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DOE OSTI2024

Surface-to-Interior Transport Timescales and Ventilation Patterns in a Time-Dependent Circulation Driven by Sustained Climate Warming

Abstract The effect of climate warming in response to rising atmospheric CO 2 on the ventilation of the ocean remains uncertain. Here we make theoretical advances in elucidating the relationship between ideal age and transit time distribution (TTD) in a time-dependent flow. Subsequently, we develop an offline tracer-transport model to characterize the ventilation patterns and time scales in the time-evolving circulation for the 1850–2300 period as simulated with the Community Earth System Model version 1 (CESMv1) under a business-as-usual warming scenario. We found that by 2300 2.1% less water originates from the high-latitude deep water formation regions (both hemispheres) compared to 1850. In compensation, there is an increase in the water originating from the subantarctic. We also found that slowing meridional overturning circulation causes a gradual increase in mean age during the 1850–2300 period, with a globally averaged mean-age increase of ∼110 years in 2300. Where and when the water will be re-exposed to the atmosphere depends on the post-2300 circulation. For example, if we assume that the circulation persists in its year-2300 state (scenario 1), the mean interior-to-surface transit time in year 1850 is ∼1140 years. In contrast, if we assume that the circulation abruptly recovers to its year-1850 state (scenario 2), the mean interior-to-surface transit time in 1850 is only ∼740 years. By 2300, these differences become even larger; in scenario 1, the mean interior-to-surface transit time increases by ∼200 years, whereas scenario 2 decreases by ∼80 years. The dependence of interior-to-surface transit time on the future ocean circulation produces an additional unavoidable uncertainty in the long-term durability of marine carbon dioxide removal strategies. Significance Statement The ocean’s circulation, when altered by climate warming, can affect its capacity to absorb heat and CO 2 , which are crucial for the global climate. In our study, we investigated how global warming, caused by rising CO 2 levels, might impact the ocean circulation—the way water moves from deep ocean to the surface and vice versa. We discovered that by 2300, if we continue on our current warming trajectory, the origins of water within the ocean will shift, with less coming from deep, cold zones near the poles and more from subantarctic regions. As a result, deep water will take longer time before it resurfaces than shallow water. How quickly this water travels from deep regions to the surface could change, depending on the state of future ocean circulation. If the circulation remains as predicted in 2300, this journey will take longer. Conversely, if it reverts to the pattern in 1850, the process will be quicker. This variability introduces added uncertainty to strategies aimed at mitigating climate change by storing CO 2 in the ocean. Our work highlights the intricate ways in which climate change can influence our oceans, potentially affecting our plans to mitigate global warming.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

U.S. Nuclear Declaratory Policy 2021: the Renewed Debate about Sole Purpose and No-First-Use. Annotated Bibliography

Declaratory policy and public statements about the potential use of nuclear weapons serve many important roles. They provide an assessment of the security environment, and inform the public debate. These statements also enhance deterrence messages and signals towards adversaries, and reassure allies and partners. On the global level, U.S. declaratory policy has the potential to shape international trends and norms, influence nuclear proliferation, and it may also affect the policy decisions of other nuclear possessors. As the Biden administration reviews the elements of U.S. nuclear declaratory policy, the issue of sole purpose and no-first-use is likely to resurface. Previous administrations have examined these policies in multiple rounds of review, and they decided that the time was not right for such declarations. This literature review was prepared to inform the debate by collecting some of the most prominent articles on the topic that highlight the potential risks and benefits of these policies.

29 ENERGY PLANNING, POLICY, AND ECONOMY↗

DOE OSTI2022

Non-Destructive In-Process Assessment of Thermal Spray Repairs

This exploratory project, entitled “Non-Destructive In-process Assessment of Thermal Spray Repairs,” evaluated the capabilities and limitations of four non-destructive testing (NDE) technologies for detection of defects in as-sprayed thermal spray coatings: acousto-ultrasonics, vibro-thermography, thermal wave infrared (IR) imaging, and flash IR thermography. The project goal was to identify a single technology suitable for use as an in-process inspection for two common classes of defects in thermal spray coatings, porosity and disbonds. Two rounds of test coupons were fabricated with intentionally seeded defects in AISI 420 stainless steel coatings deposited by twin wire arc (TWA) spray onto gray cast iron substrates. These standardized test coupons allowed the sensitivity of the four NDE methods to be directly compared. The results indicated that the acousto-ultrasonic method will not meet requirements for accuracy, inspection time, and reproducibility, while the vibrothermography method will not meet requirements for integration within remanufacturing cells and process flows. The IR methods, thermal wave imaging and flash thermography, both exhibited acceptable accuracy and reproducibility; however, the former method does not meet the requirement for inspection time. Flash IR thermography met all requirements in the initial round of testing, and that result was confirmed in a second round of testing on samples with a larger, more complex geometry. A final recommendation for further development of flash IR thermography was therefore made based upon i) detection performance, and ii) feasibility of deployment into the target application of resurfacing CAT engine blocks and headers.

36 MATERIALS SCIENCE↗

DOE OSTI2023

Iodine Air Sampling: Installation and Preliminary Results

The F-Area wetlands are a known sink for radioiodine generated at the Savannah River Site (SRS). Wastewater containing iodine-129 ( 129 I) was discharged into the F-Area Seepage Basins for disposal, but the acidity of the wastewater mobilized some of the contaminants from the basin soil through the vadose zone and into the groundwater; ultimately creating a groundwater plume that extends towards Fourmile Branch and its associated wetland areas. Dissolved radioiodine specifically has migrated to the nearby F-Area wetlands, where it persists as a contaminant of concern. Accumulation and resurfacing of 129 I in the wetlands and nearby areas creates a potential secondary source zone where changes in biogeochemical conditions could result in the release of this sequestered 129 I to the air. Monitoring data has indicated that 129 I has a seasonal behavior at several surface water stations, with high concentrations during summertime and low concentrations during wintertime. Still, it is not known which factors control the seasonal behavior of 129 I. Further, it has been reported that 129 I contributed approximately 23% to the 2019 SRS offsite air pathway dose to the representative person for that year (SRNS, 2020), but air measurements of 129 I have never been taken in the F-Area wetlands. Because air emissions of 129 I from the wetlands have never been investigated, it is not known if this could be a potential release pathway that needs to be included in the site conceptual model. To address these unknowns, the Savannah River National Laboratory (SRNL) has an applied research task to investigate whether 129 I in the wetlands is emitted to the air and, if so, whether air concentrations exhibit seasonal variation. This report presents information about the system recently installed in the F-Area wetlands for measuring 129 I, as well as analysis results for samples collected June through August 2023. Quantification of this constituent will provide a better understanding of the contribution of airborne 129 I from the F-Area wetlands to the offsite dose and better inform ongoing and future remedial actions.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2022

Transport Affordable Clean Hydrogen Energy via Existing Pipeline Infrastructure (CRADA 573)

Our Nation’s vast network of oil pipelines span over 230,000 miles connecting remote energy producing regions to distant markets. The COVID-19 pandemic’s influence on oil prices intensified technical and economic vulnerabilities afflicting the Trans-Alaska Pipeline System (TAPS, operating below 25% capacity) that may soon resurface as energy demand shifts to low carbon sources. Through the opportunity afforded by the Arctic Advanced Manufacturing Program, I’ve toured the great State of Alaska learning about its culture, unique energy challenges, business ecosystem, research institutions, and regulatory agencies. With encouragement and support from dedicated Alaskans and my professional mentors, I’ve founded Mighty Pipeline for the purpose of developing and commercializing proprietary technology and hardware to convert oil pipelines into clean hydrogen energy transmission systems. Leveraging the advanced technical capabilities of Pacific Northwest National Laboratory, we’ve demonstrated proof-of-concept (TRL = 3) and are seeking pre-pilot development project opportunities to conduct hardware and system level tests. If we successfully achieve technical and regulatory milestones, Mighty Pipeline’s technology could be available to help facilitate bulk clean hydrogen energy export this decade.

08 HYDROGEN↗

DOE OSTI2024

In-Plane Liftout and Push-to-Pull for In Situ Mechanical Testing of Irradiated Inconel X-750

A streamlined sample preparation method for nanomechanical testing is needed to improve the quality of specimens, reduce the cost, and increase the versatility of specimen fabrication. This work outlines an in-plane liftout focused ion beam (FIB) fabrication procedure to prepare electron-transparent specimens for in situ transmission electron microscopy (TEM) nanomechanical testing. Ion etching and electron backscatter diffraction (EBSD) techniques were used to lift out a [110] oriented grain from a neutron-irradiated bulk X-750 alloy. Careful control of voltages and currents ensured precision. Top surface thinning sweeps prevented resurfacing and redeposition while dog-bone geometries were shaped with a 1:4 gauge width-to-milling pattern diameter ratio. Nanotensile testing in the TEM with a picoindenter allowed for the estimation of an ultimate tensile strength of 2.41 GPa, and inspection revealed a high density of bubbles in the X-750 matrix. The proposed fabrication procedure is significant for preparing samples from radioactive materials, studying complex structures that are orientation-dependent, and analyzing desired planar areas.

36 MATERIALS SCIENCE↗

DOE OSTI2020

Endogenic and Exogenic Contributions to Visible-wavelength Spectra of Europa’s Trailing Hemisphere

The composition of Europa’s trailing hemisphere reflects the combined influences of endogenous geologic resurfacing and exogenous sulfur radiolysis. Using spatially resolved visible-wavelength spectra of Europa obtained with the Hubble Space Telescope, we map multiple spectral features across the trailing hemisphere and compare their geographies with the distributions of large-scale geology, magnetospheric bombardment, and surface color. Based on such comparisons, we interpret some aspects of our spectra as indicative of purely exogenous sulfur radiolysis products and other aspects as indicative of radiolysis products formed from a mixture of endogenous material and magnetospheric sulfur. The spatial distributions of two of the absorptions seen in our spectra—a widespread downturn toward the near-UV and a distinct feature at 530 nm—appear consistent with sulfur allotropes previously suggested from ground-based spectrophotometry. However, the geographies of two additional features—an absorption feature at 360 nm and the spectral slope at red wavelengths—are more consistent with endogenous material that has been altered by sulfur radiolysis. We suggest irradiated sulfate salts as potential candidates for this material, but we are unable to identify particular species with the available data.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2024

Dramatic Rebrightening of the Type-changing Stripped-envelope Supernova SN 2023aew

Abstract Multipeaked supernovae with precursors, dramatic light-curve rebrightenings, and spectral transformation are rare, but are being discovered in increasing numbers by modern night-sky transient surveys like the Zwicky Transient Facility. Here, we present the observations and analysis of SN 2023aew, which showed a dramatic increase in brightness following an initial luminous (−17.4 mag) and long (∼100 days) unusual first peak (possibly precursor). SN 2023aew was classified as a Type IIb supernova during the first peak but changed its type to resemble a stripped-envelope supernova (SESN) after the marked rebrightening. We present comparisons of SN 2023aew’s spectral evolution with SESN subtypes and argue that it is similar to SNe Ibc during its main peak. P-Cygni Balmer lines are present during the first peak, but vanish during the second peak’s photospheric phase, before H α resurfaces again during the nebular phase. The nebular lines ([O i ], [Ca ii ], Mg i ], H α ) exhibit a double-peaked structure that hints toward a clumpy or nonspherical ejecta. We analyze the second peak in the light curve of SN 2023aew and find it to be broader than that of normal SESNe as well as requiring a very high 56 Ni mass to power the peak luminosity. We discuss the possible origins of SN 2023aew including an eruption scenario where a part of the envelope is ejected during the first peak and also powers the second peak of the light curve through interaction of the SN with the circumstellar medium.

Sharma, Yashvi (ORCID:0000000345311745)↗

NASA NTRS1976

Comparison of large crater and multiringed basin populations on Mars, Mercury, and the moon

The maximum regional areal densities of large impact craters on Mars, Mercury, and the moon appear to be inversely proportional to the surface areas of the planets. This would not be expected if the objects impacting the planetary surfaces came from common sources and were moving with high velocities relative to the planets; rather, a uniform areal density would be anticipated. Another way of stating the observation is that each planet was bombarded by the same number of objects. Two speculative explanations for the observation are that: (1) all planets underwent a uniform bombardment but were resurfaced by processes proportional to planetary surface area, or (2) equally populated families of objects, moving about the sun in orbits similar to those of the planets, were independently depopulated by the respective planets.

Malin, M. C.↗

NASA NTRS1980

Near-surface flow of volcanic gases on Io

Significant near-surface flow of gas several hundred kilometers from Pele (Plume 1) on Io is indicated by a series of bright, elongate albedo markings. Particles produced at small, local vents are apparently carried as much as 70 km farther 'downwind' from Pele. The gas densities and velocities necessary to suspend 0.1 to 10 micron particles at such a distance imply mass flow rates of 10 to the 7th - 10 to the 9th g/sec. Such flow rates are consistent with other estimates of mass transport by the plume. The large flow rates so far from the source allow an estimate of the rate of resurfacing of Io by lava flows and pyroclastics that is independent of estimates based on meteorite flux or on the amount of solids carried within the plumes themselves.

Lee, S. W.↗

NASA NTRS1981

Martian thermal history, core segregation, and tectonics

A series of calculated thermal histories of Mars is presented, and their possible relation to surface tectonic history is discussed. The models include convective heat transport through an empirical approximation, and heating by radioactivity and core segregation. Initial temperature and the timing and duration of core segregation are treated as free parameters. The initial temperature is the main determinant of Martian thermal evolution: as it is varied from 20 to 100% of the present mean temperature, the maximum in surface heat flux moves from very recent to very early in Martian history. For the latter cases, the details of core segregation control the detailed timing of a peak in the thermal flux that exceeded 100 mW/sq m. It is suggested that the early disruption of cratered terrain crust in the northern hemisphere and subsequent volcanic resurfacing may have been related to core segregation. This would be consistent with a scenario in which an early period of core segregation generated a marked peak in the thermal flux that may have led to extensive partial melting and volcanism. This scenario would require Mars to have had an initial mean temperature comparable to the present value.

Davies, G. F.↗

NASA NTRS1981

Boron and beryllium in Gamma Geminorum

Observations have been made of the B II resonance line at 1362 A in the A0 IV star Gamma Gem with the Princeton spectrometer on the Copernicus satellite at a spectral resolution of 0.05 A. Complementary ground-based observations of the Be II resonance lines at 3130 and 3131 A have been made at Mauna Kea Observatory with a comparable resolution. A model-atmosphere abundance analysis has been done which includes the effects of the lines that blend with the B II and Be II lines. Previous data on Alpha Lyr and Alpha CMa for B II (which blends with a V III feature) have been reanalyzed with the help of new photographic and Reticon data from Mauna Kea which enable the determination of the V abundance. The results show that Gamma Gem is depleted in B by a factor of 5-10 relative to Alpha Lyr and other normal B stars and depleted in Be by at least a factor of four. By comparison, the hot Am star Alpha CMa is B-deficient by about three orders of magnitude and Be-deficient by at least fifteen times. It is suggested that the abundance deficiencies are due to diffusion, and that Alpha CMa is intrinsically a slow rotator, and Gamma Gem is a slightly evolved slow rotator where some, but not all, of the B and Be has resurfaced.

Boesgaard, A. M.↗

NASA NTRS1981

Martian cratering revisited - Implications for early geologic evolution

Consideration is given to the geological history of Mars as inferred from cratering statistics. The geomorphology of the cratered terrain in Terra Tyrrhena is described in detail, and crater counts made from Viking images of cratered terrain as well as pure cratered areas from the Southern Hemisphere, craters superposing both the intercrater plains and dissected terrain, and plains units in the Northern Hemisphere are presented. Comparison of the Martian crater counts with those obtained for the lunar highlands reveals the distribution functions to be quite similar for crater diameters greater than 8 km, indicating their derivation from the same population of bodies, with an integrated Mars/moon crater flux ratio of at least 0.75. Monte Carlo simulations reveal that if this ratio was due to resurfacing processes, then the Martian population is probably a remnant of obliteration by both inter- and intra-crater plains acting in concert. Results also suggest that most of the endogenetic activity in the cratered terrain occured before the end of heavy bombardment and that two stages of geologic activity were present.

Gurnis, M.↗

NASA NTRS1980

Mars Tharsis region - Volcanotectonic events in the stratigraphic record

It is pointed out that the most recent volcanism and much of the oldest tectonic activity on Mars have apparently occurred within the Tharsis region. Detailed geologic mapping from Viking images has provided new information on the evolutionary history of the region. The eruptive sequence and areal extent of lava flows in the Tharsis region have been defined by stratigraphic studies and crater counts made on individual flow units. Faults and fractures transecting these units provide a record of changing tectonic intensity during the period of high volcanic activity. Volcanism began with the resurfacing of basement rocks early in the history of the region and continued without large interruptions through nine major eruptive episodes. Volcanic centers shifted from place to place but resurgent activity occurred at several volcanoes. Volcanism culminated during the foration of large shield volcanoes along Tharsis Montes and thereafter appears to have gradually declined.

Scott, D. H.↗

NASA NTRS1982

Late-stage summit activity of Martian shield volcanoes

The preservation of morphologically fresh lava flows which pre-date the most recent episodes of caldera collapse at the summits of Ascraeus, Arsia and Olympus Montes indicates that explosive eruptions were not associated with this stage of Tharsis shield volcanism. The existence of resurfaced floor segments, complex wrinkle ridges, and lava terraces within the summit craters suggests that lava lakes comprised the dominant form of the intra-caldera activity. Multiple collapse episodes on Ascraeus and Olympus Montes are indicated by the nested summit craters. The most plausible cause of caldera collapse appears to be large-scale sub-terminal effusive activity, which is corroborated by the previously recognized existence of large lava flows on the flanks of these volcanoes. Due to the implied sequence of large-scale explosive (silicic) volcanism followed by effusive (basaltic) activity, it appears highly unlikely that ignimbrites or other forms of pyroclastic flows (previously proposed as possible deposits within the Olympus Mons aureole material) were ever erupted from the Tharsis Montes.

Mouginis-Mark, P. J.↗

NASA NTRS1982

The structure and evolution of ancient impact basins on Mars

It is pointed out that characteristic styles of degradation and modification of obvious Martian basins make it possible to recognize more subtle expressions. This approach is seen as providing not only additional basins to the existing inventory but also fundamental clues for initial impact basin structure and stratigraphy. It also reveals the long-lasting influence of basin formation on the crust of Mars in spite of extensive erosion and resurfacing. Consideration is given to five clear examples of modified impact basins, and regions around each that have undergone similar processes (fracturing, collapse, channeling) are delineated. These processes among the different basins are then compared, and similar zones of modification are correlated with concentric basin rings. Consideration is then given to the implications of these observations for current models of basin formation and to the role of impact basins in controlling regional tectonics. The results indicate that large multiring impact scars leave a major but sometimes subtle imprint on the geologic structure of stable crustal regions on Mars.

Schultz, P. H.↗

NASA NTRS1982

Formation of the Galilean satellites in a gaseous nebula

A model for Galilean satellite formation is developed in which the satellites accrete in the presence of a dense, gaseous disk-shaped nebula and rapidly form optically thick, gravitationally bound primordial atmospheres. Partially differentiated structures are obtained for both Ganymede and Callisto, although the amount of partial differentiation of Callisto is small, possibly approaching zero for a narrow size distribution of infalling planetesimals. A nominal nebula of approximately 0.1 Jupiter masses is constructed by employing the likely surface density profiles and existing Jupiter collapse calculations. It is shown that satellites accrete very rapidly (dynamical time scales of 100-10,000 years) and their optically thick gaseous envelopes are unable to eliminate the heat of accretion by radiation. Water-saturated, convective, adiabatic envelopes form, through which planetesimals fall, break up, and partially disseminate their mass. The resulting satellite surface temperatures during accretion are calculated. It is concluded that the extensive differentiation undergone by Ganymede may provide the right environment for subsequent resurfacing, whereas the relative lack of differentiation for Callisto may explain the inferred absence of endogenic tectonism.

Lunine, J. I.↗

NASA NTRS1983

Lunar and Planetary Science Conference, 13th, Houston, TX, March 15-19, 1982, Proceedings. Part 2

The second part of the proceedings of the Thirteenth Lunar and Planetary Science Conference considers sedimentary processes and crustal cycling on Venus, a model for the formation of the earth's core, evidence of resurfacing in the lunar nearside highlands, the geology of Tethys, thermal stresses in planetary elastic lithospheres, the petrology and comparative thermal and mechanical histories of clasts in breccia 62236, lunar paleointensity data and its implications for the origin of lunar magnetism, and a model for the accumulation of solar wind radiation damage effects in lunar dust grains. Also discussed are fluid inclusions in stony meteorites, nuclear track and compositional studies of olivines in CI and CM chondrites, the impact of an asteroid or comet in the ocean and the extinction of terrestrial life, cooling rates for glass-containing lunar compositions, and the homogeneity of lava flows.

Boynton, W. V.↗