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Satellite Remote Sensing of Tropical Precipitation and Ice Clouds for GCM Verification

This project, supported by the NASA New Investigator Program, has primarily been funding a graduate student, Darren McKague. Since August 1999 Darren has been working part time at Raytheon, while continuing his PhD research. Darren is planning to finish his thesis work in May 2001, thus some of the work described here is ongoing. The proposed research was to use GOES visible and infrared imager data and SSM/I microwave data to obtain joint distributions of cirrus cloud ice mass and precipitation for a study region in the Eastern Tropical Pacific. These joint distributions of cirrus cloud and rainfall were to be compared to those from the CSU general circulation model to evaluate the cloud microphysical amd cumulus parameterizations in the GCM. Existing algorithms were to be used for the retrieval of cloud ice water path from GOES (Minnis) and rainfall from SSM/I (Wilheit). A theoretical study using radiative transfer models and realistic variations in cloud and precipitation profiles was to be used to estimate the retrieval errors. Due to the unavailability of the GOES satellite cloud retrieval algorithm from Dr. Minnis (a co-PI), there was a change in the approach and emphasis of the project. The new approach was to develop a completely new type of remote sensing algorithm - one to directly retrieve joint probability density functions (pdf's) of cloud properties from multi-dimensional histograms of satellite radiances. The usual approach is to retrieve individual pixels of variables (i.e. cloud optical depth), and then aggregate the information. Only statistical information is actually needed, however, and so a more direct method is desirable. We developed forward radiative transfer models for the SSM/I and GOES channels, originally for testing the retrieval algorithms. The visible and near infrared ice scattering information is obtained from geometric ray tracing of fractal ice crystals (Andreas Macke), while the mid-infrared and microwave scattering is computed with Mie scattering. The radiative transfer is performed with the Spherical Harmonic Discrete Ordinate Method (developed by the PI), and infrared molecular absorption is included with the correlated k-distribution method. The SHDOM radiances have been validated by comparison to version 2 of DISORT (the community "standard" discrete-ordinates radiative transfer model), however we use SHDOM since it is computationally more efficient.

Evans, K. Franklin↗

Tropical Oceanic Precipitation Processes Over Warm Pool: 2D and 3D Cloud Resolving Model Simulations

Rainfall is a key link in the hydrologic cycle as well as the primary heat source for the atmosphere. The vertical distribution of convective latent-heat release modulates the large-scale circulations of the topics. Furthermore, changes in the moisture distribution at middle and upper levels of the troposphere can affect cloud distributions and cloud liquid water and ice contents. How the incoming solar and outgoing longwave radiation respond to these changes in clouds is a major factor in assessing climate change. Present large-scale weather and climate model simulate processes only crudely, reducing confidence in their predictions on both global and regional scales. One of the most promising methods to test physical parameterizations used in General Circulation Models (GCMs) and climate models is to use field observations together with Cloud Resolving Models (CRMs). The CRMs use more sophisticated and physically realistic parameterizations of cloud microphysical processes, and allow for their complex interactions with solar and infrared radiative transfer processes. The CRMs can reasonably well resolve the evolution, structure, and life cycles of individual clouds and clouds systems. The major objective of this paper is to investigate the latent heating, moisture and momentum budgets associated with several convective systems developed during the TOGA COARE IFA - westerly wind burst event (late December, 1992). The tool for this study is the Goddard Cumulus Ensemble (GCE) model which includes a 3-class ice-phase microphysics scheme.

Tao, W.-K.↗

Mesoscale Convective Systems During SCSMEX: Simulations with a Regional Climate Model and a Cloud-Resolving Model

The South China Sea Monsoon Experiment (SCSMEX) was conducted in May-June 1998. One of its major objectives is to better understand the key physical processes for the onset and evolution of the summer monsoon over Southeast Asia and southern China (Lau et al. 2000). Multiple observation platforms (e.g., soundings, Doppler radar, ships, wind seafarers, radiometers, etc.) during SCSMEX provided a first attempt at investigating the detailed characteristics of convection and circulation changes, associated with monsoons over the South China Sea region. SCSMEX also provided precipitation derived from atmospheric budgets (Johnson and Ciesielski 2002) and comparison to those obtained from the Tropical Rainfall Measuring Mission (TRMM). In this paper, a regional climate model and a cloud-resolving model are used to perform multi-day integrations to understand the precipitation processes associated with the summer monsoon over Southeast Asia and southern China. The regional climate model is used to understand the soil - precipitation interaction and feedback associated with a flood event that occurred in and around China's Atlantic River during SCSMEX. Sensitivity tests on various land surface models, cumulus parameterization schemes (CASE), sea surface temperature (SST) variations and midlatitude influences are also performed to understand the processes associated with the onset of the monsoon over the S. China Sea during SCSMEX. Cloud-resolving models (CRMs) use more sophisticated and physically realistic parameterizations of cloud microphysical processes with very fine spatial and temporal resolution. One of the major characteristics of CRMs is an explicit interaction between clouds, radiation and the land/ocean surface. It is for this reason that GEWEX (Global Energy and Water Cycle Experiment) has formed the GCSS (GEWEX Cloud System Study) expressly for the purpose of improving the representation of the moist processes in large-scale models using CRMs. The Goddard Cumulus Ensemble (GCE) model is a CRM and is used to simulate convective systems associated with the onset of the South China Sea monsoon in 1998. The BRUCE model includes the same land surface model, cloud physics, and radiation scheme used in the regional climate model. A comparison between the results from the GCE model and regional climate model is performed.

Tao, W. K.↗

Diurnal Variation of Precipitation During MC3E Campaign

The diurnal variation of precipitation processes in the United States (US) is well recognized but incompletely understood (Cabone et al. 2002). The diurnal cycle of precipitation has been studied using surface rainfall data, radar reflectivity data, and satellite-derived cloudiness and precipitation (Wallace 1975; Dai et al. 1999; Carbone et al. 2002; Carbone and Tuttle, 2008; Parker and Ahijevych, 2007; Matsui et al. 2010 and others). These observations indicate that the summer-time precipitation most of the North America and typically feature late-afternoon precipitation maxima. These diurnal variation of precipitation can also be generally categorized into three different types: 1) afternoon rainfall maxima due to mesoscale and local circulations over the south and east of the Mississippi and Ohio valleys, 2) nocturnal rainfall maxima from eastward-propagating mesoscale convective systems (MCSs) over the Lee side of Rocky Mountain regions and 3) afternoon rainfall maxima in the Appalachian Mountains, and then propagate eastward toward the coast. The main objective of this paper is to use a regional cloud-scale model with very high-resolution (i.e., WRF) to examine the WRF ability to simulate diurnal variation of precipitation. Specifically, the study will (1) identify the physical processes responsible to diurnal variation of precipitation, (2) examine the sensitivity of resolution (2, 6, 18, and 30 km) to model simulated diurnal variation of precipitation and (3) identify the relationships between microphysics and cumulus parameterization schemes.

Tao, Wei-Kuo↗

Evaluation of Model Microphysics Within Precipitation Bands of Extratropical Cyclones

It is hypothesized microphysical predictions have greater uncertainties/errors when there are complex interactions that result from mixed phased processes like riming. Use Global Precipitation Measurement (GPM) Mission ground validation studies in Ontario, Canada to verify and improve parameterizations. The WRF realistically simulated the warm frontal snowband at relatively short lead times (1014 h). The snowband structire is sensitive to the microphysical parameterization used in WRF. The Goddard and SBUYLin most realistically predicted the band structure, but overpredicted snow content. The double moment Morrison scheme best produced the slope of the snow distribution, but it underpredicted the intercept. All schemes and the radar derived (which used dry snow ZR) underpredicted the surface precipitation amount, likely because there was more cloud water than expected. The Morrison had the most cloud water and the best precipitation prediction of all schemes.

Colle, Brian A.↗

Differences in Lightning—Storm Microphysical Relationships in Subtropical South America Versus the Continental U.S. and Their Impact on Model Lightning Parameterizations

Satellite studies have shown that some of the deepest convection with high lightning flash rates occurs downstream of the Andes in subtropical South America (SSA). Using high resolution ground‐based observations in SSA, we explore the relationship between lightning and radar‐inferred storm microphysics. Results show these storms have significantly larger 35‐dBZ volumes and more graupel per lightning flash compared to storms in the U.S. We then test microphysics‐based lightning parameterizations for storms in SSA on a 1‐km convection‐permitting simulation of a mesoscale convective system. Results from the simulation match well with observed flash rates. If parameterizations based on U.S. storms had been applied, flash rates would have been overestimated by a factor of eight. These results suggest that storms in SSA are fundamentally different compared to storms in the U.S., and caution should be exercised when applying microphysics‐based lightning parameterizations in different regions of the world.

54 ENVIRONMENTAL SCIENCES↗

Parameterizations of Depositional Growth of Cloud Ice in a Bulk Microphysical Scheme

The conversion of cloud ice to snow by depositional growth, designated P(sub SFI), in the Goddard Cumulus Ensemble Model cloud physics parameterization is examined. The original formulation of P(sub SFI) is shown to produce excessive conversion of cloud ice to snow because of an implicit assumption that the relative humidity is 100% with respect to water even though the air may actually be quite less humid. Two possible corrections to this problem are proposed, the first involving application of a relative humidity dependent correction factor to the original formulation of P(sub SFI), and the second involving a new formulation of P(sub SFI) based on the equation for depositional growth of cloud ice.

Braun, Scott A.↗

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-Resolving Model Simulations

Cloud microphysics are inevitably affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds. Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effects of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates for convective clouds. Recently, two detailed spectral-bin microphysical schemes were implemented into the Goddard Cumulus Ensemble (GCE) model. The formulation for the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e.,pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail]. Each type is described by a special size distribution function containing many categories (i.e. 33 bins). Atmospheric aerosols are also described using number density size-distribution functions.A spectral-bin microphysical model is very expensive from a from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep tropical clouds in the west Pacific warm pool region using identical thermodynamic conditions but with different concentrations of CCN: a low "clean" concentration and a high "dirty" concentration. Besides the initial differences in aerosol concentration, preliminary results indicate that the low CCN concentration case produces rainfall at the surface sooner than the high CCN case but has less cloud water mass aloft. Because the spectral-bin model explicitly calculates and allows for the examination of both the mass and number concentration of species in each size categor, a detailed analysis of the instantaneous size spectrum can be obtained for the two cases. It is shown that since the low CCN case produces fewer droplets, larger sized develop due to the greater condensational and collectional growth, leading to a broader size spectrum in comparison to the high CCN case.

Tao, Wei-Kuo↗

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-Resolving Model Simulations

Cloud microphysics are inevitable affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds. Therefore, size distribution parameterized as spectral bin microphysics are needed to explicitly study the effect of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates convective clouds. Recently, two detailed spectral-bin microphysical schemes were implemented into the Goddard Cumulus Ensembel (GCE) model. The formulation for the explicit spectral-bim microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e., pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), groupel and frozen drops/hall] Each type is described by a special size distribution function containing many categories (i.e., 33 bins). Atmospheric aerosols are also described using number density size-distribution functions.A spectral-bin microphysical model is very expensive from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep cloud systems in the west Pacific warm pool region and in the mid-latitude using identical thermodynamic conditions but with different concentrations of CCN: a low "clean" concentration and a high "dirty" concentration. Besides the initial differences in aerosol concentration, preliminary results indicate that the low CCN concentration case produces rainfall at the surface sooner than the high CCN case but has less cloud water mass aloft. Because the spectral-bim model explicitly calculates and allows for the examination of both the mass and number concentration of cpecies in each size category, a detailed analysis of the instantaneous size spectrum can be obtained for the two cases. It is shown that since the low CCN case produces fever droplets, larger size develop due to greater condencational and collectional growth, leading to a broader size spectrum in comparison to the high CCN case.

Tao, Wei-Kuo↗

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-resolving Model Simulations

Cloud microphysics is inevitably affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds. Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effects of atmospheric aerosol concentration on cloud development, r d a U production, and rainfall rates for convective clouds. Recently, two detailed spectral-bin microphysical schemes were implemented into the Goddard Cumulus Ensembe1 (GCE) model. The formulation for the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e. pristine ice crystals (columnar and platelike), snow (dendrites and aggregates), graupel and frozen drops/hail]. Each type is described by a special size distribution function containing many categories (i.e. 33 bins). Atmospheric aerosols are also described using number density size-distribution functions. A spectral-bin microphysical model is very expensive from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep tropical clouds in the west Pacific warm pool region and in the mid-latitude continent with different concentrations of CCN: a low "c1ean"concentration and a high "dirty" concentration. In addition, differences and similarities between bulk microphysics and spectral-bin microphysical schemes will be examined and discussed.

Tao, Wei-Kuo↗

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-Resolving Model Simulations

Cloud microphysics is inevitably affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds. Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effects of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates for convective clouds. Recently, two detailed spectral-bin microphysical schemes were implemented into the Goddard Cumulus Ensembel (GCE) model. The formulation for the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e. pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail]. Each type is described by a special size distribution function containing many categories (i.e. 33 bins). Atmospheric aerosols are also described using number density size distribution functions. A spectral-bin microphysical model is very expensive from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep tropical clouds in the west Pacific warm pool region and in the mid-latitude continent with different concentrations of CCN: a low "c1ean"concentration and a high "dirty" concentration. In addition, differences and similarities between bulk microphysics and spectral-bin microphysical schemes will be examined and discussed.

Tao, Wei-Kuo↗

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-Resolving Model Simulations

Cloud microphysics are inevitably affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds. Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effects of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates for convective clouds. Recently, two detailed spectral-bin microphysical schemes were implemented into the Goddard Cumulus Ensemble (GCE) model. The formulation for the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles (i.e., pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail). Each type is described by a special size distribution function containing many categories (i.e. 33 bins). Atmospheric aerosols are also described using number density size-distribution functions. A spectral-bin microphysical model is very expensive from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep cloud systems in the west Pacific warm pool region, in the sub-tropics (Florida) and in the mid-latitude using identical thermodynamic conditions but with different concentrations of CCN: a low 'clean' concentration and a high 'dirty' concentration.

Tao, Wei-Kuo↗

The Impact of Aerosols on Cloud and Precipitation Processes: Cloud-Resolving Model Simulations

Cloud microphysics are inevitable affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds, Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effect of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates for convective clouds. Recently, a detailed spectral-bin microphysical scheme was implemented into the the Goddard Cumulus Ensemble (GCE) model. The formulation for the explicit spectral-bim microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e., pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail]. Each type is described by a special size distribution function containing many categories (i.e., 33 bins). Atmospheric aerosols are also described using number density size-distribution functions.

Tao, Wei-Kuo↗

The Role of Aerosols on Precipitation Processes: Cloud Resolving Model Simulations

Cloud microphysics is inevitably affected by the smoke particle (CCN, cloud condensation nuclei) size distributions below the clouds. Therefore, size distributions parameterized as spectral bin microphysics are needed to explicitly study the effects of atmospheric aerosol concentration on cloud development, rainfall production, and rainfall rates for convective clouds. Recently, a detailed spectral-bin microphysical scheme was implemented into the Goddard Cumulus Ensemble (GCE) model. The formulation for the explicit spectral bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (i.e., cloud droplets and raindrops), and several types of ice particles [i.e. pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail]. Each type is described by a special size distribution function containing many categories (i.e., 33 bins). Atmospheric aerosols are also described using number density size-distribution functions. The model is tested by studying the evolution of deep cloud systems in the west Pacific warm pool region, the sub-tropics (Florida) and midlatitudes using identical thermodynamic conditions but with different concentrations of CCN: a low "clean" concentration and a high "dirty" concentration. Results indicate that the low CCN concentration case produces rainfall at the surface sooner than the high CeN case but has less cloud water mass aloft. Because the spectral-bin model explicitly calculates and allows for the examination of both the mass and number concentration of species in each size category, a detailed analysis of the instantaneous size spectrum can be obtained for these cases. It is shown that since the low (CN case produces fewer droplets, larger sizes develop due to greater condensational and collection growth, leading to a broader size spectrum in comparison to the high CCN case. Sensitivity tests were performed to identify the impact of ice processes, radiation and large-scale influence on cloud-aerosol interactive processes, especially regarding surface rainfall amounts and characteristics (i.e., heavy or convective versus light or stratiform types). In addition, an inert tracer was included to follow the vertical redistribution of aerosols by cloud processes. We will also give a brief review from observational evidence on the role of aerosol on precipitation processes.

Tao, Wei-Kuo↗

New, Improved Bulk-microphysical Schemes for Studying Precipitation Processes in WRF: Comparisons with Other Schemes - Part 1

Advances in computing power allow atmospheric prediction models to be mn at progressively finer scales of resolution, using increasingly more sophisticated physical parameterizations and numerical methods. The representation of cloud microphysical processes is a key component of these models, over the past decade both research and operational numerical weather prediction models have started using more complex microphysical schemes that were originally developed for high-resolution cloud-resolving models (CRMs). A recent report to the United States Weather Research Program (USWRP) Science Steering Committee specifically calls for the replacement of implicit cumulus parameterization schemes with explicit bulk schemes in numerical weather prediction (NWP) as part of a community effort to improve quantitative precipitation forecasts (QPF). An improved Goddard bulk microphysical parameterization is implemented into a state-of the-art of next generation of Weather Research and Forecasting (WRF) model. High-resolution model simulations are conducted to examine the impact of microphysical schemes on two different weather events (a midlatitude linear convective system and an Atllan"ic hurricane). The results suggest that microphysics has a major impact on the organization and precipitation processes associated with a summer midlatitude convective line system. The 31CE scheme with a cloud ice-snow-hail configuration led to a better agreement with observation in terms of simulated narrow convective line and rainfall intensity. This is because the 3ICE-hail scheme includes dense ice precipitating (hail) particle with very fast fall speed (over 10 m/s). For an Atlantic hurricane case, varying the microphysical schemes had no significant impact on the track forecast but did affect the intensity (important for air-sea interaction)

Tao, W.-K.↗

Parameterization of the Vertical Variability of Tropical Cirrus Cloud Microphysical and Optical Properties

Cloud Integrating Nephelometers (CIN) were flown on the U. North Dakota Citation aircraft and the NASA WB-57 aircraft for the purpose of measuring in-situ the optical extinction coefficient and the asymmetry parameter (g) at a wavelength of 635 nm of primarily ice particles encountered during the NASA CRYSTAL-FACE study of large cumulus clouds (Cu) and their anvils found in the southern Florida region. The probes performance was largely successful and produced archived data for vertical profiles of extinction, asymmetry parameter, and effective radius (Re), the latter being obtained by combining CIN and CVI (total water; Oregon State U.) measurements. Composites of the CIN and CVI data describing the average microphysical and optical behavior of the Cu and their anvils showed the following: The extinction increases with height as a result of the size of the particles also decreasing with height as shown by the Re measurements; near the top of anvils the size of the primary ice particles is about 10-um radius; and the value of g does not vary significantly with height and has a mean value of about 0.73 consistent with the idea that ambient ice crystals are primarily of complex shape and reflect solar radiation more efficiently than particles of pristine crystal shape. Other observations include: The g measurements were found to be an indicator of the phase of the cloud permitting identification of the clouds with water droplets, rain, and ice; visual ranges as small as several tens of meters were occasionally found in "extinction cores" that coincided with strong updraft cores; and comparison of the cloud probes on the Citation showed significant disagreement.

Gerber, Hermann E.↗

Saharan Dust Event Impacts on Cloud Formation and Radiation over Western Europe

We investigated the impact of mineral dust particles on clouds, radiation and atmospheric state during a strong Saharan dust event over Europe in May 2008, applying a comprehensive online-coupled regional model framework that explicitly treats particle-microphysics and chemical composition. Sophisticated parameterizations for aerosol activation and ice nucleation, together with two-moment cloud microphysics are used to calculate the interaction of the different particles with clouds depending on their physical and chemical properties. The impact of dust on cloud droplet number concentration was found to be low, with just a slight increase in cloud droplet number concentration for both uncoated and coated dust. For temperatures lower than the level of homogeneous freezing, no significant impact of dust on the number and mass concentration of ice crystals was found, though the concentration of frozen dust particles reached up to 100 l-1 during the ice nucleation events. Mineral dust particles were found to have the largest impact on clouds in a temperature range between freezing level and the level of homogeneous freezing, where they determined the number concentration of ice crystals due to efficient heterogeneous freezing of the dust particles and modified the glaciation of mixed phase clouds. Our simulations show that during the dust events, ice crystals concentrations were increased twofold in this temperature range (compared to if dust interactions are neglected). This had a significant impact on the cloud optical properties, causing a reduction in the incoming short-wave radiation at the surface up to -75Wm-2. Including the direct interaction of dust with radiation caused an additional reduction in the incoming short-wave radiation by 40 to 80Wm-2, and the incoming long-wave radiation at the surface was increased significantly in the order of +10Wm-2. The strong radiative forcings associated with dust caused a reduction in surface temperature in the order of -0.2 to -0.5K for most parts of France, Germany, and Italy during the dust event. The maximum difference in surface temperature was found in the East of France, the Benelux, and Western Germany with up to -1 K. This magnitude of temperature change was sufficient to explain a systematic bias in numerical weather forecasts during the period of the dust event.

Bangert, M.↗

Retrieval of Polar Stratospheric Cloud Microphysical Properties from Lidar Measurements: Dependence on Particle Shape Assumptions

A retrieval algorithm has been developed for the microphysical analysis of polar stratospheric cloud (PSC) optical data obtained using lidar instrumentation. The parameterization scheme of the PSC microphysical properties allows for coexistence of up to three different particle types with size-dependent shapes. The finite difference time domain (FDTD) method has been used to calculate optical properties of particles with maximum dimensions equal to or less than 2 mu m and with shapes that can be considered more representative of PSCs on the scale of individual crystals than the commonly assumed spheroids. Specifically. these are irregular and hexagonal crystals. Selection of the optical parameters that are input to the inversion algorithm is based on a potential data set such as that gathered by two of the lidars on board the NASA DC-8 during the Stratospheric Aerosol and Gas Experiment 0 p (SAGE) Ozone Loss Validation experiment (SOLVE) campaign in winter 1999/2000: the Airborne Raman Ozone and Temperature Lidar (AROTEL) and the NASA Langley Differential Absorption Lidar (DIAL). The 0 microphysical retrieval algorithm has been applied to study how particle shape assumptions affect the inversion of lidar data measured in leewave PSCs. The model simulations show that under the assumption of spheroidal particle shapes, PSC surface and volume density are systematically smaller than the FDTD-based values by, respectively, approximately 10-30% and approximately 5-23%.

Reichardt, J.↗