Towards a new era for warm dense matter diagnostics
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Physics - Plasma physics↗
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Experimental Study of the Fundamental Properties of Warm Dense Mixtures
The aim of the proposed research was to provide a multi-scale study of the properties of warm dense hydrocarbons, by studying the thermodynamic properties through the equation of state and the microscopic properties by x-ray scattering. Understanding the fundamental properties of warm dense mixtures is an intellectual challenge due to the complexity of the system. Unlike liquids or gases, where constituent particle interactions occur through collisions or bonding between valence electrons, in these strongly coupled systems the atoms will be partially ionized and compressed so tightly together that interactions between the inner core electrons can play a role in the systems chemistry. Advances in computational capabilities and development of new theoretical models have been used to predict the properties of mixtures but there is currently no experimental data of the fundamental interaction between the particles in mixtures to test these predictions against. The proposed research was to experimentally investigate the interaction of the different species in hydrocarbons by measuring the compressibility of substances with different carbon and hydrogen ratios and the complexity of the microscopic interactions through elastic and inelastic x-ray scattering. To study the bulk properties of warm dense hydrocarbons we established the Warm Dense Matter Research Laboratory (WDMRL) in the Institute for Shock Physics at Washington State University. The goal was for experiments in the WDMRL to determine shock loading conditions of interest in the hydrocarbon mixtures. We planned on using Hugoniot EOS measurements and a range of carbon and hydrogen concentrations to determine conditions when the EOS of the mixture varied significantly from that of the classical mixing model. Even though shock transit measurements through aluminum foils suggested pressures upto 400GPa, the experiments in the WDMRL were unsuccessful in getting usable shockwave compression data above 100GPa in polystyrene which was below the pressure of interest for hydrocarbon mixtures (>200GPa). To complete the project, we tested a technique using x-ray phase contrast imaging to map the location of tracer layers in a test sample of polycarbonate to record the material motion in dynamically compressed samples. A technique that will be useful for future warm dense matter experiments. These experiments used <200nm gold layers in polycarbonate samples to measure the material velocity and shock speed using x-ray phase contrast imaging. These results were compared to continuum surface measurements performed at ISP and show that the tracer layer technique can measure hydrodynamic properties accurately in dynamically compressed materials.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Ionization by XFEL radiation produces distinct structure in liquid water
In the warm dense matter (WDM) regime, where condensed, gas, and plasma phases coexist, matter frequently exhibits unusual properties that cannot be described by contemporary theory. Experiments reporting phenomena in WDM are therefore of interest to advance our physical understanding of this regime, which is found in dwarf stars, giant planets, and fusion ignition experiments. Using 7.1 keV X-ray free electron laser radiation (nominally 5×10 5 J/cm 2 ), we produced and probed transient WDM in liquid water. Wide-angle X-ray scattering (WAXS) from the probe reveals a new ~9 Å structure that forms within 75 fs. By 100 fs, the WAXS peak corresponding to this new structure is of comparable magnitude to the ambient water peak, which is attenuated. Simulations suggest that the experiment probes a superposition of two regimes. In the first, fluences expected at the focus severely ionize the water, which becomes effectively transparent to the probe. In the second, out-of-focus pump radiation produces O 1+ and O 2+ ions, which rearrange due to Coulombic repulsion over 10 s of fs. Our simulations account for a decrease in ambient water signal and an increase in low-angle X-ray scattering but not the experimentally observed 9 Å feature, presenting a new challenge for theory.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Solar-metallicity gas in the extended halo of a galaxy at z ∼ 0.12
ABSTRACT We present the detection and analysis of a weak low-ionization absorber at z = 0.121 22 along the sightline of the blazar PG 1424+240, using spectroscopic data from both HST/COS and STIS. The absorber is a weak Mg ii analogue, with an incidence of weak C ii and Si ii, along with multicomponent C iv and O vi. The low ions are tracing a dense (nH ∼ 10−3 cm−3) parsec-scale cloud of solar or higher metallicity. The kinematically coincident higher ions are either from a more diffuse (nH ∼ 10−5–10−4 cm−3) photoionized phase of kiloparsec-scale dimensions or are tracing a warm (T ∼ 2 × 105 K) collisionally ionized transition temperature plasma layer. The absorber resides in a galaxy overdense region, with 18 luminous (>L*) galaxies within a projected radius of 5 Mpc and velocity of 750 km s−1. The multiphase properties, high metallicity, and proximity to a 1.4L* galaxy, at ρ ∼ 200 kpc and separation |Δv| = 11 km s−1, favour the possibility of the absorption tracing circumgalactic gas. The absorber serves as an example of weak Mg ii–O vi systems as a means to study multiphase high-velocity clouds in external galaxies.
Pradeep, Jayadev↗
Soft X-ray measurements of transport and MHD activity in the core and edge NSTX plasma (Final Technical Report)
A comprehensive suite of innovative diagnostic instrumentation and techniques has been developed by the Johns Hopkins collaboration for measurements of transport and MHD activity in the core and edge of the National Spherical Torus Experiment (NSTX) at the Princeton Plasma Physics Laboratory (PPPL). These include ultrafast multi-energy poloidal soft X-ray arrays, high spatial resolution multi-energy tangential soft X-ray arrays, high spectral resolution transmission grating imaging VUV spectrometers and ultrafast bolometric arrays, which measure over a broad range of spatial, spectral, and temporal scales the emission from ohmic, RF, and beam driven NSTX plasmas. The instrumentation was designed to fulfill the specific measurement needs of the Spherical Torus (ST) magnetic fusion concept and is accompanied by a comprehensive set of numerical tools for data analysis and modeling, aimed at determining as many as possible plasma parameters and at extracting as much as possible physics information from NSTX experiments. The Johns Hopkins diagnostics have been and continue to be instrumental for essentially all the NSTX experiments. In addition, our own research and experiments using these diagnostics has led over the years to fundamental conclusions for the ST fusion physics, such as the establishment of near neoclassical impurity transport in the NSTX core and edge plasma, and the critical role of the Global Alfven Eigenmode (GAE) MHD activity for the ST core electron thermal transport. The Johns Hopkins Diagnostics continue to be operational on the upgraded NSTX-U and will provide key plasma information in its upcoming high field, current and power experimental campaigns. The present report summarizes the main technical characteristics and measurement capabilities of the diagnostic instrumentation and methods developed within our research and describes a key physics result achieved during this research. Success in our research was made possible also by the excellent support and cooperation of the NSTX research team and of PPPL researchers, who are warmly acknowledged here.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Shock physics in warm dense matter: A quantum hydrodynamics perspective
Abstract Warm dense matter (WDM), an exotic, highly compressed state of matter between solid and plasma phases, is of high current interest, in particular for astrophysics and inertial confinement fusion. For the latter, in particular the propagation of compression shocks is crucial. The main unknown in the shock propagation in WDM is the behaviour of the electrons since they are governed by correlations, quantum and spin effects that need to be accounted for simultaneously. Here we describe the shock dynamics of the warm dense electron gas using a quantum hydrodynamic model. From the numerical hydrodynamic simulations, we observe that the quantum Bohm pressure induces shear force that weakens the formation and strength of the shock. In addition, the Bohm pressure induces an electron density response that takes the form of oscillations. This is confirmed by the theoretical analysis of the early stage of the shock formation. Our theoretical and numerical analyses allow us to identify characteristic dimensionless shock propagation parameters at which the effect of the Bohm force is important.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Characterizing laser-heated polymer foams with simultaneous x-ray fluorescence spectroscopy and Thomson scattering at the Matter in Extreme Conditions Endstation at LCLS
Understanding the behavior of polymer foams at high energy density conditions is crucial to advance inertial fusion energy research. Here, we present a new experimental platform designed to measure the thermodynamic state of these materials at megabar pressures. At the Matter in Extreme Conditions Endstation of the Linac Coherent Light Source, we heat samples using an optical, high-intensity, femtosecond laser and dynamically probe them with ultra-short, coherent x-ray pulses of high peak brightness. We perform x-ray Thomson scattering measurements in forward and backward scattering geometries to capture both collective and non-collective electron behavior in the sample. Simultaneously, x-ray fluorescence spectroscopy is used to measure the emission from a mid-Z dopant, providing complementary information on the plasma conditions. By combining these techniques, we obtain temporally resolved temperature measurements of the transient warm dense matter states. Our initial experiments designed to benchmark the platform with carbon samples yielded data resolving the ultrafast response to laser heating with sub-picosecond resolution, measuring plasma temperatures exceeding 50 eV. These findings lay the foundation for precision studies of the dynamic evolution of laser-heated polymer foams.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Static linear density response from X-ray Thomson scattering measurements: a case study of warm dense beryllium
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Physics - Plasma physics↗
Stochastic and mixed density functional theory within the projector augmented wave formalism for simulation of warm dense matter
Stochastic density functional theory (DFT) and mixed stochastic-deterministic DFT are burgeoning approaches for the calculation of the equation of state and transport properties in materials under extreme conditions. In the intermediate warm dense matter regime, a state between correlated condensed matter and kinetic plasma, electrons can range from being highly localized around nuclei to delocalized over the whole simulation cell. The plane-wave basis pseudopotential approach is thus the typical tool of choice for modeling such systems at the DFT level. Unfortunately, stochastic DFT methods scale as the square of the maximum plane-wave energy in this basis. To reduce the effect of this scaling and improve the overall description of the electrons within the pseudopotential approximation, we present stochastic and mixed DFT approaches developed and implemented within the projector augmented wave formalism. In conclusion, we compare results between the different DFT approaches for both single-point and molecular dynamics trajectories and present calculations of self-diffusion coefficients of solid density carbon from 1 to 50 eV.
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
Investigation of the fermion sign problem in warm dense Beryllium
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Physics - Plasma physics↗
Understanding warm dense matter: from theory to experiment
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Physics - Plasma physics↗
Mixed stochastic-deterministic time-dependent density functional theory: application to stopping power of warm dense carbon
Warm dense matter (WDM) describes an intermediate phase, between condensed matter and classical plasmas, found in natural and man-made systems. In a laboratory setting, WDM is often created dynamically. It is typically laser or pulse-power generated and can be difficult to characterize experimentally. Measuring the energy loss of high energy ions, caused by a WDM target, is both a promising diagnostic and of fundamental importance to inertial confinement fusion research. However, electron coupling, degeneracy, and quantum effects limit the accuracy of easily calculable kinetic models for stopping power, while high temperatures make the traditional tools of condensed matter, e.g. time-dependent density functional theory (TD-DFT), often intractable. In this study, we have developed a mixed stochastic-deterministic approach to TD-DFT which provides more efficient computation while maintaining the required precision for model discrimination. Recently, this approach showed significant improvement compared to models when compared to experimental energy loss measurements in WDM carbon. Here, we describe this approach and demonstrate its application to warm dense carbon stopping across a range of projectile velocities. We compare direct stopping-power calculation to approaches based on combining homogeneous electron gas response with bound electrons, with parameters extracted from our TD-DFT calculations.
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
Superstructure Optimization of Waste Plastic Pyrolysis, Integrating Thermal, Catalytic, and Plasma Technologies with Machine Learning
Global plastic waste generation exceeds 430 million tonnes per year, yet fewer than 9% are recycled in the United States. Pyrolysis offers a chemical recycling route at scale, but existing techno-economic and life cycle assessments fix product yields to single pure polymers, producing economic and environmental outputs that break down when the feed composition changes. Here, we present a superstructure optimization framework that addresses this by embedding a composition-aware random forest yield predictor, trained on 566 pyrolysis experiments, within a full-scale process simulation. Product distributions update automatically as feed allocation shifts across four reactor chemistries: conventional thermal, catalytic (HZSM-5), thermal oxo-degradation, and nonequilibrium CO2 plasma. The optimal superstructure achieves minimum selling prices of −0.56 to −0.76/kg feed and global warming potentials of −0.276 to −0.322 kg CO2-eq/kg feed across four commodity price scenarios, confirming profitable, carbon-negative operation without tipping fees. Carbon abatement costs of $\$$0.46 to $\$$1.25/kg CO2-eq are competitive with direct air capture. Sensitivity analysis shows that the catalytic-plasma split fraction is the single largest driver of both economic and climate performance, while hydrocracking allocation in the wax upgrading stage is emission-neutral across the full variable range. Mixed plastic waste streams, evaluated as composition-variable feedstocks rather than pure resins, are profitable and carbon-negative across realistic market conditions. These results give a quantitative basis for reactor selection, circular economy investment, and policy design targeting chemical recycling on a large scale.
Life cycle assessment↗
Unlocking the Future of Aircraft Manufacturing: The Environmental Benefits of Laser Patterning for Surface Enhancement of Aircraft-Certified Alloys
Surface protection and functional modification of aircraft-certified aluminum alloys are essential for corrosion resistance, durability, and long-term airworthiness. At the same time, increasingly restrictive environmental regulations motivate the development of alternatives to legacy wet-chemical surface treatments. This study presents an integrated assessment of ultrafast femtosecond laser surface texturing as a surface functionalization approach for Aluminum 6061 alloys within an aerospace manufacturing and sustainability context. Ultrashort-pulse laser processing enables controlled micro- and nano-scale surface topographical modification with limited thermal impact, allowing adjustment of wettability and surface functionality while preserving bulk material integrity. As a dry and contactless process, femtosecond laser treatment eliminates the use of hazardous chemicals, reduces consumable inputs, and generates minimal secondary waste. A streamlined cradle-to-gate life cycle assessment conducted in accordance with ISO 14040/14044 indicates a lower global-warming potential per functional unit compared with conventional surface treatments, including anodization, plasma-assisted coatings, and organic coating systems. Complementary qualitative analyses addressing environmental health and safety, supply-chain risk, and ESG alignment indicate potential advantages related to occupational safety, regulatory compliance, waste management, and end-of-life recyclability. The investigation is performed on planar Aluminum 6061 reference surfaces with a treated area of 25 mm 2 , providing a controlled laboratory-scale basis for analyzing process behavior, functional surface modification, and associated environmental metrics. Within this defined scope, the results support further evaluation of femtosecond laser surface texturing as a surface engineering option for future aerospace manufacturing.
corrosion resistance↗
Quantum kinetic modeling of KEEN waves in a warm-dense regime
We report the first fully kinetic, quantum study of kinetic electrostatic electron nonlinear (KEEN) waves, showing that quantum diffraction systematically erodes the classical trapping mechanism, narrows harmonic locking to the fundamental, and hastens post-drive decay. Electrons are evolved with a second-order Strang-split 1D1V Wigner–Poisson solver that couples conservative semi-Lagrangian WENO advection to an analytic Fourier space update for the non-local Wigner term, while ions remain classical. We focus on collisionless dynamics in a weakly coupled regime, providing a controlled baseline before collisional extensions. Short, frequency-tuned ponderomotive pulses drive KEEN formation in a uniform Maxwellian plasma; as the dimensionless quantum parameter H rises from the classical limit to values relevant to warm-dense matter, doped semiconductors, and 2D electron systems, the drive threshold increases, higher harmonics are damped, trapped electron vortices diffuse, and the subplasma electrostatic energy relaxes to a lower stationary level, as confirmed by continuous wavelet analysis. These microscopic changes carry macroscopic weight. Ignition-scale capsules now compress matter to regimes where the electron de Broglie wavelength rivals the Debye length, making classical kinetic descriptions insufficient. By extending KEEN physics into this quantum domain, our results offer a potential diagnostic of non-equilibrium electron dynamics for next-generation inertial-confinement designs and high-energy-density platforms, indicating that predictive fusion modeling may benefit from the integration of kinetic fidelity with quantum effects.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Study of x-ray fluorescence spectroscopy from high-energy-density plasmas (Final Report)
The primary objective of this subcontract was to support the development of x-ray fluorescence spectroscopy (XFS) as a diagnostic tool for high-energy-density (HED) plasmas. Several experimental campaigns were completed to develop and benchmark XFS at various plasmas conditions of interest for inertial confinement fusion and HED science. The experimental measurements at the Omega laser facility used x-ray absorption spectroscopy (XAS) to determine the plasma temperature from the shape of the K-edge to benchmark XFS data. During the course of these experiments, it was found that XAS can also constrain ionization from bound-bound absorption features, and it became a primary diagnostic in this study. Several experimental campaigns were conducted at the Omega laser facility to refine XAS and XFS measurements of warm dense copper.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Investigation into the transport properties of planetary interiors through inelastic X-ray scattering experiments and quantum molecular dynamics (Final Technical Report)
This was a two-year research project for the period 08/15/2018 - 08/14/2020 conducted at the University of Nevada, Reno using Pronghorn, a newly built high-performance cluster located at the University. The short-term project goal was to provide computational support for the experimental campaigns at LCLS through data analysis of previous and upcoming scheduled experiments, along with performing state-of-the-art atomistic simulations of dense plasmas. The longer-term goal was to create a new computational high energy density physics group located at the University of Nevada, Reno. Guided by results from past and future high-resolution scattering experiments, we aimed to research and develop non-equilibrium and non-adiabatic atomistic simulations of dense plasmas that went beyond the Born-Oppenheimer approximation
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Sensitivity of magnetohydrodynamic simulations of Joule-heated conductors to the vaporization curve in equations of state
Magnetohydrodynamic (MHD) simulations of electrically exploded aluminum and copper rods demonstrate a technique to validate equations of state (EOS) for rapidly Joule-heated conductors. The balance of internal and magnetic forces at the conductor-insulator interface drives the metal there along the vaporization phase boundary. Variations between critical points and vaporization curves in existing models predict differing densities and temperatures in MHD simulations for these models. Here, the inclusion of Maxwell constructs in the liquid-vapor biphase region of the EOS caused the rod surface to vaporize earlier in time than unmodified tables with van der Waals loops. Velocimetry of recent experiments is used to validate the location of the vaporization curve in existing EOS models and differentiate between the vapor dome treatments. Dielectric coatings applied to the metal surface restricted the conductor’s expansion and diverted the metal into the warm dense matter regime.
36 MATERIALS SCIENCE↗