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All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Linking optical spectra to free charges in donor/acceptor heterojunctions: cross-correlation of transient microwave and optical spectroscopy

The primary photoexcited species in excitonic semiconductors is a bound electron–hole pair, or exciton. An important strategy for producing separated electrons and holes in photoexcited excitonic semiconductors is the use of donor/acceptor heterojunctions, but the degree to which the carriers can escape their mutual Coulomb attraction is still debated for many systems. Here, we employ a combined pump–probe ultrafast transient absorption (TA) spectroscopy and time-resolved microwave conductivity (TRMC) study on a suite of model excitonic heterojunctions consisting of mono-chiral semiconducting single-walled carbon nanotube (s-SWCNT) electron donors and small-molecule electron acceptors. Comparison of the charge-separated state dynamics between TA and TRMC photoconductance reveals a quantitative match over the 0.5 microsecond time scale. Charge separation yields derived from TA allow extraction of s-SWCNT hole mobilities of ca. 1.5 cm 2 V -1 s -1 (at 9 GHz) by TRMC. We find that the correlation between the techniques conclusively demonstrates that photoinduced charge carriers separated across these heterojunctions do not form bound charge transfer states, but instead form free/mobile charge carriers.

36 MATERIALS SCIENCE↗
NASA NTRS2015

Cloud-to-Ground Lightning Estimates Derived from SSMI Microwave Remote Sensing and NLDN

Lightning observations are collected using ground-based and satellite-based sensors. The National Lightning Detection Network (NLDN) in the United States uses multiple ground sensors to triangulate the electromagnetic signals created when lightning strikes the Earth's surface. Satellite-based lightning observations have been made from 1998 to present using the Lightning Imaging Sensor (LIS) on the NASA Tropical Rainfall Measuring Mission (TRMM) satellite, and from 1995 to 2000 using the Optical Transient Detector (OTD) on the Microlab-1 satellite. Both LIS and OTD are staring imagers that detect lightning as momentary changes in an optical scene. Passive microwave remote sensing (85 and 37 GHz brightness temperatures) from the TRMM Microwave Imager (TMI) has also been used to quantify characteristics of thunderstorms related to lightning. Each lightning detection system has fundamental limitations. TRMM satellite coverage is limited to the tropics and subtropics between 38 deg N and 38 deg S, so lightning at the higher latitudes of the northern and southern hemispheres is not observed. The detection efficiency of NLDN sensors exceeds 95%, but the sensors are only located in the USA. Even if data from other ground-based lightning sensors (World Wide Lightning Location Network, the European Cooperation for Lightning Detection, and Canadian Lightning Detection Network) were combined with TRMM and NLDN, there would be enormous spatial gaps in present-day coverage of lightning. In addition, a globally-complete time history of observed lightning activity is currently not available either, with network coverage and detection efficiencies varying through the years. Previous research using the TRMM LIS and Microwave Imager (TMI) showed that there is a statistically significant correlation between lightning flash rates and passive microwave brightness temperatures. The physical basis for this correlation emerges because lightning in a thunderstorm occurs where ice is first present in the cloud and electric charge separation occurs. These ice particles efficiently scatter the microwave radiation at the 85 and 37 GHz frequencies, thus leading to large brightness temperature depressions. Lightning flash rate is related to the total amount of ice passing through the convective updraft regions of thunderstorms. Confirmation of this relationship using TRMM LIS and TMI data, however, remains constrained to TRMM observational limits of the tropics and subtropics. Satellites from the Defense Meteorology Satellite Program (DMSP) have global coverage and are equipped with passive microwave imagers that, like TMI, observe brightness temperatures at 85 and 37 GHz. Unlike the TRMM satellite, however, DMSP satellites do not have a lightning sensor, and the DMSP microwave data has never been used to derive global lightning. In this presentation, a relationship between DMSP Special Sensor Microwave Imager (SSMI) data and ground-based cloud-to-ground (CG) lightning data from NLDN is investigated to derive a spatially complete time history of CG lightning for the USA study area. This relationship is analogous to the established using TRMM LIS and TMI data. NLDN has the most spatially and temporally complete CG lightning data for the USA, and therefore provides the best opportunity to find geospatially coincident observations with SSMI sensors. The strongest thunderstorms generally have minimum 85 GHz Polarized Corrected brightness Temperatures (PCT) less than 150 K. Archived radar data was used to resolve the spatial extent of the individual storms. NLDN data for that storm spatial extent defined by radar data was used to calculate the CG flash rate for the storm. Similar to results using TRMM sensors, a linear model best explained the relationship between storm-specific CG flash rates and minimum 85 GHz PCT. However, the results in this study apply only to CG lightning. To extend the results to weaker storms, the probability of CG lightning (instead of the flash rate) was calculated for storms having 85 GHz PCT greater than 150 K. NLDN data was used to determine if a CG strike occurred for a storm. This probability of CG lightning was plotted as a function of minimum 85 GHz PCT and minimum 37 GHz PCT. These probabilities were used in conjunction with the linear model to estimate the CG flash rate for weaker storms with minimum 85 GHz PCTs greater than 150 K. Results from the investigation of CG lightning and passive microwave radiation signals agree with the previous research investigating total lightning and brightness temperature. Future work will take the established relationships and apply them to the decades of available DMSP data for the USA to derive a map of CG lightning flash rates. Validation of this method and uncertainty analysis will be done by comparing the derived maps of CG lightning flash rates against existing NLDN maps of CG lightning flash rates.

Winesett, Thomas↗
NASA NTRS2003

Preliminary Optical And Electric Field Pulse Statistics From Storm Overflights During The Altus Cumulus Electrification Study

The Altus Cumulus Electrification Study (ACES) was conducted during the month of August, 2002 in an area near Key West, Florida. One of the goals of this uninhabited aerial vehicle (UAV) study was to collect high resolution optical pulse and electric field data from thunderstorms. During the month long campaign, we acquired 5294 lightning generated optical pulses with associated electric field changes. Most of these observations were made while close to the top of the storms. We found filtered mean and median 10-10% optical pulse widths of 875 and 830 microns respectively while the 50-50% mean and median optical pulse widths are 422 and 365 microns respectively. These values are similar to previous results as are the 10-90% mean and median rise times of 327 and 265 microns. The peak electrical to optical pulse delay mean and median were 209 and 145 microns which is longer than one would expect from theoretical results. The results of the pulse analysis will contribute to further validation of the Optical Transient Detector (OTD) and the Lightning Imaging Sensor (LIS) satellites. Pre-launch estimates of the flash detection efficiency were based on a small sample of optical pulse measurements associated with less than 350 lightning discharges collected by NASA U-2 aircraft in the early 1980s. Preliminary analyses of the ACES measurements show that we have greatly increased the number of optical pulses available for validation of the LIS and other orbital lightning optical sensors. Since the Altus was often close to the cloud tops, many of the optical pulses are from low-energy pulses. From these low-energy pulses, we can determine the fraction of optical lightning pulses below the thresholds of LIS, OTD, and any future satellite-based optical sensors such as the geostationary Lightning Mapping Sensor.

Mach, D. A.↗
NASA NTRS2013

The Galex Time Domain Survey. I. Selection And Classification of Over a Thousand Ultraviolet Variable Sources

We present the selection and classification of over a thousand ultraviolet (UV) variable sources discovered in approximately 40 deg(exp 2) of GALEX Time Domain Survey (TDS) NUV images observed with a cadence of 2 days and a baseline of observations of approximately 3 years. The GALEX TDS fields were designed to be in spatial and temporal coordination with the Pan-STARRS1 Medium Deep Survey, which provides deep optical imaging and simultaneous optical transient detections via image differencing. We characterize the GALEX photometric errors empirically as a function of mean magnitude, and select sources that vary at the 5 sigma level in at least one epoch. We measure the statistical properties of the UV variability, including the structure function on timescales of days and years. We report classifications for the GALEX TDS sample using a combination of optical host colors and morphology, UV light curve characteristics, and matches to archival X-ray, and spectroscopy catalogs. We classify 62% of the sources as active galaxies (358 quasars and 305 active galactic nuclei), and 10% as variable stars (including 37 RR Lyrae, 53 M dwarf flare stars, and 2 cataclysmic variables). We detect a large-amplitude tail in the UV variability distribution for M-dwarf flare stars and RR Lyrae, reaching up to absolute value(Δm) = 4.6 mag and 2.9 mag, respectively. The mean amplitude of the structure function for quasars on year timescales is five times larger than observed at optical wavelengths. The remaining unclassified sources include UV-bright extragalactic transients, two of which have been spectroscopically confirmed to be a young core-collapse supernova and a flare from the tidal disruption of a star by dormant supermassive black hole. We calculate a surface density for variable sources in the UV with NUV less than 23 mag and absolute value(Δm) greater than 0.2 mag of approximately 8.0, 7.7, and 1.8 deg(exp −2) for quasars, active galactic nuclei, and RR Lyrae stars, respectively. We also calculate a surface density rate in the UV for transient sources, using the effective survey time at the cadence appropriate to each class, of approximately 15 and 52 deg(exp −2 yr−1 for M dwarfs and extragalactic transients, respectively.

Gezari, S.↗
NASA NTRS2001

Preliminary Design of a Lightning Optical Camera and ThundEr (LOCATE) Sensor

The preliminary design of an optical/acoustical instrument is described for making highly accurate real-time determinations of the location of cloud-to-ground (CG) lightning. The instrument, named the Lightning Optical Camera And ThundEr (LOCATE) sensor, will also image the clear and cloud-obscured lightning channel produced from CGs and cloud flashes, and will record the transient optical waveforms produced from these discharges. The LOCATE sensor will consist of a full (360 degrees) field-of-view optical camera for obtaining CG channel image and azimuth, a sensitive thunder microphone for obtaining CG range, and a fast photodiode system for time-resolving the lightning optical waveform. The optical waveform data will be used to discriminate CGs from cloud flashes. Together, the optical azimuth and thunder range is used to locate CGs and it is anticipated that a network of LOCATE sensors would determine CG source location to well within 100 meters. All of this would be accomplished for a relatively inexpensive cost compared to present RF lightning location technologies, but of course the range detection is limited and will be quantified in the future. The LOCATE sensor technology would have practical applications for electric power utility companies, government (e.g. NASA Kennedy Space Center lightning safety and warning), golf resort lightning safety, telecommunications, and other industries.

Phanord, Dieudonne D.↗
DOE OSTI2025

Ultrabroadband THz conductivity of gated graphene in- and out-of-equilibrium

We employ ultrabroadband terahertz (THz) spectroscopy to expose the high-frequency transport properties of Dirac fermions in monolayer graphene. By controlling the carrier concentration via tunable electrical gating, both equilibrium and transient optical conductivities are obtained for a range of Fermi levels. The frequency-dependent equilibrium response is determined through a combination of time-domain THz and Fourier-transform infrared spectroscopy for energies up to the near-infrared, which also provides a measure of the gate-voltage dependent Fermi level. Transient changes in the real and imaginary parts of the graphene conductivity are electro-optically resolved for frequencies up to 15 THz after near-infrared femtosecond excitation, both at the charge-neutral point and for higher electrostatic-doping levels. Modeling of the THz response provides insight into changes of the carrier spectral weights and scattering rates, and reveals an additional broad-frequency ($$\approx$$ 8 THz) component to the photo-induced response, which we attribute to the zero-momentum mode of quantum-critical transport observed here in large-area CVD graphene.

Coslovich, G↗
NASA NTRS1986

Searches for low-energy counterparts of gamma-ray bursters

The results of six studies concerning the identification of low-energy counterparts of gamma-ray bursters (GRBs) are reported. From these results, it is concluded that the near-infrared observations of GRBs from IRAS pose serious difficulties for several GRB models. No precedent or plausible explanation is found for the optical flash detected on February 8, 1984 by Pedersen et al. (1984) other than that the flash originated on a GRB. The star in the middle of the 1944 optical transient error box has an ultraviolet excess which is significant at the 95 percent confidence level, a result which strongly suggests that the object is indeed the quiescent GRB optical counterpart. If true, then GRBs are probably low-mass contact binaries caused by thermonuclear or accretion instabilities at distances of roughly 1 kpc.

Schaefer, B. E.↗
NASA NTRS2007

Differences in the Optical Characteristics of Continental US Ground and Cloud Flashes as Observed from Space

Continental US lightning flashes observed by the Optical Transient Detector (OTD) are categorized according to flash type (ground or cloud flash) using US National Lightning Detection Network (TM) (NLDN) data. The statistics of the ground and cloud flash optical parameters (e.g., radiance, area, duration, number of optical groups, and number of optical events) are inter-compared. On average, the ground flash cloud-top emissions are more radiant, illuminate a larger area, are longer lasting, and have more optical groups and optical events than those cloud-top emissions associated with cloud flashes. Given these differences, it is suggested that the methods of Bayesian Inference could be used to help discriminate between ground and cloud flashes. The ability to discriminate flash type on-orbit is highly desired since such information would help researchers and operational decision makers better assess the intensification, evolutionary state, and severe weather potential of thunderstorms. This work supports risk reduction activities presently underway for the future launch of the GOES-R Geostationary Lightning Mapper (GLM).

Koshak, William↗
DOE OSTI2022

Characterisations of the HinOTORI telescope with a three-color imager at Ali Observatory in Western Tibet

HinOTORI is a new telescope supported by an international collaboration project between China and Japan. It is a 50 centimeter telescope equipped with simultaneous three-color imagers (u',R C , and I C bands). It is located at Ali Observatory at an altitude of 5100m. Thanks to the high altitude and extreme dryness, Ali site is one of the most suitable sites for optical astrometry. HinOTORI telescope aims at detecting optical transients such as the counterparts of gravitational wave (GW) sources, supernovae, gamma-ray bursts (GRB) and so on. This paper describes the site information, design of simultaneous three-color optical layout, system instruments and whole control system. We also report some telescope characterisations for three bands (u'/R C /I C ) respectively, such as Hartmann constant (0.49"/0.56"/0.60"), best focus position (3.922/3.920/3.903 mm), PSF FWHM size (3.755/3.328/3.167pixels), total transmittance and limiting magnitude (15.69/17.57/17.05mag, 10 σ 30 seconds exposure time). With different airmass observation data, the atmospheric extinction coefficients of three bands (0.366/0.061/0.026) were also derived.

47 OTHER INSTRUMENTATION↗
NASA NTRS1986

Gamma-ray burst and spectroscopy instrumentation development at the Goddard Space Flight Center

This paper summarizes the activities that are specifically related to the development of instrumentation for gamma-ray astronomy. Three programs are described: (1) the Gamma-Ray Imaging Spectrometer (GRIS), a balloon-borne array of seven germanium detectors for high-resolution spectrographic studies of persistent gamma-ray sources; (2) the Transient Gamma-Ray Spectrometer (TGRS), a single radiatively-cooled germanium detector for the spectrographic study of gamma-ray bursts, and (3) the Rapidly Moving Telescope (RMT), a ground-based optical telescope for the detection and study of short-lived optical transients, particularly those that occur in coincidence with gamma-ray bursts.

Teegarden, B. J.↗
NASA NTRS1993

Solar cycle variation of interplanetary disturbances observed as Doppler scintillation transients

Interplanetary disturbances characterized by plasma that is more turbulence and/or moves faster than the background solar wind are readily defected as transients in Doppler scintillation measurements of the near-Sun solar wind. Systematic analysis of over 23,000 hours of Pioneer Venus Orbiter Doppler measurements obtained inside 0.5 AU during 1979-1987 have made it possible for the first time to investigate the frequency of occurrence of Doppler scintillation transients under solar minimum conditions and to determine its dependence on solar cycle. On the basis of a total of 142 transients, Doppler scintillation transient rates vary from a high of 0.22 in 1979 (one every 4.6 days) to a low of 0.077 transients/d in 1986 (one every 13 days), a decrease by almost a factor of 3 from solar maximum to solar minimum. This solar cycle variation, the strongest yet of any solar wind Doppler scintillation property, is highly correlated with both solar activity characterized by sunspot number and the coronal mass ejection rates deduced from Solswind and Solar Maximum Mission (SMM) coronagraph observations. These results indicate that coronal mass ejections and Doppler scintillation transients are closely related not just during solar maximum, as occasional individual comparisons have shown in the past, but throughout the entire solar cycle, and strengthen the notation that the Doppler scintillation and optical transients are different manifestations of the same physical phenomenon. The magnitudes of the transients, as described by the ratio of peak to pretransient scintillation levels (EF for enhancement factor), and their distribution iwth heliocentric distance also vary with solar cycle. While EF tends to diminish with increasing heliocentric distance during high solar activity, it is more evenly distributed during low solar activity. EF is also lower during solar minimum, as 13% of the transients during solar maximum have values exceeding 23, the highest EF observed during solar minimum. These results are consistent with the fact that occasional major fast-moving interplanetary shocks that are observed during solar maximum are very rate during solar minimum.

Woo, Richard↗
NASA NTRS1997

The Optical Counterpart to Gamma-Ray Burst GRB 970228 Observed Using the Hubble Space Telescope

Although more than 2,000 astronomical gamma-ray bursts (GRBS) have been detected, and numerous models proposed to explain their occurrence, they have remained enigmatic owing to the lack of an obvious counterpart at other wavelengths. The recent ground-based detection of a transient optical source in the vicinity of GRB970228 may therefore have provided a breakthrough. The optical counterpart appears to be embedded in an extended source which, if a galaxy, as has been suggested would lend weight to those models that place GRBs at cosmological distances. Here we report, observations using the Hubble Space Telescope of the transient counterpart and extended source 26 and 39 days after the initial gamma-ray outburst. We find that the counterpart has faded since the initial detection (and continues to fade), but the extended source exhibits no significant change in brightness between the two dates of the observations reported here. The size and apparent constancy of the extended source imply that it is extragalactic, but its faintness makes a definitive statement about its nature difficult. Nevertheless, the decay profile of the transient source is consistent with a popular impulsive-fireball model13, which assumes a merger between two neutron stars in a distant galaxy.

Sahu, K. C.↗
DOE OSTI2026

Direct Observation of Ultrafast Defect-Bound and Free Exciton Dynamics in Defect-Engineered WS 2 Monolayers

Defects in two-dimensional transition metal dichalcogenides (TMDCs) broadly affect their optical and electronic properties. Directly capturing the ultrafast processes of exciton trapping and defect-bound exciton formation is crucial for understanding and advancing defect-mediated optoelectronics and quantum technologies. However, the weak transient optical absorption of defect-bound excitons has limited their experimental observation to date. Here, we report the direct observation of the ultrafast dynamics of defect-bound excitons in monolayer WS 2 crystals with a high density of monosulfur vacancies (V S ) and W-site defect complexes (S W V S ) resulting from synthesis by alkali metal halide-assisted chemical vapor deposition. The dynamics of excitons bound to these defects, along with their coherent interactions with free excitons, are elucidated using ultrafast optical spectroscopy. Using above band-edge photoexcitation, we find that both free and defect-bound excitons simultaneously form within 300 fs from hot carrier relaxation. The defect-bound excitons exhibit shorter lifetimes than free excitons, leading to a population difference of the corresponding excitonic states and free exciton trapping within a 1–100 ps window. Band-edge photoexcitation of free and defect-bound exciton states reveals ultrafast interconversion within ∼150 fs (comparable to our temporal resolution), indicating possible coherent coupling between these states. We further demonstrate efficient up-conversion of defect-bound excitons to free excitons with photon energies up to ∼300 meV below the free exciton resonance. In conclusion, these findings provide insights into the ultrafast dynamics of defect-bound excitons in TMDCs and their coupling with free excitons, which are relevant to defect-engineered optoelectronic, quantum photonic, and valleytronic applications.

36 MATERIALS SCIENCE↗
NASA NTRS1986

A search for optical flashes from the 'Perseus Flasher'

The results of an extended search for short-timescale optical flashes from a four square-degree area centered on the coordinates of the Perseus Flasher are reported. The photographed optical flash was of brightness mB = -1.7 and had a duration of roughly 0.5 s. In 70 hours of observation no celestial optical flashes were detected in the region of the Perseus Flasher to a limiting magnitude of 7.1 for a one-second flash. Neither X-ray nor optical flashes were seen. A survey of archived photographic images of the Perseus Flasher revealed no optical transients in over 700 hours of total exposure time to a limiting magnitude of mB about 4-5 for a one-second flash. Based on the ETC data base, possible terrestrial sources of optical flashes which might account for the phenomenon are discussed.

Vanderspek, Roland K.↗
NASA NTRS2008

Potential Use of a Bayesian Network for Discriminating Flash Type from Future GOES-R Geostationary Lightning Mapper (GLM) data

Continuous monitoring of the ratio of cloud flashes to ground flashes may provide a better understanding of thunderstorm dynamics, intensification, and evolution, and it may be useful in severe weather warning. The National Lighting Detection Network TM (NLDN) senses ground flashes with exceptional detection efficiency and accuracy over most of the continental United States. A proposed Geostationary Lightning Mapper (GLM) aboard the Geostationary Operational Environmental Satellite (GOES-R) will look at the western hemisphere, and among the lightning data products to be made available will be the fundamental optical flash parameters for both cloud and ground flashes: radiance, area, duration, number of optical groups, and number of optical events. Previous studies have demonstrated that the optical flash parameter statistics of ground and cloud lightning, which are observable from space, are significantly different. This study investigates a Bayesian network methodology for discriminating lightning flash type (ground or cloud) using the lightning optical data and ancillary GOES-R data. A Directed Acyclic Graph (DAG) is set up with lightning as a "root" and data observed by GLM as the "leaves." This allows for a direct calculation of the joint probability distribution function for the lighting type and radiance, area, etc. Initially, the conditional probabilities that will be required can be estimated from the Lightning Imaging Sensor (LIS) and the Optical Transient Detector (OTD) together with NLDN data. Directly manipulating the joint distribution will yield the conditional probability that a lightning flash is a ground flash given the evidence, which consists of the observed lightning optical data [and possibly cloud data retrieved from the GOES-R Advanced Baseline Imager (ABI) in a more mature Bayesian network configuration]. Later, actual GLM and NLDN data can be used to refine the estimates of the conditional probabilities used in the model; i.e., the Bayesian network is a learning network. Methods for efficient calculation of the conditional probabilities (e.g., an algorithm using junction trees), finding data conflicts, goodness of fit, and dealing with missing data will also be addressed.

Solakiewiz, Richard↗
NASA NTRS1999

Optical Detection of Lightning from Space

Two primary detection techniques (optical and RF) have a proven capability for detecting lightning from low earth orbit. However, the lightning processes that generate the optical and RF signals are vastly different providing significantly different information content from each sensor type. Because of the intervening ionosphere, low frequency RF components do not reach satellite altitudes. As a consequence, many of the processes associated with the major energy release of a lightning event (i.e. return strokes, k-changes, recoil streamers, etc), in all likelihood contribute little to the RF signal arriving at the satellite. The optical output from lighting, on the other hand, has been shown to be highly correlated with the energetic, charge-transferring processes mentioned above. On the down side, the optical energy, while essentially unaffected by the atmosphere once it emerges from the cloud, is heavily scattered within the cloud. While there is little absorption by the cloud, the great optical depth makes the total light energy emerging from the cloud to be dependent on where in the cloud the lightning occurred. Analyses suggest that when lightning is confined to the lowest regions of the cloud, the light is strongly attenuated and detection becomes problematic. Fortunately, the vast majority of lightning flashes are comprised of channels that propagate through the middle of the cloud and higher. These flashes produce bright signals at the top of a cloud and are readily detectable. Presently, we have two optical instruments in orbit. The Optical Transient Detector (OTD) has been orbiting the earth since April, 1995, while the Lightning Imaging Sensor (LIS) was launched on the Tropical Rainfall Measuring Mission (TRMM) in November of 1997. Both instruments are relatively small, solid state optical imagers, designed specifically to detect and locate lightning activity from low earth orbit with high detection efficiency and location accuracy.

Christian, H. J.↗