Instability of a Mechanical System Induced by an Impinging Fluid Jet
Theoretical and experimental determination of critical loading by impinging fluid jet and instability of mechanical system
Feldt, W. T.↗
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Stereo Imaging Velocimetry of Mixing Driven by Buoyancy Induced Flow Fields
Mixing of two fluids generated by steady and particularly g-jitter acceleration is fundamental towards the understanding of transport phenomena in a microgravity environment. We propose to carry out flight and ground-based experiments to quantify flow fields due to g-jitter type of accelerations using Stereo Imaging Velocimetry (SIV), and measure the concentration field using laser fluorescence. The understanding of the effects of g-jitter on transport phenomena is of great practical interest to the microgravity community and impacts the design of experiments for the Space Shuttle as well as the International Space Station. The aim of our proposed research is to provide quantitative data to the community on the effects of g-jitter on flow fields due to mixing induced by buoyancy forces. The fundamental phenomenon of mixing occurs in a broad range of materials processing encompassing the growth of opto-electronic materials and semiconductors, (by directional freezing and physical vapor transport), to solution and protein crystal growth. In materials processing of these systems, crystal homogeneity, which is affected by the solutal field distribution, is one of the major issues. The understanding of fluid mixing driven by buoyancy forces, besides its importance as a topic in fundamental science, can contribute towards the understanding of how solutal fields behave under various body forces. The body forces of interest are steady acceleration and g-jitter acceleration as in a Space Shuttle environment or the International Space Station. Since control of the body force is important, the flight experiment will be carried out on a tunable microgravity vibration isolation mount, which will permit us to precisely input the desired forcing function to simulate a range of body forces. To that end, we propose to design a flight experiment that can only be carried out under microgravity conditions to fully exploit the effects of various body forces on fluid mixing. Recent flight experiments, by the P.I. through collaboration with the Canadian Space Agency (STS-85, August 1997), aimed at determining the stability of the interface between two miscible liquids inside an enclosure show that a long liquid column (5 cm) under microgravity isolation conditions can be stable, i.e. the interface remains sharp and vertical over a short time scale; thus transport occurs by molecular mass diffusion. On the other hand, when the two liquids were excited from a controlled vibration source (Microgravity Vibration Isolation Mount) two to four mode large amplitude quasi-stationary waves were observed. The data was limited to CCD recording of the dynamics of the interface between the two fluids. We propose to carry out flight experiments to quantify the dynamics of the flow field using Stereo Imaging Velocimetry and measure the concentration field using laser fluorescence. The results will serve as a basis to understand effects of g-jitter on transport phenomena, in this case mass diffusion. As the measurement of the kinematics of the flow field will shed light on the instability mechanism. The research will allow measurement of the flow field in microgravity environment to prove two hypotheses: (1) Maxwell's hypothesis: finite convection always exists in diffusing systems, and (2) Quasi-stationary waves inside a bounded enclosure in a microgravity environment is generated by Kelvin-Helmholtz instability; resonance of the interface which produces incipient mixing is due to Rayleigh-Taylor instability. The first hypothesis can be used as a benchmark experiment to illustrate diffusive mixing. The second hypothesis will lead to the understanding of g-jitter effects on buoyancy driven flow fields which occur in many situations involving materials processing, and other basic fluid physics phenomena. In addition, the second hypothesis will also provide insight in how Rayleigh-Taylor and Kelvin-Helmholtz instabilities propagate concentration fronts during mixing. Measurement of the flow field using SIV is important because it is the flow field which causes instability at the interface between the two fluids. Mixing driven by buoyancy induced flow fields will be addressed both experimentally and computationally. The experimental effort will address the kinematics of mixing: stretching, transport and chaos. Quantification of the mechanisms of mixing will consists of measuring the flow field using the SIV system at Glenn and capturing the dynamics of the interface, to measure mass transport, using a CCD camera. These experiments will be carried out within the framework of Earth's gravity and g-jitter microgravity acceleration as in a Space Shuttle environment or the International Space Station. The g-jitter will be induced and controlled using a tunable vibration isolation platform to isolate against vibration as well as input periodic and random vibration to the system. The parametric range of the microgravity experiment will be extended from the experiments on STS-85 to investigate higher mode quasi-stationary waves (8 to 12), as well as resonance regions which leads to chaos and turbulence. Ground-based experiments will focus on effects of vibration on stably stratified fluid layers in order to scale for possible scenarios in a microgravity environment. These vibrations will be subjected perpendicular to the concentration field on the ground since the parallel case can only be carried out in a microgravity environment. The concept of dynamical similarity will be applied to tune the experiments as closely as possible to a Space Shuttle environment or the International Space Station. The computational effort will take advantage of the Computational Laboratory at Glenn to corroborate the experimental findings with predictions of the dynamics of the flow field using the codes FLUENT (finite difference based) and FIDAP (finite element based). We will investigate two important cases, single-fluid model to address dilute systems with negligible jump in viscosity and the more general two-fluid model which accounts for finite jump in viscosity. Apart from its microgravity relevance, this experiment is well suited to study dynamics in nonlinear systems.
Duval, W. M. B.↗
Evaluating Stage Motion for Automated Electron Microscopy
Abstract Precise control is an essential and elusive quality of emerging self-driving transmission electron microscopes (TEMs). It is widely understood these instruments must be capable of performing rapid, high-volume, and arbitrary movements for practical self-driving operation. However, stage movements are difficult to automate at scale, owing to mechanical instability, hysteresis, and thermal drift. Such difficulties pose major barriers to artificial intelligence-directed microscope designs that require repeatable, precise movements. To guide design of emerging instruments, it is necessary to understand the behavior of existing mechanisms to identify rate limiting steps for full autonomy. Here, we describe a general framework to evaluate stage motion in any TEM. We define metrics to evaluate stage degrees of freedom, propose solutions to improve performance, and comment on fundamental limits to automated experimentation using present hardware.
47 OTHER INSTRUMENTATION↗
Nonlinear deformation and elasticity of BCC refractory metals and alloys
Application of isotropic pressure or uniaxial strain alters the elastic properties of materials; sufficiently large strains can drive structural transformations. Linear elasticity describes stability against infinitesimal strains, while nonlinear elasticity describes the response to finite deformations. Here, it was previously shown that uniaxial strain along [100] drives refractory metals and alloys towards mechanical instabilities. These include an extensional instability, and a symmetry-breaking orthorhombic distortion caused by a Jahn-Teller-Peierls instability that splays the cubic lattice vectors. Here we analyze these transitions in depth. Eigenvalues and eigenvectors of the Wallace tensor identify and classify linear instabilities in the presence of strain. We show that both instabilities are discontinuous, leading to discrete jumps in the lattice parameters. We provide physical intuition for the instabilities by analyzing the changes in first-principles energy, stress, bond lengths, and angles upon application of strain. Electronic band structure calculations show differential occupation of bonding and antibonding orbitals, driven by the changing bond lengths and leading to the structural transformations. Strain thresholds for these instabilities depend on the valence electron count.
36 MATERIALS SCIENCE↗
Formation of the outer planets and satellites
A mechanism for the formation of the outer planets is proposed, the basis of which is the idea that the giant planets contain an excess of chemically condensable materials over solar composition. Planetary cores were formed by the clumping together of chemically condensed bodies forming a thin disk in the solar nebula. Gas surrounding a core becomes unstable against collapse onto the core. In the case of Jupiter and Saturn, much of the collapsing gas goes into orbit about the formed planet, forming a relatively thin circumplanetary disks with differential rotation in the prograde sense. For Uranus and Neptune, the dynamical collapse mechanism is unlikely. A disk of gas around Uranus may have been formed during a collision of the protoplanet with a large body. The circumplanetary disks then form the basis for formation of satellite systems, in which the Goldreich-Ward instability mechanism plays a role.
Cameron, A. G. W.↗
Full-Scale Direct Numerical Simulation of Two- and Three-Dimensional Instabilities and Rivulet Formulation in Heated Falling Films
A thin film draining on an inclined plate has been studied numerically using finite element method. Three-dimensional governing equations of continuity, momentum and energy with a moving boundary are integrated in an arbitrary Lagrangian Eulerian frame of reference. Kinematic equation is solved to precisely update interface location. Rivulet formation based on instability mechanism has been simulated using full-scale computation. Comparisons with long-wave theory are made to validate the numerical scheme. Detailed analysis of two- and three-dimensional nonlinear wave formation and spontaneous rupture forming rivulets under the influence of combined thermocapillary and surface-wave instabilities is performed.
Krishnamoorthy, S.↗
Chemo‐Mechanical Coupling in Hydrogels: Dynamics in the Diffusion‐Limited Regime
Hydrogels are characterized by substantial volume changes in response to external stimuli, making them promising candidates for developing smart materials with enhanced adaptability and responsiveness. By integrating chemical reactions, hydrogels acquire dynamic and tunable responsiveness to external stimuli through chemo‐mechanical coupling, expanding their potential in emerging applications. However, capturing their transient behavior remains challenging due to the complex interplay of chemical reactions, solvent transport, and polymer network deformation. Classical theories capture equilibrium swelling but fail to describe time‐dependent phenomena. To address this, a time‐dependent continuum model is developed that explicitly couples these processes. Volume phase transition in hydrogels with homogeneous chemical reactions is investigated, then the effects of reaction kinetics on these transitions are analyzed. The coupling of these mechanisms is further explored through a study of transient mechanical instabilities. To illustrate the impact of distinct reaction and diffusion timescales, a photo‐active gripper is studied for robotic applications. Finally, a photo‐active microswimmer that exhibits non‐reciprocal motion is proposed to highlight the solvent diffusion for locomotion at the micro‐ and nano‐ scales. The work establishes that transient dynamics of chemo‐mechanical hydrogels generate functions not accessible by steady state models and provides a predictive platform for designing adaptive materials in emerging applications.
chemo-mechanical coupling↗
Effect of inlet throttling on thermohydraulic instability in a large scale water-based RCCS: An experimental study
The objective of the present experimental study is to investigate the effect of inlet throttling on the thermohydraulic stability of a large scale water-based Reactor Cavity Cooling System (RCCS). The test was performed using the water-based Natural convection Shutdown heat removal Test Facility (NSTF) at Argonne, which represented a ½ axial scale and 12.5° sector slice of the full scale Framatome 625 MW t SC-HTGR RCCS concept. A two-phase steady state was first established through direct condensate refill, followed by increased inlet throttling over 10 stages, corresponding to a loss coefficient K over the range of 0.05–653. With the inlet throttling gradually increased, the system experienced a unique transition process between stabilization and destabilization. Through a stability analysis, three instability mechanisms were identified in the present test, including a compound mechanism due to both natural circulation oscillations (NCOs) and density wave oscillations (DWOs), Type-II DWOs, and geysering.
22 GENERAL STUDIES OF NUCLEAR REACTORS↗
A04-0491 - Reduced Electrolyte Reactivity of Pitch-Carbon Coated Si Nanoparticles for Li-Ion Battery Anodes
Silicon-based anodes for Li-ion batteries (LIB) have the potential to increase the energy density over graphite-based LIB anodes. However, silicon anodes exhibit poor cycle and calendar lifetimes due to mechanical instabilities and high chemical reactivity with the carbonate-based electrolytes that are typically used in LIBs. In this work, we synthesize a pitch-carbon coated silicon nanoparticle composite active material for LIB anodes that exhibits reduced chemical reactivity with the carbonate electrolyte compared to an uncoated silicon anode. Silicon primary particle sizes <10 nm minimize micro-scale mechanical degradation of the anode composite, while conformal coatings of pitch-carbon minimized the parasitic reactions between the silicon and the electrolyte. When matched with a high voltage NMC622 cathode, the pitch-carbon coated Si anode retains -75% of its initial capacity over 1000 cycles. Efforts to increase the areal loading of the pitch-carbon coated silicon anodes to realize real energy density improvements over graphite anodes results in severe mechanical degradation on the electrode level. Developing procedures to engineer the architecture of the composite silicon anode may be a solution to this mechanical challenge.
DIRECT ENERGY CONVERSION,ENERGY STORAGE↗
Pitch Carbon-coated Ultrasmall Si Nanoparticle Lithium-ion Battery Anodes Exhibiting Reduced Reactivity with Carbonate-based Electrolyte
Silicon anodes for lithium-ion batteries (LIBs) have the potential for higher energy density compared to conventionally used graphite-based LIB anodes. However, silicon anodes exhibit poor cycle and calendar lifetimes due to mechanical instabilities and high chemical and electrochemical reactivity with the carbonate-based electrolytes that are typically used in LIBs. In this work, we synthesize a pitch carbon-coated silicon nanoparticle composite active material for LIB anodes that exhibits reduced chemical reactivity with carbonate-based electrolytes compared to an uncoated silicon anode. Silicon primary particle sizes less than 10 nm diameter minimize micro-scale mechanical degradation of the anode composite, while conformal coatings of pitch carbon minimize the parasitic reactions between the silicon and the electrolyte. When matched with a high voltage NMC622 (LiNi 0.6 Mn 0.2 Co 0.2 O 2 ) cathode, the pitch carbon-coated silicon anode retains approximately 75% of its initial capacity at the end of 1000 cycles. Increasing the areal loading of the pitch carbon-coated silicon anodes to realize energy density improvements over graphite anodes results in severe mechanical degradation on the electrode level, highlighting a remaining challenge to be addressed in future work.
25 ENERGY STORAGE↗
Numerical investigation of the influence of shear and thermal stratification on the wind turbine tip‐vortex stability
Summary The interaction between wind turbine wakes and atmospheric turbulence is characterised by complex dynamics. In this study, two major components of the atmospheric boundary layer dynamics have been isolated, namely, the mean velocity profile shear and the thermal stratification, to examine their impact on the near‐wake development by undertaking a series of highly resolved large‐eddy simulations. Subsequently, instantaneous flow fields are extracted from the simulations and used to conduct Fourier analysis and proper orthogonal decomposition (POD) and compute the mean kinetic energy fluxes by different POD modes to better understand the tip‐vortex instability mechanisms. Our findings indicate that shear can significantly affect the breakup of the wind turbine tip‐vortices and the shape and stable length of the wake, whereas thermal stratification seems to only have limited contribution to the spatial development of the near‐wake field. Finally, our analysis shows that the applied perturbation frequency determines the tip‐vortex breakup location as it controls the onset of the mutual inductance instability.
17 WIND ENERGY↗
Secondary instabilities in compressible boundary layers
The secondary instability mechanisms in a two-dimensional (2-D) compressible boundary layer over a flat plate have been examined for a range of Mach numbers up to 4.5. For subsonic and low supersonic flows, fundamental resonance dominates when the amplitude of the (2-D) primary disturbance is high, while subharmonic resonance prevails in an environment with a low primary disturbance. At a high supersonic Mach number of 4.5, the secondary instability of the second-mode primary is stronger than that of the first-mode primary. Further, the subharmonic and the combination resonance modes, which are slightly detuned from the subharmonic, are the dominant instabilities. The influence of the propagation direction of the primary disturbance on secondary instabilities is investigated at Mach 1.6. Whereas the fundamental and the subharmonic disturbances propagate synchronously with a 2-D primary wave, this is not true for an oblique primary. A subset of the secondary instability results is verified against direct numerical simulations. Some comparisons between spatial and temporal secondary instabilities have been made at Mach 1.6.
Ng, Lian L.↗
Transition Analysis for the CRM-NLF Wind Tunnel Configuration using Transport Equation Models and Linear Stability Correlations
Transition models based on auxiliary transport equations augmenting the Reynolds-averaged Navier-Stokes (RANS) framework rely upon transition correlations that were derived from a limited number of low-speed experiments. Furthermore, these models often account for only a subset of the relevant transition mechanisms and/or cannot accurately predict the sensitivity of those mechanisms to the changes in significant flow parameters. A preceding investigation had targeted the assessment of the transport-equation-based transition models in NASA's OVERFLOW 2.3b solver, namely, the amplification factor transport (AFT-2017b) equation model coupled with the Spalart-Allmaras RANS model and the Langtry-Menter transition models (LM2009 without crossflow effects and LM2015 including the modeling of crossflow transition) implemented with Menter’s shear-stress transport equation (SST2003) RANS model. Comparisons with recent measurements at transonic freestream conditions on the Common Research Model with Natural Laminar Flow (CRM-NLF) reinforced our earlier finding that all three of the above models significantly underpredict the reported extent of the laminar flow region over the entire span of the wing, regardless of the dominant instability mechanism(s) underlying the onset of the transition process. The underprediction of the laminar flow extent was attributed to the failure of the above models in accounting for the stabilizing effect of compressibility on the amplification of Tollmien-Schlichting instabilities. Based on previous linear stability studies related to compressibility effects, the present work proposes modifications to the two classes of transition models that reduce to the original form of each model at low subsonic speeds and do not require any nonlocal flow information or additional transport equation(s). The modifications are shown to significantly improve the predicted laminar extent of the flow and compare well against the data from the CRM-NLF experiment. Additionally, a previous assessment of transition prediction based on the dual, nonparallel N -factor method in conjunction with linear parabolized stability equations (PSE) is extended to additional angles of attack to provide the first comprehensive assessment of transition models based on nonparallel disturbance amplification over the CRM-NLF. In general, the transition criterion based on the dual, nonparallel N-factor method with N TS = N CF = 6 is reasonably successful at correlating with the measured transition fronts at R eMAC = 15 million for all angles of attack investigated herein and provides additional validation of the improved predictions from the compressibility-corrected transition models.
CFD modeling↗
Transition Analysis for the CRM-NLF Wind Tunnel Configuration using Transport Equation Models and Linear Stability Correlations
Transition models based on auxiliary transport equations augmenting the Reynolds-averaged Navier-Stokes (RANS) framework rely upon transition correlations that were derived from a limited number of low-speed experiments. Furthermore, these models often account for only a subset of the relevant transition mechanisms and/or cannot accurately predict the sensitivity of those mechanisms to the changes in significant flow parameters. A preceding investigation had targeted the assessment of the transport-equation-based transition models in NASA's OVERFLOW 2.3b solver, namely, the amplification factor transport (AFT-2017b) equation model coupled with the Spalart-Allmaras RANS model and the Langtry-Menter transition models (LM2009 without crossflow effects and LM2015 including the modeling of crossflow transition) implemented with Menter’s shear-stress transport equation (SST2003) RANS model. Comparisons with recent measurements at transonic freestream conditions on the Common Research Model with Natural Laminar Flow (CRM-NLF) reinforced our earlier finding that all three of the above models significantly underpredict the reported extent of the laminar flow region over the entire span of the wing, regardless of the dominant instability mechanism(s) underlying the onset of the transition process. The underprediction of the laminar flow extent was attributed to the failure of the above models in accounting for the stabilizing effect of compressibility on the amplification of Tollmien-Schlichting instabilities. Based on previous linear stability studies related to compressibility effects, the present work proposes modifications to the two classes of transition models that reduce to the original form of each model at low subsonic speeds and do not require any nonlocal flow information or additional transport equation(s). The modifications are shown to significantly improve the predicted laminar extent of the flow and compare well against the data from the CRM-NLF experiment. Additionally, a previous assessment of transition prediction based on the dual, nonparallel N -factor method in conjunction with linear parabolized stability equations (PSE) is extended to additional angles of attack to provide the first comprehensive assessment of transition models based on nonparallel disturbance amplification over the CRM-NLF. In general, the transition criterion based on the dual, nonparallel N-factor method with N TS = N CF = 6 is reasonably successful at correlating with the measured transition fronts at R eMAC = 15 million for all angles of attack investigated herein and provides additional validation of the improved predictions from the compressibility-corrected transition models.
CFD modeling↗
Elucidating the Link Between Alkali Metal Ions and Reaction-Transport Mechanisms in Cathode Electrodes for Alkali-ion Batteries
Our long-term goal is to improve the reliability of electrode materials and their ability to transport and store various metal ions for electrochemical energy storage applications. The main objective of this work was to investigate the intrinsic relationship between the role of alkali metal ions and electrochemically driven mechanical stability and kinetic properties of battery materials. The overall question was “What is the role of alkali metal ions on the electrochemical and mechanical behavior of cathode electrodes? Our guiding hypothesis was that intercalation of larger alkali metal ions (Na and K) inevitably alters the coupled transport-reaction processes during battery operation in organic electrolytes, leading to more intensive chemo-mechanical instabilities in cathode electrodes, resulting in rapid capacity fade. To validate the hypothesis, we experimentally characterized the reaction-transport processes and governing forces driving the instability of electrode materials in different alkali metal-ion environments. The project had three main tasks. The first one was to investigate intercalation-induced strains and associated stress generation, and their impact on structural deformations in composite cathode electrodes. The second task focused on identifying potential-dependent dynamic changes in the electrode-electrolyte interface in alkali metal ion batteries. The last task was focused on determining how larger alkali metal ions with slower diffusivity affect the transport-mechanics coupling at faster scan rates, compared to smaller ions with faster diffusivity in electrodes. We shortly provided the outcome of each task in the accomplishment section. This project produced 10 peer-reviewed publications (9 research papers and one review manuscript) and supported two Ph.D. students, who graduated from Oklahoma State University.
25 ENERGY STORAGE↗
Diffusion Flame Tip Instabilities of a Wide Sample in Microgravity
This work is a study of diffusion flame tip instabilities of a wide thermally thin sample in a microgravity environment. The purpose of this work is to determine the thermodiffusive and hydrodynamic instability mechanisms which cause a spreading diffusion flame to become corrugated and later fragment into smaller separate flames that we call flamelets. These thermodiffusive and hydrodynamic mechanisms are prominent forces in the near limit because buoyancy is quashed in the microgravity environment. A fundamental knowledge of the underlying mechanisms controlling the extinction limit of a diffusion flame can be applied to any real world device involving a spreading diffusion flame as well as fire safety applications on earth and in space. Our work, which combines microgravity experiments, theoretical models, and numerical computation, is a joint effort between NASA and Michigan State University. Experiments in the 2.2 second drop tower at NASA Lewis Research Center in the Microgravity Combustion Branch have been a preliminary step in locating a region where these instabilities are prevalent. These positive results will be discussed as well as the second phase of our project and future plans and recommendations.
Oravecz, Lisa↗
Boundary Layer Transition over Blunt Hypersonic Vehicles Including Effects of Ablation-Induced Out-Gassing
Computations are performed to study the boundary layer instability mechanisms pertaining to hypersonic flow over blunt capsules. For capsules with ablative heat shields, transition may be influenced both by out-gassing associated with surface pyrolysis and the resulting modification of surface geometry including the formation of micro-roughness. To isolate the effects of out-gassing, this paper examines the stability of canonical boundary layer flows over a smooth surface in the presence of gas injection into the boundary layer. For a slender cone, the effects of out-gassing on the predominantly second mode instability are found to be stabilizing. In contrast, for a blunt capsule flow dominated by first mode instability, out-gassing is shown to be destabilizing. Analogous destabilizing effects of outgassing are also noted for both stationary and traveling modes of crossflow instability over a blunt sphere-cone configuration at angle of attack.
Li, Fei↗