form factors of the QCD energy-momentum tensor (EMT) are studied in the instanton liquid model (ILM) of the QCD vacuum. In this approach, the breaking of conformal symmetry is encoded in the form of stronger-than-Poisson fluctuations in the number of instantons. For the trace of the EMT, it is shown that the gluonic trace anomaly term contributes half the pion mass, with the other half coming from the quark-mass-dependent σ term. The Q 2 dependence of the form factors is governed by glueball and scalar meson exchanges. For the EMT, the spin-0 (trace) and spin-2 (traceless rank-2 tensor) form factors are computed at next-to-leading order in the instanton density using effective quark operators. Relations between the gluon and quark contributions to the EMT form factors are derived. The form factors are also expressed in terms of the pion light-front wave functions in the ILM. The results at the low resolution scale of the inverse instanton size are evolved to higher scales using the renormalization group equation. The ILM results compare well with those of recent lattice QCD calculations. Published by the American Physical Society 2024

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Emergent Dimer-Model Topological Order and Quasiparticle Excitations in Liquid Crystals: Combinatorial Vortex Lattices

Liquid crystals have proven to provide a versatile experimental and theoretical platform for studying topological objects such as vortices, skyrmions, and hopfions. In parallel, in hard condensed matter physics, the concept of topological phases and topological order has been introduced in the context of spin liquids to investigate emergent phenomena like quantum Hall effects and high-temperature superconductivity. Here, we bridge these two seemingly disparate perspectives on topology in physics. Combining experiments and simulations, we show how topological defects in liquid crystals can be used as versatile building blocks to create complex, highly degenerate topological phases, which we refer to as “combinatorial vortex lattices” (CVLs). CVLs exhibit extensive residual entropy and support locally stable quasiparticle excitations in the form of charge-conserving topological monopoles, which can act as mobile information carriers and be linked via Dirac strings. CVLs can be rewritten and reconfigured on demand, endowed with various symmetries, and modified through laser-induced topological surgery—an essential capability for information storage and retrieval. We demonstrate experimentally the realization, stability, and precise optical manipulation of CVLs, thus opening new avenues for understanding and technologically exploiting higher-hierarchy topology in liquid crystals and other ordered media.

36 MATERIALS SCIENCE↗

Spin-orbit correlations in the nucleon in the large- N c limit

We study the twist-3 spin-orbit correlations of quarks described by the nucleon matrix elements of the parity-odd rank-2 tensor QCD operator (the parity-odd partner of the QCD energy-momentum tensor). Our treatment is based on the effective dynamics emerging from the spontaneous breaking of chiral symmetry and the mean-field picture of the nucleon in the large- N c limit. The twist-3 QCD operators are converted to effective operators, in which the QCD interactions are replaced by spin-flavor-dependent chiral interactions of the quarks with the pion field. We compute the nucleon matrix elements of the twist-3 effective operators and discuss the role of the chiral interactions in the spin-orbit correlations. We derive the first-quantized representation in the mean-field picture and develop a quantum-mechanical interpretation. The chiral interactions give rise to new spin-orbit couplings and qualitatively change the correlations compared to the quark model picture. We also derive the twist-3 matrix elements in the topological soliton picture where the quarks are integrated out (skyrmion). The methods used here can be extended to other QCD operators describing higher-twist nucleon structure and generalized parton distributions. Published by the American Physical Society 2024

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Celestial operator product expansions and w 1+∞ symmetry for all spins

The operator product expansion of massless celestial primary operators of arbitrary spin is investigated. Poincaré symmetry is found to imply a set of recursion relations on the operator product expansion coefficients of the leading singular terms at tree-level in a holomorphic limit. The symmetry constraints are solved by an Euler beta function with arguments that depend simply on the right-moving conformal weights of the operators in the product. These symmetry-derived coefficients are shown not only to match precisely those arising from momentum-space tree-level collinear limits, but also to obey an infinite number of additional symmetry transformations that respect the algebra of w 1+∞ . In tree-level minimally-coupled gravitational theories, celestial currents are constructed from light transforms of conformally soft gravitons and found to generate the action of w 1+∞ on arbitrary massless celestial primaries. Results include operator product expansion coefficients for fermions as well as those arising from higher-derivative non-minimal couplings of gluons and gravitons.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Effects of Anisotropic Strain on Spin–Orbit Torque Produced by the Dirac Nodal Line Semimetal IrO 2

We report spin-torque ferromagnetic resonance studies of the efficiency of the damping-like (ξ DL ) spin–orbit torque exerted on an adjacent ferromagnet film by current flowing in epitaxial (001) and (110) IrO 2 thin films. IrO 2 possesses Dirac nodal lines (DNLs) in the band structure that are gapped by spin–orbit coupling, which could enable a very high spin Hall conductivity, σ SH . We find that the (001) films do exhibit exceptionally high ξ DL ranging from 0.45 at 293 K to 0.65 at 30 K, which sets the lower bounds of σ SH to be 1.9 × 10 5 and 3.75 × 10 5 Ω –1 m –1 , respectively, 10 times higher and of opposite sign than the theoretical prediction. Furthermore, ξ DL and σ SH are substantially reduced in anisotropically strained (110) films. Here, we suggest that this high sensitivity to anisotropic strain is because of changes in contributions to σ SH near the DNLs.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Tuning the charge transfer character of the multiexciton state in singlet fission

Intramolecular singlet fission (SF) produces the multiexciton correlated triplet pair state, (T 1 T 1 ), prior to the formation of free triplet excitons. The nature of the multiexciton state is complex, as generation of the (T 1 T 1 ) state may involve a charge transfer (CT) intermediate and has been shown to have both mixed electronic and spin characters. According to transient absorption spectroscopy, a linear terrylene-3,4:11,12-bis(dicarboximide) dimer (TDI 2 ) exhibits solvent-dependent excited-state dynamics. As solvent polarity increases from 1,2,4-trichlorobenzene (ε = 2.2) to chlorobenzene (ε = 5.6) to 1,2-dichlorobenzene (ε = 9.9), the SF rate in TDI2 increases and the multiexciton state, which can be thought of as a linear combination of the 1 (S 1 S 0 ), CT, and (T 1 T 1 ) states, gains more CT character. Eventually, the CT state becomes a trap state as indicated by symmetry-breaking charge separation in TDI2 in pyridine (ε = 12.3). The dielectric environment influences not only the SF rate and the relative contributions of the 1 (S 1 S 0 ), CT, and (T 1 T 1 ) states to the overall multiexciton state but also the rate at which the state mixing evolves, with faster dynamics in higher polarity solvents. More importantly, the tunability and presence of strong CT character in the multiexciton state have implications for SF applications since they often rely on electron transfer from the free triplet excitons. This enhanced CT character in the (T 1 T 1 ) state may assist with two-electron transfer directly from the (T 1 T 1 ) state, allowing for facile extraction of charges in intramolecular SF systems whose (T 1 T 1 ) states do not always efficiently dissociate to two triplet excitons.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Laser spectroscopy for the study of exotic nuclei

Investigation into the properties and structure of unstable nuclei far from stability is a key avenue of research in modern nuclear physics. These efforts are motivated by the continual observation of unexpected structure phenomena in nuclei with unusual proton-to-neutron ratios. In recent decades, laser spectroscopy techniques have made significant contributions in our understanding of exotic nuclei in different mass regions encompassing almost the entire nuclear chart. This is achieved through determining multiple fundamental properties of nuclear ground and isomeric states, such as nuclear spins, magnetic dipole and electric quadrupole moments and charge radii, via the measurement of hyperfine structures and isotope shifts in the atomic or ionic spectra of the nuclei of interest. These properties offer prominent tests of recently developed state-of-the-art nuclear theory and help to stimulate new developments in improving the many-body methods and nucleon–nucleon interactions at the core of these models. With the aim of exploring more exotic short-lived nuclei located ever closer to the proton and neutron driplines, laser spectroscopy techniques, with their continuous technological developments towards higher resolution and higher sensitivity, are extensively employed at current- and next-generation radioactive ion beam facilities worldwide. Ongoing efforts in parallel promise to improve the availability of these even more exotic species at next-generation facilities. Very recently, an innovative application of laser spectroscopy on molecules containing short-lived nuclei has been demonstrated offering additional opportunities for several fields of research, e.g. fundamental symmetry studies and astrophysics. Here, in this review, the basic nuclear properties measurable with laser spectroscopy will be introduced. How these observables are associated with nuclear structure and nucleon–nucleon interactions will be discussed. Following this, a general overview of different laser spectroscopy methods will be given with particular emphasis on technical advancements reported in recent years. The main focus of this article is to review the numerous highlights that have resulted from studying exotic nuclei in different mass regions with laser spectroscopy techniques since the last edition in this series. Finally, the challenges facing the field in addition to future opportunities will be discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Strong Hilbert space fragmentation and fractons from subsystem and higher-form symmetries

Here, we introduce a route to Hilbert space fragmentation in high dimensions leveraging the group-word formalism. We show that taking strongly fragmented models in one dimension and “lifting” to higher dimensions using subsystem symmetries can yield strongly fragmented dynamics in higher dimensions, with subdimensional (e.g., lineonic) excitations. This provides a route to higher-dimensional strong fragmentation, and also a route to fractonic behavior. Meanwhile, lifting one-dimensional fragmented models to higher dimensions using higher-form symmetries yields models with topologically robust fragmentation. In three or more spatial dimensions, one can also “mix and match” subsystem and higher-form symmetries, leading to canonical fracton models such as X cube. We speculate that this approach could also yield a route to non-Abelian fractons. These constructions unify a number of phenomena that have been discussed in the literature, as well as furnishing models with unique properties.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Structure of domain walls in chiral spin liquids

The chiral spin liquid is a canonical state of quantum spins combining topological and symmetry-breaking order, and possible experimental realizations have attracted growing interest. We examine the physics at interfaces between chiral spin liquid domains of opposite chirality. We show that a self-consistent mean-field description of spinons remains possible in the vicinity of a domain wall and use this to formulate a Ginzburg–Landau theory of the domain wall. The bulk of a chiral spin liquid contains gapped spinon excitations and gauge fluctuations, set by a finite spinon mass and a nonzero spinon Chern number. A third class of excitations consists of amplitude fluctuations of the spinon hoppings, which admit a geometric interpretation in terms of effective vielbein fields. These fluctuations are usually neglected because they are irrelevant for a homogeneous chiral spin liquid and are suppressed in standard large- N treatments. Going beyond the purely topological Chern–Simons limit, we incorporate these fluctuations into an effective field theoretic framework and show that they generate momentum-dependent corrections, including Chern–Simons-like linear terms and higher-order contributions, beyond the universal topological limit. We then analyze nontopological properties, including domain wall tension and edge velocity, and explain how they modify observables relative to the uniform case. These results connect measurable, nonuniversal quantities such as domain wall width, domain wall tension, and edge velocity to microscopic parameters and provide concrete targets for experiments.

domain walls↗

Construction of hopfion crystals

Hopfions, three-dimensional topological solitons characterized by nontrivial Hopf indices, represent a fundamental class of field configurations that emerge across diverse areas of physics. Despite extensive studies of isolated hopfions, a framework for constructing spatially ordered arrays of hopfions, i.e., hopfion crystals, has been lacking. Here, we present a systematic approach for generating hopfion crystals with cubic symmetry by combining the Hopf map with rational mapping techniques. By superposing helical waves in ℝ 4 , we construct hopfion crystals with tunable Hopf indices and controllable topology. We demonstrate simple cubic, face-centered cubic, and body-centered cubic hopfion crystals and extend our framework to create crystals of more complex topological structures, including axially symmetric tori, torus links, and torus knots with higher Hopf indices. Our results provide a foundation for searching hopfions in real materials and studying their collective phenomena.

3-dimensional systems↗

Exploring Anomalous Photoelectron Angular Distributions in the Photoelectron Spectra of Gd 3 O 3 – : Study of Gd 3 O 2 – and Gd 3 O 3 – Using Photoelectron Spectroscopy and Density Functional Theory Calculations

Anion photoelectron (PE) spectra of lanthanide oxide clusters obtained previously have exhibited anomalous photoelectron angular distributions which were attributed to strong PE–valence electron (PEVE) interactions. Here, to further explore this effect, we have obtained the PE spectra of Gd 3 O 2 – and Gd 3 O 3 – , two clusters that have similarly complex electronic structures but contrasting symmetries. The spectra exhibit manifolds of detachment transitions at similar binding energies in a 0.5 eV window of energy. The electron affinity of Gd 3 O 2 is measured to be 1.29 ± 0.05 eV, and that of Gd 3 O 3 is 1.31 ± 0.05 eV. As seen in previous studies on lanthanide oxide cluster anions in lower than conventional oxidation states, transitions in spectra obtained lower photon energies are more congested than those obtained with higher photon energy, a signature of strong PEVE interactions. While the detachment transitions have predominantly parallel photoelectron angular distributions (PAD), the PAD varies across the manifold of transitions in the PE spectrum of Gd 3 O 3 – in a way that suggests four different subgroups of transitions. Results of calculations on Gd 3 O 2 – suggest kite or V-shape structures with antiferromagnetic coupling between one of the 4f 7 subshells with the two others. Calculations on Gd 3 O 3 – more definitively point to ring structures with a nearly isoenergetic ferromagnetically coupled high spin (24-tet) state and a dectet state in which one of the 4f 7 subshells is antiferromagnetically coupled with the other two. Taking these results as qualitative, we propose that strong mixing between the unperturbed states predicted computationally leads to overlapping transitions with different PADs.

anions↗

Detectors in weakly-coupled field theories

We initiate a study of asymptotic detector operators in weakly-coupled field theories. These operators describe measurements that can be performed at future null infinity in a collider experiment. In a conformal theory they can be identified with light-ray operators, and thus have a direct relation to the spectrum of the theory. After a general discussion of the underlying physical picture, we show how infrared divergences of general detector operators can be renormalized in perturbation theory, and how they give rise to detector anomalous dimensions. We discuss in detail how this renormalization can be performed at the intersections of the Regge trajectories where non-trivial mixing occurs, which is related to the poles in anomalous dimensions at special values of spin. Finally, we discuss novel horizontal trajectories in scalar theories and show how they contribute to correlation functions. Our calculations are done in the example of Φ 4 theory in d = 4 - ϵ dimensions, but the methods are applicable more broadly. At the Wilson-Fisher fixed point our results include an explicit expression for the Pomeron light-ray operator at two loops, as well as a prediction for the value of the Regge intercept at five loops.

47 OTHER INSTRUMENTATION↗

Spin-lattice and spin-electronic interactions in the van der Waals semiconductor C⁢o 2 ⁢P 2 ⁢S 6

Here, we report the results of a temperature-dependent reflection spectroscopy study, across a wide energy range (~ 0.01 to 3 eV), of unsubstituted and 40% Zn substituted for Co, for the transition-metal phosphorus trichalcogenide, C⁢o 2 ⁢P 2 ⁢S 6 . We observe a transition from a paramagnetic to antiferromagnetic state with a Néel temperature at T N ~ 120 K that is completely suppressed in Zn-substituted samples. At 300 K we identify four narrow (~ 1 meV) infrared active phonon modes while at 70 K (below T N ) we observe that the low-energy phonons, dominated by Co motion, resolve into two modes. These low-energy modes are asymmetric, indicating coupling to a broad electronic continuum. We also report a broad (~ 30 meV) low-temperature infrared absorption band that appears near T N that we suggest is determined by a multiphonon-assisted 2-magnon absorption process. At 300 K in higher-energy spectra, we observe considerable absorption starting from 0.20 ± 0.02 eV which we associate with inter-C⁢o 2+ ion 3⁢d transitions. At temperatures below T N the number of electronic absorption bands increases from 4 to 6, indicating a lowering of the symmetry around the C⁢o 2+ ions. On substituting 40% Zn for Co, the antiferromagnetic transition is suppressed along with temperature-dependent changes in the phonon and electronic spectra. The temperature-dependent spectral changes indicate strongly correlated behavior between the infrared active lattice vibrations, the electronic excitations, and magnetism in unsubstituted C⁢o 2 ⁢P 2 ⁢S 6 .

2-dimensional systems↗

Quantifying magnetic field driven lattice distortions in kagome metals at the femto-scale using scanning tunneling microscopy

A wide array of unusual phenomena has recently been uncovered in kagome solids. The charge density wave (CDW) state in the kagome superconductor AV 3 Sb 5 , in particular, intrigued the community; the CDW phase appears to break the time-reversal symmetry despite the absence of spin magnetism, which has been tied to exotic orbital loop currents possibly intertwined with magnetic field tunable crystal distortions. To test this connection, precise determination of the lattice response to an applied magnetic field is crucial but can be challenging at the atomic scale. We establish a scanning tunneling microscopy (STM) based method to study the evolution of the AV 3 Sb 5 atomic structure as a function of magnetic field. The method substantially reduces the errors of typical STM measurements, which are at the order of 1% when measuring an in-plane lattice constant change. Here, we find that the out-of-plane lattice constant of AV 3 Sb 5 remains unchanged (within 10 —6 ) by the application of both in-plane and out-of-plane magnetic fields. We also reveal that the in-plane lattice response to magnetic field is at most at the order of 0.05%. Our experiments provide further constraints on time-reversal symmetry breaking in kagome metals and establish a tool for higher-resolution extraction of the field-lattice coupling at the nanoscale applicable to other quantum materials.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗