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The Stratospheric Aerosol and Gas Experiment II (SAGE II) design and in-orbit performance

The design and in-orbit performance data are presented for the Stratospheric Aerosol and Gas Experiment II (SAGE II) instrument which was launched by Shuttle on the Earth Radiation Budget Satellite. SAGE II is a sun photometer that measures the extinction of solar radiation caused by the earth's atmosphere in seven spectral channels ranging in center wavelength from 0.385 to 1.02 micrometers. These measurements, which occur twice each orbit during satellite sunrise and sunset, are inverted to yield vertical distributions of stratospheric aerosols, ozone, water vapor, and nitrogen dioxide. The SAGE II instrument consists of a Cassegrain telescope with a two axis gimbal mounting, a grating spectrometer, and a 12 bit data system. The instrument tracks the solar centroid in the azimuth plane and vertically scans the instrument's instantaneous field of view across the sun for tangent altitudes ranging from the earth's horizon to 150 km. SAGE II is a third generation instrument following the highly successful Stratospheric Aerosol Measurement II (SAM II) and SAGE I programs.

Mauldin, L. E., III↗

Latitudinal variation of spectral optical thickness and columnar size distribution of the El Chichon stratospheric aerosol layer

Measurements are presented for the spectral optical thickness of El Chichon's stratospheric aerosol layer, obtained during an airborne latitudinal survey in April and May of 1983. Columnar aerosol size distributions of the stratosphere are derived by inverting the aerosol optical thickness measurements as a function of wavelength and from spectral aerosol depth measurements obtained during an airborne survey in October and November 1982. Spectral optical thickness data and the derived size distributions from both airborne missions show latitidunal regions with similar characteristics. Airborne solar radiometer measurements are shown to be useful in studies of the latitudinal variations of optical and related particle size characteristics of the stratospheric aerosol layer.

Spinhirne, J. D.↗

Effects of El Chichon volcanic effluents on stratospheric aerosol dynamics

The effects of El Chichon's April 1982 eruption on stratospheric aerosol dynamics are presently discussed in terms of log-normal size distributions over 15-20 km sample altitudes between 30 and 45 deg N over the contiguous U.S. After collection, samples were studied by SEM, and log-normal size distributions were fitted to the data-points obtained. It is found that stratospheric aerosol behavior is explainable by the laws of aerosol mechanics more easily than has been the case for tropospheric aerosol, for which the source-sink relationship is much more complex.

Pueschel, R. F.↗

The Stratospheric Aerosol and Gas Experiment (SAGE III) on the International Space Station (ISS) Mission

The Stratospheric Aerosol and Gas Experiment III on the International Space Station (SAGE III/ISS) mission will provide the science community with high-vertical resolution and nearly global observations of ozone, aerosols, water vapor, nitrogen dioxide, and other trace gas species in the stratosphere and upper-troposphere. SAGE III/ISS measurements will extend the long-term Stratospheric Aerosol Measurement (SAM) and SAGE data record begun in the 1970s. The multi-decadal SAGE ozone and aerosol data sets have undergone intense scrutiny and are considered the international standard for accuracy and stability. SAGE data have been used to monitor the effectiveness of the Montreal Protocol. Key objectives of the mission are to assess the state of the recovery in the distribution of ozone, to re-establish the aerosol measurements needed by both climate and ozone models, and to gain further insight into key processes contributing to ozone and aerosol variability. The space station mid-inclination orbit allows for a large range in latitude sampling and nearly continuous communications with payloads. The SAGE III instrument is the fifth in a series of instruments developed for monitoring atmospheric constituents with high vertical resolution. The SAGE III instrument is a moderate resolution spectrometer covering wavelengths from 290 nm to 1550 nm. Science data is collected in solar occultation mode, lunar occultation mode, and limb scatter measurement mode. A SpaceX Falcon 9 launch vehicle will provide access to space. Mounted in the unpressurized section of the Dragon trunk, SAGE III will be robotically removed from the Dragon and installed on the space station. SAGE III/ISS will be mounted to the ExPRESS Logistics Carrier-4 (ELC-4) location on the starboard side of the station. To facilitate a nadir view from this location, a Nadir Viewing Platform (NVP) payload was developed which mounts between the carrier and the SAGE III Instrument Payload (IP).

Cisewski, Michael↗

Measurements of stratospheric aerosols over Mauna Loa, Hawaii and Boulder, Colorado

The direct solar radiation transmission record at Mauna Loa, dating from 1958 to the present, revealed with remarkable precision the presence of stratospheric aerosol from volcanic activity. This record can be used to quantify the intensity of the stratospheric volcanic aerosol perturbation following a significant eruption in reference to the Agung event in 1963. The Mount St. Helens' stratospheric cloud was first detected by lidar at 18 km over Mauna Loa on 17 July. The atmospheric transmission was seen to decrease slightly after that time, but only a few tenths of 1 percent. Although it is still fairly early to draw a definite conclusion on the ultimate magnitude of the Mount St. Helens stratospheric aerosol from the Mauna Loa results, it can be stated that the stratospheric aerosol optical depth presently observed is comparable with that observed from Fuego which erupted in 1974. At Boulder, Colorado, the atmospheric debris from Mount St. Helens was observed by lidar on a number of occasions. Also, observations of the diffuse, total and direct transmission of solar radiation were made on June 3 and 4. The latter set of observations is useful for deriving information on the scattering properties of the volcanic cloud. The lidar and solar radiation data are presented and some of their special features are discussed.

Deluisi, J. J.↗

Lidar Observations of Stratospheric Aerosol Layer After the Mt. Pinatubo Volcanic Eruption

The volcano Mt. Pinatubo located on the Luzon Island, Philippines, had explosively erupted on June 15, 1991. The volcanic eruptions such as volcanic ash, SO2 and H2O reached into the stratosphere over 30 km altitude by the NOAA-11 satellite observation and this is considered one of the biggest volcanic eruptions in this century. A grandiose volcanic eruption influences the atmosphere seriously and causes many climatic effects globally. There had been many impacts on radiation, atmospheric temperature and stratospheric ozone after some past volcanic eruptions. The main cause of volcanic influence depends on stratospheric aerosol, that stay long enough to change climate and other meteorological conditions. Therefore it is very important to watch stratospheric aerosol layers carefully and continuously. Standing on this respect, we do not only continue stratospheric aerosol observation at Tsukuba but also have urgently developed another lidar observational point at Naha in Okinawa Island. This observational station could be thought valuable since there is no lidar observational station in this latitudinal zone and it is much nearer to Mt. Pinatubo. Especially, there is advantage to link up these two stations on studying the transportation mechanism in the stratosphere. In this paper, we present the results of lidar observations at Tsukuba and Naha by lidar systems with Nd:YAG laser.

Nagai, Tomohiro↗

Intercomparison of stratospheric water vapor observed by satellite experiments - Stratospheric Aerosol and Gas Experiment II versus Limb Infrared Monitor of the Stratosphere and Atmospheric Trace Molecule Spectroscopy

A comparison is made of the stratospheric water vapor measurements made by the satellite sensors of the Stratospheric Aerosol and Gas Experiment II (SAGE II), the Nimbus-7 LIMS, and the Spacelab 3 Atmospheric Trace Molecule Spectroscopy (ATMOS) experiment. It was found that, despite differences in the measurement techniques, sampling bias, and observational periods, the three experiments have disclosed a generally consistent pattern of stratospheric water vapor distribution. The only significant difference occurs at high southern altitudes in May below 18 km, where LIMS measurements were 2-3 ppmv greater than those of SAGE II and ATMOS.

Chiou, E. W.↗

Global distribution of stratospheric aerosols by satellite measurements

A description is given of the first-ever global stratospheric aerosol climatology which is being developed by the earth-orbiting SAM II and SAGE satellite-based sensors. These sensors use the technique of solar occulation; that is, for every spacecraft sunrise and sunset, the modulation of solar intensity caused by the intervening earth-limb is measured. These data are mathematically inverted to yield vertical profiles of aerosol extinction coefficients with 1 km resolution. The data show seasonal variations which are similar in each hemisphere, with strong correlation between aerosol extinction and the corresponding temperature field. Typical values of extinction in the stratosphere are found to be about 0.0001 to 0.0002 per km at 1 micrometer; stratospheric optical depths at this wavelength are about 0.002. The peak extinction in the stratospheric aerosol layer follows the tropopause with altitude, with peak extinction ratios about 10 km above the local tropopause.

Mccormick, M. P.↗

Lower stratospheric aerosols at a tropical latitude station

A pulsed ruby lidar has been in regular operation at the tropical station Trivandrum (8 deg 33 sec N, 76 deg 57 sec E) since October 1986. The lidar data were analyzed to obtain monthly mean aerosol extinction at lower stratospheric altitudes. The monthly mean variation of aerosol extinction shows a peak in March to April with a trough in the winter months. This behavior is compared with that of temperature at the same altitude, obtained from balloonsonde measurements at the same station. It is found that there is a negative correlation between the two with high extinction values corresponding to low temperature values and vice versa. This is attributed to the stratospheric aerosol microphysical processes. The association of stratospheric aerosol extinction with the tropopause altitude and temperature was studied along with the implications of these results.

Krishnamurthy, B. V.↗

Stratospheric aerosol modification by supersonic transport and space shuttle operations - Climate implications

The potential effects on stratospheric aerosols of supersonic transport emissions of sulfur dioxide gas and submicron soot granules, and space shuttle rocket emissions of aluminum oxide particulates are estimated. An interactive particle-gas model of the stratospheric aerosol layer is used to calculate changes due to exhaust emissions, and an accurate radiation transport model is employed to compute the effect of aerosol changes on the earth's average surface temperature. It is concluded that the release of large numbers of small particles (soot or aluminum oxide) into the stratosphere should not lead to a corresponding significant increase in the concentration of large, optically active aerosols, but that the increase in large particles is severely limited by the total mass of sulfate available to make large particles in situ, and by the rapid loss of small seed particles via coagulation. We find that a fleet of several hundred advanced supersonic aircraft operating daily at 20 km, or the launch of one space shuttle rocket per week, could produce roughly a 20% increase in the large-particle concentration of the stratosphere. We find, in addition, that aerosol increases of this magnitude would reduce the global surface temperature by less than 0.01 K.

Turco, R. P.↗

Latitudinal and altitudinal variation of size distribution of stratospheric aerosols inferred from SAGE aerosol extinction coefficient measurements at two wavelengths

A method of retrieving aerosol size distribution from the measured extinction of solar radiation at wavelengths of 0.45 microns and 1.0 microns has recently been proposed. This method is utilized to obtain latitudinal and altitudinal variations of size distributions of stratospheric aerosols from the Stratospheric Aerosol and Gas Experiment data for March 1979. Small particles are found in the lower stratosphere of the tropical region, and large particles are found at higher altitudes and latitudes in both hemispheres. Results of this study are consistent with the suggestion that the upper troposphere in tropical regions is a source of condensation nuclei in the stratosphere, and they become mature as they move to higher altitudes and latitude.

Yue, G. K.↗

The application of lidar to stratospheric aerosol studies

The global climatology and understanding of stratospheric aerosols evolving primarily from lidar and satellite measurements is presented. The importance of validation of these remotely sensed data with in situ measurements is also discussed. The advantage of lidar for providing high vertical and horizontal resolution and its independence from a remote source for measurement will become evident with examples of long term lidar data sets at fixed sites and the use of lidar on airborne platforms. Volcanic impacts of the last 20 years are described with emphasis on the last 8 years where satellite data are available. With satellite and high resolution lidar measurements, an understanding of the global circulation of volcanic material is attempted along with the temporal change of aerosol physical parameters and the stratospheric cleansing or decay times associated with these eruptions.

Mccormick, M. P.↗

Stratospheric aerosol modification by supersonic transport operations with climate implications

The potential effects on stratospheric aerosois of supersonic transport emissions of sulfur dioxide gas and submicron size soot granules are estimated. An interactive particle-gas model of the stratospheric aerosol is used to compute particle changes due to exhaust emissions, and an accurate radiation transport model is used to compute the attendant surface temperature changes. It is shown that a fleet of several hundred supersonic aircraft, operating daily at 20 km, could produce about a 20% increase in the concentration of large particles in the stratosphere. Aerosol increases of this magnitude would reduce the global surface temperature by less than 0.01 K.

Toon, O. B.↗

Nitrogen-sulfur compounds in stratospheric aerosols

Two forms of nitrosyl sulfuric acid (NOHSO4 and NOHS2O7) have been tentatively identified in stratospheric aerosols. The first of these can be formed either directly from gas reactions of NO2 with SO2 or by gas-particle interactions between NO2 and H2SO4. The second product may form when SO3 is involved. Estimates based on these reactions suggest that the maximum quantity of NO that might be absorbed in stratospheric aerosols could vary from one-third to twice the amount of NO in the surrounding air. If these reactions occur in the stratosphere, then a mechanism exists for removing nitrogen oxides from that region by aerosol particle fallout. This process may typify another natural means that helps cleanse the lower stratosphere of excessive pollutants.

Farlow, N. H.↗

High-latitude stratospheric aerosols measured by the SAM II satellite system in 1978 and 1979

Results of the first year of data collection by the SAM (Stratospheric Aerosol Measurement) II satellite system are presented. Almost 10,000 profiles of stratospheric aerosol extinction in the Arctic and Antarctic regions are used to construct plots of weekly averaged aerosol extinction versus altitude and time and stratospheric optical depth versus time. Corresponding temperature fields are presented. These data show striking similarities in the aerosol behavior for corresponding seasons. Wintertime polar stratospheric clouds that are strongly correlated with temperature are documented. They are much more prevalent in the Antarctic stratosphere during the cold austral winter and increase the stratospheric optical depths by as much as an order of magnitude for a period of about 2 months. These clouds might represent a sink for stratospheric water vapor and must be considered in the radiative budget for this region and time.

Mccormick, M. P.↗

Comparing Simultaneous Stratospheric Aerosol and Ozone Lidar Measurements with SAGE 2 Data after the Mount Pinatubo Eruption

Stratospheric aerosol and ozone profiles obtained simultaneously from the lidar station at the University of L'Aquila (42.35 deg N, 13.33 deg E, 683 m above sea level) during the first 6 months following the eruption of Mount Pinatubo are compared with corresponding nearby Stratospheric Aerosol and Gas Experiment (SAGE) 2 profiles. The agreement between the two data sets is found to be reasonably good. The temporal change of aerosol profiles obtained by both techniques showed the intrusion and growth of Pinatubo aerosols. In addition, ozone concentration profiles derived from an empirical time-series model based on SAGE 2 ozone data obtained before the Pinatubo eruption are compared with measured profiles. Good agreement is shown in the 1991 profiles, but ozone concentrations measured in January 1992 were reduced relative to time-series model estimates. Possible reasons for the differences between measured and model-based ozone profiles are discussed.

Yue, G. K.↗

Balloon-borne observations of stratospheric aerosol in Antarctica from 1972 to 1984

Stratospheric levels of particles with r or = 0.15 microns were monitored with optical particle counters in approximately monthly balloon soundings at Laramie, Wyoming (41 deg N) since 1971. These measurements were used to characterize the background stratospheric aerosol layer and the disturbed layer following major volcanic eruptions. Levels of particles with r or = 0.01 microns have also been measured with balloon-borne counters since 1973. The latter are collectively called condensation nuclei (CN) as they are characteristic of aerosol in the early stages of growth. While they dominate the size distribution in the tropsophere, they are a trace species in the undisturbed stratosphere. From 1972 until 1980, annual balloon soundings from McMurdo Station (78 deg S) and/or Amundsen-Scott Station (90 deg S), in Antarctica, have also been conducted to crudely monitor Southern Hemisphere aerosol levels. These measurements were continued in 1983 and 1984. Profiles of r 0.15 microns aerosol concentrations as measured during January at the south pole from 1972 to 1975 and in 1980 are given. The former are typical of undisturbed conditions and indicate the small degree of variability under these conditions. The latter indicates the effect of minor volcanic activity, visible in the 10 to 15 km region.

Hofmann, D. J.↗

A comparison of dustsonde and LIDAR measurements of stratospheric aerosols

This paper describes the results and analysis of an experiment to compare the stratospheric aerosol profiles as measured by a balloon-borne in situ particle counter and by the backscattered light from a ground-based laser radar (LIDAR) operating at a wavelength of 6943 A. The profile comparison agrees within the experimental errors for particles with radii greater than 0.25 micrometer and for altitudes between 15 and 28 kilometers. Following the calibration tests, the LIDAR was used to monitor the stratospheric aerosols at Hampton, Virginia. Enhanced backscatter appeared sporadically in November and December of 1974 over Hampton; scattering ratios averaged over altitude increments of 450 meters range from 1.10 at 20 kilometers in early November to 3.3 at 17 kilometers on December 18. The source of this enhanced backscattering is attributed to the aerosols associated with the eruption of the Fuego volcano in Guatemala in mid-October.

Remsberg, E. E.↗