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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 109 records · Page 6
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Evaluation of Niowave's Proposed Solvent Washing Approach

Niowave, Inc., is a domestic supplier of medical and industrial isotopes from uranium (U) and radium (Ra). The company has recently entered into a cooperative agreement with the U.S. Department of Energy’s National Nuclear Security Administration (NNSA) and plans to deploy a superconducting electron accelerator (LINAC) to fission U for molybdenum-99 ( 99 Mo) production without the need for a nuclear reactor or highly enriched uranium (HEU). NNSA provided funding to the Savannah River National Laboratory (SRNL) to support Niowave in this effort. SRNL evaluated the application of the solvent washing process for Niowave.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2023

Mo-99 Concentration and processing by Solvent Extraction and Ion Exchange

Normally derived from its transient-equilibrium parent molybdenum-99 ( 99 Mo) (t½ = 66 h), the short-lived isotope technetium-99m ( 99m Tc) (t ½ = 6.0 h) is the most widely used medical isotope in diagnostic imaging today. The National Nuclear Security Administration’s (NNSA’s) Material Management and Minimization (M3) program—established under the auspices of the American Medical Isotope Production Act—has been tasked with facilitating the work of domestic 99 Mo suppliers that do not use highly enriched uranium (HEU). Superconducting electron linear accelerators that employ high-Z converter targets can generate bremsstrahlung photons and neutron fluxes that can induce photonuclear reactions and uranium (U) fission. Argonne, in collaboration with industrial partners, has been developing the process chemistry for superconducting linear accelerator (LINAC)-irradiated triuranium octoxide (U 3 O 8 ) targets to produce 99 Mo. In short, the process involves dissolving the irradiated targets in nitric acid, which simultaneously releases valuable fission products (xenon and iodine). After adjusting the acid concentration, producers process the feed using tri-n-butyl phosphate (TBP), then mix the raffinate derived from this extraction cycle with a phosphinic acid such as Cyanex 272 or di(2-ethylhexyl) phosphoric acid (HDEHP), which is selective for Mo (molybdenum liquid liquid extraction [MoLLE]). In the next step, a concentration column comprising an anion exchange platform is used to decontaminate the remaining fission products, generating a pure 99 Mo stream in sodium hydroxide (NaOH)/sodium chloride (NaCl).

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2023

Progress on an Electron Beam Profile Monitor at the Fermilab Main Injector

The current program at Fermilab involves the construction of a new superconducting linear accelerator (LINAC) to replace the existing warm version. The new LINAC, together with other planned improvements, is in support of proton beam intensities in the Main Injector (MI) that will exceed 2 MW. Measuring the transverse profiles of these high intensity beams in a ring requires non-invasive techniques. The MI uses ionization profile monitors as its only profile system. An alternative technique involves measuring the deflection of a probe beam of electrons with a trajectory perpendicular to the proton beam. This type of device was installed in MI and initial studies of it have been previously presented. This paper will present the status and recent studies of the device utilizing different techniques.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Real time heat load calculation software based on EPICS for Fermilab PIP-II CM tests

Fermilab has a project to improve the proton beam energy which is called PIP-II (the 2nd Proton Improvement Plan). There is a superconducting linear accelerator, LINAC, to improve the proton beam power and the LINAC consists of 5 types of cryomodules (CM), 1 HWR CM, 2 SSR1 CM, 4 SSR2 CM, LB650 CM, and HB650 CM. The prototypes of these cryomodules are being tested at Fermilab’s CryoModule Test Facility (CMTF). Heat load measurements are an important part of the prototype CM testing. The CMTF cryogenic control system was developed based on the ACNET (Accelerator Control NETwork) for CM testing for other projects, but the PIP-II cryogenic control system will be implemented using the Experimental Physics and Industrial Control System (EPICS). As part of the prototype CM testing campaign an EPICS based control system has been implemented at CMTF. This EPICS cryogenic control system includes real time heat load calculation software utilizing the Fortran implementation of Hepak. This paper details the real time heat load calculation software developed for the prototype CM testing including the first results from the HB 650 CM.

Yoon, S. [Fermilab]↗
DOE OSTI2026

Real time heat load calculation software based on EPICS for Fermilab PIP-II CM tests

Fermilab has a project to improve the proton beam energy which is called PIP-II (the 2nd Proton Improvement Plan). There is a superconducting linear accelerator, LINAC, to improve the proton beam power and the LINAC consists of 5 types of cryomodules (CM), 1 HWR CM, 2 SSR1 CM, 4 SSR2 CM, LB650 CM, and HB650 CM. The prototypes of these cryomodules are being tested at Fermilab’s CryoModule Test Facility (CMTF). Heat load measurements are an important part of the prototype CM testing. The CMTF cryogenic control system was developed based on the ACNET (Accelerator Control NETwork) for CM testing for other projects, but the PIP-II cryogenic control system will be implemented using the Experimental Physics and Industrial Control System (EPICS). As part of the prototype CM testing campaign, an EPICS based control system has been implemented at CMTF. This EPICS cryogenic control system includes real-time heat load calculation software utilizing the Fortran implementation of Hepak. This paper details the real time heat load calculation software developed for the prototype CM testing including the first results from the HB650 CM.

Yoon, S. [Fermilab]↗
DOE OSTI2023

Visual, Optical and Replica Inspections: Surface Preparation of 650 MHz NB Cavity for PIP-II Linac

Surface preparation of niobium superconducting RF cavities is a critical step for achieving good RF performance under the superconducting state. Surface defect, roughness, and contamination affect the accelerating gradient and quality factor of the cavities. We report surface inspection methods used to control the surface processing of 650 MHz cavities designated for the pre-production and prototype cryomodules for PIP-II linac. The cavity surface was routinely inspected visually, with an optical camera, and by microscopic scanning of surface replicas. This article covers details on the surface inspection methods and surface polishing process used to repair the surface.

43 PARTICLE ACCELERATORS↗
DOE OSTI2025

Control of microphonics for a superconducting radio-frequency photo-injector cryomodule

A superconducting radio-frequency photo-injector cryomodule is being developed for the high-energy upgrade of the Linac Coherent Light Source (LCLS-II-HE). This effort is a collaboration between the Facility for Rare Isotope Beams at Michigan State University (MSU), Argonne National Laboratory, Helmholtz-Zentrum Dresden-Rossendorf, and SLAC National Accelerator Laboratory. The cryomodule features a 185.7 MHz superconducting quarter-wave resonator (QWR) designed to operate with an RF electric field of 30 MV/m at the photo-cathode. Mechanical vibrations must be controlled for operation with stable amplitude and phase. The first prototype cryomodule was cold-tested at MSU with a QWR, fundamental power coupler, tuner, and cathode stalk. In the cold test, we observed microphonics that made it difficult to control the RF phase at high gradient. The cryogenic circuit was identified as a likely culprit. This paper presents our studies of microphonics during the cryomodule cold test and follow-up investigations at room temperature. Our findings provided valuable feedback for modifications to the cryogenic circuit and a successful second cold test of the cryomodule.

Accelerator Physics↗
DOE OSTI2023

Design Study of a Superconducting Quadrupole Magnet System Sustainable Under Dark Current Heating in ILC Main Linac

The International Linear Collider (ILC) main linac comprises a series of 12 m-long cryomodules. The cryomodule contains eight 9-cell superconducting (SC) RF (SRF) cavities and an SC quadrupole magnet combined with dipole correctors to focus and steer electron and positron beams. The magnets are installed between the SRF cavity string and at the longitudinal center of a common cryomodule/cryostat. These magnets are conductively cooled by pure aluminum channels thermally connected to a 2 K two-phase helium pipe for cooling the SRF cavities. A recent study shows that field-emitted electrons, so-called “dark current” initiated in the SRF cavities, are transmitted through the SRF cavity string and reach the SC magnet. The energy is inevitably absorbed in the SC coil due to the magnetic field, resulting in risks of a quench caused by the coil heating. We are investigating alternate magnet designs by using Nb $_{3}$ Sn or $\text{MgB}_{2}$ SC and by adding the dark current absorber surrounding the beam-pipe to realize sustainable magnet operation under the dark current heating. We report the design study of the magnet system and interfaces to the cryomodule accommodating it with the SRF cavities.

43 PARTICLE ACCELERATORS↗
DOE OSTI2024

Flattening the field during injection in the Fermilab booster using dipole corrector magnets

The FNAL Booster is a fast cycling 15 Hz resonant circuit synchrotron accelerating proton beam from 400 MeV to 8 GeV. The linac pulse injected into the Booster is ~32 μsec long and fills the ring by multi-turn charge-exchange injection. As part of the PIP-II project, the Booster injection energy and repetition rate will be increased to 800 MeV and 20 Hz respectively. Due to much reduced average current in the new superconducting PIP-II linac, the injection time will increase to 550 μs. A shorter machine cycle coupled to a longer injection time make flattening the injection porch B-field during injection important requirement for successful PIP-II operation. We aim to achieve: (1) flattening of the net bending during injection using dipole correctors, and (2) using a new system based on an Altera FPGA board, reduction of the cycle-to-cycle bending field variation caused by current jitter in the Gradient Magnet Power Supply (GMPS). While the flat injection scheme is essential to future PIP-II operations, it should also noticeably improve efficiency for present HEP operations.

43 PARTICLE ACCELERATORS↗
DOE OSTI2024

Flattening the Field during Injection in the Fermilab Booster using Dipole Corrector Magnets

The FNAL Booster is a fast cycling 15 Hz resonant circuit synchrotron accelerating proton beam from 400 MeV to 8 GeV. The linac pulse injected into the Booster is ˜32 usec long and fills the ring by multi-turn charge-exchange injection. As part of the PIP-II project, the Booster injection energy and repetition rate will be increased to 800 MeV and 20 Hz respectively. Due to much reduced average current in the new superconducting PIP-II linac, the injection time will increase to 550us. A shorter machine cycle coupled to a longer injection time make flattening the injection porch B-field during injection important requirement for successful PIP-II operation. We aim to achieve: (1) flattening of the net bending during injection using dipole correctors, and (2) using a new system based on an Altera FPGA board, reduction of the cycle-to-cycle bending field variation caused by current jitter in the Gradient Magnet Power Supply (GMPS). While the flat injection scheme is essential to future PIP-II operations, it should also noticeably improve efficiency for present HEP operations.

43 PARTICLE ACCELERATORS↗
DOE OSTI2022

Facility upgrade for superheavy-element research at RIKEN

The RIKEN Nishina Center (RNC) executed an accelerator upgrade project for the heavy-ion linac (called RILAC). A superconducting RIKEN linear accelerator (SRILAC) and a new superconducting electron-cyclotron-resonance ion source (SC-ECRIS) to boost the final energy and intensity were constructed, aimed at synthesizing a new superheavy element, 119, through a hot fusion reaction. The project included the construction of a gas-filled recoil ion separator (GARIS-III) suitable for detecting the residues of the hot-fusion reaction. To avoid research interruption during the SRILAC construction period (2017–2019) and gain experience in hot-fusion reaction processes, GARIS-II located in the GARIS experimental hall in LINAC building was moved to the E6 experimental hall in Nishina building. Certain exploratory measurements were performed employing the beams accelerated by RILAC2 and the RIKEN ring cyclotron (RRC), which is a part of the existing accelerator complex of the radioactive isotope beam factory (RIBF). Further, commissioning experiments with the upgraded facility (SRILAC and GARIS-III) were performed. The upgrade project and its commissioning results are chronologically described in this article.

43 PARTICLE ACCELERATORS↗
DOE OSTI2020

Heavy ion beam physics at Facility for Rare Isotope Beams

The Facility for Rare Isotope Beams (FRIB) will be the world's premier rare-isotope beam facility. Experiments with the majority (~80%) of the isotope predicted to exist will become available. The FRIB facility is based on a superconducting (SC) heavy ion linac with output energy above 200 MeV/u for any ions at beam power of 400 kW. FRIB includes a target facility for in-flight production of rare isotopes. A three-stage fragment separator will be used to prepare fast rare isotope beams with high-purity for nuclear physics experiments. The installation work of the accelerator and experimental systems is approaching completion and multi-stage beam commissioning activities started in summer 2017 with expected project completion in early 2022. In conclusion, the commencement of operation for users' experiments is planned immediately following the project completion.

43 PARTICLE ACCELERATORS↗
DOE OSTI2025

Compact cryomodule for mobile stand-alone superconducting industrial accelerators

Superconducting RF (SRF) accelerators have the potential to be more profitable in comparison with normally conducting accelerators, as long they can be made compact, achieve operational simplicity, autonomy, trans- portability, satisfactory energy efficiency, as well as have reasonable costs. The development of SRF technologies such as Nb 3 Sn coating, conductively-cooled resonators, and high-capacity liquid-helium-free cryocoolers made SRF accelerators mobile and energetically and economically efficient at a beam power of tens of kW. One of the key elements of such an accelerator is the cryomodule, which must have minimal thermal losses to enable operation from low power cryoheads and enable conductive cooling of SRF resonator. In this research we present the design and test results of a compact cryomodule for an industrial stand-alone SRF linear accelerator proto- type, based on 650 MHz elliptical resonators, being developed at Fermi National Accelerator Laboratory.

43 PARTICLE ACCELERATORS↗
DOE OSTI2023

PIP-II Project Overview and Status

The Proton Improvement Plan II (PIP-II) project is an essential upgrade to Fermilab’s particle accelerator complex to enable the world’s most intense neutrino beam for LBNF/DUNE and a broad particle physics program for many decades to come. PIP-II will deliver 1.2 MW of proton beam power from the Main Injector, upgradeable to multi-MW capability. The central element of PIP-II is an 800 MeV superconducting radio frequency (SRF) linac, which comprises a room temperature front end followed by an SRF section. The SRF section consists of five different flavors of cavities/cryomodules, including Half Wave Resonators (HWR), Single Spoke and elliptical resonators operating at, or above, state-of-the-art parameters. The first two PIP-II cryomodules, Half Wave Resonator (HWR) and Single Spoke Resonator 1 (SSR1) were installed in the PIP-II Injector Test facility (PIP2IT) and have accelerated beam to above 17 MeV. PIP-II is the first U.S. accelerator project that will be constructed with significant contributions from international partners, including India, Italy, France, United Kingdom and Poland. The project was baselined in April 2022, and the construction phase is underway.

43 PARTICLE ACCELERATORS↗
DOE OSTI2020

Development and Optimization of a Purification Process to Recover 99 Mo from Low-enriched Uranium

Supported by the DOE-NNSA Office of Material Management & Minimization (M3), a number of domestic entities are pursuing non-highly enriched uranium (non-HEU) production of 99 Mo. As the production technologies of 99Mo pivot toward low-enriched uranium (LEU) or molybdenum targets, new reaction channels and accelerators are being evaluated. Superconducting electron linear accelerators (LINACs) with high-Z converter targets can generate bremsstrahlung photons and neutron fluxes that are capable of inducing photonuclear reactions and LEU fission. A particular advantage of a LINAC is that it does not rely on HEU-fueled reactor cores (which are currently slated for LEU conversion) and can operate on an almost continuous basis. Regarding the chemical purification of 99 Mo from irradiated uranium targets under acidic digestion, there exists a procedure known as Cintichem or modifications thereof with respect to LEU (LEU Modified Cintichem process, LMC). The process relies on a number of selective precipitation steps and column chromatography to purify Mo. It is important to note that LMC prescribes the addition of stable Mo to carry 99 Mo on alpha benzoin oxime, which reduces the specific activity of 99 Mo. This is especially important for processing 99 Mo batches with lower activities (~33 Ci of 99 Mo per batch).

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2022

Solvent Recovery and Management at the Savannah River Site H-Canyon Facility

NIOWAVE, Inc. is a domestic supplier of medical and industrial isotopes from uranium and radium. The Savannah River National laboratory (SRNL) is currently providing support to NIOWAVE, which plans to deploy a superconducting electron linear accelerator (LINAC) to fission uranium for Mo-99 production without the need for a nuclear reactor or HEU. The uranium from the Mo-99 production targets will be purified using a modified PUREX (Plutonium Uranium Reduction Extraction) solvent extraction process to recover the uranium in the product stream. The uranium will then be precipitated as an oxalate which is calcined to U 3 O 8 to fabricate pellets for new Mo-99 targets. In previous support provided to NIOWAVE, the SRNL demonstrated a solvent washing process to remove degradation products from the tributyl phosphate (TBP) solvent used in the modified PUREX process under development for uranium recovery. To supplement this technology demonstration, NIOWAVE requested the SRNL to provide summary information on the solvent recovery and management activities which are used at the Savannah River Site (SRS) H-Canyon facility. An existing reference document for the reprocessing of irradiated HEU fuels at the SRS was used as the primary reference for the solvent management activities; although, other reference documents were used to provide supplementary information. The information provided includes a brief summary of the solvent degradation issues which have been observed in the H-Canyon solvent extraction cycles and resulting process safety concerns. The solvent recovery processes for the three cycles of solvent extraction used in the H-Canyon were subsequently described including the process equipment which consists of the continuous and batch solvent washers, pumps, and tanks. A final section is provided on the monitoring and analysis of solvent quality based on the previous work performed at the SRNL for NIOWAVE and past research and development activities performed to support the solvent extraction processes in both the SRS F-Canyon and H-Canyon facilities.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2023

Final Technical Report: Innovative Magnetron Power Sources for Superconducting RF (SRF) Accelerators

In this project, MUONS is designing and building custom magnetrons at Richardson Electronics (RELL) to test the predictions of the models and make improvements to the designs to match the needs of NP SRF accelerators and their life-cycle costs. To increase lifetime, the filament temperature is controlled by a feedback circuit that includes a model of back streaming of electrons. The gain of the magnetron is optimized by the design of an input port. A permanent magnet design with trim coil for amplitude adjustment reduces energy consumption. Moving the construction of the magnetron from prototype to manufacturing includes the utilization of RELL processes and designs. To the extent that outgassing of materials influences the lifetime of the magnetron, methods for minimizing outgassing was explored. Further experimentation of the potential of sub-critical voltage operation continues to be explored. The commercialization goal of the project will be naturally achieved as RELL already has world-wide marketing, sales, and support to exploit the assembly-line capabilities generated by this project to enable magnetron technologies for NP accelerators.

43 PARTICLE ACCELERATORS↗
DOE OSTI2025

PID-Regulated Heating System for PIP-II Reference Line

The Proton Improvement Plan 2 (PIP-II) centers on building a new superconducting linear particle accelerator (Linac) at Fermilab. At the heart of the accelerator is the reference line. It is a critical system that defines the ideal path for the beam as it passes through magnets, RF cavities, and other beamline elements. Temperature stability is crucial for the reliable operation of RF components, such as mixers and filters. Fluctuations affect key performance parameters like conversion loss, isolation, and linearity. To mitigate any drift caused by ambient temperature changes, a heating plate assembly is utilized to maintain key components at a controlled temperature of 40 C. Utilizing an actively regulated heating system, a metal-oxide-semiconductor field-effect transistor (MOSFET) based power control circuit which provides input to a controller; forming a closed-loop system that maintains the desired setpoints with high precision.

Mosher, Alexander [U. Illinois, Chicago]↗